Vortex phenomena are ubiquitous in nature. In optics, despite the availability of numerous techniques for vortex generation and detection, topological protection of vortex transport with desired orbital angular momentum (OAM) remains a challenge. Here, by use of topological disclination, we demonstrate a scheme to confine and guide vortices featuring arbitrary high-order charges. Such a scheme relies on twofold topological protection: a non-trivial winding in momentum space due to chiral symmetry, and a non-trivial winding in real space due to the complex coupling of OAM modes across the disclination structure. We unveil a vorticity-coordinated rotational symmetry, which sets up a universal relation between the vortex topological charge and the rotational symmetry order of the system. As an example, we construct photonic disclination lattices with a single core but different Cn symmetries and achieve robust transport of an optical vortex with preserved OAM solely corresponding to one selected zero-energy vortex mode at the mid-gap. Furthermore, we show that such topological structures can be used for vortex filtering to extract a chosen OAM mode from mixed excitations. Our results illustrate the fundamental interplay of vorticity, disclination and higher-order topology, which may open a new pathway for the development of OAM-based photonic devices such as vortex guides, fibres and lasers.
{"title":"Topological orbital angular momentum extraction and twofold protection of vortex transport","authors":"Zhichan Hu, Domenico Bongiovanni, Ziteng Wang, Xiangdong Wang, Daohong Song, Jingjun Xu, Roberto Morandotti, Hrvoje Buljan, Zhigang Chen","doi":"10.1038/s41566-024-01564-2","DOIUrl":"https://doi.org/10.1038/s41566-024-01564-2","url":null,"abstract":"<p>Vortex phenomena are ubiquitous in nature. In optics, despite the availability of numerous techniques for vortex generation and detection, topological protection of vortex transport with desired orbital angular momentum (OAM) remains a challenge. Here, by use of topological disclination, we demonstrate a scheme to confine and guide vortices featuring arbitrary high-order charges. Such a scheme relies on twofold topological protection: a non-trivial winding in momentum space due to chiral symmetry, and a non-trivial winding in real space due to the complex coupling of OAM modes across the disclination structure. We unveil a vorticity-coordinated rotational symmetry, which sets up a universal relation between the vortex topological charge and the rotational symmetry order of the system. As an example, we construct photonic disclination lattices with a single core but different <i>C</i><sub><i>n</i></sub> symmetries and achieve robust transport of an optical vortex with preserved OAM solely corresponding to one selected zero-energy vortex mode at the mid-gap. Furthermore, we show that such topological structures can be used for vortex filtering to extract a chosen OAM mode from mixed excitations. Our results illustrate the fundamental interplay of vorticity, disclination and higher-order topology, which may open a new pathway for the development of OAM-based photonic devices such as vortex guides, fibres and lasers.</p>","PeriodicalId":18926,"journal":{"name":"Nature Photonics","volume":"15 1","pages":""},"PeriodicalIF":35.0,"publicationDate":"2024-11-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142673513","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-11-12DOI: 10.1038/s41566-024-01563-3
X. Wang, P. Garg, M. S. Mirmoosa, A. G. Lamprianidis, C. Rockstuhl, V. S. Asadchy
The realization of photonic time crystals is a major opportunity but also comes with considerable challenges. The most pressing one, potentially, is the requirement for a substantial modulation strength in the material properties to create a noticeable momentum bandgap. Reaching that noticeable bandgap in optics is highly demanding with current, and possibly also future materials platforms because their modulation strength is small by tendency. Here we demonstrate that by introducing temporal variations in a resonant material, the momentum bandgap can be drastically expanded with modulation strengths in reach with known low-loss materials and realistic laser pump powers. The resonance can emerge from an intrinsic material resonance or a suitably spatially structured material supporting a structural resonance. Our concept is validated for resonant bulk media and optical metasurfaces and paves the way towards the first experimental realizations of photonic time crystals.
{"title":"Expanding momentum bandgaps in photonic time crystals through resonances","authors":"X. Wang, P. Garg, M. S. Mirmoosa, A. G. Lamprianidis, C. Rockstuhl, V. S. Asadchy","doi":"10.1038/s41566-024-01563-3","DOIUrl":"https://doi.org/10.1038/s41566-024-01563-3","url":null,"abstract":"<p>The realization of photonic time crystals is a major opportunity but also comes with considerable challenges. The most pressing one, potentially, is the requirement for a substantial modulation strength in the material properties to create a noticeable momentum bandgap. Reaching that noticeable bandgap in optics is highly demanding with current, and possibly also future materials platforms because their modulation strength is small by tendency. Here we demonstrate that by introducing temporal variations in a resonant material, the momentum bandgap can be drastically expanded with modulation strengths in reach with known low-loss materials and realistic laser pump powers. The resonance can emerge from an intrinsic material resonance or a suitably spatially structured material supporting a structural resonance. Our concept is validated for resonant bulk media and optical metasurfaces and paves the way towards the first experimental realizations of photonic time crystals.</p>","PeriodicalId":18926,"journal":{"name":"Nature Photonics","volume":"1 1","pages":""},"PeriodicalIF":35.0,"publicationDate":"2024-11-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142599378","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-11-04DOI: 10.1038/s41566-024-01561-5
Chenxia Kan, Pengjie Hang, Shibo Wang, Biao Li, Xuegong Yu, Xinbo Yang, Yuxin Yao, Wei Shi, Stefaan De Wolf, Jun Yin, Daoyong Zhang, Degong Ding, Cao Yu, Shaofei Yang, Jiteng Zhang, Jia Yao, Xiaohong Zhang, Deren Yang
Monolithic perovskite/silicon tandem solar cells have achieved promising performance. However, hole transport layers that are commonly used for the perovskite top cell suffer from defects, non-conformal deposition or de-wetting of the overlying perovskite on the textured silicon bottom cells. These issues detrimentally affect device reproducibility and scalability, and thus commercialization. Here we address these challenges through the co-deposition of copper(I) thiocyanate and perovskite, where effective perovskite grain boundary passivation and efficient hole collection are simultaneously achieved by the embedded copper(I) thiocyanate, which creates local hole-collecting contacts. Fabricated monolithic perovskite/silicon tandem devices achieve a certified power conversion efficiency of 31.46% for 1 cm2 area devices. Aside from good reproducibility and scalability, our tandem cells exhibit excellent stability, maintaining 93.8% of their initial power conversion efficiency after about 1,200 h of maximum power point tracking at 45 °C, and 90.2% after over 1,000 h of damp-heat testing at 85 °C and 85% relative humidity. Co-deposition of copper thiocyanate with perovskite on textured silicon enables an efficient perovskite-silicon tandem solar cell with a certified power conversion efficiency of 31.46% for 1 cm2 area devices.
{"title":"Efficient and stable perovskite-silicon tandem solar cells with copper thiocyanate-embedded perovskite on textured silicon","authors":"Chenxia Kan, Pengjie Hang, Shibo Wang, Biao Li, Xuegong Yu, Xinbo Yang, Yuxin Yao, Wei Shi, Stefaan De Wolf, Jun Yin, Daoyong Zhang, Degong Ding, Cao Yu, Shaofei Yang, Jiteng Zhang, Jia Yao, Xiaohong Zhang, Deren Yang","doi":"10.1038/s41566-024-01561-5","DOIUrl":"10.1038/s41566-024-01561-5","url":null,"abstract":"Monolithic perovskite/silicon tandem solar cells have achieved promising performance. However, hole transport layers that are commonly used for the perovskite top cell suffer from defects, non-conformal deposition or de-wetting of the overlying perovskite on the textured silicon bottom cells. These issues detrimentally affect device reproducibility and scalability, and thus commercialization. Here we address these challenges through the co-deposition of copper(I) thiocyanate and perovskite, where effective perovskite grain boundary passivation and efficient hole collection are simultaneously achieved by the embedded copper(I) thiocyanate, which creates local hole-collecting contacts. Fabricated monolithic perovskite/silicon tandem devices achieve a certified power conversion efficiency of 31.46% for 1 cm2 area devices. Aside from good reproducibility and scalability, our tandem cells exhibit excellent stability, maintaining 93.8% of their initial power conversion efficiency after about 1,200 h of maximum power point tracking at 45 °C, and 90.2% after over 1,000 h of damp-heat testing at 85 °C and 85% relative humidity. Co-deposition of copper thiocyanate with perovskite on textured silicon enables an efficient perovskite-silicon tandem solar cell with a certified power conversion efficiency of 31.46% for 1 cm2 area devices.","PeriodicalId":18926,"journal":{"name":"Nature Photonics","volume":"19 1","pages":"63-70"},"PeriodicalIF":32.3,"publicationDate":"2024-11-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142574314","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-11-01DOI: 10.1038/s41566-024-01555-3
Y. A. Yang, W.-T. Luo, J.-L. Zhang, S.-Z. Wang, Chang-Ling Zou, T. Xia, Z.-T. Lu
Quantum metrology with non-classical states offers a promising route to improved precision in physical measurements. The quantum effects of Schrödinger-cat superpositions or entanglements enable measurement uncertainties to reach below the standard quantum limit. However, the challenge of maintaining a long coherence time for such non-classical states often prevents full exploitation of the quantum advantage in metrology. Here we demonstrate a long-lived Schrödinger-cat state of optically trapped 173Yb (I = 5/2) atoms. The cat state, a superposition of two oppositely directed and furthest-apart spin states, is generated by a nonlinear spin rotation. Protected in a decoherence-free subspace against inhomogeneous light shifts of an optical lattice, the cat state persists for a coherence time of 1.4(1) × 103 s. A magnetic field is measured using Ramsey interferometry, demonstrating a scheme of Heisenberg-limited metrology for atomic magnetometry, quantum information processing and searching for new physics beyond the Standard Model. Using spin-5/2 nuclei of 173Yb atoms trapped in an optical lattice, a Schrödinger-cat state persists for a coherence time of 1.4 × 103 s. In measuring external magnetic fields, the cat state exhibits a sensitivity approaching the Heisenberg limit.
使用非经典状态的量子计量学为提高物理测量精度提供了一条前景广阔的途径。薛定谔猫叠加或纠缠的量子效应使测量的不确定性达到标准量子极限以下。然而,要使这种非经典状态保持较长的相干时间,往往会阻碍在计量学中充分发挥量子优势。在这里,我们展示了光学捕获的 173Yb (I = 5/2) 原子的长寿命薛定谔猫态。猫态是两个方向相反、相距最远的自旋态的叠加,由非线性自旋旋转产生。猫态在无退相干子空间中受到光晶格不均匀光偏移的保护,其相干时间为 1.4(1) × 103 秒。利用拉姆齐干涉测量法测量磁场,为原子磁力测量、量子信息处理和寻找标准模型之外的新物理学展示了一种海森堡限制计量方案。
{"title":"Minute-scale Schrödinger-cat state of spin-5/2 atoms","authors":"Y. A. Yang, W.-T. Luo, J.-L. Zhang, S.-Z. Wang, Chang-Ling Zou, T. Xia, Z.-T. Lu","doi":"10.1038/s41566-024-01555-3","DOIUrl":"10.1038/s41566-024-01555-3","url":null,"abstract":"Quantum metrology with non-classical states offers a promising route to improved precision in physical measurements. The quantum effects of Schrödinger-cat superpositions or entanglements enable measurement uncertainties to reach below the standard quantum limit. However, the challenge of maintaining a long coherence time for such non-classical states often prevents full exploitation of the quantum advantage in metrology. Here we demonstrate a long-lived Schrödinger-cat state of optically trapped 173Yb (I = 5/2) atoms. The cat state, a superposition of two oppositely directed and furthest-apart spin states, is generated by a nonlinear spin rotation. Protected in a decoherence-free subspace against inhomogeneous light shifts of an optical lattice, the cat state persists for a coherence time of 1.4(1) × 103 s. A magnetic field is measured using Ramsey interferometry, demonstrating a scheme of Heisenberg-limited metrology for atomic magnetometry, quantum information processing and searching for new physics beyond the Standard Model. Using spin-5/2 nuclei of 173Yb atoms trapped in an optical lattice, a Schrödinger-cat state persists for a coherence time of 1.4 × 103 s. In measuring external magnetic fields, the cat state exhibits a sensitivity approaching the Heisenberg limit.","PeriodicalId":18926,"journal":{"name":"Nature Photonics","volume":"19 1","pages":"89-94"},"PeriodicalIF":32.3,"publicationDate":"2024-11-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142561971","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-11-01DOI: 10.1038/s41566-024-01556-2
Omer Kneller, Chen Mor, Nikolai D. Klimkin, Noa Yaffe, Michael Krüger, Doron Azoury, Ayelet J. Uzan-Narovlansky, Yotam Federman, Debobrata Rajak, Barry D. Bruner, Olga Smirnova, Serguei Patchkovskii, Yann Mairesse, Misha Ivanov, Nirit Dudovich
Attosecond transient absorption resolves the instantaneous response of a quantum system as it interacts with a laser field, by mapping its sub-cycle dynamics onto the absorption spectrum of attosecond pulses. However, the quantum dynamics are imprinted in the amplitude, phase and polarization state of the attosecond pulses. Here we introduce attosecond transient interferometry and measure the transient phase, as we follow its evolution within the optical cycle. We demonstrate how such phase information enables us to decouple the multiple quantum paths induced in a light-driven system, isolating their coherent contribution and retrieving their temporal evolution. Applying attosecond transient interferometry reveals the Stark shift dynamics in helium and retrieves long-term electronic coherences in neon. Finally, we present a vectorial generalization of our scheme, theoretically demonstrating the ability to isolate the underlying anomalous current in light-driven topological materials. Our scheme provides a direct insight into the interplay of light-induced dynamics and topology. Attosecond transient interferometry holds the potential to considerably extend the scope of attosecond metrology, revealing the underlying coherences in light-driven complex systems.
{"title":"Attosecond transient interferometry","authors":"Omer Kneller, Chen Mor, Nikolai D. Klimkin, Noa Yaffe, Michael Krüger, Doron Azoury, Ayelet J. Uzan-Narovlansky, Yotam Federman, Debobrata Rajak, Barry D. Bruner, Olga Smirnova, Serguei Patchkovskii, Yann Mairesse, Misha Ivanov, Nirit Dudovich","doi":"10.1038/s41566-024-01556-2","DOIUrl":"https://doi.org/10.1038/s41566-024-01556-2","url":null,"abstract":"<p>Attosecond transient absorption resolves the instantaneous response of a quantum system as it interacts with a laser field, by mapping its sub-cycle dynamics onto the absorption spectrum of attosecond pulses. However, the quantum dynamics are imprinted in the amplitude, phase and polarization state of the attosecond pulses. Here we introduce attosecond transient interferometry and measure the transient phase, as we follow its evolution within the optical cycle. We demonstrate how such phase information enables us to decouple the multiple quantum paths induced in a light-driven system, isolating their coherent contribution and retrieving their temporal evolution. Applying attosecond transient interferometry reveals the Stark shift dynamics in helium and retrieves long-term electronic coherences in neon. Finally, we present a vectorial generalization of our scheme, theoretically demonstrating the ability to isolate the underlying anomalous current in light-driven topological materials. Our scheme provides a direct insight into the interplay of light-induced dynamics and topology. Attosecond transient interferometry holds the potential to considerably extend the scope of attosecond metrology, revealing the underlying coherences in light-driven complex systems.</p>","PeriodicalId":18926,"journal":{"name":"Nature Photonics","volume":"16 1","pages":""},"PeriodicalIF":35.0,"publicationDate":"2024-11-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142561970","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-10-31DOI: 10.1038/s41566-024-01552-6
Gordon Robb
Imaging in the water window has traditionally relied on large synchrotron radiation sources. Now, a tabletop tunable X-ray source which generates water-window X-ray photons from a low energy electron beam interacting with a van der Waals crystal has been demonstrated.
水窗成像历来依赖于大型同步辐射源。现在,一种台式可调 X 射线源已经问世,它能通过低能量电子束与范德华晶体的相互作用产生水窗 X 射线光子。
{"title":"Small tunable X-ray sources may have large impact","authors":"Gordon Robb","doi":"10.1038/s41566-024-01552-6","DOIUrl":"10.1038/s41566-024-01552-6","url":null,"abstract":"Imaging in the water window has traditionally relied on large synchrotron radiation sources. Now, a tabletop tunable X-ray source which generates water-window X-ray photons from a low energy electron beam interacting with a van der Waals crystal has been demonstrated.","PeriodicalId":18926,"journal":{"name":"Nature Photonics","volume":"18 11","pages":"1129-1130"},"PeriodicalIF":32.3,"publicationDate":"2024-10-31","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142556348","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-10-31DOI: 10.1038/s41566-024-01562-4
Oliver Graydon
{"title":"Refractive index engineering makes skin transparent","authors":"Oliver Graydon","doi":"10.1038/s41566-024-01562-4","DOIUrl":"10.1038/s41566-024-01562-4","url":null,"abstract":"","PeriodicalId":18926,"journal":{"name":"Nature Photonics","volume":"18 11","pages":"1136-1136"},"PeriodicalIF":32.3,"publicationDate":"2024-10-31","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142556349","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-10-31DOI: 10.1038/s41566-024-01557-1
Nikolay I. Zheludev
Photonics can play a pivotal role in bringing time crystals to the domain of optical ‘timetronics’ — an information and data technology that relies on the unique functionalities of this sophisticated yet esoteric state of matter.
{"title":"Time crystals for photonics and timetronics","authors":"Nikolay I. Zheludev","doi":"10.1038/s41566-024-01557-1","DOIUrl":"10.1038/s41566-024-01557-1","url":null,"abstract":"Photonics can play a pivotal role in bringing time crystals to the domain of optical ‘timetronics’ — an information and data technology that relies on the unique functionalities of this sophisticated yet esoteric state of matter.","PeriodicalId":18926,"journal":{"name":"Nature Photonics","volume":"18 11","pages":"1123-1125"},"PeriodicalIF":32.3,"publicationDate":"2024-10-31","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142556351","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-10-31DOI: 10.1038/s41566-024-01559-z
Giampaolo Pitruzzello
Nature Photonics spoke with Hatice Altug, from the École Polytechnique Fédérale de Lausanne (EPFL), Thomas Krauss, from the University of York, and Malini Olivo from the Agency for Science, Technology and Research (A*STAR) about optical biosensors and their prospects and challenges for clinical translation.
{"title":"Optical biosensors towards the clinic","authors":"Giampaolo Pitruzzello","doi":"10.1038/s41566-024-01559-z","DOIUrl":"10.1038/s41566-024-01559-z","url":null,"abstract":"Nature Photonics spoke with Hatice Altug, from the École Polytechnique Fédérale de Lausanne (EPFL), Thomas Krauss, from the University of York, and Malini Olivo from the Agency for Science, Technology and Research (A*STAR) about optical biosensors and their prospects and challenges for clinical translation.","PeriodicalId":18926,"journal":{"name":"Nature Photonics","volume":"18 11","pages":"1126-1128"},"PeriodicalIF":32.3,"publicationDate":"2024-10-31","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142556347","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}