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Entanglement Properties of Gauge Theories from Higher-Form Symmetries 高形式对称规范理论的纠缠性质
IF 12.5 1区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2025-01-02 DOI: 10.1103/physrevx.15.011001
Wen-Tao Xu, Tibor Rakovszky, Michael Knap, Frank Pollmann
We explore the relationship between higher-form symmetries and entanglement properties in lattice gauge theories with discrete gauge groups, which can exhibit both topologically ordered phases and higher-form symmetry-protected topological (SPT) phases. Our study centers on a generalization of the Fradkin-Shenker model describing Z2 lattice gauge theory with matter, where the Gauss law constraint can be either emergent or exact. The phase diagram includes a topologically ordered deconfined phase and a nontrivial SPT phase protected by a 1-form and a 0-form symmetry, among others. We obtain the following key findings: First, the entanglement properties of the model depend on whether the 1-form symmetries and the Gauss law constraint are exact or emergent. For the emergent Gauss law, the entanglement spectrum (ES) of the nontrivial SPT phase exhibits degeneracies, which are robust at low energies against weak perturbations that explicitly break the exact 1-form symmetry. When the Gauss law and the 1-form symmetry are both exact, the ES degeneracy is extensive. This extensive degeneracy turns out to be fragile and can be removed completely by infinitesimal perturbations that explicitly break the exact 1-form symmetry while keeping the Gauss law exact. Second, we consider the ES in the topologically ordered phase where 1-form symmetries are spontaneously broken. In contrast to the ES of the nontrivial SPT phase, we find that spontaneous higher-form symmetry breaking removes “half” of the ES levels, leading to a nondegenerate ES in the topologically ordered phase, in general. Third, we derive a connection between spontaneous higher-form symmetry breaking and the topological entanglement entropy (TEE). Using this relation, we investigate the entanglement entropy that can be distilled in the deconfined phase of the original Fradkin-Shenker model using gauge-invariant measurements. We show that the TEE is robust against the measurement when the 1-form symmetry is emergent but it is fragile when the 1-form symmetry is exact. Our results demonstrate the advantage of higher-form symmetries for understanding entanglement properties of gauge theories. Published by the American Physical Society 2025
本文研究了具有离散规范群的晶格规范理论中高形式对称性与纠缠特性之间的关系,该理论可以同时表现出拓扑有序相和高形式对称保护拓扑相。我们的研究集中在用物质描述Z2晶格规范理论的Fradkin-Shenker模型的推广上,其中高斯定律约束可以是紧急的也可以是精确的。相位图包括一个拓扑有序的定义相位和一个由1形式和0形式对称保护的非平凡SPT相位等。首先,模型的纠缠特性取决于1型对称性和高斯定律约束是精确的还是突现的。对于涌现的高斯定律,非平凡SPT相的纠缠谱(ES)表现出简并,在低能量下对明显打破精确的1-形式对称的弱扰动具有鲁棒性。当高斯定律和1型对称都是精确时,ES简并是广泛的。这种广泛的简并性被证明是脆弱的,可以被无穷小的扰动完全消除,这些扰动明确地打破了精确的1型对称,同时保持了高斯定律的精确性。其次,我们考虑了拓扑有序相中的ES,其中1-form对称性被自发破坏。与非平凡SPT相的ES相比,我们发现自发的高形式对称破缺消除了“一半”的ES能级,导致拓扑有序相中的非简并ES。第三,我们推导了自发高形式对称破缺与拓扑纠缠熵(TEE)之间的联系。利用这一关系,我们研究了可以在原始Fradkin-Shenker模型的定义相位中使用量规不变测量提取的纠缠熵。我们证明了当1-形式对称出现时,TEE对测量具有鲁棒性,但当1-形式对称精确时,TEE是脆弱的。我们的结果证明了高形式对称性在理解规范理论的纠缠特性方面的优势。2025年由美国物理学会出版
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引用次数: 0
Unconventional Coherence Peak in Cuprate Superconductors 铜超导体中的非常规相干峰
IF 12.5 1区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-12-31 DOI: 10.1103/physrevx.14.041072
Zheng Li, Chao Mu, Pengfei Li, Wei Wu, Jiangping Hu, Tao Xiang, Kun Jiang, Jianlin Luo
The Hebel-Slichter coherence peak, observed in the spin-lattice relaxation rate 1</a:mn>/</a:mo>T</a:mi>1</a:mn></a:msub></a:math> just below the critical temperature <c:math xmlns:c="http://www.w3.org/1998/Math/MathML" display="inline"><c:msub><c:mi>T</c:mi><c:mi mathvariant="normal">c</c:mi></c:msub></c:math>, serves as a crucial experimental validation of the Bardeen-Cooper-Schrieffer pairing symmetry in conventional superconductors. However, no coherence peak in <f:math xmlns:f="http://www.w3.org/1998/Math/MathML" display="inline"><f:mn>1</f:mn><f:mo>/</f:mo><f:msub><f:mi>T</f:mi><f:mn>1</f:mn></f:msub></f:math> has been observed in unconventional superconductors like cuprates. In this study, an unconventional coherence peak is identified for the first time using nuclear quadrupole resonance on <h:math xmlns:h="http://www.w3.org/1998/Math/MathML" display="inline"><h:mrow><h:msub><h:mrow><h:mi>YBa</h:mi></h:mrow><h:mrow><h:mn>2</h:mn></h:mrow></h:msub><h:msub><h:mrow><h:mi>Cu</h:mi></h:mrow><h:mrow><h:mn>4</h:mn></h:mrow></h:msub><h:msub><h:mrow><h:mi mathvariant="normal">O</h:mi></h:mrow><h:mrow><h:mn>8</h:mn></h:mrow></h:msub></h:mrow></h:math>, pointing to a distinctive pairing symmetry. The spin-lattice relaxation rate in nuclear quadrupole resonance and nuclear magnetic resonance with nuclear spin <k:math xmlns:k="http://www.w3.org/1998/Math/MathML" display="inline"><k:mi>I</k:mi><k:mo>></k:mo><k:mn>1</k:mn><k:mo>/</k:mo><k:mn>2</k:mn></k:math> comprises the magnetic relaxation rate <m:math xmlns:m="http://www.w3.org/1998/Math/MathML" display="inline"><m:mn>1</m:mn><m:mo>/</m:mo><m:msubsup><m:mi>T</m:mi><m:mn>1</m:mn><m:mi>mag</m:mi></m:msubsup></m:math>, which probes magnetic fluctuations, and the quadrupole relaxation rate <o:math xmlns:o="http://www.w3.org/1998/Math/MathML" display="inline"><o:mn>1</o:mn><o:mo>/</o:mo><o:msubsup><o:mi>T</o:mi><o:mn>1</o:mn><o:mrow><o:mi>quad</o:mi></o:mrow></o:msubsup></o:math>, which probes charge fluctuations. By utilizing <q:math xmlns:q="http://www.w3.org/1998/Math/MathML" display="inline"><q:mrow><q:mmultiscripts><q:mrow><q:mi>Cu</q:mi></q:mrow><q:mprescripts/><q:none/><q:mrow><q:mn>63</q:mn></q:mrow></q:mmultiscripts></q:mrow></q:math> and <s:math xmlns:s="http://www.w3.org/1998/Math/MathML" display="inline"><s:mrow><s:mmultiscripts><s:mrow><s:mi>Cu</s:mi></s:mrow><s:mprescripts/><s:none/><s:mrow><s:mn>65</s:mn></s:mrow></s:mmultiscripts></s:mrow></s:math> isotopes, we successfully distinguish <u:math xmlns:u="http://www.w3.org/1998/Math/MathML" display="inline"><u:mn>1</u:mn><u:mo>/</u:mo><u:msubsup><u:mi>T</u:mi><u:mn>1</u:mn><u:mi>mag</u:mi></u:msubsup></u:math> and <w:math xmlns:w="http://www.w3.org/1998/Math/MathML" display="inline"><w:mn>1</w:mn><w:mo>/</w:mo><w:msubsup><w:mi>T</w:mi><w:mn>1</w:mn><w:mrow><w:mi>quad</w:mi></w:mrow></w:msubsup></w:math> of <y:math xmlns:y="http://www.w3.org/1998/Math/MathML" display="inline"><y:mrow><y:msub><y:mrow><y:mi>YBa</y:mi></y:mrow><y:mrow><y:mn>2
在低于临界温度Tc的自旋-晶格弛豫速率1/T1处观察到Hebel-Slichter相干峰,这是常规超导体中Bardeen-Cooper-Schrieffer配对对称性的重要实验验证。然而,在铜等非常规超导体中,没有观察到1/T1的相干峰。在这项研究中,利用核四极共振首次在YBa2Cu4O8上发现了一个非常规的相干峰,指出了一个独特的配对对称性。核四极共振和核自旋为1 >;1/2的核磁共振中的自旋-晶格弛豫率包括探测磁波动的磁弛豫率1/T1mag和探测电荷波动的四极弛豫率1/T1quad。利用Cu63和Cu65同位素,我们成功地区分了YBa2Cu4O8的1/T1mag和1/T1quad,并发现与传统超导体不同,在1/T1quad中存在相干峰,而在1/T1mag中不存在相干峰。我们的发现表明,当弛豫是由超细场的波动引起时,非常规超导体在1/T1下不会出现相干峰。相反,当电场梯度波动引起弛豫时,由于电荷和磁波动之间的相干因子不同,预计会出现相干峰。我们对YBa2Cu4O8链的1/T1的成功测量表明,如果满足主导四极弛豫的条件,这一现象可以为探索其他超导体中配对机制的非常规性质提供一种新的方法。2024年由美国物理学会出版
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引用次数: 0
Engineering Hierarchical Symmetries 工程层次对称
IF 12.5 1区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-12-27 DOI: 10.1103/physrevx.14.041070
Zhanpeng Fu, Roderich Moessner, Hongzheng Zhao, Marin Bukov
The capacity to custom tailor the properties of quantum matter and materials is a central requirement for enlarging their range of possible functionalities. A particularly promising route is the use of driving protocols to engineer specific desired properties with a high degree of control and flexibility. Here, we present such a program for the tunable generation of sequences of symmetries on controllable timescales. Concretely, our general driving protocol for many-body systems generates a sequence of prethermal regimes, each exhibiting a lower symmetry than the preceding one. We provide an explicit construction of effective Hamiltonians exhibiting these symmetries, which imprints emergent quasiconservation laws hierarchically, enabling us to engineer the respective symmetries and concomitant orders in nonequilibrium matter. We provide explicit examples, including spatiotemporal and topological phenomena, as well as a spin chain realizing the symmetry ladder SU(2)→U(1)→Z2→E. Our results have direct applications in experiments with quantum simulators. Published by the American Physical Society 2024
定制量子物质和材料特性的能力是扩大其可能功能范围的核心要求。一个特别有前途的路线是使用驱动协议来设计具有高度控制和灵活性的特定期望属性。在此,我们提出了一个在可控时间尺度上可调生成对称序列的程序。具体地说,我们对多体系统的一般驱动协议产生一系列的预热状态,每一个都表现出比前一个更低的对称性。我们提供了显示这些对称性的有效哈密顿量的明确构造,它在层次上烙印了涌现的准守恒定律,使我们能够在非平衡物质中设计各自的对称性和伴随的顺序。我们提供了明确的例子,包括时空和拓扑现象,以及实现对称阶梯SU(2)→U(1)→Z2→E的自旋链。我们的结果在量子模拟器的实验中有直接的应用。2024年由美国物理学会出版
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引用次数: 0
Hopping of the Center-of-Mass of Single G Centers in Silicon-on-Insulator 绝缘体上硅单G中心质心的跳变
IF 12.5 1区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-12-27 DOI: 10.1103/physrevx.14.041071
Alrik Durand, Yoann Baron, Péter Udvarhelyi, Félix Cache, Krithika V. R., Tobias Herzig, Mario Khoury, Sébastien Pezzagna, Jan Meijer, Jean-Michel Hartmann, Shay Reboh, Marco Abbarchi, Isabelle Robert-Philip, Adam Gali, Jean-Michel Gérard, Vincent Jacques, Guillaume Cassabois, Anaïs Dréau
Among the wealth of single fluorescent defects recently detected in silicon, the G center catches interest for its telecom single-photon emission that could be coupled to a metastable electron spin triplet. The G center is a unique defect where the standard Born-Oppenheimer approximation used in solid-state physics breaks down as one of its atoms, a silicon atom in interstitial position Si(i), can move between six sites. The impact of its displacement, due either to coherent tunneling or to random jumps from one site to another, on the optical properties of G centers is still largely unknown, especially in silicon-on-insulator (SOI) samples. Here, we investigate the displacement of the center of mass of the G center in silicon. By performing photoluminescence experiments at single-defect scale, we show that individual G defects in SOI exhibit several emission dipoles and zero-phonon line fine structures with splittings up to approximately 1 meV, both indicating a motion of the defect central atom over time. Combining polarization and spectral analysis at the single-photon level, we evidence that the reconfiguration dynamics is drastically different from the one of the unperturbed G center in bulk silicon where the mobile atom is fully delocalized over all six sites through tunneling. The SOI structure freezes the Si(i) delocalization of the G defect and, as a result, enables one to isolate linearly polarized optical lines. Under above-band-gap optical excitation, the central atom of G centers in SOI behaves as if it were in a six-slot roulette wheel, randomly alternating between localized crystal sites at each optical cycle. Comparative measurements in a bulk silicon sample and calculations highlight that strain is likely the dominant perturbation impacting the G center geometry. These results shed light on the importance of the atomic reconfiguration dynamics to understand and control the photoluminescence properties of the G center in silicon. More generally, these findings emphasize the impact of strain fluctuations inherent to SOI wafers for future quantum integrated photonics applications based on color centers in silicon. Published by the American Physical Society 2024
在最近在硅中检测到的大量单荧光缺陷中,G中心因其可与亚稳电子自旋三重态耦合的电信单光子发射而引起了人们的兴趣。G中心是一种独特的缺陷,在固态物理中使用的标准玻恩-奥本海默近似被破坏,因为它的一个原子,一个硅原子在间隙位置Si(i),可以在六个位置之间移动。由于相干隧穿或从一个位置到另一个位置的随机跳跃,其位移对G中心光学性质的影响在很大程度上仍然未知,特别是在绝缘体上硅(SOI)样品中。在这里,我们研究了硅中G中心的质心位移。通过在单缺陷尺度上进行光致发光实验,我们发现SOI中的单个G缺陷表现出几个发射偶极子和零声子线精细结构,分裂高达约1 meV,两者都表明缺陷中心原子随时间的运动。结合单光子水平的偏振和光谱分析,我们证明了重构动力学与块体硅中未受扰动的G中心完全不同,其中移动原子通过隧道在所有六个位置上完全离域。SOI结构冻结了G缺陷的Si(i)离域,从而使人们能够隔离线极化的光学线路。在带隙以上光激发下,SOI中G中心原子的行为就像一个六槽轮盘赌,在每个光循环中随机地在局域晶体位置之间交替。在大量硅样品中的比较测量和计算强调应变可能是影响G中心几何形状的主要扰动。这些结果揭示了原子重构型动力学对于理解和控制硅中G中心的光致发光性质的重要性。更一般地说,这些发现强调了SOI晶圆固有的应变波动对未来基于硅色心的量子集成光子学应用的影响。2024年由美国物理学会出版
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引用次数: 0
Exhaustive Characterization of Quantum Many-Body Scars Using Commutant Algebras 用交换代数穷举表征量子多体伤痕
IF 12.5 1区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-12-26 DOI: 10.1103/physrevx.14.041069
Sanjay Moudgalya, Olexei I. Motrunich
We study quantum many-body scars (QMBS) in the language of commutant algebras, which are defined as symmetry algebras of of local Hamiltonians. This framework explains the origin of dynamically disconnected subspaces seen in models with exact QMBS, i.e., the large “thermal” subspace and the small “nonthermal” subspace, which are attributed to the existence of unconventional nonlocal conserved quantities in the commutant; hence, it unifies the study of conventional symmetries and weak ergodicity-breaking phenomena into a single framework. Furthermore, this language enables us to use the von Neumann double commutant theorem to formally write down the exhaustive algebra of Hamiltonians with a desired set of QMBS, which demonstrates that QMBS survive under large classes of local perturbations. We illustrate this using several standard examples of QMBS, including the spin-1/2 ferromagnetic, AKLT, spin-1 XY π-bimagnon, and the electronic η-pairing towers of states; in each of these cases, we explicitly write down a set of generators for the full algebra of Hamiltonians with these QMBS. Understanding this hidden structure in QMBS Hamiltonians also allows us to recover results of previous “brute-force” numerical searches for such Hamiltonians. In addition, this language clearly demonstrates the equivalence of several unified formalisms for QMBS proposed in the literature and also illustrates the connection between two apparently distinct classes of QMBS Hamiltonians—those that are captured by the so-called Shiraishi-Mori construction and those that lie beyond. Finally, we show that this framework motivates a precise definition for QMBS that automatically implies that they violate the conventional eigenstate thermalization hypothesis, and we discuss its implications to dynamics. Published by the American Physical Society 2024
本文用交换代数的语言研究了量子多体伤痕(QMBS),将其定义为局部哈密顿算子的对称代数。该框架解释了具有精确QMBS模型的动态不连通子空间的起源,即大的“热”子空间和小的“非热”子空间,这归因于交换子中非常规的非局部守恒量的存在;因此,它将传统对称性和弱遍历破缺现象的研究统一到一个单一的框架中。此外,这种语言使我们能够利用von Neumann双交换定理,正式地写出具有期望QMBS集合的哈密顿算子的穷举代数,证明了QMBS在大类别的局部扰动下存活。我们用几个标准的QMBS的例子来说明这一点,包括自旋为1/2的铁磁性,AKLT,自旋为1的XY π-bimagnon,和电子偶态塔;在每一种情况下,我们都明确地写出了一组生成器对于这些QMBS的哈密顿矩阵的完整代数。理解这个隐藏在QMBS哈密顿量中的结构,也使我们能够恢复以前对这种哈密顿量进行“暴力”数值搜索的结果。此外,这种语言清楚地证明了文献中提出的QMBS的几种统一形式的等价性,并说明了两种明显不同的QMBS哈密顿量之间的联系——那些被所谓的白石-森构造捕获的和那些超越的。最后,我们证明了这个框架激发了QMBS的精确定义,自动暗示它们违反传统的特征态热化假设,我们讨论了它对动力学的影响。2024年由美国物理学会出版
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引用次数: 0
Saturation and Recurrence of Quantum Complexity in Random Local Quantum Dynamics 随机局部量子动力学中量子复杂性的饱和与递归
IF 12.5 1区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-12-24 DOI: 10.1103/physrevx.14.041068
Michał Oszmaniec, Marcin Kotowski, Michał Horodecki, Nicholas Hunter-Jones
Quantum complexity is a measure of the minimal number of elementary operations required to approximately prepare a given state or unitary channel. Recently, this concept has found applications beyond quantum computing—in studying the dynamics of quantum many-body systems and the long-time properties of anti–de Sitter black holes. In this context, Brown and Susskind [] conjectured that the complexity of a chaotic quantum system grows linearly in time up to times exponential in the system size, saturating at a maximal value, and remaining maximally complex until undergoing recurrences at doubly exponential times. In this work, we prove the saturation and recurrence of complexity in two models of chaotic time evolutions based on (i) random local quantum circuits and (ii) stochastic local Hamiltonian evolution. Our results advance an understanding of the long-time behavior of chaotic quantum systems and could shed light on the physics of black-hole interiors. From a technical perspective, our results are based on establishing new quantitative connections between the Haar measure and high-degree approximate designs, as well as the fact that random quantum circuits of sufficiently high depth converge to approximate designs. Published by the American Physical Society 2024
量子复杂性是对近似准备给定状态或单一通道所需的最小基本操作数的度量。最近,这一概念在量子计算之外的应用——研究量子多体系统的动力学和反德西特黑洞的长时间特性。在这种情况下,Brown和Susskind[]推测混沌量子系统的复杂性随时间线性增长,直到系统大小的指数倍,在最大值时饱和,并保持最大复杂性,直到经历双指数次的递归。在这项工作中,我们证明了基于(i)随机局部量子电路和(ii)随机局部哈密顿演化的两种混沌时间演化模型的复杂性的饱和和递归。我们的研究结果促进了对混沌量子系统长期行为的理解,并可能揭示黑洞内部的物理学。从技术角度来看,我们的结果是基于在哈尔测量和高度近似设计之间建立新的定量联系,以及足够高深度的随机量子电路收敛到近似设计的事实。2024年由美国物理学会出版
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引用次数: 0
Room-Temperature Solid-State Maser Amplifier 室温固态脉泽放大器
IF 12.5 1区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-12-18 DOI: 10.1103/physrevx.14.041066
Tom Day, Maya Isarov, William J. Pappas, Brett C. Johnson, Hiroshi Abe, Takeshi Ohshima, Dane R. McCamey, Arne Laucht, Jarryd J. Pla
Masers once represented the state of the art in low-noise microwave amplification technology but eventually became obsolete due to their need for cryogenic cooling. Masers based on solid-state spin systems perform most effectively as amplifiers, since they provide a large density of spins and can, therefore, operate at relatively high powers. While solid-state maser oscillators have been demonstrated at room temperature, continuous-wave amplification in these systems has only ever been realized at cryogenic temperatures. Here, we report on a continuous-wave solid-state maser amplifier operating at room temperature. We achieve this feat using a practical setup that includes an ensemble of nitrogen-vacancy center spins in a diamond crystal, a strong permanent magnet, and a simple laser diode. We describe important amplifier characteristics including gain, bandwidth, compression power, and noise temperature and discuss the prospects of realizing a room-temperature near-quantum-noise-limited amplifier with this system. Finally, we show that in a different mode of operation the spins can be used to reduce the microwave noise in an external circuit to cryogenic levels, all without the requirement for physical cooling. Published by the American Physical Society 2024
微波激射器曾经代表了低噪声微波放大技术的最新水平,但最终由于需要低温冷却而过时。基于固态自旋系统的脉泽最有效地作为放大器,因为它们提供大密度的自旋,因此可以在相对高的功率下工作。虽然固态脉泽振荡器已经在室温下被证明,但这些系统中的连续波放大只能在低温下实现。在这里,我们报告了在室温下工作的连续波固态脉泽放大器。我们使用了一个实际的装置来实现这一壮举,该装置包括金刚石晶体中的氮空位中心自旋,一个强大的永磁体和一个简单的激光二极管。我们描述了放大器的重要特性,包括增益、带宽、压缩功率和噪声温度,并讨论了利用该系统实现室温近量子噪声限制放大器的前景。最后,我们证明了在不同的操作模式下,自旋可以用来将外部电路中的微波噪声降低到低温水平,而不需要物理冷却。2024年由美国物理学会出版
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引用次数: 0
Numerical Study of Neutral and Charged Microgel Suspensions: From Single-Particle to Collective Behavior 中性和带电微凝胶悬浮液的数值研究:从单粒子到集体行为
IF 12.5 1区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-12-18 DOI: 10.1103/physrevx.14.041067
Giovanni Del Monte, Emanuela Zaccarelli
We perform extensive molecular dynamics simulations of an ensemble of realistic microgel particles in swollen conditions in a wide range of packing fractions ζ. We compare neutral and charged microgels, where we consider charge distribution adherent to experimental conditions. Through a detailed analysis of single-particle behavior, we are able to identify the different regimes occurring upon increasing concentration: from shrinking to deformation and interpenetration, always connecting our findings with available experimental observations. We then link these single-particle features with the collective behavior of the suspension, finding evidence of a structural reentrance that has no counterpart in the dynamics. Hence, while the maximum of the radial distribution function displays a nonmonotonic behavior with increasing ζ, the dynamics, quantified by the microgels’ mean-squared displacement, always slows down. This behavior, at odds with the simple Hertzian model, can be described by a phenomenological multi-Hertzian model, which takes into account the enhanced internal stiffness of the core. However, also this model fails when deformation enters into play, whereby more realistic many-body models are required. Thanks to our analysis, we are able to unveil the key physical mechanisms, shrinking and deformation, giving rise to the structural reentrance that holds up to very large packing fractions. We further identify key similarities and differences between neutral and charged microgels, for which we detect at high enough ζ the fusion of charged shells, previously invoked to explain key experimental findings, and responsible for the structural reentrance. Overall, our study establishes a powerful framework to uncover the physics of microgel suspensions, paving the way to tackle different regimes, e.g., high temperature, and internal architectures, such as for hollow and ultralow-cross-linked microgels, where experimental evidence is still limited. Published by the American Physical Society 2024
我们执行广泛的分子动力学模拟的现实微凝胶颗粒在膨胀条件下的广泛的包装分数ζ的集合。我们比较中性和带电微凝胶,我们认为电荷分布坚持实验条件。通过对单粒子行为的详细分析,我们能够确定浓度增加时发生的不同机制:从收缩到变形和相互渗透,始终将我们的发现与现有的实验观察联系起来。然后,我们将这些单粒子特征与悬浮液的集体行为联系起来,找到了在动力学中没有对应的结构再入口的证据。因此,尽管径向分布函数的最大值随着ζ的增加呈现出非单调的行为,但由微凝胶的均方位移量化的动力学总是减慢。这种与简单赫兹模型不一致的行为,可以用一个考虑到核心内部刚度增强的多赫兹模型来描述。然而,当变形发生时,这种模型也会失效,因此需要更真实的多体模型。由于我们的分析,我们能够揭示关键的物理机制,收缩和变形,导致结构重新进入,可以容纳非常大的填料分数。我们进一步确定了中性微凝胶和带电微凝胶之间的关键相似性和差异,我们在足够高的ζ处检测到带电壳层的融合,之前被用来解释关键的实验发现,并负责结构再入口。总的来说,我们的研究建立了一个强大的框架来揭示微凝胶悬浮液的物理特性,为解决不同的制度铺平了道路,例如高温,以及内部结构,例如空心和超低交联微凝胶,其中实验证据仍然有限。2024年由美国物理学会出版
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引用次数: 0
Exploring Quantum Materials with Resonant Inelastic X-Ray Scattering 利用共振非弹性 X 射线散射探索量子材料
IF 12.5 1区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-12-13 DOI: 10.1103/physrevx.14.040501
M. Mitrano, S. Johnston, Young-June Kim, M. P. M. Dean
Understanding quantum materials—solids in which interactions among constituent electrons yield a great variety of novel emergent quantum phenomena—is a forefront challenge in modern condensed matter physics. This goal has driven the invention and refinement of several experimental methods, which can spectroscopically determine the elementary excitations and correlation functions that determine material properties. Here we focus on the future experimental and theoretical trends of resonant inelastic x-ray scattering (RIXS), which is a remarkably versatile and rapidly growing technique for probing different charge, lattice, spin, and orbital excitations in quantum materials. We provide a forward-looking introduction to RIXS and outline how this technique is poised to deepen our insight into the nature of quantum materials and of their emergent electronic phenomena. Published by the American Physical Society 2024
理解量子材料--其中各组成电子之间的相互作用产生了大量新出现的量子现象的固体--是现代凝聚态物理学的一项前沿挑战。这一目标推动了多种实验方法的发明和改进,这些方法可以通过光谱测定决定材料特性的基本激发和相关函数。共振非弹性 X 射线散射(RIXS)是一种用途广泛、发展迅速的技术,用于探测量子材料中不同的电荷、晶格、自旋和轨道激发。我们对 RIXS 进行了前瞻性的介绍,并概述了这项技术将如何加深我们对量子材料性质及其新出现的电子现象的洞察。 美国物理学会出版 2024
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引用次数: 0
Magnetoresistance Oscillations in Vertical Junctions of 2D Antiferromagnetic Semiconductor CrPS4 二维反铁磁半导体CrPS4垂直结的磁阻振荡
IF 12.5 1区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-12-13 DOI: 10.1103/physrevx.14.041065
Pengyuan Shi, Xiaoyu Wang, Lihao Zhang, Wenqin Song, Kunlin Yang, Shuxi Wang, Ruisheng Zhang, Liangliang Zhang, Takashi Taniguchi, Kenji Watanabe, Sen Yang, Lei Zhang, Lei Wang, Wu Shi, Jie Pan, Zhe Wang
Magnetoresistance (MR) oscillations serve as a hallmark of intrinsic quantum behavior, traditionally observed only in conducting systems. Here we report the discovery of MR oscillations in an insulating system, the vertical junctions of CrPS4 which is a two-dimensional A-type antiferromagnetic semiconductor. Systematic investigations of MR peaks under varying conditions, including electrode materials, magnetic field direction, temperature, voltage bias, and layer number, elucidate a correlation between MR oscillations and spin-canted states in CrPS4. Experimental data and analysis point out the important role of the in-gap electronic states in generating MR oscillations, and we propose that spin selected interlayer hopping of localized defect states may be responsible for it. Our findings not only illuminate the unusual electronic transport in CrPS4 but also underscore the potential of van der Waals magnets for exploring interesting phenomena. Published by the American Physical Society 2024
磁阻(MR)振荡是本征量子行为的标志,传统上只在导电系统中观察到。在这里,我们报告了在绝缘系统--二维 A 型反铁磁半导体 CrPS4 的垂直结中发现磁阻振荡的情况。在电极材料、磁场方向、温度、电压偏置和层数等不同条件下对磁共振峰值的系统研究,阐明了 CrPS4 中磁共振振荡与自旋倾斜态之间的相关性。实验数据和分析指出了隙内电子态在产生磁共振振荡中的重要作用,并提出局部缺陷态的自旋选择层间跳跃可能是产生磁共振振荡的原因。我们的发现不仅揭示了 CrPS4 中不寻常的电子传输,还强调了范德华磁体在探索有趣现象方面的潜力。 美国物理学会出版 2024
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引用次数: 0
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Physical Review X
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