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Artificial Intelligence-Enhanced Metamaterial Bragg Multilayers for Radiative Cooling
IF 3.7 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-10-08 DOI: 10.1002/adpr.202400088
David Osuna Ruiz, Maite Aznarez-Sanado, Pilar Herrera-Plaza, Miguel Beruete

A full numerical study combining artificial intelligence (AI) methods and electromagnetic simulation software on a multilayered structure for radiative cooling (RC) is investigated. The original structure is made of SiO2/Si nanometer-thick layers that make a Bragg mirror for wavelengths in the solar irradiance window (0.3–4 μm). The structures are then optimized in terms of the calculated net cooling power and characterized via the reflected and absorbed incident light as a function of their structural parameters. This investigation provides with optimal designs of beyond-Bragg, all-dielectric, ultra-broadband mirrors that provide net cooling powers in the order of ≈100 W m−2, similar to the best-performing structures in literature. Furthermore, it explains AI's success in producing these structures and enables the analysis of resonant conditions in metal-free multilayers with unconventional layer thickness distributions, offering innovative tools for designing highly efficient structures in RC.

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引用次数: 0
1 × N All-Logic Optical Switch Based on Polymer Platform Using Multimode Interferometer
IF 3.7 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-10-08 DOI: 10.1002/adpr.202400118
Guoyan Zeng, Daming Zhang, Fei Wang, Xibin Wang, Yuexin Yin

The compact and broadband optical switch with a large port count is demanded with the increasing communication capacity. In this article, a universal method for modeling the 1 × N switch using multimode interferometer (MMI) through transmission matrixes is proposed. Herein, the reasons for the narrowing of the operating bandwidth switch are analyzed. As a proof of concept, a wide bandwidth 1 × 4 switch, which has an insertion loss lower than 23.7 dB, and a cross talk better than −10 dB at 1550 nm are simulated, designed, and fabricated. The cross talk throughout the C band is lower than −8.5 dB. According to the experimental result, the 1 × 4 switch with four-equal-length modulating arms shows a 32 nm bandwidth for −10 dB cross talk which is 13 times larger than traditional switch. The switch realizes a multi-port logic optical switch by modulation. The 1 × N switch based on the generalized Mach–Zehnder interferometer (GMZI) structure reduce the footprint significantly compared with the 1 × N switch consisting of a 1 × 2 switch cascade. It is believed that 1 × N switch based on GMZI structures is a promising solution to increase integration density.

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引用次数: 0
Ultrafast Terahertz Superconductor Van der Waals Metamaterial Photonic Switch 超快太赫兹超导体范德华超材料光子开关
IF 3.7 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-10-07 DOI: 10.1002/adpr.202470029
Kaveh Delfanazari

2D Layered Superconductors

In article number 2400045, Kaveh Delfanazari showcases methods for the realization of ultrafast terahertz (THz) metamaterial photonic switches on a few nanometer-thick layered high-temperature superconductor van der Waals (vdWs). The metamaterial array offers active modulation of THz amplitude and phase with an ultrafast-picosecond-switching timescale. The device holds promise for the development of future THz communication circuits and systems operating at cryogenic temperatures.

二维层状超导体 在编号为 2400045 的文章中,Kaveh Delfanazari 展示了在几纳米厚的层状高温超导体范德华(vdWs)上实现超快太赫兹(THz)超材料光子开关的方法。该超材料阵列可主动调制太赫兹振幅和相位,开关时间超快,可达皮秒级。该装置有望用于开发未来在低温条件下运行的太赫兹通信电路和系统。
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引用次数: 0
Structural Colors Derived from the Combination of Core–Shell Particles with Cellulose 核壳粒子与纤维素结合产生的结构色彩
IF 3.7 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-10-07 DOI: 10.1002/adpr.202470027
Regina Leiner, Lukas Siegwardt, Catarina Ribeiro, Jonas Dörr, Christian Dietz, Robert W. Stark, Markus Gallei

Core–Shell Particles

Essential features of functional optical materials are their interaction with light and underlying structures. In article number 2400091, Markus Gallei and co-workers report the combination of structural colors with cellulose, a renewable and biodegradable biopolymer. The latter acts as reinforcement agents, maintaining the polymer opal film’s structural color and mechanochromic material behavior.

核壳粒子 功能性光学材料的基本特征是与光和底层结构的相互作用。在文章编号 2400091 中,Markus Gallei 及其合作者报告了结构色与纤维素(一种可再生和生物降解的生物聚合物)的结合。纤维素是一种可再生、可生物降解的生物聚合物,可作为增强剂,保持聚合物蛋白石薄膜的结构颜色和机械变色材料特性。
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引用次数: 0
Room-Temperature Lasing of Dual-Metal Nanoparticle Surface Lattice Resonance with Monolithic InGaAs Multiple Quantum Wells on GaAs Substrates
IF 3.7 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-09-30 DOI: 10.1002/adpr.202400120
Wen-Hsuan Hsieh, Chia-Jui Chang, Cheng-Ching Li, Kuo-Ping Chen, Jhih-Sheng Wu, Chia-Yen Huang, Tien-Chang Lu

This study demonstrates the surface lattice resonance (SLR) laser utilizing asymmetric dual-metallic nanoparticle arrays, incorporating a high-refractive-index material, which exhibits a confinement factor of 16%, enhancing the coupling between metal and dielectric materials. Multiple quantum wells (MQWs) are integrated with plasmonic SLR in the proposed structure. Through theoretical design and experimental validation, the MQW plasmonic SLR laser exhibits excellent high Q-factor and stable operation at room temperature. This demonstration enhances laser performance and achieves low-threshold operation with a laser threshold as low as ≈2.39 MW cm−2. This study's design of plasmonic SLR lasers further advances the realization of optoelectronic device applications.

这项研究展示了利用非对称双金属纳米粒子阵列的表面晶格共振(SLR)激光器,该激光器采用了高折射率材料,具有 16% 的约束因子,增强了金属和介电材料之间的耦合。在所提出的结构中,多个量子阱(MQW)与质子 SLR 集成在一起。通过理论设计和实验验证,MQW 质子 SLR 激光器表现出卓越的高 Q 值因子,并能在室温下稳定工作。该演示提高了激光性能,实现了低阈值工作,激光阈值低至≈2.39 MW cm-2。这项研究设计的等离子体 SLR 激光器进一步推动了光电器件应用的实现。
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引用次数: 0
A Two-Stage Polymerization Strategy for Preparing Polymer-Network Liquid Crystals with Oxygen-Sensing Property 制备具有氧传感特性的聚合物网络液晶的两阶段聚合策略
IF 3.7 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-09-09 DOI: 10.1002/adpr.202470026
Zongdai Liu, Zhibo Zhang, Yi Zhang, Dan Luo, Kun-Lin Yang

Polymer-Network Liquid Crystals

In article number 2300340, Dan Luo, Kun-Lin Yang, and co-workers show that after partially completed photopolymerization, the polymer network liquid crystal undergoes a secondary polymerization to form an isotropic polymer network when it is heated beyond its clearing point, resulting in an irreversible optical appearance change from transparent to cloudy. It enables applications such as a heating stopwatch and oxygen sensing.

聚合物网络液晶 在编号为 2300340 的文章中,Dan Luo、Kun-Lin Yang 及合作者展示了聚合物网络液晶在部分完成光聚合后,当加热超过其清澈点时,会发生二次聚合,形成各向同性的聚合物网络,从而导致从透明到浑浊的不可逆光学外观变化。它可用于加热秒表和氧气传感等应用。
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引用次数: 0
Progress on Coherent Perovskites Emitters: From Light-Emitting Diodes under High Current Density Operation to Laser Diodes 相干 Perovskites 发射器的研究进展:从高电流密度下的发光二极管到激光二极管
IF 3.7 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-09-09 DOI: 10.1002/adpr.202470024
Gayoung Lee, Yejin Jun, Hyeonji Lee, Kwangdong Roh

Coherent Perovskites Emitters

In article number 2400033, Kwangdong Roh and co-workers provide a comprehensive overview of the historical progress in perovskite lasers and light-emitting didoes, along with important design considerations essential for their development.

相干过氧化物发光器 在编号为 2400033 的文章中,Kwangdong Roh 及其合作者全面概述了过氧化物激光器和发光二级管的历史进展,以及对其发展至关重要的重要设计考虑因素。
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引用次数: 0
Relative Permittivity and Optoelectronic Performances of Halide Perovskites: Study of Combined First-Principles Simulation and Combinatorial Synthesis 卤化物包荧光体的相对导率和光电性能:第一原理模拟与组合合成的结合研究
IF 3.7 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-09-04 DOI: 10.1002/adpr.202400039
SangMyeong Lee, Hee Jung Kim, Young Ju Kim, Geon Woo Yoon, Oh Yeong Gong, Won Bin Kim, Hyun Suk Jung

Owing to their excellent optoelectronic properties, halide perovskites (HPs) have garnered significant attention in the field of optoelectronics. However, conventional HPs-based optoelectronic devices primarily are fabricated using solution-based processes, implying that extremely time-consuming needs to individually synthesize their composition-dependent optoelectronic properties. This study demonstrates the feasibility of combining first-principles simulations with combinatorial synthesis, comparing the effects of HP properties on optoelectronic devices using this combined approach. The first-principles simulations confirm that increasing the ratio of small halide ions increased the band gap by k·p perturbation theory and harmonic oscillator models. By fabricating HP thin films with compositional gradients using combinatorial synthesis, it is confirmed that an increase in band gap corresponds to a decrease in static relative permittivity. Furthermore, HP-based optoelectronic devices are fabricated to measure their photoelectric conversion efficiency and responsivity based on the simulated and measured relative permittivity, including time-resolved photoluminescence. The findings demonstrate the influence of the relative permittivity on device performance, elucidating the relationship between band structure and relative permittivity. Therefore, in this study, the potential of combining first-principles simulations with combinatorial synthesis is confirmed by comparing the relative permittivity characteristics of optoelectronics developed using this combined approach.

卤化物过氧化物(HPs)具有优异的光电特性,因此在光电领域备受关注。然而,基于卤化物的传统光电器件主要采用溶液法制造,这意味着需要耗费大量时间来单独合成其与成分相关的光电特性。本研究证明了第一原理模拟与组合合成相结合的可行性,并利用这种组合方法比较了 HP 特性对光电器件的影响。第一原理模拟证实,通过k-p扰动理论和谐波振荡器模型,增加小卤离子的比例可以增大带隙。通过使用组合合成法制造具有成分梯度的 HP 薄膜,证实了带隙的增大与静态相对介电常数的减小相对应。此外,还制作了基于 HP 的光电器件,根据模拟和测量的相对介电常数测量其光电转换效率和响应度,包括时间分辨光致发光。研究结果表明了相对介电常数对器件性能的影响,阐明了带状结构与相对介电常数之间的关系。因此,在本研究中,通过比较使用这种组合方法开发的光电器件的相对介电常数特性,证实了第一原理模拟与组合合成相结合的潜力。
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引用次数: 0
High-Power GaN-Based Blue Laser Diodes Degradation Investigation and Anti-aging Solution 大功率氮化镓基蓝色激光二极管的降解研究与抗老化解决方案
IF 3.7 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-09-04 DOI: 10.1002/adpr.202400119
Enming Zhang, Yue Zeng, Wenyu Kang, Zhibai Zhong, Yushou Wang, Tongwei Yan, Shaohua Huang, Zhongying Zhang, Kechuang Lin, Junyong Kang

Gallium nitride (GaN)-based semiconductor laser diodes (LDs) have garnered significant attention due to their promising applications. However, high-power LDs face serious degradation issues that limit their practical use. This study investigates the degradation factors of 437 nm and 6.3 W LDs by comparing light–current–voltage (L–I–V) characteristics, transmission electron microscopy (TEM), cathodoluminescence (CL), and secondary ion mass spectroscopy (SIMS) before and after 1000-h aging. The diffusion of mirror coating from the resonant cavity surface is identified as a key factor contributing to high-power LD degradation, which has not been reported in milliwatt-level LDs. Meanwhile, the mechanisms behind the LD degradation are profiled and summarized together with the diffusion and other factors. On basis of the mechanism exploration, an anti-aging technology for high-power GaN-based LDs is developed by using aluminum nitride for passivation layer and sapphire materials for mirror film. This anti-aging technology has been verified, and a nearly ten-time degradation suppression is achieved from 1000 h. This study elucidates the degradation mechanisms of high-power GaN LDs and provides an effective technology to extend their lifespan, thereby prompting the practical applications of high-power LDs.

基于氮化镓(GaN)的半导体激光二极管(LD)因其广阔的应用前景而备受关注。然而,高功率 LD 面临着严重的降解问题,限制了其实际应用。本研究通过比较老化 1000 小时前后的光-电流-电压(L-I-V)特性、透射电子显微镜(TEM)、阴极发光(CL)和二次离子质谱(SIMS),研究了 437 nm 和 6.3 W LD 的降解因子。研究发现,镜面涂层从谐振腔表面扩散是导致大功率 LD 退化的一个关键因素,而这在毫瓦级 LD 中尚未见报道。同时,对 LD 退化背后的机制进行了剖析,并结合扩散和其他因素进行了总结。在机理探索的基础上,利用氮化铝作为钝化层和蓝宝石材料作为镜面膜,开发出了大功率氮化镓基 LD 的抗老化技术。该研究阐明了大功率氮化镓基 LD 的降解机理,为延长其使用寿命提供了有效技术,从而推动了大功率 LD 的实际应用。
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引用次数: 0
Maximizing the Electromagnetic Efficiency of Spintronic Terahertz Emitters 最大化自旋电子太赫兹发射器的电磁效率
IF 3.7 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-09-04 DOI: 10.1002/adpr.202400064
Pierre Koleják, Geoffrey Lezier, Daniel Vala, Baptiste Mathmann, Lukáš Halagačka, Zuzana Gelnárová, Yannick Dusch, Jean-François Lampin, Nicolas Tiercelin, Kamil Postava, Mathias Vanwolleghem

Optically pumped spintronic terahertz emitters (STEs) have, in less than a decade, strongly impacted terahertz (THz) source technology, by the combination of their Fourier-limited ultrafast response, their phononless emission spectrum and their wavelength-independent operation. However, the intrinsic strength of the inverse spin Hall effect governing these devices introduces a challenge: the optical-to-terahertz conversion efficiency is considerably lower than traditional sources. It is therefore primordial to maximize at least their electromagnetic efficiency independently of the spin dynamics at play. Using a rigorous time-domain treatment of the electromagnetic generation and extraction processes, an optimized design is presented and experimentally confirmed. With respect to the strongest reported spintronic THz emitters it achieves a 250% enhancement of the emitted THz field and therefore an 8 dB increase of emitted power. This experimental achievement brings STE close to the symbolic barrier of mW levels. The design strategy is generically applicable to any kind of ultrafast spin-to-charge conversion (S2C) system. On a broader level, our work highlights how a rigorous handling of the purely electromagnetic aspects of THz spintronic devices can uncover overlooked aspects of their operation and lead to substantial improvements.

光泵浦自旋电子太赫兹发射器(STE)具有傅里叶限制的超快响应、无声子发射光谱和与波长无关的操作等特点,在不到十年的时间里对太赫兹(THz)信号源技术产生了重大影响。然而,制约这些设备的反自旋霍尔效应的内在强度带来了一个挑战:光到太赫兹的转换效率大大低于传统源。因此,在不考虑自旋动力学作用的情况下,至少最大限度地提高电磁效率是最基本的要求。通过对电磁产生和提取过程进行严格的时域处理,提出了一种优化设计,并得到了实验证实。与已报道的最强自旋电子太赫兹发射器相比,它实现了发射太赫兹场 250% 的增强,因此发射功率增加了 8 dB。这一实验成果使 STE 接近毫瓦级的象征性障碍。该设计策略一般适用于任何类型的超快自旋-电荷转换(S2C)系统。在更广泛的层面上,我们的工作突出了如何严格处理太赫兹自旋电子器件的纯电磁方面,从而发现其运行中被忽视的方面,并带来实质性的改进。
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引用次数: 0
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Advanced Photonics Research
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