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High-throughput radiochemistry with phased “design of experiments” facilitates rapid and parallelized copper-mediated radiofluorination optimization. 高通量放射化学与阶段性的“实验设计”促进快速和并行的铜介导的放射性氟化优化。
IF 3 4区 医学 Q1 RADIOLOGY, NUCLEAR MEDICINE & MEDICAL IMAGING
Nuclear medicine and biology
Pub Date : 2025-11-01 DOI: 10.1016/j.nucmedbio.2025.109144
Gregory Bowden, Eric Webb, Kevin Cheng, Angela Han, Maxwell Geisler, Shelbie Cingoranelli, Melanie Sanford, Peter Scott
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引用次数: 0
Photomediated Radiohalogenation of Aryl Thianthrenium Salts Using 77Br, 125I, and 211At 用77Br、125I和21at进行芳基硫鎓盐的放射卤化
IF 3 4区 医学 Q1 RADIOLOGY, NUCLEAR MEDICINE & MEDICAL IMAGING
Nuclear medicine and biology
Pub Date : 2025-11-01 DOI: 10.1016/j.nucmedbio.2025.109133
Paul Martorano , Mehran Makvandi , Surendra Reddy Gundam , Siran Qian , Robert Mach , Jay Wright , Hsiaoju Lee
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引用次数: 0
Electroamalgamation-and Chromatography-Based Eu/Tb Separation Procedures as a Proof of Concept for Separating 155Tb from Alpha-Irradiated 153Eu 基于电合并和色谱的Eu/Tb分离程序作为从α辐照的153Eu中分离155Tb的概念验证
IF 3 4区 医学 Q1 RADIOLOGY, NUCLEAR MEDICINE & MEDICAL IMAGING
Nuclear medicine and biology
Pub Date : 2025-11-01 DOI: 10.1016/j.nucmedbio.2025.109134
Madhushan Serasinghe , Patrick Bokolo , Jack Lydon , James Guthrie , Steven Kelley , D. Scott Wilbur , Yawen Li , Dmitri Medvedev , Cathy Cutler , Carolyn Anderson , Silvia Jurisson , Heather Hennkens
{"title":"Electroamalgamation-and Chromatography-Based Eu/Tb Separation Procedures as a Proof of Concept for Separating 155Tb from Alpha-Irradiated 153Eu","authors":"Madhushan Serasinghe , Patrick Bokolo , Jack Lydon , James Guthrie , Steven Kelley , D. Scott Wilbur , Yawen Li , Dmitri Medvedev , Cathy Cutler , Carolyn Anderson , Silvia Jurisson , Heather Hennkens","doi":"10.1016/j.nucmedbio.2025.109134","DOIUrl":"10.1016/j.nucmedbio.2025.109134","url":null,"abstract":"","PeriodicalId":19363,"journal":{"name":"Nuclear medicine and biology","volume":"150 ","pages":"Article 109134"},"PeriodicalIF":3.0,"publicationDate":"2025-11-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145474077","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"医学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Breakthrough in 11C methylation of biologically interesting molecules: the case of [11C]PiB 生物学意义分子11C甲基化的突破：以[11C]PiB为例
IF 3 4区 医学 Q1 RADIOLOGY, NUCLEAR MEDICINE & MEDICAL IMAGING
Nuclear medicine and biology
Pub Date : 2025-11-01 DOI: 10.1016/j.nucmedbio.2025.109182
Muhammad Otabashi, Paolo Novelli, Romaric Gérardy, Simon Cerfontaine, Laura Trump, Fabrice Morelle, Corentin Warnier
{"title":"Breakthrough in 11C methylation of biologically interesting molecules: the case of [11C]PiB","authors":"Muhammad Otabashi, Paolo Novelli, Romaric Gérardy, Simon Cerfontaine, Laura Trump, Fabrice Morelle, Corentin Warnier","doi":"10.1016/j.nucmedbio.2025.109182","DOIUrl":"10.1016/j.nucmedbio.2025.109182","url":null,"abstract":"","PeriodicalId":19363,"journal":{"name":"Nuclear medicine and biology","volume":"150 ","pages":"Article 109182"},"PeriodicalIF":3.0,"publicationDate":"2025-11-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145474110","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"医学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Iminophosphorane Amino Acids as Precursors for 11C-Urea Radiotracers 亚磷酰氨基酸作为11c -尿素放射性示踪剂的前体
IF 3 4区 医学 Q1 RADIOLOGY, NUCLEAR MEDICINE & MEDICAL IMAGING
Nuclear medicine and biology
Pub Date : 2025-11-01 DOI: 10.1016/j.nucmedbio.2025.109128
Hala Almeneim , Hunter Valley , Abhishek Patel , Braeden Mair , Maxime Munch , Uzair Ismailani , Benjamin Rotstein
{"title":"Iminophosphorane Amino Acids as Precursors for 11C-Urea Radiotracers","authors":"Hala Almeneim , Hunter Valley , Abhishek Patel , Braeden Mair , Maxime Munch , Uzair Ismailani , Benjamin Rotstein","doi":"10.1016/j.nucmedbio.2025.109128","DOIUrl":"10.1016/j.nucmedbio.2025.109128","url":null,"abstract":"","PeriodicalId":19363,"journal":{"name":"Nuclear medicine and biology","volume":"150 ","pages":"Article 109128"},"PeriodicalIF":3.0,"publicationDate":"2025-11-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145474161","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"医学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
The Development of a Radiotracer Library for the Investigation of Cancer Cachexia with Positron Emission Tomography 用正电子发射断层扫描研究癌症恶病质的放射性示踪文库的建立
IF 3 4区 医学 Q1 RADIOLOGY, NUCLEAR MEDICINE & MEDICAL IMAGING
Nuclear medicine and biology
Pub Date : 2025-11-01 DOI: 10.1016/j.nucmedbio.2025.109129
Fraser Edgar , Lisa Duff , Emma Brown , Gavin Brown , Dmitry Soloviev , David Lewis
{"title":"The Development of a Radiotracer Library for the Investigation of Cancer Cachexia with Positron Emission Tomography","authors":"Fraser Edgar , Lisa Duff , Emma Brown , Gavin Brown , Dmitry Soloviev , David Lewis","doi":"10.1016/j.nucmedbio.2025.109129","DOIUrl":"10.1016/j.nucmedbio.2025.109129","url":null,"abstract":"","PeriodicalId":19363,"journal":{"name":"Nuclear medicine and biology","volume":"150 ","pages":"Article 109129"},"PeriodicalIF":3.0,"publicationDate":"2025-11-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145474162","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"医学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Estimation of the binding potential of the PET ligand [18F]FEDAC to translocator protein 18 kDa (TSPO) in the brain of experimental stroke model rats 脑卒中模型大鼠脑内PET配体FEDAC与转运蛋白18kda （TSPO）结合电位的估计[18F]
IF 3 4区 医学 Q1 RADIOLOGY, NUCLEAR MEDICINE & MEDICAL IMAGING
Nuclear medicine and biology
Pub Date : 2025-11-01 DOI: 10.1016/j.nucmedbio.2025.109579
Tomoteru Yamasaki , Yiding Zhang , Wakana Mori , Katsushi Kumata , Hidekatsu Wakizaka , Daisuke Arashi , Yusuke Kurihara , Masanao Ogawa , Nobuki Nengaki , Masayuki Fujinaga , Ming-Rong Zhang

Purpose

Translocator protein 18 kDa (TSPO) is a biomarker for neuroinflammation, and [18F]FEDAC was developed as a clinically usable radioligand for its imaging. Here, quantitative PET analyses of [18F]FEDAC in the brain of transient middle cerebral artery occlusion (tMCAO) rats were conducted for the first time.

Methods

Quantitative PET analysis was performed on rats subjected to tMCAO, with blood sampling also conducted as part of the study. To estimate the kinetic parameters of [18F]FEDAC, two-tissue compartment model (2TCM) and simplified reference tissue model (SRTM) analyses were conducted.

Results

The input rate (K1) and distribution volume (VT) (a macroparameter consisting of the K1–k4 rate constants from 2TCM analysis) of [18F]FEDAC in the ipsilateral area of tMCAO rats were 0.38 ± 0.19 mL/cm3/min and 5.4 ± 2.7 mL/cm3, respectively, which are roughly twice as high as those in the contralateral area. These results strongly suggest that ipsilateral binding potential (BPND), a quantitative index derived from the VT ratio with respect to the reference region, depends not only on the binding of [18F]FEDAC to TSPO, but also on increases in the input rate from blood. Therefore, in SRTM analyses, we corrected apparent BPND using R1, an index for probe delivery. In validation studies, SRTM analysis with the corrected BPND (corBPND), using the cerebellum as a reference, showed a high correlation with direct BPND (k3/k4) in 2TCM analyses.

Conclusion

The acquisition of quantitative PET images of TSPO distribution in the tMCAO rat brain was successfully achieved by scaling with corBPND.
目的转位蛋白18kda （TSPO）是神经炎症的生物标志物，[18F]FEDAC被开发为临床可用的放射配体用于其成像。本文首次对短暂性大脑中动脉闭塞（tMCAO）大鼠脑内[18F]FEDAC进行定量PET分析。方法对大鼠进行定量PET分析，并采血。为了估计[18F]FEDAC的动力学参数，我们进行了双组织室模型（2TCM）和简化参比组织模型（SRTM）分析。结果[18F]FEDAC在tMCAO大鼠同侧区的输入速率（K1）和分布体积（VT）分别为0.38±0.19 mL/cm3/min和5.4±2.7 mL/cm3，约为对侧区的2倍。这些结果强烈表明，同侧结合电位（BPND），一个由相对于参考区域的VT比率得出的定量指标，不仅取决于[18F]FEDAC与TSPO的结合，还取决于血液输入率的增加。因此，在SRTM分析中，我们使用R1（探针传递的指标）校正了明显的BPND。在验证研究中，以小脑为参照，SRTM分析与校正后的BPND （corBPND）在2个中医分析中显示与直接BPND （k3/k4）高度相关。结论corBPND标度法可成功获取TSPO分布的定量PET图像。
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引用次数: 0
Evaluating mRNA Delivery Using Nuclear Medicine 利用核医学评估mRNA传递
IF 3 4区 医学 Q1 RADIOLOGY, NUCLEAR MEDICINE & MEDICAL IMAGING
Nuclear medicine and biology
Pub Date : 2025-11-01 DOI: 10.1016/j.nucmedbio.2025.109117
James Humphries , Andrea Witjaksono , Abishek Poudel , Karine Mardon , Mary-anne Migotto , Seth Cheetham , Christopher Howard , Kristofer Thurecht
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引用次数: 0
Development and Validation of Blood-Brain Barrier-Penetrating Bispecific Antibodies for Brain ImmunoPET in Alzheimer's Disease and Glioblastoma 用于阿尔茨海默病和胶质母细胞瘤的脑免疫pet血脑屏障穿透双特异性抗体的研制和验证
IF 3 4区 医学 Q1 RADIOLOGY, NUCLEAR MEDICINE & MEDICAL IMAGING
Nuclear medicine and biology
Pub Date : 2025-11-01 DOI: 10.1016/j.nucmedbio.2025.109102
Lara Garcia-Varela , Dag Sehlin , Alberto Ouro , Jessica Codesido , María Muñoz , Sahar Roshanbin , Emma Ramos-Docampo , Ximena Aguilar , Noemí Gómez-Lado , Tomás Sobrino , Pablo Aguiar , Stina Syvaenen
{"title":"Development and Validation of Blood-Brain Barrier-Penetrating Bispecific Antibodies for Brain ImmunoPET in Alzheimer's Disease and Glioblastoma","authors":"Lara Garcia-Varela ,&nbsp;Dag Sehlin ,&nbsp;Alberto Ouro ,&nbsp;Jessica Codesido ,&nbsp;María Muñoz ,&nbsp;Sahar Roshanbin ,&nbsp;Emma Ramos-Docampo ,&nbsp;Ximena Aguilar ,&nbsp;Noemí Gómez-Lado ,&nbsp;Tomás Sobrino ,&nbsp;Pablo Aguiar ,&nbsp;Stina Syvaenen","doi":"10.1016/j.nucmedbio.2025.109102","DOIUrl":"10.1016/j.nucmedbio.2025.109102","url":null,"abstract":"","PeriodicalId":19363,"journal":{"name":"Nuclear medicine and biology","volume":"150 ","pages":"Article 109102"},"PeriodicalIF":3.0,"publicationDate":"2025-11-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145473536","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"医学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Imaging with Nanobody-based bimodal PET/fluorescence tracers for improved clinical decision making 基于纳米体的双峰PET/荧光示踪剂成像改善临床决策
IF 3 4区 医学 Q1 RADIOLOGY, NUCLEAR MEDICINE & MEDICAL IMAGING
Nuclear medicine and biology
Pub Date : 2025-11-01 DOI: 10.1016/j.nucmedbio.2025.109148
Jelena Saliën , Sam Floru , Romane Vizier , Jessica Bridoux , Victor Goncalves , Franck Denat , Sophie Hernot
{"title":"Imaging with Nanobody-based bimodal PET/fluorescence tracers for improved clinical decision making","authors":"Jelena Saliën ,&nbsp;Sam Floru ,&nbsp;Romane Vizier ,&nbsp;Jessica Bridoux ,&nbsp;Victor Goncalves ,&nbsp;Franck Denat ,&nbsp;Sophie Hernot","doi":"10.1016/j.nucmedbio.2025.109148","DOIUrl":"10.1016/j.nucmedbio.2025.109148","url":null,"abstract":"","PeriodicalId":19363,"journal":{"name":"Nuclear medicine and biology","volume":"150 ","pages":"Article 109148"},"PeriodicalIF":3.0,"publicationDate":"2025-11-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145473568","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"医学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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