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Health risk assessment of Cu, As, Cd and Pb in the broiler breast in Shenyang, China 沈阳地区肉鸡乳房铜、砷、镉、铅健康风险评价
Pub Date : 2022-07-20 DOI: 10.1080/10807039.2022.2101430
Boyuan Guan, Xiakouna Amantai, Yuxia Chai, Xinping Chen, X. Yue, Xueli Yu
Abstract In this cross-sectional study, inductively coupled plasma mass spectrometry (ICP-MS) was used to determine the levels of Cu, Pb, Cd, and As in 55 chicken breast samples collected in Shenyang, China. The estimated daily intake (EDI), target hazard quotient (THQ), total hazard index (HI), and target cancer risk (TCR) were calculated to evaluate potential health risks from broiler breast consumption in different age groups. Heavy metal concentration in broiler breast samples was below the maximum residue limit (MRL) set by national and international regulations. Principal component analysis (PCA) results were similar to those of the hierarchical cluster analysis (HCA), mutually validating the two distinct groups of Pb-Cd-As and Cu, which indicated that there were similar sources for Pb, Cd and As but differ from that of Cu. EDI values for these metals in broiler breasts were far below the corresponding provisional tolerable daily intake values. THQ and HI were well below 1, indicating that there were no non-carcinogenic health risks for residents. The TCR from Pb was negligible in different age groups and the TCR of children exposed to As and Cd were acceptable. However, due to the non-degradability and bioaccumulation of metals, it is recommended that children, especially female children, should be the focus of future long-term surveillance when assessing the carcinogenicity of these metals.
摘要采用电感耦合等离子体质谱法(ICP-MS)测定了沈阳55份鸡胸肉样品中Cu、Pb、Cd和As的含量。计算估计日摄入量(EDI)、目标危害商(THQ)、总危害指数(HI)和目标癌症风险(TCR),评价不同年龄组肉鸡食用乳房的潜在健康风险。肉鸡胸肉样品中重金属含量低于国家和国际规定的最大残留限量。主成分分析(PCA)结果与层次聚类分析(HCA)结果相似,相互验证了Pb-Cd-As和Cu两组不同的来源,表明Pb、Cd和As的来源相似,但与Cu的来源不同。肉鸡胸脯中这些金属的EDI值远低于相应的临时每日耐受摄入量。THQ和HI均远低于1,表明居民不存在非致癌性健康风险。铅的TCR在不同年龄组中可以忽略不计,暴露于砷和镉的儿童的TCR是可以接受的。然而,由于金属的不可降解性和生物蓄积性,建议在评估这些金属的致癌性时,儿童,特别是女童应成为未来长期监测的重点。
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引用次数: 1
Variations of fungal communities in lead–zinc tailings located in Northwestern China 西北地区铅锌尾矿中真菌群落的变化
Pub Date : 2022-07-19 DOI: 10.1080/10807039.2022.2098466
Yuanyuan Shen, Haijuan Li, Yuan Liu, Tianpeng Gao, Guangwen Li, M. Zuo, Jing Ji, Changming Li, Xiangkai Li, Yueli Chen, Z. Yin, Jing Li, Wenli Zhang
Abstract Investigation of microbial community structures is critical for situ-remediation of heavy metal contaminated soils. For this purpose, we used high-throughput 18S rRNA sequencing method to analyze soil fungal communities in the Shanping village (SPC) and Yanzibian (YZB) tailings situated in northwestern China. The relationships of the fungal community and the environmental factors, including heavy metals and soil chemical properties were analyzed. The results showed that the fungal community richness and diversity in the soils were both trending as control soil > contaminated soil. The compositions and relative abundances of the fungal populations in the two tailings were different, however the dominant fungal phyla of which were almost the same, mainly including Ascomycota, Basidiomycota, Calcarisporillomycota, Mortierellomycota, and Rozellomycota. Further, the Canonical correlation analysis and spearman correlation analyses revealed that Cd, Pb, Cu, Zn, Cr, TP, NO3 −-N, TN, and/or pH were predominantly positive correlation factors for the most abundant fungal phyla Ascomycota and Basidiomycota. Together, we have sorted out certain fungal species, such as s_unclassified_p_Ascomycota, s_unclassified_c_Sordariomycetes, s_Talaromyces_solicola, and s_Cutaneotrichosporon_curvatus, which are probably tolerant to heavy metals in these specific tailing soils. Overall, our results have provided an initial perspective of the fugal community variations of these specific tailing ponds.
微生物群落结构的研究是重金属污染土壤现状修复的关键。为此,我们采用高通量18S rRNA测序方法对中国西北山坪村(SPC)和燕子边(YZB)尾矿的土壤真菌群落进行了分析。分析了真菌群落与重金属、土壤化学性质等环境因子的关系。结果表明:土壤真菌群落丰富度和多样性均呈对照土>污染土的趋势;两种尾矿中真菌种群的组成和相对丰度不同,但优势真菌门基本相同,主要包括子囊菌门、担子菌门、钙孢菌门、Mortierellomycota和Rozellomycota。典型相关分析和spearman相关分析表明,Cd、Pb、Cu、Zn、Cr、TP、NO3−-N、TN和/或pH是子囊菌门和担子菌门数量最多的正相关因子。我们一起整理出了一些真菌种类,如s_unclassified_p_Ascomycota、s_unclassified_c_Sordariomycetes、s_Talaromyces_solicola和s_Cutaneotrichosporon_curvatus,它们可能对这些特定的尾矿土壤中的重金属具有耐受能力。总的来说,我们的研究结果为这些特定尾矿库的真菌群落变化提供了初步的视角。
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引用次数: 1
Comparison of adsorption behavior of Pb(II) by acid–alkali and chitosan modified biochar derived from kiwifruit branch 酸碱改性和壳聚糖改性猕猴桃枝生物炭对铅(II)的吸附性能比较
Pub Date : 2022-07-15 DOI: 10.1080/10807039.2022.2098467
Ling Jiang, Xiu Yi, Kejian Yang, Mengfan Li, Huihui Rao, Xinxin Wu, Ya-xin Li, Chaoqun Gao
Abstract In this work, the kiwifruit branch, a kind of agricultural waste, was reused as a raw material to prepare biochar adsorbent for the removal of Pb(II) from aqueous solution. Then pristine biochar (BC) was further modified to form acid–alkali modified biochar (OBC) and chitosan modified biochar (CBC) to enhance adsorption efficiency toward Pb(II). Characterization experiments with SEM, FTIR and XRD suggested that surface functional groups and crystallization degree of OBC and CBC were all increased in comparison with BC. Batch sorption experiments showed that, compared with BC, the adsorption capacity of Pb(II) by OBC and CBC were improved by 19.57 and 8.37%, respectively. The pseudo-second-order model and the Freundlich model were better for describing the kinetics and isotherms for Pb(II) adsorption onto OBC and CBC, respectively. Accordingly, chemisorption on the heterogeneous adsorption surface played a dominant role in Pb(II) removal.
摘要以农业废弃物猕猴桃枝为原料,制备生物炭吸附剂,用于去除水中的铅(II)。然后对原始生物炭(BC)进行进一步改性,形成酸碱改性生物炭(OBC)和壳聚糖改性生物炭(CBC),以提高对Pb(II)的吸附效率。SEM、FTIR和XRD表征实验表明,与BC相比,OBC和CBC的表面官能团和结晶程度均有所提高。批量吸附实验表明,与BC相比,OBC和CBC对Pb(II)的吸附量分别提高了19.57%和8.37%。拟二阶模型和Freundlich模型分别较好地描述了铅(II)在OBC和CBC上的吸附动力学和等温线。因此,非均相吸附表面的化学吸附对Pb(II)的去除起主导作用。
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引用次数: 2
Implications of toxicity testing for health risk assessment of vapor-phase and PM2.5-bound polycyclic aromatic hydrocarbons during the diesel engine combustion 柴油发动机燃烧过程中气相和pm2.5结合的多环芳烃毒性测试对健康风险评估的影响
Pub Date : 2022-07-14 DOI: 10.1080/10807039.2022.2098465
Guan-Fu Chen, Ying-Chi Lin, Yu Lin, Chia-Chi Wang, Wei-Hsiang Chen
Abstract It is challenging to estimate the health risks posed by exposure to particulate pollutants due to limited information for chemicals bound to particles in toxicity databases. This study predicted the cancer risks posed by the vapor-phase and fine particulate matter (PM2.5)-bound polycyclic aromatic hydrocarbon (PAH) emissions during diesel combustion in an industrialized city in southern Taiwan by using two different approaches. In the first approach, the cancer risks were estimated based on the vapor-phase and PM2.5-bound PAH concentrations in the exhausts, while the observations of the vapor-phase and PM2.5-bound samples in the in vitro cell toxicity tests, including Ames test, 3-(4,5-dimethylthiazol-2-yl)-2,5-diphenyltetrazolium bromide (MTT) assay, and tumor necrosis factor-alpha (TNF-alpha) detection were employed to modify the risks posed by the PM2.5-bound emission in the second approach. The results show that the vapor-phase concentrations of total PAH (30,944-118,565 ng/m3) and benzo(a)pyrene toxic equivalence quotient (BaP-TEQ; 8.2–69.1 ng/m3) were significantly higher than the PM2.5-bound concentrations (the total concentration and BaP-TEQ were 11.9–45.0 and 0.27–12.94 ng/m3, respectively), resulting in the dominance of the vapor-phase risk (71–98%) over the total risk (8.92 × 10−9–1.03 × 10−7). With the modification of the cell test results, the total risks were increased to 1.62 × 10−8–1.33 × 10−7. The ratios of the PM2.5-bound risk to the total risk in different conditions have been increased by 2–26 times (from 2–29% to 45–61%), suggesting the mixture effect of PM-bound pollutants on health risk assessment.
由于毒性数据库中与颗粒结合的化学物质的信息有限,估计暴露于颗粒污染物所造成的健康风险具有挑战性。本研究采用两种不同的方法预测台湾南部某工业化城市柴油燃烧过程中蒸汽相和细颗粒物(PM2.5)结合的多环芳烃(PAH)排放所造成的癌症风险。在第一种方法中,根据废气中气相和pm2.5结合的多环芳烃浓度估计癌症风险,而在体外细胞毒性试验中,包括Ames试验、3-(4,5-二甲基噻唑-2-基)-2,5-二苯基溴化四唑(MTT)试验和肿瘤坏死因子- α (tnf - α)检测,采用气相和pm2.5结合样品的观察结果来修改第二种方法中pm2.5结合排放带来的风险。结果表明:总多环芳烃气相浓度(30,944 ~ 118,565 ng/m3)和苯并(a)芘毒性等效商(BaP-TEQ;8.2 ~ 69.1 ng/m3)显著高于pm2.5结合浓度(总浓度11.9 ~ 45.0和BaP-TEQ分别为0.27 ~ 12.94 ng/m3),导致气相风险(71 ~ 98%)高于总风险(8.92 × 10−9 ~ 1.03 × 10−7)。随着细胞检测结果的修改,总风险增加到1.62 × 10−8-1.33 × 10−7。在不同条件下,pm2.5结合风险占总风险的比例增加了2-26倍(从2-29%增加到45-61%),表明pm结合污染物对健康风险评估的混合效应。
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引用次数: 0
Significant effect of COVID-19 induced lockdown on air quality of the Indian Metropolitan City Kolkata using Air Quality Index and Health Air Quality Index 使用空气质量指数和健康空气质量指数分析新冠肺炎引发的封锁对印度大都市加尔各答空气质量的显著影响
Pub Date : 2022-07-11 DOI: 10.1080/10807039.2022.2093155
Syed Yakub Ali, Pallavi Mukherjee, Sangeeta Sunar, S. Saha, Priti Saha, Suvankar Dutta, S. Goswami
Abstract The lockdown, commencing in India from March 23, 2020 to control the escalation of Covid-19 cases, exhibited a positive impact on the air quality. The study attempts to assess the outcome of lockdown on the air quality of Kolkata, India followed by the comparison of six priority pollutants during pre-lockdown, lockdown, and unlock phases. Averaged concentrations of PM10 (72%), PM2.5 (73%), NOx (84%), SO2 (48%), and CO (61%) showed reduction throughout lockdown in comparison with pre-lockdown phase, although no significant reduction was observed in ground-level Ozone. Unlock Phases I and II showed similar concentrations of the pollutants as that in the lockdown period whereas, in unlock Phase-III, the air quality became comparable to that before lockdown. Statistical analysis confirmed that the reduction in air pollution is attributed to atmospheric factors. PCA analysis established significant positive correlation between particulate matters, CO, SO2, and NO x ; however, no significant correlation was observed between NO x and O3. January and December showed the highest load of most of the pollutants. Health risk was evaluated by calculating the Relative risk and Health Air Quality Index, which showed maximum health risk during the pre-lockdown and minimum during lockdown and unlock Phase-II with the highest contributor being PM10. The study outcome manifests a reduction in environmental pollution as a result of controlled anthropogenic activities.
为控制新冠肺炎疫情升级,印度从2020年3月23日开始实施封锁措施,对空气质量产生了积极影响。该研究试图评估封锁对印度加尔各答空气质量的影响,然后比较了封锁前、封锁和解锁阶段的六种优先污染物。与封城前相比,在封城期间,PM10(72%)、PM2.5(73%)、氮氧化物(84%)、二氧化硫(48%)和一氧化碳(61%)的平均浓度有所下降,但地面臭氧没有显著下降。“解锁”一、二期污染物浓度与封城前基本持平,“解锁”三期空气质量与封城前基本持平。统计分析证实,空气污染的减少归因于大气因素。PCA分析表明,颗粒物、CO、SO2与NO x呈显著正相关;而一氧化氮与一氧化氮之间无显著相关性。1月和12月是大多数污染物的最高负荷。通过计算相对风险和健康空气质量指数对健康风险进行了评估,结果表明,封城前的健康风险最大,封城解锁阶段的健康风险最小,PM10的贡献最大。研究结果表明,由于受控制的人为活动,环境污染有所减少。
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引用次数: 1
Association between urinary metal levels and slow vital capacity in Chinese preschoolers 中国学龄前儿童尿金属水平与肺活量缓慢的关系
Pub Date : 2022-07-03 DOI: 10.1080/10807039.2022.2084029
Yang Liu, Lili Yu, Hongxian Ji, Meiqin Zhu, Yanli Liu, Yechun Fu, Yaofang Zhang, Hongbo Li, Yanying Duan, Hongcheng Ding, J. Wang
Abstract Objectives Heavy metal exposure has been associated with lung function decline, but there is still a lack of evidence on preschoolers. In this study, we evaluated cross-sectional associations between urinary metal levels and slow vital capacity (SVC) in preschoolers. Methods A total of 1284 children were selected from seven-kindergartens. Urinary concentrations of 23 metals were measured by inductively coupled plasma mass spectrometry. Utilized least absolute shrinkage and selection operator penalized regression was used to select the metals independently associated with SVC. Generalized linear models were used to evaluate the association between urinary metals level and SVC. Result In the single-metal model, we observed negative associations between urinary aluminum, copper, zinc, rubidium, lead and SVC, comparing extreme quartiles the regression coefficients β (95% CI) were −41.01 (95% CI: −78.02, −4.01, P for trend = 0.029), −62.91 (95% CI: −99.85, −25.96, P for trend = 0.004), −33.48 (95% CI: −69.95, 3.00, P for trend = 0.042), −49.45 (95% CI: −86.10, −12.81, P for trend = 0.012) and −55.64 (95% CI: −91.88, −19.40, P for trend = 0.005), respectively. Urinary copper was negatively associated with SVC in boys, urinary zinc and lead were negatively associated with SVC in girls. Similar results were obtained in the multiple-metal model, the β for copper comparing extreme quartiles was −98.90 (-95% CI: −165.50, −32.29, P for trend = 0.006) in boys, the β for zinc and lead comparing extreme quartiles were −54.50 (95% CI: −107.60, −1.41, P for trend = 0.012), −84.32 (95% CI: −151.40, −17.24, P for trend = 0.016) in girls. Conclusions The levels of urinary aluminum, copper, zinc, rubidium, lead were negatively associated with SVC in preschoolers. These associations were different between boys and girls. Further prospective and experimental studies are warranted to clarify the underlying mechanisms.
目的重金属暴露与肺功能下降有关,但对学龄前儿童的影响尚缺乏证据。在这项研究中,我们评估了学龄前儿童尿金属水平与慢肺活量(SVC)之间的横断面关联。方法选取7所幼儿园1284名幼儿。用电感耦合等离子体质谱法测定了尿中23种金属的浓度。利用最小绝对收缩和选择算子惩罚回归来选择与SVC独立相关的金属。采用广义线性模型评价尿金属水平与SVC之间的关系。结果在单金属模型中,我们观察到尿铝、铜、锌、铷、铅和SVC之间存在负相关,比较极端四分位数,回归系数β (95% CI)分别为- 41.01 (95% CI: - 78.02, - 4.01, P为趋势= 0.029)、- 62.91 (95% CI: - 99.85, - 25.96, P为趋势= 0.004)、- 33.48 (95% CI: - 69.95, 3.00, P为趋势= 0.042)、- 49.45 (95% CI: - 86.10, - 12.81, P为趋势= 0.012)和- 55.64 (95% CI: - 91.88, - 19.40, P为趋势= 0.005)。尿铜与男孩SVC呈负相关,尿锌和铅与女孩SVC呈负相关。在多金属模型中也得到了类似的结果,男孩中铜的β比较极端四分位数为- 98.90 (-95% CI: - 165.50, - 32.29, P为趋势= 0.006),女孩中锌和铅的β比较极端四分位数为- 54.50 (95% CI: - 107.60, - 1.41, P为趋势= 0.012),- 84.32 (95% CI: - 151.40, - 17.24, P为趋势= 0.016)。结论学龄前儿童尿中铝、铜、锌、铷、铅水平与SVC呈负相关。这些联系在男孩和女孩之间是不同的。需要进一步的前瞻性和实验性研究来阐明潜在的机制。
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引用次数: 1
Evaluation of ecological security and ecological maintenance based on pressure-state-response (PSR) model, case study: Fuzhou city, China 基于压力-状态-响应(PSR)模型的生态安全与生态维持评价——以福州市为例
Pub Date : 2022-07-01 DOI: 10.1080/10807039.2022.2081835
Shuhui Lai, Jinming Sha, A. Eladawy, Xiaomei Li, Jinliang Wang, E. Kurbanov, Zejing Lin, Long Wu, Run Han, Yung-Chih Su
Abstract Since the modern industrial revolution, the speed of urbanization has accelerated, resulting in a series of ecological environment problems. Fujian province will begin to implement the policy of strengthening the provincial capital in October 2021. Therefore, it is crucial to analyze the ecological maintenance status of Fuzhou and provide a relevant reference for Fuzhou to be built into a national central city. This article takes Fuzhou city as the research area, collects land use data in 2000, 2010, and 2020 from Globeland30, combines remote sensing image data, statistical yearbook data, and Digital Elevation Model (DEM) data, and based on Pressure-State-Responses (PSR) model. A total of 15 indicators were selected to construct the ecological security evaluation system of Fuzhou in 2000, 2010, and 2020, and the weight of each indicator was determined by analytic hierarchy process. Spatial autocorrelation was used to analyze the correlation degree of the land use ecological security index in Fuzhou. The concept of ecological maintenance was introduced to analyze the status of ecological maintenance in Fuzhou during the third period. Finally, the diagnostic model of obstacle factors was used to determine the main obstacle factors affecting ecological security in Fuzhou. The results showed that from 2000 to 2020, the area of cultivated land, grassland and bare land decreased year by year, and transferred 320.63 km2, 25.34 km2 and 9.85 km2 to the artificial surface respectively. The high-value ecological security indexes in 2000, 2010 and 2020 were 27.54%, 28.67% and 30.93% respectively. Therefore, the overall level of ecological security in Fuzhou has improved, but there is a large gap in local ecological security. The area with moderate ecological maintenance degree accounted for 60.15%. From the perspective of the whole city, the very poor ecological maintenance degree mainly concentrated in the downtown area and Pingtan Island, while the very good ecological maintenance degree accounted for very little, mainly distributed in the northwest of Fuzhou. The ecological security index showed the characteristics of high and low-value agglomeration, and the distribution of four clusters in three periods was similar. The main obstacle factors of ecological security in three periods are highway density, population density, surface temperature, intensity of human interference, landscape diversity, GDP per capita, and regional development degree. The ecological security evaluation and ecological maintenance of Fuzhou city is beneficial to provide an efficient decision support tool for the ecological environment protection of Fuzhou City.
现代工业革命以来,城市化速度加快,导致了一系列生态环境问题。福建省将于2021年10月开始实施加强省会的政策。因此,分析福州的生态维护现状,为福州建设国家中心城市提供相关参考至关重要。本文以福州市为研究区,结合遥感影像数据、统计年鉴数据和数字高程模型(DEM)数据,基于压力-状态-响应(PSR)模型,采集了2000年、2010年和2020年的Globeland30土地利用数据。选取2000年、2010年和2020年的15个指标构建福州市生态安全评价体系,并采用层次分析法确定各指标的权重。采用空间自相关方法分析福州市土地利用生态安全指数的相关程度。引入生态维护的概念,分析福州市第三期生态维护的现状。最后,利用障碍因子诊断模型确定了影响福州市生态安全的主要障碍因子。结果表明:2000 - 2020年,耕地、草地和裸地面积逐年减少,向人工地表转移的面积分别为320.63 km2、25.34 km2和9.85 km2;2000年、2010年和2020年高值生态安全指数分别为27.54%、28.67%和30.93%。因此,福州市整体生态安全水平有所提高,但局部生态安全存在较大差距。生态维持程度中等的面积占60.15%。从全市来看,生态维护度极差的主要集中在市区和平潭岛,生态维护度极好的占比极低,主要分布在福州西北部。生态安全指数呈现出高值集聚和低值集聚的特征,3个时期4个集聚区分布相似。公路密度、人口密度、地表温度、人为干扰强度、景观多样性、人均GDP和区域发展程度是3个时期生态安全的主要障碍因子。福州市生态安全评价与生态维护有利于为福州市生态环境保护提供有效的决策支持工具。
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引用次数: 25
Forecasting groundwater quality using automatic exponential smoothing model (AESM) in Xianyang City, China 应用自动指数平滑模型(AESM)预测咸阳市地下水水质
Pub Date : 2022-06-17 DOI: 10.1080/10807039.2022.2087176
Abel Nsabimana, Jianhua Wu, Jitian Wu, Fei Xu
Abstract To reasonably ensure good groundwater quality for the safety of users, it is necessary to monitor the evolution of physicochemical parameters of water. This study assessed the evolution of groundwater quality in Xianyang City (Central China) for 6 years and forecasted the water quality index (WQI) using the automatic exponential smoothing model (AESM). The results revealed that pH, Mn, NH4 +, HCO3 − and Ca2+ increased significantly within 6 years. However, there was a slight decrease in K+, NO3 −, SiO2, and Mg2+. Over the course of 6 years, seven out of fourteen wells maintained excellent or good water quality, whereas groundwater quality in the remaining wells fluctuated from excellent to good or from good to poor. The WQI index increased for nine wells, and five of them including well 173, well 457, well 46, well 26, and well C4 manifested an exponential increase of WQI, which was mainly caused by high concentrations of Mn, NH4 +, and NO3 −. The forecast accuracy verified by MASE and sMAPE, which ranged from 0.35 to 1.06 and from 0.04 to 0.69, respectively, demonstrated that the predictions were reliable. The AESM was tested in groundwater quality prediction, indicating that it might be used for actual scientific studies.
摘要为了合理保障地下水水质,保障用户的安全,有必要对水体理化参数的演变进行监测。本文对咸阳市近6年地下水水质变化进行了评价,并采用自动指数平滑模型(AESM)对水质指数(WQI)进行了预测。结果表明,pH、Mn、NH4 +、HCO3−和Ca2+在6年内显著升高。而K+、NO3−、SiO2和Mg2+含量略有下降。在6年的时间里,14口井中有7口保持优良或良好的水质,而其余井的地下水质量在优良到良好或从良好到差之间波动。其中,173、457、46、26、C4 5口井WQI呈指数级上升,主要是由于高浓度Mn、NH4 +和NO3−造成的。MASE和sMAPE的预测精度分别在0.35 ~ 1.06和0.04 ~ 0.69之间,表明预测是可靠的。在地下水水质预测中进行了试验,表明该方法可用于实际的科学研究。
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引用次数: 8
Polycyclic aromatic hydrocarbons (PAHs) exposure through cooking environment and assessment strategies for human health implications 多环芳烃(PAHs)通过烹饪环境暴露及对人类健康影响的评估策略
Pub Date : 2022-06-01 DOI: 10.1080/10807039.2022.2081836
Lochan Singh, Tripti Agarwal
Abstract The polycyclic aromatic hydrocarbons’ (PAHs) exposure through day to day cooking activities has been a serious concern for human health due to their carcinogenic nature. Given the Covid-19 conditions, where people are spending extended time indoors, the likely exposure to these compounds will increase for the members involved/not involved in cooking. In this context, this review summarizes different studies undertaken worldwide on PAHs from cooking activities, the sources of exposure (fumes/emissions, dust/depositions), effect of scale (households/restaurants/neighborhoods) of cooking, monitoring process, risk assessment (air sampling and urinary metabolites), global distribution pattern. Proportionately higher number of studies was focused on cooking fumes and emissions while very limited studies aimed at kitchen depositions and dust. Most of the studies have not reported the size of particulate matter considered for determining PAHs exposure from cooking fumes and emissions. The evaluation of reported data becomes more complicated due to difference in sampling and expression units, the number and types of PAHs (parent, oxygenated-PAHs, i.e., o-PAHs, nitro-PAHs, i.e., n-PAHs) studied/found, lack of other intrinsic information (site and control parameters), lack of specific regulations etc. Therefore, such studies require method standardization for future policy development. This review also highlights the gaps and challenges in existing knowledge and future prospects. Graphical Abstract
摘要:多环芳烃(PAHs)由于其致癌性,在日常烹饪活动中暴露已成为人类健康的一个严重问题。鉴于Covid-19的情况,人们在室内花费的时间更长,参与/不参与烹饪的成员可能会增加接触这些化合物的机会。在此背景下,本综述总结了世界范围内关于烹饪活动、暴露源(烟雾/排放、粉尘/沉积)、烹饪规模(家庭/餐馆/社区)的影响、监测过程、风险评估(空气采样和尿液代谢物)、全球分布格局的不同研究。比例较高的研究集中在烹饪油烟和排放物上,而针对厨房沉积物和灰尘的研究非常有限。大多数研究都没有报告用于确定烹饪烟雾和排放物中多环芳烃暴露的颗粒物的大小。由于采样和表达单位的不同,所研究/发现的多环芳烃(亲本、氧合多环芳烃即o-PAHs、硝基多环芳烃即n-PAHs)的数量和类型不同,缺乏其他内在信息(地点和控制参数),缺乏具体规定等,使得报告数据的评价变得更加复杂。因此,这类研究需要方法标准化,以便于未来的政策制定。本综述还强调了现有知识和未来前景方面的差距和挑战。图形抽象
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引用次数: 2
Spatio-temporal analysis of ecological vulnerability in arid region: A case study of hexi corridor, northwest China 干旱区生态脆弱性时空分析——以河西走廊为例
Pub Date : 2022-05-31 DOI: 10.1080/10807039.2022.2081834
Wei Wei, Congying Liu, Chun-fang Liu, B. Xie, Jun-ju Zhou, Shengxiang Nan
Abstract Ecological vulnerability is one of the core issues in the study of achieving sustainable development and is important for ecological conservation and environmental management, especially for ecologically vulnerable regions. Scientific assessment of ecological vulnerability can improve decision-making capacity and provide appropriate information for sustainable development. The Hexi Corridor is located in the inland northwest of China, and its ecological environment is very fragile. Under the influence of climate change and human activities, the Hexi Corridor is facing a crisis of ecological degradation. Therefore, this paper assessed the influence of various factors on ecological vulnerability, followed the principles of scientificity and data accessibility, and constructed a comprehensive assessment framework to reflect the spatio-temporal characteristics of ecological vulnerability in the Hexi Corridor from three aspects: natural factors, socio-economic factors and human interference factors so as to provide theoretical and practical guidance for regional ecological protection. The results showed that: (1) The ecological vulnerability of the Hexi Corridor was dominated by extreme vulnerability, mainly in the arid desert region, while mildly and lowly vulnerable areas were mainly distributed in the southern Qilian Mountains and the plain oasis region, which was closely related to its physical geography. The index values showed an overall decreasing trend, and the environmental situation was improving from 2000 to 2020. (2) The distribution of ecological vulnerability had obvious directional characteristics, and it gradually decreased from north to south. Moreover, it exhibited a significant positive spatial correlation, and its spatial aggregation pattern was basically consistent with the spatial distribution state. (3) Based on the spatio-temporal patterns of ecological vulnerability, the Hexi Corridor was divided into five zones: ecological core protection zone, integrated ecological monitoring zone, ecological optimization concern zone, ecological restoration management zone and ecological potential governance zone. Different environmental protection policies have been taken for different zones according to its basic conditions. Graphical Abstract Highlights Spatial principal component analysis (SPCA) method was used to analyze the ecological vulnerability factors based on the GIS technology. The partitions of ecological vulnerability for configuration and optimization has been classified and practical application. Geographic detector and national policies were considered for ecological vulnerability driver factors.
生态脆弱性是实现可持续发展研究的核心问题之一,对生态保护和环境管理具有重要意义,对生态脆弱地区尤为重要。科学的生态脆弱性评价可以提高决策能力,为可持续发展提供适当的信息。河西走廊地处中国西北内陆,生态环境十分脆弱。受气候变化和人类活动的影响,河西走廊正面临生态退化的危机。因此,本文评价了各因素对生态脆弱性的影响,遵循科学性和数据可及性原则,构建了综合评价框架,从自然因素、社会经济因素和人为干扰因素三个方面反映河西走廊生态脆弱性的时空特征,为区域生态保护提供理论和实践指导。结果表明:(1)河西走廊的生态脆弱性以极端脆弱性为主,主要分布在干旱荒漠地区,中度和低脆弱性地区主要分布在祁连山南部和平原绿洲地区,这与其自然地理位置密切相关。2000 - 2020年,各指数值总体呈下降趋势,环境状况呈改善趋势。②生态脆弱性分布具有明显的方向性特征,自北向南逐渐减小。空间上表现出显著的正相关关系,其空间聚集格局与空间分布状态基本一致。(3)基于生态脆弱性时空格局,将河西走廊划分为生态核心保护区、综合生态监测区、生态优化关注区、生态修复管理区和生态潜力治理区5个区域。不同区域根据其基本条件采取了不同的环境保护政策。基于GIS技术,采用空间主成分分析(SPCA)方法对生态脆弱性因子进行分析。对生态脆弱性分区进行了分类,并进行了实际应用。考虑了地理探测器和国家政策对生态脆弱性的驱动因素。
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引用次数: 1
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Human and Ecological Risk Assessment: An International Journal
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