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Femtosecond Bessel laser beam induced concentric rings on SiC for circular symmetry wide-viewing angle structural color 飞秒贝塞尔激光束在碳化硅上诱导同心圆环,实现圆形对称宽视角结构色
IF 4.6 2区 物理与天体物理 Q1 OPTICS Pub Date : 2024-09-17 DOI: 10.1016/j.optlastec.2024.111813

The laser-induced structural coloring technique holds significant potential for various applications due to its precision, controllability, and versatility across different materials. However, laser-induced structural colors face the problems of durability, homogeneity and indistinguishability, which are not conducive to their application as large-scale identifiable markers. In this paper, an innovative approach has been developed to achieve a circular-symmetric structural color display on durable SiC surfaces by fabricating periodic concentric ring structure arrays using the sidelobe light field of a femtosecond zero-order Bessel beam. The research involved a systematic study of the effects of laser power and pulse number on SiC, along with a detailed analysis of the micro-nanostructures evolving on the SiC surface after laser scanning. Additionally, an examination of the characteristics of circular-symmetric structural color displays and their wide viewing angles in periodic circular structures was conducted. Finally, a comparison was made between the structural color display effects of a concentric ring structure generated by a single pulse and the Laser-Induced Periodic Surface Structures (LIPSS) generated by three pulses. This comparison underscores the potential application of alternating between the high saturation color of the concentric ring structure and the low saturation dark light of the LIPSS for anti-counterfeit coding purposes. The findings of this research present promising opportunities for low-cost mass manufacturing in anti-counterfeit labeling and the advanced processing of photonic devices using SiC.

激光诱导结构着色技术因其精确性、可控性和在不同材料上的通用性而在各种应用中具有巨大潜力。然而,激光诱导结构色面临着耐久性、同质性和不可区分性等问题,不利于其作为大规模可识别标记的应用。本文开发了一种创新方法,利用飞秒零阶贝塞尔光束的侧射光场制作周期性同心环结构阵列,从而在耐用的碳化硅表面实现圆形对称结构色显示。研究包括系统研究激光功率和脉冲数对碳化硅的影响,以及详细分析激光扫描后在碳化硅表面演变的微纳米结构。此外,还研究了周期性圆形结构中圆形对称结构彩色显示器的特性及其宽视角。最后,还比较了单脉冲产生的同心环结构与三个脉冲产生的激光诱导周期表面结构(LIPSS)的结构色彩显示效果。这一对比强调了同心环结构的高饱和度色彩和激光诱导周期表面结构的低饱和度暗光交替显示在防伪编码上的潜在应用。这项研究成果为防伪标签的低成本大规模制造和使用碳化硅的光子设备的先进加工带来了大好机会。
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引用次数: 0
Mid-infrared self-pulse generation and enhanced pulse compression in Ho3+/Pr3+ co-doped lasers Ho3+/Pr3+ 共掺杂激光器中的中红外自脉冲生成和增强型脉冲压缩
IF 4.6 2区 物理与天体物理 Q1 OPTICS Pub Date : 2024-09-17 DOI: 10.1016/j.optlastec.2024.111788

The stable ∼ 3 μm self-pulsing laser has been achieved for the first time, along with compact and efficient pulse compression and amplification, based on the growth of novel Ho,Pr:GdScO3 crystals. Using the conventional Czochralski method, we have grown novel Ho,Pr:GdScO3 crystals with three different polarization-directions and discovered the self-pulsing effect within the crystals. Leveraging this phenomenon, we have successfully obtained linearly-polarized self-pulsing lasers in the mid-infrared (MIR) band and demonstrated the strong stability of the pulse trains both theoretically and experimentally. In addition, a novel pulse compression and enhancement method has been developed to maximize the performance of the self-pulsed Ho,Pr:GdScO3 lasers. Compared to self-pulsed lasers, the novel low-loss pulse compression can provide a more compact and efficient solution for enhancing the peak power of laser pulses. The results combine self-pulsed Ho,Pr:GdScO3 crystals with pulse compression and enhancement techniques to facilitate miniaturization and integration of high-peak-power, narrow-pulse-width MIR pulsed lasers.

基于新型 Ho,Pr:GdScO3晶体的生长,我们首次实现了稳定的 ∼ 3 μm 自脉冲激光,以及紧凑高效的脉冲压缩和放大。利用传统的 Czochralski 方法,我们生长出了具有三种不同偏振方向的新型 Ho,Pr:GdScO3 晶体,并发现了晶体内部的自脉冲效应。利用这一现象,我们成功获得了中红外(MIR)波段的线性偏振自脉冲激光器,并在理论和实验上证明了脉冲序列的强大稳定性。此外,我们还开发了一种新颖的脉冲压缩和增强方法,以最大限度地提高自脉冲 Ho,Pr:GdScO3 激光器的性能。与自脉冲激光器相比,新型低损耗脉冲压缩能为增强激光脉冲的峰值功率提供更紧凑、更高效的解决方案。该成果将自脉冲 Ho,Pr:GdScO3 晶体与脉冲压缩和增强技术相结合,促进了高峰值功率、窄脉冲宽度近红外脉冲激光器的小型化和集成化。
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引用次数: 0
Design and numerical investigation of Cs2SnI6 vacancy-ordered double perovskite solar cell Cs2SnI6 空位有序双包晶太阳能电池的设计与数值研究
IF 4.6 2区 物理与天体物理 Q1 OPTICS Pub Date : 2024-09-17 DOI: 10.1016/j.optlastec.2024.111820

Perovskite solar cells (PSCs) represent an emerging technology in solar photovoltaics due to their outstanding optical and electrical characteristics. The urgency of lead-free solar materials has increased due to the environmental concerns. In light of these considerations, Cs2SnI6, a high-performance tin-based double perovskite, holds the potential to be a key absorber material in promoting the cell efficiency. In this paper, a device design of lead-free Cs2SnI6-based PSC is proposed based on an n-i-p planar structure. Through a comprehensive analysis by simulation using SCAPS-1D, the impacts of electron transport layer materials (SnO2, TiO2, CdS, GO, MZO) and hole transport layer materials (MoO3, Cu2O, CuI, Spiro-OMeTAD) with varying thicknesses as well as the donor density, acceptor density and the absorber thickness have been examined. Additionally, an examination is conducted on the performance metrics of PSCs, encompassing Voc, Jsc, FF, and PCE, while taking into consideration the influences of temperature, Rseries, and Rshunt. The results show that the optimized FTO/SnO2/Cs2SnI6/MoO3/Au device presents the highest PCE of 22.60 % at 300 K temperature, together with a visible quantum efficiency of 99.49 %. The appropriate thicknesses of the ETL, HTL, and absorber layer for achieving the optimal performances are 50 nm, 200 nm, and 450 nm, respectively. Also, the donor density and acceptor density for the best efficiency are both at 1018 cm−3. The values of Rseries, and Rshunt are 2 Ω cm2 and 6000 Ω cm2, respectively. This investigation demonstrates that the proposed vacancy-ordered double perovskite Cs2SnI6 solar cell is promising for photovoltaic devices due to the highlighted characteristics and optical parameters.

过氧化物太阳能电池(PSC)具有出色的光学和电气特性,是太阳能光伏领域的一项新兴技术。由于环境问题,无铅太阳能材料的需求日益迫切。有鉴于此,Cs2SnI6--一种高性能锡基双过氧化物--有望成为提高电池效率的关键吸收材料。本文提出了一种基于 ni-i-p 平面结构的无铅 Cs2SnI6 基 PSC 器件设计。通过使用 SCAPS-1D 进行模拟综合分析,考察了不同厚度的电子传输层材料(SnO2、TiO2、CdS、GO、MZO)和空穴传输层材料(MoO3、Cu2O、CuI、Spiro-OMeTAD)以及供体密度、受体密度和吸收体厚度的影响。此外,还考察了 PSC 的性能指标,包括 Voc、Jsc、FF 和 PCE,同时考虑了温度、Rseries 和 Rshunt 的影响。结果表明,经过优化的 FTO/SnO2/Cs2SnI6/MoO3/Au 器件在 300 K 温度下的 PCE 最高,达到 22.60%,可见量子效率为 99.49%。为实现最佳性能,ETL、HTL 和吸收层的合适厚度分别为 50 nm、200 nm 和 450 nm。此外,实现最佳效率的供体密度和受体密度均为 1018 cm-3。Rseries 和 Rshunt 的值分别为 2 Ω cm2 和 6000 Ω cm2。这项研究表明,所提出的空位有序双包晶 Cs2SnI6 太阳能电池具有突出的特性和光学参数,有望用于光伏设备。
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引用次数: 0
Optical coherence measurement-based penetration depth monitoring of stainless steel sheets in laser lap welding using long short-term memory network 在激光搭接焊中利用长短期记忆网络对不锈钢板进行基于光学相干测量的渗透深度监测
IF 4.6 2区 物理与天体物理 Q1 OPTICS Pub Date : 2024-09-17 DOI: 10.1016/j.optlastec.2024.111811

The industrial production site for laser lap welding of thin stainless steel plates puts strict requests on the level and fluctuation stability of penetration depth. Hence, the penetration depth monitoring is increasingly garnering attention. This research proposes an optical coherence measurement-based approach to monitor penetration depth utilizing machine learning in laser lap welding for stainless steel sheets. After the acquisition of the keyhole depth signal by the coherent light beam, it is found that there is a significant association relationship between the reconstructed keyhole depth obtained by empirical modal decomposition and the penetration depth curve, but meanwhile a penetration depth monitoring error also exists. Accordingly, based on the cross-correlation analysis and numerical simulation, it is revealed that the formation mechanism and sources of this error are related to the “bottom melt layer thickness”, “hysteresis property” and “multiple reflections”. On this basis, a long short-term memory network is built to memorize the historical information of the reconstructed keyhole depth for predicting the penetration depth at each moment. The experimental results demonstrate that the prediction model has high accuracy and good generalization ability, and thus effective monitoring for penetration depth can be achieved.

不锈钢薄板激光搭接焊的工业生产现场对熔透深度的水平和波动稳定性有着严格的要求。因此,熔深监测越来越受到重视。本研究提出了一种基于光学相干测量的方法,利用机器学习在不锈钢板激光搭接焊中监测熔透深度。通过相干光束采集锁孔深度信号后发现,经验模态分解得到的重构锁孔深度与熔透深度曲线之间存在显著的关联关系,但同时也存在熔透深度监测误差。据此,基于交叉相关分析和数值模拟,揭示了该误差的形成机理和来源与 "底部熔层厚度"、"滞后特性 "和 "多重反射 "有关。在此基础上,建立了一个长短期记忆网络,用于记忆重建钥匙孔深度的历史信息,以预测每个时刻的穿透深度。实验结果表明,该预测模型具有较高的准确性和良好的泛化能力,从而可以实现对渗透深度的有效监测。
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引用次数: 0
Structure, spectroscopy and laser operation at ∼ 2.8 μm of a novel Er:SGGG crystal 新型 Er:SGGG 晶体的结构、光谱和 2.8 μm 波长的激光操作
IF 4.6 2区 物理与天体物理 Q1 OPTICS Pub Date : 2024-09-17 DOI: 10.1016/j.optlastec.2024.111797

We demonstrate the crystal structure, spectroscopy and laser performance of a novel Er:SGGG crystal grown successfully by Czochralski (Cz) method. The lattice constant is refined to be 12.42 Å and the FWHM of the crystal’s X-ray rocking curve is only 86.4″, indicating an excellent quality. The segregation coefficient of Er3+ ions in SGGG is determined to be 1.2. The Er:SGGG crystal displays a specialty in broadening spectrum. There is a wide absorption band near 962 nm, with an absorption bandwidth of 19 nm and a peak absorption coefficient of 5.57 cm−1. Under the conditions of 969 nm laser diode (LD) pumping, with a 400 Hz repetition rate and 300 μs pulse duration, a maximum power 404 mW with slope efficiency of 15.6 % at 2.8 μm is achieved on the Er:SGGG crystal. The M2 factors of horizontal and vertical are 1.4 and 1.5, respectively. The results indicate the mid-infrared laser output can be generated in the Er:SGGG crystal, and it is a potential and promising candidate for 2.8 μm laser material.

我们展示了用 Czochralski(Cz)方法成功生长的新型 Er:SGGG 晶体的晶体结构、光谱和激光性能。晶体的晶格常数被细化为 12.42 Å,X 射线摇摆曲线的 FWHM 仅为 86.4″,表明晶体质量极佳。经测定,SGGG 中 Er3+ 离子的偏析系数为 1.2。Er:SGGG 晶体在拓宽光谱方面具有特殊性。在 962 nm 附近有一个很宽的吸收带,吸收带宽为 19 nm,峰值吸收系数为 5.57 cm-1。在 969 nm 激光二极管(LD)泵浦、400 Hz 重复频率和 300 μs 脉冲持续时间条件下,Er:SGG 晶体在 2.8 μm 波长处的最大功率为 404 mW,斜率效率为 15.6%。水平和垂直的 M2 因子分别为 1.4 和 1.5。结果表明,Er:SGGG 晶体可以产生中红外激光输出,是一种有潜力、有前途的 2.8 μm 激光材料。
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引用次数: 0
A triplexer chip with cascaded butterfly multimode interference couplers by femtosecond laser microprocessing 利用飞秒激光微处理技术实现的带级联蝶形多模干涉耦合器的三重器芯片
IF 4.6 2区 物理与天体物理 Q1 OPTICS Pub Date : 2024-09-17 DOI: 10.1016/j.optlastec.2024.111753

A triplexer chip utilizing three cascaded butterfly multimode interference (MMI) couplers to output three optical signals from their respective ports is proposed. The chip consists of a borosilicate glass substrate, a JA photoresist core layer, and an RZJ photoresist cladding. The beam propagation method (BPM) is used to design and optimize the chip. The femtosecond laser processing is investigated, and the chip is processed with a laser power of 1.6 mW and an ablation speed of 4 mm/s. Tests show that the chip meets the design specifications with a low insertion loss of 4.34 dB, an extinction ratio of more than 15 dB, a crosstalk of less than −15 dB, and a 3 dB bandwidth up to 76.8 nm.

本文提出了一种三路光耦合器芯片,利用三个级联蝶形多模干涉(MMI)耦合器从各自端口输出三路光信号。该芯片由硼硅玻璃基板、JA 光刻胶核心层和 RZJ 光刻胶包层组成。芯片的设计和优化采用了光束传播法(BPM)。对飞秒激光加工进行了研究,芯片的加工激光功率为 1.6 mW,烧蚀速度为 4 mm/s。测试表明,该芯片符合设计规范,插入损耗低至 4.34 dB,消光比大于 15 dB,串扰小于 -15 dB,带宽达 3 dB,最高可达 76.8 nm。
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引用次数: 0
Study on the surface performance strengthening of AlCrN coated cemented carbide by micro-texture laser preparation process 利用微纹理激光制备工艺强化铝铬镍涂层硬质合金表面性能的研究
IF 4.6 2区 物理与天体物理 Q1 OPTICS Pub Date : 2024-09-17 DOI: 10.1016/j.optlastec.2024.111819

The combined application of coating and surface texture technology on the material surface can enhance its performance. However, the two procedure and their joint mechanism have not been fully revealed. Therefore, this paper takes the micro-textured coated cemented carbide as the research object, and focuses on the influence of preparation procedure and process parameters on surface characteristics and friction behavior. The results show that compared with the coating textured (XT) sample, the textured coating (XW) sample has more advantages in micro-hardness, microstructure and wear degree. The Rockwell hardness of the XT sample is better. Compared with the single coating sample, the coating micro-hardness of the XW sample is increased by 10 %, the Rockwell hardness is reduced by 2 %, the average grain size is reduced by 7.9 %, and the friction force is reduced by 6.2 %. Additionally, within a certain range, the increase of Al content will increase the sample hardness, reduce friction, and inhibit the Cr content and the growth of CrN phase grains. Complete process parameter optimization based on the ideal solution.

在材料表面联合应用涂层和表面纹理技术可以提高材料的性能。然而,这两种工艺及其联合机理尚未完全揭示。因此,本文以微纹理涂层硬质合金为研究对象,重点探讨了制备程序和工艺参数对表面特性和摩擦行为的影响。结果表明,与涂层纹理(XT)试样相比,纹理涂层(XW)试样在显微硬度、显微组织和磨损程度方面更具优势。XT 样品的洛氏硬度更好。与单涂层试样相比,XW 试样的涂层显微硬度提高了 10%,洛氏硬度降低了 2%,平均晶粒度降低了 7.9%,摩擦力降低了 6.2%。此外,在一定范围内,Al 含量的增加会提高试样硬度,降低摩擦力,并抑制 Cr 含量和 CrN 相晶粒的生长。基于理想方案的完整工艺参数优化。
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引用次数: 0
All-solid-state continuous-wave mode-locked Er:Lu2O3 laser at 3 µm 3 微米波长的全固态连续波模式锁定 Er:Lu2O3 激光器
IF 4.6 2区 物理与天体物理 Q1 OPTICS Pub Date : 2024-09-16 DOI: 10.1016/j.optlastec.2024.111787

In this paper, we demonstrated stable continuous-wave passively mode-locked operation of an Er:Lu2O3 laser at 3 µm, utilizing a semiconductor saturable absorber mirror (SESAM). By operating the laser in a dry nitrogen environment and utilizing a thermoelectric cooler (TEC) temperature control device to mitigate the thermal effects of Er:Lu2O3 and enhance laser stability, we further compensated for group delay dispersion within the laser cavity through chirped mirrors, an shortest pulse duration of 12.0 ps at a average output power of 150 mW was achieved, which occurred at a center wavelength of 2844 nm, and a pulse repetition rate of 83.5 MHz. Additionally, we achieved a maximum continuous-wave mode-locked output power of 213 mW at an absorbed pump power of 8.3 W, equivalent to a pulse energy of 1.3 nJ. The RF spectrum analysis of the pulse train indicated a high SNR of nearly 70 dB, signifying excellent stability. To the best of our knowledge, This is the first report on the realization of an ultrashort pulse width mode-locked Er:Lu2O3 laser in the mid-infrared band.

在本文中,我们利用半导体可饱和吸收镜 (SESAM) 演示了 3 µm 波长的 Er:Lu2O3 激光器的稳定连续波被动模式锁定运行。我们通过啁啾镜进一步补偿了激光腔内的群延迟色散,在中心波长为 2844 nm、脉冲重复率为 83.5 MHz 时,以 150 mW 的平均输出功率实现了 12.0 ps 的最短脉冲持续时间。此外,在吸收泵功率为 8.3 W 时,我们实现了 213 mW 的最大连续波锁相输出功率,相当于 1.3 nJ 的脉冲能量。对脉冲序列的射频频谱分析表明,信噪比高达近 70 dB,这标志着出色的稳定性。据我们所知,这是首次报道在中红外波段实现超短脉宽模式锁定的 Er:Lu2O3 激光器。
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引用次数: 0
Damage performance of alumina ceramic by femtosecond laser induced air filamentation 飞秒激光诱导空气丝化对氧化铝陶瓷的损伤性能
IF 4.6 2区 物理与天体物理 Q1 OPTICS Pub Date : 2024-09-16 DOI: 10.1016/j.optlastec.2024.111781

Hard and brittle materials, such as ceramics, are extensively utilized in defense and military protection. Studies on laser damage to ceramic materials have garnered significant attention, with a focus on efficient disruption over long-range. The femtosecond laser filamentation allows energy transfer on the order of kilometers, providing a unique advantage for applications requiring long-distance destruction. However, the interaction mechanism between femtosecond laser filamentation with hard and brittle materials remains unclear. This study initially simulates the interaction of femtosecond lasers with alumina ceramics at various pulse energies using the two-temperature equation. The results reveal the variation in electron and lattice temperature under the irradiation of femtosecond laser. Subsequently, the damage performance caused by femtosecond laser filamentation on ceramic materials, considering various pulse energies, filament positions, and ablation times are systematically investigated. Additionally, at a pulse energy of 4 mJ, the filament length focused by a 500 mm lens can extend up to 25 mm, resulting in an ablation hole with a diameter of 340 µm and a depth of 440 µm along the middle part of the filament. The power-clamping effect ensures uniform damage hole morphology and size across the entire filament, attributable to the constant filament diameter and plasma intensity. This elucidates the damage mechanism of filaments and adequately validates the effectiveness of this method, establishing a theoretical foundation for investigating laser remote damage of hard and brittle materials.

陶瓷等硬脆材料被广泛应用于国防和军事保护领域。有关激光破坏陶瓷材料的研究备受关注,其重点是远距离高效破坏。飞秒激光丝化可实现千米级的能量传递,为需要远距离破坏的应用提供了独特的优势。然而,飞秒激光丝与硬脆材料之间的相互作用机制仍不清楚。本研究利用双温方程初步模拟了不同脉冲能量下飞秒激光与氧化铝陶瓷的相互作用。结果显示了飞秒激光照射下电子和晶格温度的变化。随后,考虑到不同的脉冲能量、灯丝位置和烧蚀时间,系统地研究了飞秒激光灯丝对陶瓷材料造成的损伤性能。此外,在脉冲能量为 4 mJ 时,500 毫米透镜聚焦的灯丝长度可延长至 25 毫米,从而在灯丝中间部分形成直径为 340 微米、深度为 440 微米的烧蚀孔。由于灯丝直径和等离子强度恒定,功率夹持效应可确保整个灯丝上的损伤孔形态和大小一致。这阐明了灯丝的损伤机理,充分验证了该方法的有效性,为研究硬脆材料的激光遥感损伤奠定了理论基础。
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引用次数: 0
Ad hoc calibration of interferometric system for measuring nanometer-scale displacements induced by laser ultrasound 测量激光超声诱导的纳米级位移的干涉测量系统的临时校准
IF 4.6 2区 物理与天体物理 Q1 OPTICS Pub Date : 2024-09-16 DOI: 10.1016/j.optlastec.2024.111779

Laser Ultrasound (LUS) is commonly used in many fields including thickness measurement and defect inspection. In a conventional LUS system, a piezo-based transducer (PZT) is generally used for detecting the ultrasound echo waves, which requires direct contact with a specimen and thus prolongs measurement time when any lateral scanning is necessary. We present a novel non-contact interferometric system based on a 3 × 3 optical fiber coupler. Even though the 3 × 3 interferometric system works stably at any operating point and allows quantitative measurements, it is generally known that careful calibration is necessary before main measurements. Experimentally, it was observed that the surface displacement, induced by the ultrasound wave of LUS, of a cornea phantom was so minute that averaging was necessary. In this study, we discovered that by using the multiple data sets acquired for averaging, we could obtain the system ad hoc characteristic ellipse without performing the conventional calibration process. Furthermore, by utilizing coherent average we could extract the displacement with a 0.14 nm sensitivity. We could also measure the thickness variation, induced by ocular pressure, of the cornea phantom with a resolution of 4.3 μm by measuring the time of a round trip of the ultrasound wave. This straightforward system, composed solely of a 3 × 3 coupler, is expected to promise a compact and efficient solution to diverse applications.

激光超声(LUS)通常用于厚度测量和缺陷检测等多个领域。在传统的 LUS 系统中,通常使用压电式传感器(PZT)来检测超声回波,这需要直接接触试样,因此在需要进行横向扫描时会延长测量时间。我们提出了一种基于 3 × 3 光纤耦合器的新型非接触干涉测量系统。尽管 3 × 3 干涉测量系统可在任何工作点稳定工作,并可进行定量测量,但众所周知,在进行主要测量之前,必须进行仔细校准。实验发现,由 LUS 超声波引起的角膜模型表面位移非常微小,因此必须进行平均。在这项研究中,我们发现利用获取的多组数据进行平均,可以获得系统的临时特征椭圆,而无需执行传统的校准过程。此外,通过利用相干平均,我们还能以 0.14 nm 的灵敏度提取位移。我们还可以通过测量超声波的往返时间来测量眼压引起的角膜模型厚度变化,分辨率为 4.3 μm。这一简单的系统仅由一个 3 × 3 耦合器组成,有望为各种应用提供紧凑高效的解决方案。
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引用次数: 0
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Optics and Laser Technology
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