Pub Date : 2025-01-31DOI: 10.1140/epjd/s10053-025-00953-8
S. S. A. S. Bukhari, R. Gottschalk, A. Lindinger
We report two-photon excited fluorescence of dyes for refracted laser beams by utilizing tailored laser pulses. A fluorescence contrast difference due to phase shaping could be achieved between different coumarin dyes. Particularly, an increased contrast difference is obtained for configurations close to the Brewster angle. Furthermore, by using a subsequent deformable phase plate for spatial shaping it was possible to precisely adjust the laser beam for controlled refraction at the liquid dye surface. A polarization-dependent refraction was observed when directing the shaped laser beam on the curved liquid adhesion meniscus close to the cuvette wall. This results in a refraction-dependent contrast difference. The presented method could be utilized for surface-sensitive biophotonic imaging applications.
{"title":"Two-photon excited fluorescence with shaped laser pulses for refractive beams","authors":"S. S. A. S. Bukhari, R. Gottschalk, A. Lindinger","doi":"10.1140/epjd/s10053-025-00953-8","DOIUrl":"10.1140/epjd/s10053-025-00953-8","url":null,"abstract":"<p>We report two-photon excited fluorescence of dyes for refracted laser beams by utilizing tailored laser pulses. A fluorescence contrast difference due to phase shaping could be achieved between different coumarin dyes. Particularly, an increased contrast difference is obtained for configurations close to the Brewster angle. Furthermore, by using a subsequent deformable phase plate for spatial shaping it was possible to precisely adjust the laser beam for controlled refraction at the liquid dye surface. A polarization-dependent refraction was observed when directing the shaped laser beam on the curved liquid adhesion meniscus close to the cuvette wall. This results in a refraction-dependent contrast difference. The presented method could be utilized for surface-sensitive biophotonic imaging applications.</p>","PeriodicalId":789,"journal":{"name":"The European Physical Journal D","volume":"79 2","pages":""},"PeriodicalIF":1.5,"publicationDate":"2025-01-31","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1140/epjd/s10053-025-00953-8.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143109936","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2025-01-29DOI: 10.1140/epjd/s10053-025-00956-5
Victor I. Romanenko, Nataliya V. Kornilovska, Leonid P. Yatsenko
We consider the interaction of a two-level atom with two counter-propagating light pulses of different carrier frequencies. To ensure adiabatic interaction, the pulse duration is much longer than both the inverse frequency difference and the maximum Rabi frequencies of the pulses. For the first time, we examine the case where the atom is initially prepared in a superposition of the ground and excited states with a momentum difference corresponding to one-photon recoil. We identify the conditions under which the atom’s final state is determined by the phase difference of the momentum components of the initial atomic wave. Given the large pulse duration, the interference effects depend critically on the rate of spontaneous emission from the excited state. We analyze the role of spontaneous emission using the Monte Carlo wave function method. The results of our calculations elucidate the influence of spontaneous radiation on both the momentum transferred to the atom and the interference outcome of the two atomic waves.
{"title":"Controlling atomic wave interference by counter-propagating light pulses of different carrier frequencies","authors":"Victor I. Romanenko, Nataliya V. Kornilovska, Leonid P. Yatsenko","doi":"10.1140/epjd/s10053-025-00956-5","DOIUrl":"10.1140/epjd/s10053-025-00956-5","url":null,"abstract":"<p>We consider the interaction of a two-level atom with two counter-propagating light pulses of different carrier frequencies. To ensure adiabatic interaction, the pulse duration is much longer than both the inverse frequency difference and the maximum Rabi frequencies of the pulses. For the first time, we examine the case where the atom is initially prepared in a superposition of the ground and excited states with a momentum difference corresponding to one-photon recoil. We identify the conditions under which the atom’s final state is determined by the phase difference of the momentum components of the initial atomic wave. Given the large pulse duration, the interference effects depend critically on the rate of spontaneous emission from the excited state. We analyze the role of spontaneous emission using the Monte Carlo wave function method. The results of our calculations elucidate the influence of spontaneous radiation on both the momentum transferred to the atom and the interference outcome of the two atomic waves.</p>","PeriodicalId":789,"journal":{"name":"The European Physical Journal D","volume":"79 1","pages":""},"PeriodicalIF":1.5,"publicationDate":"2025-01-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143109801","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2025-01-28DOI: 10.1140/epjd/s10053-025-00957-4
D. Buljubasic, P. K. Kariuki, J. Okumu
Reported triple differential cross sections (TDCS) for electron-impact ionization of nitrogen molecule have been calculated by employing distorted-wave Born approximation (DWBA) and independent-atom model (IAM), for incident electron energy of 500 eV, and ejected electron energies of 37 eV, 74 eV, and 205 eV, in coplanar asymmetric geometry. Scattering amplitudes of independent nitrogen atoms calculated in the DWBA were used to determine the TDCS of the molecule in IAM. The obtained results are compared to available experimental and theoretical data. Reasonably good qualitative and quantitative agreement was found for low to intermediate ejected electron energies, in terms of binary and recoil peak prediction. Quantitative discrepancies at higher ejected electron energies are attributed to the DWBA limitations.
{"title":"Electron-impact ionization TDCS of a nitrogen molecule using the DWBA and IAM-AR","authors":"D. Buljubasic, P. K. Kariuki, J. Okumu","doi":"10.1140/epjd/s10053-025-00957-4","DOIUrl":"10.1140/epjd/s10053-025-00957-4","url":null,"abstract":"<p>Reported triple differential cross sections (TDCS) for electron-impact ionization of nitrogen molecule have been calculated by employing distorted-wave Born approximation (DWBA) and independent-atom model (IAM), for incident electron energy of 500 eV, and ejected electron energies of 37 eV, 74 eV, and 205 eV, in coplanar asymmetric geometry. Scattering amplitudes of independent nitrogen atoms calculated in the DWBA were used to determine the TDCS of the molecule in IAM. The obtained results are compared to available experimental and theoretical data. Reasonably good qualitative and quantitative agreement was found for low to intermediate ejected electron energies, in terms of binary and recoil peak prediction. Quantitative discrepancies at higher ejected electron energies are attributed to the DWBA limitations.\u0000</p>","PeriodicalId":789,"journal":{"name":"The European Physical Journal D","volume":"79 1","pages":""},"PeriodicalIF":1.5,"publicationDate":"2025-01-28","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143109365","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2025-01-28DOI: 10.1140/epjd/s10053-025-00952-9
Nisreen Kh. Abdalameer, Nadia Jasim Ghdeeb, Kawther A. Khalaph, Yasmine Taha
Nanoscale selenium oxide is a significant substance because of its extensive use in health, manufacturing, and electronics. The present study involves the manufacture of selenium oxide nanoparticles using Syzygium Aromaticum flower plant extract as a reducing agent and employing cold plasma technology to enhance the nanosynthesis process. An investigation was conducted to analyze the impact of various synthesis circumstances on the characteristics of the resultant particles, including particle size, size distribution, and form. Scanning electron microscopy and ultraviolet–visible spectroscopy have been used to investigate the physicochemical characteristics of the nanoparticles produced. The findings demonstrated that using clove flower extract as an eco-friendly and renewable substance in the synthesis procedure enhanced the characteristics of nano selenium oxide, thereby presenting a viable substitute for conventional chemical-based approaches. The cold plasma technique has shown efficacy in precisely regulating particle size and dispersion. The work highlights the significance of using natural resources with contemporary technologies in synthesizing nanomaterials. It paves the way for further investigations into using plant extracts in nanotechnology applications.