首页 > 最新文献

Physical Review X最新文献

英文 中文
Multipolar Anisotropy in Anomalous Hall Effect from Spin-Group Symmetry Breaking 自旋群对称破缺中反常霍尔效应的多极各向异性
IF 12.5 1区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2025-07-07 DOI: 10.1103/physrevx.15.031006
Zheng Liu, Mengjie Wei, Wenzhi Peng, Dazhi Hou, Yang Gao, Qian Niu
The traditional view of the anomalous Hall effect (AHE) in ferromagnets is that it arises from the magnetization perpendicular to the measurement plane and that there is a linear dependence on the latter. Underlying such a view is the thinking that the AHE is a time-reversal symmetry breaking phenomenon and can therefore be treated in terms of a power series in the magnetic order. However, this view is squarely challenged by a number of recent experiments, urging for a thorough theoretical investigation on the fundamental level. We find that for strong magnets, it is more appropriate and fruitful to regard the AHE as a spin-group symmetry breaking phenomenon where the critical parameter is the spin-orbit interaction strength, which involves a much smaller energy scale. In collinear ferromagnets, the spin-orbit coupling breaks the ∞2′ spin rotation symmetry, and the key to characterizing such symmetry breaking is the identification of spin-orbit vectors which transform regularly under spin-group operations. Born out of our framework is a rich multipolar relationship between the anomalous Hall conductivity and the magnetization direction, with each pole being expanded progressively in powers of the spin-orbit coupling strength. For the leading order contribution, i.e., the dipole, its isotropic part corresponds to the traditional view, and its anisotropic part can lead to the in-plane AHE where the magnetization lies within the measurement plane. Beyond the dipolar structure, the octupolar structure offers the leading order source of nonlinearity and hence introduces unique anisotropy where the dipolar structure cannot. Our theory thus offers a unified explanation for the in-plane AHE recently observed in various ferromagnets, and further extends the candidate material systems. It can also be generalized to study the anomalous Hall effect in crystals with any periodic spin structure and to study the nonlinear Hall effect and the spin Hall effect. Our theory lays the ground for decoding the coupling between various transport and optical phenomena and the magnetic orders. Published by the American Physical Society 2025
关于铁磁体中反常霍尔效应的传统观点认为,反常霍尔效应是由垂直于测量平面的磁化引起的,并且与测量平面的磁化呈线性关系。这种观点的基础是认为AHE是一种时间反转对称性破缺现象,因此可以用磁序的幂级数来处理。然而,这一观点受到了最近一些实验的直接挑战,迫切需要在基本层面上进行彻底的理论研究。我们发现,对于强磁体,将AHE视为一种自旋-群对称破缺现象更为合适和有效,其关键参数是自旋-轨道相互作用强度,涉及的能量尺度要小得多。在共线铁磁体中,自旋轨道耦合破坏了∞2’自旋旋转对称性,表征这种对称性破坏的关键是识别自旋群操作下有规则变换的自旋轨道向量。从我们的框架中诞生了异常霍尔电导率与磁化方向之间丰富的多极关系,每个极点在自旋轨道耦合强度的幂次上逐步扩展。对于阶贡献即偶极子,其各向同性部分符合传统观点,其各向异性部分可导致磁化位于测量平面内的面内AHE。除了偶极结构之外,八极结构提供了非线性的主要来源,因此引入了偶极结构所不能的独特的各向异性。因此,我们的理论为最近在各种铁磁体中观察到的面内AHE提供了统一的解释,并进一步扩展了候选材料体系。它也可以推广到研究任意周期自旋结构晶体中的反常霍尔效应,以及研究非线性霍尔效应和自旋霍尔效应。我们的理论为解码各种输运和光现象与磁序之间的耦合奠定了基础。2025年由美国物理学会出版
{"title":"Multipolar Anisotropy in Anomalous Hall Effect from Spin-Group Symmetry Breaking","authors":"Zheng Liu, Mengjie Wei, Wenzhi Peng, Dazhi Hou, Yang Gao, Qian Niu","doi":"10.1103/physrevx.15.031006","DOIUrl":"https://doi.org/10.1103/physrevx.15.031006","url":null,"abstract":"The traditional view of the anomalous Hall effect (AHE) in ferromagnets is that it arises from the magnetization perpendicular to the measurement plane and that there is a linear dependence on the latter. Underlying such a view is the thinking that the AHE is a time-reversal symmetry breaking phenomenon and can therefore be treated in terms of a power series in the magnetic order. However, this view is squarely challenged by a number of recent experiments, urging for a thorough theoretical investigation on the fundamental level. We find that for strong magnets, it is more appropriate and fruitful to regard the AHE as a spin-group symmetry breaking phenomenon where the critical parameter is the spin-orbit interaction strength, which involves a much smaller energy scale. In collinear ferromagnets, the spin-orbit coupling breaks the ∞</a:mi>2</a:mn>′</a:mo></a:msup></a:math> spin rotation symmetry, and the key to characterizing such symmetry breaking is the identification of spin-orbit vectors which transform regularly under spin-group operations. Born out of our framework is a rich multipolar relationship between the anomalous Hall conductivity and the magnetization direction, with each pole being expanded progressively in powers of the spin-orbit coupling strength. For the leading order contribution, i.e., the dipole, its isotropic part corresponds to the traditional view, and its anisotropic part can lead to the in-plane AHE where the magnetization lies within the measurement plane. Beyond the dipolar structure, the octupolar structure offers the leading order source of nonlinearity and hence introduces unique anisotropy where the dipolar structure cannot. Our theory thus offers a unified explanation for the in-plane AHE recently observed in various ferromagnets, and further extends the candidate material systems. It can also be generalized to study the anomalous Hall effect in crystals with any periodic spin structure and to study the nonlinear Hall effect and the spin Hall effect. Our theory lays the ground for decoding the coupling between various transport and optical phenomena and the magnetic orders. <jats:supplementary-material> <jats:copyright-statement>Published by the American Physical Society</jats:copyright-statement> <jats:copyright-year>2025</jats:copyright-year> </jats:permissions> </jats:supplementary-material>","PeriodicalId":20161,"journal":{"name":"Physical Review X","volume":"9 1","pages":""},"PeriodicalIF":12.5,"publicationDate":"2025-07-07","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144577863","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Flat-Band (De)localization Emulated with a Superconducting Qubit Array 用超导量子比特阵列模拟平带(De)定位
IF 12.5 1区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2025-06-16 DOI: 10.1103/physrevx.15.021091
Ilan T. Rosen, Sarah Muschinske, Cora N. Barrett, David A. Rower, Rabindra Das, David K. Kim, Bethany M. Niedzielski, Meghan Schuldt, Kyle Serniak, Mollie E. Schwartz, Jonilyn L. Yoder, Jeffrey A. Grover, William D. Oliver
Arrays of coupled superconducting qubits are analog quantum simulators able to emulate a wide range of tight-binding models in parameter regimes that are difficult to access or adjust in natural materials. In this work, we use a superconducting qubit array to emulate a tight-binding model on the rhombic lattice, which features flat bands. Enabled by broad adjustability of the dispersion of the energy bands and of on-site disorder, we examine regimes where flat-band localization and Anderson localization compete. We observe disorder-induced localization for dispersive bands and disorder-induced delocalization for flat bands. Remarkably, we find a sudden transition between the two regimes and, in its vicinity, the semblance of quantum critical scaling. Published by the American Physical Society 2025
耦合超导量子比特阵列是一种模拟量子模拟器,能够模拟各种紧结合模型,这些模型在天然材料中难以获得或调整。在这项工作中,我们使用超导量子比特阵列来模拟菱形晶格上的紧密结合模型,其特征是平坦带。由于能带色散和现场无序的广泛可调性,我们研究了平带定位和安德森定位竞争的制度。我们观察到色散带的无序诱导定位和平坦带的无序诱导离域。值得注意的是,我们发现了两种状态之间的突然转变,并且在其附近,类似于量子临界尺度。2025年由美国物理学会出版
{"title":"Flat-Band (De)localization Emulated with a Superconducting Qubit Array","authors":"Ilan T. Rosen, Sarah Muschinske, Cora N. Barrett, David A. Rower, Rabindra Das, David K. Kim, Bethany M. Niedzielski, Meghan Schuldt, Kyle Serniak, Mollie E. Schwartz, Jonilyn L. Yoder, Jeffrey A. Grover, William D. Oliver","doi":"10.1103/physrevx.15.021091","DOIUrl":"https://doi.org/10.1103/physrevx.15.021091","url":null,"abstract":"Arrays of coupled superconducting qubits are analog quantum simulators able to emulate a wide range of tight-binding models in parameter regimes that are difficult to access or adjust in natural materials. In this work, we use a superconducting qubit array to emulate a tight-binding model on the rhombic lattice, which features flat bands. Enabled by broad adjustability of the dispersion of the energy bands and of on-site disorder, we examine regimes where flat-band localization and Anderson localization compete. We observe disorder-induced localization for dispersive bands and disorder-induced delocalization for flat bands. Remarkably, we find a sudden transition between the two regimes and, in its vicinity, the semblance of quantum critical scaling. <jats:supplementary-material> <jats:copyright-statement>Published by the American Physical Society</jats:copyright-statement> <jats:copyright-year>2025</jats:copyright-year> </jats:permissions> </jats:supplementary-material>","PeriodicalId":20161,"journal":{"name":"Physical Review X","volume":"70 1","pages":""},"PeriodicalIF":12.5,"publicationDate":"2025-06-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144304494","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Fault-Tolerant Logical Measurements via Homological Measurement 通过同调度量实现的容错逻辑度量
IF 12.5 1区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2025-06-10 DOI: 10.1103/physrevx.15.021088
Benjamin Ide, Manoj G. Gowda, Priya J. Nadkarni, Guillaume Dauphinais
We introduce homological measurement, a framework for measuring the logical Pauli operators encoded in Calderbank-Shor-Steane stabilizer codes. The framework is based on the algebraic description of such codes as chain complexes. Protocols such as lattice surgery and some of its recent generalizations are shown to be special cases of homological measurement. Using this framework, we develop a specific protocol called edge expanded homological measurement for fault-tolerant measurement of arbitrary logical Pauli operators of general quantum low density parity-check codes, requiring a number of ancillary qubits growing only linearly with the weight of the logical operator measured, and guarantee that the distance of the code is preserved. We further benchmark our protocol numerically in a photonic architecture based on Gottesman-Kitaev-Preskill qubits, showing that the logical error rates of various codes are on par with other methods requiring more ancilla qubits. Published by the American Physical Society 2025
介绍了一种测量编码在calderbank - shorr - steane稳定码中的逻辑泡利算子的框架——同调测量。该框架基于链配合物等代码的代数描述。晶格手术等方案及其最近的一些推广被证明是同调测量的特殊情况。在此框架下,我们开发了一种称为边缘扩展同调测量的特定协议,用于一般量子低密度奇偶校验码的任意逻辑泡利算子的容错测量,该协议要求辅助量子比特的数量仅随所测量逻辑算子的权重线性增长,并保证码的距离保持不变。我们进一步在基于Gottesman-Kitaev-Preskill量子比特的光子架构中对我们的协议进行数值基准测试,表明各种代码的逻辑错误率与其他需要更多辅助量子比特的方法相当。2025年由美国物理学会出版
{"title":"Fault-Tolerant Logical Measurements via Homological Measurement","authors":"Benjamin Ide, Manoj G. Gowda, Priya J. Nadkarni, Guillaume Dauphinais","doi":"10.1103/physrevx.15.021088","DOIUrl":"https://doi.org/10.1103/physrevx.15.021088","url":null,"abstract":"We introduce homological measurement, a framework for measuring the logical Pauli operators encoded in Calderbank-Shor-Steane stabilizer codes. The framework is based on the algebraic description of such codes as chain complexes. Protocols such as lattice surgery and some of its recent generalizations are shown to be special cases of homological measurement. Using this framework, we develop a specific protocol called edge expanded homological measurement for fault-tolerant measurement of arbitrary logical Pauli operators of general quantum low density parity-check codes, requiring a number of ancillary qubits growing only linearly with the weight of the logical operator measured, and guarantee that the distance of the code is preserved. We further benchmark our protocol numerically in a photonic architecture based on Gottesman-Kitaev-Preskill qubits, showing that the logical error rates of various codes are on par with other methods requiring more ancilla qubits. <jats:supplementary-material> <jats:copyright-statement>Published by the American Physical Society</jats:copyright-statement> <jats:copyright-year>2025</jats:copyright-year> </jats:permissions> </jats:supplementary-material>","PeriodicalId":20161,"journal":{"name":"Physical Review X","volume":"40 1","pages":""},"PeriodicalIF":12.5,"publicationDate":"2025-06-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144260069","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Nonequilibrium Dynamics of Long-Range Interacting Fermions 远距离相互作用费米子的非平衡动力学
IF 12.5 1区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2025-06-10 DOI: 10.1103/physrevx.15.021089
T. Zwettler, G. Del Pace, F. Marijanovic, S. Chattopadhyay, T. Bühler, C.-M. Halati, L. Skolc, L. Tolle, V. Helson, G. Bolognini, A. Fabre, S. Uchino, T. Giamarchi, E. Demler, J. P. Brantut
A fundamental problem of out-of-equilibrium physics is the speed at which the order parameter grows upon crossing a phase transition. Here, we investigate the ordering dynamics in a Fermi gas undergoing a density-wave phase transition induced by quenching infinite-range, cavity-mediated interactions. We observe, in real time, the exponential rise of the order parameter and track its growth over several orders of magnitude. Remarkably, the growth rate can exceed the Fermi energy by an order of magnitude, consistent with predictions from a linearized instability analysis. This case contrasts with the ordering process driven by short-range interactions. We then generalize our results to linear interaction ramps, where deviations from the adiabatic behavior are captured by a simple dynamical ansatz. Our study offers a paradigmatic example of the interplay between strong short- and long-range interactions in quantum nonequilibrium dynamics. Published by the American Physical Society 2025
非平衡物理的一个基本问题是序参量在跨越相变时增长的速度。在这里,我们研究了费米气体中由猝灭无限范围、腔介导的相互作用引起的密度波相变的有序动力学。我们实时观察到序参数的指数上升,并跟踪其在几个数量级上的增长。值得注意的是,增长率可以超过费米能量一个数量级,这与线性化不稳定性分析的预测一致。这种情况与由短程相互作用驱动的排序过程形成对比。然后,我们将我们的结果推广到线性相互作用斜坡,其中从绝热行为的偏差被一个简单的动态分析捕获。我们的研究提供了量子非平衡动力学中强短期和长期相互作用之间相互作用的范例。2025年由美国物理学会出版
{"title":"Nonequilibrium Dynamics of Long-Range Interacting Fermions","authors":"T. Zwettler, G. Del Pace, F. Marijanovic, S. Chattopadhyay, T. Bühler, C.-M. Halati, L. Skolc, L. Tolle, V. Helson, G. Bolognini, A. Fabre, S. Uchino, T. Giamarchi, E. Demler, J. P. Brantut","doi":"10.1103/physrevx.15.021089","DOIUrl":"https://doi.org/10.1103/physrevx.15.021089","url":null,"abstract":"A fundamental problem of out-of-equilibrium physics is the speed at which the order parameter grows upon crossing a phase transition. Here, we investigate the ordering dynamics in a Fermi gas undergoing a density-wave phase transition induced by quenching infinite-range, cavity-mediated interactions. We observe, in real time, the exponential rise of the order parameter and track its growth over several orders of magnitude. Remarkably, the growth rate can exceed the Fermi energy by an order of magnitude, consistent with predictions from a linearized instability analysis. This case contrasts with the ordering process driven by short-range interactions. We then generalize our results to linear interaction ramps, where deviations from the adiabatic behavior are captured by a simple dynamical ansatz. Our study offers a paradigmatic example of the interplay between strong short- and long-range interactions in quantum nonequilibrium dynamics. <jats:supplementary-material> <jats:copyright-statement>Published by the American Physical Society</jats:copyright-statement> <jats:copyright-year>2025</jats:copyright-year> </jats:permissions> </jats:supplementary-material>","PeriodicalId":20161,"journal":{"name":"Physical Review X","volume":"88 1","pages":""},"PeriodicalIF":12.5,"publicationDate":"2025-06-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144260070","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Nonlocal Moments and Mott Semimetal in the Chern Bands of Twisted Bilayer Graphene 扭曲双层石墨烯Chern带中的非局域矩和莫特半金属
IF 12.5 1区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2025-06-09 DOI: 10.1103/physrevx.15.021087
Patrick J. Ledwith, Junkai Dong, Ashvin Vishwanath, Eslam Khalaf
Twisted bilayer graphene (TBG) has elements in common with two paradigmatic examples of strongly correlated physics: quantum Hall physics and Hubbard physics. On one hand, TBG hosts flat topological Landau-level-like bands which exhibit the quantum anomalous Hall effects under the right conditions. On the other hand, these bands are characterized by concentrated charge density and show signs of extensive entropy usually attributed to local moments. The combination of these features leads to a question: Can decoupled moments emerge in an isolated topological band, despite the lack of exponentially localized Wannier orbitals? In this work, we answer the question affirmatively by proposing a minimal model for the flat topological bands in TBG that combines topology and charge concentration at the AA sites, leading to analytic wave functions that closely approximate those of the Bistritzer-MacDonald model with realistic parameters. Importantly, charge concentration also leads to Berry curvature concentration at Γ, giving rise to a small parameter s that makes the model analytically tractable. We show that, rather surprisingly, the model hosts nearly decoupled flavor moments without invoking any extra degrees of freedom. These moments are nonlocal due to topology-enforced power-law tails, yet have parametrically small overlap. We develop a systematic diagrammatic expansion in which the self-energy can be computed exactly to leading order in s2 in the fluctuating moment regime and predict momentum-resolved spectral functions for future experiments to verify. Our key discovery is a charge-neutrality state we refer to as the “Mott semimetal” characterized by high flavor entropy and a Mott gap that exists throughout most of the Brillouin zone but closes at the Γ point. At Γ, the spectral function contains a single Dirac cone per spin per valley and responds to perturbations in an exotic manner that is distinct from any other theoretical picture of TBG. Away from neutrality, the Mott semimetal gaps out in a spectrally imbalanced manner, with one Mott band having zero quasiparticle residue at the Γ point. The model accurately reproduces results from finite-temperature thermodynamic measurements, leads to new experimental predictions, and resolves the problem of the emergence of Hubbard physics in isolated topological bands. Published by the Ame
扭曲双层石墨烯(TBG)与量子霍尔物理和哈伯德物理这两个强相关物理学的典型例子有一些共同之处。一方面,TBG具有平坦的拓扑类朗道能级带,在适当的条件下表现出量子反常霍尔效应。另一方面,这些能带的特点是电荷密度集中,并表现出通常归因于局部矩的广泛熵的迹象。这些特征的结合导致了一个问题:尽管缺乏指数局域化的万尼尔轨道,解耦矩能否出现在孤立的拓扑带中?在这项工作中,我们通过提出一个结合拓扑和AA点电荷浓度的TBG平坦拓扑带的最小模型,肯定地回答了这个问题,从而得到了与具有现实参数的Bistritzer-MacDonald模型非常接近的解析波函数。重要的是,电荷浓度也会导致Γ处的贝里曲率浓度,从而产生一个小参数s,使模型易于分析。我们表明,相当令人惊讶的是,该模型承载了几乎解耦的风味时刻,而没有调用任何额外的自由度。由于拓扑强制幂律尾,这些矩是非局部的,但参数上的重叠很小。我们开发了一个系统的图解展开,其中自能可以精确地计算到脉动矩状态下s2的领先阶,并预测动量分辨谱函数,以供将来的实验验证。我们的主要发现是一种电荷中性状态,我们称之为“莫特半金属”,其特点是高风味熵和莫特间隙存在于大部分布里温区,但在Γ点关闭。在Γ,谱函数包含每个自旋每个谷的单个狄拉克锥,并以一种独特的方式响应摄动,这与任何其他理论的TBG图像都不同。远离中性,莫特半金属以光谱不平衡的方式出现间隙,其中一个莫特带在Γ点上具有零准粒子残留。该模型准确地再现了有限温度热力学测量的结果,导致了新的实验预测,并解决了孤立拓扑带中出现哈伯德物理的问题。2025年由美国物理学会出版
{"title":"Nonlocal Moments and Mott Semimetal in the Chern Bands of Twisted Bilayer Graphene","authors":"Patrick J. Ledwith, Junkai Dong, Ashvin Vishwanath, Eslam Khalaf","doi":"10.1103/physrevx.15.021087","DOIUrl":"https://doi.org/10.1103/physrevx.15.021087","url":null,"abstract":"Twisted bilayer graphene (TBG) has elements in common with two paradigmatic examples of strongly correlated physics: quantum Hall physics and Hubbard physics. On one hand, TBG hosts flat topological Landau-level-like bands which exhibit the quantum anomalous Hall effects under the right conditions. On the other hand, these bands are characterized by concentrated charge density and show signs of extensive entropy usually attributed to local moments. The combination of these features leads to a question: Can decoupled moments emerge in an isolated topological band, despite the lack of exponentially localized Wannier orbitals? In this work, we answer the question affirmatively by proposing a minimal model for the flat topological bands in TBG that combines topology and charge concentration at the AA sites, leading to analytic wave functions that closely approximate those of the Bistritzer-MacDonald model with realistic parameters. Importantly, charge concentration also leads to Berry curvature concentration at Γ</a:mi></a:math>, giving rise to a small parameter <d:math xmlns:d=\"http://www.w3.org/1998/Math/MathML\" display=\"inline\"><d:mi>s</d:mi></d:math> that makes the model analytically tractable. We show that, rather surprisingly, the model hosts nearly decoupled flavor moments without invoking any extra degrees of freedom. These moments are nonlocal due to topology-enforced power-law tails, yet have parametrically small overlap. We develop a systematic diagrammatic expansion in which the self-energy can be computed exactly to leading order in <f:math xmlns:f=\"http://www.w3.org/1998/Math/MathML\" display=\"inline\"><f:msup><f:mi>s</f:mi><f:mn>2</f:mn></f:msup></f:math> in the fluctuating moment regime and predict momentum-resolved spectral functions for future experiments to verify. Our key discovery is a charge-neutrality state we refer to as the “Mott semimetal” characterized by high flavor entropy and a Mott gap that exists throughout most of the Brillouin zone but closes at the <h:math xmlns:h=\"http://www.w3.org/1998/Math/MathML\" display=\"inline\"><h:mi mathvariant=\"normal\">Γ</h:mi></h:math> point. At <k:math xmlns:k=\"http://www.w3.org/1998/Math/MathML\" display=\"inline\"><k:mi mathvariant=\"normal\">Γ</k:mi></k:math>, the spectral function contains a single Dirac cone per spin per valley and responds to perturbations in an exotic manner that is distinct from any other theoretical picture of TBG. Away from neutrality, the Mott semimetal gaps out in a spectrally imbalanced manner, with one Mott band having zero quasiparticle residue at the <n:math xmlns:n=\"http://www.w3.org/1998/Math/MathML\" display=\"inline\"><n:mi mathvariant=\"normal\">Γ</n:mi></n:math> point. The model accurately reproduces results from finite-temperature thermodynamic measurements, leads to new experimental predictions, and resolves the problem of the emergence of Hubbard physics in isolated topological bands. <jats:supplementary-material> <jats:copyright-statement>Published by the Ame","PeriodicalId":20161,"journal":{"name":"Physical Review X","volume":"50 1","pages":""},"PeriodicalIF":12.5,"publicationDate":"2025-06-09","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144252030","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Emergent Dimer-Model Topological Order and Quasiparticle Excitations in Liquid Crystals: Combinatorial Vortex Lattices 液晶中的涌现二聚体模型拓扑秩序和准粒子激发:组合涡旋晶格
IF 12.5 1区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2025-06-06 DOI: 10.1103/physrevx.15.021084
Cuiling Meng, Jin-Sheng Wu, Žiga Kos, Jörn Dunkel, Cristiano Nisoli, Ivan I. Smalyukh
Liquid crystals have proven to provide a versatile experimental and theoretical platform for studying topological objects such as vortices, skyrmions, and hopfions. In parallel, in hard condensed matter physics, the concept of topological phases and topological order has been introduced in the context of spin liquids to investigate emergent phenomena like quantum Hall effects and high-temperature superconductivity. Here, we bridge these two seemingly disparate perspectives on topology in physics. Combining experiments and simulations, we show how topological defects in liquid crystals can be used as versatile building blocks to create complex, highly degenerate topological phases, which we refer to as “combinatorial vortex lattices” (CVLs). CVLs exhibit extensive residual entropy and support locally stable quasiparticle excitations in the form of charge-conserving topological monopoles, which can act as mobile information carriers and be linked via Dirac strings. CVLs can be rewritten and reconfigured on demand, endowed with various symmetries, and modified through laser-induced topological surgery—an essential capability for information storage and retrieval. We demonstrate experimentally the realization, stability, and precise optical manipulation of CVLs, thus opening new avenues for understanding and technologically exploiting higher-hierarchy topology in liquid crystals and other ordered media. Published by the American Physical Society 2025
液晶已被证明为研究拓扑对象(如漩涡、天空边缘和跳跃)提供了一个通用的实验和理论平台。同时,在硬凝聚态物理中,拓扑相和拓扑序的概念也被引入到自旋液体中,用于研究量子霍尔效应和高温超导等涌现现象。在这里,我们将这两种看似不同的物理学拓扑学观点联系起来。结合实验和模拟,我们展示了如何将液晶中的拓扑缺陷用作多功能构建块来创建复杂的,高度退化的拓扑相,我们称之为“组合涡晶格”(CVLs)。cvl具有广泛的剩余熵,支持电荷守恒拓扑单极子形式的局部稳定准粒子激发,可以作为移动信息载体并通过狄拉克弦连接。cvl可以根据需要重写和重新配置,赋予各种对称性,并通过激光诱导拓扑手术进行修改,这是信息存储和检索的基本能力。我们通过实验证明了cvl的实现、稳定性和精确的光学操作,从而为理解和技术开发液晶和其他有序介质中的更高层次拓扑开辟了新的途径。2025年由美国物理学会出版
{"title":"Emergent Dimer-Model Topological Order and Quasiparticle Excitations in Liquid Crystals: Combinatorial Vortex Lattices","authors":"Cuiling Meng, Jin-Sheng Wu, Žiga Kos, Jörn Dunkel, Cristiano Nisoli, Ivan I. Smalyukh","doi":"10.1103/physrevx.15.021084","DOIUrl":"https://doi.org/10.1103/physrevx.15.021084","url":null,"abstract":"Liquid crystals have proven to provide a versatile experimental and theoretical platform for studying topological objects such as vortices, skyrmions, and hopfions. In parallel, in hard condensed matter physics, the concept of topological phases and topological order has been introduced in the context of spin liquids to investigate emergent phenomena like quantum Hall effects and high-temperature superconductivity. Here, we bridge these two seemingly disparate perspectives on topology in physics. Combining experiments and simulations, we show how topological defects in liquid crystals can be used as versatile building blocks to create complex, highly degenerate topological phases, which we refer to as “combinatorial vortex lattices” (CVLs). CVLs exhibit extensive residual entropy and support locally stable quasiparticle excitations in the form of charge-conserving topological monopoles, which can act as mobile information carriers and be linked via Dirac strings. CVLs can be rewritten and reconfigured on demand, endowed with various symmetries, and modified through laser-induced topological surgery—an essential capability for information storage and retrieval. We demonstrate experimentally the realization, stability, and precise optical manipulation of CVLs, thus opening new avenues for understanding and technologically exploiting higher-hierarchy topology in liquid crystals and other ordered media. <jats:supplementary-material> <jats:copyright-statement>Published by the American Physical Society</jats:copyright-statement> <jats:copyright-year>2025</jats:copyright-year> </jats:permissions> </jats:supplementary-material>","PeriodicalId":20161,"journal":{"name":"Physical Review X","volume":"36 1","pages":""},"PeriodicalIF":12.5,"publicationDate":"2025-06-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144236905","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Phase Diagram of Extensive-Rank Symmetric Matrix Denoising beyond Rotational Invariance 超越旋转不变性的广义秩对称矩阵去噪的相位图
IF 12.5 1区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2025-06-06 DOI: 10.1103/physrevx.15.021085
Jean Barbier, Francesco Camilli, Justin Ko, Koki Okajima
Matrix denoising is central to signal processing and machine learning. Its statistical analysis when the matrix to infer has a factorized structure with a rank growing proportionally to its dimension remains a challenge, except when it is rotationally invariant. In this case, the information-theoretic limits and an efficient Bayes-optimal denoising algorithm, called the rotational invariant estimator, are known. Beyond this setting, few results can be found. The reason is that the model is not a usual spin system because of the growing rank dimension, nor a matrix model (as appearing in high-energy physics) due to the lack of rotation symmetry, but rather a hybrid between the two. In this paper, we make progress toward the understanding of Bayesian matrix denoising when the hidden signal is a factored matrix XX⊺ that is not rotationally invariant. Monte Carlo simulations suggest the existence of a denoising-factorization transition separating a phase where denoising using the rotational-invariant estimator remains Bayes-optimal due to universality properties of the same nature as in random matrix theory, from one where universality breaks down and better denoising is possible, though algorithmically hard. We also argue that it is only beyond the transition that factorization, i.e., estimating X itself, becomes possible up to irresolvable ambiguities. On the theoretical side, we combine mean-field techniques in an interpretable multiscale fashion in order to access the minimum mean-square error and mutual information. Interestingly, our alternative method yields equations reproducible by the replica approach of Sakata and Kabashima. Using numerical insights, we delimit the portion of phase diagram where we conjecture the mean-field theory to be exact and correct it using universality when it is not. Our complete matches well the numerics in the whole phase diagram when considering finite-size effects. Published by the American Physical Society 2025
矩阵去噪是信号处理和机器学习的核心。当要推断的矩阵具有秩与维数成比例增长的分解结构时,它的统计分析仍然是一个挑战,除非它是旋转不变的。在这种情况下,信息论的极限和有效的贝叶斯最优去噪算法,称为旋转不变估计,是已知的。在此设置之外,几乎找不到结果。原因是该模型不是通常的自旋系统,因为秩维不断增加,也不是矩阵模型(如在高能物理中出现的),因为缺乏旋转对称性,而是两者的混合。在本文中,我们在理解当隐藏信号是一个非旋转不变的因子矩阵XX⊺时的贝叶斯矩阵去噪方面取得了进展。蒙特卡罗模拟表明,存在一个去噪分解过渡,将一个阶段分离开来,在这个阶段中,由于与随机矩阵理论相同的普适性,使用旋转不变估计器进行去噪仍然是贝叶斯最优的,而在这个阶段中,普适性被打破,更好的去噪是可能的,尽管在算法上很难。我们还认为,只有在过渡之外,因式分解,即估计X本身,才有可能达到无法解决的歧义。在理论方面,我们以可解释的多尺度方式结合平均场技术,以获得最小均方误差和互信息。有趣的是,我们的替代方法产生的方程可以通过Sakata和Kabashima的复制方法再现。在相图中,我们用数值方法对平均场理论进行了精确的推测,并在不精确时使用普适性对其进行了修正。当考虑有限尺寸效应时,我们的完全符合整个相图中的数值。2025年由美国物理学会出版
{"title":"Phase Diagram of Extensive-Rank Symmetric Matrix Denoising beyond Rotational Invariance","authors":"Jean Barbier, Francesco Camilli, Justin Ko, Koki Okajima","doi":"10.1103/physrevx.15.021085","DOIUrl":"https://doi.org/10.1103/physrevx.15.021085","url":null,"abstract":"Matrix denoising is central to signal processing and machine learning. Its statistical analysis when the matrix to infer has a factorized structure with a rank growing proportionally to its dimension remains a challenge, except when it is rotationally invariant. In this case, the information-theoretic limits and an efficient Bayes-optimal denoising algorithm, called the rotational invariant estimator, are known. Beyond this setting, few results can be found. The reason is that the model is not a usual spin system because of the growing rank dimension, nor a matrix model (as appearing in high-energy physics) due to the lack of rotation symmetry, but rather a hybrid between the two. In this paper, we make progress toward the understanding of Bayesian matrix denoising when the hidden signal is a factored matrix X</a:mi></a:mrow>X</a:mi></a:mrow>⊺</a:mo></a:mrow></a:msup></a:mrow></a:math> that is not rotationally invariant. Monte Carlo simulations suggest the existence of a denoising-factorization transition separating a phase where denoising using the rotational-invariant estimator remains Bayes-optimal due to universality properties of the same nature as in random matrix theory, from one where universality breaks down and better denoising is possible, though algorithmically hard. We also argue that it is only beyond the transition that factorization, i.e., estimating <e:math xmlns:e=\"http://www.w3.org/1998/Math/MathML\" display=\"inline\"><e:mrow><e:mi mathvariant=\"bold\">X</e:mi></e:mrow></e:math> itself, becomes possible up to irresolvable ambiguities. On the theoretical side, we combine mean-field techniques in an interpretable multiscale fashion in order to access the minimum mean-square error and mutual information. Interestingly, our alternative method yields equations reproducible by the replica approach of Sakata and Kabashima. Using numerical insights, we delimit the portion of phase diagram where we conjecture the mean-field theory to be exact and correct it using universality when it is not. Our complete matches well the numerics in the whole phase diagram when considering finite-size effects. <jats:supplementary-material> <jats:copyright-statement>Published by the American Physical Society</jats:copyright-statement> <jats:copyright-year>2025</jats:copyright-year> </jats:permissions> </jats:supplementary-material>","PeriodicalId":20161,"journal":{"name":"Physical Review X","volume":"42 1","pages":""},"PeriodicalIF":12.5,"publicationDate":"2025-06-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144236906","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Demonstration of Algorithmic Quantum Speedup for an Abelian Hidden Subgroup Problem 一类阿贝尔隐子群问题的量子加速算法论证
IF 12.5 1区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2025-06-05 DOI: 10.1103/physrevx.15.021082
Phattharaporn Singkanipa, Victor Kasatkin, Zeyuan Zhou, Gregory Quiroz, Daniel A. Lidar
Simon’s problem is to find a hidden period (a bitstring) encoded into an unknown 2-to-1 function. It is one of the earliest problems for which an exponential quantum speedup was proven for ideal, noiseless quantum computers, albeit in the oracle model. Here, using two different 127-qubit IBM Quantum superconducting processors, we demonstrate an algorithmic quantum speedup for a variant of Simon’s problem where the hidden period has a restricted Hamming weight w. For sufficiently small values of w and for circuits involving up to 58 qubits, we demonstrate an exponential speedup, albeit of a lower quality than the speedup predicted for the noiseless algorithm. The speedup exponent and the range of w values for which an exponential speedup exists are significantly enhanced when the computation is protected by dynamical decoupling. Further enhancement is achieved with measurement error mitigation. This case constitutes a demonstration of a bona fide quantum advantage for an Abelian hidden subgroup problem. Published by the American Physical Society 2025
Simon的问题是找到一个隐藏的周期(一个位串)编码成一个未知的2对1函数。这是指数量子加速最早被证明适用于理想的无噪声量子计算机的问题之一,尽管是在oracle模型中。在这里,使用两个不同的127量子位IBM量子超导处理器,我们展示了一种算法量子加速,用于西蒙问题的一个变体,其中隐藏周期具有有限的汉明权重w。对于足够小的w值和涉及多达58量子位的电路,我们展示了指数级加速,尽管质量低于无噪声算法预测的加速。在动态解耦保护下,加速指数和存在指数加速的w值范围得到了显著提高。进一步的增强是通过降低测量误差来实现的。这种情况构成了一个真正的量子优势的阿贝尔隐子群问题的演示。2025年由美国物理学会出版
{"title":"Demonstration of Algorithmic Quantum Speedup for an Abelian Hidden Subgroup Problem","authors":"Phattharaporn Singkanipa, Victor Kasatkin, Zeyuan Zhou, Gregory Quiroz, Daniel A. Lidar","doi":"10.1103/physrevx.15.021082","DOIUrl":"https://doi.org/10.1103/physrevx.15.021082","url":null,"abstract":"Simon’s problem is to find a hidden period (a bitstring) encoded into an unknown 2-to-1 function. It is one of the earliest problems for which an exponential quantum speedup was proven for ideal, noiseless quantum computers, albeit in the oracle model. Here, using two different 127-qubit IBM Quantum superconducting processors, we demonstrate an algorithmic quantum speedup for a variant of Simon’s problem where the hidden period has a restricted Hamming weight w</a:mi></a:math>. For sufficiently small values of <c:math xmlns:c=\"http://www.w3.org/1998/Math/MathML\" display=\"inline\"><c:mi>w</c:mi></c:math> and for circuits involving up to 58 qubits, we demonstrate an exponential speedup, albeit of a lower quality than the speedup predicted for the noiseless algorithm. The speedup exponent and the range of <e:math xmlns:e=\"http://www.w3.org/1998/Math/MathML\" display=\"inline\"><e:mi>w</e:mi></e:math> values for which an exponential speedup exists are significantly enhanced when the computation is protected by dynamical decoupling. Further enhancement is achieved with measurement error mitigation. This case constitutes a demonstration of a bona fide quantum advantage for an Abelian hidden subgroup problem. <jats:supplementary-material> <jats:copyright-statement>Published by the American Physical Society</jats:copyright-statement> <jats:copyright-year>2025</jats:copyright-year> </jats:permissions> </jats:supplementary-material>","PeriodicalId":20161,"journal":{"name":"Physical Review X","volume":"39 1","pages":""},"PeriodicalIF":12.5,"publicationDate":"2025-06-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144228572","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Catalog of C -Paired Spin-Momentum Locking in Antiferromagnetic Systems 反铁磁系统中C对自旋动量锁定的目录
IF 12.5 1区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2025-06-05 DOI: 10.1103/physrevx.15.021083
Mengli Hu, Xingkai Cheng, Zhenqiao Huang, Junwei Liu
Antiferromagnetic materials (AFMs) have been gaining lots of attention due to their great potential in spintronics devices and the recently discovered novel spin structure in the momentum space, i.e., C-paired spin-valley or spin-momentum locking (CSML), where spins and valleys or momenta are locked to each other due to the crystal symmetry guaranteeing zero magnetization. Here, we systematically study CSMLs and propose a general theory and algorithm using little cogroup and coset representatives, which reveals that 12 elementary kinds of CSMLs, determined by the geometric relation of spins and valleys and the essential symmetry guaranteeing zero magnetization, are sufficient to fully represent all possible CSMLs. By combining the proposed algorithm and high-throughput first-principles calculations, we predict 38 magnetic point groups and identify 142 experimentally verified AFMs that can realize CSML. Besides predicting new materials, our theory can naturally reveal underlying mechanisms of CSMLs’ responses to external fields. As an example, two qualitatively different types of piezomagnetism via occupation imbalance or spin tilting are predicted in RbV2Te2O. The algorithm and conclusions can be directly extended to the locking between valley or momentum and any other pseudovector degree of freedom, e.g., Berry curvature, as exemplified in RbV2Te2O and the new proposed piezo-Hall effect, where a strain can induce a nonzero anomalous Hall conductance. In addition, the proposed concept and methodology can be straightforwardly applied to other symmetry groups, such as spin group. Published by the American Physical Society 2025
反铁磁材料(AFMs)由于其在自旋电子学器件中的巨大潜力以及最近在动量空间中发现的新的自旋结构,即c对自旋谷或自旋动量锁定(CSML),其中自旋和自旋谷或动量由于晶体对称性保证零磁化而相互锁定。本文系统地研究了csml,并提出了一种利用小共群和共集表示的一般理论和算法,结果表明,由自旋和谷的几何关系和保证零磁化的基本对称性所决定的12种基本csml足以充分表示所有可能的csml。通过将该算法与高通量第一性原理计算相结合,我们预测了38个磁点群,并鉴定了142个实验验证的可实现CSML的原子力显微镜。除了预测新材料外,我们的理论还可以自然地揭示csml对外部场响应的潜在机制。以RbV2Te2O为例,通过占位不平衡和自旋倾斜预测了两种性质不同的压磁性。该算法和结论可以直接推广到谷或动量与任何其他伪矢量自由度之间的锁定,例如RbV2Te2O和新提出的压电霍尔效应,其中应变可以诱导非零异常霍尔电导。此外,所提出的概念和方法可以直接应用于其他对称群,如自旋群。2025年由美国物理学会出版
{"title":"Catalog of C -Paired Spin-Momentum Locking in Antiferromagnetic Systems","authors":"Mengli Hu, Xingkai Cheng, Zhenqiao Huang, Junwei Liu","doi":"10.1103/physrevx.15.021083","DOIUrl":"https://doi.org/10.1103/physrevx.15.021083","url":null,"abstract":"Antiferromagnetic materials (AFMs) have been gaining lots of attention due to their great potential in spintronics devices and the recently discovered novel spin structure in the momentum space, i.e., C</a:mi></a:mrow></a:math>-paired spin-valley or spin-momentum locking (CSML), where spins and valleys or momenta are locked to each other due to the crystal symmetry guaranteeing zero magnetization. Here, we systematically study CSMLs and propose a general theory and algorithm using little cogroup and coset representatives, which reveals that 12 elementary kinds of CSMLs, determined by the geometric relation of spins and valleys and the essential symmetry guaranteeing zero magnetization, are sufficient to fully represent all possible CSMLs. By combining the proposed algorithm and high-throughput first-principles calculations, we predict 38 magnetic point groups and identify 142 experimentally verified AFMs that can realize CSML. Besides predicting new materials, our theory can naturally reveal underlying mechanisms of CSMLs’ responses to external fields. As an example, two qualitatively different types of piezomagnetism via occupation imbalance or spin tilting are predicted in <c:math xmlns:c=\"http://www.w3.org/1998/Math/MathML\" display=\"inline\"><c:mrow><c:mrow><c:msub><c:mrow><c:mi>RbV</c:mi></c:mrow><c:mrow><c:mn>2</c:mn></c:mrow></c:msub></c:mrow><c:mrow><c:msub><c:mrow><c:mi>Te</c:mi></c:mrow><c:mrow><c:mn>2</c:mn></c:mrow></c:msub></c:mrow><c:mi mathvariant=\"normal\">O</c:mi></c:mrow></c:math>. The algorithm and conclusions can be directly extended to the locking between valley or momentum and any other pseudovector degree of freedom, e.g., Berry curvature, as exemplified in <f:math xmlns:f=\"http://www.w3.org/1998/Math/MathML\" display=\"inline\"><f:mrow><f:mrow><f:msub><f:mrow><f:mi>RbV</f:mi></f:mrow><f:mrow><f:mn>2</f:mn></f:mrow></f:msub></f:mrow><f:mrow><f:msub><f:mrow><f:mi>Te</f:mi></f:mrow><f:mrow><f:mn>2</f:mn></f:mrow></f:msub></f:mrow><f:mi mathvariant=\"normal\">O</f:mi></f:mrow></f:math> and the new proposed piezo-Hall effect, where a strain can induce a nonzero anomalous Hall conductance. In addition, the proposed concept and methodology can be straightforwardly applied to other symmetry groups, such as spin group. <jats:supplementary-material> <jats:copyright-statement>Published by the American Physical Society</jats:copyright-statement> <jats:copyright-year>2025</jats:copyright-year> </jats:permissions> </jats:supplementary-material>","PeriodicalId":20161,"journal":{"name":"Physical Review X","volume":"10 1","pages":""},"PeriodicalIF":12.5,"publicationDate":"2025-06-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144228524","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Defect Complexes in CrSBr Revealed Through Electron Microscopy and Deep Learning 通过电子显微镜和深度学习发现CrSBr中的缺陷复合物
IF 12.5 1区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2025-06-04 DOI: 10.1103/physrevx.15.021080
Mads Weile, Sergii Grytsiuk, Aubrey Penn, Daniel G. Chica, Xavier Roy, Kseniia Mosina, Zdenek Sofer, Jakob Schiøtz, Stig Helveg, Malte Rösner, Frances M. Ross, Julian Klein
Atomic defects underpin the properties of van der Waals materials, and their understanding is essential for advancing quantum and energy technologies. Scanning transmission electron microscopy is a powerful tool for defect identification in atomically thin materials, and extending it to multilayer and beam-sensitive materials would accelerate their exploration. Here, we establish a comprehensive defect library in a bilayer of the magnetic quasi-1D semiconductor CrSBr by combining atomic-resolution imaging, deep learning, and calculations. We apply a custom-developed machine learning work flow to detect, classify, and average point vacancy defects. This classification enables us to uncover several distinct Cr interstitial defect complexes, combined Cr and Br vacancy defect complexes, and lines of vacancy defects that extend over many unit cells. We show that their occurrence is in agreement with our computed structures and binding energy densities, reflecting the intriguing layer interlocked crystal structure of CrSBr. Our calculations show that the interstitial defect complexes give rise to highly localized electronic states. These states are of particular interest due to the reduced electronic dimensionality and magnetic properties of CrSBr and are, furthermore, predicted to be optically active. Our results broaden the scope of defect studies in challenging materials and reveal new defect types in bilayer CrSBr that can be extrapolated to the bulk and to over 20 materials belonging to the same FeOCl structural family. Published by the American Physical Society 2025
原子缺陷是范德华材料特性的基础,对它们的理解对于推进量子和能源技术至关重要。扫描透射电子显微镜是识别原子薄材料缺陷的有力工具,将其扩展到多层材料和光束敏感材料将加速其探索。本文采用原子分辨率成像、深度学习和计算相结合的方法,建立了磁性准一维半导体CrSBr双层结构的综合缺陷库。我们应用定制开发的机器学习工作流程来检测、分类和平均点空缺缺陷。这种分类使我们能够发现几种不同的Cr间质缺陷复合物,结合Cr和Br的空位缺陷复合物,以及延伸到许多单位细胞的空位缺陷线。我们发现它们的出现与我们计算的结构和结合能密度一致,反映了CrSBr有趣的层联锁晶体结构。我们的计算表明,间隙缺陷复合物会产生高度局域化的电子态。由于CrSBr的电子维数和磁性降低,这些状态特别令人感兴趣,此外,预测它们具有光学活性。我们的研究结果拓宽了具有挑战性材料缺陷研究的范围,揭示了双层CrSBr中新的缺陷类型,这些缺陷类型可以外推到块体和属于同一FeOCl结构家族的20多种材料。2025年由美国物理学会出版
{"title":"Defect Complexes in CrSBr Revealed Through Electron Microscopy and Deep Learning","authors":"Mads Weile, Sergii Grytsiuk, Aubrey Penn, Daniel G. Chica, Xavier Roy, Kseniia Mosina, Zdenek Sofer, Jakob Schiøtz, Stig Helveg, Malte Rösner, Frances M. Ross, Julian Klein","doi":"10.1103/physrevx.15.021080","DOIUrl":"https://doi.org/10.1103/physrevx.15.021080","url":null,"abstract":"Atomic defects underpin the properties of van der Waals materials, and their understanding is essential for advancing quantum and energy technologies. Scanning transmission electron microscopy is a powerful tool for defect identification in atomically thin materials, and extending it to multilayer and beam-sensitive materials would accelerate their exploration. Here, we establish a comprehensive defect library in a bilayer of the magnetic quasi-1D semiconductor CrSBr by combining atomic-resolution imaging, deep learning, and calculations. We apply a custom-developed machine learning work flow to detect, classify, and average point vacancy defects. This classification enables us to uncover several distinct Cr interstitial defect complexes, combined Cr and Br vacancy defect complexes, and lines of vacancy defects that extend over many unit cells. We show that their occurrence is in agreement with our computed structures and binding energy densities, reflecting the intriguing layer interlocked crystal structure of CrSBr. Our calculations show that the interstitial defect complexes give rise to highly localized electronic states. These states are of particular interest due to the reduced electronic dimensionality and magnetic properties of CrSBr and are, furthermore, predicted to be optically active. Our results broaden the scope of defect studies in challenging materials and reveal new defect types in bilayer CrSBr that can be extrapolated to the bulk and to over 20 materials belonging to the same FeOCl structural family. <jats:supplementary-material> <jats:copyright-statement>Published by the American Physical Society</jats:copyright-statement> <jats:copyright-year>2025</jats:copyright-year> </jats:permissions> </jats:supplementary-material>","PeriodicalId":20161,"journal":{"name":"Physical Review X","volume":"5 1","pages":""},"PeriodicalIF":12.5,"publicationDate":"2025-06-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144219268","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
期刊
Physical Review X
全部 Acc. Chem. Res. ACS Applied Bio Materials ACS Appl. Electron. Mater. ACS Appl. Energy Mater. ACS Appl. Mater. Interfaces ACS Appl. Nano Mater. ACS Appl. Polym. Mater. ACS BIOMATER-SCI ENG ACS Catal. ACS Cent. Sci. ACS Chem. Biol. ACS Chemical Health & Safety ACS Chem. Neurosci. ACS Comb. Sci. ACS Earth Space Chem. ACS Energy Lett. ACS Infect. Dis. ACS Macro Lett. ACS Mater. Lett. ACS Med. Chem. Lett. ACS Nano ACS Omega ACS Photonics ACS Sens. ACS Sustainable Chem. Eng. ACS Synth. Biol. Anal. Chem. BIOCHEMISTRY-US Bioconjugate Chem. BIOMACROMOLECULES Chem. Res. Toxicol. Chem. Rev. Chem. Mater. CRYST GROWTH DES ENERG FUEL Environ. Sci. Technol. Environ. Sci. Technol. Lett. Eur. J. Inorg. Chem. IND ENG CHEM RES Inorg. Chem. J. Agric. Food. Chem. J. Chem. Eng. Data J. Chem. Educ. J. Chem. Inf. Model. J. Chem. Theory Comput. J. Med. Chem. J. Nat. Prod. J PROTEOME RES J. Am. Chem. Soc. LANGMUIR MACROMOLECULES Mol. Pharmaceutics Nano Lett. Org. Lett. ORG PROCESS RES DEV ORGANOMETALLICS J. Org. Chem. J. Phys. Chem. J. Phys. Chem. A J. Phys. Chem. B J. Phys. Chem. C J. Phys. Chem. Lett. Analyst Anal. Methods Biomater. Sci. Catal. Sci. Technol. Chem. Commun. Chem. Soc. Rev. CHEM EDUC RES PRACT CRYSTENGCOMM Dalton Trans. Energy Environ. Sci. ENVIRON SCI-NANO ENVIRON SCI-PROC IMP ENVIRON SCI-WAT RES Faraday Discuss. Food Funct. Green Chem. Inorg. Chem. Front. Integr. Biol. J. Anal. At. Spectrom. J. Mater. Chem. A J. Mater. Chem. B J. Mater. Chem. C Lab Chip Mater. Chem. Front. Mater. Horiz. MEDCHEMCOMM Metallomics Mol. Biosyst. Mol. Syst. Des. Eng. Nanoscale Nanoscale Horiz. Nat. Prod. Rep. New J. Chem. Org. Biomol. Chem. Org. Chem. Front. PHOTOCH PHOTOBIO SCI PCCP Polym. Chem.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
0
微信
客服QQ
Book学术公众号 扫码关注我们
反馈
×
意见反馈
请填写您的意见或建议
请填写您的手机或邮箱
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
现在去查看 取消
×
提示
确定
Book学术官方微信
Book学术文献互助
Book学术文献互助群
群 号:604180095
Book学术
文献互助 智能选刊 最新文献 互助须知 联系我们:info@booksci.cn
Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。
Copyright © 2023 Book学术 All rights reserved.
ghs 京公网安备 11010802042870号 京ICP备2023020795号-1