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Cellulose Functional Gels: Physical Design and Promising Applications (Adv. Phys. Res. 6/2025) 纤维素功能凝胶:物理设计和前景应用(物理学报)。研究》6/2025)
IF 2.8 Pub Date : 2025-06-12 DOI: 10.1002/apxr.202570014
Minxin Wang, Geyuan Jiang, Xiaoyu Guo, Suqing Zeng, Dawei Zhao

Emerging Cellulose Ionogels

Through the physical construction of molecular network structures, soft gel materials derived from biomass cellulose can acquire a range of distinctive properties and be used in high-value applications. Article number 2500020 by Xiaoyu Guo, Suqing Zeng, Dawei Zhao and co-workers explores the design of functional gels through molecular-scale physical enhancement methods, thereby broadening the potential applications of cellulose gels in emerging flexible electronics. The integration of attractive physical processing techniques with molecular-scale design represents a promising research avenue for cellulose gels. This study provides valuable insights for the future development of smart gels and wearable devices.

新兴的纤维素离子凝胶通过分子网络结构的物理构建,来源于生物质纤维素的软凝胶材料可以获得一系列独特的性能,并具有高价值的应用。文章编号2500020郭晓宇、曾素清、赵大伟等人通过分子尺度物理增强方法探索功能凝胶的设计,从而拓宽了纤维素凝胶在新兴柔性电子产品中的潜在应用。有吸引力的物理加工技术与分子尺度设计的结合代表了纤维素凝胶的一个有前途的研究途径。该研究为智能凝胶和可穿戴设备的未来发展提供了有价值的见解。
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引用次数: 0
Sloppiness Consistency in Biomechanical Models and Its Inspired Dual-Space Model Optimization (Adv. Phys. Res. 6/2025) 生物力学模型的马虎一致性及其启发的双空间模型优化(物理学报)。研究》6/2025)
IF 2.8 Pub Date : 2025-06-12 DOI: 10.1002/apxr.202570016
Jiabao Tang, Wenyang Liu, Yiqi Mao, Shujuan Hou

Sloppiness Consistency Drives Balance in Mechanical Modeling

The study by Wenyang Liu, Shujuan Hou and co-workers (see article number 2500002) introduces an information-geometry-based approach for simplifying biomechanical constitutive models. By analyzing parameter sensitivity matrices, it reveals the inherent “sloppiness” of soft tissue models and constructs a parameter hyperspace with a four-step optimization strategy to reduce model complexity while maintaining identifiability and predictive accuracy, as successfully demonstrated in brain tissue and patellar tendon models.

刘文阳、侯淑娟及其同事(见文章编号2500002)的研究介绍了一种基于信息几何的方法来简化生物力学本构模型。通过分析参数敏感性矩阵,揭示软组织模型固有的“马虎性”,并采用四步优化策略构建参数超空间,以降低模型复杂性,同时保持模型的可识别性和预测准确性,这在脑组织和髌骨肌腱模型中得到了成功证明。
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引用次数: 0
Issue Information (Adv. Phys. Res. 5/2025) 发行信息(物理广告)研究》5/2025)
IF 2.8 Pub Date : 2025-06-12 DOI: 10.1002/apxr.202570015
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引用次数: 0
Resolving Localized Plasmonic and Photonic Modes of Gold Nanosponges via Cathodoluminescence Spectroscopy 利用阴极发光光谱技术分辨金纳米海绵的局部等离子体和光子模式
IF 2.8 Pub Date : 2025-06-12 DOI: 10.1002/apxr.202500049
Paul H. Bittorf, Masoud Taleb, Dong Wang, Peter Schaaf, Nahid Talebi

Localizing optical fields at deep sub-wavelength scales has applications in ultra-strong light-matter interactions and in efficient coupling to quantum emitters. Surface plasmon polaritons can be confined within and on the surfaces of nanostructures on spatial scales of only a few nanometers. However, they generally suffer from significant dissipation. Porous gold nanosponges and percolated thin films demonstrate an interestingly highly-localized plasmonic feature with an enhancement factor and quality factor beyond what is achievable with localized plasmons in nanostructures. Here, the characteristics of plasmon resonances in porous gold nanoparticles are explored using cathodoluminescence spectroscopy. It is demonstrated that visible light can be localized inside the nanosponges at spatial scales as small as 20 nm, forming dipole-like resonances. Moreover, it is shown that at specific wavelengths the entire structure supports a collective resonance, with the emitted light exhibiting polarization that represents an average over all possible dipolar emission directions. The analysis demonstrates the potential of gold nanosponges for exploring the intricate physics of localized resonances and their collective responses, and it paves the way toward their applications in controlling emissions from quantum emitters.

深亚波长尺度的局部光场定位在超强光-物质相互作用和量子发射体的有效耦合中具有应用价值。表面等离激元极化子可以被限制在纳米结构的内部和表面上,空间尺度只有几纳米。然而,它们通常会遭受严重的耗散。多孔金纳米海绵和渗透薄膜显示出一种有趣的高度定域等离子体特征,其增强因子和质量因子超出了纳米结构中定域等离子体所能达到的。本文利用阴极发光光谱技术研究了多孔金纳米粒子的等离子体共振特性。结果表明,可见光可以在小至20 nm的空间尺度上定位在纳米海绵内部,形成偶极子共振。此外,研究表明,在特定波长下,整个结构支持集体共振,发射的光表现出极化,代表了所有可能的偶极发射方向的平均值。该分析证明了金纳米海绵在探索局部共振及其集体反应的复杂物理方面的潜力,并为其在控制量子发射器发射方面的应用铺平了道路。
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引用次数: 0
Electrical Conductivity in Fibrous Composites 纤维复合材料的导电性
IF 2.8 Pub Date : 2025-06-12 DOI: 10.1002/apxr.202500040
Luke Hunter, Sergio Bertazzo

Carbon fiber and other fibrous composites are widely used in structural components for wind turbines and aircraft. These applications not only require high strength and low weight but also tailored electrical properties. Designing new composites that can resist lightning strikes or be used in bioelectronics relies on accurately predicting their electrical conductivities. Yet most models of conductivity in these composites lack a geometrically meaningful basis, particularly if applied far from the percolation threshold which often occurs in the earliest 1% of the composite design space. An electrical model that is grounded in real fiber geometries and arrangements is derived. New equations are obtained, combining materials science and network physics, that accurately predict individual fiber overlap, neighbor distributions, and percolation thresholds in systems of overlapping shapes. Combining these equations with the new electrical model of a “foamy cluster”, yielded excellent predictions of conductivity in many different types of fibrous composites.

碳纤维和其他纤维复合材料广泛用于风力涡轮机和飞机的结构部件。这些应用不仅需要高强度和低重量,而且需要定制的电气性能。设计能够抵抗雷击或用于生物电子学的新型复合材料依赖于准确预测其电导率。然而,这些复合材料的大多数电导率模型缺乏几何上有意义的基础,特别是在远离渗透阈值的情况下,渗透阈值通常发生在复合材料设计空间的前1%。推导了基于真实纤维几何形状和排列的电模型。结合材料科学和网络物理,获得了新的方程,可以准确预测重叠形状系统中的单个纤维重叠,邻居分布和渗透阈值。将这些方程与“泡沫簇”的新电模型相结合,得出了许多不同类型纤维复合材料的导电性的极好预测。
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引用次数: 0
Enhancing Signal Purity in Josephson Structure Measurements 提高约瑟夫森结构测量信号纯度
IF 2.8 Pub Date : 2025-06-09 DOI: 10.1002/apxr.202500032
Ivan A. Nazhestkin, Georgy I. Gubochkin, Jonathan Shvartzberg, Sai-Prasad M. Rajam, Sergei V. Egorov, Vladimir L. Gurtovoi, Valery V. Ryazanov, Vasily S. Stolyarov, Dmitry S. Yakovlev

Superconducting Josephson structures play a significant role in quantum-state engineering. Achieving high-fidelity quantum state measurements in superconducting Josephson structures requires ultra-low noise environments and robust signal purification techniques. Here, the advanced low-noise signal measurement system designed for dilution refrigerators is presented, integrating multi-stage cryogenic filtering and electromagnetic shielding strategies to suppress noise sources across a broad frequency spectrum. The effectiveness of low-pass RC filters is demonstrated, silver-epoxy microwave absorbers, and optimized ground isolation to achieve an unprecedented noise reduction, enabling sub-nanoampere switching current distribution measurements superior to commerical systems at mK temperatures. The system is optimized for precision studies of superconductor-insulator-superconductor, superconductor-ferromagnet-superconductor, and superconductor-normal metal-superconductor Josephson junctions with low critical currents. This approach establishes a reliable framework for next-generation quantum electronic experiments, ensuring that observed switching phenomena are governed by intrinsic device physics rather than environmental perturbations.

超导约瑟夫森结构在量子态工程中起着重要的作用。在超导约瑟夫森结构中实现高保真量子态测量需要超低噪声环境和稳健的信号净化技术。本文介绍了一种先进的用于稀释冰箱的低噪声信号测量系统,该系统集成了多级低温滤波和电磁屏蔽策略,可以在宽频谱范围内抑制噪声源。低通RC滤波器、银环氧树脂微波吸收器和优化的接地隔离的有效性得到了证明,从而实现了前所未有的降噪效果,使亚纳安培开关电流分布测量优于mK温度下的商业系统。该系统是优化的精密研究超导体-绝缘体-超导体,超导体-铁磁-超导体,超导体-正常金属-超导体约瑟夫森结与低临界电流。这种方法为下一代量子电子实验建立了一个可靠的框架,确保观察到的开关现象是由内在器件物理而不是环境扰动控制的。
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引用次数: 0
Special Issue Editorial: Quantum Anomalies in Condensed Matter 特刊社论:凝聚态物质中的量子异常
IF 2.8 Pub Date : 2025-06-03 DOI: 10.1002/apxr.202500056
Michael T. Pettes, Avadh Saxena
<p>A symmetry that exists in the classical regime but is broken in the quantum realm may create what field theorists refer to as a quantum anomaly. Three of these symmetries in classical field theory that are broken in the quantum regime offer significant potential for enabling new technologies in the condensed matter context: the scale (conformal) anomaly, axial (chiral) anomaly, and parity anomaly. For example, the chiral anomaly in Weyl semimetals manifests as unusual magneto-transport phenomena, such as negative longitudinal magnetoresistance. Similarly, the parity anomaly can induce a half-quantized Hall effect, and the scale anomaly is predicted to generate anomalous thermoelectric currents. Observing these effects in topological materials not only tests quantum field theory in a laboratory setting but also advances our understanding of symmetry breaking in novel quantum phases. This paradigm is gaining ground in both theory and experiments on new topological materials which are allowing the research community to begin to realize their signatures in condensed matter as depicted in the Venn diagram of <b>Figure</b> 1. Although we emphasize that experimental evidence in solids remains scarce, this interdisciplinary field is opening a new frontier in physics research with promise for a unique set of new potential device applications. Technologies enabled by quantum anomalies include ultra-sensitive micro-bolometric detectors, dark matter detectors, far infrared optical modulators, low-dissipation ballistic transporters, terahertz-based qubits, terahertz polarization state controls, passive magnetic field sensors, stable topological superconductors that host Majorana fermions (i.e., topological quantum computing), and qubits topologically protected against decoherence among possibly others. This has been expressed in a simple language accessible to materials scientists and physicists alike in a perspective article (202400189, https://doi.org/10.1002/apxr.202400189), which describes how each anomaly's measurable non-conserved current offers a window into quantum symmetry breaking in condensed matter, particularly topological quantum materials.</p><p>This special issue brings together an additional five technical articles that illustrate these concepts in various condensed matter systems. First, the theoretical basis is described in two articles. Maxim Chernodub et al. (202300058, https://doi.org/10.1002/apxr.202300058) report on how the scale (conformal) anomaly can produce electric currents at the boundaries of materials exposed to static magnetic fields, using scalar quantum electrodynamics simulations. The authors reveal significant differences between quantum anomaly-driven currents and classical Meissner currents, suggesting measurable effects in Dirac semimetals, and providing insights into anomaly-induced phenomena with potential applications in quantum electronics and anomaly-based sensors. The paper by Claudio Coriano et al. (202400043,
存在于经典体系中的对称性在量子领域被打破,可能会产生场理论家所说的量子异常。经典场论中的三种对称性在量子体系中被打破,为凝聚态环境中的新技术提供了巨大的潜力:尺度(共形)异常、轴向(手性)异常和宇称异常。例如,Weyl半金属中的手性异常表现为不寻常的磁输运现象,如负纵向磁电阻。同样,宇称异常可以诱导半量子化霍尔效应,尺度异常可以预测产生异常热电电流。在拓扑材料中观察这些效应不仅在实验室环境中验证了量子场理论,而且还促进了我们对新量子相对称性破缺的理解。这种范式在新拓扑材料的理论和实验中都取得了进展,这使得研究团体开始在图1的维恩图中所示的凝聚态物质中实现它们的特征。尽管我们强调固体的实验证据仍然很少,但这个跨学科领域正在开辟物理学研究的新前沿,并有望为一系列独特的新潜在设备应用提供前景。由量子异常实现的技术包括超灵敏微辐射探测器、暗物质探测器、远红外光调制器、低耗散弹道传输器、基于太赫兹的量子比特、太赫兹偏振状态控制、被动磁场传感器、承载马约拉纳费米子的稳定拓扑超导体(即拓扑量子计算),以及在拓扑上防止退相干的量子比特等。在一篇透视文章(202400189,https://doi.org/10.1002/apxr.202400189)中,材料科学家和物理学家都可以用一种简单的语言来表达这一点,该文章描述了每种异常的可测量非守恒电流如何为凝聚态物质,特别是拓扑量子材料中的量子对称性破断提供了一个窗口。这个特刊汇集了另外五篇技术文章,在各种凝聚态系统中说明了这些概念。首先,分两篇文章阐述了理论基础。Maxim Chernodub等人(202300058,https://doi.org/10.1002/apxr.202300058)利用标量量子电动力学模拟,报告了尺度(共形)异常如何在暴露于静态磁场的材料边界产生电流。作者揭示了量子异常驱动电流与经典迈斯纳电流之间的显着差异,表明在狄拉克半金属中可测量的效应,并提供了在量子电子学和基于异常的传感器中潜在应用的异常诱导现象的见解。Claudio Coriano等人的论文(202400043,https://doi.org/10.1002/apxr.202400043)在4D时空共形场论(CFTs)中连接了手性异常驱动的相互作用。作者研究了如何在CFT框架内描述由热梯度驱动的引力手性异常,强调了异常极的作用及其相关的非局部作用,进一步强调了通过异常振幅和可测量的法拉第效应推导出的求和规则来探测类轴子准粒子的潜力,从而将基础量子场理论与实验凝聚态物理联系起来。接下来,在两篇文章中描述了晶格电子结构计算在拓扑材料(包括狄拉克半金属和拓扑近藤绝缘体)缺陷中的作用。Elizabeth Peterson等人(202300111,https://doi.org/10.1002/apxr.202300111)在其期刊封面文章中报道了碲空位如何利用第一性原理密度泛函理论(DFT)影响Dirac材料HfTe5和ZrTe5的电子结构和异常输运性质。作者表明,Te空位通过改变费米能以下的传导带,引入电子和空穴载流子,从而使负纵向磁阻(NLMR)的相互矛盾的实验观察结果合理化,从而显著影响电子行为。作者证明了这些空位对观察到的输运现象有很大的影响,但重要的是不排除潜在的真正的量子异常的表现,如在含有这些缺陷的材料中的手性异常。Jian-Xin Zhu等人(202500003,https://doi.org/10.1002/apxr.202500003)描述了TKIs的局部电子结构,以及单一杂质如何影响不同拓扑状态下的表面状态。作者揭示了拥有单个狄拉克锥的强tki在单一散射下抑制杂质诱导的共振态,显示出拓扑保护。 相反,具有两个狄拉克锥的弱tki即使在酉极限下也支持鲁棒杂质束缚态。重要的是,作者提出了一种通过扫描隧道显微镜实验区分TKI相的新途径,为强相关系统的拓扑保护提供了更深入的了解。最后一篇文章说明了对实验签名的初步尝试,这些实验签名可能通过在新的拓扑材料中表达自己的异常而实现。Jin Hu等人(202300145,https://doi.org/10.1002/apxr.202300145)报道了他们对中心对称层状化合物Mn2-xZnxSb的拓扑霍尔效应(the)的观察,揭示了一个惊人的成分依赖行为。利用霍尔效应和磁光克尔效应测量,作者证明了高zn样品(x &gt;0.6)表示THE在低温下增强,而低锌样品则表现出相反的趋势,随着温度的升高THE逐渐增大。这种二分法归因于两种体制之间不同的自旋织构和磁畴结构,表明尽管有中心对称晶格,但手性磁有序。研究结果表明,Mn₂xxznxsb是一个平台,在这个平台上,与拓扑异常相关的不同磁机制可以通过化学取代来调节。在凝聚态物质中实现量子异常的任何一种潜在技术都将成为下一代应用的突破,例如精确量子传感和探测。与此同时,实现这一技术潜力将需要克服理论和实验方面的重大障碍。研究人员必须从琐碎的能带贡献中分离出真正的拓扑信号,稳定产生量子反常霍尔效应等现象的精细手性自旋织构,并设计出在背景噪声中可靠测量微小反常电流的技术。这种平衡的乐观主义强调了该领域的前瞻性愿景,即随着材料设计和测量的不断创新,量子异常可能会从有趣的实验室好奇心发展到材料科学变革性设备的基础。作者声明无利益冲突。
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引用次数: 0
Integrating First Principles Calculations and Machine Learning to Study the ReNiO2/Ti3C2 Heterojunctions for Sodium Ion Batteries 结合第一性原理计算和机器学习研究钠离子电池ReNiO2/Ti3C2异质结
IF 2.8 Pub Date : 2025-06-03 DOI: 10.1002/apxr.202500052
Yuanyuan Cui, Chengyu Zhang, Luxin Niu, Jiao Zheng, Xin Liu, Sihan Yang, Yanfeng Gao

Due to the large size of sodium ions and their slow redox kinetics in electrochemical processes, the sodium ion batteries currently are still far from satisfactory. This study investigates the electrical transport properties of ReNiO2/ Ti3C2 heterojunctions in sodium ion batteries through a combination of first principles calculations and machine learning analysis. The ReNiO2/Ti3C2 heterojunctions exhibit metallic characteristics and enhanced electronic conductivity due to the hybridization of p-d orbitals and the strengthening of Ni─Ti metal bonds. The sodium ion migration energy barrier decreases with increasing rare earth atomic number, facilitating ion transport. Machine learning analysis identifies key factors influencing ion and electron transport rates, including strain, lattice constants, and doping concentration. These findings provide theoretical guidance for designing more efficient negative electrodes for sodium ion batteries.

由于钠离子体积大,电化学过程中氧化还原动力学慢,目前钠离子电池的性能还远远不能令人满意。本研究通过第一性原理计算和机器学习分析相结合的方法研究了钠离子电池中ReNiO2/ Ti3C2异质结的电输运性质。由于p-d轨道的杂化和Ni - Ti金属键的强化,ReNiO2/Ti3C2异质结表现出金属特性和电子导电性的增强。随着稀土原子序数的增加,钠离子迁移能垒降低,有利于离子迁移。机器学习分析确定影响离子和电子传输速率的关键因素,包括应变、晶格常数和掺杂浓度。这些发现为设计更高效的钠离子电池负极提供了理论指导。
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引用次数: 0
Quantum Anomalies in Condensed Matter 凝聚态物质中的量子异常
IF 2.8 Pub Date : 2025-05-27 DOI: 10.1002/apxr.202400189
Michael T. Pettes, Shi-Zeng Lin, Elizabeth A. Peterson, Jian-Xin Zhu, Laurel E. Winter, Johanna C. Palmstrom, Jinkyoung Yoo, Nicholas S. Sirica, Prashant Padmanabhan, Priscila F. S. Rosa, Sean M. Thomas, Avadh Saxena

Quantum materials provide a fertile ground in which to test and realize unusual phenomena such as quantum anomalies predicted by quantum field theory. There are three important symmetries that are broken when classical field theory is moved into the quantum regime, the scale anomaly, the axial (chiral) anomaly, and the parity anomaly. Several potential device applications may be realized by the discovery of quantum anomalies in condensed matter, enabled by the new physics they embody, including ultra-sensitive dark matter detectors, far infrared optical modulators, micro-bolometric detectors, low-dissipation ballistic transporters, terahertz-based qubits, terahertz polarization state controls, passive magnetic field sensors, stable topological superconductors that host Majorana fermions, and qubits topologically protected against decoherence. In this perspective article, the definition of these quantum anomalies is laid out, how little is known in the context of condensed matter, and how quantum anomalies are predicted to manifest as anomalous electronic, thermal, and magnetic behavior in experiments on topological quantum materials, including Weyl and Dirac semimetals. Furthermore, the importance that mechanical strain and defects will play in modifying signatures of quantum anomalies is discussed.

量子材料为测试和实现量子场理论预测的量子异常等不寻常现象提供了肥沃的土壤。当经典场论进入量子态时,有三种重要的对称性被打破,即尺度异常、轴向(手性)异常和宇称异常。一些潜在的器件应用可能通过凝聚态物质中量子异常的发现而实现,包括超灵敏暗物质探测器、远红外光调制器、微辐射探测器、低耗散弹道传输体、基于太赫兹的量子比特、太赫兹偏振状态控制、被动磁场传感器、承载马约拉纳费米子的稳定拓扑超导体、量子比特在拓扑结构上防止退相干。在这篇观点文章中,这些量子异常的定义被列出,在凝聚态物质的背景下所知的是多么少,以及如何预测量子异常在拓扑量子材料(包括Weyl和Dirac半金属)的实验中表现为异常的电子、热和磁性行为。此外,还讨论了机械应变和缺陷对修正量子异常特征的重要性。
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引用次数: 0
GaAs Growth on Ge-Buffered Discontinuous (111)-Faceted V-Groove Silicon Substrates 锗缓冲不连续(111)面v型槽硅衬底上的砷化镓生长
IF 2.8 Pub Date : 2025-05-19 DOI: 10.1002/apxr.202500026
Makhayeni Mtunzi, Hui Jia, Mateus G. Masteghin, Yaonan Hou, Haotian Zeng, Huiwen Deng, Jae-Seong Park, Chong Chen, Jun Li, Xingzhao Yan, Ilias Skandalos, Frederic Gardes, Mingchu Tang, Alwyn Seeds, Huiyun Liu

The propagation of antiphase boundaries (APBs) and threading dislocations (TDs) poses a significant impediment to the realisation of high-quality group III–V semiconductors grown on group IV platforms. The complete annihilation of APBs and a substantial reduction in threading dislocation density (TDD) are essential for achieving high-efficiency III–V devices compatible with complementary metal-oxide semiconductor (CMOS) technology. In this study, a novel growth technique is proposed and developed to fabricate a faceted germanium (Ge) buffer on a discontinuous (111)-faceted V-groove silicon (Si) substrate with a 500 nm flat ridge width. Subsequently, a GaAs buffer is grown on the Ge/V-groove Si virtual substrate using a ramped temperature growth process to minimise the prevalence of line and planar defects in the buffer structure. An APB-free GaAs buffer is successfully achieved, as confirmed by cross-sectional and plan-view transmission electron microscopy (TEM) and atomic force microscopy (AFM) analyses. The faceted Ge buffer layer obtained through this innovative approach alleviates the stringent fabrication requirements and intricate processing typically associated with conventional continuous V-groove Si substrates. This advancement facilitates the development of photonic integrated circuits by providing a simplified and efficient alternative substrate solution.

反相边界(apb)和螺纹位错(td)的传播是在IV族平台上实现高质量III-V族半导体的重要障碍。apb的完全湮灭和螺纹位错密度(TDD)的大幅降低是实现与互补金属氧化物半导体(CMOS)技术兼容的高效率III-V器件的必要条件。在这项研究中,提出并开发了一种新的生长技术,用于在具有500 nm平脊宽度的不连续(111)面v槽硅(Si)衬底上制造面锗(Ge)缓冲材料。随后,在Ge/ v槽Si虚拟衬底上使用升温生长过程生长GaAs缓冲器,以最大限度地减少缓冲结构中线和面缺陷的流行。通过横断面、平面透射电镜(TEM)和原子力显微镜(AFM)分析证实,成功制备了不含apb的GaAs缓冲液。通过这种创新方法获得的多面Ge缓冲层减轻了传统连续v槽Si衬底的严格制造要求和复杂的加工过程。这一进步通过提供一种简化和高效的替代衬底解决方案,促进了光子集成电路的发展。
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Advanced Physics Research
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