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Effects of partial Eu filling in the unfilled skutterudite CoP3 未填充沸石 CoP3 中部分 Eu 填充的影响
IF 3.7 2区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2024-07-25 DOI: 10.1103/physrevb.110.035156
Zicheng Tao, Chao Zhang, Jian Yuan, Renjie Zhang, Xia Wang, Zhenhai Yu, Wei Xia, Yaobo Huang, Shihao Zhang, Yanfeng Guo
The unfilled skutterudite CoP3 hosts extremely large magnetoresistance (∼2 × 104% at 30 T and 2 K), large hole mobility (∼2 × 104 cm2V1s1, 2 K), and a fourfold quadratic contact point (QCP) above the Fermi level in the electronic structure. We unveil herein that the partial filling of Eu onto the icosahedral void sites of CoP3 can shift the QCP to lie below the Fermi level while retaining the high carrier mobility (∼1.6 × 104 cm2V1s1, 2 K). Unlike nonmagnetic CoP3, partially filled skutterudite Eu0.412Co4P12 is a soft ferromagnet with almost isotropic magnetism. Additionally, an intriguing topological Hall effect is observed, likely hinting an unusual spin texture. In this paper, we provide useful insights into the interplay between magnetism and the nontrivial feature of the electronic band structure, which would guide more efforts in studying this issue.
未填充的矽卡岩 CoP3 具有极高的磁阻(在 30 T 和 2 K 条件下为 2 × 104%)、极高的空穴迁移率(在 2 K 条件下为 2 × 104 cm2V-1s-1)以及高于费米级的四倍二次接触点(QCP)。我们在此揭示,在 CoP3 的二十面体空位上部分填充 Eu 可以将 QCP 移至费米水平以下,同时保持高载流子迁移率(∼1.6 × 104 cm2V-1s-1,2 K)。与非磁性 CoP3 不同,部分填充的沸石 Eu0.412Co4P12 是一种软铁磁体,具有几乎各向同性的磁性。此外,我们还观察到一种有趣的拓扑霍尔效应,这可能暗示了一种不寻常的自旋纹理。在本文中,我们就磁性与电子带结构的非偶性特征之间的相互作用提出了有益的见解,这将为研究这一问题提供更多的指导。
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引用次数: 0
Squeezed and nascent vortices in a thin normal layer with proximity induced superconductivity 具有邻近诱导超导性的法向薄层中的挤压涡旋和新生涡旋
IF 3.7 2区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2024-07-25 DOI: 10.1103/physrevb.110.014517
D. Yu. Vodolazov
It is theoretically found that in-plane vortices may exist in a thin normal metal (N) layer (with thickness dN much smaller than the coherence length ξN) that covers a superconductor (S). Vortices enter the N layer with proximity-induced superconductivity at a sufficiently large in-plane magnetic field. These vorticies have squeezed cores and are located (pinned) near the SN interface. At large magnetic fields, we find a nascent vortex state, which is a spatially modulated state along the finite length N layer with zero vorticity. This state does not exist in a finite length single S layer.
理论发现,在覆盖超导体(S)的普通金属(N)薄层(厚度 dN 远远小于相干长度ξN)中可能存在面内涡流。在足够大的面内磁场下,涡流进入 N 层,并具有近似诱导超导性。这些旋涡具有挤压核心,位于 SN 接口附近(被钉住)。在大磁场下,我们会发现一种新生涡旋态,它是沿有限长度 N 层的空间调制态,涡度为零。这种状态并不存在于有限长度的单 S 层中。
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引用次数: 0
SU(4) symmetry breaking and induced superconductivity in graphene quantum Hall edges 石墨烯量子霍尔边的 SU(4) 对称破缺和诱导超导性
IF 3.7 2区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2024-07-25 DOI: 10.1103/physrevb.110.024518
Joseph J. Cuozzo, Enrico Rossi
In graphene, the approximate SU(4) symmetry associated with the spin and valley degrees of freedom in the quantum Hall (QH) regime is reflected in the fourfold degeneracy of graphene's Landau levels (LLs). Interactions and the Zeeman effect break such approximate symmetry and lift the corresponding degeneracy of the LLs. We study how the breaking of the approximate SU(4) symmetry affects the properties of graphene's QH edge modes located in proximity to a superconductor. We show how the lifting of the fourfold degeneracy qualitatively modifies the transport properties of the QH-superconductor heterojunction. For the zero LL, by placing the edge modes in proximity to a superconductor, it is, in principle, possible to realize a 1D topological superconductor supporting Majoranas in the presence of sufficiently strong Zeeman field. We estimate the topological gap of such a topological superconductor and relate it to the properties of the QH-superconductor interface.
在石墨烯中,与量子霍尔(QH)制度中的自旋和谷自由度相关的近似 SU(4) 对称性反映在石墨烯的朗道水平(LLs)的四倍退化性中。相互作用和泽曼效应打破了这种近似对称性,并解除了 LLs 的相应退化性。我们研究了近似 SU(4) 对称性的打破如何影响靠近超导体的石墨烯 QH 边缘模式的特性。我们展示了四重退变性的解除是如何定性地改变 QH-超导体异质结的传输特性的。对于零 LL,通过将边缘模式置于超导体附近,原则上可以实现在足够强的泽曼场存在下支持马约拉纳斯的一维拓扑超导体。我们估算了这种拓扑超导体的拓扑间隙,并将其与 QH 超导体界面的特性联系起来。
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引用次数: 0
Coexistence of antiferromagnetic cubic and ferromagnetic tetragonal polymorphs in epitaxial CuMnSb films 外延铜锰锑薄膜中反铁磁性立方多晶体和铁磁性四方多晶体的共存
IF 3.7 2区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2024-07-25 DOI: 10.1103/physrevb.110.014436
A. Ciechan, P. Dłużewski, S. Kret, K. Gas, L. Scheffler, C. Gould, J. Kleinlein, M. Sawicki, L. W. Molenkamp, P. Bogusławski
High-resolution transmission electron microscopy and superconducting quantum interference device magnetometry shows that epitaxial CuMnSb films exhibit a coexistence of two magnetic phases, coherently intertwined in nanometric scales. The dominant α phase is half-Heusler cubic antiferromagnet with the Néel temperature of 62 K, the equilibrium structure of bulk CuMnSb. The secondary phase is its ferromagnetic tetragonal β polymorph with the Curie temperature of about 100 K. First principles calculations provide a consistent interpretation of experiment, since (i) total energy of βCuMnSb is higher than that of αCuMnSb only by 0.12 eV per formula unit, which allows for epitaxial stabilization of this phase, (ii) the metallic character of βCuMnSb favors the Ruderman-Kittel-Kasuya-Yoshida ferromagnetic coupling, and (iii) the calculated effective Curie-Weiss magnetic moment of Mn ions in both phases is about 5.5μB, favorably close to the measured value. Calculated properties of all point native defects indicate that the most likely to occur are MnCu antisites. They affect magnetic properties of epilayers, but they cannot induce the ferromagnetic order in CuMnSb. Combined, the findings highlight a practical route towards fabrication of functional materials in which coexisting polymorphs provide complementing functionalities in one host.
高分辨率透射电子显微镜和超导量子干涉装置磁强计显示,外延铜锰锑薄膜呈现出两种磁性相共存的现象,并在纳米尺度上相干地交织在一起。占主导地位的 α 相是半休斯勒立方反铁磁体,奈尔温度为 62 K,这是块状铜锰锑的平衡结构。第二相是其铁磁性四方 β 多晶体,居里温度约为 100 K。第一性原理计算提供了与实验一致的解释,因为 (i) β-CuMnSb 的总能量只比α-CuMnSb 高 0.(ii) β-CuMnSb 的金属特性有利于 Ruderman-Kittel-Kasuya-Yoshida 铁磁耦合;(iii) 两种相中 Mn 离子的有效居里-韦斯磁矩计算值约为 5.5μB,非常接近测量值。所有点原生缺陷的计算特性表明,最有可能出现的是锰铜反位。它们会影响外延层的磁性能,但不能诱导铜锰锑中的铁磁秩序。综上所述,这些发现突出了制造功能材料的实用途径,即共存的多晶体在一个宿主中提供互补功能。
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引用次数: 0
Quasi-two-dimensional frustrated spin-1 triangular lattice antiferromagnet Ca3NiNb2O9: A proximate spin liquid 准二维受挫自旋-1 三角晶格反铁磁体 Ca3NiNb2O9:一种近似自旋液体
IF 3.7 2区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2024-07-25 DOI: 10.1103/physrevb.110.024430
Sonia Deswal, Deepu Kumar, Dibyata Rout, Surjeet Singh, Pradeep Kumar
The spin-1 triangular lattice Heisenberg antiferromagnet Ca3NiNb2O9 and its sister compounds are conjectured to promote the formation of many-body quantum entangled states such as a quantum spin liquid (QSL), an exotic phase which features fractionalized quasiparticle excitations and emergent gauges. We probe the single crystal of Ca3NiNb2O9 using an in-depth Raman spectroscopic technique. Our measurements provide evidence for the fractionalized excitations, suggesting that the current system is in close proximity to the QSL phase. This is also in line with the proposed higher-order fractional magnetization plateau in this system, as these plateaus have an intricate relationship with the spin entanglement. We observed unconventional underlying scattering as a broad continuum with an intensity that shows fermionic statistics. Additionally, phonon modes show Fano asymmetry, also conjectured as a fingerprint of the spin-liquid phase, and above a critical Raman shift also show fermionic statistics in their intensity evolution.
据推测,自旋-1 三角晶格海森堡反铁磁体 Ca3NiNb2O9 及其姊妹化合物能促进多体量子纠缠态的形成,如量子自旋液体(QSL),这是一种奇异的相,具有分数化的准粒子激发和新兴量规的特征。我们利用深入的拉曼光谱技术对 Ca3NiNb2O9 单晶体进行了探测。我们的测量结果提供了分数化激发的证据,表明当前系统接近于 QSL 阶段。这也与该体系中提出的高阶分数磁化高原相吻合,因为这些高原与自旋纠缠有着错综复杂的关系。我们观察到非常规的底层散射是一个宽广的连续体,其强度显示出费米子统计量。此外,声子模式显示出法诺不对称性,这也被推测为自旋液相的指纹,在临界拉曼位移以上,其强度演变也显示出费米子统计。
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引用次数: 0
Anderson-Higgs amplitude mode in Josephson junctions 约瑟夫森结中的安德森-希格斯振幅模式
IF 3.7 2区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2024-07-25 DOI: 10.1103/physrevb.110.024517
P. Vallet, J. Cayssol
The Anderson-Higgs mode in a superconductor corresponds to a collective and coherent oscillation of the order parameter amplitude. We propose to detect this mode in a tunnel Josephson junction between two singlet s-wave diffusive superconductors in presence of a THz external irradiation at angular frequency ω. By solving the Keldysh-Usadel equations, we obtain that the current-voltage relation exhibits a series of peaks of which only a subset is enhanced by the Anderson-Higgs mode. Furthermore, at zero bias, the junction features an ac current oscillating at 2ω, which is resonant when ω hits the superconducting gap, thereby indicating the activation of the Anderson-Higgs mode.
超导体中的安德森-希格斯模式对应于阶参量振幅的集体相干振荡。通过求解凯尔迪什-乌萨德尔方程,我们得出电流-电压关系呈现一系列峰值,其中只有一个子集由安德森-希格斯模式增强。此外,在零偏压条件下,结中的交流电流振荡于 2ω,当ℏω触及超导间隙时会产生共振,从而表明安德森-希格斯模式被激活。
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引用次数: 0
Liouvillian skin effect in a one-dimensional open many-body quantum system with generalized boundary conditions 具有广义边界条件的一维开放多体量子系统中的刘维肤效应
IF 3.7 2区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2024-07-25 DOI: 10.1103/physrevb.110.045440
Liang Mao, Xuanpu Yang, Ming-Jie Tao, Haiping Hu, Lei Pan
The non-Hermitian skin effect, in which eigenstates of non-Hermitian Hamiltonians are localized at one boundary in the open boundary condition, has attracted great interest recently. In this paper, we investigate the skin effect in one-dimensional dissipative quantum many-body systems, which we call the Liouvillian skin effect (LSE). We rigorously identify the existence of the LSE for generalized boundary conditions by solving the Liouvillian superoperator of an exactly solvable model with the advantage of the Bethe ansatz. The LSE is sensitive to boundary conditions where the signature is reflected in eigenfunctions of the system. We confirm that the LSE is fragile to a tiny coflow boundary hopping with non-Hermitian current but can survive a counterflow boundary hopping in the thermodynamic limit. Our work provides a prototypical example of exactly solvable dissipative quantum many-body lattice systems exhibiting the LSE for generalized boundary conditions. It can be further extended to other integrable open quantum many-body models.
在开放边界条件下,非赫米提哈密顿的特征状态被局部化在一个边界上,这种非赫米提趋肤效应最近引起了人们的极大兴趣。在本文中,我们研究了一维耗散量子多体系统中的趋肤效应,我们称之为刘维趋肤效应(LSE)。我们利用贝特方差的优势,通过求解一个精确可解模型的 Liouvillian 超算子,严格确定了广义边界条件下 LSE 的存在。LSE 对边界条件很敏感,其特征反映在系统的特征函数中。我们证实,LSE 易受非赫米提电流的微小同流边界跳变影响,但在热力学极限中却能经受住逆流边界跳变。我们的工作提供了一个可精确求解的耗散量子多体晶格系统的原型,该系统在广义边界条件下表现出 LSE。它可以进一步扩展到其他可积分的开放量子多体模型。
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引用次数: 0
Realignment and suppression of charge density waves in the rare-earth tritellurides RTe3 (R=La, Gd, Er) 稀土三碲化物 RTe3(R=镧、钆、铒)中电荷密度波的调整和抑制
IF 3.7 2区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2024-07-25 DOI: 10.1103/physrevb.110.014111
Saif Siddique, James L. Hart, Drake Niedzielski, Ratnadwip Singha, Myung-Geun Han, Stephen D. Funni, Michael Colletta, Mehrdad T. Kiani, Noah Schnitzer, Natalie L. Williams, Lena F. Kourkoutis, Yimei Zhu, Leslie M. Schoop, Tomás A. Arias, Judy J. Cha
The rare-earth tritellurides have a rich phase diagram that includes charge density waves (CDWs), superconductivity, and magnetic order, offering a platform to study the interplay between these phases on a square-net system. Prior studies have shown that defects can affect the CDW characteristics in these materials, yet coupling between the CDW order and the underlying microstructure has not been studied at the nanoscale. Here we use scanning transmission electron microscopy at cryogenic temperatures to directly visualize the effects of defects on the CDW order and provide a spatially resolved microscopic correlation between the CDW transition and structural defects. We show that in the presence of extended defects, such as dislocations and stacking faults, the weak orthorhombicity of the rare-earth tritellurides is lost and the material becomes pseudotetragonal. Since the orthorhombicity acts as a symmetry breaking field for the CDW transitions in rare-earth tritellurides, the presence of these extended defects modulates the energetics of the CDWs and suppresses the ground-state CDW phase at low temperature.
稀土三碲化物具有丰富的相图,其中包括电荷密度波 (CDW)、超导性和磁序,为研究这些相在方网系统上的相互作用提供了一个平台。先前的研究表明,缺陷会影响这些材料中的 CDW 特性,但还没有在纳米尺度上研究过 CDW 秩与底层微结构之间的耦合。在这里,我们使用低温扫描透射电子显微镜直接观察缺陷对 CDW 秩的影响,并提供 CDW 转变与结构缺陷之间的空间分辨微观关联。我们发现,在存在扩展缺陷(如位错和堆积断层)的情况下,稀土三碲化物的弱正交性会消失,材料会变成伪四方晶。由于正交性是稀土三碲化物中 CDW 转变的对称性断裂场,这些扩展缺陷的存在调节了 CDW 的能量,并在低温下抑制了基态 CDW 相。
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引用次数: 0
Entanglement entropy of topological phases with multipole symmetry 多极对称拓扑相的纠缠熵
IF 3.7 2区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2024-07-25 DOI: 10.1103/physrevb.110.045146
Hiromi Ebisu
We study entanglement entropy of unusual ZN topological stabilizer codes which admit fractional excitations with restricted mobility constraint in a manner akin to fracton topological phases. It is widely known that the subleading term of the entanglement entropy of a disk geometry in conventional topologically ordered phases is related to the total number of the quantum dimension of the fractional excitations. We show that, in our model, such a relation does not hold, i.e., the total number of the quantum dimension varies depending on the system size, whereas the subleading term of the entanglement entropy takes a constant number irrespective to the system size. We give a physical interpretation of this result in the simplest case of the model. More thorough analysis on the entanglement entropy of the model on generic lattices is also presented.
我们研究了不寻常的 ZN 拓扑稳定器代码的纠缠熵,这些代码以类似于分形拓扑相的方式接纳了具有流动性限制约束的分数激元。众所周知,传统拓扑有序相中圆盘几何的纠缠熵的次项与分数激发的量子维总数有关。我们的研究表明,在我们的模型中,这种关系并不成立,即量子维度的总数随系统大小的变化而变化,而纠缠熵的次导项则是一个常数,与系统大小无关。我们在模型的最简单情况下给出了这一结果的物理解释。我们还对该模型在一般晶格上的纠缠熵进行了更深入的分析。
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引用次数: 0
Spin-correlation transport and multiple resistive states in multiferroic tunnel junctions 多铁氧体隧道结中的自旋相关传输和多电阻态
IF 3.7 2区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2024-07-25 DOI: 10.1103/physrevb.110.024428
Xiaolin Zhang, Lei Yin, Sicong Zhu, Ruiqing Cheng, Yao Wen, Jun He
Multiferroic tunneling junctions (MFTJs), which comprise magnetic electrodes and extremely thin ferroelectric tunneling barriers, are promising contenders for nonvolatile memory applications. Noncollinear antiferromagnetic Mn3Sn with time-reversal symmetry-breaking polarization properties and ferroelectric αIn2Se3 may open up the possibility of constructing room-temperature MFTJs. In this study, we investigate the spin-correlation transport in the MFTJs with Mn3Sn/BN/αIn2Se3/Mn3Sn structure using first-principles calculations. The resistance in this structure can be manipulated by tuning the directions of both the Néel vector of Mn3Sn and the electric polarization of the αIn2Se3 layer. Thus, multiple tunneling resistive states can be realized. We predict that huge tunneling magnetoresistance up to 6650% can be obtained by switching the magnetically oriented Néel vectors of Mn3Sn, and more than 8000% tunneling electrical resistance can be obtained by controlling the ferroelectric structure of αIn2Se3. Our work underscores the potential applications of Mn3Sn in multiferroic nonvolatile memories and lays the foundation for the development of ultrafast and efficient spintronic devices utilizing antiferromagnets.
多铁电体隧道结(MFTJ)由磁性电极和极薄的铁电体隧道势垒组成,是非易失性存储器应用的有力竞争者。具有打破时间反转对称极化特性的非共轭反铁磁性 Mn3Sn 和铁电性 α-In2Se3 为构建室温 MFTJ 提供了可能。在本研究中,我们利用第一原理计算研究了具有 Mn3Sn/BN/α-In2Se3/Mn3Sn 结构的 MFTJ 中的自旋相关传输。这种结构中的电阻可以通过调整 Mn3Sn 的奈尔矢量方向和 α-In2Se3 层的电极化方向来操纵。因此,可以实现多种隧道电阻态。我们预测,通过切换 Mn3Sn 的磁定向奈尔矢量,可以获得高达 6650% 的巨大隧穿磁阻;通过控制 α-In2Se3 的铁电结构,可以获得超过 8000% 的隧穿电阻。我们的研究强调了 Mn3Sn 在多铁性非易失性存储器中的潜在应用,并为利用反铁磁体开发超快、高效的自旋电子器件奠定了基础。
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引用次数: 0
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Physical Review B
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