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Correlated optical convolutional neural network with "quantum speedup". 具有 "量子加速 "功能的相关光学卷积神经网络
IF 19.4 1区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2024-01-31 DOI: 10.1038/s41377-024-01376-7
Yifan Sun, Qian Li, Ling-Jun Kong, Xiangdong Zhang

Compared with electrical neural networks, optical neural networks (ONNs) have the potentials to break the limit of the bandwidth and reduce the consumption of energy, and therefore draw much attention in recent years. By far, several types of ONNs have been implemented. However, the current ONNs cannot realize the acceleration as powerful as that indicated by the models like quantum neural networks. How to construct and realize an ONN with the quantum speedup is a huge challenge. Here, we propose theoretically and demonstrate experimentally a new type of optical convolutional neural network by introducing the optical correlation. It is called the correlated optical convolutional neural network (COCNN). We show that the COCNN can exhibit "quantum speedup" in the training process. The character is verified from the two aspects. One is the direct illustration of the faster convergence by comparing the loss function curves of the COCNN with that of the traditional convolutional neural network (CNN). Such a result is compatible with the training performance of the recently proposed quantum convolutional neural network (QCNN). The other is the demonstration of the COCNN's capability to perform the QCNN phase recognition circuit, validating the connection between the COCNN and the QCNN. Furthermore, we take the COCNN analog to the 3-qubit QCNN phase recognition circuit as an example and perform an experiment to show the soundness and the feasibility of it. The results perfectly match the theoretical calculations. Our proposal opens up a new avenue for realizing the ONNs with the quantum speedup, which will benefit the information processing in the era of big data.

与电神经网络相比,光神经网络(ONNs)具有突破带宽限制和降低能耗的潜力,因此近年来备受关注。迄今为止,已有多种类型的光神经网络得以实现。然而,目前的 ONN 无法实现量子神经网络等模型所显示的强大加速能力。如何构建并实现量子加速的 ONN 是一个巨大的挑战。在此,我们从理论上提出并通过实验证明了一种引入光相关性的新型光卷积神经网络。它被称为相关光卷积神经网络(COCNN)。我们证明,COCNN 在训练过程中可以表现出 "量子加速"。我们从两个方面验证了这一特性。一是通过比较 COCNN 与传统卷积神经网络(CNN)的损失函数曲线,直接说明了收敛速度更快。这一结果与最近提出的量子卷积神经网络(QCNN)的训练性能相吻合。另一方面,COCNN 演示了执行 QCNN 相位识别电路的能力,验证了 COCNN 与 QCNN 之间的联系。此外,我们还以 COCNN 模拟 3 量子位 QCNN 相位识别电路为例,进行了实验,以证明其合理性和可行性。实验结果与理论计算结果完全吻合。我们的建议为实现量子加速的ONNs开辟了一条新途径,这将有利于大数据时代的信息处理。
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引用次数: 0
A new route towards polarized luminescence: 0D/2D nanocomposites. 实现极化发光的新途径:0D/2D 纳米复合材料。
IF 19.4 1区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2024-01-31 DOI: 10.1038/s41377-023-01370-5
Andries Meijerink

Combining wide bandgap 2D inorganic materials and blue-light-emitting 0D carbon dots in 0D/2D heterojunction nanocomposites was shown to give rise to unique optical properties and a multifunctional prototype device was developed, capable of polarized light luminescence, modulation and detection.

研究表明,将宽带隙二维无机材料与发射蓝光的 0D 碳点结合在 0D/2D 异质结纳米复合材料中,可产生独特的光学特性,并开发出一种多功能原型器件,能够进行偏振光发光、调制和检测。
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引用次数: 0
Observation of transition from superfluorescence to polariton condensation in CsPbBr3 quantum dots film. 观测 CsPbBr3 量子点薄膜从超荧光到极化子凝聚的转变。
IF 19.4 1区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2024-01-30 DOI: 10.1038/s41377-024-01378-5
Danqun Mao, Linqi Chen, Zheng Sun, Min Zhang, Zhe-Yu Shi, Yongsheng Hu, Long Zhang, Jian Wu, Hongxing Dong, Wei Xie, Hongxing Xu

The superfluorescence effect has received extensive attention due to the many-body physics of quantum correlation in dipole gas and the optical applications of ultrafast bright radiation field based on the cooperative quantum state. Here, we demonstrate not only to observe the superfluorescence effect but also to control the cooperative state of the excitons ensemble by externally applying a regulatory dimension of coupling light fields. A new quasi-particle called cooperative exciton-polariton is revealed in a light-matter hybrid structure of a perovskite quantum dot thin film spin-coated on a Distributed Bragg Reflector. Above the nonlinear threshold, polaritonic condensation occurs at a nonzero momentum state on the lower polariton branch owning to the vital role of the synchronized excitons. The phase transition from superfluorescence to polariton condensation exhibits typical signatures of a decrease of the linewidth, an increase of the macroscopic coherence as well as an accelerated radiation decay rate. These findings are promising for opening new potential applications for super-brightness and unconventional coherent light sources and could enable the exploitation of cooperative effects for quantum optics.

超荧光效应因偶极子气体中量子关联的多体物理学以及基于协同量子态的超快明亮辐射场的光学应用而受到广泛关注。在这里,我们不仅观察到了超荧光效应,还证明了通过外部施加耦合光场的调节维度来控制激子集合的合作态。在分布式布拉格反射器上自旋涂覆的过氧化物量子点薄膜的光-物质混合结构中,一种名为合作激子-极化子的新准粒子被揭示出来。在非线性阈值之上,由于同步激子的重要作用,在下极子分支的非零动量态发生了极子凝聚。从超荧光到极化子凝聚的相变表现出线宽减小、宏观相干性增强以及辐射衰减速率加快等典型特征。这些发现有望为超亮度和非常规相干光源开辟新的潜在应用领域,并能使量子光学利用合作效应成为可能。
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引用次数: 0
Vectorial adaptive optics: expanding the frontiers of optical correction. 矢量自适应光学:拓展光学校正的前沿。
IF 19.4 1区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2024-01-30 DOI: 10.1038/s41377-023-01358-1
Qiming Zhang, Min Gu

Researchers at the University of Oxford have introduced a groundbreaking technique called vectorial adaptive optics (V-AO), which extends the capabilities of traditional adaptive optics to correct for both polarization and phase aberrations. This novel approach opens new possibilities for manipulating the complex vectorial field in optical systems, enabling higher-dimensional feedback correction.

牛津大学的研究人员推出了一种名为矢量自适应光学(V-AO)的开创性技术,它扩展了传统自适应光学的功能,可同时校正偏振和相位像差。这种新颖的方法为操纵光学系统中的复杂矢量场提供了新的可能性,实现了更高维度的反馈校正。
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引用次数: 0
Radiative loss of coherence in free electrons: a long-range quantum phenomenon. 自由电子相干性的辐射损失:一种长程量子现象。
IF 19.4 1区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2024-01-26 DOI: 10.1038/s41377-023-01361-6
Cruz I Velasco, Valerio Di Giulio, F Javier García de Abajo

Quantum physics rules the dynamics of small objects as they interact over microscopic length scales. Nevertheless, quantum correlations involving macroscopic distances can be observed between entangled photons as well as in atomic gases and matter waves at low temperatures. The long-range nature of the electromagnetic coupling between charged particles and extended objects could also trigger quantum phenomena over large distances. Here, we reveal a manifestation of quantum mechanics that involves macroscopic distances and results in a nearly complete depletion of coherence associated with which-way free-electron interference produced by electron-radiation coupling in the presence of distant extended objects. This is a ubiquitous effect that we illustrate through a rigorous theoretical analysis of a two-path electron beam interacting with a semi-infinite metallic plate and find the inter-path coherence to vanish proportionally to the path separation at zero temperature and exponentially at finite temperature. The investigated regime of large distances originates in the coupling of the electron to radiative modes assisted by diffraction at material structures but without any involvement of material excitations. Besides the fundamental interest of this macroscopic quantum phenomenon, our results suggest an approach to measuring the vacuum temperature and nondestructively sensing the presence of distant objects.

量子物理学规定了小物体在微观长度尺度上相互作用时的动力学。然而,在纠缠光子之间以及低温下的原子气体和物质波中,可以观察到涉及宏观距离的量子相关性。带电粒子和扩展物体之间电磁耦合的长程性质也可能引发大距离的量子现象。在这里,我们揭示了量子力学的一种表现形式,它涉及到宏观距离,并导致与电子辐射耦合产生的自由电子干涉相关的相干性几乎完全耗尽。我们通过对与半无限金属板相互作用的双路径电子束进行严格的理论分析来说明这种无处不在的效应,发现路径间的相干性在零温度下与路径分离成比例消失,而在有限温度下呈指数消失。所研究的大距离机制源于电子与辐射模式的耦合,该耦合由材料结构的衍射辅助,但不涉及任何材料激发。除了对这一宏观量子现象的基本兴趣之外,我们的研究结果还提出了一种测量真空温度和非破坏性地感知遥远物体存在的方法。
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引用次数: 0
Spatio-temporal coupled mode theory for nonlocal metasurfaces. 非局部元曲面的时空耦合模式理论
IF 19.4 1区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2024-01-24 DOI: 10.1038/s41377-023-01350-9
Adam Overvig, Sander A Mann, Andrea Alù

Diffractive nonlocal metasurfaces have recently opened a broad range of exciting developments in nanophotonics research and applications, leveraging spatially extended-yet locally patterned-resonant modes to control light with new degrees of freedom. While conventional grating responses are elegantly captured by temporal coupled mode theory, current approaches are not well equipped to capture the arbitrary spatial response observed in the nascent field of nonlocal metasurfaces. Here, we introduce spatio-temporal coupled mode theory (STCMT), capable of elegantly capturing the key features of the resonant response of wavefront-shaping nonlocal metasurfaces. This framework can quantitatively guide nonlocal metasurface design while maintaining compatibility with local metasurface frameworks, making it a powerful tool to rationally design and optimize a broad class of ultrathin optical components. We validate this STCMT framework against full-wave simulations of various nonlocal metasurfaces, demonstrating that this tool offers a powerful semi-analytical framework to understand and model the physics and functionality of these devices, without the need for computationally intense full-wave simulations. We also discuss how this model may shed physical insights into nonlocal phenomena in photonics and the functionality of the resulting devices. As a relevant example, we showcase STCMT's flexibility by applying it to study and rapidly prototype nonlocal metasurfaces that spatially shape thermal emission.

衍射非局部元表面最近在纳米光子学研究和应用领域取得了令人兴奋的广泛发展,利用空间扩展但局部图案化的共振模式,以新的自由度控制光。时间耦合模式理论可以优雅地捕捉传统光栅的响应,但目前的方法还不能很好地捕捉非局部元表面这一新兴领域中观察到的任意空间响应。在这里,我们引入了时空耦合模式理论(STCMT),它能够优雅地捕捉波前成形非局部元表面共振响应的关键特征。该框架可定量指导非局部元表面设计,同时与局部元表面框架保持兼容,是合理设计和优化各类超薄光学元件的有力工具。我们根据各种非局部元表面的全波模拟验证了 STCMT 框架,证明该工具提供了一个强大的半分析框架,可用于理解和模拟这些器件的物理和功能,而无需进行计算量巨大的全波模拟。我们还讨论了这一模型如何为光子学中的非局部现象以及由此产生的设备功能提供物理启示。作为一个相关实例,我们将 STCMT 应用于研究和快速原型非局部元表面,从而展示了 STCMT 的灵活性。
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引用次数: 0
Geometric phase-encoded stimuli-responsive cholesteric liquid crystals for visualizing real-time remote monitoring: humidity sensing as a proof of concept. 用于可视化实时远程监控的几何相位编码刺激响应胆甾型液晶:湿度传感概念验证。
IF 19.4 1区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2024-01-24 DOI: 10.1038/s41377-023-01360-7
Shi-Long Li, Zhao-Yi Chen, Peng Chen, Wei Hu, Chaohong Huang, Sen-Sen Li, Xuejia Hu, Yan-Qing Lu, Lu-Jian Chen

Liquid crystals are a vital component of modern photonics, and recent studies have demonstrated the exceptional sensing properties of stimuli-responsive cholesteric liquid crystals. However, existing cholesteric liquid crystal-based sensors often rely on the naked eye perceptibility of structural color or the measurement of wavelength changes by spectrometric tools, which limits their practical applications. Therefore, developing a platform that produces recognizable sensing signals is critical. In this study, we present a visual sensing platform based on geometric phase encoding of stimuli-responsive cholesteric liquid crystal polymers that generates real-time visual patterns, rather than frequency changes. To demonstrate this platform's effectiveness, we used a humidity-responsive cholesteric liquid crystal polymer film encoded with a q-plate pattern, which revealed that humidity causes a shape change in the vortex beam reflected from the encoded cholesteric liquid crystal polymers. Moreover, we developed a prototype platform towards remote humidity monitoring benefiting from the high directionality and long-range transmission properties of laser beams carrying orbital angular momentum. Our approach provides a novel sensing platform for cholesteric liquid crystals-based sensors that offers promising practical applications. The ability to generate recognizable sensing signals through visual patterns offers a new level of practicality in the sensing field with stimuli-responsive cholesteric liquid crystals. This platform might have significant implications for a broad readership and will be of interest to researchers working in the field of photonics and sensing technology.

液晶是现代光子学的重要组成部分,最近的研究已经证明了刺激响应型胆甾液晶的卓越传感特性。然而,现有的基于胆甾型液晶的传感器通常依赖于肉眼对结构颜色的感知,或通过光谱工具对波长变化的测量,这限制了它们的实际应用。因此,开发一种能产生可识别传感信号的平台至关重要。在本研究中,我们提出了一种基于刺激响应型胆甾液晶聚合物几何相位编码的视觉传感平台,它能产生实时视觉图案,而不是频率变化。为了证明这一平台的有效性,我们使用了一种用 q 板图案编码的湿度响应型胆甾液晶聚合物薄膜,结果表明湿度会导致编码胆甾液晶聚合物反射的涡流光束发生形状变化。此外,我们还利用携带轨道角动量的激光束的高方向性和远距离传输特性,开发了一个用于远程湿度监测的原型平台。我们的方法为基于胆甾液晶的传感器提供了一种新型传感平台,具有广阔的实际应用前景。通过视觉图案产生可识别传感信号的能力为刺激响应型胆甾液晶传感领域的实用性提供了一个新的高度。该平台可能会对广大读者产生重大影响,光子学和传感技术领域的研究人员也会对此感兴趣。
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引用次数: 0
Operando monitoring of dendrite formation in lithium metal batteries via ultrasensitive tilted fiber Bragg grating sensors. 通过超灵敏倾斜光纤布拉格光栅传感器对锂金属电池中树枝状晶粒的形成进行操作性监测。
IF 19.4 1区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2024-01-22 DOI: 10.1038/s41377-023-01346-5
Xile Han, Hai Zhong, Kaiwei Li, Xiaobin Xue, Wen Wu, Nan Hu, Xihong Lu, Jiaqiang Huang, Gaozhi Xiao, Yaohua Mai, Tuan Guo

Lithium (Li) dendrite growth significantly deteriorates the performance and shortens the operation life of lithium metal batteries. Capturing the intricate dynamics of surface localized and rapid mass transport at the electrolyte-electrode interface of lithium metal is essential for the understanding of the dendrite growth process, and the evaluation of the solutions mitigating the dendrite growth issue. Here we demonstrate an approach based on an ultrasensitive tilted fiber Bragg grating (TFBG) sensor which is inserted close to the electrode surface in a working lithium metal battery, without disturbing its operation. Thanks to the superfine optical resonances of the TFBG, in situ and rapid monitoring of mass transport kinetics and lithium dendrite growth at the nanoscale interface of lithium anodes have been achieved. Reliable correlations between the performance of different natural/artificial solid electrolyte interphases (SEIs) and the time-resolved optical responses have been observed and quantified, enabling us to link the nanoscale ion and SEI behavior with the macroscopic battery performance. This new operando tool will provide additional capabilities for parametrization of the batteries' electrochemistry and help identify the optimal interphases of lithium metal batteries to enhance battery performance and its safety.

锂(Li)枝晶的生长会严重降低锂金属电池的性能并缩短其使用寿命。捕捉锂金属电解质-电极界面表面局部快速质量传输的复杂动态,对于理解枝晶生长过程和评估缓解枝晶生长问题的解决方案至关重要。在此,我们展示了一种基于超灵敏倾斜光纤布拉格光栅(TFBG)传感器的方法,该传感器可插入工作中的锂金属电池电极表面附近,且不会干扰电池的运行。借助 TFBG 的超精细光学共振,实现了对锂阳极纳米级界面的质量传输动力学和锂枝晶生长的现场快速监测。我们观察并量化了不同天然/人工固态电解质相间层(SEI)的性能与时间分辨光学响应之间的可靠相关性,使我们能够将纳米级离子和 SEI 行为与宏观电池性能联系起来。这一新的操作工具将为电池电化学参数化提供更多能力,并有助于确定锂金属电池的最佳相间层,从而提高电池性能和安全性。
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引用次数: 0
Tantalum pentoxide: a new material platform for high-performance dielectric metasurface optics in the ultraviolet and visible region. 五氧化钽:紫外线和可见光区域高性能介电元表面光学的新材料平台。
IF 19.4 1区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2024-01-22 DOI: 10.1038/s41377-023-01330-z
Cheng Zhang, Lu Chen, Zhelin Lin, Junyeob Song, Danyan Wang, Moxin Li, Okan Koksal, Zi Wang, Grisha Spektor, David Carlson, Henri J Lezec, Wenqi Zhu, Scott Papp, Amit Agrawal

Dielectric metasurfaces, composed of planar arrays of subwavelength dielectric structures that collectively mimic the operation of conventional bulk optical elements, have revolutionized the field of optics by their potential in constructing high-efficiency and multi-functional optoelectronic systems on chip. The performance of a dielectric metasurface is largely determined by its constituent material, which is highly desired to have a high refractive index, low optical loss and wide bandgap, and at the same time, be fabrication friendly. Here, we present a new material platform based on tantalum pentoxide (Ta2O5) for implementing high-performance dielectric metasurface optics over the ultraviolet and visible spectral region. This wide-bandgap dielectric, exhibiting a high refractive index exceeding 2.1 and negligible extinction coefficient across a broad spectrum, can be easily deposited over large areas with good quality using straightforward physical vapor deposition, and patterned into high-aspect-ratio subwavelength nanostructures through commonly-available fluorine-gas-based reactive ion etching. We implement a series of high-efficiency ultraviolet and visible metasurfaces with representative light-field modulation functionalities including polarization-independent high-numerical-aperture lensing, spin-selective hologram projection, and vivid structural color generation, and the devices exhibit operational efficiencies up to 80%. Our work overcomes limitations faced by scalability of commonly-employed metasurface dielectrics and their operation into the visible and ultraviolet spectral range, and provides a novel route towards realization of high-performance, robust and foundry-manufacturable metasurface optics.

介电元表面由亚波长介电结构平面阵列组成,可共同模拟传统体光学元件的工作原理,在构建高效多功能片上光电系统方面具有巨大潜力,为光学领域带来了革命性的变化。介电元表面的性能很大程度上取决于其组成材料,人们非常希望它具有高折射率、低光学损耗和宽带隙,同时又便于制造。在此,我们提出了一种基于五氧化二钽(Ta2O5)的新材料平台,用于实现紫外和可见光谱区的高性能介电元表面光学器件。这种宽带隙电介质具有超过 2.1 的高折射率和在宽光谱范围内可忽略不计的消光系数,可通过简单的物理气相沉积法轻松实现大面积高质量沉积,并可通过常用的基于氟气的反应离子刻蚀法将其图案化为高光谱比的亚波长纳米结构。我们实现了一系列具有代表性光场调制功能的高效紫外线和可见光超表面,包括偏振无关的高数值孔径透镜、自旋选择性全息投影和生动的结构色彩生成,这些器件的运行效率高达 80%。我们的工作克服了常用超表面电介质的可扩展性及其在可见光和紫外光谱范围内运行所面临的限制,为实现高性能、坚固耐用和可代工制造的超表面光学器件提供了一条新的途径。
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引用次数: 0
Waveguide-based augmented reality displays: a highlight. 基于波导的增强现实显示器:亮点。
IF 19.4 1区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2024-01-18 DOI: 10.1038/s41377-023-01371-4
Jannick P Rolland, Jeremy Goodsell

Augmented reality (AR), which emerged in the 1960s, remains a focal point of interest given its capacity to overlay the real world with digitally presented information through optical combiners. The prevalent combiner, commonly known as the waveguide in the AR literature, is prized for its compact design and generous eyebox-essential elements in human-centric technology. Nonetheless, these combiners encounter unique challenges in meeting various other requirements of the human visual system. This paper highlights a recent review of technological advancements and presents a forward-looking perspective on the future of AR technology.

20 世纪 60 年代兴起的增强现实(AR)技术,通过光学合路器将数字信息叠加到现实世界中,因此一直是人们关注的焦点。普遍使用的合路器(在增强现实技术文献中通常称为波导)因其紧凑的设计和宽敞的眼罩而备受推崇,这些都是以人为本的技术中必不可少的元素。然而,这些合路器在满足人类视觉系统的其他各种要求方面遇到了独特的挑战。本文重点回顾了最近的技术进步,并从前瞻性的角度展望了 AR 技术的未来。
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引用次数: 0
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Light, science & applications
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