Nature Materials最新文献

英文中文

Electric-field-induced orbital angular momentum in metals 电场诱导的金属轨道角动量

IF 37.2 1区材料科学 Q1 CHEMISTRY, PHYSICAL

Nature Materials

Pub Date : 2024-09-30 DOI: 10.1038/s41563-024-01978-x

Kyung-Jin Lee, Vincent Cros, Hyun-Woo Lee

Electrons in solids carry orbital angular momentum in diverse non-equilibrium situations. This orbital current is often overlooked when considering electronic transport. Here we discuss how recent studies of orbital current are enabling more opportunities for technological advancements rooted in angular momentum.

固体中的电子在各种非平衡状态下携带轨道角动量。在考虑电子传输时，这种轨道电流常常被忽视。在此，我们将讨论最近对轨道电流的研究如何为以角动量为基础的技术进步带来更多机会。

引用次数: 0

An approach to identify and synthesize memristive III–V semiconductors 识别和合成记忆性 III-V 半导体的方法

IF 37.2 1区材料科学 Q1 CHEMISTRY, PHYSICAL

Nature Materials

Pub Date : 2024-09-30 DOI: 10.1038/s41563-024-01991-0

A class of III–V semiconductors with memristive properties has been created by combining computational screening and experimental synthesis. The synthesized compounds have gate-tunable synaptic functions, and could be used to create energy-efficient, reprogrammable logic devices that are compatible with existing silicon technology.

通过计算筛选和实验合成相结合的方法，创造出了一类具有记忆特性的 III-V 半导体。合成的化合物具有门调节突触功能，可用于制造与现有硅技术兼容的高能效、可重新编程的逻辑器件。

引用次数: 0

Tailoring phases on the device 设备上的定制阶段

IF 37.2 1区材料科学 Q1 CHEMISTRY, PHYSICAL

Nature Materials

Pub Date : 2024-09-30 DOI: 10.1038/s41563-024-01940-x

Yongjoon Lee, Heejun Yang

A phase engineering strategy, using a device configuration consisting of 2D channel materials and patterned electrodes, has been demonstrated. It achieves various phase configurations of 2D materials and versatile functions that can be tailored in situ.

利用由二维通道材料和图案化电极组成的设备配置，展示了一种相工程策略。它实现了二维材料的各种相态配置，以及可就地定制的多功能。

引用次数: 0

Tracking the irreversible light-induced creation of extended polar order from disorder 追踪光诱导下从无序中产生扩展极性秩序的不可逆过程

IF 37.2 1区材料科学 Q1 CHEMISTRY, PHYSICAL

Nature Materials

Pub Date : 2024-09-30 DOI: 10.1038/s41563-024-01992-z

Ultrafast laser light can create emergent polar orders in specially designed thin-film heterostructures. A single-shot X-ray diffraction study, over a timescale of seven orders of magnitude, has revealed how one such polar supercrystal forms with lattice periodicities of tens of nanometres.

超快激光能在专门设计的薄膜异质结构中产生新的极性秩序。一项时间跨度为七个数量级的单次 X 射线衍射研究揭示了这种极性超晶体是如何形成的，其晶格周期可达数十纳米。

引用次数: 0

Unconventional metal phase stabilizing metastable 2D materials 非常规金属相稳定可蜕变二维材料

IF 37.2 1区材料科学 Q1 CHEMISTRY, PHYSICAL

Nature Materials

Pub Date : 2024-09-30 DOI: 10.1038/s41563-024-01915-y

Yeonhee Lee, Gyeong-Hwan Kim, Jwa-Min Nam

Monolayers of metastable 1T′-phase transition metal dichalcogenides can be rapidly grown and stabilized on 4H-phase gold nanowires, providing a hybrid system for ultrasensitive surface-enhanced Raman scattering detection.

可在 4H 相金纳米线上快速生长和稳定可蜕变的 1T′ 相过渡金属二钙化物单层，为超灵敏表面增强拉曼散射检测提供了一种混合系统。

引用次数: 0

Tackling food allergies by microbiome modulation 通过调节微生物组解决食物过敏问题

IF 37.2 1区材料科学 Q1 CHEMISTRY, PHYSICAL

Nature Materials

Pub Date : 2024-09-30 DOI: 10.1038/s41563-024-02009-5

Benjamin J. Marsland, Nicola L. Harris

An oral immunotherapy consisting of an inulin-based gel loaded with an allergen successfully suppresses food allergy in mice.

一种口服免疫疗法包括一种含有过敏原的菊粉基凝胶，它能成功抑制小鼠对食物的过敏。

引用次数: 0

Pin the vortex on the superconductor 将涡旋固定在超导体上

IF 37.2 1区材料科学 Q1 CHEMISTRY, PHYSICAL

Nature Materials

Pub Date : 2024-09-30 DOI: 10.1038/s41563-024-01990-1

Xavier Obradors, Teresa Puig

Increasing the electronic carrier density in the overdoped state of high-temperature superconductors enhances the critical current density due to higher efficiency of vortex pinning defects.

在高温超导体的过掺杂状态下，电子载流子密度的增加会提高临界电流密度，这是因为涡流钉缺陷的效率更高。

引用次数: 0

Damage-free transfer printing 无损转印

IF 37.2 1区材料科学 Q1 CHEMISTRY, PHYSICAL

Nature Materials

Pub Date : 2024-09-30 DOI: 10.1038/s41563-024-01988-9

Yanzhen Li, Jiangtao Su, Xiaodong Chen

Precise stress control of thin films enables damage-free dry transfer printing onto flexible substrates.

对薄膜进行精确的应力控制，可在柔性基底上进行无损干式转印。

引用次数: 0

The hierarchical structure of organic mixed ionic–electronic conductors and its evolution in water 有机离子电子混合导体的分层结构及其在水中的演化

IF 41.2 1区材料科学 Q1 CHEMISTRY, PHYSICAL

Nature Materials

Pub Date : 2024-09-27 DOI: 10.1038/s41563-024-02016-6

Yael Tsarfati, Karen C. Bustillo, Benjamin H. Savitzky, Luke Balhorn, Tyler J. Quill, Adam Marks, Jennifer Donohue, Steven E. Zeltmann, Christopher J. Takacs, Alexander Giovannitti, Iain McCulloch, Colin Ophus, Andrew M. Minor, Alberto Salleo

Polymeric organic mixed ionic–electronic conductors underpin several technologies in which their electrochemical properties are desirable. These properties, however, depend on the microstructure that develops in their aqueous operational environment. We investigated the structure of a model organic mixed ionic–electronic conductor across multiple length scales using cryogenic four-dimensional scanning transmission electron microscopy in both its dry and hydrated states. Four-dimensional scanning transmission electron microscopy allows us to identify the prevalent defects in the polymer crystalline regions and to analyse the liquid crystalline nature of the polymer. The orientation maps of the dry and hydrated polymers show that swelling-induced disorder is mostly localized in discrete regions, thereby largely preserving the liquid crystalline order. Therefore, the liquid crystalline mesostructure makes electronic transport robust to electrolyte ingress. This study demonstrates that cryogenic four-dimensional scanning transmission electron microscopy provides multiscale structural insights into complex, hierarchical structures such as polymeric organic mixed ionic–electronic conductors, even in their hydrated operating state.

聚合有机离子电子混合导体是多种技术的基础，其电化学特性是这些技术所需要的。然而，这些特性取决于它们在水性工作环境中形成的微观结构。我们利用低温四维扫描透射电子显微镜研究了一种有机离子电子混合导体模型在干燥和水合状态下的多长度尺度结构。通过四维扫描透射电子显微镜，我们可以确定聚合物结晶区域的普遍缺陷，并分析聚合物的液晶性质。干聚合物和水合聚合物的取向图显示，膨胀引起的无序主要集中在离散区域，从而在很大程度上保持了液晶秩序。因此，液晶介观结构使电子传输不受电解质侵入的影响。这项研究表明，低温四维扫描透射电子显微镜可提供多尺度结构洞察，以了解复杂的分层结构，如聚合物有机混合离子电子导体，即使在其水合工作状态下也是如此。

{"title":"The hierarchical structure of organic mixed ionic–electronic conductors and its evolution in water","authors":"Yael Tsarfati, Karen C. Bustillo, Benjamin H. Savitzky, Luke Balhorn, Tyler J. Quill, Adam Marks, Jennifer Donohue, Steven E. Zeltmann, Christopher J. Takacs, Alexander Giovannitti, Iain McCulloch, Colin Ophus, Andrew M. Minor, Alberto Salleo","doi":"10.1038/s41563-024-02016-6","DOIUrl":"https://doi.org/10.1038/s41563-024-02016-6","url":null,"abstract":"<p>Polymeric organic mixed ionic–electronic conductors underpin several technologies in which their electrochemical properties are desirable. These properties, however, depend on the microstructure that develops in their aqueous operational environment. We investigated the structure of a model organic mixed ionic–electronic conductor across multiple length scales using cryogenic four-dimensional scanning transmission electron microscopy in both its dry and hydrated states. Four-dimensional scanning transmission electron microscopy allows us to identify the prevalent defects in the polymer crystalline regions and to analyse the liquid crystalline nature of the polymer. The orientation maps of the dry and hydrated polymers show that swelling-induced disorder is mostly localized in discrete regions, thereby largely preserving the liquid crystalline order. Therefore, the liquid crystalline mesostructure makes electronic transport robust to electrolyte ingress. This study demonstrates that cryogenic four-dimensional scanning transmission electron microscopy provides multiscale structural insights into complex, hierarchical structures such as polymeric organic mixed ionic–electronic conductors, even in their hydrated operating state.</p>","PeriodicalId":19058,"journal":{"name":"Nature Materials","volume":"11 1","pages":""},"PeriodicalIF":41.2,"publicationDate":"2024-09-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142322016","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Automated discovery of reprogrammable nonlinear dynamic metamaterials 自动发现可重新编程的非线性动态超材料

IF 37.2 1区材料科学 Q1 CHEMISTRY, PHYSICAL

Nature Materials

Pub Date : 2024-09-24 DOI: 10.1038/s41563-024-02008-6

Giovanni Bordiga, Eder Medina, Sina Jafarzadeh, Cyrill Bösch, Ryan P. Adams, Vincent Tournat, Katia Bertoldi

Harnessing the rich nonlinear dynamics of highly deformable materials has the potential to unlock the next generation of functional smart materials and devices. However, unlocking such potential requires effective strategies to spatially engineer material architectures within the nonlinear dynamic regime. Here we introduce an inverse-design framework to discover flexible mechanical metamaterials with a target nonlinear dynamic response. The desired dynamic task is encoded via optimal tuning of the full-scale metamaterial geometry through an inverse-design approach powered by a fully differentiable simulation environment. By deploying such a strategy, mechanical metamaterials are tailored for energy focusing, energy splitting, dynamic protection and nonlinear motion conversion. Furthermore, our design framework can be expanded to automatically discover reprogrammable architectures capable of switching between different dynamic tasks. For instance, we encode two strongly competing tasks—energy focusing and dynamic protection—within a single architecture, using static precompression to switch between these behaviours. The discovered designs are physically realized and experimentally tested, demonstrating the robustness of the engineered tasks. Our approach opens an untapped avenue towards designer materials with tailored robotic-like reprogrammable functionalities. A framework is presented to automate the design of flexible metamaterial structures that can execute desired nonlinear dynamic tasks and have reprogrammable functionality.

利用高度可变形材料丰富的非线性动力学特性，有可能开发出下一代功能性智能材料和设备。然而，释放这种潜力需要有效的策略，在非线性动态机制内对材料结构进行空间工程设计。在此，我们介绍一种逆向设计框架，用于发现具有目标非线性动态响应的柔性机械超材料。通过完全可微分仿真环境驱动的反设计方法，对全尺寸超材料几何形状进行优化调整，从而对所需的动态任务进行编码。通过采用这种策略，机械超材料可实现能量聚焦、能量分离、动态保护和非线性运动转换。此外，我们的设计框架还可以扩展到自动发现能够在不同动态任务之间切换的可重编架构。例如，我们将两个相互竞争的任务--能量集中和动态保护--编码到一个架构中，利用静态预压缩在这些行为之间进行切换。我们对所发现的设计进行了物理实现和实验测试，证明了工程任务的鲁棒性。我们的方法开辟了一条尚未开发的途径，使设计材料具有量身定制的类似机器人的可重新编程功能。

{"title":"Automated discovery of reprogrammable nonlinear dynamic metamaterials","authors":"Giovanni Bordiga, Eder Medina, Sina Jafarzadeh, Cyrill Bösch, Ryan P. Adams, Vincent Tournat, Katia Bertoldi","doi":"10.1038/s41563-024-02008-6","DOIUrl":"10.1038/s41563-024-02008-6","url":null,"abstract":"Harnessing the rich nonlinear dynamics of highly deformable materials has the potential to unlock the next generation of functional smart materials and devices. However, unlocking such potential requires effective strategies to spatially engineer material architectures within the nonlinear dynamic regime. Here we introduce an inverse-design framework to discover flexible mechanical metamaterials with a target nonlinear dynamic response. The desired dynamic task is encoded via optimal tuning of the full-scale metamaterial geometry through an inverse-design approach powered by a fully differentiable simulation environment. By deploying such a strategy, mechanical metamaterials are tailored for energy focusing, energy splitting, dynamic protection and nonlinear motion conversion. Furthermore, our design framework can be expanded to automatically discover reprogrammable architectures capable of switching between different dynamic tasks. For instance, we encode two strongly competing tasks—energy focusing and dynamic protection—within a single architecture, using static precompression to switch between these behaviours. The discovered designs are physically realized and experimentally tested, demonstrating the robustness of the engineered tasks. Our approach opens an untapped avenue towards designer materials with tailored robotic-like reprogrammable functionalities. A framework is presented to automate the design of flexible metamaterial structures that can execute desired nonlinear dynamic tasks and have reprogrammable functionality.","PeriodicalId":19058,"journal":{"name":"Nature Materials","volume":"23 11","pages":"1486-1494"},"PeriodicalIF":37.2,"publicationDate":"2024-09-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142317082","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

首页上一页

下一页尾页

类型

全部化学•材料生命科学医学物理工程技术环境•农林材料科学地球科学法学管理学化学环境科学与生态学计算机科学教育学经济学农林科学人文科学生物学数学物理与天体物理心理学综合性期刊其他工业工程理学历史学农学文学信息工程

数据库

全部 ACS Publications Elsevier ieeexplore Springer The Royal Society of Chemistry Wiley

期刊

Nature Materials

全部 Acc. Chem. Res. ACS Applied Bio Materials ACS Appl. Electron. Mater. ACS Appl. Energy Mater. ACS Appl. Mater. Interfaces ACS Appl. Nano Mater. ACS Appl. Polym. Mater. ACS BIOMATER-SCI ENG ACS Catal. ACS Cent. Sci. ACS Chem. Biol. ACS Chemical Health & Safety ACS Chem. Neurosci. ACS Comb. Sci. ACS Earth Space Chem. ACS Energy Lett. ACS Infect. Dis. ACS Macro Lett. ACS Mater. Lett. ACS Med. Chem. Lett. ACS Nano ACS Omega ACS Photonics ACS Sens. ACS Sustainable Chem. Eng. ACS Synth. Biol. Anal. Chem. BIOCHEMISTRY-US Bioconjugate Chem. BIOMACROMOLECULES Chem. Res. Toxicol. Chem. Rev. Chem. Mater. CRYST GROWTH DES ENERG FUEL Environ. Sci. Technol. Environ. Sci. Technol. Lett. Eur. J. Inorg. Chem. IND ENG CHEM RES Inorg. Chem. J. Agric. Food. Chem. J. Chem. Eng. Data J. Chem. Educ. J. Chem. Inf. Model. J. Chem. Theory Comput. J. Med. Chem. J. Nat. Prod. J PROTEOME RES J. Am. Chem. Soc. LANGMUIR MACROMOLECULES Mol. Pharmaceutics Nano Lett. Org. Lett. ORG PROCESS RES DEV ORGANOMETALLICS J. Org. Chem. J. Phys. Chem. J. Phys. Chem. A J. Phys. Chem. B J. Phys. Chem. C J. Phys. Chem. Lett. Analyst Anal. Methods Biomater. Sci. Catal. Sci. Technol. Chem. Commun. Chem. Soc. Rev. CHEM EDUC RES PRACT CRYSTENGCOMM Dalton Trans. Energy Environ. Sci. ENVIRON SCI-NANO ENVIRON SCI-PROC IMP ENVIRON SCI-WAT RES Faraday Discuss. Food Funct. Green Chem. Inorg. Chem. Front. Integr. Biol. J. Anal. At. Spectrom. J. Mater. Chem. A J. Mater. Chem. B J. Mater. Chem. C Lab Chip Mater. Chem. Front. Mater. Horiz. MEDCHEMCOMM Metallomics Mol. Biosyst. Mol. Syst. Des. Eng. Nanoscale Nanoscale Horiz. Nat. Prod. Rep. New J. Chem. Org. Biomol. Chem. Org. Chem. Front. PHOTOCH PHOTOBIO SCI PCCP Polym. Chem.

﹀