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Coherent Control of Thermal Radiation with Nanophotonics 热辐射的纳米光子学相干控制
IF 3.9 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-08-31 DOI: 10.1002/adpr.202500019
Yuanrong Zhang, Qi Tian, Shuang Zheng, Max Yan, Minming Zhang

Incoherence of traditional thermal emission, such as blackbody radiation with broad bandwidth and omnidirectional nature, fundamentally restricts their practical applicability. Nanophotonic structures—particularly those engineered with subwavelength scale features—exhibit thermal radiation properties that markedly diverge from conventional emitters, enabling precise spectral and directional modulation of thermal emission. Herein, recent developments and challenges in the coherence control of thermal radiation with nanophotonics platforms are reviewed. First, the fundamental properties of thermal radiation and approaches for thermal radiation calculation are introduced. Also, recent developments of coherence control are presented, which are divided into three parts, including temporal coherence, spatial coherence, and polarization state of thermal radiation. As coherence control holds great potential for various infrared applications, the representative applications, such as infrared sensing, radiative cooling, thermal camouflage, and imaging, are subsequently introduced. Finally, a conclusion is made and the future developments of coherence control are prospected. By synthesizing current researches, this work highlights the transformative potential of coherent thermal radiation control and its impact on next-generation technologies, offering new perspectives in the areas of infrared thermal emission.

传统的热辐射,如黑体辐射具有宽带宽和全向性,其不相干性从根本上制约了其实际应用。纳米光子结构——特别是那些具有亚波长尺度特征的纳米光子结构——表现出与传统发射器明显不同的热辐射特性,从而实现了热辐射的精确光谱和方向调制。本文综述了纳米光子学平台在热辐射相干控制方面的最新进展和面临的挑战。首先,介绍了热辐射的基本性质和热辐射的计算方法。本文还介绍了相干性控制的最新进展,并将其分为时间相干性、空间相干性和热辐射偏振态三部分。由于相干控制在各种红外应用中具有巨大的潜力,因此介绍了具有代表性的应用,如红外传感、辐射冷却、热伪装和成像。最后,对相干控制的发展进行了展望。通过综合目前的研究,本工作突出了相干热辐射控制的变革潜力及其对下一代技术的影响,为红外热发射领域提供了新的视角。
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引用次数: 0
Comparison of Glass Material and Laser Excitation Regime for Upconversion-Based 3D Volumetric Display 基于上转换的三维体积显示中玻璃材料和激光激发机制的比较
IF 3.9 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-08-28 DOI: 10.1002/adpr.202500158
Yunle Wei, Thomas de Prinse, Xuanzhao Pan, Erik P. Schartner, Nelson Tansu, Ramez Elgammal, Matthew Kappers, Nigel A. Spooner, Heike Ebendorff-Heidepriem

Two-step, two-frequency (TSTF) upconversion in rare-earth-ion (REI) doped solids is a proven strategy for achieving 3D volumetric displays, with potential applications in defence, healthcare, education, manufacturing, and entertainment. Early studies have primarily focused on REI-doped fluoride glasses or single crystals, which efficiently support TSTF upconversion due to their low-phonon energy. However, these materials are challenging to produce at the size and quality required for commercial applications. This study explores tellurite and germanate glasses as scalable, low-phonon-energy alternatives by benchmarking their TSTF upconversion performance against fluoride glass for Er3+ green fluorescence. Tellurite and germanate glasses exhibit dimmer green upconversion under continuous-wave excitation, while tellurite glass unexpectedly outperforms fluoride glass when both lasers are pulsed with properly adjusted modulation parameters. Rate equation-based simulations are used to explain these findings. In particular, tellurite glass exhibits brighter emission than fluoride glass under synchronized dual-pulsed excitation due to its much higher ground- and excited-state absorption cross sections and radiative decay rate, which compensate for its shorter 4S3/2 lifetime. Green voxel generation is demonstrated in a large ≈4 × 4 × 4 cm3 Er3+-doped tellurite glass cube with high optical quality. These results open new directions for REI-doped glass development and laser design for TSTF upconversion-based 3D volumetric displays.

稀土离子(REI)掺杂固体中的两步双频(TSTF)上转换是实现3D体积显示的一种经过验证的策略,在国防,医疗保健,教育,制造和娱乐方面具有潜在的应用前景。早期的研究主要集中在rei掺杂氟化物玻璃或单晶上,由于它们的低声子能量,它们有效地支持TSTF上转换。然而,这些材料在商业应用所需的尺寸和质量上是具有挑战性的。本研究探讨了碲酸盐和锗酸盐玻璃作为可扩展的低声子能量替代品,通过对其TSTF上转换性能与氟化物玻璃的Er3+绿色荧光进行基准测试。碲酸盐和锗酸盐玻璃在连续波激发下表现出较暗的绿色上转换,而碲酸盐玻璃在适当调节调制参数的激光脉冲下的表现出乎意料地优于氟化物玻璃。基于速率方程的模拟被用来解释这些发现。在同步双脉冲激励下,碲酸盐玻璃由于具有更高的基态和激发态吸收截面和辐射衰减率,补偿了其较短的4S3/2寿命,表现出比氟化物玻璃更亮的发射。在高光学质量的≈4 × 4 × 4 cm3掺Er3+的大碲酸盐玻璃立方体中证明了绿色体素的生成。这些结果为rei掺杂玻璃的开发和基于TSTF上转换的三维体积显示器的激光器设计开辟了新的方向。
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引用次数: 0
Multimodal Luminescence from LaAlO3:Eu3+ via Trap Modulation for High-Temperature Applications 高温应用中LaAlO3:Eu3+的多模态发光
IF 3.9 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-08-28 DOI: 10.1002/adpr.202500092
Abdulelah Alolayan, Nimai Pathak, Kawsar Ali, Yuanbing Mao

Persistent phosphors with high charge storage capacity are promising for a wide range of applications, mostly demonstrated at room temperature. Designing such long-persistent phosphor (LPP) applicable at higher temperature is largely unexplored and challenging. To prevent spontaneous charge release and ensure long-term data retention, high-temperature LPPs must feature multilevel traps with sufficient activation energies. In this report, LaAlO3:Eu3+ (LAO:E) phosphor is investigated with multiple traps and four integrated luminescent emissions: down-conversion photoluminescence and radioluminescence, thermally stimulated luminescence, persistent luminescence (PersL), and optically stimulated luminescence (OSL). Unlike earlier optical storage phosphors, our LAO:E phosphor possesses charge carriers that are released from these traps, ranging from shallow trap 1 to deep trap 4, across various temperatures. The potential for the long-term storage of charge carriers at both room and elevated temperatures is also examined. Supported by experimental data and density functional theory calculations, we establish a correlation between the various traps and the desired PersL and OSL properties of the LAO:E phosphor. Additionally, a comprehensive trapping–detrapping mechanism for charge carriers is developed. The studies here are expected to pave the way for designing advanced multimode phosphors for a wide range of applications at high temperatures.

具有高电荷存储能力的持久性荧光粉具有广泛的应用前景,主要是在室温下进行的。设计这种适用于高温的长持久性荧光粉(LPP)在很大程度上是未知的,也是具有挑战性的。为了防止自发电荷释放并确保长期数据保留,高温LPPs必须具有具有足够活化能的多层陷阱。本文研究了LaAlO3:Eu3+ (LAO:E)荧光粉的多陷阱和四种集成发光发射:下转换光致发光和辐射致发光、热激发发光、持续发光(PersL)和光激发发光(OSL)。与早期的光存储荧光粉不同,我们的LAO:E荧光粉具有从这些陷阱中释放的电荷载流子,从浅陷阱1到深陷阱4,在不同的温度下。在室温和高温下长期储存载流子的潜力也进行了研究。在实验数据和密度泛函理论计算的支持下,我们建立了各种陷阱与LAO:E荧光粉所需的PersL和OSL特性之间的相关性。此外,还开发了一种全面的电荷载流子捕获-脱陷机制。这些研究有望为设计先进的多模荧光粉铺平道路,以在高温下广泛应用。
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引用次数: 0
Generalized Heterodyne Interferometry in Kerr Materials Kerr材料中的广义外差干涉测量
IF 3.9 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-08-28 DOI: 10.1002/adpr.202500020
Arnaud Rogemont, Rajath Sawant, Aurélien Coillet, Benoit Cluzel

Interferometry has long been used to measure the phase of light signals. Combined with a heterodyne detection scheme, it allows to simultaneously record amplitude and phase variations. In this work, these well-known techniques are exploited to evaluate the nonlinear phase induced by the optical Kerr effect during the propagation of a laser pulse in a nonlinear medium. It is shown that the nonlinear index can easily be retrieved when the accumulated phase remains small, but counter-intuitive results can be observed at higher powers. In particular, the combination of pulsed excitation and Kerr nonlinearity results in nonlinear variations of the amplitude of the interference pattern, whose shape depends on the pulse profile and the dispersion of the propagation medium.

干涉测量法早就被用来测量光信号的相位。结合外差检测方案,它允许同时记录振幅和相位变化。在这项工作中,利用这些众所周知的技术来评估激光脉冲在非线性介质中传播过程中由光学克尔效应引起的非线性相位。结果表明,当累积相位较小时,非线性指标可以很容易地恢复,但在较高的功率下,可以观察到反直觉的结果。特别是,脉冲激励和克尔非线性的结合导致干涉图样振幅的非线性变化,其形状取决于脉冲轮廓和传播介质的色散。
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引用次数: 0
Nonvolatile and Low-Loss Reconfigurable Optical Switches Using Sb2S3 Phase Change Material 采用Sb2S3相变材料的非易失性和低损耗可重构光开关
IF 3.9 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-08-28 DOI: 10.1002/adpr.202500067
Nisadur Rahman, Hasan Khaled Rouf

For developing effective reconfigurable photonic devices, low-loss phase change materials, such as Sb2S3, can be a good choice. Sb2S3-tunable directional couplers (DCs) have the lowest insertion loss in both amorphous and crystalline states. However, they suffer from a large coupling length issue, which can be overcome by combining with hybrid plasmonic waveguides (HPWGs). Herein, a Sb2S3-assisted HPWG-based reconfigurable, nonvolatile 1 × 2 switch that has been designed using an asymmetric DC is proposed. The proposed switch has dual-polarization functionality (operates in both transverse electric and TM modes) indicating its broader applicability and flexibility in integrated photonic systems where polarization diversity is often required. The optical characteristics and coupling behavior with phase transitions have been numerically examined. With a compact coupling length of 46 μm, the proposed 1 × 2 switch achieves a low insertion loss of ≈0.5 dB and a small crosstalk of <−10 dB over a bandwidth of 70 nm (1510–1580 nm).

为了开发有效的可重构光子器件,低损耗相变材料,如Sb2S3,是一个很好的选择。sb2s3可调谐定向耦合器(DCs)在非晶和晶体状态下都具有最低的插入损耗。然而,它们存在较大的耦合长度问题,这可以通过与混合等离子体波导(HPWGs)相结合来克服。本文提出了一种基于sb2s3辅助的hpwg可重构、非易失性的1 × 2开关,该开关采用非对称直流设计。所提出的开关具有双极化功能(在横向电模式和TM模式下工作),表明其在通常需要极化多样性的集成光子系统中具有更广泛的适用性和灵活性。对其光学特性和相变耦合特性进行了数值研究。该1 × 2开关的耦合长度为46 μm,在70 nm (1510-1580 nm)的带宽范围内,插入损耗低至约0.5 dB,串扰小至<;−10 dB。
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引用次数: 0
Recent Advances in χ(2)-Based Nonlinear Frequency Conversion of Fiber Lasers 基于χ(2)的光纤激光器非线性变频研究进展
IF 3.9 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-08-24 DOI: 10.1002/adpr.202500012
Bing Han, Yiming Tao, Wei Deng, Lu Chen, Bo Hu, Qian Cheng, Yihan Qiu, Mengqiu Fan, Houkun Liang, Ting Feng, Han Wu

Lasers operating in the visible and 3–20 μm mid-infrared (MIR) spectral ranges have become indispensable tools with broad and significant applications in fields such as display technology, biomedicine, laser-guide-star systems, and nonlinear optics. To meet the growing demand for high-performance visible and MIR lasers, nonlinear frequency conversion of fiber lasers has emerged as a promising approach, offering flexible wavelength tunability, high conversion efficiency, and high output power. This review highlights recent advances in the χ(2)-based nonlinear frequency conversion of fiber lasers in both visible and MIR wavelength regions. First, the progress in χ(2)-based frequency conversion of conventional fiber lasers, including frequency doubling, sum-frequency generation, difference frequency generation, and optical parametric oscillation, is reviewed. Additionally, the characteristics and performance of various novel fiber lasers in nonlinear frequency conversion applications, including random fiber lasers, incoherent and spectrum-tailorable superfluorescent fiber sources, and ultrafast fiber lasers, are presented. Finally, the prospects and challenges associated with the frequency conversion of fiber lasers are discussed, providing insights into future directions and potential solutions.

在可见光和3-20 μm中红外(MIR)光谱范围内工作的激光器已成为显示技术、生物医学、激光导星系统和非线性光学等领域中不可缺少的重要工具。为了满足对高性能可见和MIR激光器日益增长的需求,光纤激光器的非线性频率转换已成为一种有前途的方法,具有灵活的波长可调性,高转换效率和高输出功率。本文综述了在可见光和MIR波长区域基于χ(2)的光纤激光器非线性频率转换的最新进展。首先,综述了基于χ(2)的传统光纤激光器变频技术的研究进展,包括倍频、和频产生、差频产生和光参量振荡。此外,还介绍了各种新型光纤激光器在非线性变频应用中的特点和性能,包括随机光纤激光器、非相干和可调谱超荧光光纤光源以及超快光纤激光器。最后,讨论了光纤激光器频率转换的前景和挑战,并对未来的发展方向和潜在的解决方案提供了见解。
{"title":"Recent Advances in χ(2)-Based Nonlinear Frequency Conversion of Fiber Lasers","authors":"Bing Han,&nbsp;Yiming Tao,&nbsp;Wei Deng,&nbsp;Lu Chen,&nbsp;Bo Hu,&nbsp;Qian Cheng,&nbsp;Yihan Qiu,&nbsp;Mengqiu Fan,&nbsp;Houkun Liang,&nbsp;Ting Feng,&nbsp;Han Wu","doi":"10.1002/adpr.202500012","DOIUrl":"https://doi.org/10.1002/adpr.202500012","url":null,"abstract":"<p>Lasers operating in the visible and 3–20 μm mid-infrared (MIR) spectral ranges have become indispensable tools with broad and significant applications in fields such as display technology, biomedicine, laser-guide-star systems, and nonlinear optics. To meet the growing demand for high-performance visible and MIR lasers, nonlinear frequency conversion of fiber lasers has emerged as a promising approach, offering flexible wavelength tunability, high conversion efficiency, and high output power. This review highlights recent advances in the χ<sup>(2)</sup>-based nonlinear frequency conversion of fiber lasers in both visible and MIR wavelength regions. First, the progress in χ<sup>(2)</sup>-based frequency conversion of conventional fiber lasers, including frequency doubling, sum-frequency generation, difference frequency generation, and optical parametric oscillation, is reviewed. Additionally, the characteristics and performance of various novel fiber lasers in nonlinear frequency conversion applications, including random fiber lasers, incoherent and spectrum-tailorable superfluorescent fiber sources, and ultrafast fiber lasers, are presented. Finally, the prospects and challenges associated with the frequency conversion of fiber lasers are discussed, providing insights into future directions and potential solutions.</p>","PeriodicalId":7263,"journal":{"name":"Advanced Photonics Research","volume":"6 12","pages":""},"PeriodicalIF":3.9,"publicationDate":"2025-08-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://advanced.onlinelibrary.wiley.com/doi/epdf/10.1002/adpr.202500012","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145666105","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Transformer Encoder–Decoder Framework for Nonlinear Pulse Evolution and Inverse Modeling 变压器编码器-解码器框架的非线性脉冲演化和逆建模
IF 3.9 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-08-21 DOI: 10.1002/adpr.202500149
Dinesh Kumar Murugan, Rajkumar Joseph, Nithyanandan Kanagaraj

Modeling and understanding the nonlinear pulse evolution in optical systems is crucial for developing modern photonic technologies. The pulse evolution often involves a complex interplay of various effects, and modeling its dynamics heavily relies on numerical simulations. Supercontinuum generation, a highly nonlinear phenomenon involving the propagation of ultrashort pulses through optical fibers, is one example of such a nonlinear dynamical problem. The idea of modeling both forward and inverse processes using a transformer-based encoder–decoder approach is put forth. To the best of the knowledge, this might be the first work to apply this framework to the task, highlighting its effectiveness in capturing complex dynamics. While the primary focus is on the transformer-based encoder–decoder model, a variety of other network architectures is also explored to evaluate model accuracy and to highlight their ability to predict complex nonlinear dynamics at a fraction of the computational cost of traditional numerical methods. This article demonstrates the potential of transformer-based approaches for modeling nonlinear optical systems and their ability to generalize to other physical systems.

对光学系统中非线性脉冲演化的建模和理解对于现代光子技术的发展至关重要。脉冲的演化往往涉及各种效应的复杂相互作用,其动力学建模严重依赖于数值模拟。超连续统的产生是一种涉及超短脉冲在光纤中传播的高度非线性现象,是这种非线性动力学问题的一个例子。提出了利用基于变压器的编码器-解码器方法对正反过程建模的思想。据我所知,这可能是第一个将这个框架应用于任务的工作,突出了它在捕获复杂动态方面的有效性。虽然主要关注的是基于变压器的编码器-解码器模型,但也探索了各种其他网络架构,以评估模型的准确性,并强调它们以传统数值方法的一小部分计算成本预测复杂非线性动力学的能力。本文展示了基于变压器的非线性光学系统建模方法的潜力及其推广到其他物理系统的能力。
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引用次数: 0
Floquet-Engineered Noise-Resilient Terahertz Receiver with Modular Phased Array Architecture for Scalable Chip-Scale Communication 用于可扩展芯片级通信的模块化相控阵结构的杂波工程抗噪太赫兹接收机
IF 3.9 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-08-21 DOI: 10.1002/adpr.202500079
Kosala Herath, Malin Premaratne, Sergi Abadal, Sharadhi Gunathilake, Eduard Alarcón, Ampalavanapillai Nirmalathas

The transition to multichip and accelerator-rich computing architectures has exposed the limitations of conventional wired interconnects, including bandwidth constraints, latency, and power inefficiencies. While wireless interconnects provide a scalable alternative, existing transceiver technologies often lack the interference resilience required for efficient multichip communication. To address these challenges, a terahertz (THz) modular phased array (MPA) transmitter and a 2D semiconductor quantum well (2DSQW)-based nanoreceiver are introduced, enabling noise-resilient signal demodulation without bulky processing hardware. The dual-carrier MPA model enhances beam focusing precision while suppressing grating lobes and mitigating polarization mismatch with the receiver. The receiver response is characterized using Floquet engineering, leveraging the quantum behavior of charge carriers in time-periodic radiation fields to achieve accurate polarization-dependent response tuning. The 2DSQW-based receiver's unique geometric design facilitates spatial modulation, ensuring robust noise suppression and interference detection. This architecture is particularly well-suited for vertical communication in multichip quantum processors, where high wiring density and thermal constraints hinder scalability. By operating the MPA transmitter at elevated temperatures while maintaining the receiver at lower temperatures, effective thermal isolation is achieved. The proposed THz dual-carrier MPA and 2DSQW-based receiver provide a high-bandwidth, low-power solution for scalable wireless multichip communication in both classical and quantum computing systems.

向多芯片和富含加速器的计算架构的过渡暴露了传统有线互连的局限性,包括带宽限制、延迟和功率效率低下。虽然无线互连提供了一种可扩展的替代方案,但现有的收发器技术往往缺乏有效的多芯片通信所需的抗干扰能力。为了解决这些挑战,我们引入了太赫兹(THz)模块化相控阵(MPA)发射器和基于二维半导体量子阱(2DSQW)的纳米接收器,从而实现了抗噪声信号解调,而无需庞大的处理硬件。双载波MPA模型提高了光束聚焦精度,同时抑制了光栅瓣,减轻了与接收机的偏振失配。接收机响应采用Floquet工程进行表征,利用时间周期辐射场中载流子的量子行为来实现精确的极化相关响应调谐。基于2dsqw的接收器独特的几何设计有助于空间调制,确保鲁棒的噪声抑制和干扰检测。这种架构特别适合多芯片量子处理器的垂直通信,因为高布线密度和热限制阻碍了可扩展性。通过在高温下操作MPA变送器,同时将接收器保持在较低温度下,可以实现有效的热隔离。所提出的太赫兹双载波MPA和基于2dsqw的接收器为经典和量子计算系统中的可扩展无线多芯片通信提供了高带宽、低功耗的解决方案。
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引用次数: 0
Photoluminescence Properties of Type-II GaSb/GaAs Quantum Rings ii型GaSb/GaAs量子环的光致发光特性
IF 3.9 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-08-21 DOI: 10.1002/adpr.202500125
Shumithira Gandan, Anna Musiał, Wojciech Rudno-Rudziński, Marek G. Mikulicz, Denise Montesdeoca, Michael Schmidt, Juan S. D. Morales, Andrew J. Marshall, Anthony Krier, Peter J. Carrington, Grzegorz Sęk

Type-II quantum rings (QRs) exhibit unique physics with great potential for future technologies. In this work, the magneto-optical properties and carrier dynamics of single- and ten-layer stacked GaSb/GaAs QR ensembles fabricated by molecular beam epitaxy are investigated. Activation energies extracted in both single- and ten-layer structures with temperature-dependent photoluminescence (PL), establish recombination dynamics closely linked to the growth method of the nanostructures. Clear optical absorption characteristics are also determined with PL-excitation experiments. In addition, transient temperature-dependent PL reveals distinct recombination pathways through nontrivial carrier decay behavior. With increasing excitation power density, a strong blue shift in peak position energies is observed due to evolving carrier kinetics across low and high excitation regimes. Finally, optical Aharonov–Bohm oscillations are demonstrated for the first time in type-II QRs. The data presented here are expected to advance the optimization of growth and physical properties of GaSb/GaAs QRs.

ii型量子环(QRs)具有独特的物理特性,具有巨大的未来技术潜力。本文研究了分子束外延制备的单层和十层叠置GaSb/GaAs QR系综的磁光特性和载流子动力学。利用温度依赖光致发光(PL)技术提取单层和十层结构的活化能,建立了与纳米结构生长方式密切相关的重组动力学。通过pl激发实验确定了清晰的光学吸收特性。此外,瞬态温度相关的PL通过非平凡的载流子衰变行为揭示了不同的重组途径。随着激发功率密度的增加,由于载流子动力学在低激发和高激发状态下的演变,观察到峰值位置能量的强蓝移。最后,在ii型QRs中首次证明了光学Aharonov-Bohm振荡。本文提出的数据有望促进GaSb/GaAs QRs的生长和物理性质的优化。
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引用次数: 0
Ultrashort-Pulsed Laser Diffusion Enhancement in Liquids for Cold Extraction of Coffee in an Analytically Validated Low-Fluence Regime 在分析验证的低通量条件下,超短脉冲激光在咖啡冷萃取液中的扩散增强
IF 3.9 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-08-21 DOI: 10.1002/adpr.202500115
Tina Friedenauer, Simela Kordhishte, Wiebke L. M. Narz, Tobias Bessel, Lucie K. Tintrop, Maryam Vosough, Amir Salemi, Cedric Thom, Sven W. Meckelmann, Maximilian Spellauge, Alexander Sommeryns, Christoph Rehbock, Torsten C. Schmidt, Oliver J. Schmitz, Heinz P. Huber, Stephan Barcikowski

Coffee is one of the most popular beverages, characterized by a complex composition and individual flavor profiles, strongly affected by extraction methods. A continuous and scalable cold extraction method based on irradiation of coffee particle dispersions (<200 μm) with a picosecond-pulsed laser is exploited, analyzing the influence of laser fluence (20–690 mJ cm−2) and pulse number (1–10) on the extract composition. The results highlight the generation of a unique volatile aroma profile at low fluence (35 mJ cm−2) and a reduced acidity in the liquid phase, which is neither correlated with a global temperature increase nor with changes in the specific surface area. This unique aroma profile is attributed to pulsed laser diffusion enhancement in liquids, resulting in localized heating and substance-specific alteration of the extraction kinetics, with energy consumption three times lower than classical hot coffee extraction and the potential for technical scale processing.

咖啡是最受欢迎的饮料之一,其特点是成分复杂,风味独特,深受提取方法的影响。研究了皮秒脉冲激光辐照咖啡颗粒分散体(<200 μm)的连续可扩展冷萃取方法,分析了激光能量(20 ~ 690 mJ cm−2)和脉冲数(1 ~ 10)对萃取物成分的影响。研究结果表明,在低通量(35 mJ cm−2)下产生了独特的挥发性香气,液相酸度降低,这与全球温度升高和比表面积变化无关。这种独特的香气特征归因于脉冲激光在液体中的扩散增强,导致局部加热和物质特异性的提取动力学改变,能耗比传统的热咖啡提取低三倍,具有技术规模加工的潜力。
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引用次数: 0
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Advanced Photonics Research
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