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Impact of water characteristics on UV disinfection of unfiltered water 水质特性对未过滤水紫外线消毒的影响
IF 2.3 4区 环境科学与生态学 Pub Date : 2022-10-17 DOI: 10.2166/wqrj.2022.006
Mehrnaz Soleimanpour Makuei, Faezeh Ketabchi, Nicolás M. Peleato
The objective of this study was to examine the impact of unfiltered water conditions on UV disinfection. UV biodosimetry tests were conducted over a year using water samples from two treatment plants that apply UV without filtration. The influence of turbidity, absorbance, and zeta potential on UV dose–response curves was analyzed to evaluate relationships between unfiltered water quality and log-inactivation of surrogate organisms. It was observed that diminishing inactivation with increasing UV dose (tailing effect) was governed principally by the surface charge of particulate matter. The increased tailing level observed in raw waters was postulated to be due to having more neutral surface charges, resulting in elevated electrostatic attraction between particles and microorganisms that increased UV resistance. Inactivation at a dose of 35 mJ/cm2 in water samples with low turbidity levels (0.38 NTU) and relatively negative surface charge resulted in 3.0 log-removal in comparison with 2.2 and 2.0 log-removal for samples with turbidity levels of 1.57 and 0.61 NTU, respectively. The results of this study highlight the risks of UV disinfection of unfiltered supplies with respect to the effects of water quality characteristics on UV effectiveness and could be employed to optimize the estimation of UV disinfection potential.
本研究的目的是考察未经过滤的水条件对紫外线消毒的影响。紫外线生物剂量测定试验在一年多的时间里进行,使用的水样来自两个未经过滤的紫外线处理厂。分析了浊度、吸光度和zeta电位对紫外线剂量-响应曲线的影响,以评估未过滤水质与替代生物对数失活之间的关系。观察到,随紫外线剂量增加而减弱的失活(尾效应)主要是由颗粒物的表面电荷决定的。在原水中观察到的尾矿水平增加被认为是由于具有更多的中性表面电荷,导致颗粒和微生物之间的静电吸引力增强,从而增加了抗紫外线能力。在低浊度水平(0.38 NTU)和相对负表面电荷的水样中,35 mJ/cm2剂量的失活导致3.0对数去除,而浊度水平为1.57和0.61 NTU的水样分别为2.2和2.0对数去除。本研究的结果突出了未经过滤的用品在水质特性对紫外线有效性的影响方面的紫外线消毒风险,并可用于优化紫外线消毒潜力的估计。
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引用次数: 0
Comparative photo-degradative treatment of dyeing industry wastewater containing diazo dye by UV/Peroxydate and UV/Persulfate − oxidation processes UV/过氧酸盐和UV/过硫酸盐氧化法对比光降解染料废水
IF 2.3 4区 环境科学与生态学 Pub Date : 2022-09-05 DOI: 10.2166/wqrj.2022.012
Yasmine Laftani, Baylassane Chatib, A. Boussaoud, M. Hachkar, Mohammed El Makhfouk
Generation of anion sulfate radicals (SO4•−) and hydroxyl radicals (HO•) by UV/Persulfate and the UV/Peroxydate processes have been successfully studied to degrade Ponceau S dye. Under [PS] = 0.06 mM; [H2O2] = 2 mM; [S2O82-] = 2 mM, the UV/Persulfate process was effective (kapp = 0.163 min−1) than the UV/Peroxydate process (kapp = 0.054 min−1). The lack of dissolved oxygen, the excess of hydrogen peroxide (H2O2) dosage at 2 mM, and the alkaline pH of 10.01 significantly reduced the UV/Peroxydate efficiency. The scavenging effect of the hydrogenocarbonates and nitrates on the PS dye degradation by the UV/Persulfate process was significant, whereas chlorides had a slight influence. The composition of seawater in chlorides, sulfates, carbonates, and bromides decreased the photoactivity of the studied processes. The presence of phenol showed that the reactive affinity of the (HO•) is more superior to the SO4•−. The UV/Persulfate process achieved 82.35% of chemical oxygen demand removal against 59.56% for the UV/Peroxydate in about 100 min. This study demonstrated that the UV/Persulfate process is a viable option for PS dye degradation. To the best of our knowledge, this is the first report for studying the PS dye degradation under some varying new operational factors. However, the identification of by-products, their nature, and their concentration requires special attention.
研究了紫外/过硫酸盐和紫外/过氧酸两种工艺降解Ponceau S染料时产生的阴离子硫酸盐自由基(SO4•−)和羟基自由基(HO•)。[PS] = 0.06 mM;[H2O2] = 2 mM;[S2O82-] = 2 mM时,UV/过硫酸盐工艺(kapp = 0.163 min−1)比UV/过氧酸盐工艺(kapp = 0.054 min−1)更有效。溶解氧不足、过氧化氢(H2O2)用量过量(2 mM)和碱性pH为10.01显著降低了UV/过氧酸盐的效率。氢化碳酸盐和硝酸盐对紫外光/过硫酸盐法降解PS染料的清除作用显著,而氯化物的影响较小。海水中氯化物、硫酸盐、碳酸盐和溴化物的组成降低了所研究过程的光活性。苯酚的存在表明(HO•)的反应亲和性优于SO4•−。在约100 min的时间内,UV/过硫酸盐法的化学需氧量去除率为82.35%,而UV/过氧酸盐法的化学需氧量去除率为59.56%。研究表明,UV/过硫酸盐法是PS染料降解的可行选择。据我们所知,这是研究PS染料在不同新操作因素下降解的第一份报告。但是,副产物的鉴定、它们的性质和它们的浓度需要特别注意。
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引用次数: 0
Application of machine learning approaches in predicting estuarine dissolved oxygen (DO) under a limited data environment 机器学习方法在有限数据环境下预测河口溶解氧中的应用
IF 2.3 4区 环境科学与生态学 Pub Date : 2022-08-11 DOI: 10.2166/wqrj.2022.002
M. A. Z. Siddik
The application of machine learning (ML) approaches to predict estuarine dissolved oxygen (DO) from a set of environmental covariates including nutrients remains unexplored due to nutrient data unavailability. Employing data from 12 southwest coastal Florida water quality stations, the applicability of four ML models – support vector machine (SVM), random forest (RF), decision tree, and Wang–Mendel – was examined in predicting DO under a limited nutrient data environment. Monthly water temperature, pH, salinity, total nitrogen (TN), and total phosphorus (TP) data were used for model development. The multiple linear regression model was trained as benchmarks to compare the ML model performances. The site-specific RF and SVM showed superior model efficiency (Nash–Sutcliffe Efficiency > 0.80) when all the predictor variables were used for model development. However, models trained without nutrients demonstrated reduced prediction accuracy. Modeling by synthesizing all site data under TN-limited, TP-limited, and TN- & TP-co-limited regimes illustrated a preferable performance of RF. Overall, the study rendered two crucial conclusions that could complement the existing approaches to estimate total daily loads for environmental management: (1) nutrients serve as a necessary predictor of estuarine DO dynamics and (2) RF performs better among the ML methods under a limited data environment.
由于营养数据不可用,机器学习(ML)方法在从一组包括营养素在内的环境协变量预测河口溶解氧(DO)方面的应用尚未探索。利用佛罗里达州西南沿海12个水质站的数据,检验了四个ML模型——支持向量机(SVM)、随机森林(RF)、决策树和王-孟德尔——在有限营养数据环境下预测DO的适用性。月水温、pH、盐度、总氮(TN)和总磷(TP)数据用于模型开发。将多元线性回归模型作为基准进行训练,以比较ML模型的性能。当所有预测变量都用于模型开发时,位点特异性RF和SVM显示出优越的模型效率(Nash–Sutcliffe效率>0.80)。然而,在没有营养素的情况下训练的模型显示预测准确性降低。通过在TN限制、TP限制和TN-&TP共限制条件下合成所有站点数据进行建模,表明RF具有较好的性能。总的来说,该研究得出了两个关键结论,可以补充现有的环境管理总日负荷估计方法:(1)营养物质是河口DO动力学的必要预测因子;(2)在有限的数据环境下,RF在ML方法中表现更好。
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引用次数: 2
Oxygen aeration efficiency of gabion spillway by soft computing models 石笼溢洪道充氧效率的软计算模型
IF 2.3 4区 环境科学与生态学 Pub Date : 2022-08-06 DOI: 10.2166/wqrj.2022.009
Rathod Srinivas, N. K. Tiwari
The current paper deals with the performance evaluation of the application of three soft computing algorithms such as adaptive neuro-fuzzy inference system (ANFIS), backpropagation neural network (BPNN), and deep neural network (DNN) in predicting oxygen aeration efficiency (OAE20) of the gabion spillways. Besides, classical equations, namely multivariate linear and nonlinear regressions (MVLR and MVNLR), including previous studies, were also employed in predicting OAE20 of the gabion spillways. The analysis of results showed that the DNN demonstrated relatively lower error values (root mean square error, RMSE = 0.03465; mean square error, MSE = 0.00121; mean absolute error, MAE = 0.02721) and the highest value of correlation coefficient, CC = 0.9757, performed the best in predicting OAE20 of the gabion spillways; however, other applied models, such as ANFIS, BPNN, MVLR, and MVNLR, were giving comparable results evaluated to statistical appraisal metrics of the relative significance of input parameters based on sensitivity investigation, the porosity (n) of gabion materials was observed to be the most critical parameter, and gabion height (P) had the least impact over OAE20 of the spillways.
本文对自适应神经模糊推理系统(ANFIS)、反向传播神经网络(BPNN)和深度神经网络(DNN)三种软计算算法在石笼溢洪道曝气效率(OAE20)预测中的应用进行了性能评价。此外,包括以往研究在内的经典方程,即多元线性和非线性回归(MVLR和MVNLR),也被用于预测石笼溢洪道的OAE20。结果分析表明,DNN的误差值相对较低(均方根误差,RMSE=0.03465;均方误差,MSE=0.00121;平均绝对误差,MAE=0.02721),相关系数最高值CC=0.757对石笼溢洪道OAE20的预测效果最好;然而,其他应用模型,如ANFIS、BPNN、MVLR和MVNLR,根据敏感性调查,给出了与输入参数相对显著性的统计评估指标相比较的结果,石笼材料的孔隙率(n)是最关键的参数,石笼高度(P)对溢洪道OAE20的影响最小。
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引用次数: 4
Effective phosphate removal from sewage water using zerovalent iron nanomaterial as an adsorbent 零价铁纳米材料吸附剂有效去除污水中的磷酸盐
IF 2.3 4区 环境科学与生态学 Pub Date : 2022-07-30 DOI: 10.2166/wqrj.2022.007
Ipsita Som, Sourav Suman, Mouni Roy, Srimanta Gupta, R. Saha
In recent times, nano zerovalent iron (nZVI) particles have attracted significant attention from researchers for their effectiveness in removing phosphates, a hazardous contaminant, found in groundwater and surface water. nZVI possesses some excellent characteristics such as high reactivity, high surface area, and effective surface-to-volume ratio. In this study, nZVI was characterized by X-ray diffraction, Brunauer–Emmett–Teller (BET) surface area analyzer, Fourier transform infra-red (FT-IR), field emission scanning electron microscopy (FESEM), and transmission electron microscopy (TEM) techniques. The effect of variations in nZVI dosage, pH, ionic strength, and coexisting anions on the removal of phosphate from laboratory-based synthetic water was explored. A maximum phosphate removal efficiency of 96% was achieved at an initial phosphate concentration of 25 mg/L, a nZVI dosage of 560 mg/L, and a shaking rate of 500 rpm, and pH 2 was attained within 120 min. Kinetic and equilibrium studies revealed that the adsorption of phosphate follows a pseudo-2nd-order kinetic model and a Temkin isotherm model, respectively. A thermodynamic study confirmed that phosphate adsorption is a spontaneous and endothermic process. Finally, nZVI was proved to be stable up to five cycles. nZVI was further applied for the removal of phosphate from sewage water, which was collected from Saheb bandh, Purulia district of West Bengal, Eastern India.
近年来,纳米零价铁(nZVI)颗粒因其在去除地下水和地表水中发现的有害污染物磷酸盐方面的有效性而引起了研究人员的极大关注。nZVI具有高反应性、高比表面积和有效表面积比等优良特性。在本研究中,通过X射线衍射、Brunauer–Emmett–Teller(BET)表面积分析仪、傅立叶变换红外光谱(FT-IR)、场发射扫描电子显微镜(FESEM)和透射电子显微镜(TEM)技术对nZVI进行了表征。探讨了nZVI用量、pH、离子强度和共存阴离子的变化对实验室合成水中磷酸盐去除的影响。在初始磷酸盐浓度为25mg/L、nZVI剂量为560mg/L、振荡速率为500rpm、pH值在120min内达到2的条件下,磷酸盐的最大去除效率达到96%。动力学和平衡研究表明,磷酸盐的吸附分别遵循假二阶动力学模型和Temkin等温线模型。热力学研究证实,磷酸盐的吸附是一个自发的吸热过程。最后,nZVI被证明在五个循环内是稳定的。nZVI被进一步应用于从印度东部西孟加拉邦普鲁利亚区的Saheb bandh收集的污水中去除磷酸盐。
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引用次数: 2
Effect of hydrodynamic condition on algae control based on montmorillonite modified lime-ceramic sand-lake sediments 水动力条件对蒙脱土改性石灰-陶瓷沙湖沉积物抑藻效果的影响
IF 2.3 4区 环境科学与生态学 Pub Date : 2022-07-21 DOI: 10.2166/wqrj.2022.008
Ting Xia, Shihong Wang, Hang Yan, Zaizhuang Gao, Yao Qiu, Fang Yuan, Guang-yong Huang, Jun Zhou
Montmorillonite modified lime-ceramic sand-lake sediment (LC-sediments) was synthesized and its algae removal efficiency was investigated in this study. Montmorillonite not only improved the morphology and surface area of original LC-sediments, but also promoted the algal removal rate due to its inherent properties such as accumulating an electric charge, acting as a flocculant, and displaying a local bridging effect. Based on parameter optimization including the ratio of raw materials, agent dosage, initial algae density, pH and, a determination of overlying water, the effect of hydrodynamic conditions on the algal removal process was researched. Under the optimal condition, the removal rates of turbidity, algae density and chlorophyll a could reach 86, 88 and 68%, respectively. As verified with a response surface model, it was shown that low disturbance (stirring) of the algae could promote algal removal by montmorillonite modified LC-sediment. Furthermore, a water column was utilized to approximatively simulate the flocculation and algae control in shallow lakes. This study solved the problem of reducing the dosage of lake sediment and improving the removal efficiency of algae without causing secondary pollution to the environment. It was expected to provide a certain theoretical basis for clay flocculation-based algae control in a real environment.
合成了蒙脱土改性石灰陶瓷砂湖沉积物(lc -沉积物),并对其除藻效果进行了研究。蒙脱土不仅改善了原始lc -沉积物的形态和表面积,而且由于其固有的特性,如积聚电荷、絮凝剂和局部桥接作用,也提高了藻类的去除率。通过对原料配比、药剂用量、初始藻密度、pH、上覆水等参数的优化,研究了水动力条件对除藻过程的影响。在最优条件下,对浊度、藻密度和叶绿素a的去除率分别可达86%、88%和68%。响应面模型验证了低扰动(搅拌)对蒙脱土改性lc -沉积物除藻效果的促进作用。此外,还采用水柱模拟浅水湖泊的絮凝和藻类控制。本研究解决了在不造成环境二次污染的情况下,减少湖泊底泥投加量,提高藻类去除效率的问题。期望为实际环境中基于粘土絮凝剂的藻类控制提供一定的理论依据。
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引用次数: 1
Nitrate removal from groundwater using an activated sludge as a source of bacteria 利用活性污泥作为细菌源从地下水中去除硝酸盐
IF 2.3 4区 环境科学与生态学 Pub Date : 2022-07-08 DOI: 10.2166/wqrj.2022.005
Mohammed Amarine, Sarah Jerroumi, B. Lekhlif, Y. Zouheir, Amine Chafik, El Mostafa Mliji, J. Echaabi
In this study, the denitrification of nitrate-contaminated groundwater by the heterotrophic denitrification (HD) method was studied to produce drinking water. Preliminary tests were carried out in a denitrification reactor, consisting of an opaque PVC column filled with a plastic packing, and fed with a synthetic solution based on glycerol, in which activated sludge bacteria were added. The performance of the reactor was monitored by measuring physicochemical parameters such as pH, turbidity, nitrates, and nitrites. This monitoring was carried out for different tests within the same reactor to evaluate the adaptation possibilities of the denitrifying bacteria. At the end of each test when the substrate was exhausted, a new synthetic solution was added to the reactor under discontinuous aeration (aeration period = 1 h). The results obtained showed that the nitrate removal efficiency reached a value of 99.42% after 8 h of treatment depending on the adaptation of the denitrifying bacteria. This experiment also showed that the concentration of produced nitrite depends on the aeration mode and it reached a value below the detection limit in the sequential aeration mode after 12 h of treatment under discontinuous aeration (aeration period = 1 h).
本研究采用异养反硝化(HD)法对硝酸盐污染地下水进行反硝化,生产饮用水。初步试验是在反硝化反应器中进行的,该反应器由一个充满塑料填料的不透明PVC柱组成,并加入基于甘油的合成溶液,其中添加了活性污泥细菌。通过测量pH值、浊度、硝酸盐和亚硝酸盐等理化参数来监测反应器的性能。对同一反应器内的不同试验进行了监测,以评估反硝化细菌的适应可能性。每次试验结束,底物用完后,在间断曝气(曝气时间= 1 h)的条件下,向反应器中加入新的合成溶液。结果表明,根据反硝化菌的适应情况,处理8 h后硝酸盐去除率可达99.42%。本实验还表明,产亚硝酸盐的浓度与曝气方式有关,在间断曝气(曝气周期= 1 h)处理12 h后,连续曝气方式的产亚硝酸盐浓度达到了低于检出限的值。
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引用次数: 1
Numerical investigation of the multiphase flow patterns and removal effect in a large dissolved air flotation 大型溶气浮选多相流型及去除效果的数值研究
IF 2.3 4区 环境科学与生态学 Pub Date : 2022-06-20 DOI: 10.2166/wqrj.2022.024
J. Tang, Yun Long, Yu Fu, X. Long, Zuti Zhang
The standard k–ε model coupled with the mixture model was used to study two-phase flow in a large dissolved air flotation (DAF) unit. The numerical results can simulate fairly well the velocity vectors and air volume fraction distribution data of a DAF unit from the literature. The typical DAF structure parameters were analyzed in detail to investigate their predicted influences on the internal flow structure and removal effect. The simulations indicated that the short length of the separation zone was not conducive to the formation of a stratified flow pattern, and the turbulent kinetic energy at the bottom of the separation zone increased as the length decreased. With the increase in the height of the DAF tank, the horizontal flow structure in the separation zone would be disrupted and, the distribution range and the intensity of the turbulence kinetic energy increased. Further analysis showed that the formation of horizontal stratified flow facilitated the removal of bubbles, and the formation of stratified flow is related to the size of the DAF unit. Detailed analyses showed that the reduction of DAF height and the increase of separation zone length were beneficial to improve the bubble removal efficiency. Finally, a theoretical analysis was carried out to study the relationship between DAF parameters and the removal effect. The results revealed that when the horizontal flow structure was not destroyed and stratified flow occurred, the bubble removal efficiency was positively linearly related to the length of the separation zone. The removal efficiency increases as DAF height decreases.
采用标准k–ε模型和混合物模型相结合的方法研究了大型溶解空气浮选(DAF)装置中的两相流。数值结果可以很好地模拟文献中DAF单元的速度矢量和空气体积分数分布数据。详细分析了典型的DAF结构参数,研究了它们对内部流动结构和去除效果的预测影响。模拟结果表明,分离区的短长度不利于分层流型的形成,分离区底部的湍流动能随着长度的减小而增加。随着DAF池高度的增加,分离区的水平流动结构将被破坏,湍流动能的分布范围和强度也将增加。进一步分析表明,水平分层流的形成有利于气泡的去除,分层流的产生与DAF单元的大小有关。详细分析表明,降低DAF高度和增加分离区长度有利于提高气泡去除效率。最后,对DAF参数与去除效果的关系进行了理论分析。结果表明,当水平流结构未被破坏而发生分层流时,气泡去除效率与分离区长度呈正线性关系。去除效率随着DAF高度的降低而增加。
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引用次数: 0
Machine learning for water quality classification 水质分类的机器学习
IF 2.3 4区 环境科学与生态学 Pub Date : 2022-05-30 DOI: 10.2166/wqrj.2022.004
Saleh Y. Abuzir, Yousef S. Abuzir
In the past years, there has been a lot of interest in water quality and its prediction as there are many pollutants that affect water quality. The techniques provided herein will help us in controlling and reducing the risks of water pollution. In this study, we will discuss concepts related to machine learning models and their applications for water quality classification (WQC). Three machine learning algorithms, J48, Naive Bayes, and multi-layer perceptron (MLP), were used for WQC prediction. The dataset used contains 10 features, and in order to evaluate the machine's algorithms and their performance, some accuracy measurements were used. Our study showed that the proposed models can accurately classify water quality. By analyzing the results, it was found that the MLP algorithm achieved the highest accuracy for WQC prediction as compared to other algorithms.
在过去的几年里,由于有许多污染物会影响水质,人们对水质及其预测产生了很大的兴趣。本文提供的技术将有助于我们控制和降低水污染的风险。在本研究中,我们将讨论与机器学习模型相关的概念及其在水质分类(WQC)中的应用。将J48、朴素贝叶斯和多层感知器(MLP)三种机器学习算法用于WQC预测。所使用的数据集包含10个特征,为了评估机器的算法及其性能,使用了一些精度测量。我们的研究表明,所提出的模型可以准确地对水质进行分类。通过分析结果发现,与其他算法相比,MLP算法实现了最高的WQC预测精度。
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引用次数: 6
Corrigendum: Water Quality Research Journal 57 (1), 1–19: Methylene blue removal using prepared activated carbon from grape wood wastes: adsorption process analysis and modelling, Seyyed Alireza Mousavi, Davood Shahbazi, Arezoo Mahmoudi and Parastoo Darvishi, doi: 10.2166/wqrj.2021.015 张晓明,张晓明,张晓明,等。活性炭去除葡萄木渣中亚甲基蓝的研究进展[j] .环境科学与技术,2016 (1):1 - 9
IF 2.3 4区 环境科学与生态学 Pub Date : 2022-05-19 DOI: 10.2166/wqrj.2022.001
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引用次数: 0
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Water Quality Research Journal
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