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Helium-induced broadening and shifting in the first overtone of hydrogen fluoride 氦引起氟化氢第一泛音的加宽和移位
IF 1.9 3区 物理与天体物理 Q2 OPTICS Pub Date : 2026-03-01 Epub Date: 2025-12-05 DOI: 10.1016/j.jqsrt.2025.109787
I.A. Tolstikov , A.V. Domanskaya , O.O. Diachkova , R.E. Asfin
Spectra of HF mixtures with helium were recorded at elevated pressures ranging from 1 to 11 atm at 297.8(2) K. The rovibrational lines in the first overtone band were fitted with Voigt and Rautian profiles. The broadening and shifting coefficients for 19 lines in the first overtone are reported. An estimate for the velocity changing shifting coefficients for 11 lines is obtained. To the best of our knowledge, most of the reported line parameters are novel. Herman–Wallis coefficients were determined from the line intensity distribution as well.
在297.8(2)k的高压下,记录了HF -氦混合物在1 ~ 11 atm范围内的光谱,第一泛音波段的振动谱线符合Voigt和Rautian谱线。报道了第一泛音中19条线的加宽系数和移位系数。得到了11条线的速度变化位移系数的估计。据我们所知,大多数报道的线路参数都是新的。赫尔曼-沃利斯系数也由线强度分布确定。
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引用次数: 0
N2-broadening coefficients and their temperature exponents for ethylene lines: A semi-empirical approach for (exo)planetary studies 乙烯谱线的n2 -展宽系数及其温度指数:外行星研究的半经验方法
IF 1.9 3区 物理与天体物理 Q2 OPTICS Pub Date : 2026-03-01 Epub Date: 2025-11-19 DOI: 10.1016/j.jqsrt.2025.109758
Sarah Clavier , Michael Rey , Jeanna Buldyreva
Nitrogen-broadening coefficients for ethylene absorption lines in the ν7 band are computed theoretically to fill in the enormous gaps existing in available experimental data. A semi-empirical method relying on the Anderson theory is employed for this purpose, with the model parameters adjusted on some rare room-temperature measurements and used further for calculations in extended temperature ranges. The spectroscopically active molecule C2H4 is rigorously treated as an asymmetric top, and its energy levels and wavefunctions are accurately computed by a quantum-chemistry methodology based on ab initio potential energy surfaces. Theoretical broadening values are obtained for the temperature range 100–1000 K relevant to studies of planetary and exoplanetary atmospheres. These values are further analyzed by the traditional power law to get the associated temperature-dependence exponents. Comparisons of the computed theoretical results with previous measurements and calculations are provided at a low temperature of 173 K to validate the theoretical method chosen. Since the power law describes perfectly the considered temperature range, the sets of reference-temperature broadening coefficients and their temperature exponents can be safely used for higher temperatures where semi-classical approaches applicability only grows. These data are provided for the quantum numbers 0J47, K26 and the three P-, Q-, R-branches of the ν7 band, i.e. represent the most comprehensive up-to-date description of N2-broadened ethylene linewidths suitable for integration into spectroscopic databases and high-temperature simulations of (exo)planetary atmospheres.
从理论上计算了ν7波段乙烯吸收谱线的氮展宽系数,以填补现有实验数据中存在的巨大空白。为此,采用了一种基于安德森理论的半经验方法,在一些罕见的室温测量上调整模型参数,并进一步用于扩大温度范围的计算。对具有光谱活性的分子C2H4进行了严格的非对称顶处理,并采用基于从头算势能面的量子化学方法精确计算了其能级和波函数。得到了与行星和系外行星大气研究有关的100 - 1000k温度范围的理论展宽值。利用传统幂律法对这些值进行进一步分析,得到相应的温度依赖指数。在173 K的低温条件下,将计算的理论结果与以往的测量和计算结果进行了比较,以验证所选择的理论方法。由于幂律完美地描述了所考虑的温度范围,参考温度展宽系数集合及其温度指数可以安全地用于更高的温度,而半经典方法的适用性只会增加。这些数据是为量子数0≤J≤47,K≤26和ν7波段的三个P-, Q-, r -分支提供的,即代表了最新最全面的n2加宽乙烯线宽描述,适合集成到光谱数据库和(外)行星大气的高温模拟中。
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引用次数: 0
Volumetric optical properties of alumina-carbon soot hybrid medium in high-speed aircraft plumes 高速飞机羽流中铝碳烟灰混合介质的体积光学性质
IF 1.9 3区 物理与天体物理 Q2 OPTICS Pub Date : 2026-03-01 Epub Date: 2026-01-07 DOI: 10.1016/j.jqsrt.2026.109808
JingYing Li, XiaoXiao Song, ShanShan Fan
The spectral radiation characteristics of aircraft exhaust plumes are significantly influenced by the volumetric optical properties of alumina-carbon soot hybrid media. This study develops a dedicated computational algorithm to determine these properties by establishing realistic models for alumina and carbon soot clusters in the plume and derives formulas for calculating the volumetric optical properties per unit volume of the hybrid medium. The characteristics are analyzed in the ultraviolet (280 nm) and infrared (4.3 µm) bands. The results show that: (1) In the ultraviolet band, the extinction process is primarily governed by scattering from alumina particles, with carbon soot particles accounting for over 99% of the absorption. Conversely, in the infrared band, extinction is dominated by absorption from carbon soot particles, while the contribution of alumina particles to extinction is only 2%–4.5%. (2) In the ultraviolet band, the volumetric scattering phase function of the hybrid medium exhibits strong forward scattering, which decreases with increasing carbon soot content. In the infrared band, the scattering phase function becomes relatively flat, demonstrating isotropic scattering characteristics. (3) Regarding polarization properties, the volumetric linear polarization degree in the ultraviolet band is predominantly negative, and the circular polarization displays a distribution from strong right-handed in the forward direction to strong left-handed in the backward direction. In the infrared band, the linear polarization exhibits a strictly even-symmetric positive distribution about 90°, and the circular polarization shows strict central symmetry about 90°. The conclusions of this study provide a theoretical basis for multi-band radiation characteristic modeling and target identification of high-speed aircraft exhaust plumes.
铝碳混合介质的体积光学特性对飞机排气羽流的光谱辐射特性有显著影响。本研究开发了一种专用的计算算法,通过建立羽流中氧化铝和碳烟簇的现实模型来确定这些特性,并推导出计算混合介质单位体积体积光学特性的公式。在紫外(280 nm)和红外(4.3µm)波段分析了其特性。结果表明:(1)在紫外波段,消光过程主要受氧化铝颗粒的散射控制,碳烟颗粒占吸收的99%以上;相反,在红外波段,碳烟灰颗粒的吸收主导了消光,而氧化铝颗粒对消光的贡献仅为2%-4.5%。(2)在紫外波段,混合介质的体积散射相函数表现出强烈的前向散射,随碳烟含量的增加而减小。在红外波段,散射相函数变得相对平坦,表现出各向同性散射特性。(3)在极化特性上,紫外波段的体积线极化度以负极化为主,圆极化呈现由正向强右手向反向强左手的分布。在红外波段,线偏振呈严格均匀对称的约90°正分布,圆偏振呈严格中心对称的约90°正分布。研究结果为高速飞机排气羽流多波段辐射特性建模和目标识别提供了理论依据。
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引用次数: 0
Transmittance of Gaussian beam in anisotropic jet engine exhaust turbulence 各向异性喷气发动机排气湍流中高斯光束的透射率
IF 1.9 3区 物理与天体物理 Q2 OPTICS Pub Date : 2026-03-01 Epub Date: 2026-01-08 DOI: 10.1016/j.jqsrt.2026.109816
Yahya Baykal
Transmittance is a metric that provides information on how much of the intensity is transferred to the receiver for a given medium. One of the definitions of transmittance is the ratio of the average received intensity in the presence of turbulence to the received intensity in the absence of turbulence. Under such definition, transmittance is found in an anisotropic jet engine exhaust turbulent environment. For various receiver points, transmittances versus the wireless optical communication (WOC) link and anisotropic jet engine exhaust turbulence parameters are presented. The results are useful for designers of WOC links that are installed in the premises such as the airports that possess jet engine exhaust turbulence.
透光率是一种度量,它提供了给定介质中有多少强度被传递到接收器的信息。透光率的定义之一是存在湍流时的平均接收强度与没有湍流时的接收强度之比。在此定义下,得到了各向异性喷气发动机排气湍流环境下的透光率。对于不同的接收点,给出了无线光通信(WOC)链路的透射率和各向异性喷气发动机排气湍流参数。这些结果对于安装在具有喷气发动机排气湍流的机场等场所的WOC链路的设计者是有用的。
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引用次数: 0
Tunable pixelated graphene based thermal infrared emitter array and its electrothermal characterization 基于可调谐像素化石墨烯的热红外发射器阵列及其电热特性
IF 1.9 3区 物理与天体物理 Q2 OPTICS Pub Date : 2026-03-01 Epub Date: 2026-01-08 DOI: 10.1016/j.jqsrt.2026.109817
Yibai Zhong , Xiu Liu , Zexiao Wang , Jingyi Zou , Tianyi Huang , Sen Lin , Xiao Luo , Zhuo Li , Rui Cheng , Xu Zhang , Sheng Shen
In this work, we design and fabricate tunable pixelated infrared emitter arrays based on graphene transistors. We use finite element analysis to simulate a 5-by-3 pixelated emitter array, where localized heating area can be confined within a size of 25 μm and reaches more than 10 K temperature rise within 3 μs. By applying fast sweeping scheme with electrostatic voltage inputs, tunable surface patterns assembling dynamic alphabetical letters of microscale sizes are demonstrated and captured via thermal mapping with its thermal emission variation caused by localized temperature rise. Our results show that thermal emission can be highly localized and reconfigurable both spatially and temporally, which paves the way for developing and boosting the performance of microscale and nanoscale thermally driven devices for communication, characterization, sensing and actuation.
在这项工作中,我们设计和制造了基于石墨烯晶体管的可调谐像素化红外发射器阵列。利用有限元方法模拟了一个5 × 3像素的发射极阵列,该阵列的局部加热区域可以限制在25 μm内,并在3 μs内达到10 K以上的温升。通过采用静电电压输入的快速扫描方案,展示并捕获了由微尺度动态字母组成的可调表面图案,并通过热成像捕获了其局部温升引起的热发射变化。我们的研究结果表明,热发射在空间和时间上都是高度局域化和可重构的,这为开发和提高用于通信、表征、传感和驱动的微尺度和纳米尺度热驱动器件的性能铺平了道路。
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引用次数: 0
Mikhail Tretyakov’s scientific legacy 米哈伊尔·特列季亚科夫的科学遗产
IF 1.9 3区 物理与天体物理 Q2 OPTICS Pub Date : 2026-03-01 Epub Date: 2026-01-05 DOI: 10.1016/j.jqsrt.2025.109803
Andrei A. Vigasin , Jonathan Tennyson , Oleg L. Polyansky
Mikhail Yurievich Tretyakov (1958–2024) was a leading spectroscopist working at terahertz and microwave wavelengths. He made substantial advances in sub-millimeter spectrometers and performed spectroscopic studies on isolated gaseous, molecular complexes and, in particular, the water dimer. He also studied molecular interactions and line shapes, using them to develop ideas about the physics of the water continuum. In this memorial paper, we review Mikail Tretyakov’s life and his major scientific achievements.
米哈伊尔·尤里耶维奇·特列季亚科夫(1958-2024)是研究太赫兹和微波波长的主要光谱学家。他在亚毫米光谱仪方面取得了重大进展,并对分离的气体、分子复合物,特别是水二聚体进行了光谱研究。他还研究了分子间的相互作用和线条的形状,并用它们来发展关于水连续体物理学的想法。本文回顾了特列季亚科夫的一生和他的主要科学成就。
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引用次数: 0
Study of linear depolarization ratios across a wide range of scattering angles for particles of diverse sizes, shapes, and complex refractive indices 不同尺寸、形状和复折射率粒子在大散射角范围内的线性退极化比研究
IF 1.9 3区 物理与天体物理 Q2 OPTICS Pub Date : 2026-03-01 Epub Date: 2025-11-21 DOI: 10.1016/j.jqsrt.2025.109761
Prakash Gautam , Justin B. Maughan , Hans Moosmüller , Kurt Ehlers , Christopher M. Sorensen
Polarimetry is a valuable technique for remote sensing of atmospheric aerosol particles, with the linear depolarization ratio (LDR) being a key parameter used to characterize particle properties. This study investigates the LDRs of various aerosol particles, including nearly spherical and irregular aluminum oxide (Al2O3), Arizona Road Dust (AZRD), and molybdenum disulfide (MoS2) particles, using both laboratory measurements conducted at a wavelength of 532 nm over a scattering angle range from 0.32° to 177.6° and theoretical model computations for spheroids and Gaussian random spheres. The results demonstrate that the LDR is strongly influenced by particle size, shape, and refractive index, with significant variations across different scattering angles. In the forward-scattering regime, LDR values are small due to scattering being dominated by diffraction, while in the side-scattering regime, LDR increases, peaking around 140° to 160°, before decreasing in the back-scattering regime. This study further explores the relationship between LDR and particle morphology, as well as the impact of the imaginary part of the complex refractive index on LDR, with results showing that higher absorption leads to lower LDRs. Overall, this study contributes to a better understanding of how LDR behaves for different particle types and scattering angles, enhancing our understanding of the optical properties of aerosol particles towards improved polarimetric remote sensing retrievals.
偏振法是遥感大气气溶胶粒子的一项有价值的技术,线性去极化比(LDR)是表征气溶胶粒子特性的关键参数。本文研究了各种气溶胶颗粒的LDRs,包括近球形和不规则的氧化铝(Al2O3),亚利桑那道路粉尘(AZRD)和二硫化钼(MoS2)颗粒,使用波长为532 nm,散射角范围为0.32°至177.6°的实验室测量和球形和高斯随机球体的理论模型计算。结果表明,LDR受颗粒大小、形状和折射率的影响较大,且在不同散射角度下变化显著。在前向散射区,由于散射以衍射为主,LDR值很小,而在侧向散射区,LDR值增加,在140°~ 160°左右达到峰值,后向散射区LDR值下降。本研究进一步探讨了LDR与粒子形态的关系,以及复折射率虚部对LDR的影响,结果表明吸收越高,LDR越低。总的来说,本研究有助于更好地理解LDR在不同颗粒类型和散射角度下的行为,增强我们对气溶胶颗粒光学特性的理解,从而改进偏振遥感检索。
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引用次数: 0
Semiclassical dynamics of the lemniscate ordered emitters enhanced by plasmon-polaritons in nanorings 纳米粒子中等离子体极化增强的微星有序发射体的半经典动力学
IF 1.9 3区 物理与天体物理 Q2 OPTICS Pub Date : 2026-03-01 Epub Date: 2025-11-11 DOI: 10.1016/j.jqsrt.2025.109740
Gennadiy Burlak , Gustavo Medina-Ángel
The semiclassical dynamics of optical nanoemitters (NEs) arranged in the shape of a Bernoulli lemniscate (LB), enhanced by plasmon–polaritons (PPs) in a lattice of conducting nanorings (NRs), are investigated. The coupling of PP and NE is mediated by a common optical field and NE with a finite lifetime of pumping are considered. Using the FDTD approach, it is found that the field structure and the NE dynamics significantly depend on the plasma frequency of the NR. If the intersection point of the LB branches (the region of high NE density) is located inside the NR gaps, a significant increase in the laser field strength and quantum cross-correlations in the NE subsystem occurs. This effect may be exploited to create new types of emitting devices using dispersed nano-objects in modern nanoelectronics.
研究了导电纳米晶格中等离子体极化子(PPs)增强的伯努利透镜状光学纳米发射体(NEs)的半经典动力学。PP和NE的耦合是由一个共同光场介导的,并考虑了具有有限抽运寿命的NE。利用时域有限差分方法,发现场结构和NE动力学显著依赖于NR的等离子体频率。如果LB分支的交点(高NE密度区域)位于NR间隙内,则NE子系统中的激光场强和量子互相关会显著增加。在现代纳米电子学中,利用这种效应可以利用分散的纳米物体来制造新型的发射器件。
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引用次数: 0
Microwave-optical double-resonance spectroscopy of rubidium-87 atoms in a microcell 微电池中铷-87原子的微波光学双共振光谱
IF 1.9 3区 物理与天体物理 Q2 OPTICS Pub Date : 2026-03-01 Epub Date: 2026-01-15 DOI: 10.1016/j.jqsrt.2026.109829
Alexandra A. Idrisova , Armen D. Sargsyan , David H. Sarkisyan , Victor I. Balykin , Anton E. Afanasiev
We studied spectral properties of atoms in a microcell of 80 μm length using the microwave-optical double-resonance (DR) spectroscopy in the presence of a magnetic field. The obtained spectra were compared with similar ones from atoms in a macroscopic vapor cell. The comparison demonstrates the potential of microcells for implementation of compact magnetometers. The effect of radiation trapping has been investigated as a limiting factor of the width of double-resonance spectral lines.
在磁场作用下,利用微波-光学双共振(DR)光谱学研究了80 μm长度微电池中原子的光谱特性。所得光谱与宏观蒸汽池中原子的相似光谱进行了比较。通过比较,证明了微电池在实现紧凑型磁力计方面的潜力。研究了辐射俘获作为双共振谱线宽度的限制因素的影响。
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引用次数: 0
Multi-channel modulation of vortex auto-focusing Airy beams and full-polarization states detection on a monolithic metasurface 单片超表面涡旋自聚焦Airy光束的多通道调制与全偏振态检测
IF 1.9 3区 物理与天体物理 Q2 OPTICS Pub Date : 2026-03-01 Epub Date: 2026-01-11 DOI: 10.1016/j.jqsrt.2026.109815
Guoxia Han , Kaiqi Liu , Feiyang Zhang , Yuhui Peng , Yihan Tian , Xiaolong Liu , Xianghua Yu
Combining the advantages of both auto-focusing Airy beams and vortex beams, the vortex auto-focusing Airy (VAFA) beam has received increasing attentions. However, conventional methods to generate VAFA beams usually require the utilization of bulky devices and complex optical systems, and the applications of VAFA beams are rarely reported. In this work, a novel method to generate and modulate multimode VAFA beams with a single monolayer metasurface is proposed based on the angularly spacing arrangement array and polarization multiplexing. Through spatial multiplexing and polarization multiplexing, we have significantly expanded the modulation capacity of a single-layer metasurface, enabling the synchronous and independent control of multiple optical channels. Based on this approach, we achieved complex manipulation of multimode VAFA beams and the generation of VAFA beams array. Additionally, leveraging the VAFA beam arrays, we designed a polarization-detection metasurface capable of full-polarization states detection. This work not only offers a fresh perspective on the flexible production of multiple beams with a single monolayer metasurface, but also presents the applications in the field of polarization detection of complex Airy beams, holding great potential for a wide range of applications in laser processing and optical communication.
涡流自聚焦Airy (VAFA)光束结合了自聚焦Airy光束和涡旋光束的优点,越来越受到人们的关注。然而,传统的产生VAFA光束的方法通常需要使用笨重的设备和复杂的光学系统,并且VAFA光束的应用很少被报道。本文提出了一种基于角度间距排列阵列和偏振复用的单层超表面多模VAFA波束产生和调制方法。通过空间复用和极化复用,我们极大地扩展了单层超表面的调制能力,实现了多个光通道的同步和独立控制。在此基础上,实现了多模VAFA波束的复杂操纵和VAFA波束阵列的生成。此外,利用VAFA波束阵列,我们设计了一个能够检测全极化状态的偏振检测超表面。该研究不仅为单层超表面柔性生产多束光束提供了新的视角,而且在复杂艾里光束偏振检测领域也有了应用前景,在激光加工和光通信领域具有广阔的应用前景。
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引用次数: 0
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Journal of Quantitative Spectroscopy & Radiative Transfer
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