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Charged organic ligands inserting/supporting the nanolayer spacing of vanadium oxides for high-stability/efficiency zinc-ion batteries. 带电有机配体插入/支撑钒氧化物纳米层间距，用于高稳定性/高效率锌离子电池。
IF 16.3 1区 综合性期刊 Q1 MULTIDISCIPLINARY SCIENCES
National Science Review
Pub Date : 2024-09-20 eCollection Date: 2024-10-01 DOI: 10.1093/nsr/nwae336
Guoqiang Yuan, Yichun Su, Xiangling Zhang, Biao Gao, Jinliang Hu, Yangyang Sun, Wenting Li, Zhan Zhang, Mohsen Shakouri, Huan Pang

Given their high safety, environmental friendliness and low cost, aqueous zinc-ion batteries (AZIBs) have the potential for high-performance energy storage. However, issues with the structural stability and electrochemical kinetics during discharge/charge limit the development of AZIBs. In this study, vanadium oxide electrodes with organic molecular intercalation were designed based on intercalating 11 kinds of charged organic carboxylic acid ligands between 2D layers to regulate the interlayer spacing. The negatively charged carboxylic acid group can neutralize Zn2+, reduce electrostatic repulsion and enhance electrochemical kinetics. The intercalated organic molecules increased the interlayer spacing. Among them, the 0.028EDTA · 0.28NH4 + · V2O5 · 0.069H2O was employed as the cathode with a high specific capacity (464.6 mAh g-1 at 0.5 A g-1) and excellent rate performance (324.4 mAh g-1 at 10 A g-1). Even at a current density of 20 A g-1, the specific capacity after 2000 charge/discharge cycles was 215.2 mAh g-1 (capacity retention of 78%). The results of this study demonstrate that modulation of the electrostatic repulsion and interlayer spacing through the intercalation of organic ligands can enhance the properties of vanadium-based materials.

锌离子水电池（AZIBs）具有安全性高、环保和成本低的特点，有望成为高性能的储能电池。然而，放电/充电过程中的结构稳定性和电化学动力学问题限制了 AZIB 的发展。本研究基于在二维层之间插层 11 种带电的有机羧酸配体来调节层间距，设计出了具有有机分子插层的氧化钒电极。带负电荷的羧酸基团可以中和 Zn2+，减少静电排斥，增强电化学动力学。插层有机分子增加了层间距。其中，0.028EDTA - 0.28NH4 + - V2O5 - 0.069H2O 被用作阴极，具有较高的比容量（0.5 A g-1 时为 464.6 mAh g-1）和优异的速率性能（10 A g-1 时为 324.4 mAh g-1）。即使在电流密度为 20 A g-1 时，经过 2000 次充放电循环后，比容量仍为 215.2 mAh g-1（容量保持率为 78%）。这项研究的结果表明，通过插层有机配体来调节静电排斥力和层间距，可以提高钒基材料的性能。
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引用次数: 0
Electron spins from a molecular perspective: an interview with Song Gao. 从分子角度看电子自旋：高松访谈录。
IF 16.3 1区 综合性期刊 Q1 MULTIDISCIPLINARY SCIENCES
National Science Review
Pub Date : 2024-09-14 eCollection Date: 2024-09-01 DOI: 10.1093/nsr/nwae327
Shang-Da Jiang, He Zhu

Spin chemistry has emerged as an interdisciplinary field that focuses on electron spins in molecules and related applications in physics, chemistry, biology, materials science and information science. It will play a crucial role in technological innovations. The chemistry of spins is deeply related to the essence of chemical bonds, chemical catalysis, enzyme catalysis, optical and electromagnetic properties, quantum computation and quantum precision measurements. The related research is intersectional, cutting-edge and has a wide range of application prospects. National Science Review (NSR) recently interviewed Prof. Song Gao to discuss spin chemistry. Prof. Gao is a renowned inorganic chemist and an academician of Chinese Academy of Sciences. He is the president of Sun Yat-sen University and the founder of the Spin-X Institute of South China University of Technology. He is recognized as a leader in coordination chemistry and molecular magnetism, and has strong academic influence. Since 2008, he has served on the International Advisory Committee of International Conference on Molecule-Based Magnets, and organized and chaired its 2010 conference. Prof. Gao's primary research topics include molecular nanomagnets; the relationship between geometric structures, electronic structures and magnetism of molecules; and the spin states and reactivity of molecules.

自旋化学是一个跨学科领域，主要研究分子中的电子自旋以及在物理学、化学、生物学、材料科学和信息科学中的相关应用。它将在技术创新中发挥至关重要的作用。自旋化学与化学键、化学催化、酶催化、光学和电磁特性、量子计算和量子精密测量的本质有着深刻的联系。相关研究具有交叉性、前沿性和广泛的应用前景。国家科学评论》（NSR）近日采访了高松教授，探讨自旋化学。高松教授是著名的无机化学家、中国科学院院士。他是中山大学校长，也是华南理工大学自旋X研究所的创始人。他是配位化学和分子磁学领域公认的领军人物，具有很强的学术影响力。自 2008 年以来，他一直担任国际分子磁会议国际顾问委员会委员，并组织和主持了 2010 年的会议。高教授的主要研究课题包括分子纳米磁体；分子的几何结构、电子结构和磁性之间的关系；分子的自旋态和反应性。
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引用次数: 0
Redox mediators towards practical aqueous batteries. 实现实用水电池的氧化还原媒介。
IF 16.3 1区 综合性期刊 Q1 MULTIDISCIPLINARY SCIENCES
National Science Review
Pub Date : 2024-09-10 eCollection Date: 2024-10-01 DOI: 10.1093/nsr/nwae320
Jiafeng Lei, Yi-Chun Lu
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引用次数: 0
The past, present and future of high-performance fibers. 高性能纤维的过去、现在和未来。
IF 16.3 1区 综合性期刊 Q1 MULTIDISCIPLINARY SCIENCES
National Science Review
Pub Date : 2024-09-04 eCollection Date: 2024-10-01 DOI: 10.1093/nsr/nwae310
Zhenzhen Liu, Yan Wang, Junrong Yu, Yinjun Chen, Meifang Zhu

This paper summarizes the recent progress of diverse high-performance fibers in their properties, applications and the challenges.

本文总结了各种高性能纤维在性能、应用和挑战方面的最新进展。
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引用次数: 0
Machine learning automation. 机器学习自动化。
IF 16.3 1区 综合性期刊 Q1 MULTIDISCIPLINARY SCIENCES
National Science Review
Pub Date : 2024-08-27 eCollection Date: 2024-08-01 DOI: 10.1093/nsr/nwae288
Zongben Xu, Zhi-Hua Zhou, Wenwu Zhu
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引用次数: 0
Sustainable catalysts for propylene synthesis. 丙烯合成的可持续催化剂。
IF 16.3 1区 综合性期刊 Q1 MULTIDISCIPLINARY SCIENCES
National Science Review
Pub Date : 2024-08-23 eCollection Date: 2024-09-01 DOI: 10.1093/nsr/nwae273
Mingyuan He
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引用次数: 0
Optimizing Cu electrocatalysis using programmed alternating current. 利用程序化交流电优化铜电催化。
IF 16.3 1区 综合性期刊 Q1 MULTIDISCIPLINARY SCIENCES
National Science Review
Pub Date : 2024-08-23 eCollection Date: 2024-09-01 DOI: 10.1093/nsr/nwae298
Jonathan Lei, Song Lin
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引用次数: 0
Approaches to tracing the geographic origin of wildlife trade. 追踪野生动植物贸易地理来源的方法。
IF 16.3 1区 综合性期刊 Q1 MULTIDISCIPLINARY SCIENCES
National Science Review
Pub Date : 2024-08-21 eCollection Date: 2024-09-01 DOI: 10.1093/nsr/nwae286
Tong Tong Gu, Hao Zhang, Yu Xin He, Jing Yang Hu, Li Yu
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引用次数: 0
Perspectives on phase engineering of nanomaterials. 纳米材料相工程的前景。
IF 16.3 1区 综合性期刊 Q1 MULTIDISCIPLINARY SCIENCES
National Science Review
Pub Date : 2024-08-20 eCollection Date: 2024-09-01 DOI: 10.1093/nsr/nwae289
Zhenyu Shi, Yuxuan Wu, Xinyang Ruan, Wei Zhai, Zijian Li, Li Zhai, An Zhang, Hua Zhang

This perspective highlights the representative progress of phase engineering of nanomaterials (PEN) with an emphasis on noble metals and transition metal dichalcogenides, and proposes future directions in this emerging field.

本视角着重介绍了纳米材料（PEN）相工程的代表性进展，重点是贵金属和过渡金属二钙化物，并提出了这一新兴领域的未来发展方向。
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引用次数: 0
Uncollected polythene fragments size-dependently alter soil multifunctionality via mediating bacterial drivers in dryland. 未收集的聚乙烯碎片通过介导旱地中的细菌驱动因素改变土壤的多功能性。
IF 16.3 1区 综合性期刊 Q1 MULTIDISCIPLINARY SCIENCES
National Science Review
Pub Date : 2024-08-16 eCollection Date: 2024-09-01 DOI: 10.1093/nsr/nwae281
Ze-Ying Zhao, Peng-Yang Wang, Xiao-Bin Xiong, Yinglong Chen, Hong-Yan Tao, Wen-Ying Wang, Yajie Song, Muhammad Ashraf, Li Zhu, Yun-Li Xiao, Shi-Sheng Li, Fang-Kun Yang, Meng-Ying Li, Jing Cao, Xiang-Wen Fang, Levis Kavagi, You-Cai Xiong
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引用次数: 0
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