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The interaction between urban heat island intensity and sea-breeze effect. 城市热岛强度与海风效应的相互作用。
IF 3.7 3区 综合性期刊 Q1 MULTIDISCIPLINARY SCIENCES Pub Date : 2025-11-06 DOI: 10.1098/rsta.2024.0578
Prathap Ramamurthy, Jean Carlos Pena, Sarah Liu, Jorge Gonzalez-Cruz

The article investigates the interaction between the sea-breeze circulation and the urban heat island effect in Houston, Texas, located on the Gulf of Mexico coast. The analysis focuses on the summer period in 2022 during the Convective-cloud Urban Boundary-layer Experiment and the Tracking Aerosol Cloud Convection Interactions Experiment. The work, which exclusively used ground-based observations, found a high degree of intra-urban variability in both the temperature and the humidity field during the sea-breeze days. Near-surface virtual potential temperature during the sea-breeze episodes in the metropolitan area varied by almost 10 K, with urban regions near the coast experiencing lower temperature than the inland region. The urban heat island effect was strong enough to create persistent hot spots even during the sea-breeze episodes. On land-breeze days, both the temperature and the humidity fields were more uniform with little spatial variability. The depth of the sea-breeze circulation was captured using X-band radar and radiosondes; it averaged around 1500-2000 m above ground level. The thermal gradient due to the interaction between the sea-breeze circulation and the urban heat island effect led to secondary flows that influenced local convective activity.This article is part of the theme issue 'Urban heat spreading above and below ground'.

本文研究了位于墨西哥湾沿岸的德克萨斯州休斯敦市的海风环流与城市热岛效应的相互作用。重点分析了2022年夏季对流-云城市边界层实验和气溶胶云对流相互作用跟踪实验。这项工作完全使用地面观测,发现在海风天气期间,温度和湿度场在城市内部都有高度的变化。海风事件期间,大都市地区近地面虚位温变化近10 K,沿海城市地区温度低于内陆地区。城市热岛效应强到足以在海风期间产生持续的热点。在陆风日,温度场和湿度场较为均匀,空间变异性较小。利用x波段雷达和无线电探空仪捕获海风环流深度;平均海拔在1500-2000米左右。海风环流与城市热岛效应相互作用产生的热梯度导致二次流的产生,从而影响局地对流活动。这篇文章是“城市热量在地上和地下传播”主题的一部分。
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引用次数: 0
Modelling the transport and deposition of sediment-microplastics fluxes in a braided river, using Delft3D. 使用Delft3D模拟辫状河中沉积物微塑料通量的运输和沉积。
IF 3.7 3区 综合性期刊 Q1 MULTIDISCIPLINARY SCIENCES Pub Date : 2025-10-23 DOI: 10.1098/rsta.2024.0442
Lucrecia Alvarez Barrantes, Anne Baar, Roberto Fernández, Christopher Hackney, Daniel Parsons, Robert M Dorrell

Rivers polluted by plastics have become sites where mixtures of microplastics and sediment particles are transported by the river current and deposited in the riverbed. A hydromorphodynamic numerical model was developed using Delft3D (software specialized in simulating natural water systems), to simulate the sedimentation, erosion, resuspension and transport of microplastics together with sediment particles, introducing an innovative model with an active riverbed. The model was used to understand the distribution patterns, morphological changes and load balances of plastic debris in a river. The study case is an artificial braided river with a non-buoyant suspended microplastic load. The results simulate a sediment bed that acts as a source of microplastic storage near the point of release. The high deposition of microplastics increases the capacity of the river flow to erode the banks and channels, resulting in deeper channels and larger river bars. The highest amounts of microplastics were deposited in the inner channel banks, and the highly suspended microplastic load is transported in the main channel thalweg. The model can be used as a more accurate method to predict the dynamics of microplastic fluxes in rivers, providing better tools to understand how much plastic enters the ocean from the river environment.This article is part of the Theo Murphy meeting issue 'Sedimentology of plastics: state of the art and future directions'.

被塑料污染的河流已经成为微塑料和沉积物颗粒的混合物被水流运输并沉积在河床上的场所。利用Delft3D(专门用于模拟自然水系统的软件)开发了一个水形态动力学数值模型,以模拟微塑料连同沉积物颗粒的沉积、侵蚀、再悬浮和运输,引入了一个具有活动河床的创新模型。该模型用于了解河流中塑料垃圾的分布模式、形态变化和负荷平衡。研究对象为具有非浮力悬浮微塑性载荷的人工辫状河。结果模拟了一个沉积物床,它在释放点附近作为微塑料储存的来源。微塑料的大量沉积增加了河流侵蚀河岸和河道的能力,导致河道变深,河坝变大。微塑料沉积量最高的是内河堤,高度悬浮的微塑料载荷在主河堤中运输。该模型可以作为一种更准确的方法来预测河流中微塑料通量的动态,为了解有多少塑料从河流环境进入海洋提供更好的工具。本文是西奥·墨菲会议议题“塑料沉积学:技术现状和未来方向”的一部分。
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引用次数: 0
A step towards microlitter risk assessment: modelling microlitter storage potential of the UK seabed. 迈向微垃圾风险评估的一步:模拟英国海底微垃圾储存潜力。
IF 3.7 3区 综合性期刊 Q1 MULTIDISCIPLINARY SCIENCES Pub Date : 2025-10-23 DOI: 10.1098/rsta.2024.0428
Adil Bakir, Adam Porter, Ceri Lewis, Jon Barry, Robert Brookes, William Procter, Briony Silburn, Alexandra Rachael McGoran, Clement Garcia, Claire Mason, Stefan Bolam, David Stephen Clare, Keith Cooper, Anna Downie, Jim Ellis, Daniel Wood, Claire Phillips, Tamara S Galloway

Seafloor sediments have been defined as sinks for microplastics in the marine environment and could therefore represent suitable matrices for their long-term monitoring. Previous studies indicated the widespread distribution of microlitter in seafloor sediments for the UK. In the present study, observations from 2017 to 2021 were used to produce a microlitter distribution model (unitless), derived from physical properties of the seabed that are known to drive the storage capacity of microlitter. The predicted distribution model was converted into a geospatial data layer and plotted against additional open access data layers for likely sources of marine litter (e.g. marine structures) as well as data layers for more sensitive features around the UK (e.g. marine protected areas (MPAs)). Visualization of the accumulation zones for microlitter against the different layers allowed the identification of areas potentially at risk from an increased addition of microlitter from various sources (e.g. dredge disposal sites). Identification of potential risks and prioritization for different zones of action would help the development of national and regional monitoring strategies while reducing costs of multi-compartment, larger scale monitoring programmes. Additional observations and targeted monitoring data are needed to link potential sources of accumulations for microplastics with a higher level of certainty.This article is part of the Theo Murphy meeting issue 'Sedimentology of plastics: state of the art and future directions'.

海底沉积物被定义为海洋环境中微塑料的汇,因此可以作为长期监测微塑料的合适基质。先前的研究表明,英国海底沉积物中微垃圾分布广泛。在本研究中,研究人员利用2017年至2021年的观测数据建立了一个微凋落物分布模型(无单位),该模型来自海底的物理特性,已知这些特性会驱动微凋落物的储存容量。预测的分布模型被转换成地理空间数据层,并与其他开放获取数据层(例如海洋结构)以及英国周围更敏感特征(例如海洋保护区(MPAs))的数据层进行绘图。对不同层的微垃圾堆积区进行可视化,可以确定可能因各种来源的微垃圾增加而面临风险的区域(例如疏浚处置场地)。确定潜在风险和确定不同行动区的优先次序将有助于制定国家和区域监测战略,同时减少多部门、更大规模监测方案的费用。需要更多的观察和有针对性的监测数据,以更高的确定性将微塑料的潜在积聚源联系起来。本文是西奥·墨菲会议议题“塑料沉积学:技术现状和未来方向”的一部分。
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引用次数: 0
The influence of flow on the amount, retention and loss of plastic pollution in an urban river. 流动对城市河流中塑料污染的数量、滞留和损失的影响。
IF 3.7 3区 综合性期刊 Q1 MULTIDISCIPLINARY SCIENCES Pub Date : 2025-10-23 DOI: 10.1098/rsta.2023.0023
Jacob Haney, Xia Zhu, Mary Long, Bailey A Schwenk, Timothy J Hoellein, Wilfred M Wollheim, Richard B Lammers, Shan Zuidema, Chelsea M Rochman

Urban rivers are hypothesized to be major transporters of plastic pollution into lakes and oceans, with storm events playing a pivotal role. However, few studies investigate microplastic and macroplastic contamination and transport across a river basin, and how it varies with flow. Here, we sampled microplastic (less than 5 mm) and macroplastic (greater than 5 mm) from four sites along an urban river in Ontario, Canada, during baseflow and stormflow. To contextualize their fate and transport through river reaches, we sampled macroplastic stored in the riparian zone, overhanging vegetation, floating in surface water and riverbed and sampled microplastic from the surface water, water column and sediment. At baseflow, most macroplastic was found in the riparian zone (ranging from 0.1 to 4.7 pieces per m2). During stormflow, concentrations (micro and macro) rise and fall with discharge. Moreover, the composition of microplastics in the water column shifts from fibre- to rubber-dominated during higher flows. The mobilization of denser (e.g. rubber) particles during flow is consistent with greater water velocities during storms. Finally, using our data and flow patterns from 2022 to 2023, we estimate that approximately 522 billion microplastic particles and 20 754 macroplastic items, equalling approximately 36 000 and 160 kg by mass, respectively, are transported to Lake Ontario annually.This article is part of the Theo Murphy meeting issue 'Sedimentology of plastics: state of the art and future directions'.

城市河流被认为是塑料污染进入湖泊和海洋的主要载体,风暴事件起着关键作用。然而,很少有研究调查微塑料和宏观塑料污染和跨流域运输,以及它如何随流量变化。在这里,我们从加拿大安大略省一条城市河流的四个地点取样了基流和暴雨流期间的微塑料(小于5毫米)和大塑料(大于5毫米)。为了了解它们的命运和在河流流域的运输,我们采集了储存在河岸带、悬垂植被、地表水和河床中漂浮的宏观塑料,并采集了地表水、水柱和沉积物中的微塑料。在基流中,大多数宏观塑性发现于河岸带(每平方米0.1至4.7个)。在暴雨过程中,浓度(微观和宏观)随流量而上升和下降。此外,在水流较大时,水柱中的微塑料成分从纤维为主转变为橡胶为主。在流动过程中,密度较大的(如橡胶)颗粒的动员与风暴期间较大的水速是一致的。最后,利用我们的数据和2022年至2023年的流动模式,我们估计每年约有5220亿个微塑料颗粒和20754个大塑料颗粒,分别相当于约36,000和160公斤的质量,被运送到安大略湖。本文是西奥·墨菲会议议题“塑料沉积学:技术现状和未来方向”的一部分。
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引用次数: 0
Flash-flood-driven litter accumulation on beaches studied with aerial imagery and machine learning on Sicily's northeastern coast, southern Italy. 在意大利南部西西里岛东北海岸,利用航空图像和机器学习研究了山洪暴发导致的海滩垃圾堆积。
IF 3.7 3区 综合性期刊 Q1 MULTIDISCIPLINARY SCIENCES Pub Date : 2025-10-23 DOI: 10.1098/rsta.2024.0427
Jun Seok Oh, Carolin Leluschko, Christoph Tholen, Marcello Gugliotta

This study examines the distributions and dynamics of litter accumulation in a part of the northeastern coast of Sicily, southern Italy, using a multidisciplinary approach with manned and unmanned aerial systems imagery, a machine-learning algorithm and analysis of meteorological data. Aerial imagery shows that litter accumulations are present on beaches near the river mouths and potentially after flash floods. At least five distinct flash flood events depositing litter have been inferred since March 2015 to January 2024 in the study area. Meteorological data show that high precipitation, resulting in flash floods, and prevailing wind direction from the sea are the primary contributors to litter accumulation in this area. The algorithm applied on drone imagery on one of the accumulations detected a composition of polystyrene (42.6%), wood (35.6%), polyurethane (6.1%) and polyethylene terephthalate (5.4%). The general composition of the litter accumulation and its distribution near river mouths suggests that its source is associated with the input from nearby towns through mismanagement on the riverbeds, followed by flash floods. This study highlights the importance of considering river floods when investigating litter dynamics in coastal environments, as well as the potential of using aerial imagery and machine learning to help assess this problem.This article is part of the Theo Murphy meeting issue 'Sedimentology of plastics: state of the art and future directions'.

本研究考察了意大利南部西西里岛东北海岸部分地区凋落物的分布和动态,采用多学科方法,包括有人驾驶和无人驾驶航空系统图像、机器学习算法和气象数据分析。航空图像显示,在河口附近的海滩上存在垃圾堆积,可能是在山洪暴发后。从2015年3月到2024年1月,研究区至少发生了5次不同的山洪暴发事件。气象资料显示,高降水导致的山洪暴发和来自海洋的盛行风向是该地区凋落物堆积的主要原因。该算法将无人机图像应用于其中一个聚苯乙烯(42.6%)、木材(35.6%)、聚氨酯(6.1%)和聚对苯二甲酸乙二醇酯(5.4%)的组合物。凋落物堆积的总体组成及其在河口附近的分布表明,其来源与附近城镇因河床管理不善而造成的投入有关,随后发生了山洪暴发。这项研究强调了在调查沿海环境中的垃圾动态时考虑河流洪水的重要性,以及使用航空图像和机器学习来帮助评估这一问题的潜力。本文是西奥·墨菲会议议题“塑料沉积学:技术现状和未来方向”的一部分。
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引用次数: 0
Influence of microplastics on small-scale soil surface roughness and implications for wind transport of microplastic particles. 微塑料对小尺度土壤表面粗糙度的影响及其对微塑料颗粒风输运的影响。
IF 3.7 3区 综合性期刊 Q1 MULTIDISCIPLINARY SCIENCES Pub Date : 2025-10-23 DOI: 10.1098/rsta.2024.0446
Annie Ockelford, Joanna Bullard, Cheryl McKenna Neuman, Patrick O'Brien

Microplastics are an anthropogenic contaminant widely recognized for their effect on marine and freshwater systems, but their terrestrial effects remain less well studied. The inclusion of microplastics in soils has the potential to affect a range of different soil properties, including bulk density, hydraulic conductivity and aggregation. Soil properties affect the susceptibility of soils to wind erosion, and it is therefore likely that where the quantity of microplastics present in soils is sufficient to change soil properties, it may also change the response of soils to wind erosion. This paper quantifies whether the presence of microplastics in sediments affects the development of small-scale soil surface roughness (SSR) properties during wind erosion, and whether there are any relationships between indices of SSR and microplastic flux due to wind erosion. Two contrasting substrates (well-sorted sand and poorly sorted soil) and two types of microplastic (polyethylene beads and polyester fibres) are used. SSR is quantified using geostatistically derived indicators calculated from high-resolution laser scans of the soil surface with and without microplastics, and before and after wind erosion simulated using a wind tunnel. Our results reveal the relative size of the microplastic to the mineral sediment is key to controlling microplastic flux.This article is part of the Theo Murphy meeting issue 'Sedimentology of plastics: state of the art and future directions'.

微塑料因其对海洋和淡水系统的影响而被广泛认为是一种人为污染物,但其对陆地的影响仍未得到充分研究。土壤中含有微塑料可能会影响一系列不同的土壤特性,包括体积密度、水力导电性和聚集性。土壤性质影响土壤对风蚀的敏感性,因此,当土壤中存在的微塑料数量足以改变土壤性质时,它可能也会改变土壤对风蚀的反应。本文量化了沉积物中微塑料的存在是否影响风蚀过程中小尺度土壤表面粗糙度(SSR)特性的发展,以及SSR指标与风蚀引起的微塑料通量之间是否存在关系。使用了两种不同的基质(分类良好的沙子和分类不良的土壤)和两种微塑料(聚乙烯珠和聚酯纤维)。SSR是通过高分辨率激光扫描计算的地质统计学衍生指标来量化的,这些指标是通过有和没有微塑料的土壤表面,以及风洞模拟风蚀前后计算的。研究结果表明,微塑性与矿物沉积物的相对尺寸是控制微塑性通量的关键。本文是西奥·墨菲会议议题“塑料沉积学:技术现状和未来方向”的一部分。
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引用次数: 0
Temporal variation in microplastic abundance in sediment, fish and shrimp: a case study in the Thames Estuary, UK. 沉积物、鱼和虾中微塑料丰度的时间变化:英国泰晤士河口的案例研究。
IF 3.7 3区 综合性期刊 Q1 MULTIDISCIPLINARY SCIENCES Pub Date : 2025-10-23 DOI: 10.1098/rsta.2025.0040
Alexandra Rachael McGoran, Paul Frederick Clark, Brian Smith, David Morritt

Microplastics are abundant in marine and terrestrial habitats, with rivers transporting particles to the sea. The River Thames catchment, UK, encompasses 15 million residents and many pollution sources. Temporal trends in microplastic abundance are sparse, with ad hoc studies in the estuary demonstrating great variability in concentrations. Taking a seasonal approach to time-series data collection, sediment and biota were sampled every three months over 2 yr. To account for the heterogeneity of microplastics in sediment, three grab samples were collected per survey. On average, 1000 ± 1100 (s.d.) plastic items kg-1 were recovered from sediment, with significantly more from samples in July (summer) and September (autumn) 2020. The recorded concentrations were comparable with studies worldwide. Biota in the estuary are exposed to this plastic. Fish (Osmerus eperlanus, Platichthys flesus, Solea solea) and shrimp (Crangon crangon) contained on average 1.59 ± 2.62 items per individuals and 0.39 ± 0.95 items per individual, respectively. The greatest proportion of contaminated individuals was in December 2018 (winter; 75%) followed by March and June 2019 (spring; 42% and summer; 43%, respectively). Seasonal factors, such as rainfall, can affect plastic accumulation in an estuarine system, but these microplastics are not always bioavailable. Understanding the drivers of this variability is key in designing mitigation strategies and managing risk.This article is part of the Theo Murphy meeting issue 'Sedimentology of plastics: state of the art and future directions'.

微塑料在海洋和陆地栖息地中大量存在,河流将颗粒输送到海洋中。英国的泰晤士河集水区居住着1500万居民和许多污染源。微塑料丰度的时间趋势是稀疏的,在河口的特别研究表明浓度有很大的变化。采用季节性方法收集时间序列数据,在2年内每三个月对沉积物和生物群进行采样。为了考虑沉积物中微塑料的异质性,每次调查收集了三个抓取样本。从沉积物中平均回收了1000±1100 (s.d) kg-1的塑料物品,2020年7月(夏季)和9月(秋季)的样品中回收的塑料物品明显更多。记录的浓度与世界范围内的研究相当。河口的生物群暴露在这种塑料中。鱼(Osmerus eperlanus)、鲽鱼(Platichthys flesus)、鲽鱼(Solea Solea Solea)和对虾(Crangon Crangon Crangon)的平均含量分别为1.59±2.62种和0.39±0.95种。感染比例最高的是2018年12月(冬季;75%),其次是2019年3月和6月(春季;42%和夏季;43%)。季节性因素,如降雨,会影响河口系统中的塑料积累,但这些微塑料并不总是生物可利用的。了解这种可变性的驱动因素是设计缓解策略和管理风险的关键。本文是西奥·墨菲会议议题“塑料沉积学:技术现状和未来方向”的一部分。
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引用次数: 0
Natural and anthropogenic factors driving the distribution of seafloor litter along coastal submarine canyons of southern Italy. 自然和人为因素驱动意大利南部沿海海底峡谷海底垃圾的分布。
IF 3.7 3区 综合性期刊 Q1 MULTIDISCIPLINARY SCIENCES Pub Date : 2025-10-23 DOI: 10.1098/rsta.2023.0026
Martina Pierdomenico, Daniele Casalbore, Denise Petronelli, Silvia Morgana, Domenico Ridente, Francesco Chiocci

Submarine canyons are recognized as accumulation areas for litter and conduits for deep-sea transport. Through the analysis of seafloor videos, we assess litter distribution in canyons of southern Italy, characterized by differences in morphology, connection to sediment sources and anthropogenic pressures. Litter was detected in all canyons, with highly variable concentration ranging from 0.1 to more than 100 items/100 m and a dominance of plastic, indicating a terrestrial or coastal origin for most of the litter. The lowest densities were from Cuma Canyon, incising the continental shelf edge at some distance from the coast and thus detached from major terrestrial inputs, while the highest were reported from the Messina Strait, where rivers draining highly populated areas debouche directly into offshore canyon heads. Canyon head proximity to rivers and densely populated coasts appears to be the main driver of litter abundance, although the uneven distribution between canyons reflects more closely the effect of geomorphological features, sediment transport and oceanographic processes, responsible for different abundances along the canyons' thalweg. Oceanographic processes and sediment transport can be involved in downcanyon litter transport; the latter is dominant in the case of gravity flows, which may deliver debris to the lowest canyon reaches, so far largely unexplored.This article is part of the Theo Murphy meeting issue 'Sedimentology of plastics: state of the art and future directions'.

海底峡谷被认为是垃圾堆积区和深海运输的通道。通过对海底视频的分析,我们评估了意大利南部峡谷的凋落物分布,其特征是形态差异、与沉积物来源的联系和人为压力。在所有峡谷中都检测到凋落物,其浓度变化很大,从0.1到100多件/100 m不等,并且以塑料为主,表明大多数凋落物来自陆地或沿海。密度最低的是库马峡谷,它在离海岸一段距离的地方切割了大陆架边缘,从而与主要的陆地输入分离,而密度最高的是墨西拿海峡,在那里,流经人口稠密地区的河流直接汇入离岸峡谷的源头。峡谷头部靠近河流和人口密集的海岸似乎是凋落物丰度的主要驱动因素,尽管峡谷之间的不均匀分布更密切地反映了地貌特征、沉积物运输和海洋过程的影响,这些因素导致了峡谷沿高程的不同丰度。海洋过程和泥沙搬运可能参与峡谷下凋落物搬运;后者在重力流的情况下占主导地位,重力流可能会将碎片运送到峡谷的最低处,到目前为止,这些地方基本上还没有被探索过。本文是西奥·墨菲会议议题“塑料沉积学:技术现状和未来方向”的一部分。
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引用次数: 0
Temporarily trapped: stormwater pond sediment is a key transient sink for microplastic debris. 暂时滞留:雨水塘沉积物是微塑料碎片的一个关键的瞬态汇。
IF 3.7 3区 综合性期刊 Q1 MULTIDISCIPLINARY SCIENCES Pub Date : 2025-10-23 DOI: 10.1098/rsta.2023.0029
Patricia L Corcoran, Alexa Holland, Kelly Evans, Nina Kozikowski, Rebecca Sarazen

Average microplastic (MP) abundances in each of 15 stormwater ponds in London, Canada ranged from 0.7 ± 0.7 particles per gram of dry weight sediment (g-1 dw) to greater than 2323 ± 4643 g-1 dw. Omitting one wetland cell and one hybrid pond produced a significantly higher median MP abundance for forebay versus main basin samples (p = 0.0058), and inlets produced greater mean abundances than outlets and open areas (20 ± 49, 10 ± 17, 4 ± 4 g-1 dw, respectively). Considering all 15 ponds, the industrial/commercial and construction ponds produced higher means (684 ± 2387 g-1 dw; 19 ± 22 g-1 dw) than residential and open counterparts (6 ± 10 g-1 dw; 6 ± 11 g-1 dw). Fragments were the most common particle type in all but one pond, and fibre concentrations relative to other particle types were greatest in residential ponds. Copious styrene butadiene rubber (SBR) particles in an industrial pond are considered tyre wear due to proximity to manufacturers' parking areas and loading docks, and an automotive technology training school. Paint/coating chips accounted for 25% of the fragments analysed. With greater MP abundances than in sediment from tributaries, lakes and beaches of the same watershed, stormwater ponds prove to be exceptional transient sinks for MP debris.This article is part of the Theo Murphy meeting issue 'Sedimentology of plastics: state of the art and future directions'.

在加拿大伦敦的15个雨水池塘中,每克干重沉积物(g-1 dw)的平均微塑料(MP)丰度从0.7±0.7个颗粒到大于2323±4643个g-1 dw。忽略一个湿地池和一个混合池,前湾的中位数MP丰度显著高于主要盆地样本(p = 0.0058),并且入口的平均丰度高于出口和开放区域(分别为20±49、10±17和4±4 g-1 dw)。在所有15个池塘中,工业/商业和建筑池塘产生的平均值(684±2387 g-1 dw; 19±22 g-1 dw)高于住宅和开放池塘(6±10 g-1 dw; 6±11 g-1 dw)。除1个池塘外,其余池塘中碎片是最常见的颗粒类型,而住宅池塘中纤维浓度相对于其他颗粒类型最高。由于靠近制造商的停车场和装卸码头以及汽车技术培训学校,工业池塘中大量的丁苯橡胶(SBR)颗粒被认为是轮胎磨损。油漆/涂层碎片占分析碎片的25%。与同一流域的支流、湖泊和海滩的沉积物相比,雨水池的多聚磷含量更高,因此证明雨水池是多聚磷碎片的特殊瞬时汇。本文是西奥·墨菲会议议题“塑料沉积学:技术现状和未来方向”的一部分。
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引用次数: 0
The effects of sediment properties on the aeolian abrasion and surface characteristics of microplastics. 泥沙性质对微塑料风蚀磨损及表面特性的影响。
IF 3.7 3区 综合性期刊 Q1 MULTIDISCIPLINARY SCIENCES Pub Date : 2025-10-23 DOI: 10.1098/rsta.2024.0443
Lucrecia Alvarez Barrantes, Joanna Bullard, Samuel Davis, Cheryl McKenna Neuman, Patrick O'Brien, Paul Roach, Zhaoxia Zhou

Microplastics (less than 5 mm diameter) are significant environmental contaminants whose small sizes and low densities facilitate transport by wind. Transport by wind erosion alongside soils or sediments results in mechanical abrasion of the plastic surfaces which can alter their physical and chemical properties. This paper uses laboratory simulations to determine the effects of up to 216 h of aeolian abrasion on polyethylene microplastics by angular, sub-rounded and rounded mineral sediments. During the abrasion process the mineral particles break down producing small fragments which adhere to the microplastic surfaces altering their surface roughness and chemistry. With increasing duration of abrasion the microplastic surface becomes coated with mineral fragments changing the dominant surface element from carbon to oxygen and silicon reflecting the composition of the erodents. The coating develops more rapidly when microplastics are abraded with angular sediments as these produce a lot of small fragments within the first 1-2 h. However, after more than 200 h of abrasion all the erodents had similar effects. A conceptual model of microplastic surface change is presented in which the plastic cracks and fractures, then flattens along with increasing density of sediment fragment cover. Surface changes may affect the ability of the plastics to transport airborne contaminants.This article is part of the Theo Murphy meeting issue 'Sedimentology of plastics: state of the art and future directions'.

微塑料(直径小于5mm)是一种重要的环境污染物,其体积小、密度低,有利于风的传播。随着土壤或沉积物的风蚀,塑料表面会发生机械磨损,从而改变其物理和化学性质。本文采用实验室模拟的方法,确定了角状、次圆形和圆形矿物沉积物对聚乙烯微塑料长达216小时的风蚀作用的影响。在磨损过程中,矿物颗粒分解产生小碎片,附着在微塑料表面,改变其表面粗糙度和化学性质。随着磨损时间的延长,微塑性表面被矿物碎片包裹,使主要的表面元素从碳变为氧和硅,反映了侵蚀物的组成。当微塑料被角状沉积物磨损时,涂层发展得更快,因为这些沉积物在最初的1-2小时内会产生大量的小碎片。然而,在超过200小时的磨损后,所有侵蚀物的效果都是相似的。提出了一种微塑性表面变化的概念模型,其中塑性裂纹和断裂随着沉积物碎片覆盖密度的增加而变平。表面的变化可能影响塑料输送空气中污染物的能力。本文是西奥·墨菲会议议题“塑料沉积学:技术现状和未来方向”的一部分。
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Philosophical Transactions of the Royal Society A: Mathematical, Physical and Engineering Sciences
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