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Broadband hyperspectral imaging 宽带高光谱成像
IF 32.3 1区 物理与天体物理 Q1 OPTICS Pub Date : 2025-01-07 DOI: 10.1038/s41566-024-01597-7
Giampaolo Pitruzzello
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引用次数: 0
Spontaneous phase locking in a broad-area semiconductor laser 广域半导体激光器的自发锁相
IF 35 1区 物理与天体物理 Q1 OPTICS Pub Date : 2025-01-07 DOI: 10.1038/s41566-024-01604-x
Stefan Bittner, Marc Sciamanna

Broad-area semiconductor lasers are used in many high-power applications; however, their spatio-temporal dynamics are complex and intrinsically unstable due to the interaction between transverse lasing modes. Here a dynamical and ultrahigh-resolution spatio-spectral analysis of commercial broad-area lasers reveals multiplets of phase-locked first- and second-order transverse modes that are spontaneously created by the nonlinear dynamics of the laser. Phase locking between modes of different transverse order is confirmed by comparing the linewidths of the lasing modes with that of their beat note and by a direct measurement of their phase fluctuation correlations. The spontaneous phase locking is unexpected since the overall dynamics are unstable and the system lacks any intentional feature to induce locking. This partially synchronized dynamical state with groups of coexisting synchronized and unsynchronized laser modes is similar to chimera states found in networks of coupled oscillators, indicating that such states may exist in a wider range of systems than previously assumed.

宽域半导体激光器在许多高功率应用中都有使用;然而,由于横向激光模式之间的相互作用,它们的时空动态非常复杂,而且本质上并不稳定。在此,我们对商用宽域激光器进行了动态和超高分辨率时空谱分析,揭示了激光器非线性动力学自发产生的锁相一阶和二阶横向模式的多重序列。通过比较不同横向阶数模式的线宽与它们的节拍音符的线宽,以及直接测量它们的相位波动相关性,证实了不同横向阶数模式之间的锁相。自发锁相是意料之外的,因为整体动力学是不稳定的,而且系统缺乏任何诱导锁相的有意特征。这种由同步和非同步激光模式群共存的部分同步动力学状态类似于耦合振荡器网络中的嵌合态,表明这种状态可能存在于比以前假设的更广泛的系统中。
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引用次数: 0
Optical atomic clock interrogation using an integrated spiral cavity laser 使用集成螺旋腔激光器的光学原子钟查询
IF 35 1区 物理与天体物理 Q1 OPTICS Pub Date : 2025-01-06 DOI: 10.1038/s41566-024-01588-8
William Loh, David Reens, Dave Kharas, Alkesh Sumant, Connor Belanger, Ryan T. Maxson, Alexander Medeiros, William Setzer, Dodd Gray, Kyle DeBry, Colin D. Bruzewicz, Jason Plant, John Liddell, Gavin N. West, Sagar Doshi, Matthew Roychowdhury, May E. Kim, Danielle Braje, Paul W. Juodawlkis, John Chiaverini, Robert McConnell

Optical atomic clocks have demonstrated revolutionary advances in precision timekeeping, but their applicability to the real world is critically dependent on whether such clocks can operate outside the laboratory. Photonic integration offers one compelling solution to address the miniaturization and ruggedization needed to enable clock portability, but brings with it a new set of challenges in recreating the functionality of an optical clock using chip-scale building blocks. The clock laser used for atom interrogation is one particular point of uncertainty, as the performance of the meticulously engineered bulk-cavity-stabilized lasers would be exceptionally difficult to transfer to chip. Here we demonstrate that an integrated ultrahigh-quality-factor spiral cavity, when interfaced with a 1,348 nm seed laser, is able to reach a fractional frequency instability of 7.5 × 10−14 on chip. On frequency doubling the light to 674 nm, we use this laser to interrogate the narrow-linewidth transition of 88Sr+ and showcase the operation of a Sr-ion clock with short-term instability averaging down as (3.9times 1{0}^{-14}/sqrt{tau }) (τ, averaging time). Our demonstration of a high-performance optical atomic clock interrogated by an integrated spiral cavity laser opens the door for future advanced clock systems to be entirely constructed using lightweight, portable and mass-manufacturable integrated optics and electronics.

光学原子钟在精确计时方面已经显示出革命性的进步,但它们对现实世界的适用性关键取决于这种钟能否在实验室之外运行。光子集成提供了一个引人注目的解决方案,以解决实现时钟便携性所需的小型化和坚固化问题,但在使用芯片级构建块重新创建光学时钟功能方面带来了一系列新的挑战。用于原子探测的时钟激光器是一个特别的不确定点,因为精心设计的体腔稳定激光器的性能将非常难以转移到芯片上。在这里,我们证明了集成的超高质量因子螺旋腔,当与1348 nm种子激光器接口时,能够在芯片上达到7.5 × 10−14的分数频率不稳定性。当频率加倍到674 nm时,我们使用该激光器来研究88Sr+的窄线宽跃迁,并展示了sr离子时钟的运行,其短期不稳定性平均为(3.9times 1{0}^{-14}/sqrt{tau }) (τ,平均时间)。我们演示的高性能光学原子钟由集成螺旋腔激光器进行查询,为未来先进的时钟系统打开了大门,该系统将完全使用轻质、便携式和可批量生产的集成光学和电子技术构建。
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引用次数: 0
Ultrafast nano-imaging of dark excitons 暗激子的超快纳米成像
IF 32.3 1区 物理与天体物理 Q1 OPTICS Pub Date : 2025-01-03 DOI: 10.1038/s41566-024-01568-y
David Schmitt, Jan Philipp Bange, Wiebke Bennecke, Giuseppe Meneghini, AbdulAziz AlMutairi, Marco Merboldt, Jonas Pöhls, Kenji Watanabe, Takashi Taniguchi, Sabine Steil, Daniel Steil, R. Thomas Weitz, Stephan Hofmann, Samuel Brem, G. S. Matthijs Jansen, Ermin Malic, Stefan Mathias, Marcel Reutzel
Understanding the impact of spatial heterogeneity on the behaviour of two-dimensional materials represents one of the grand challenges in applying these materials in optoelectronics and quantum information science. For transition metal dichalcogenide heterostructures in particular, direct access to heterogeneities in the dark-exciton landscape with nanometre spatial and ultrafast time resolution is highly desired but remains largely elusive. Here we report how ultrafast dark-field momentum microscopy can spatio-temporally resolve dark-exciton formation dynamics in a twisted WSe2/MoS2 heterostructure with a time resolution of 55 fs and a spatial resolution of 480 nm. This enables us to directly map spatial heterogeneity in the electronic and excitonic structure, and to correlate this with the dark-exciton formation and relaxation dynamics. The advantage of the simultaneous ultrafast nanoscale dark-field momentum microscopy and spectroscopy reported here is that it enables spatio-temporal imaging of the photoemission spectral function that carries energy- and momentum-resolved information on the single-particle band structure, many-body interactions and correlation phenomena. Dark-field momentum microscopy makes it possible to spatio-temporally and spatio-spectrally resolve the dark-exciton dynamics in a twisted transition metal dichalcogenide heterostructure.
了解空间异质性对二维材料行为的影响是将这些材料应用于光电子学和量子信息科学的重大挑战之一。特别是对于过渡金属二硫化物异质结构,在纳米空间和超快时间分辨率下直接获得暗激子景观中的异质性是非常需要的,但在很大程度上仍然难以实现。在这里,我们报道了超快暗场动量显微镜如何在时空上分辨扭曲WSe2/MoS2异质结构中的暗激子形成动力学,时间分辨率为55 fs,空间分辨率为480 nm。这使我们能够直接绘制电子和激子结构的空间异质性,并将其与暗激子的形成和弛豫动力学联系起来。本文报道的超快纳米尺度暗场动量显微镜和光谱学的优势在于,它可以对携带单粒子带结构、多体相互作用和相关现象的能量和动量分辨信息的光电发射光谱函数进行时空成像。
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引用次数: 0
Intrinsic optical bistability of photon avalanching nanocrystals 光子雪崩纳米晶体的固有光学双稳性
IF 32.3 1区 物理与天体物理 Q1 OPTICS Pub Date : 2025-01-03 DOI: 10.1038/s41566-024-01577-x
Artiom Skripka, Zhuolei Zhang, Xiao Qi, Benedikt Ursprung, Peter Ercius, Bruce E. Cohen, P. James Schuck, Daniel Jaque, Emory M. Chan
Optically bistable materials respond to a single input with two possible optical outputs, contingent on excitation history. Such materials would be ideal for optical switching and memory, but the limited understanding of intrinsic optical bistability (IOB) prevents the development of nanoscale IOB materials suitable for devices. Here we demonstrate IOB in Nd3+-doped KPb2Cl5 avalanching nanoparticles, which switch with high contrast between luminescent and non-luminescent states, with hysteresis characteristic of bistability. We elucidate a non-thermal mechanism in which IOB originates from suppressed non-radiative relaxation in Nd3+ ions and from the positive feedback of photon avalanching, resulting in extreme, >200th-order optical nonlinearities. The modulation of laser pulsing tunes the hysteresis widths, and dual-laser excitation enables transistor-like optical switching. This control over nanoscale IOB establishes avalanching nanoparticles for photonic devices in which light is used to manipulate light. Intrinsic optical bistability in Nd3+-doped KPb2Cl5 avalanching nanoparticles enables high-contrast switching between luminescent and non-luminescent states and transistor-like optical responses. A non-thermal mechanism is discussed and >200th-order optical nonlinearities are shown to be possible.
光学双稳材料响应一个单一的输入与两个可能的光输出,取决于激发历史。这种材料将是光开关和存储的理想材料,但是对固有光双稳性(IOB)的有限理解阻碍了适合器件的纳米级IOB材料的发展。我们在Nd3+掺杂的KPb2Cl5雪崩纳米颗粒中展示了IOB,它在发光和非发光状态之间具有高对比度切换,具有双稳性的滞后特性。我们阐明了一种非热机制,其中IOB源于Nd3+离子的抑制非辐射弛豫和光子雪崩的正反馈,导致极端的200阶光学非线性。激光脉冲的调制可以调节迟滞宽度,双激光激发可以实现类似晶体管的光开关。这种对纳米级IOB的控制为光子器件建立了雪崩纳米粒子,其中光被用来操纵光。
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引用次数: 0
Hetero-integrated perovskite/Si3N4 on-chip photonic system 异质集成钙钛矿/氮化硅片上光子系统
IF 35 1区 物理与天体物理 Q1 OPTICS Pub Date : 2025-01-02 DOI: 10.1038/s41566-024-01603-y
Kun Liao, Yaxiao Lian, Maotao Yu, Zhuochen Du, Tianxiang Dai, Yaxin Wang, Haoming Yan, Shufang Wang, Cuicui Lu, C. T. Chan, Rui Zhu, Dawei Di, Xiaoyong Hu, Qihuang Gong

Integrated photonic chips hold substantial potential in optical communications, computing, light detection and ranging, sensing, and imaging, offering exceptional data throughput and low power consumption. A key objective is to build a monolithic on-chip photonic system that integrates light sources, processors and photodetectors on a single chip. However, this remains challenging due to limitations in materials engineering, chip integration techniques and design methods. Perovskites offer simple fabrication, tolerance to lattice mismatch, flexible bandgap tunability and low cost, making them promising for hetero-integration with silicon photonics. Here we propose and experimentally realize a near-infrared monolithic on-chip photonic system based on a perovskite/silicon nitride photonic platform, developing nano-hetero-integration technology to integrate efficient light-emitting diodes, high-performance processors and sensitive photodetectors. Photonic neural networks are implemented to perform photonic simulations and computer vision tasks. Our network efficiently predicts the topological invariant in a two-dimensional disordered Su–Schrieffer–Heeger model and simulates nonlinear topological models with an average fidelity of 87%. In addition, we achieve a test accuracy of over 85% in edge detection and 56% on the CIFAR-10 dataset using a scaled-up architecture. This work addresses the challenge of integrating diverse nanophotonic components on a chip, offering a promising solution for chip-integrated multifunctional photonic information processing.

集成光子芯片在光通信、计算、光探测和测距、传感和成像方面具有巨大的潜力,提供卓越的数据吞吐量和低功耗。一个关键目标是建立一个集成光源、处理器和光电探测器的单片片上光子系统。然而,由于材料工程、芯片集成技术和设计方法的限制,这仍然具有挑战性。钙钛矿具有简单的制造、对晶格失配的容错性、灵活的带隙可调性和低成本等优点,使它们有望与硅光子学进行异质集成。本文提出并实验实现了一种基于钙钛矿/氮化硅光子平台的近红外单片光子系统,发展了集成高效发光二极管、高性能处理器和灵敏光电探测器的纳米异质集成技术。光子神经网络被用于执行光子模拟和计算机视觉任务。我们的网络有效地预测了二维无序Su-Schrieffer-Heeger模型的拓扑不变量,并以87%的平均保真度模拟了非线性拓扑模型。此外,我们在边缘检测方面达到了85%以上的测试准确率,在CIFAR-10数据集上使用缩放架构达到了56%。这项工作解决了在芯片上集成各种纳米光子元件的挑战,为芯片集成多功能光子信息处理提供了一个有前途的解决方案。
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引用次数: 0
Non-Hermitian hybrid silicon photonic switching 非厄米杂化硅光子开关
IF 35 1区 物理与天体物理 Q1 OPTICS Pub Date : 2025-01-02 DOI: 10.1038/s41566-024-01579-9
Xilin Feng, Tianwei Wu, Zihe Gao, Haoqi Zhao, Shuang Wu, Yichi Zhang, Li Ge, Liang Feng

Leveraging the entire space of complex dielectric permittivity, non-Hermitian photonics has fundamentally altered wave propagation with complex optical potentials and has ushered in a host of new photonic applications. Through parity–time symmetry and its breaking—a delicate interplay between gain and loss—even the interaction between just two entities becomes counter-intuitive and intriguing. Here we realize, through hybrid III–V/Si integration, a scalable non-Hermitian switching network on a two-layer integrated photonic chip. Our platform is a hybrid, with a bottom silicon layer and a top InGaAsP layer that provides optical gain. By tuning the gain level in the top layer, vertically coupled waveguides operate below or above the exceptional point, where light is switched across two layers, among different input–output ports. For a single switching unit, the switching dynamics are ultrafast, on the order of 100 ps. In a large switching network, non-blocking and other diverse connectivities are established in single-wavelength and wavelength-selective switching, with high extinction ratios. Our approach adds scalable non-Hermitian switching to photonic design toolkits to simultaneously boost the switching time and bandwidth density to cutting-edge levels, therefore paving the way for compact and ultrafast monolithic integrated silicon photonics in next-generation optical information networks.

利用复杂介电常数的整个空间,非厄米光子从根本上改变了具有复杂光势的波传播,并开创了一系列新的光子应用。通过奇偶时间对称性及其破坏——增益与损失之间微妙的相互作用——即使只是两个实体之间的相互作用也变得反直觉而有趣。本文通过III-V /Si混合集成,在两层集成光子芯片上实现了可扩展的非厄米交换网络。我们的平台是一个混合平台,底部是硅层,顶部是提供光学增益的InGaAsP层。通过调整顶层的增益水平,垂直耦合波导在异常点以下或之上工作,在异常点上,光在不同的输入输出端口之间在两层之间切换。对于单个开关单元,开关动态非常快,约为100ps。在大型交换网络中,在单波长和波长选择交换中建立了非阻塞和其他多种连接,具有高消光比。我们的方法将可扩展的非厄米开关添加到光子设计工具包中,同时将开关时间和带宽密度提高到尖端水平,从而为下一代光信息网络中的紧凑和超快单片集成硅光子学铺平了道路。
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引用次数: 0
Observation of loss-enhanced magneto-optical effect 观测损耗增强磁光效应
IF 32.3 1区 物理与天体物理 Q1 OPTICS Pub Date : 2024-12-19 DOI: 10.1038/s41566-024-01592-y
Ya-Ping Ruan, Jiang-Shan Tang, Zhipeng Li, Haodong Wu, Wenpeng Zhou, Longqi Xiao, Jianfeng Chen, Shi-Jun Ge, Wei Hu, Han Zhang, Cheng-Wei Qiu, Wuming Liu, Hui Jing, Yan-Qing Lu, Keyu Xia
Magneto-optical (MO) effects have a pivotal role in modern photonic devices for light manipulation and sensing, but the study of these effects has so far been limited to the MO Faraday and Kerr effects. Conventional MO systems encounter considerable intrinsic losses, markedly hampering their ability to amplify the MO effects. Here we introduce a loss-enhanced MO effect to sublinearly amplify the frequency response of a non-Hermitian optical cavity under different background magnetic fields. This exceptional MO effect relies on an architecture of MO material embedded in a Fabry–Pérot cavity, accompanied by a polarization-dependent optical absorption, that is, linear dichroism, to construct a reconfigurable exceptional point. The experimental results show that two eigenmodes of the Fabry–Pérot cavity exhibit sublinear frequency splitting. By electrically reconfiguring the absorber, the eigenfrequency shift can be adaptively enhanced under different background magnetic fields. Using this effect, we demonstrate the detection of subtle magnetic field variations in a strong background, with the system’s response magnified by a factor exceeding 10 and sensitivity increased threefold compared with its conventional Hermitian counterpart. Our study leverages exceptional physics to study the MO effect and develops a new class of reconfigurable MO devices equipped with enhanced sensitivity for potential integration with photonic systems. The authors introduce a loss-enhanced magneto-optical effect and sublinearly amplify the frequency response of a non-Hermitian optical cavity under different background magnetic fields. This effect is exploited to detect subtle magnetic field variations against a strong background with enhanced system response and sensitivity.
磁光效应(MO)在现代光操纵和传感光子器件中起着关键作用,但迄今为止对这些效应的研究仅限于MO法拉第效应和克尔效应。传统的MO系统遇到相当大的内在损失,明显阻碍了它们放大MO效应的能力。本文引入损耗增强MO效应来亚线性放大非厄米光腔在不同背景磁场下的频率响应。这种特殊的MO效应依赖于MO材料嵌入法布里-帕姆罗腔的结构,伴随着偏振依赖的光学吸收,即线性二色性,来构建一个可重构的特殊点。实验结果表明,法布里-普氏腔的两个本征模表现出亚线性频裂。通过电重构吸收器,可以自适应增强不同背景磁场下的本征频移。利用这一效应,我们展示了在强背景下检测细微磁场变化的能力,与传统的厄米对应物相比,系统的响应放大了10倍以上,灵敏度提高了3倍。我们的研究利用特殊的物理学来研究MO效应,并开发了一类新的可重构MO器件,该器件具有增强的灵敏度,可以与光子系统集成。
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引用次数: 0
Ultrabright molecular scintillators enabled by lanthanide-assisted near-unity triplet exciton recycling 由镧系元素辅助的近单位三重激子再循环实现的超亮分子闪烁体
IF 32.3 1区 物理与天体物理 Q1 OPTICS Pub Date : 2024-12-13 DOI: 10.1038/s41566-024-01586-w
Jiahui Xu, Rui Luo, Zichao Luo, Jun Xu, Zhen Mu, Hongyu Bian, Siew Yin Chan, Benjamin Yue Hao Tan, Dongzhi Chi, Zhongfu An, Guichuan Xing, Xian Qin, Changyang Gong, Yiming Wu, Xiaogang Liu
The secondary X-rays generated by the interaction of high-energy particles with scintillators can be converted into lower-energy excitons through thermalization, emitting light in the process. Capturing these secondary X-ray quanta efficiently is key to enhancing scintillation performance and boosting radiation detector sensitivity. Here we report a molecular design strategy using organic ligands to reclaim energy lost during the relaxation of secondary X-rays. This approach results in an enhancement in radioluminescence within lanthanide metal complexes by more than three orders of magnitude. By controlling the triplet energy of these ligands, we enable lanthanide centres to capture dark triplet excitons with near-unity extraction efficiency. These excitons arise from the absorption of secondary X-rays and transferred to the lanthanide centres through resonance energy transfer. This process delivers radioluminescence with orders of magnitude higher efficiency than existing organic or commercial inorganic scintillators. Tailoring metal centres and their coordination environments allows these organolanthanide scintillators to tune their spectra from ultraviolet to near-infrared, with lifetimes adjustable from tens of nanoseconds to hundreds of microseconds. These molecular scintillators enable high-resolution radiographic imaging and X-ray-mediated photodynamic therapy. Our findings not only unravel the link between scintillation performance and triplet exciton recycling but also lay the foundation for designing highly efficient organic scintillators that could revolutionize various fields. Researchers use organic ligands to reclaim energy lost during the relaxation of secondary X-rays generated by the interaction of high-energy particles with scintillators. Enhanced radioluminescence within lanthanide metal complexes and capture of dark triplet excitons with near-unity extraction efficiency are achieved.
高能粒子与闪烁体相互作用产生的二次 X 射线可通过热化转化为低能激子,并在此过程中发光。有效捕捉这些次级 X 射线量子是提高闪烁性能和辐射探测器灵敏度的关键。在此,我们报告了一种利用有机配体回收二次 X 射线弛豫过程中损失的能量的分子设计策略。这种方法使镧系元素金属复合物的放射发光增强了三个数量级以上。通过控制这些配体的三重态能量,我们使镧系元素中心能够以接近统一的萃取效率捕获暗三重态激子。这些激子产生于对二次 X 射线的吸收,并通过共振能量转移转移到镧系元素中心。与现有的有机或商用无机闪烁体相比,这一过程的辐射效率要高出几个数量级。对金属中心及其配位环境进行定制,可使这些有机镧系闪烁体的光谱范围从紫外到近红外,寿命可从几十纳秒到几百微秒不等。这些分子闪烁体可实现高分辨率放射成像和 X 射线介导的光动力疗法。我们的发现不仅揭示了闪烁性能与三重激子再循环之间的联系,还为设计高效有机闪烁体奠定了基础,从而为各个领域带来革命性的变化。
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引用次数: 0
Tunnelling escape of waves 隧道式波浪的逃逸
IF 35 1区 物理与天体物理 Q1 OPTICS Pub Date : 2024-12-03 DOI: 10.1038/s41566-024-01578-w
David A. B. Miller, Zeyu Kuang, Owen D. Miller

Applications of waves in communications, information processing and sensing need a clear understanding of how many strongly coupled channels or degrees of freedom exist in and out of volumes of space and how the coupling falls off for larger numbers. Numerical results are possible, and some heuristics exist, but there has been no simple physical picture and explanation for arbitrary volumes. By considering waves from a bounding spherical volume, we show a clear onset of a tunnelling escape of waves that both defines a limiting number of well-coupled channels for any volume and explains the subsequent rapid fall-off of coupling strengths. The approach works over all size scales, from nanophotonics and small radiofrequency antennas up to imaging optics. It gives a unified view from the multipole expansions common for antennas and small objects to the limiting plane and evanescent waves of large optics, showing that all such waves can escape to propagation to some degree, by tunnelling if necessary, and gives a precise diffraction limit.

波在通信、信息处理和传感中的应用需要清楚地了解有多少强耦合通道或自由度存在于空间体积内外,以及耦合如何在更大的数字中下降。数值结果是可能的,并且存在一些启发式的方法,但是对于任意体积还没有简单的物理图像和解释。通过考虑来自边界球形体积的波,我们显示了波隧穿逃逸的清晰开始,这既定义了任何体积的良好耦合通道的有限数量,也解释了随后耦合强度的快速下降。这种方法适用于各种尺寸,从纳米光子学和小型射频天线到成像光学。它给出了一个统一的观点,从天线和小物体常见的多极展开到大光学的极限平面和倏逝波,表明所有这些波都可以在某种程度上逃逸传播,必要时通过隧穿,并给出了精确的衍射极限。
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引用次数: 0
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Nature Photonics
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