首页 > 最新文献

Nature Photonics最新文献

英文 中文
Terabit-scale high-fidelity diamond data storage 百万兆位级高保真钻石数据存储
IF 32.3 1区 物理与天体物理 Q1 OPTICS Pub Date : 2024-11-27 DOI: 10.1038/s41566-024-01573-1
Jingyang Zhou, Jia Su, Junyu Guan, Yichen Yang, Wentao Ji, Mengqi Wang, Fazhan Shi, Kangwei Xia, Ya Wang, Jiangfeng Du
In the era of digital information, realizing efficient and durable data storage solutions is paramount. Innovations in storage capacity, data throughput, device lifespan and energy consumption are pressing necessities for the continuous progression of practical digital data storage technologies. Here we present a diamond storage medium that exploits fluorescent vacancy centres as robust storage units and provides a high storage density of 14.8 Tbit cm−3, a short write time of 200 fs and an estimated ultralong maintenance-free lifespan on the scale of millions of years. High-speed readout through plane and volume imaging is demonstrated with a high fidelity exceeding 99%, showing that the approach addresses the practical demands of digital data storage and provides a promising solution for future storage requirements. A diamond storage medium that uses fluorescent vacancy centres as robust storage units provides a high storage density of 14.8 Tbit cm−3.
在数字信息时代,实现高效耐用的数据存储解决方案至关重要。存储容量、数据吞吐量、设备寿命和能耗方面的创新是实用数字数据存储技术不断进步的迫切需要。我们在此介绍一种金刚石存储介质,它利用荧光空缺中心作为坚固的存储单元,可提供 14.8 Tbit cm-3 的高存储密度、200 fs 的短写入时间以及预计数百万年的超长免维护寿命。通过平面和体积成像展示了高速读出,保真度超过 99%,这表明该方法满足了数字数据存储的实际需求,并为未来的存储需求提供了一个前景广阔的解决方案。
{"title":"Terabit-scale high-fidelity diamond data storage","authors":"Jingyang Zhou, Jia Su, Junyu Guan, Yichen Yang, Wentao Ji, Mengqi Wang, Fazhan Shi, Kangwei Xia, Ya Wang, Jiangfeng Du","doi":"10.1038/s41566-024-01573-1","DOIUrl":"10.1038/s41566-024-01573-1","url":null,"abstract":"In the era of digital information, realizing efficient and durable data storage solutions is paramount. Innovations in storage capacity, data throughput, device lifespan and energy consumption are pressing necessities for the continuous progression of practical digital data storage technologies. Here we present a diamond storage medium that exploits fluorescent vacancy centres as robust storage units and provides a high storage density of 14.8 Tbit cm−3, a short write time of 200 fs and an estimated ultralong maintenance-free lifespan on the scale of millions of years. High-speed readout through plane and volume imaging is demonstrated with a high fidelity exceeding 99%, showing that the approach addresses the practical demands of digital data storage and provides a promising solution for future storage requirements. A diamond storage medium that uses fluorescent vacancy centres as robust storage units provides a high storage density of 14.8 Tbit cm−3.","PeriodicalId":18926,"journal":{"name":"Nature Photonics","volume":"18 12","pages":"1327-1334"},"PeriodicalIF":32.3,"publicationDate":"2024-11-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142718257","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Optical pumping of electronic quantum Hall states with vortex light 用涡旋光对电子量子霍尔态进行光抽运
IF 32.3 1区 物理与天体物理 Q1 OPTICS Pub Date : 2024-11-26 DOI: 10.1038/s41566-024-01565-1
Deric Session, Mahmoud Jalali Mehrabad, Nikil Paithankar, Tobias Grass, Christian J. Eckhardt, Bin Cao, Daniel Gustavo Suárez Forero, Kevin Li, Mohammad S. Alam, Kenji Watanabe, Takashi Taniguchi, Glenn S. Solomon, Nathan Schine, Jay Sau, Roman Sordan, Mohammad Hafezi
A fundamental requirement for quantum technologies is the ability to coherently control the interaction between electrons and photons. However, in many scenarios involving the interaction between light and matter, the exchange of linear or angular momentum between electrons and photons is not feasible, a condition known as the dipole approximation limit. An example of a case beyond this limit that has remained experimentally elusive is when the interplay between chiral electrons and vortex light is considered, where the orbital angular momentum of light can be transferred to electrons. Here we present a mechanism for such an orbital angular momentum transfer from optical vortex beams to electronic quantum Hall states. Specifically, we identify a robust contribution to the radial photocurrent, in an annular graphene sample within the quantum Hall regime, that depends on the vorticity of light. This phenomenon can be interpreted as an optical pumping scheme, where the angular momentum of photons is transferred to electrons, generating a radial current, and the current direction is determined by the vorticity of the light. Our findings offer fundamental insights into the optical probing and manipulation of quantum coherence, with wide-ranging implications for advancing quantum coherent optoelectronics. Orbital angular momentum transfer from optical vortex beams to electronic quantum Hall states is reported in a graphene sheet, showing a robust contribution to the radial photocurrent that depends on the vorticity of light.
量子技术的一个基本要求是能够连贯地控制电子和光子之间的相互作用。然而,在许多涉及光与物质相互作用的情况下,电子和光子之间的线性或角动量交换是不可行的,这种情况被称为偶极近似极限。手性电子和涡旋光之间的相互作用就是超越这一极限的一个例子,在这种情况下,光的轨道角动量可以转移到电子上。在这里,我们提出了一种从光学涡旋光束到电子量子霍尔态的轨道角动量转移机制。具体来说,我们发现在量子霍尔机制下的环形石墨烯样品中,径向光电流的强大贡献取决于光的涡度。这种现象可以解释为一种光泵浦方案,即光子的角动量传递给电子,产生径向电流,电流方向由光的涡度决定。我们的发现为量子相干性的光学探测和操纵提供了基本见解,对推动量子相干光电子学的发展具有广泛影响。
{"title":"Optical pumping of electronic quantum Hall states with vortex light","authors":"Deric Session, Mahmoud Jalali Mehrabad, Nikil Paithankar, Tobias Grass, Christian J. Eckhardt, Bin Cao, Daniel Gustavo Suárez Forero, Kevin Li, Mohammad S. Alam, Kenji Watanabe, Takashi Taniguchi, Glenn S. Solomon, Nathan Schine, Jay Sau, Roman Sordan, Mohammad Hafezi","doi":"10.1038/s41566-024-01565-1","DOIUrl":"10.1038/s41566-024-01565-1","url":null,"abstract":"A fundamental requirement for quantum technologies is the ability to coherently control the interaction between electrons and photons. However, in many scenarios involving the interaction between light and matter, the exchange of linear or angular momentum between electrons and photons is not feasible, a condition known as the dipole approximation limit. An example of a case beyond this limit that has remained experimentally elusive is when the interplay between chiral electrons and vortex light is considered, where the orbital angular momentum of light can be transferred to electrons. Here we present a mechanism for such an orbital angular momentum transfer from optical vortex beams to electronic quantum Hall states. Specifically, we identify a robust contribution to the radial photocurrent, in an annular graphene sample within the quantum Hall regime, that depends on the vorticity of light. This phenomenon can be interpreted as an optical pumping scheme, where the angular momentum of photons is transferred to electrons, generating a radial current, and the current direction is determined by the vorticity of the light. Our findings offer fundamental insights into the optical probing and manipulation of quantum coherence, with wide-ranging implications for advancing quantum coherent optoelectronics. Orbital angular momentum transfer from optical vortex beams to electronic quantum Hall states is reported in a graphene sheet, showing a robust contribution to the radial photocurrent that depends on the vorticity of light.","PeriodicalId":18926,"journal":{"name":"Nature Photonics","volume":"19 2","pages":"156-161"},"PeriodicalIF":32.3,"publicationDate":"2024-11-26","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142712783","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Terawatt-attosecond hard X-ray free-electron laser at high repetition rate 高重复率的兆瓦-秒硬 X 射线自由电子激光器
IF 32.3 1区 物理与天体物理 Q1 OPTICS Pub Date : 2024-11-25 DOI: 10.1038/s41566-024-01566-0
Jiawei Yan, Weilun Qin, Ye Chen, Winfried Decking, Philipp Dijkstal, Marc Guetg, Ichiro Inoue, Naresh Kujala, Shan Liu, Tianyun Long, Najmeh Mirian, Gianluca Geloni
Ångstrom and attosecond are the fundamental spatiotemporal scales for electron dynamics in various materials. Although attosecond pulses with wavelengths comparable to the atomic scales are expected to be a key tool in advancing attosecond science, producing high-power hard X-ray attosecond pulses at ångstrom wavelengths remains a formidable challenge. Here, we report the generation of terawatt-scale attosecond hard X-ray pulses using a free-electron laser in a special operation mode. We achieved 9 keV single-spike X-ray pulses with a mean pulse energy of around 180 μJ, exceeding previous reports by more than an order of magnitude, and an estimated average pulse duration of 200 as at full-width at half-maximum. Exploiting the unique capability of the European XFEL, which can deliver ten pulse trains per second with each containing hundreds of pulses at megahertz repetition rates, this study demonstrates the generation of attosecond X-ray pulses at a 2.25 MHz repetition rate. These intense high-repetition-rate attosecond X-ray pulses present transformative prospects for structural and electronic damage-free X-ray measurements and attosecond time-resolved X-ray methodologies, heralding a new era in ultrafast X-ray science. Using the European XFEL free-electron laser, researchers demonstrate terawatt-scale, attosecond hard X-ray pulses. Ten pulse trains per second, each containing hundreds of pulses at megahertz repetition rates, are achieved. Such short and intense pulses at high repetition rate enable unprecedented damage-free X-ray measurements with attosecond temporal resolution.
埃秒和阿秒是各种材料中电子动力学的基本时空尺度。尽管波长与原子尺度相当的阿秒脉冲有望成为推动阿秒科学发展的关键工具,但在埃秒波长上产生大功率硬 X 射线阿秒脉冲仍然是一项艰巨的挑战。在此,我们报告了使用自由电子激光器在特殊运行模式下产生太瓦级阿秒硬 X 射线脉冲的情况。我们获得了 9 keV 的单尖峰 X 射线脉冲,其平均脉冲能量约为 180 μJ,比之前的报道高出一个数量级以上,估计平均脉冲持续时间为 200 秒(全宽半最大值)。欧洲 XFEL 每秒可产生十个脉冲串,每个脉冲串包含数百个百万赫兹重复率的脉冲,本研究利用这一独特能力,展示了以 2.25 MHz 重复率产生的阿秒 X 射线脉冲。这些强烈的高重复率阿秒 X 射线脉冲为结构和电子无损伤 X 射线测量以及阿秒时间分辨 X 射线方法带来了变革性的前景,预示着超快 X 射线科学进入了一个新时代。
{"title":"Terawatt-attosecond hard X-ray free-electron laser at high repetition rate","authors":"Jiawei Yan, Weilun Qin, Ye Chen, Winfried Decking, Philipp Dijkstal, Marc Guetg, Ichiro Inoue, Naresh Kujala, Shan Liu, Tianyun Long, Najmeh Mirian, Gianluca Geloni","doi":"10.1038/s41566-024-01566-0","DOIUrl":"10.1038/s41566-024-01566-0","url":null,"abstract":"Ångstrom and attosecond are the fundamental spatiotemporal scales for electron dynamics in various materials. Although attosecond pulses with wavelengths comparable to the atomic scales are expected to be a key tool in advancing attosecond science, producing high-power hard X-ray attosecond pulses at ångstrom wavelengths remains a formidable challenge. Here, we report the generation of terawatt-scale attosecond hard X-ray pulses using a free-electron laser in a special operation mode. We achieved 9 keV single-spike X-ray pulses with a mean pulse energy of around 180 μJ, exceeding previous reports by more than an order of magnitude, and an estimated average pulse duration of 200 as at full-width at half-maximum. Exploiting the unique capability of the European XFEL, which can deliver ten pulse trains per second with each containing hundreds of pulses at megahertz repetition rates, this study demonstrates the generation of attosecond X-ray pulses at a 2.25 MHz repetition rate. These intense high-repetition-rate attosecond X-ray pulses present transformative prospects for structural and electronic damage-free X-ray measurements and attosecond time-resolved X-ray methodologies, heralding a new era in ultrafast X-ray science. Using the European XFEL free-electron laser, researchers demonstrate terawatt-scale, attosecond hard X-ray pulses. Ten pulse trains per second, each containing hundreds of pulses at megahertz repetition rates, are achieved. Such short and intense pulses at high repetition rate enable unprecedented damage-free X-ray measurements with attosecond temporal resolution.","PeriodicalId":18926,"journal":{"name":"Nature Photonics","volume":"18 12","pages":"1293-1298"},"PeriodicalIF":32.3,"publicationDate":"2024-11-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.nature.com/articles/s41566-024-01566-0.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142697110","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Topological orbital angular momentum extraction and twofold protection of vortex transport 拓扑轨道角动量提取与涡流传输的双重保护
IF 32.3 1区 物理与天体物理 Q1 OPTICS Pub Date : 2024-11-20 DOI: 10.1038/s41566-024-01564-2
Zhichan Hu, Domenico Bongiovanni, Ziteng Wang, Xiangdong Wang, Daohong Song, Jingjun Xu, Roberto Morandotti, Hrvoje Buljan, Zhigang Chen
Vortex phenomena are ubiquitous in nature. In optics, despite the availability of numerous techniques for vortex generation and detection, topological protection of vortex transport with desired orbital angular momentum (OAM) remains a challenge. Here, by use of topological disclination, we demonstrate a scheme to confine and guide vortices featuring arbitrary high-order charges. Such a scheme relies on twofold topological protection: a non-trivial winding in momentum space due to chiral symmetry, and a non-trivial winding in real space due to the complex coupling of OAM modes across the disclination structure. We unveil a vorticity-coordinated rotational symmetry, which sets up a universal relation between the vortex topological charge and the rotational symmetry order of the system. As an example, we construct photonic disclination lattices with a single core but different Cn symmetries and achieve robust transport of an optical vortex with preserved OAM solely corresponding to one selected zero-energy vortex mode at the mid-gap. Furthermore, we show that such topological structures can be used for vortex filtering to extract a chosen OAM mode from mixed excitations. Our results illustrate the fundamental interplay of vorticity, disclination and higher-order topology, which may open a new pathway for the development of OAM-based photonic devices such as vortex guides, fibres and lasers. Topological protection in disclination lattices that relies on non-trivial winding in momentum space and real space is used to confine and guide vortices that feature arbitrary high-order charges. This approach could help in the development of orbital angular momentum-based photonic devices.
涡旋现象在自然界无处不在。在光学领域,尽管有许多用于涡旋产生和检测的技术,但利用所需的轨道角动量(OAM)对涡旋传输进行拓扑保护仍然是一项挑战。在这里,我们利用拓扑分离技术展示了一种限制和引导具有任意高阶电荷的涡旋的方案。这种方案依赖于两方面的拓扑保护:手性对称导致的动量空间中的非三维缠绕,以及OAM 模式在整个剥离结构中的复杂耦合导致的实空间中的非三维缠绕。我们揭示了一种涡旋协调旋转对称性,它在涡旋拓扑电荷和系统旋转对称阶数之间建立了一种普遍关系。例如,我们构建了具有单核但不同 Cn 对称性的光子析构晶格,并实现了光涡旋的稳健传输,其保留的 OAM 完全对应于中隙处的一个选定零能涡旋模式。此外,我们还证明了这种拓扑结构可用于涡旋滤波,从混合激发中提取所选的 OAM 模式。我们的研究结果说明了涡度、偏离和高阶拓扑的基本相互作用,这可能为开发基于 OAM 的光子器件(如涡导、光纤和激光器)开辟一条新途径。
{"title":"Topological orbital angular momentum extraction and twofold protection of vortex transport","authors":"Zhichan Hu, Domenico Bongiovanni, Ziteng Wang, Xiangdong Wang, Daohong Song, Jingjun Xu, Roberto Morandotti, Hrvoje Buljan, Zhigang Chen","doi":"10.1038/s41566-024-01564-2","DOIUrl":"10.1038/s41566-024-01564-2","url":null,"abstract":"Vortex phenomena are ubiquitous in nature. In optics, despite the availability of numerous techniques for vortex generation and detection, topological protection of vortex transport with desired orbital angular momentum (OAM) remains a challenge. Here, by use of topological disclination, we demonstrate a scheme to confine and guide vortices featuring arbitrary high-order charges. Such a scheme relies on twofold topological protection: a non-trivial winding in momentum space due to chiral symmetry, and a non-trivial winding in real space due to the complex coupling of OAM modes across the disclination structure. We unveil a vorticity-coordinated rotational symmetry, which sets up a universal relation between the vortex topological charge and the rotational symmetry order of the system. As an example, we construct photonic disclination lattices with a single core but different Cn symmetries and achieve robust transport of an optical vortex with preserved OAM solely corresponding to one selected zero-energy vortex mode at the mid-gap. Furthermore, we show that such topological structures can be used for vortex filtering to extract a chosen OAM mode from mixed excitations. Our results illustrate the fundamental interplay of vorticity, disclination and higher-order topology, which may open a new pathway for the development of OAM-based photonic devices such as vortex guides, fibres and lasers. Topological protection in disclination lattices that relies on non-trivial winding in momentum space and real space is used to confine and guide vortices that feature arbitrary high-order charges. This approach could help in the development of orbital angular momentum-based photonic devices.","PeriodicalId":18926,"journal":{"name":"Nature Photonics","volume":"19 2","pages":"162-169"},"PeriodicalIF":32.3,"publicationDate":"2024-11-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.nature.com/articles/s41566-024-01564-2.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142673513","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Expanding momentum bandgaps in photonic time crystals through resonances 通过共振扩大光子时间晶体的动量带隙
IF 32.3 1区 物理与天体物理 Q1 OPTICS Pub Date : 2024-11-12 DOI: 10.1038/s41566-024-01563-3
X. Wang, P. Garg, M. S. Mirmoosa, A. G. Lamprianidis, C. Rockstuhl, V. S. Asadchy
The realization of photonic time crystals is a major opportunity but also comes with considerable challenges. The most pressing one, potentially, is the requirement for a substantial modulation strength in the material properties to create a noticeable momentum bandgap. Reaching that noticeable bandgap in optics is highly demanding with current, and possibly also future materials platforms because their modulation strength is small by tendency. Here we demonstrate that by introducing temporal variations in a resonant material, the momentum bandgap can be drastically expanded with modulation strengths in reach with known low-loss materials and realistic laser pump powers. The resonance can emerge from an intrinsic material resonance or a suitably spatially structured material supporting a structural resonance. Our concept is validated for resonant bulk media and optical metasurfaces and paves the way towards the first experimental realizations of photonic time crystals. Optical realization of photonic time crystals can be achieved by using temporal variations in a resonant material to expand the momentum bandgap, even at low modulation strengths, with known low-loss materials and realistic laser pump powers.
实现光子时间晶体是一个重大机遇,但同时也面临着相当大的挑战。最紧迫的挑战可能是要求材料特性具有相当大的调制强度,以产生明显的动量带隙。要在光学领域达到这种明显的带隙,对目前的材料平台,甚至未来的材料平台都有很高的要求,因为它们的调制强度往往很小。在这里,我们证明了通过在共振材料中引入时间变化,可以极大地扩展动量带隙,其调制强度与已知的低损耗材料和实际激光泵浦功率相当。共振可以来自材料本身的共振,也可以来自支持结构共振的适当空间结构材料。我们的概念得到了共振块体介质和光学元表面的验证,并为光子时间晶体的首次实验实现铺平了道路。
{"title":"Expanding momentum bandgaps in photonic time crystals through resonances","authors":"X. Wang, P. Garg, M. S. Mirmoosa, A. G. Lamprianidis, C. Rockstuhl, V. S. Asadchy","doi":"10.1038/s41566-024-01563-3","DOIUrl":"10.1038/s41566-024-01563-3","url":null,"abstract":"The realization of photonic time crystals is a major opportunity but also comes with considerable challenges. The most pressing one, potentially, is the requirement for a substantial modulation strength in the material properties to create a noticeable momentum bandgap. Reaching that noticeable bandgap in optics is highly demanding with current, and possibly also future materials platforms because their modulation strength is small by tendency. Here we demonstrate that by introducing temporal variations in a resonant material, the momentum bandgap can be drastically expanded with modulation strengths in reach with known low-loss materials and realistic laser pump powers. The resonance can emerge from an intrinsic material resonance or a suitably spatially structured material supporting a structural resonance. Our concept is validated for resonant bulk media and optical metasurfaces and paves the way towards the first experimental realizations of photonic time crystals. Optical realization of photonic time crystals can be achieved by using temporal variations in a resonant material to expand the momentum bandgap, even at low modulation strengths, with known low-loss materials and realistic laser pump powers.","PeriodicalId":18926,"journal":{"name":"Nature Photonics","volume":"19 2","pages":"149-155"},"PeriodicalIF":32.3,"publicationDate":"2024-11-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.nature.com/articles/s41566-024-01563-3.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142599378","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Author Correction: Image-guided computational holographic wavefront shaping 作者更正:图像引导的计算全息波前整形
IF 32.3 1区 物理与天体物理 Q1 OPTICS Pub Date : 2024-11-06 DOI: 10.1038/s41566-024-01585-x
Omri Haim, Jeremy Boger-Lombard, Ori Katz
{"title":"Author Correction: Image-guided computational holographic wavefront shaping","authors":"Omri Haim, Jeremy Boger-Lombard, Ori Katz","doi":"10.1038/s41566-024-01585-x","DOIUrl":"10.1038/s41566-024-01585-x","url":null,"abstract":"","PeriodicalId":18926,"journal":{"name":"Nature Photonics","volume":"19 1","pages":"116-116"},"PeriodicalIF":32.3,"publicationDate":"2024-11-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.nature.com/articles/s41566-024-01585-x.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142589101","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Efficient and stable perovskite-silicon tandem solar cells with copper thiocyanate-embedded perovskite on textured silicon 在纹理硅上使用硫氰酸铜嵌入包晶石的高效稳定的包晶石-硅串联太阳能电池
IF 32.3 1区 物理与天体物理 Q1 OPTICS Pub Date : 2024-11-04 DOI: 10.1038/s41566-024-01561-5
Chenxia Kan, Pengjie Hang, Shibo Wang, Biao Li, Xuegong Yu, Xinbo Yang, Yuxin Yao, Wei Shi, Stefaan De Wolf, Jun Yin, Daoyong Zhang, Degong Ding, Cao Yu, Shaofei Yang, Jiteng Zhang, Jia Yao, Xiaohong Zhang, Deren Yang
Monolithic perovskite/silicon tandem solar cells have achieved promising performance. However, hole transport layers that are commonly used for the perovskite top cell suffer from defects, non-conformal deposition or de-wetting of the overlying perovskite on the textured silicon bottom cells. These issues detrimentally affect device reproducibility and scalability, and thus commercialization. Here we address these challenges through the co-deposition of copper(I) thiocyanate and perovskite, where effective perovskite grain boundary passivation and efficient hole collection are simultaneously achieved by the embedded copper(I) thiocyanate, which creates local hole-collecting contacts. Fabricated monolithic perovskite/silicon tandem devices achieve a certified power conversion efficiency of 31.46% for 1 cm2 area devices. Aside from good reproducibility and scalability, our tandem cells exhibit excellent stability, maintaining 93.8% of their initial power conversion efficiency after about 1,200 h of maximum power point tracking at 45 °C, and 90.2% after over 1,000 h of damp-heat testing at 85 °C and 85% relative humidity. Co-deposition of copper thiocyanate with perovskite on textured silicon enables an efficient perovskite-silicon tandem solar cell with a certified power conversion efficiency of 31.46% for 1 cm2 area devices.
单片式过氧化物/硅串联太阳能电池已经取得了可喜的性能。然而,通常用于顶部包晶石电池的空穴传输层存在缺陷、不规则沉积或纹理硅底部电池上覆包晶石的去湿问题。这些问题严重影响了设备的可重复性和可扩展性,进而影响了商业化。在这里,我们通过硫氰酸铜(I)和包晶石的共沉积来解决这些难题,嵌入的硫氰酸铜(I)可同时实现有效的包晶石晶界钝化和高效的空穴收集,从而形成局部空穴收集接触。在 1 平方厘米面积的器件上,制作的单片闪长岩/硅串联器件的功率转换效率达到了 31.46%。除了良好的重现性和可扩展性外,我们的串联电池还表现出卓越的稳定性,在 45 °C、最大功率点跟踪约 1,200 小时后,仍能保持 93.8% 的初始功率转换效率;在 85 °C、相对湿度 85% 的条件下,经过超过 1,000 小时的湿热测试后,仍能保持 90.2% 的转换效率。
{"title":"Efficient and stable perovskite-silicon tandem solar cells with copper thiocyanate-embedded perovskite on textured silicon","authors":"Chenxia Kan, Pengjie Hang, Shibo Wang, Biao Li, Xuegong Yu, Xinbo Yang, Yuxin Yao, Wei Shi, Stefaan De Wolf, Jun Yin, Daoyong Zhang, Degong Ding, Cao Yu, Shaofei Yang, Jiteng Zhang, Jia Yao, Xiaohong Zhang, Deren Yang","doi":"10.1038/s41566-024-01561-5","DOIUrl":"10.1038/s41566-024-01561-5","url":null,"abstract":"Monolithic perovskite/silicon tandem solar cells have achieved promising performance. However, hole transport layers that are commonly used for the perovskite top cell suffer from defects, non-conformal deposition or de-wetting of the overlying perovskite on the textured silicon bottom cells. These issues detrimentally affect device reproducibility and scalability, and thus commercialization. Here we address these challenges through the co-deposition of copper(I) thiocyanate and perovskite, where effective perovskite grain boundary passivation and efficient hole collection are simultaneously achieved by the embedded copper(I) thiocyanate, which creates local hole-collecting contacts. Fabricated monolithic perovskite/silicon tandem devices achieve a certified power conversion efficiency of 31.46% for 1 cm2 area devices. Aside from good reproducibility and scalability, our tandem cells exhibit excellent stability, maintaining 93.8% of their initial power conversion efficiency after about 1,200 h of maximum power point tracking at 45 °C, and 90.2% after over 1,000 h of damp-heat testing at 85 °C and 85% relative humidity. Co-deposition of copper thiocyanate with perovskite on textured silicon enables an efficient perovskite-silicon tandem solar cell with a certified power conversion efficiency of 31.46% for 1 cm2 area devices.","PeriodicalId":18926,"journal":{"name":"Nature Photonics","volume":"19 1","pages":"63-70"},"PeriodicalIF":32.3,"publicationDate":"2024-11-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142574314","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Minute-scale Schrödinger-cat state of spin-5/2 atoms 自旋 5/2 原子的微尺度薛定谔猫态
IF 32.3 1区 物理与天体物理 Q1 OPTICS Pub Date : 2024-11-01 DOI: 10.1038/s41566-024-01555-3
Y. A. Yang, W.-T. Luo, J.-L. Zhang, S.-Z. Wang, Chang-Ling Zou, T. Xia, Z.-T. Lu
Quantum metrology with non-classical states offers a promising route to improved precision in physical measurements. The quantum effects of Schrödinger-cat superpositions or entanglements enable measurement uncertainties to reach below the standard quantum limit. However, the challenge of maintaining a long coherence time for such non-classical states often prevents full exploitation of the quantum advantage in metrology. Here we demonstrate a long-lived Schrödinger-cat state of optically trapped 173Yb (I = 5/2) atoms. The cat state, a superposition of two oppositely directed and furthest-apart spin states, is generated by a nonlinear spin rotation. Protected in a decoherence-free subspace against inhomogeneous light shifts of an optical lattice, the cat state persists for a coherence time of 1.4(1) × 103 s. A magnetic field is measured using Ramsey interferometry, demonstrating a scheme of Heisenberg-limited metrology for atomic magnetometry, quantum information processing and searching for new physics beyond the Standard Model. Using spin-5/2 nuclei of 173Yb atoms trapped in an optical lattice, a Schrödinger-cat state persists for a coherence time of 1.4 × 103 s. In measuring external magnetic fields, the cat state exhibits a sensitivity approaching the Heisenberg limit.
使用非经典状态的量子计量学为提高物理测量精度提供了一条前景广阔的途径。薛定谔猫叠加或纠缠的量子效应使测量的不确定性达到标准量子极限以下。然而,要使这种非经典状态保持较长的相干时间,往往会阻碍在计量学中充分发挥量子优势。在这里,我们展示了光学捕获的 173Yb (I = 5/2) 原子的长寿命薛定谔猫态。猫态是两个方向相反、相距最远的自旋态的叠加,由非线性自旋旋转产生。猫态在无退相干子空间中受到光晶格不均匀光偏移的保护,其相干时间为 1.4(1) × 103 秒。利用拉姆齐干涉测量法测量磁场,为原子磁力测量、量子信息处理和寻找标准模型之外的新物理学展示了一种海森堡限制计量方案。
{"title":"Minute-scale Schrödinger-cat state of spin-5/2 atoms","authors":"Y. A. Yang, W.-T. Luo, J.-L. Zhang, S.-Z. Wang, Chang-Ling Zou, T. Xia, Z.-T. Lu","doi":"10.1038/s41566-024-01555-3","DOIUrl":"10.1038/s41566-024-01555-3","url":null,"abstract":"Quantum metrology with non-classical states offers a promising route to improved precision in physical measurements. The quantum effects of Schrödinger-cat superpositions or entanglements enable measurement uncertainties to reach below the standard quantum limit. However, the challenge of maintaining a long coherence time for such non-classical states often prevents full exploitation of the quantum advantage in metrology. Here we demonstrate a long-lived Schrödinger-cat state of optically trapped 173Yb (I = 5/2) atoms. The cat state, a superposition of two oppositely directed and furthest-apart spin states, is generated by a nonlinear spin rotation. Protected in a decoherence-free subspace against inhomogeneous light shifts of an optical lattice, the cat state persists for a coherence time of 1.4(1) × 103 s. A magnetic field is measured using Ramsey interferometry, demonstrating a scheme of Heisenberg-limited metrology for atomic magnetometry, quantum information processing and searching for new physics beyond the Standard Model. Using spin-5/2 nuclei of 173Yb atoms trapped in an optical lattice, a Schrödinger-cat state persists for a coherence time of 1.4 × 103 s. In measuring external magnetic fields, the cat state exhibits a sensitivity approaching the Heisenberg limit.","PeriodicalId":18926,"journal":{"name":"Nature Photonics","volume":"19 1","pages":"89-94"},"PeriodicalIF":32.3,"publicationDate":"2024-11-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142561971","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Attosecond transient interferometry 阿秒瞬态干涉测量
IF 32.3 1区 物理与天体物理 Q1 OPTICS Pub Date : 2024-11-01 DOI: 10.1038/s41566-024-01556-2
Omer Kneller, Chen Mor, Nikolai D. Klimkin, Noa Yaffe, Michael Krüger, Doron Azoury, Ayelet J. Uzan-Narovlansky, Yotam Federman, Debobrata Rajak, Barry D. Bruner, Olga Smirnova, Serguei Patchkovskii, Yann Mairesse, Misha Ivanov, Nirit Dudovich
Attosecond transient absorption resolves the instantaneous response of a quantum system as it interacts with a laser field, by mapping its sub-cycle dynamics onto the absorption spectrum of attosecond pulses. However, the quantum dynamics are imprinted in the amplitude, phase and polarization state of the attosecond pulses. Here we introduce attosecond transient interferometry and measure the transient phase, as we follow its evolution within the optical cycle. We demonstrate how such phase information enables us to decouple the multiple quantum paths induced in a light-driven system, isolating their coherent contribution and retrieving their temporal evolution. Applying attosecond transient interferometry reveals the Stark shift dynamics in helium and retrieves long-term electronic coherences in neon. Finally, we present a vectorial generalization of our scheme, theoretically demonstrating the ability to isolate the underlying anomalous current in light-driven topological materials. Our scheme provides a direct insight into the interplay of light-induced dynamics and topology. Attosecond transient interferometry holds the potential to considerably extend the scope of attosecond metrology, revealing the underlying coherences in light-driven complex systems. Sub-cycle phase-resolved attosecond interferometry is developed. The obtained phase information enables us to decouple the multiple quantum paths induced in a light-driven system, isolating their coherent contribution and retrieving their temporal evolution.
阿秒瞬态吸收通过将量子系统的子周期动力学映射到阿秒脉冲的吸收光谱上,解析了量子系统与激光场相互作用时的瞬时响应。然而,量子动力学烙印在阿秒脉冲的振幅、相位和偏振态中。在此,我们引入了阿秒瞬态干涉测量法,并测量瞬态相位,同时跟踪其在光学周期内的演变。我们展示了这种相位信息如何使我们能够解耦光驱动系统中诱导的多个量子路径,分离它们的相干贡献并检索它们的时间演变。应用阿秒瞬态干涉测量揭示了氦中的斯塔克偏移动力学,并检索了氖中的长期电子相干性。最后,我们介绍了我们方案的矢量广义化,从理论上证明了隔离光驱动拓扑材料中潜在异常电流的能力。我们的方案直接揭示了光诱导动力学和拓扑学的相互作用。阿秒瞬态干涉测量有可能大大扩展阿秒计量学的范围,揭示光驱动复杂系统中的潜在一致性。
{"title":"Attosecond transient interferometry","authors":"Omer Kneller, Chen Mor, Nikolai D. Klimkin, Noa Yaffe, Michael Krüger, Doron Azoury, Ayelet J. Uzan-Narovlansky, Yotam Federman, Debobrata Rajak, Barry D. Bruner, Olga Smirnova, Serguei Patchkovskii, Yann Mairesse, Misha Ivanov, Nirit Dudovich","doi":"10.1038/s41566-024-01556-2","DOIUrl":"10.1038/s41566-024-01556-2","url":null,"abstract":"Attosecond transient absorption resolves the instantaneous response of a quantum system as it interacts with a laser field, by mapping its sub-cycle dynamics onto the absorption spectrum of attosecond pulses. However, the quantum dynamics are imprinted in the amplitude, phase and polarization state of the attosecond pulses. Here we introduce attosecond transient interferometry and measure the transient phase, as we follow its evolution within the optical cycle. We demonstrate how such phase information enables us to decouple the multiple quantum paths induced in a light-driven system, isolating their coherent contribution and retrieving their temporal evolution. Applying attosecond transient interferometry reveals the Stark shift dynamics in helium and retrieves long-term electronic coherences in neon. Finally, we present a vectorial generalization of our scheme, theoretically demonstrating the ability to isolate the underlying anomalous current in light-driven topological materials. Our scheme provides a direct insight into the interplay of light-induced dynamics and topology. Attosecond transient interferometry holds the potential to considerably extend the scope of attosecond metrology, revealing the underlying coherences in light-driven complex systems. Sub-cycle phase-resolved attosecond interferometry is developed. The obtained phase information enables us to decouple the multiple quantum paths induced in a light-driven system, isolating their coherent contribution and retrieving their temporal evolution.","PeriodicalId":18926,"journal":{"name":"Nature Photonics","volume":"19 2","pages":"134-141"},"PeriodicalIF":32.3,"publicationDate":"2024-11-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.nature.com/articles/s41566-024-01556-2.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142561970","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Small tunable X-ray sources may have large impact 小型可调谐 X 射线源可能产生巨大影响
IF 32.3 1区 物理与天体物理 Q1 OPTICS Pub Date : 2024-10-31 DOI: 10.1038/s41566-024-01552-6
Gordon Robb
Imaging in the water window has traditionally relied on large synchrotron radiation sources. Now, a tabletop tunable X-ray source which generates water-window X-ray photons from a low energy electron beam interacting with a van der Waals crystal has been demonstrated.
水窗成像历来依赖于大型同步辐射源。现在,一种台式可调 X 射线源已经问世,它能通过低能量电子束与范德华晶体的相互作用产生水窗 X 射线光子。
{"title":"Small tunable X-ray sources may have large impact","authors":"Gordon Robb","doi":"10.1038/s41566-024-01552-6","DOIUrl":"10.1038/s41566-024-01552-6","url":null,"abstract":"Imaging in the water window has traditionally relied on large synchrotron radiation sources. Now, a tabletop tunable X-ray source which generates water-window X-ray photons from a low energy electron beam interacting with a van der Waals crystal has been demonstrated.","PeriodicalId":18926,"journal":{"name":"Nature Photonics","volume":"18 11","pages":"1129-1130"},"PeriodicalIF":32.3,"publicationDate":"2024-10-31","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142556348","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
期刊
Nature Photonics
全部 Acc. Chem. Res. ACS Applied Bio Materials ACS Appl. Electron. Mater. ACS Appl. Energy Mater. ACS Appl. Mater. Interfaces ACS Appl. Nano Mater. ACS Appl. Polym. Mater. ACS BIOMATER-SCI ENG ACS Catal. ACS Cent. Sci. ACS Chem. Biol. ACS Chemical Health & Safety ACS Chem. Neurosci. ACS Comb. Sci. ACS Earth Space Chem. ACS Energy Lett. ACS Infect. Dis. ACS Macro Lett. ACS Mater. Lett. ACS Med. Chem. Lett. ACS Nano ACS Omega ACS Photonics ACS Sens. ACS Sustainable Chem. Eng. ACS Synth. Biol. Anal. Chem. BIOCHEMISTRY-US Bioconjugate Chem. BIOMACROMOLECULES Chem. Res. Toxicol. Chem. Rev. Chem. Mater. CRYST GROWTH DES ENERG FUEL Environ. Sci. Technol. Environ. Sci. Technol. Lett. Eur. J. Inorg. Chem. IND ENG CHEM RES Inorg. Chem. J. Agric. Food. Chem. J. Chem. Eng. Data J. Chem. Educ. J. Chem. Inf. Model. J. Chem. Theory Comput. J. Med. Chem. J. Nat. Prod. J PROTEOME RES J. Am. Chem. Soc. LANGMUIR MACROMOLECULES Mol. Pharmaceutics Nano Lett. Org. Lett. ORG PROCESS RES DEV ORGANOMETALLICS J. Org. Chem. J. Phys. Chem. J. Phys. Chem. A J. Phys. Chem. B J. Phys. Chem. C J. Phys. Chem. Lett. Analyst Anal. Methods Biomater. Sci. Catal. Sci. Technol. Chem. Commun. Chem. Soc. Rev. CHEM EDUC RES PRACT CRYSTENGCOMM Dalton Trans. Energy Environ. Sci. ENVIRON SCI-NANO ENVIRON SCI-PROC IMP ENVIRON SCI-WAT RES Faraday Discuss. Food Funct. Green Chem. Inorg. Chem. Front. Integr. Biol. J. Anal. At. Spectrom. J. Mater. Chem. A J. Mater. Chem. B J. Mater. Chem. C Lab Chip Mater. Chem. Front. Mater. Horiz. MEDCHEMCOMM Metallomics Mol. Biosyst. Mol. Syst. Des. Eng. Nanoscale Nanoscale Horiz. Nat. Prod. Rep. New J. Chem. Org. Biomol. Chem. Org. Chem. Front. PHOTOCH PHOTOBIO SCI PCCP Polym. Chem.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
0
微信
客服QQ
Book学术公众号 扫码关注我们
反馈
×
意见反馈
请填写您的意见或建议
请填写您的手机或邮箱
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
现在去查看 取消
×
提示
确定
Book学术官方微信
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术
文献互助 智能选刊 最新文献 互助须知 联系我们:info@booksci.cn
Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。
Copyright © 2023 Book学术 All rights reserved.
ghs 京公网安备 11010802042870号 京ICP备2023020795号-1