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Revolutionizing solid-state single-photon sources with multifunctional metalenses. 利用多功能金属透镜革新固态单光子源。
IF 19.4 1区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2024-01-17 DOI: 10.1038/s41377-023-01372-3
Fei Ding

Ultrathin multifunctional metalenses are demonstrated to control the multiple degrees of freedom of a single-photon source in hexagonal boron nitride.

展示了超薄多功能金属透镜,用于控制六方氮化硼中单光子源的多个自由度。
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引用次数: 0
Highly-coherent second-harmonic generation in a chip-scale source. 在芯片级信号源中产生高相干二次谐波。
IF 19.4 1区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2024-01-17 DOI: 10.1038/s41377-023-01359-0
Xuanyi Liu, Hongyan Fu

A highly efficient second-harmonic source is integrated into a silicon nitride microring resonator, unlocking the potential for advanced chip-scale devices such as miniaturized atomic clocks and fully integrated self-referenced microcombs.

将高效二次谐波源集成到氮化硅微孔谐振器中,为微型原子钟和完全集成的自参考微蜂窝等先进芯片级设备的开发挖掘了潜力。
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引用次数: 0
Single photon emitter deterministically coupled to a topological corner state. 与拓扑角态确定耦合的单光子发射器。
IF 19.4 1区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2024-01-17 DOI: 10.1038/s41377-024-01377-6
Mujie Rao, Fulong Shi, Zhixuan Rao, Jiawei Yang, Changkun Song, Xiaodong Chen, Jianwen Dong, Ying Yu, Siyuan Yu

Incorporating topological physics into the realm of quantum photonics holds the promise of developing quantum light emitters with inherent topological robustness and immunity to backscattering. Nonetheless, the deterministic interaction of quantum emitters with topologically nontrivial resonances remains largely unexplored. Here we present a single photon emitter that utilizes a single semiconductor quantum dot, deterministically coupled to a second-order topological corner state in a photonic crystal cavity. By investigating the Purcell enhancement of both single photon count and emission rate within this topological cavity, we achieve an experimental Purcell factor of Fp = 3.7. Furthermore, we demonstrate the on-demand emission of polarized single photons, with a second-order autocorrelation function g(2)(0) as low as 0.024 ± 0.103. Our approach facilitates the customization of light-matter interactions in topologically nontrivial environments, thereby offering promising applications in the field of quantum photonics.

将拓扑物理学纳入量子光子学领域,有望开发出具有固有拓扑稳健性和抗反向散射能力的量子光发射器。然而,量子发射器与拓扑非琐碎共振的确定性相互作用在很大程度上仍未得到探索。在这里,我们展示了一种单光子发射器,它利用单个半导体量子点,与光子晶体腔中的二阶拓扑角态确定性耦合。通过研究该拓扑腔内单光子计数和发射率的珀塞尔增强,我们获得了 Fp = 3.7 的实验珀塞尔因子。此外,我们还证明了偏振单光子的按需发射,其二阶自相关函数 g(2)(0) 低至 0.024 ± 0.103。我们的方法有助于在拓扑学上非难环境中定制光-物质相互作用,从而为量子光子学领域提供了广阔的应用前景。
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引用次数: 0
Near infrared emissions from both high efficient quantum cutting (173%) and nearly-pure-color upconversion in NaY(WO4)2:Er3+/Yb3+ with thermal management capability for silicon-based solar cells. NaY(WO4)2:Er3+/Yb3+ 中的高效量子切割(173%)和近乎纯色的上转换产生的近红外辐射,可用于硅基太阳能电池的热管理。
IF 19.4 1区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2024-01-16 DOI: 10.1038/s41377-023-01365-2
Duan Gao, Baojiu Chen, Xuezhu Sha, Yuhang Zhang, Xin Chen, Li Wang, Xizhen Zhang, Jinsu Zhang, Yongze Cao, Yichao Wang, Lei Li, Xiangping Li, Sai Xu, Hongquan Yu, Lihong Cheng

Raising photoelectric conversion efficiency and enhancing heat management are two critical concerns for silicon-based solar cells. In this work, efficient Yb3+ infrared emissions from both quantum cutting and upconversion were demonstrated by adjusting Er3+ and Yb3+ concentrations, and thermo-manage-applicable temperature sensing based on the luminescence intensity ratio of two super-low thermal quenching levels was discovered in an Er3+/Yb3+ co-doped tungstate system. The quantum cutting mechanism was clearly decrypted as a two-step energy transfer process from Er3+ to Yb3+. The two-step energy transfer efficiencies, the radiative and nonradiative transition rates of all interested 4 f levels of Er3+ in NaY(WO4)2 were confirmed in the framework of Föster-Dexter theory, Judd-Ofelt theory, and energy gap law, and based on these obtained efficiencies and rates the quantum cutting efficiency was furthermore determined to be as high as 173% in NaY(WO4)2: 5 mol% Er3+/50 mol% Yb3+ sample. Strong and nearly pure infrared upconversion emission of Yb3+ under 1550 nm excitation was achieved in Er3+/Yb3+ co-doped NaY(WO4)2 by adjusting Yb3+ doping concentrations. The Yb3+ induced infrared upconversion emission enhancement was attributed to the efficient energy transfer 4I11/2 (Er3+) + 2F7/2 (Yb3+) → 4I15/2 (Er3+) + 2F5/2 (Yb3+) and large nonradiative relaxation rate of 4I9/2. Analysis on the temperature sensing indicated that the NaY(WO4)2:Er3+/Yb3+ serves well the solar cells as thermos-managing material. Moreover, it was confirmed that the fluorescence thermal quenching of 2H11/2/4S3/2 was caused by the nonradiative relaxation of 4S3/2. All the obtained results suggest that NaY(WO4)2:Er3+/Yb3+ is an excellent material for silicon-based solar cells to improve photoelectric conversion efficiency and thermal management.

提高光电转换效率和加强热管理是硅基太阳能电池的两大关键问题。在这项工作中,通过调整 Er3+ 和 Yb3+ 的浓度,证明了量子切割和上转换产生的高效 Yb3+ 红外发射,并在 Er3+/Yb3+ 共掺杂钨酸盐体系中发现了基于两个超低热淬灭水平的发光强度比的热管理适用温度传感。量子切割机制被清晰地解密为从 Er3+ 到 Yb3+ 的两步能量转移过程。在 Föster-Dexter 理论、Judd-Ofelt 理论和能隙定律的框架下,确认了 NaY(WO4)2 中 Er3+ 所有感兴趣的 4 f 水平的两步能量传递效率、辐射和非辐射转变速率,并根据这些获得的效率和速率进一步确定了 NaY(WO4)2: 5 mol% Er3+/50 mol% Yb3+ 样品中的量子切割效率高达 173%。通过调节 Yb3+ 掺杂浓度,在 Er3+/Yb3+ 共掺杂 NaY(WO4)2 中实现了 Yb3+ 在 1550 nm 激发下强烈且近乎纯净的红外上转换发射。Yb3+ 诱导的红外上转换发射增强归因于 4I11/2 (Er3+) + 2F7/2 (Yb3+) → 4I15/2 (Er3+) + 2F5/2 (Yb3+) 的高效能量转移和 4I9/2 的巨大非辐射弛豫速率。温度传感分析表明,NaY(WO4)2:Er3+/Yb3+ 能很好地将太阳能电池用作热管理材料。此外,还证实了 2H11/2/4S3/2 的荧光热淬灭是由 4S3/2 的非辐射弛豫引起的。所有这些结果表明,NaY(WO4)2:Er3+/Yb3+ 是硅基太阳能电池的一种优良材料,可提高光电转换效率和热管理性能。
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引用次数: 0
Color liquid crystal grating based color holographic 3D display system with large viewing angle. 基于彩色液晶光栅的大视角彩色全息 3D 显示系统。
IF 19.4 1区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2024-01-15 DOI: 10.1038/s41377-023-01375-0
Di Wang, Yi-Long Li, Fan Chu, Nan-Nan Li, Zhao-Song Li, Sin-Doo Lee, Zhong-Quan Nie, Chao Liu, Qiong-Hua Wang

Holographic 3D display is highly desirable for numerous applications ranging from medical treatments to military affairs. However, it is challenging to simultaneously achieve large viewing angle and high-fidelity color reconstruction due to the intractable constraints of existing technology. Here, we conceptually propose and experimentally demonstrate a simple and feasible pathway of using a well-designed color liquid crystal grating to overcome the inevitable chromatic aberration and enlarge the holographic viewing angle, thus enabling large-viewing-angle and color holographic 3D display. The use of color liquid crystal grating allows performing secondary diffraction modulation on red, green and blue reproduced images simultaneously and extending the viewing angle in the holographic 3D display system. In principle, a chromatic aberration-free hologram generation mechanism in combination with the color liquid crystal grating is proposed to pave the way for on such a superior holographic 3D display. The proposed system shows a color viewing angle of ~50.12°, which is about 7 times that of the traditional system with a single spatial light modulator. This work presents a paradigm for achieving desirable holographic 3D display, and is expected to provide a new way for the wide application of holographic display.

全息三维显示在从医疗到军事等众多应用领域都非常受欢迎。然而,由于现有技术难以解决的限制,要同时实现大视角和高保真色彩重建具有挑战性。在此,我们从概念上提出并通过实验证明了一种简单可行的途径,即利用精心设计的彩色液晶光栅克服不可避免的色差,扩大全息视角,从而实现大视角和彩色全息三维显示。使用彩色液晶光栅可以同时对红色、绿色和蓝色再现图像进行二次衍射调制,并扩大全息 3D 显示系统的视角。从原理上讲,结合彩色液晶光栅的无色差全息图生成机制的提出,为这种卓越的全息三维显示系统铺平了道路。拟议系统的彩色视角约为 50.12°,是使用单一空间光调制器的传统系统的 7 倍。这项工作为实现理想的全息三维显示提出了一种范例,有望为全息显示的广泛应用提供一条新路。
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引用次数: 0
Highly efficient and aberration-free off-plane grating spectrometer and monochromator for EUV-soft X-ray applications. 用于超紫外软 X 射线应用的高效无像差平面外光栅光谱仪和单色仪。
IF 19.4 1区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2024-01-08 DOI: 10.1038/s41377-023-01342-9
Jie Li, Kui Li, Xiaoshi Zhang, Dimitar Popmintchev, Hao Xu, Yutong Wang, Ruixuan Li, Guangyin Zhang, Jiyue Tang, Jin Niu, Yongjun Ma, Runyu Meng, Changjun Ke, Jisi Qiu, Yunfeng Ma, Tenio Popmintchev, Zhongwei Fan

We demonstrate a novel flat-field, dual-optic imaging EUV-soft X-ray spectrometer and monochromator that attains an unprecedented throughput efficiency exceeding 60% by design, along with a superb spectral resolution of λ/Δλ > 200 accomplished without employing variable line spacing gratings. Exploiting the benefits of the conical diffraction geometry, the optical system is globally optimized in multidimensional parameter space to guarantee optimal imaging performance over a broad spectral range while maintaining circular and elliptical polarization states at the first, second, and third diffraction orders. Moreover, our analysis indicates minimal temporal dispersion, with pulse broadening confined within 80 fs tail-to-tail and an FWHM value of 29 fs, which enables ultrafast spectroscopic and pump-probe studies with femtosecond accuracy. Furthermore, the spectrometer can be effortlessly transformed into a monochromator spanning the EUV-soft X-ray spectral region using a single grating with an aberration-free spatial profile. Such capability allows coherent diffractive imaging applications to be conducted with highly monochromatic light in a broad spectral range and extended to the soft X-ray region with minimal photon loss, thus facilitating state-of-the-art imaging of intricate nano- and bio-systems, with a significantly enhanced spatiotemporal resolution, down to the nanometer-femtosecond level.

我们展示了一种新颖的平场双光学成像超紫外软X射线光谱仪和单色仪,其设计实现了前所未有的超过60%的吞吐效率,同时在不使用可变线间距光栅的情况下实现了λ/Δλ > 200的超高光谱分辨率。利用锥形衍射几何的优势,光学系统在多维参数空间中进行了全局优化,以确保在宽光谱范围内实现最佳成像性能,同时在第一、第二和第三衍射阶保持圆偏振和椭圆偏振状态。此外,我们的分析表明时间色散极小,脉冲展宽限制在 80 fs 尾对尾范围内,FWHM 值为 29 fs,从而实现了飞秒级精度的超快光谱和泵探研究。此外,该光谱仪还可以毫不费力地转化为单色仪,使用无像差空间轮廓的单个光栅,横跨超紫外-软 X 射线光谱区域。这种能力使相干衍射成像应用能够在宽光谱范围内使用高度单色光,并以最小的光子损耗扩展到软 X 射线区域,从而促进对复杂的纳米和生物系统进行最先进的成像,并显著提高时空分辨率,达到纳米-飞秒级别。
{"title":"Highly efficient and aberration-free off-plane grating spectrometer and monochromator for EUV-soft X-ray applications.","authors":"Jie Li, Kui Li, Xiaoshi Zhang, Dimitar Popmintchev, Hao Xu, Yutong Wang, Ruixuan Li, Guangyin Zhang, Jiyue Tang, Jin Niu, Yongjun Ma, Runyu Meng, Changjun Ke, Jisi Qiu, Yunfeng Ma, Tenio Popmintchev, Zhongwei Fan","doi":"10.1038/s41377-023-01342-9","DOIUrl":"10.1038/s41377-023-01342-9","url":null,"abstract":"<p><p>We demonstrate a novel flat-field, dual-optic imaging EUV-soft X-ray spectrometer and monochromator that attains an unprecedented throughput efficiency exceeding 60% by design, along with a superb spectral resolution of λ/Δλ > 200 accomplished without employing variable line spacing gratings. Exploiting the benefits of the conical diffraction geometry, the optical system is globally optimized in multidimensional parameter space to guarantee optimal imaging performance over a broad spectral range while maintaining circular and elliptical polarization states at the first, second, and third diffraction orders. Moreover, our analysis indicates minimal temporal dispersion, with pulse broadening confined within 80 fs tail-to-tail and an FWHM value of 29 fs, which enables ultrafast spectroscopic and pump-probe studies with femtosecond accuracy. Furthermore, the spectrometer can be effortlessly transformed into a monochromator spanning the EUV-soft X-ray spectral region using a single grating with an aberration-free spatial profile. Such capability allows coherent diffractive imaging applications to be conducted with highly monochromatic light in a broad spectral range and extended to the soft X-ray region with minimal photon loss, thus facilitating state-of-the-art imaging of intricate nano- and bio-systems, with a significantly enhanced spatiotemporal resolution, down to the nanometer-femtosecond level.</p>","PeriodicalId":18093,"journal":{"name":"Light, science & applications","volume":"13 1","pages":"12"},"PeriodicalIF":19.4,"publicationDate":"2024-01-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10772113/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"139377949","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Exceptional dynamics at exceptional points. 特殊点上的特殊动力
IF 19.4 1区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2024-01-08 DOI: 10.1038/s41377-023-01347-4
Wenjie Wan

Exceptional points (EPs), singularities of non-Hermitian systems, often exhibit exotic behaviors by engineering the balance between the system gain and loss. Now, EPs have been demonstrated to enable unidirectional perfect absorption/reflection at the visible light spectrum.

异常点(EPs)是非赫米特系统的奇异点,通常通过对系统增益和损耗之间的平衡进行工程设计而表现出奇特的行为。现在,EP 已被证明能够在可见光光谱下实现单向完美吸收/反射。
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引用次数: 0
Twisted microdomains in liquid crystals for polarization-insensitive phase modulation. 用于偏振不敏感相位调制的液晶中的扭曲微域。
IF 19.4 1区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2024-01-05 DOI: 10.1038/s41377-023-01351-8
Yifei Ma, Zimo Zhao, Stephen M Morris, Chao He

Polarization-independent phase modulators based upon liquid crystals (LCs) with a simple device architecture have long been desired for a range of optical applications. Recently, researchers have demonstrated a novel fabrication procedure using cholesteric LCs as a primer for achieving low polarization dependence coupled with a large phase modulation depth.

基于液晶(LC)的偏振无关相位调制器具有简单的器件结构,长期以来一直是各种光学应用的理想之选。最近,研究人员展示了一种新颖的制造程序,以胆固醇液晶为引子,实现了低偏振依赖性和大相位调制深度。
{"title":"Twisted microdomains in liquid crystals for polarization-insensitive phase modulation.","authors":"Yifei Ma, Zimo Zhao, Stephen M Morris, Chao He","doi":"10.1038/s41377-023-01351-8","DOIUrl":"10.1038/s41377-023-01351-8","url":null,"abstract":"<p><p>Polarization-independent phase modulators based upon liquid crystals (LCs) with a simple device architecture have long been desired for a range of optical applications. Recently, researchers have demonstrated a novel fabrication procedure using cholesteric LCs as a primer for achieving low polarization dependence coupled with a large phase modulation depth.</p>","PeriodicalId":18093,"journal":{"name":"Light, science & applications","volume":"13 1","pages":"8"},"PeriodicalIF":19.4,"publicationDate":"2024-01-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10766621/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"139098149","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Cavity-enhanced photoacoustic dual-comb spectroscopy. 腔体增强型光声双梳光谱学。
IF 19.4 1区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2024-01-05 DOI: 10.1038/s41377-023-01353-6
Zhen Wang, Qinxue Nie, Haojia Sun, Qiang Wang, Simone Borri, Paolo De Natale, Wei Ren

Photoacoustic dual-comb spectroscopy (DCS), converting spectral information in the optical frequency domain to the audio frequency domain via multi-heterodyne beating, enables background-free spectral measurements with high resolution and broad bandwidth. However, the detection sensitivity remains limited due to the low power of individual comb lines and the lack of broadband acoustic resonators. Here, we develop cavity-enhanced photoacoustic DCS, which overcomes these limitations by using a high-finesse optical cavity for the power amplification of dual-frequency combs and a broadband acoustic resonator with a flat-top frequency response. We demonstrate high-resolution spectroscopic measurements of trace amounts of C2H2, NH3 and CO in the entire telecommunications C-band. The method shows a minimum detection limit of 0.6 ppb C2H2 at the measurement time of 100 s, corresponding to the noise equivalent absorption coefficient of 7 × 10-10 cm-1. The proposed cavity-enhanced photoacoustic DCS may open new avenues for ultrasensitive, high-resolution, and multi-species gas detection with widespread applications.

光声双梳状光谱(DCS)通过多外差跳动将光学频域的光谱信息转换到音频频域,从而实现了高分辨率和宽带宽的无背景光谱测量。然而,由于单个梳状线的功率较低,且缺乏宽带声共振,因此探测灵敏度仍然有限。在此,我们开发了空腔增强型光声 DCS,通过使用高精细度光腔对双频梳状线进行功率放大,以及使用具有平顶频率响应的宽带声学谐振器,克服了这些限制。我们展示了在整个电信 C 波段对痕量 C2H2、NH3 和 CO 的高分辨率光谱测量。测量时间为 100 秒时,该方法的最低检测限为 0.6 ppb C2H2,对应的噪声等效吸收系数为 7 × 10-10 cm-1。所提出的空腔增强型光声 DCS 可为超灵敏、高分辨率和多种类气体检测开辟新的途径,具有广泛的应用前景。
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引用次数: 0
Ultra-simplified diffraction-based computational spectrometer. 基于衍射的超简化计算光谱仪。
IF 19.4 1区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2024-01-05 DOI: 10.1038/s41377-023-01355-4
Chuangchuang Chen, Honggang Gu, Shiyuan Liu

Miniaturizing spectrometers for compact and cost-effective mobile platforms is a major challenge in current spectroscopy research, where conventional spectrometers are impractical due to their bulky footprint. Existing miniaturized designs primarily rely on precalibrated response functions of nanophotonic structures to encode spectral information captured in a snapshot by detector arrays. Accurate spectrum reconstruction is achieved through computational techniques, but this requires precise component design, high-precision fabrication, and calibration. We propose an ultra-simplified computational spectrometer that employs a one-to-broadband diffraction decomposition strategy facilitated by a numerical regularized transform that depends only on the spectrum of the diffracted radiation. The key feature of our design is the use of a simple, arbitrarily shaped pinhole as the partial disperser, eliminating the need for complex encoding designs and full spectrum calibration. Our spectrometer achieves a reconstructed spectral peak location accuracy of better than 1 nm over a 200 nm bandwidth and excellent resolution for peaks separated by 3 nm in a bimodal spectrum, all within a compact footprint of under half an inch. Notably, our approach also reveals a breakthrough in broadband coherent diffractive imaging without requiring any prior knowledge of the broadband illumination spectrum, assumptions of non-dispersive specimens, or correction for detector quantum efficiency.

在当前的光谱学研究中,将光谱仪小型化以用于结构紧凑、成本效益高的移动平台是一项重大挑战,传统的光谱仪由于体积庞大而不实用。现有的小型化设计主要依靠纳米光子结构的预校准响应函数来编码探测器阵列在快照中捕捉到的光谱信息。精确的光谱重构可通过计算技术实现,但这需要精确的元件设计、高精度制造和校准。我们提出了一种超简化计算光谱仪,该光谱仪采用单带到宽带衍射分解策略,通过数值正则化变换实现,而数值正则化变换只取决于衍射辐射的光谱。我们设计的主要特点是使用一个简单、任意形状的针孔作为部分分散器,从而无需复杂的编码设计和全光谱校准。我们的光谱仪在 200 nm 的带宽范围内实现了优于 1 nm 的重建光谱峰定位精度,并对双峰光谱中相距 3 nm 的峰实现了出色的分辨率,所有这一切都在不到半英寸的紧凑尺寸内完成。值得注意的是,我们的方法还在宽带相干衍射成像方面取得了突破性进展,而无需事先了解宽带照明光谱、假定样品为非色散样品或对探测器量子效率进行校正。
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引用次数: 0
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Light, science & applications
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