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Non-volatile optical filter based on a Ge2Sb2Te5 assisted microring with a tunable bandwidth and extinction ratio 基于Ge2Sb2Te5辅助微环的非易失性光滤波器,具有可调带宽和消光比
Pub Date : 2023-11-02 DOI: 10.1088/1361-6463/ad066c
Yujia Zhang, Yu He, Xuhan Guo, Yikai Su
A novel non-volatile optical filter with a large bandwidth (BW) and extinction ratio (ER) tunability is first experimentally demonstrated by introducing an all-optical phase change of Ge2Sb2Te5 (GST). The Si-GST hybrid device promises flexible multi-level regulation of essential filter parameters in an ultra-compact footprint of 30 μm × 13 μm. Ultra-low power consumption is realised on account of the saving of external static power that is required in other electric-optic or optic-optic-driven filters. The GST is loaded onto two triple-waveguide directional couplers located at the coupling regions of an add-drop microring resonator. By initiating the GST phase transition with pump optical pulses, the transmitted optical power to the cross port of the triple-waveguide coupler is adjustable, hence influencing the coupling efficiency states of the microring filter. Consequently, a tunable on-off ER from 0.7 dB to 18.2 dB and a tunable BW from 0.6 nm to 3.3 nm are experimentally obtained with the aid of optically manipulating the crystallization degree of GST. Our device potentially enables the realisation of high-density photonic integrated circuits, especially in dense wavelength division multiplexing networks.
摘要通过引入GST的全光相变,首次实验证明了一种具有大带宽(BW)和消光比(ER)可调性的新型非易失性滤光片。Si-GST混合器件承诺在30 μ m × 13 μ m的超紧凑尺寸下灵活地多级调节基本滤波器参数。由于节省了其他电光或光-光驱动滤波器所需的外部静态功率,实现了超低功耗。GST被加载到两个三波导定向耦合器上,该耦合器位于加降微环谐振器的耦合区域。通过泵浦光脉冲启动GST相变,可以调节三波导耦合器交叉端口的传输光功率,从而影响微环滤波器的耦合效率状态。因此,通过光学调控GST的结晶度,实验获得了0.7 ~ 18.2 dB的可调通断ER和0.6 ~ 3.3 nm的可调BW。我们的器件有可能实现高密度光子集成电路,特别是在密集的波分复用网络中。
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引用次数: 0
Study of a metal-halide perovskite CsPbBr3 thin film deposited on a 10B layer for neutron detection 金属卤化物钙钛矿CsPbBr3薄膜沉积在10B层上用于中子探测的研究
Pub Date : 2023-11-02 DOI: 10.1088/1361-6463/ad0569
Jessica Carolina Delgado Alvarez, Chiara Provenzano, Marcella Marra, Maurizio Martino, Anna Grazia Monteduro, Sandra Moretto, Felix Pino, Matteo Polo, Gianluca Quarta, Anna Paola Caricato
Abstract Metal halide perovskite materials have received significant attention in recent years due to their promising properties and potential applications, particularly their use as scintillator detectors, which is rapidly emerging due to their promising advantages as detectors, such as low costs, fast response, high quantum yield, strong absorption, scalability, flexibility, and emission wavelength tunability. Given the effectiveness of perovskites as α particle detectors and the potential of 10 B as a neutron converter, in this paper a 10 B converting layer was coupled with an all-inorganic lead halide perovskite (CsPbBr 3 ) layer aiming to create a thermal neutron detector. Specifically, a 1 µ m thin film of 10 B and a 1 µ m thin layer of CsPbBr 3 were deposited on a suitable substrate using a laser ablation process. The fabricated detector was subjected to a comprehensive characterization, including structural, morphological, and detection properties. As output, the films exhibit macroscopically uniform behavior and good adhesion to the substrate. In terms of thermal neutron efficiency, an efficiency of (7.9 ± 0.3)% was determined with respect to a commercial detector (EJ-426), which corresponds to an intrinsic efficiency of (2.5 ± 0.1)%. Also, Monte Carlo simulations were conducted, and the optimum value of the 10 B layer thickness was found to be 2.5 µ m.
近年来,金属卤化物钙钛矿材料因其良好的性能和潜在的应用受到了广泛的关注,特别是作为闪烁体探测器的应用,由于其作为探测器具有低成本、快速响应、高量子产率、强吸收、可扩展性、灵活性和发射波长可调性等优点而迅速兴起。考虑到钙钛矿作为α粒子探测器的有效性和10b作为中子转换器的潜力,本文将10b转换层与全无机卤化铅钙钛矿(CsPbBr 3)层耦合,旨在创建热中子探测器。具体而言,采用激光烧蚀工艺在合适的衬底上沉积了1 μ m的10 B薄膜和1 μ m的CsPbBr 3薄层。制备的探测器进行了全面的表征,包括结构,形态和检测性能。作为输出,薄膜表现出宏观均匀的行为和良好的附着力基材。在热中子效率方面,相对于商用探测器(ejj -426),确定了(7.9±0.3)%的效率,对应于(2.5±0.1)%的固有效率。通过蒙特卡罗模拟,确定了10b层厚度的最优值为2.5µm。
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引用次数: 0
Anomalous Hall effect in naturally oxidized normal-metal Al/Cu double films 自然氧化铝/铜双膜的反常霍尔效应
Pub Date : 2023-11-02 DOI: 10.1088/1361-6463/ad06ed
Lijuan Zhao, Yuzhi Li, Yongzuo Wang, Peng Chen, Bing Lv, Cunxu Gao
Abstract An unexpectedly larger current-induced spin–orbit torque in oxidized Cu (CuO x )/ferromagnet (FM) than heavy-metal/FM has recently attracted intense attention in spintronic studies. Although the two mechanisms, interfacial Rashba Edelstein effect and spin-vorticity coupling, have been put forward based on the two different conductive features of CuO x , i.e. electrical insulator and gradient of electrical mobility, the detailed investigation of transport of CuO x is still lacking. Here we experimentally report the positive and negative anomalous Hall effect (AHE) in naturally oxidized normal-metal Al/Cu double films. We found that the onset temperature of AHE corresponds to magnetic transition temperature of CuO x . Furthermore, by comparing Hall resistance of the crystalline and amorphous Cu/Al double films, we identify that the positive anomalous Hall resistance attributes to magnetic moment of CuO x itself, while the negative anomalous Hall resistance can originate from the spin or orbital currents generated at the CuO x /AlO x interface interact with magnetization of CuO x and its inverse process.
氧化Cu (CuO x)/铁磁体(FM)中电流诱导的自旋轨道转矩比重金属/FM大,近年来在自旋电子学研究中引起了广泛关注。虽然基于CuO x的电绝缘体和电迁移率梯度这两种不同的导电特性,提出了界面Rashba Edelstein效应和自旋涡耦合两种机制,但对CuO x的输运还缺乏详细的研究。在这里,我们实验报道了自然氧化的正常金属Al/Cu双膜中的正、负异常霍尔效应。我们发现AHE的起始温度与CuO x的磁转变温度相对应。此外,通过比较结晶和非晶双膜的霍尔电阻,我们发现正异常霍尔电阻归因于CuO x本身的磁矩,而负异常霍尔电阻可能源于CuO x /AlO x界面上产生的自旋或轨道电流与CuO x的磁化及其逆过程相互作用。
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引用次数: 0
A High-quality Broadband Tunable Terahertz Metamaterial Absorber Based on Graphene 基于石墨烯的高质量宽带可调谐太赫兹超材料吸收体
Pub Date : 2023-11-02 DOI: 10.1088/1361-6463/ad0912
Xiongying Chao, Yan Xu, Feng Huang, Zhaoyang Chen
Abstract We design a graphene-based broadband tunable terahertz metamaterial absorber (MMA). Its structure consists of a surface graphene pattern layer, a medium layer and an underlying metal film. CST simulation results show that the absorption bandwidth for more than 90% absorption rate reaches 2.12 THz, and the range is 3.2-5.32 THz. The absorption bandwidth for more than 99% absorption rate reaches 1.38 THz, and the range is 3.45-4.83 THz, which was not achieved by most of the previous MMA. Multiple reflection interference theory is used to confirm the simulation results. In order to explore the physical mechanism of wideband absorption, we study the surface electric field distribution of the structure. We also find that the absorber has polarization insensitivity and wide-angle incidence characteristics. The absorption frequency of the absorber can be adjusted by changing the chemical potential of graphene. Therefore, the absorber has potential applications in terahertz absorption, filtering and sensing.
摘要设计了一种基于石墨烯的宽带可调谐太赫兹超材料吸收体(MMA)。其结构由表面石墨烯图案层、介质层和底层金属膜组成。CST仿真结果表明,90%吸收率以上的吸收带宽达到2.12 THz,范围为3.2 ~ 5.32 THz。99%吸收率以上的吸收带宽达到1.38 THz,范围为3.45-4.83 THz,这是之前大多数MMA无法实现的。利用多重反射干涉理论对仿真结果进行了验证。为了探索宽带吸收的物理机制,我们研究了该结构的表面电场分布。我们还发现吸收器具有偏振不敏感和广角入射特性。通过改变石墨烯的化学势,可以调节吸收剂的吸收频率。因此,该吸收剂在太赫兹吸收、滤波和传感等方面具有潜在的应用前景。
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引用次数: 0
Table-like magnetocaloric effect due to field induced inter-cluster interactions in Eu0.5Sr0.5MnO3-EuMnO3 composites Eu0.5Sr0.5MnO3-EuMnO3复合材料中场诱导簇间相互作用的表状磁热效应
Pub Date : 2023-11-01 DOI: 10.1088/1361-6463/ad030c
Wasim Akram, Muireann de h-Óra, Manisha Bansal, Rajatava Mukhopadhyay, Judith L MacManus-Driscoll, Tuhin Maity
Abstract The table-like behavior of the magnetic entropy change is generally observed in rare-earth-based alloys (e.g. La(Fe,Si) 13 , Gd 50 Co 45 Fe 5 , Gd 56 Ni 15 Al 27 Zr 2 , Gd ( 1 x y ) Co x Al y etc). Here, we report similar table-like behavior in a bulk perovskite Eu 0.5 Sr 0.5 MnO 3 –EuMnO 3 composite system with a working temperature span of ∼80 K for a field change of ∼70 kOe. AC susceptibility and time-dependent DC magnetization relaxation measurements confirm the presence of interacting ferromagnetic clusters with a Vogel–Fulcher freezing temperature of T 0 42.7 K. The Langevin function fittings of the isothermal magnetization curves show a non-monotonous variation of cluster size with temperature. We propose a model for the high-field dependency of the ferromagnetic cluster coupling in the composite system. This widens the transition temperature region of long-range order formation and hence gives rise to the table-like magnetocaloric effect in Eu 0.5 Sr 0.5 MnO 3 –EuMnO 3 composite systems.
摘要稀土基合金(如La(Fe,Si) 13、Gd 50 Co 45 Fe 5、Gd 56 Ni 15 Al 27 Zr 2、Gd(1−x−y) Co x Al y等)的磁熵变化普遍呈表状。在这里,我们报告了块状钙钛矿Eu 0.5 Sr 0.5 mno3 - euumno3复合体系中类似的表状行为,其工作温度范围为~ 80 K,场变化为~ 70 kOe。交流磁化率和随时间变化的直流磁化弛豫测量证实,在Vogel-Fulcher冻结温度为T 0 ~ 42.7 K时,存在相互作用的铁磁团簇。等温磁化曲线的朗热万函数拟合显示出团簇大小随温度的非单调变化。我们提出了复合系统中铁磁团簇耦合的高场依赖性模型。这扩大了Eu 0.5 Sr 0.5 mno3 - euumno3复合体系的长程有序形成的转变温度区域,从而产生了表状磁热效应。
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引用次数: 0
Review on High-Performance Bulk MgB2 Superconductors 高性能块体MgB2超导体研究进展
Pub Date : 2023-11-01 DOI: 10.1088/1361-6463/ad039a
Muralidhar Miryala, Malik Shadab, Srikanth Sai Arvapalli, Milos Jirsa, Jacques G Noudem
Abstract Although the fascinating effect of superconductivity was discovered more than 100 years ago, only a few low-temperature superconductors, especially Nb 3 Sn and NbTi, have reached everyday-life use. After the discovery of superconductivity in MgB 2 in 2001, a boom appeared in interest in employing MgB 2 in commercial applications, facilitated by simple crystallographic structure, high critical temperature, low-cost raw ingredients, simple and fast production, and other advantages for moderate temperature applications. It only lacks high flux pinning and good mechanical performance. In this review, the implications of manufacturing procedures on the superconducting properties, crystal and electronic structure of MgB 2 are discussed. The advantages and drawbacks of various manufacturing processes will be presented, as well as the ways how to improve MgB 2 superconducting performance. The impact of oxygen reduction, elements doping, the introduction of defects and additives, and the effect of precursor refinement on superconducting properties are here compiled to give an overview of the progress of flux pinning enhancement in bulk MgB 2 .
虽然超导的神奇作用在100多年前就被发现了,但只有少数低温超导体,特别是Nb 3sn和NbTi,已经达到了日常生活的用途。在2001年发现MgB 2的超导性后,由于其晶体结构简单、临界温度高、原料成本低、生产简单快速以及其他适合中温应用的优点,人们对将MgB 2用于商业应用产生了浓厚的兴趣。它只缺乏高的钉接剂和良好的机械性能。本文讨论了制备工艺对二氧化镁超导性能、晶体结构和电子结构的影响。介绍了各种制造工艺的优缺点,以及提高mgb2超导性能的方法。本文综述了氧还原、元素掺杂、缺陷和添加剂的引入以及前驱体细化对MgB 2超导性能的影响。
{"title":"Review on High-Performance Bulk MgB2 Superconductors","authors":"Muralidhar Miryala, Malik Shadab, Srikanth Sai Arvapalli, Milos Jirsa, Jacques G Noudem","doi":"10.1088/1361-6463/ad039a","DOIUrl":"https://doi.org/10.1088/1361-6463/ad039a","url":null,"abstract":"Abstract Although the fascinating effect of superconductivity was discovered more than 100 years ago, only a few low-temperature superconductors, especially Nb 3 Sn and NbTi, have reached everyday-life use. After the discovery of superconductivity in MgB 2 in 2001, a boom appeared in interest in employing MgB 2 in commercial applications, facilitated by simple crystallographic structure, high critical temperature, low-cost raw ingredients, simple and fast production, and other advantages for moderate temperature applications. It only lacks high flux pinning and good mechanical performance. In this review, the implications of manufacturing procedures on the superconducting properties, crystal and electronic structure of MgB 2 are discussed. The advantages and drawbacks of various manufacturing processes will be presented, as well as the ways how to improve MgB 2 superconducting performance. The impact of oxygen reduction, elements doping, the introduction of defects and additives, and the effect of precursor refinement on superconducting properties are here compiled to give an overview of the progress of flux pinning enhancement in bulk MgB 2 .","PeriodicalId":16833,"journal":{"name":"Journal of Physics D","volume":"143 ","pages":"0"},"PeriodicalIF":0.0,"publicationDate":"2023-11-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"136102578","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 1
Far-field pattern control and light-extraction enhancement of deep-ultraviolet light-emitting diodes with large-area Fresnel zone plate nano-structures 大面积菲涅耳带板纳米结构深紫外发光二极管远场模式控制和光提取增强
Pub Date : 2023-10-31 DOI: 10.1088/1361-6463/ad056a
Lingjie Wei, Manabu Taniguchi, Guo-Dong Hao, Shin-ichiro Inoue
Abstract Conventional methods using high-purity quartz lenses to control deep-ultraviolet light-emitting diode (DUV-LED) far-field patterns have limitations, including small effective apertures and high cost. We apply phase-type Fresnel zone plates to control the beam angle and enhance light extraction efficiency (LEE) for DUV-LEDs on sapphire and AlN substrates. We demonstrate highly-collimated optics-free DUV-LED emissions with full width at half maximum far-field divergence angles of 40° and 10° on sapphire and AlN substrates at a peak emission wavelength of 279 nm and 273 nm, respectively. LEE enhancements of 1.4 and 1.5 times for DUV-LEDs on sapphire and AlN substrates, respectively, are also achieved.
传统的利用高纯度石英透镜控制深紫外发光二极管(DUV-LED)远场图形的方法存在有效孔径小、成本高等局限性。我们采用相位型菲涅耳带片来控制光束角度,提高蓝宝石和AlN衬底上duv - led的光提取效率。我们在蓝宝石和AlN衬底上展示了高度准直的无光学DUV-LED发射,其最大远场发散角的一半为40°和10°,峰值发射波长分别为279 nm和273 nm。在蓝宝石和AlN衬底上的duv - led的LEE分别提高了1.4倍和1.5倍。
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引用次数: 0
Irreversible Metamagnetic Transitions in Yb3+- distorted tetragonal Pr0.45Sr0.55MnO3 Yb3+-畸变四边形Pr0.45Sr0.55MnO3的不可逆变磁跃迁
Pub Date : 2023-10-30 DOI: 10.1088/1361-6463/ad030d
Ravi Kiran Dokala, Shaona Das, Ganesh Jangam, Pankaj Kumar Mishra, Subhash Thota
Abstract Field-induced metamagnetic behavior and orbital-ordering (OO) in Yb-substituted (PrSr)MnO 3 perovskites have been reported. The occurrence of distortions in the tetragonal crystal lattice leads to a reduction in the Mn O 2 Mn bond angle, which in turn governs the temperature and field-dependent long-range magnetic orderings. Extensive magnetization measurements reveal the high Curie temperature T C ∼ 302 K ferromagnetic (FM) phase and suggest the possibility of the existence of the OO in Pr 0.45– x Yb x Sr 0.55 MnO 3 accompanied by antiferromagnetic (AFM) Néel temperature, T N , as low as 158 K. Irreversible metamagnetic transitions from the AFM phase to the FM phase occur for a specific composition x = 0.05 (Yb5) until T ⩽ 220 K. The admixture of AFM and FM metastable states is quite robust in the investigated system, whereas the AFM state is mediated by Yb 3+ ions, while the FM state arises as a result of field-driven thermo-magnetic kinetics. These results provide a constructive approach for designing novel spin-valve devices.
本文报道了yb取代mno3钙钛矿的场致变磁性和轨道有序。四方晶格中畸变的发生导致Mn−o2−Mn键角的减小,这反过来又控制了温度和场相关的远程磁有序。广泛的磁化测量揭示了高居里温度T C ~ 302 K铁磁(FM)相,并表明在Pr 0.45 - x Yb x Sr 0.55 mno3中存在OO的可能性,并伴有低至158 K的反铁磁(AFM) n温度T N。对于特定成分x = 0.05 (Yb5),在T≤220 K之前,从AFM相到FM相发生不可逆的变磁转变。在所研究的体系中,AFM和FM亚稳态的混合非常稳定,而AFM状态是由yb3 +离子介导的,而FM状态是由场驱动的热磁动力学引起的。这些结果为设计新型自旋阀装置提供了建设性的思路。
{"title":"Irreversible Metamagnetic Transitions in Yb3+- distorted tetragonal Pr<sub>0.45</sub>Sr<sub>0.55</sub>MnO<sub>3</sub>","authors":"Ravi Kiran Dokala, Shaona Das, Ganesh Jangam, Pankaj Kumar Mishra, Subhash Thota","doi":"10.1088/1361-6463/ad030d","DOIUrl":"https://doi.org/10.1088/1361-6463/ad030d","url":null,"abstract":"Abstract Field-induced metamagnetic behavior and orbital-ordering (OO) in Yb-substituted (PrSr)MnO 3 perovskites have been reported. The occurrence of distortions in the tetragonal crystal lattice leads to a reduction in the <?CDATA ${text{Mn}} - {{text{O}}_{left( 2 right)}} - {text{Mn}}$?> <mml:math xmlns:mml=\"http://www.w3.org/1998/Math/MathML\" overflow=\"scroll\"> <mml:mrow> <mml:mtext>Mn</mml:mtext> </mml:mrow> <mml:mo>−</mml:mo> <mml:mrow> <mml:msub> <mml:mrow> <mml:mtext>O</mml:mtext> </mml:mrow> <mml:mrow> <mml:mfenced close=\")\" open=\"(\"> <mml:mn>2</mml:mn> </mml:mfenced> </mml:mrow> </mml:msub> </mml:mrow> <mml:mo>−</mml:mo> <mml:mrow> <mml:mtext>Mn</mml:mtext> </mml:mrow> </mml:math> bond angle, which in turn governs the temperature and field-dependent long-range magnetic orderings. Extensive magnetization measurements reveal the high Curie temperature <?CDATA ${T_{text{C}}}$?> <mml:math xmlns:mml=\"http://www.w3.org/1998/Math/MathML\" overflow=\"scroll\"> <mml:mrow> <mml:msub> <mml:mi>T</mml:mi> <mml:mrow> <mml:mtext>C</mml:mtext> </mml:mrow> </mml:msub> </mml:mrow> </mml:math> ∼ 302 K ferromagnetic (FM) phase and suggest the possibility of the existence of the OO in Pr 0.45– x Yb x Sr 0.55 MnO 3 accompanied by antiferromagnetic (AFM) Néel temperature, <?CDATA ${T_{text{N}}}$?> <mml:math xmlns:mml=\"http://www.w3.org/1998/Math/MathML\" overflow=\"scroll\"> <mml:mrow> <mml:msub> <mml:mi>T</mml:mi> <mml:mrow> <mml:mtext>N</mml:mtext> </mml:mrow> </mml:msub> </mml:mrow> </mml:math> , as low as 158 K. Irreversible metamagnetic transitions from the AFM phase to the FM phase occur for a specific composition x = 0.05 (Yb5) until <?CDATA $T$?> <mml:math xmlns:mml=\"http://www.w3.org/1998/Math/MathML\" overflow=\"scroll\"> <mml:mi>T</mml:mi> </mml:math> ⩽ 220 K. The admixture of AFM and FM metastable states is quite robust in the investigated system, whereas the AFM state is mediated by Yb 3+ ions, while the FM state arises as a result of field-driven thermo-magnetic kinetics. These results provide a constructive approach for designing novel spin-valve devices.","PeriodicalId":16833,"journal":{"name":"Journal of Physics D","volume":"13 1","pages":"0"},"PeriodicalIF":0.0,"publicationDate":"2023-10-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"136018145","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Effect of the number of magnetic matrices on particle capture in high gradient magnetic separation 高梯度磁选中磁性基质数量对颗粒捕获的影响
Pub Date : 2023-10-30 DOI: 10.1088/1361-6463/ad005f
Yu Tian, Quanliang Cao
Abstract A comprehensive understanding of the capture process involving matrices in high gradient magnetic separation (HGMS) is crucial for the design and improvement of matrix performance. However, few existing studies have paid attention to the influence of the number of magnetic matrices on the capture process. In this work, we numerically investigate this issue in both longitudinal and transversal HGMS systems, where multiple scenarios with different particle sizes, flow rates and matrix spacing are considered. Interestingly, we show that in most cases, increasing the number of magnetic matrices along the flow direction has little to no influence on the capture radius. It has a certain effect on improving the capture radius only in a few specific cases, such as when dealing with large particles at low flow rates with closely spaced matrices or when working with small particles at high flow rates with widely spaced matrices. These phenomena are related to the appearance of repulsive magnetic forces around matrices and the distribution characteristics of magnetic forces. The obtained results indicate that, in the design of the practical HGMS system, simply increasing the number of matrices along the flow direction may not be a reasonable or effective strategy for enhancing capture performance.
全面了解高梯度磁分离(HGMS)中基质的捕获过程对于设计和提高基质性能至关重要。然而,现有的研究很少关注磁性基质数量对捕获过程的影响。在这项工作中,我们在纵向和横向HGMS系统中对这一问题进行了数值研究,其中考虑了不同粒径、流速和基质间距的多种情况。有趣的是,我们发现在大多数情况下,沿流动方向增加磁性矩阵的数量对捕获半径几乎没有影响。它仅在少数特定情况下对提高捕获半径有一定的作用,例如当处理小颗粒在低流速下与紧密间隔的矩阵或当处理小颗粒在高流速下与广泛间隔的矩阵。这些现象与基质周围排斥性磁力的出现和磁力的分布特性有关。结果表明,在实际HGMS系统的设计中,简单地增加沿流动方向的矩阵数量可能不是提高捕获性能的合理或有效的策略。
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引用次数: 0
Resistive switching behaviour of nickel nanoparticles embedded naphthalene sulfonic acid doped polyaniline nanocomposites 纳米镍包埋萘磺酸掺杂聚苯胺纳米复合材料的电阻开关行为
Pub Date : 2023-10-30 DOI: 10.1088/1361-6463/ad039d
Madhumita Bhaumik, Arjun Maity, Hendrik G. Brink, Zolile Wiseman Dlamini, SrinivasuVijaya Vallabhapurapu
Abstract Hybrid nanocomposite (NC) materials comprising organic polymers and inorganic metal nanoparticles (NPs) with unique properties are popular for their advanced technological applications including resistive switching memory devices. Herein, NCs of 2-naphthalene sulphonic acid-doped polyaniline nanotubes (PANI-NSA NTs) and nickel nanoparticles (Ni NPs) were synthesized via a facile chemical synthesis procedure where metallic Ni NPs were embedded in/deposited onto the surface of PANI-NSA NTs by a simple reduction method. Different characterization methods revealed successful deposition of weak ferromagnetic Ni NPs onto the PANI-NSA matrix. The bipolar resistive switching behaviour of the as-synthesized PANI-NSA + Ni NCs was investigated under the application of voltage stress in a two-terminal sandwiched device configuration. The fabricated indium tin oxide/PANI-NSA + Ni/silver (ITO/PANI-NSA + Ni/Ag) device displays bipolar resistive switching properties having a memory window of ∼1.5 × 10 3 , and switches effectively over 200 cycles. Ohmic conduction in the lower-voltage regime and the space-charge-limited Mott–Gurney current conduction model in the higher-voltage region were identified as major charge conduction mechanisms in the high resistive state of the device. On the other hand, in the entire low resistive state region the experimental data followed the Mott–Gurney conduction model.
摘要由有机聚合物和无机金属纳米颗粒组成的混合纳米复合材料(NC)具有独特的性能,在电阻式开关存储器件等领域具有广泛的应用前景。本文采用简单的化学合成方法,通过简单的还原法将金属Ni NPs嵌入/沉积在聚苯胺- nsa纳米管表面,合成了2-萘磺酸掺杂聚苯胺纳米管(PANI-NSA NTs)和镍纳米颗粒(Ni NPs)。不同的表征方法显示弱铁磁性Ni NPs成功沉积在PANI-NSA基体上。在双端夹层结构下,研究了合成的聚苯胺- nsa + Ni纳米材料在电压应力作用下的双极电阻开关行为。所制备的氧化铟锡/PANI-NSA + Ni/银(ITO/PANI-NSA + Ni/Ag)器件具有双极电阻开关特性,其记忆窗口为~ 1.5 × 10.3,并且有效开关超过200次循环。确定了低电压区欧姆传导和高电压区空间电荷受限Mott-Gurney电流传导模型是器件高阻状态下的主要电荷传导机制。另一方面,在整个低阻状态区,实验数据遵循Mott-Gurney传导模型。
{"title":"Resistive switching behaviour of nickel nanoparticles embedded naphthalene sulfonic acid doped polyaniline nanocomposites","authors":"Madhumita Bhaumik, Arjun Maity, Hendrik G. Brink, Zolile Wiseman Dlamini, SrinivasuVijaya Vallabhapurapu","doi":"10.1088/1361-6463/ad039d","DOIUrl":"https://doi.org/10.1088/1361-6463/ad039d","url":null,"abstract":"Abstract Hybrid nanocomposite (NC) materials comprising organic polymers and inorganic metal nanoparticles (NPs) with unique properties are popular for their advanced technological applications including resistive switching memory devices. Herein, NCs of 2-naphthalene sulphonic acid-doped polyaniline nanotubes (PANI-NSA NTs) and nickel nanoparticles (Ni NPs) were synthesized via a facile chemical synthesis procedure where metallic Ni NPs were embedded in/deposited onto the surface of PANI-NSA NTs by a simple reduction method. Different characterization methods revealed successful deposition of weak ferromagnetic Ni NPs onto the PANI-NSA matrix. The bipolar resistive switching behaviour of the as-synthesized PANI-NSA + Ni NCs was investigated under the application of voltage stress in a two-terminal sandwiched device configuration. The fabricated indium tin oxide/PANI-NSA + Ni/silver (ITO/PANI-NSA + Ni/Ag) device displays bipolar resistive switching properties having a memory window of ∼1.5 × 10 3 , and switches effectively over 200 cycles. Ohmic conduction in the lower-voltage regime and the space-charge-limited Mott–Gurney current conduction model in the higher-voltage region were identified as major charge conduction mechanisms in the high resistive state of the device. On the other hand, in the entire low resistive state region the experimental data followed the Mott–Gurney conduction model.","PeriodicalId":16833,"journal":{"name":"Journal of Physics D","volume":"22 5","pages":"0"},"PeriodicalIF":0.0,"publicationDate":"2023-10-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"136019239","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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Journal of Physics D
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