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All-optical temporal logic gates in localized exciton polaritons 局部激子极化子中的全光时序逻辑门
IF 32.3 1区 物理与天体物理 Q1 OPTICS Pub Date : 2024-08-02 DOI: 10.1038/s41566-024-01483-2
Hui Li, Fei Chen, Haoyuan Jia, Ziyu Ye, Hang Zhou, Song Luo, Junheng Shi, Zhenrong Sun, Huailiang Xu, Hongxing Xu, Tim Byrnes, Zhanghai Chen, Jian Wu
Exciton polaritons—quasi-particle excitations consisting of strongly coupled photons and excitons—present fascinating possibilities for photonic circuits, owing to their strong nonlinearity, ultrafast reaction times and their ability to form macroscopic quantum states at room temperature via non-equilibrium condensation. Past implementations of transistors and logic gates with exciton polaritons have been mostly realized using the spatial propagation of polariton fluids, which place high demands on the fabrication of the microcavities and typically require complex manipulations. In this work we have implemented the full set of logical gate functionalities (that is, temporal AND, OR and NOT gates) in localized exciton polaritons at room temperature, on the basis of precisely controlling the interplay between polariton condensate and exciton reservoir dynamics, using a two-pulse excitation scheme. The dynamics intrinsically covers the cascadability required by the logical operations, enabling efficient information processing without the need for spatial flow. The temporal polariton logic gates demonstrate advantages in ultrafast switching, universality and simplified compatibility with other dimensional controls, showing great potential for building polariton logic networks in strongly coupled light–matter systems. Researchers have achieved AND, OR and NOT gates, using localized exciton polaritons at room temperature. The logic is based on temporal gates, rather than relying on the usual spatial propagation approaches.
激子极化子--由强耦合光子和激子组成的准粒子激发--由于其强烈的非线性、超快的反应时间以及在室温下通过非平衡凝聚形成宏观量子态的能力,为光子电路带来了迷人的可能性。以往利用激子极化子实现晶体管和逻辑门的方法大多是利用极化子流体的空间传播,这对微腔的制造提出了很高的要求,通常需要复杂的操作。在这项工作中,我们利用双脉冲激发方案,在精确控制极化子凝聚态和激子储库动态之间相互作用的基础上,在室温下实现了局部激子极化子的全套逻辑门功能(即时序 AND、OR 和 NOT 门)。该动力学本质上涵盖了逻辑运算所需的级联性,无需空间流即可实现高效的信息处理。时态极化子逻辑门在超快开关、通用性和与其他维度控制的简化兼容性方面表现出优势,显示出在强耦合光物质系统中构建极化子逻辑网络的巨大潜力。
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引用次数: 0
Highly efficient printed quantum dot light-emitting diodes through ultrahigh-definition double-layer transfer printing 通过超高清双层转印实现高效印刷量子点发光二极管
IF 35 1区 物理与天体物理 Q1 OPTICS Pub Date : 2024-08-02 DOI: 10.1038/s41566-024-01496-x
Jisu Yoo, Kyunghoon Lee, U. Jeong Yang, Hyeon Hwa Song, Jae Hong Jang, Gwang Heon Lee, Megalamane S. Bootharaju, Jun Hee Kim, Kiwook Kim, Soo Ik Park, Jung Duk Seo, Shi Li, Won Seok Yu, Jong Ik Kwon, Myoung Hoon Song, Taeghwan Hyeon, Jiwoong Yang, Moon Kee Choi

Highly efficient and high-definition displays with deformable form factors are highly desirable for next-generation electronic devices. Despite the unique advantages of quantum dots (QDs), including high photoluminescence quantum yield, wide colour range and high colour purity, developing a QD patterning process for high-definition pixels and efficient QD light-emitting diodes (QLEDs) is in its early stages. Here we present highly efficient QLEDs through ultrahigh-definition double-layer transfer printing of a QD/ZnO film. Surface engineering of viscoelastic stamps enables double-layer transfer printing that can create RGB pixelated patterns with 2,565 pixels per inch and monochromic QD patterns with ~20,526 pixels per inch. The close packing of both QDs and ZnO nanoparticles by double-layer transfer printing substantially minimizes the leakage current, enhancing the external quantum efficiency of our devices to 23.3%. Furthermore, we demonstrate highly efficient wearable QLEDs fabricated by our technique. This study paves the way for the development of highly efficient, full-colour QD displays via the transfer printing technique, demonstrating great promise for next-generation display technologies.

对于下一代电子设备来说,具有可变形外形尺寸的高效高清显示器是非常理想的。尽管量子点(QDs)具有独特的优势,包括高光致发光量子产率、宽色彩范围和高色彩纯度,但开发用于高清像素和高效 QD 发光二极管(QLEDs)的 QD 图案工艺仍处于早期阶段。在此,我们通过对 QD/ZnO 薄膜进行超高清双层转印,展示了高效 QLED。粘弹性印章的表面工程实现了双层转移印花,可以创建每英寸 2,565 像素的 RGB 像素图案和每英寸 ~20,526 像素的单色 QD 图案。通过双层转印,QDs 和 ZnO 纳米粒子紧密堆积,大大降低了泄漏电流,从而将我们器件的外部量子效率提高到 23.3%。此外,我们还展示了利用我们的技术制造的高效可穿戴 QLED。这项研究为通过转移印花技术开发高效全彩色 QD 显示器铺平了道路,为下一代显示技术带来了巨大前景。
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引用次数: 0
Prospects for free-electron lasers powered by plasma-wakefield-accelerated beams 由等离子唤醒加速束驱动的自由电子激光器的前景
IF 32.3 1区 物理与天体物理 Q1 OPTICS Pub Date : 2024-08-02 DOI: 10.1038/s41566-024-01474-3
M. Galletti, R. Assmann, M. E. Couprie, M. Ferrario, L. Giannessi, A. Irman, R. Pompili, W. Wang
Plasma-wakefield-based acceleration technology has the potential to revolutionize the field of particle accelerators. By providing acceleration gradients orders of magnitude larger than conventional radiofrequency particle accelerators, this technology allows accelerators to be reduced to the centimetre length scale. It also provides a new compact approach for driving free-electron lasers, a valuable source of high-brilliance ultrashort coherent radiation within the infrared to X-ray spectral range for the study of subatomic matter, ultrafast dynamics of complex systems and X-ray nonlinear optics, among other applications. Several laboratories around the world are working on the realization of these new light sources, exploring different configurations for the plasma wakefield driver beam, plasma stage design and operational regime. This Review describes the operating principles of plasma accelerators, an overview of recent experimental milestones for plasma-driven free-electron lasers in self-amplified spontaneous emission and seeded configurations, and highlights the remaining major challenges in the field. This Review examines the principles of operation and progress made in developing free-electron lasers that feature plasma-wakefield-acceleration technology.
基于等离子唤醒场的加速技术有可能彻底改变粒子加速器领域。通过提供比传统射频粒子加速器大几个数量级的加速梯度,该技术可将加速器的长度缩减到厘米级。它还为驱动自由电子激光器提供了一种新的紧凑型方法,而自由电子激光器是红外至 X 射线光谱范围内高亮度超短相干辐射的重要来源,可用于研究亚原子物质、复杂系统的超快动力学和 X 射线非线性光学等应用。世界各地的一些实验室正在努力实现这些新光源,探索等离子体汪场驱动光束的不同配置、等离子体平台设计和运行机制。本综述介绍了等离子体加速器的工作原理,概述了自放大自发辐射和种子配置等离子体驱动自由电子激光器的最新实验里程碑,并重点介绍了该领域仍然存在的主要挑战。
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引用次数: 0
Nonlinear optical encoding enabled by recurrent linear scattering 利用递归线性散射实现非线性光学编码
IF 35 1区 物理与天体物理 Q1 OPTICS Pub Date : 2024-07-31 DOI: 10.1038/s41566-024-01493-0
Fei Xia, Kyungduk Kim, Yaniv Eliezer, SeungYun Han, Liam Shaughnessy, Sylvain Gigan, Hui Cao

Optical information processing and computing can potentially offer enhanced performance, scalability and energy efficiency. However, achieving nonlinearity—a critical component of computation—remains challenging in the optical domain. Here we introduce a design that leverages a multiple-scattering cavity to passively induce optical nonlinear random mapping with a continuous-wave laser at a low power. Each scattering event effectively mixes information from different areas of a spatial light modulator, resulting in a highly nonlinear mapping between the input data and output pattern. We demonstrate that our design retains vital information even when the readout dimensionality is reduced, thereby enabling optical data compression. This capability allows our optical platforms to offer efficient optical information processing solutions across applications. We demonstrate our design’s efficacy across tasks, including classification, image reconstruction, keypoint detection and object detection, all of which are achieved through optical data compression combined with a digital decoder. In particular, high performance at extreme compression ratios is observed in real-time pedestrian detection. Our findings open pathways for novel algorithms and unconventional architectural designs for optical computing.

光学信息处理和计算有可能提供更高的性能、可扩展性和能效。然而,实现非线性--计算的关键组成部分--在光学领域仍具有挑战性。在这里,我们介绍了一种利用多重散射腔的设计,以低功率连续波激光器被动诱导光学非线性随机映射。每个散射事件都能有效混合来自空间光调制器不同区域的信息,从而在输入数据和输出图案之间形成高度非线性映射。我们证明,即使读出维度降低,我们的设计也能保留重要信息,从而实现光学数据压缩。这种能力使我们的光学平台能够为各种应用提供高效的光学信息处理解决方案。我们展示了我们的设计在分类、图像重建、关键点检测和物体检测等任务中的功效,所有这些任务都是通过光学数据压缩结合数字解码器来实现的。特别是在实时行人检测中,我们观察到了极高压缩比下的高性能。我们的发现为光学计算的新型算法和非传统架构设计开辟了道路。
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引用次数: 0
Chirality conferral enables the observation of hyper-Raman optical activity 手性赋予可观测超拉曼光学活动
IF 32.3 1区 物理与天体物理 Q1 OPTICS Pub Date : 2024-07-31 DOI: 10.1038/s41566-024-01486-z
Robin R. Jones, John F. Kerr, Hyunah Kwon, Samuel R. Clowes, Ruidong Ji, Emilija Petronijevic, Liwu Zhang, G. Dan Pantoș, Brian Smith, Tim Batten, Peer Fischer, Daniel Wolverson, David L. Andrews, Ventsislav K. Valev
Chirality conferral is fundamental for understanding the origin of life, and it is of direct importance for synthesizing new pharmaceuticals in the face of growing antibiotic resistance. Human-made, self-assembling nanostructures replicate the biological chirality conferral processes utilizing covalent and non-covalent bonds. However, chirality conferral from one form of matter to another via electromagnetic fields is more subtle and less explored. Here we report chirality conferral between gold nanohelices and achiral molecules (crystal violet). This conferral enables the experimental observation of a physical effect predicted in 1979—hyper-Raman optical activity. To benefit from Fermi’s golden rule, the chirality conferral system was designed as doubly resonant, with the nanohelices and molecules resonating at the fundamental frequency and at the second-harmonic, respectively. We provide a theoretical framework for our results that expands the original mathematical formalism to include surface-enhanced hyper-Raman scattering and the chirality conferral process. Our results demonstrate that field-driven chirality conferral mechanisms are opening up entire fields of research, as exemplified by the discovery of a physical phenomenon. Theoretically predicted in 1979, hyper-Raman optical activity is now experimentally observed through chirality conferral from the electromagnetic field of chiral plasmonic gold nanohelices to crystal violet molecules that are achiral, sparking new science at the organic–inorganic interface.
手性赋予是了解生命起源的基础,面对日益增长的抗生素耐药性,手性赋予对合成新药具有直接的重要意义。人造自组装纳米结构利用共价键和非共价键复制了生物手性赋予过程。然而,通过电磁场从一种物质形式到另一种物质形式的手性赋予过程更为微妙,探索较少。在此,我们报告了金纳米螺旋与非手性分子(紫水晶)之间的手性赋予。这种禀赋使我们能够在实验中观测到 1979 年预测的物理效应--超拉曼光学活动。为了受益于费米黄金定律,手性赋予系统被设计为双共振,纳米螺旋和分子分别在基频和二次谐波上共振。我们为研究结果提供了一个理论框架,扩展了原始数学形式主义,将表面增强超拉曼散射和手性赋予过程纳入其中。我们的结果表明,场驱动的手性赋予机制正在开辟整个研究领域,一个物理现象的发现就是例证。
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引用次数: 0
Nonlinear processing with linear optics 线性光学非线性处理
IF 35 1区 物理与天体物理 Q1 OPTICS Pub Date : 2024-07-31 DOI: 10.1038/s41566-024-01494-z
Mustafa Yildirim, Niyazi Ulas Dinc, Ilker Oguz, Demetri Psaltis, Christophe Moser

Deep neural networks have achieved remarkable breakthroughs by leveraging multiple layers of data processing to extract hidden representations, albeit at the cost of large electronic computing power. To enhance energy efficiency and speed, the optical implementation of neural networks aims to harness the advantages of optical bandwidth and the energy efficiency of optical interconnections. In the absence of low-power optical nonlinearities, the challenge in the implementation of multilayer optical networks lies in realizing multiple optical layers without resorting to electronic components. Here we present a novel framework that uses multiple scattering, and which is capable of synthesizing programmable linear and nonlinear transformations concurrently at low optical power by leveraging the nonlinear relationship between the scattering potential, represented by data, and the scattered field. Theoretical and experimental investigations show that repeating the data by multiple scattering enables nonlinear optical computing with low-power continuous-wave light. Moreover, we empirically find that scaling of this optical framework follows a power law.

深度神经网络通过利用多层数据处理来提取隐藏表征,取得了令人瞩目的突破,尽管其代价是需要大量的电子计算能力。为了提高能效和速度,神经网络的光学实现旨在利用光带宽和光互连能效的优势。在缺乏低功耗光非线性的情况下,实现多层光学网络的挑战在于如何在不借助电子元件的情况下实现多个光学层。在这里,我们提出了一种使用多重散射的新型框架,它能够利用数据所代表的散射势与散射场之间的非线性关系,在低光功率下同时合成可编程的线性和非线性变换。理论和实验研究表明,通过多次散射重复数据,可以利用低功率连续波光实现非线性光学计算。此外,我们还根据经验发现,这种光学框架的缩放遵循幂律。
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引用次数: 0
Suppressed ion migration for high-performance X-ray detectors based on atmosphere-controlled EFG-grown perovskite CsPbBr3 single crystals 基于大气控制 EFG 生长的包晶 CsPbBr3 单晶的高性能 X 射线探测器的离子迁移抑制技术
IF 32.3 1区 物理与天体物理 Q1 OPTICS Pub Date : 2024-07-29 DOI: 10.1038/s41566-024-01480-5
Yunqiu Hua, Guodong Zhang, Xue Sun, Peng Zhang, Yingying Hao, Yadong Xu, Yujie Yang, Qianqian Lin, Xiang Li, Zhongjun Zhai, Fucai Cui, Hongjie Liu, Jiaxin Liu, Xutang Tao
Halide perovskites have shown great potential for X-ray detection in medical imaging and product inspection applications. However, the ion migration in perovskites causes large noise and baseline drift, deteriorating the X-ray detection and imaging performance. Here we adopt the atmosphere-controlled edge-defined film-fed growth (EFG) method to grow high-quality shape-controlled CsPbBr3 single crystals (SCs) in an Ar and HBr mixed atmosphere. Compared with the vertical Bridgman (VB)-CsPbBr3 SCs, the EFG-CsPbBr3 SCs show a much lower trap density, a higher resistivity (1.61 × 1010 Ω cm) and a larger ion migration activation energy (0.378 eV), decreasing the leakage current and baseline drift. An X-ray detector based on EFG-CsPbBr3 SCs hence exhibits outstanding balanced performance, with a negligible dark-current drift of 1.68 × 10−9 μA cm−1 s−1 V−1, an incredibly low detection limit of 10.81 nGyair s−1 and a sensitivity of 46,180 μC Gyair−1 cm−2 under a high electric field of 5,000 V cm−1. Furthermore, the detector maintains a stable response for 30 days. Our work provides an effective strategy to improve lead-halide perovskite SCs for high-performance X-ray detection and imaging. The researchers improve the properties of halide perovskite for high-performance X-ray detection by edge-defined film-fed crystal growth. In particular, high resistivity, low trap density, suppressed ion migration and reduced leakage current are demonstrated. They enable detectors with an extremely low detection limit and high sensitivity.
卤化物包光体在医疗成像和产品检测应用中的 X 射线探测方面显示出巨大的潜力。然而,包晶中的离子迁移会导致较大的噪声和基线漂移,从而降低 X 射线检测和成像性能。在此,我们采用气氛控制的边缘薄膜生长(EFG)方法,在 Ar 和 HBr 混合气氛中生长出高质量形状可控的 CsPbBr3 单晶(SC)。与垂直布里奇曼(VB)-CsPbBr3 单晶相比,EFG-CsPbBr3 单晶具有更低的阱密度、更高的电阻率(1.61 × 1010 Ω cm)和更大的离子迁移活化能(0.378 eV),从而降低了泄漏电流和基线漂移。因此,基于 EFG-CsPbBr3 SCs 的 X 射线探测器具有出色的平衡性能,其暗电流漂移为 1.68 × 10-9 μA cm-1 s-1 V-1,可忽略不计;在 5,000 V cm-1 的高电场下,其探测极限低至 10.81 nGyair s-1,灵敏度高达 46,180 μC Gyair-1 cm-2。此外,该探测器还能在 30 天内保持稳定的响应。我们的工作为改进铅卤化物包晶SC以实现高性能X射线探测和成像提供了一种有效的策略。
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引用次数: 0
Retraction Note: Luminescent solar concentrator efficiency enhanced via nearly lossless propagation pathways 撤稿说明:通过近乎无损的传播途径提高发光太阳能聚光器的效率
IF 32.3 1区 物理与天体物理 Q1 OPTICS Pub Date : 2024-07-25 DOI: 10.1038/s41566-024-01502-2
Kyoungwon Park, Jeongmin Yi, Suk-Young Yoon, Seong Min Park, Jiyong Kim, Hyun-Beom Shin, Swarup Biswas, Gang Yeol Yoo, Sang-Hwa Moon, Jiwan Kim, Min Suk Oh, Armin Wedel, Sohee Jeong, Hyeok Kim, Soong Ju Oh, Ho Kwan Kang, Heesun Yang, Chul Jong Han
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引用次数: 0
Author Correction: High gradient terahertz-driven ultrafast photogun 作者更正:高梯度太赫兹驱动超快光枪
IF 32.3 1区 物理与天体物理 Q1 OPTICS Pub Date : 2024-07-22 DOI: 10.1038/s41566-024-01503-1
Jianwei Ying, Xie He, Dace Su, Lingbin Zheng, Tobias Kroh, Timm Rohwer, Moein Fakhari, Günther H. Kassier, Jingui Ma, Peng Yuan, Nicholas H. Matlis, Franz X. Kärtner, Dongfang Zhang
{"title":"Author Correction: High gradient terahertz-driven ultrafast photogun","authors":"Jianwei Ying,&nbsp;Xie He,&nbsp;Dace Su,&nbsp;Lingbin Zheng,&nbsp;Tobias Kroh,&nbsp;Timm Rohwer,&nbsp;Moein Fakhari,&nbsp;Günther H. Kassier,&nbsp;Jingui Ma,&nbsp;Peng Yuan,&nbsp;Nicholas H. Matlis,&nbsp;Franz X. Kärtner,&nbsp;Dongfang Zhang","doi":"10.1038/s41566-024-01503-1","DOIUrl":"10.1038/s41566-024-01503-1","url":null,"abstract":"","PeriodicalId":18926,"journal":{"name":"Nature Photonics","volume":null,"pages":null},"PeriodicalIF":32.3,"publicationDate":"2024-07-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.nature.com/articles/s41566-024-01503-1.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141814986","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
In situ nanoscopy of single-grain nanomorphology and ultrafast carrier dynamics in metal halide perovskites 原位纳米透视金属卤化物过氧化物中的单晶粒纳米形态和超快载流子动力学
IF 32.3 1区 物理与天体物理 Q1 OPTICS Pub Date : 2024-07-17 DOI: 10.1038/s41566-024-01476-1
M. Zizlsperger, S. Nerreter, Q. Yuan, K. B. Lohmann, F. Sandner, F. Schiegl, C. Meineke, Y. A. Gerasimenko, L. M. Herz, T. Siday, M. A. Huber, M. B. Johnston, R. Huber
Designing next-generation light-harvesting devices requires a detailed understanding of the transport of photoexcited charge carriers. The record-breaking efficiencies of metal halide perovskite solar cells have been linked to effective charge-carrier diffusion, yet the exact nature of charge-carrier out-of-plane transport remains notoriously difficult to explain. The characteristic spatial inhomogeneity of perovskite films with nanograins and crystallographic disorder calls for the simultaneous and hitherto elusive in situ resolution of the chemical composition, the structural phase and the ultrafast dynamics of the local out-of-plane transport. Here we simultaneously probe the intrinsic out-of-plane charge-carrier diffusion and the nanoscale morphology by pushing depth-sensitive terahertz near-field nanospectroscopy to extreme subcycle timescales. In films of the organic–inorganic metal halide perovskite FA0.83Cs0.17Pb(I1−xClx)3 (where FA is formamidinium), domains of the cubic α-phase are clearly distinguished from the trigonal δ-phase and PbI2 nano-islands. By analysing deep-subcycle time shifts of the scattered terahertz waveform after photoexcitation, we access the vertical charge-carrier dynamics within single grains. At all of the measured locations, despite topographic irregularities, diffusion is surprisingly homogeneous on the 100 nm scale, although it varies between mesoscopic regions. Linking in situ carrier transport with nanoscale morphology and chemical composition could introduce a paradigm shift for the analysis and optimization of next-generation optoelectronics that are based on nanocrystalline materials. Transient visible-pump terahertz-probe near-field microscopy enables the simultaneous retrieval of the local chemical composition, crystallographic structure, topography and out-of-plane charge-carrier diffusion in perovskite films.
设计下一代光收集装置需要详细了解光激发电荷载流子的传输。金属卤化物包晶体太阳能电池破纪录的效率与有效的电荷载流子扩散有关,但电荷载流子平面外传输的确切性质仍然难以解释。具有纳米晶粒和晶体学无序性的透辉石薄膜所特有的空间不均匀性要求同时对化学成分、结构相和局部面外传输的超快动态进行原位解析,而这种解析迄今为止还难以实现。在这里,我们通过将深度敏感的太赫兹近场纳米光谱技术推向极端的亚周期时间尺度,同时探测了固有的面外电荷载流子扩散和纳米级形貌。在有机-无机金属卤化物包晶石 FA0.83Cs0.17Pb(I1-xClx)3(其中 FA 为甲脒基)的薄膜中,立方体 α 相域与三方体 δ 相域和 PbI2 纳米等离子体被清晰地区分开来。通过分析光激发后散射太赫兹波形的深亚周期时移,我们获得了单个晶粒内部的垂直电荷载流子动力学。在所有测量位置,尽管地形不规则,但扩散在 100 纳米尺度上出奇地均匀,尽管在中观区域之间存在差异。将原位载流子传输与纳米级形貌和化学成分联系起来,可以为分析和优化基于纳米晶体材料的下一代光电子学带来范式转变。
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引用次数: 0
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Nature Photonics
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