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Injection, confinement, and diagnosis of electrons and positrons in a permanent magnet dipole trap 永磁体偶极子阱中电子和正电子的注入、约束和诊断
IF 1.5 4区 物理与天体物理 Q3 OPTICS Pub Date : 2024-12-05 DOI: 10.1140/epjd/s10053-024-00821-x
J. von der Linden, S. Nißl, A. Deller, M. Singer, N. Belmore, C. P. Hugenschmidt, T. Sunn Pedersen, H. Saitoh, E. V. Stenson

Prerequisites for the goal of studying long-lived, magnetically confined, electron–positron pair plasmas in the laboratory include the injection of both species into the trap, long trapping times, and suitable diagnostic methods. Here we report recent progress on these tasks achieved in a simple dipole trap based on a supported permanent magnet. For the injection of electrons, both an (textbf{E}times B) drift technique (of a (sim )2–(upmu )A, 6-eV beam) and “edge injection” (from a filament emitting a few mA and biased to some tens of volts) have been demonstrated; the former is suitable for low-density beams with smaller spatial and velocity spreads, while the latter employs fluctuations arising from collective behavior. To diagnose the edge-injected electrons, image potentials and currents induced on a wall probe, the magnet case, and wall electrodes were measured. Confinement of drift-injected positrons, measured experimentally, exhibited at least two well-separated timescales. Simulations reproduced this qualitatively, using a simple model of elastic collisions with residual background gas, and point to small adjustments for increasing trapping times. In a major upgrade to diagnostic capabilities, 25 bismuth germanate detectors, placed in three reentrant ports, are able to localize annihilation gammas, which will be used in future experiments to distinguish between different loss channels.

在实验室中研究长寿命、磁约束、电子-正电子对等离子体的先决条件包括两种物质的注入、较长的捕获时间和合适的诊断方法。在这里,我们报告了在基于支撑永磁体的简单偶极子阱中实现这些任务的最新进展。对于电子注入,已经证明了(textbf{E}times B)漂移技术((sim ) 2 - (upmu ) a, 6-eV光束)和“边缘注入”(从发射几毫安并偏置到几十伏特的灯丝);前者适用于空间和速度扩散较小的低密度光束,而后者则采用由集体行为引起的波动。为了诊断边缘注入电子,测量了在壁探针、磁铁盒和壁电极上产生的成像电位和电流。通过实验测量,漂移注入正电子的约束表现出至少两个分离良好的时间尺度。模拟定性地再现了这一点,使用了一个简单的与残余背景气体的弹性碰撞模型,并指出了增加捕获时间的小调整。在诊断能力的重大升级中,25个锗酸铋探测器放置在三个可重返端口中,能够定位湮灭伽马,这将在未来的实验中用于区分不同的损失通道。
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引用次数: 0
Combination of the TD-DFT and the pixel counting method for determining electron capture cross sections for protons impacting on organic molecules 结合TD-DFT和像素计数法测定质子撞击有机分子的电子俘获截面
IF 1.5 4区 物理与天体物理 Q3 OPTICS Pub Date : 2024-12-05 DOI: 10.1140/epjd/s10053-024-00939-y
Luca A. de Oliveira, Jhaison C. de Farias, Mario A. Bernal

The electron capture by heavy charged particles is of interest in a wide range of physical applications. In radiation biophysics, electron capture cross sections (ECCS) is a key information for the implementation of Monte Carlo simulation codes. In this work, the time-dependent density functional theory (TD-DFT) has been used for the determination of ECCS for protons impacting on atoms with presence in organic compounds, in the 1–200 keV energy range. Later, these atomic cross sections were combined through the pixel counting method for determining corresponding cross section of small and large organic molecules and water, which is of primordial importance in radiation biophysics. The large organic molecules include DNA bases and a whole DNA base pair. Excellent results were obtained for the small molecules along the whole energy range. For DNA components, good results were found at high energies (100–200 keV). At lower energies, larger discrepancies were obtained when compared with other theoretical and experimental work. The possible causes for these discrepancies are deeply discussed. This work should support later works for developing a charge equalization method for classical molecular dynamics to describe fast proton collisions with organic materials.

重带电粒子的电子捕获在广泛的物理应用中引起了人们的兴趣。在辐射生物物理学中,电子俘获截面(ECCS)是实现蒙特卡罗仿真代码的关键信息。在这项工作中,时间依赖的密度泛函理论(TD-DFT)已被用于测定质子在1-200 keV能量范围内撞击有机化合物中存在的原子的ECCS。随后,通过像素计数法将这些原子截面组合起来,确定大小有机分子与水的对应截面,这在辐射生物物理学中具有至关重要的意义。大的有机分子包括DNA碱基和完整的DNA碱基对。在整个能量范围内,对小分子都取得了很好的结果。对于DNA成分,在高能量(100-200 keV)下发现了良好的结果。在较低的能量下,与其他理论和实验工作相比,得到了较大的差异。对这些差异的可能原因进行了深入的讨论。这项工作应该支持以后的工作,以发展经典分子动力学的电荷均衡方法来描述与有机材料的快速质子碰撞。
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引用次数: 0
Highly efficient nonreciprocity and nonreciprocal photonic devices in a semiconductor quantum well 半导体量子阱中的高效非互易和非互易光子器件
IF 1.5 4区 物理与天体物理 Q3 OPTICS Pub Date : 2024-12-04 DOI: 10.1140/epjd/s10053-024-00937-0
Yunran Ge, Kang Zheng, Boxiang Fang, Chunling Ding, Xiangying Hao, Rui-Bo Jin

We propose theoretically a non-magnetic optical nonreciprocity (ONR) scheme with high efficiency by employing the four-wave mixing (FWM) effect in an asymmetric semiconductor three-coupled-quantum-well (TCQW) nanostructure. Nonreciprocal transmission and nonreciprocal phase shift in this TCQW, both with high transmission rates, can be achieved using suitable parameters. Considering an orbital-angular-momentum (OAM) probe beam, the perfect nonreciprocity can be obtained based on the highly efficient FWM. Furthermore, the integration of this TCQW nanostructure into a Mach–Zehnder interferometer enables the fabrication of highly efficient optical isolators and optical circulators by selecting appropriate parameters. The optical isolator exhibits an isolation ratio of 97.76 dB and an insertion loss of 0.25 dB, while the optical circulator demonstrates a fidelity of 0.9993 and a photon survival probability of 0.9517. Our approach based on semiconductor media has the advantages of easy fabrication and good integration with adjustable parameters. In conjunction with the distinctive characteristics of the OAM beam, our protocol offers a theoretical framework for the development of highly integrated and multi-dimensional nonreciprocity and nonreciprocal photonic devices.

在非对称半导体三耦合量子阱(TCQW)纳米结构中利用四波混频(FWM)效应,从理论上提出了一种高效率的非磁性光非互易(ONR)方案。在适当的参数下,可以实现高传输速率的非倒易传输和非倒易相移。考虑轨道-角动量(OAM)探测光束,基于高效的FWM可以获得完美的非互易性。此外,将该TCQW纳米结构集成到马赫-曾德干涉仪中,通过选择适当的参数,可以制造出高效的光隔离器和光环行器。光隔离器的隔离比为97.76 dB,插入损耗为0.25 dB,光环行器的保真度为0.9993,光子存活概率为0.9517。该方法基于半导体介质,具有制作简单、集成度好、参数可调等优点。结合OAM光束的独特特性,我们的协议为高度集成和多维非互易和非互易光子器件的发展提供了理论框架。
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引用次数: 0
Modified six-state cryptographic protocol with entangled ancilla states 带有纠缠辅助状态的改进六状态加密协议
IF 1.5 4区 物理与天体物理 Q3 OPTICS Pub Date : 2024-12-04 DOI: 10.1140/epjd/s10053-024-00934-3
Rashi Jain, Satyabrata Adhikari

In a realistic situation, it is very difficult to communicate securely between two distant parties without introducing any disturbances. These disturbances might occur either due to external noise or may be due to the interference of an eavesdropper. In this work, we consider and modify the six-state Quantum Key Distribution (QKD) protocol in which Eve can construct the unitary transformation that make all ancilla states entangled at the output, which is not considered in Bruss’s work [29]. Using the above proposed modification, we would like to study the effect of entangled ancilla states on the mutual information between Alice and Eve. To achieve this task, we calculate the mutual information between Alice and Bob and Alice and Eve and identify the region where the secret key is generated even in the presence of Eve. We find that, in general, the mutual information of Alice and Eve depends not only on the disturbance D but also on the concurrence of the ancilla states. We show that the entanglement of the ancilla states helps in generating the secret key in the region where Bruss’s six-state QKD protocol failed to do so. We have further shown that it is possible to derive the disturbance-free mutual information of Alice and Eve, if Eve manipulates her entangled ancilla state in a particular manner. Thus, in this way, we can show that a secret key can be generated between Alice and Bob even if the disturbance is large enough.

在现实情况下,在两个相距遥远的方之间进行安全通信而不引入任何干扰是非常困难的。这些干扰可能是由于外界的噪音,也可能是由于窃听者的干扰。在这项工作中,我们考虑并修改了六态量子密钥分发(QKD)协议,其中Eve可以构造使所有辅助状态在输出处纠缠的幺正变换,这在Bruss的工作[29]中没有考虑到。利用上述提出的修改,我们想要研究纠缠的辅助状态对Alice和Eve之间互信息的影响。为了完成这个任务,我们计算了Alice和Bob以及Alice和Eve之间的互信息,并确定了在Eve在场的情况下生成密钥的区域。我们发现,一般来说,Alice和Eve的互信息不仅取决于干扰D,还取决于辅助状态的并发性。我们证明了辅助状态的纠缠有助于在Bruss的六状态QKD协议无法生成密钥的区域生成密钥。我们进一步证明,如果夏娃以一种特定的方式操纵她的纠缠辅助状态,就有可能推导出爱丽丝和夏娃的无干扰互信息。因此,通过这种方式,我们可以证明即使干扰足够大,也可以在Alice和Bob之间生成密钥。
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引用次数: 0
Ionic fragmentation by electron impact of isobutanol: mass spectrum, appearance energies and Wannier exponents 异丁醇的电子撞击离子破碎:质谱、显现能和万尼尔指数
IF 1.5 4区 物理与天体物理 Q3 OPTICS Pub Date : 2024-11-28 DOI: 10.1140/epjd/s10053-024-00933-4
O. L. Oliveira Junior, M. C. A. Lopes, R. A. A. Amorim

The mass spectrum (MS) and appearance energies (AEs) of the cationic fragments formed in electron collisions with isobutanol were investigated in this work using a HIDEN EPIC 300 mass spectrometer. We highlight here the discovery of 6 new cationic fragments in the literature for MS as well as 10 AEs and ps values reported for the first time. The MS was acquired for electron impact energy of 70 eV, in the mass region of 1–80 amu and with a resolution of 1 amu. Here we observed the formation of 45 cationic fragments, thus complementing some data previously reported in the literature, 6 of which were unpublished. The relative abundances of the peaks recorded in the MS show good agreement within the experimental error range, with the available values reported in the literature, where such comparison is carried out. The AEs were determined from the acquisition of isobutanol ionic fragmentation curves, for the electron impact energies covering the cationic fragment formation threshold region. The extended Wannier law was applied to obtain the AEs and Wannier exponents (p) of the fragments recorded in the MS, with relative intensity typically greater than 4% of the most intense fragment. This resulted in MS of isobutanol and data for 15 fragments, of which 10 of these fragments are reported for the first time in this work.

Graphic abstract

本研究使用 HIDEN EPIC 300 质谱仪研究了与异丁醇发生电子碰撞时形成的阳离子碎片的质谱(MS)和外观能(AEs)。我们在此重点介绍文献中发现的 6 个新的阳离子碎片质谱,以及首次报道的 10 个 AE 和 ps 值。质谱采集的电子撞击能量为 70 eV,质量范围为 1-80 amu,分辨率为 1 amu。在这里,我们观察到了 45 个阳离子碎片的形成,从而补充了之前文献中报道的一些数据,其中 6 个数据是未发表的。质谱中记录的峰的相对丰度在实验误差范围内与文献中报道的可用值显示出良好的一致性。通过获取异丁醇离子碎片曲线,确定了阳离子碎片形成阈值区域的电子撞击能量的 AE 值。应用扩展的万尼尔定律获得质谱中记录的碎片的 AE 和万尼尔指数(p),相对强度通常大于最强烈碎片的 4%。这样就得到了异丁醇的质谱和 15 个片段的数据,其中 10 个片段在本研究中首次报道。
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引用次数: 0
Short laser pulse effects on spectral dynamics of encapsulated He, Ne, Ar atoms in fullerenes 短激光脉冲对富勒烯中封装 He、Ne 和 Ar 原子光谱动力学的影响
IF 1.5 4区 物理与天体物理 Q3 OPTICS Pub Date : 2024-11-26 DOI: 10.1140/epjd/s10053-024-00935-2
Mustafa Kemal Bahar

This work elucidates the effects of a short laser pulse on the excitation and ionization dynamics of an endofullerene system trapping He, Ne, and Ar atoms. The interactions of noble gas atoms are simulated within the framework of the Single Active Electron (SAE) approximation, and the encapsulation parameters are analyzed to illustrate the excitation and ionization dynamics. The endohedral confinement is modeled using the Woods–Saxon potential, which is a practical and advantageous model that aligns well with experimental data and considers static encapsulation. By considering different numerical values of the endohedral trapping parameters in simulating encapsulation, a detailed analysis on the depth of confinement, spherical shell thickness, the inner radius, and the smoothing parameters is performed to ferret out encapsulation effects in various forms. By determining the strength range and specific frequency values (and ranges) of the laser pulse, the work interprets how electron dynamics in endohedral fullerenes are shaped under laser pulses. All parameters and their respective ranges are crucial gains for optimizing system performance.

这项研究阐明了短激光脉冲对捕获 He、Ne 和 Ar 原子的内富勒烯系统的激发和电离动力学的影响。在单活泼电子(SAE)近似的框架内模拟了惰性气体原子的相互作用,并分析了封装参数,以说明激发和电离动力学。使用伍兹-萨克森势来模拟内面封闭,这是一个实用且有利的模型,能很好地与实验数据保持一致,并考虑了静态封装。在模拟封装过程中,通过考虑不同的内切面捕集参数数值,对封闭深度、球壳厚度、内半径和平滑参数进行了详细分析,以发现各种形式的封装效应。通过确定激光脉冲的强度范围和特定频率值(及范围),这项研究解释了内面富勒烯中的电子动力学是如何在激光脉冲下形成的。所有参数及其各自的范围对于优化系统性能至关重要。
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引用次数: 0
A molecular dynamics simulation framework for investigating ionizing radiation-induced nano-bubble interactions at ultra-high dose rates 研究超高剂量率电离辐射诱导纳米气泡相互作用的分子动力学模拟框架
IF 1.5 4区 物理与天体物理 Q3 OPTICS Pub Date : 2024-11-22 DOI: 10.1140/epjd/s10053-024-00928-1
Ramin Abolfath, Niayesh Afshordi, Sohrab Rahvar, Adri C. T. van Duin, Martin Rädler, Reza Taleei, Katia Parodi, Julie Lascaud, Radhe Mohan

We present a microscopic formalism that accounts for the formation of nano-scale bubbles owing to a burst of water molecules after the passage of high energy charged particles that lead to the formation of “hot” non-ionizing excitations or thermal spikes (TS). We construct amorphous track structures to account for the formation of TS by ionizing radiation in liquid water. Subsequently, we simulate sudden expansion and collective motion of water molecules by employing a molecular dynamics (MD) simulation that allows computation of ({{mathcal {O}}}(10^6)) particle trajectories and breaking/forming of chemical bonds on the fly using a reactive force field, ReaxFF. We calculate the fluctuations of thermodynamic variables before and after TS formation to model the macroscopic abrupt changes in the system, possibly the occurrence of a first-order phase transition, and go beyond the accessible simulation times by engaging fluid dynamic equations with appropriate underlying symmetries and boundary conditions. We demonstrate the coexistence of a rapidly growing condensed state of water and a hot spot that forms a stable state of diluted water at high temperatures and pressures, possibly at a supercritical phase. Depending on the temperature of TS, the thin shell of a highly dense state of water grows by three to five times the speed of sound in water, forming a thin layer of shock wave (SW) buffer, wrapping around the nano-scale cylindrical symmetric bubble. The stability of the bubble, as a result of the incompressibility of water at ambient conditions and the surface tension, allows the transition of supersonic SW to a subsonic contact discontinuity and dissipation to thermo-acoustic sound waves. Thus, TS gradually decays to acoustic waves, a channel of deexcitation that competes with the spontaneous emission of photons, and a direct mechanism for water luminescence. We further study the mergers of nanobubbles that lead to jet-flow structures at the collision interface. We introduce a time delay in the nucleation of nano-bubbles, a novel mechanism, responsible for the growth and stability of much larger or even micro-bubbles, possibly relevant to FLASH ultra-high dose rate (UHDR).

Molecular dynamic simulation of the interaction between two ionizing radiation-induced nano-bubble formed simultaneously.

我们提出了一种微观形式主义,解释了高能带电粒子通过后水分子爆发形成纳米级气泡,从而导致 "热 "非电离激发或热尖峰(TS)的形成。我们构建了非晶轨道结构,以解释电离辐射在液态水中形成 TS 的原因。随后,我们利用分子动力学(MD)模拟来模拟水分子的突然膨胀和集体运动,该模拟可以计算粒子轨迹({{mathcal {O}} (10^6)),并利用反应力场 ReaxFF 计算化学键的断裂/形成。我们计算了 TS 形成前后的热力学变量波动,以模拟系统中的宏观突变(可能是一阶相变的发生),并通过使用具有适当基础对称性和边界条件的流体动力学方程,超越了可获得的模拟时间。我们证明了快速增长的水凝结态与在高温高压下(可能处于超临界阶段)形成稀释水稳定态的热点共存的现象。根据 TS 的温度,高浓度水状态的薄壳会以三到五倍于水中声速的速度增长,形成一层薄薄的冲击波(SW)缓冲区,包裹着纳米级的圆柱对称气泡。由于水在环境条件下的不可压缩性和表面张力,气泡的稳定性使得超音速冲击波过渡到亚音速接触不连续性,并消散为热声声波。因此,热声波逐渐衰减为声波,这是一个与光子自发辐射竞争的去激发通道,也是水发光的直接机制。我们进一步研究了纳米气泡的合并,这导致了碰撞界面上的喷流结构。我们引入了纳米气泡成核过程中的时间延迟,这是一种新的机制,负责更大甚至更微小气泡的生长和稳定性,可能与 FLASH 超高剂量率(UHDR)有关。
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引用次数: 0
Discharge characteristics and ozone generation during CO2 to CO conversion by dielectric barrier discharge packed with TiO2-coated glass beads 用涂覆 TiO2 的玻璃珠填料进行介质阻挡放电将 CO2 转化为 CO 的过程中的放电特性和臭氧生成情况
IF 1.5 4区 物理与天体物理 Q3 OPTICS Pub Date : 2024-11-21 DOI: 10.1140/epjd/s10053-024-00927-2
Mohamed El Shaer, Heba Gabr, Ahmed Zaki, Milad Awad, Mahmoud Ashraf, Mona Mobasher, Adel Phillips, Hassan Afify

A packed-bed dielectric barrier discharge was used to investigate CO2 to CO conversion under different operating conditions as frequency, CO2/Ar gas mixture composition and gas flow rate, to understand the effects of their variations on current–voltage discharge characteristics, CO2 to CO conversion ratios, CO yields, and ozone production. Using TiO2-coated glass beads has changed the discharge behavior from the glow mode to a combined filamentary and surface discharge mode, making the discharge more diffuse for higher frequencies in the range of 3.6 to 6 kHz. Higher CO2 to CO conversion and CO yield are achieved by lowering both operating frequencies and CO2 concentrations in CO2/Ar gas mixture. For TiO2-coated glass beads packed discharge, increasing discharge frequency from 3.6 to 6 kHz lower CO2 conversion from 11.2% to 2.5%, while increasing CO2 concentrations in CO2/Ar gas mixture from 10 to 40% lowers conversion from 11.2% to 5%. The enhancement of ozone production by the introduction of TiO2-coated glass beads packing material may be related to improvements of conversion ratio from CO2 to CO and CO yield showing their larger values at lower frequencies and lower CO2 percentages in CO2/Ar gas mixture. Using inexpensive and easily synthesized in large quantities catalyst material, realized by TiO2 coating of glass beads in a microwave plasma torch, has permitted to reach DBD operational modes adequate for CO production in moderate concentrations suitable for applications in medicine and agriculture.

Graphical abstract

利用填料床介质阻挡放电研究了在频率、CO2/Ar 混合气体成分和气体流速等不同操作条件下 CO2 到 CO 的转化,以了解它们的变化对电流-电压放电特性、CO2 到 CO 的转化率、CO 产量和臭氧产生量的影响。使用涂有 TiO2 的玻璃珠使放电行为从辉光模式转变为丝状放电和表面放电相结合的模式,使放电在 3.6 至 6 kHz 的较高频率范围内更具扩散性。通过降低工作频率和 CO2/Ar 混合气体中的 CO2 浓度,可实现更高的 CO2 转化率和 CO 产率。对于涂有 TiO2 的玻璃珠填料放电,放电频率从 3.6 千赫提高到 6 千赫,二氧化碳转化率从 11.2% 降至 2.5%,而 CO2/Ar 混合气体中的二氧化碳浓度从 10% 提高到 40%,转化率从 11.2% 降至 5%。引入涂有 TiO2 的玻璃微珠填料可提高臭氧的产生,这可能与二氧化碳到一氧化碳的转化率和一氧化碳产率的提高有关,在频率较低和二氧化碳/Ar 混合气体中的二氧化碳比例较低时,转化率和一氧化碳产率的数值较大。通过在微波等离子体炬中对玻璃微珠进行 TiO2 涂层,使用廉价且易于大量合成的催化剂材料,可以达到 DBD 运行模式,足以在中等浓度下生产 CO,适合应用于医药和农业领域。
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引用次数: 0
Ionization of argon atom by positron and electron impact 氩原子受正电子和电子撞击而电离
IF 1.5 4区 物理与天体物理 Q3 OPTICS Pub Date : 2024-11-21 DOI: 10.1140/epjd/s10053-024-00930-7
O. Zaidi, A. Mansouri, S. Houamer, A. Tamin, T. Khatir, C. Dal Cappello

The positron and electron impact ionization of argon 3p at 200 eV impact energy is investigated using a theoretical model called 3CWZ. Within this model all particles of the continuum are represented by Coulomb waves with variable charges Z(r), the post-collision interaction and exchange effects are also included. The triple differential cross section is calculated and compared with recent measurements of Dubois and de Lucio (Atoms 9:78, 2021) and other theories when available, for several kinematics. Our numerical results are in overall good agreement with experiments and illustrate projectile charge effects, better than other available theories.

Graphical Abstract

Lonization of argon atom by positron and electron impact

使用一种名为 3CWZ 的理论模型研究了氩 3p 在 200 eV 冲击能量下的正电子和电子冲击电离。在该模型中,连续体的所有粒子都由带有可变电荷 Z(r) 的库仑波表示,碰撞后的相互作用和交换效应也包括在内。我们计算了三重差分截面,并将其与杜波依斯和德-卢西奥(Atoms 9:78, 2021)的最新测量结果以及其他理论(如果有的话)进行了比较。我们的数值结果与实验结果总体上吻合,并且比其他现有理论更好地说明了射弹的电荷效应。
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引用次数: 0
Correction: Gravitational force-induced changes in collisionless shock wave behavior in a charge-varying nonthermal dusty plasma 更正:电荷变化的非热尘埃等离子体中引力诱发的无碰撞冲击波行为变化
IF 1.5 4区 物理与天体物理 Q3 OPTICS Pub Date : 2024-11-20 DOI: 10.1140/epjd/s10053-024-00929-0
Ahmed Redha Benrekia, Rachid Fermous, Ziane Kechidi, Rabia Amour
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引用次数: 0
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The European Physical Journal D
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