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Efficient Broadband Wavelength Conversion in AlGaAsOI Nonlinear Nanowaveguides Using Low-Power Continuous-Wave Pump
IF 7 1区 物理与天体物理 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-03-04 DOI: 10.1021/acsphotonics.4c02447
Zhengshun Lei, Weiqiang Xie, Wenqi Wei, Zihao Wang, Ting Wang, Chao Xiang, Jianjun Zhang, Yikai Su
Nonlinear wavelength conversion based on four-wave mixing (FWM) is a key function for optical signal processing in photonic integrated systems. Although various integrated waveguide platforms have been proposed for on-chip wavelength converters, it remains a great challenge to realize efficient broadband wavelength conversion using a low-power pump due to the lack of sufficient nonlinear gain in waveguides. To address this challenge, we develop centimeter-scale long, low-loss, spiral nanowaveguides on a highly nonlinear AlGaAs-on-insulator (AlGaAsOI) platform. Through dedicated waveguide dispersion engineering, we demonstrate a broadband wavelength conversion with a 3-dB bandwidth over 130 nm at the telecom bands and a flat conversion efficiency over −10 dB in the whole band, using a single continuous-wave low-power pump of ∼18 dBm. A theoretical analysis not only shows excellent agreement with our experimental results but also reveals a viable route for further performance improvement by reducing the propagation loss and/or tailoring the dimension of waveguides. The demonstrated high-performance wavelength converters provide a practical solution for compact and power-efficient wavelength conversion in optical signal processing. Furthermore, our work highlights the great potential of highly nonlinear AlGaAsOI nanowaveguides in chip-scale χ(3)-based nonlinear applications with ultrahigh performance.
{"title":"Efficient Broadband Wavelength Conversion in AlGaAsOI Nonlinear Nanowaveguides Using Low-Power Continuous-Wave Pump","authors":"Zhengshun Lei, Weiqiang Xie, Wenqi Wei, Zihao Wang, Ting Wang, Chao Xiang, Jianjun Zhang, Yikai Su","doi":"10.1021/acsphotonics.4c02447","DOIUrl":"https://doi.org/10.1021/acsphotonics.4c02447","url":null,"abstract":"Nonlinear wavelength conversion based on four-wave mixing (FWM) is a key function for optical signal processing in photonic integrated systems. Although various integrated waveguide platforms have been proposed for on-chip wavelength converters, it remains a great challenge to realize efficient broadband wavelength conversion using a low-power pump due to the lack of sufficient nonlinear gain in waveguides. To address this challenge, we develop centimeter-scale long, low-loss, spiral nanowaveguides on a highly nonlinear AlGaAs-on-insulator (AlGaAsOI) platform. Through dedicated waveguide dispersion engineering, we demonstrate a broadband wavelength conversion with a 3-dB bandwidth over 130 nm at the telecom bands and a flat conversion efficiency over −10 dB in the whole band, using a single continuous-wave low-power pump of ∼18 dBm. A theoretical analysis not only shows excellent agreement with our experimental results but also reveals a viable route for further performance improvement by reducing the propagation loss and/or tailoring the dimension of waveguides. The demonstrated high-performance wavelength converters provide a practical solution for compact and power-efficient wavelength conversion in optical signal processing. Furthermore, our work highlights the great potential of highly nonlinear AlGaAsOI nanowaveguides in chip-scale <i>χ</i><sup>(3)</sup>-based nonlinear applications with ultrahigh performance.","PeriodicalId":23,"journal":{"name":"ACS Photonics","volume":"32 1","pages":""},"PeriodicalIF":7.0,"publicationDate":"2025-03-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143539230","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Charge State Transition of Spectrally Stabilized Tin-Vacancy Centers in Diamond
IF 7 1区 物理与天体物理 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-03-04 DOI: 10.1021/acsphotonics.4c02490
Keita Ikeda, Yiyang Chen, Peng Wang, Yoshiyuki Miyamoto, Takashi Taniguchi, Shinobu Onoda, Mutsuko Hatano, Takayuki Iwasaki
Solid-state quantum emitters are important platforms for quantum information processing. The fabrication of the emitters with stable photon frequency and narrow line width is a fundamental issue, and it is essential to understand optical conditions under which the emitter keeps a bright charge state or transitions to a dark state. For these purposes, in this study, we investigate the spectral stability and charge state transition of tin-vacancy (SnV) centers in diamond. The photoluminescence excitation spectra of multiple SnV centers are basically stable over time with nearly transform-limited line widths under resonant excitation, while simultaneous irradiation of resonant and nonresonant lasers makes spectra from the SnV centers unstable. We find that the instability occurs due to the charge state transition to a dark state. The charge state transition rates are quantitatively investigated depending on the laser powers. Lastly, with first-principles calculations, we model the charge state transition of the SnV center under laser irradiation.
{"title":"Charge State Transition of Spectrally Stabilized Tin-Vacancy Centers in Diamond","authors":"Keita Ikeda, Yiyang Chen, Peng Wang, Yoshiyuki Miyamoto, Takashi Taniguchi, Shinobu Onoda, Mutsuko Hatano, Takayuki Iwasaki","doi":"10.1021/acsphotonics.4c02490","DOIUrl":"https://doi.org/10.1021/acsphotonics.4c02490","url":null,"abstract":"Solid-state quantum emitters are important platforms for quantum information processing. The fabrication of the emitters with stable photon frequency and narrow line width is a fundamental issue, and it is essential to understand optical conditions under which the emitter keeps a bright charge state or transitions to a dark state. For these purposes, in this study, we investigate the spectral stability and charge state transition of tin-vacancy (SnV) centers in diamond. The photoluminescence excitation spectra of multiple SnV centers are basically stable over time with nearly transform-limited line widths under resonant excitation, while simultaneous irradiation of resonant and nonresonant lasers makes spectra from the SnV centers unstable. We find that the instability occurs due to the charge state transition to a dark state. The charge state transition rates are quantitatively investigated depending on the laser powers. Lastly, with first-principles calculations, we model the charge state transition of the SnV center under laser irradiation.","PeriodicalId":23,"journal":{"name":"ACS Photonics","volume":"130 1","pages":""},"PeriodicalIF":7.0,"publicationDate":"2025-03-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143538995","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Exciton–Polariton Valley Hall Effect in Monolayer Semiconductors on Plasmonic Metasurface
IF 7 1区 物理与天体物理 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-03-04 DOI: 10.1021/acsphotonics.4c01554
Chien-Ju Lee, Hsin-Che Pan, Fatemeh HadavandMirzaee, Li-Syuan Lu, Fei Cheng, Tsing-Hua Her, Chih-Kang Shih, Wen-Hao Chang
Excitons in monolayer transition metal dichalcogenides (TMDs) possess the valley degree of freedom (DOF), which is regarded as a pseudospin (in addition to charge and spin DOF) and can be addressed optically by using polarized light. Incorporating monolayer TMDs into an optical microcavity in the strong coupling regime further enables the formation of valley polaritons that are half-light and half-matter quasiparticles with addressable spin and momentum through the spin–orbit interactions of light, in analogy with the spin-Hall effect in electronic systems. By placing monolayer TMDs on a plasmonic metasurface to enable strong coupling between excitons and surface plasmon polaritons (SPPs), we report here the observation of valley resolved polaritons in momentum space and a large separation in real space. The directional coupling of valley polaritons originated from the intrinsic spin-momentum locking associated with SPPs, resembling a photonic version of the valley Hall effect for polaritons. The spatially routed valley polaritons provide a unique pathway for transporting and detecting the valley DOF through circular polarization of light for valleytronic applications.
{"title":"Exciton–Polariton Valley Hall Effect in Monolayer Semiconductors on Plasmonic Metasurface","authors":"Chien-Ju Lee, Hsin-Che Pan, Fatemeh HadavandMirzaee, Li-Syuan Lu, Fei Cheng, Tsing-Hua Her, Chih-Kang Shih, Wen-Hao Chang","doi":"10.1021/acsphotonics.4c01554","DOIUrl":"https://doi.org/10.1021/acsphotonics.4c01554","url":null,"abstract":"Excitons in monolayer transition metal dichalcogenides (TMDs) possess the valley degree of freedom (DOF), which is regarded as a pseudospin (in addition to charge and spin DOF) and can be addressed optically by using polarized light. Incorporating monolayer TMDs into an optical microcavity in the strong coupling regime further enables the formation of valley polaritons that are half-light and half-matter quasiparticles with addressable spin and momentum through the spin–orbit interactions of light, in analogy with the spin-Hall effect in electronic systems. By placing monolayer TMDs on a plasmonic metasurface to enable strong coupling between excitons and surface plasmon polaritons (SPPs), we report here the observation of valley resolved polaritons in momentum space and a large separation in real space. The directional coupling of valley polaritons originated from the intrinsic spin-momentum locking associated with SPPs, resembling a photonic version of the valley Hall effect for polaritons. The spatially routed valley polaritons provide a unique pathway for transporting and detecting the valley DOF through circular polarization of light for valleytronic applications.","PeriodicalId":23,"journal":{"name":"ACS Photonics","volume":"9 1","pages":""},"PeriodicalIF":7.0,"publicationDate":"2025-03-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143538992","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Inversely Designed Compact 12-Channel Mode Decomposition Spectrometer for On-Chip Photonics
IF 7 1区 物理与天体物理 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-03-03 DOI: 10.1021/acsphotonics.4c02242
Jihoon Choi, Koray Aydin, Young Ki Hong, Heeso Noh
Through inverse design, we present and demonstrate a compact and high-resolution spectrometer for on-chip photonics based on mode decomposition. By employing the effective index method, we significantly reduce the computational resources required for optimization. In 3-dimensional simulations, the decomposition efficiency reaches up to 0.95. The spectrometer operates through mode mixing at varying ratios along wavelengths in the mode mixing region. The spectrum is reconstructed via the inverse calculation of the intensity ratios of the decomposed modes within the structure. Experimental validation is performed by fabricating the designed structure on a silicon-on-insulator platform by using electron beam lithography. The reconstructed spectrum achieves a resolution of 0.1 nm with high accuracy, evidenced by a normalized cross-correlation of 0.99. The entire structure is compact, measuring 10 × 34 μm2. This proposed design is advantageous due to its compactness, reduced computational cost, and straightforward fabrication process.
{"title":"Inversely Designed Compact 12-Channel Mode Decomposition Spectrometer for On-Chip Photonics","authors":"Jihoon Choi, Koray Aydin, Young Ki Hong, Heeso Noh","doi":"10.1021/acsphotonics.4c02242","DOIUrl":"https://doi.org/10.1021/acsphotonics.4c02242","url":null,"abstract":"Through inverse design, we present and demonstrate a compact and high-resolution spectrometer for on-chip photonics based on mode decomposition. By employing the effective index method, we significantly reduce the computational resources required for optimization. In 3-dimensional simulations, the decomposition efficiency reaches up to 0.95. The spectrometer operates through mode mixing at varying ratios along wavelengths in the mode mixing region. The spectrum is reconstructed via the inverse calculation of the intensity ratios of the decomposed modes within the structure. Experimental validation is performed by fabricating the designed structure on a silicon-on-insulator platform by using electron beam lithography. The reconstructed spectrum achieves a resolution of 0.1 nm with high accuracy, evidenced by a normalized cross-correlation of 0.99. The entire structure is compact, measuring 10 × 34 μm<sup>2</sup>. This proposed design is advantageous due to its compactness, reduced computational cost, and straightforward fabrication process.","PeriodicalId":23,"journal":{"name":"ACS Photonics","volume":"24 1","pages":""},"PeriodicalIF":7.0,"publicationDate":"2025-03-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143538996","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Replica-Assisted Super-Resolution Fluorescence Imaging in Scattering Media
IF 6.5 1区 物理与天体物理 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-03-03 DOI: 10.1021/acsphotonics.4c0246810.1021/acsphotonics.4c02468
Tengfei Wu, YoonSeok Baek, Fei Xia, Sylvain Gigan and Hilton B. de Aguiar*, 

Far-field super-resolution fluorescence microscopy has been rapidly developed for applications ranging from cell biology to nanomaterials. However, it remains a significant challenge to achieve super-resolution imaging at depth in opaque materials. In this study, we present a super-resolution microscopy technique for imaging hidden fluorescent objects through scattering media, started by exploiting the inherent object replica generation arising from the memory effect, i.e., the seemingly informationless emission speckle can be regarded as a random superposition of multiple object copies. Inspired by the concept of super-resolution optical fluctuation imaging, we use temporally fluctuating speckles to excite fluorescence signals and perform high-order cumulant analysis on the fluctuation, which can not only improve the image resolution but also increase the speckle contrast to isolate only the bright object replicas. A super-resolved image can be finally retrieved by simply unmixing the sparsely distributed replicas with their location map. This methodology allows one to overcome scattering and achieve robust super-resolution fluorescence imaging, circumventing the need for heavy computational steps.

{"title":"Replica-Assisted Super-Resolution Fluorescence Imaging in Scattering Media","authors":"Tengfei Wu,&nbsp;YoonSeok Baek,&nbsp;Fei Xia,&nbsp;Sylvain Gigan and Hilton B. de Aguiar*,&nbsp;","doi":"10.1021/acsphotonics.4c0246810.1021/acsphotonics.4c02468","DOIUrl":"https://doi.org/10.1021/acsphotonics.4c02468https://doi.org/10.1021/acsphotonics.4c02468","url":null,"abstract":"<p >Far-field super-resolution fluorescence microscopy has been rapidly developed for applications ranging from cell biology to nanomaterials. However, it remains a significant challenge to achieve super-resolution imaging at depth in opaque materials. In this study, we present a super-resolution microscopy technique for imaging hidden fluorescent objects through scattering media, started by exploiting the inherent object replica generation arising from the memory effect, i.e., the seemingly informationless emission speckle can be regarded as a random superposition of multiple object copies. Inspired by the concept of super-resolution optical fluctuation imaging, we use temporally fluctuating speckles to excite fluorescence signals and perform high-order cumulant analysis on the fluctuation, which can not only improve the image resolution but also increase the speckle contrast to isolate only the bright object replicas. A super-resolved image can be finally retrieved by simply unmixing the sparsely distributed replicas with their location map. This methodology allows one to overcome scattering and achieve robust super-resolution fluorescence imaging, circumventing the need for heavy computational steps.</p>","PeriodicalId":23,"journal":{"name":"ACS Photonics","volume":"12 3","pages":"1308–1315 1308–1315"},"PeriodicalIF":6.5,"publicationDate":"2025-03-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143641193","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Replica-Assisted Super-Resolution Fluorescence Imaging in Scattering Media
IF 7 1区 物理与天体物理 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-03-03 DOI: 10.1021/acsphotonics.4c02468
Tengfei Wu, YoonSeok Baek, Fei Xia, Sylvain Gigan, Hilton B de Aguiar
Far-field super-resolution fluorescence microscopy has been rapidly developed for applications ranging from cell biology to nanomaterials. However, it remains a significant challenge to achieve super-resolution imaging at depth in opaque materials. In this study, we present a super-resolution microscopy technique for imaging hidden fluorescent objects through scattering media, started by exploiting the inherent object replica generation arising from the memory effect, i.e., the seemingly informationless emission speckle can be regarded as a random superposition of multiple object copies. Inspired by the concept of super-resolution optical fluctuation imaging, we use temporally fluctuating speckles to excite fluorescence signals and perform high-order cumulant analysis on the fluctuation, which can not only improve the image resolution but also increase the speckle contrast to isolate only the bright object replicas. A super-resolved image can be finally retrieved by simply unmixing the sparsely distributed replicas with their location map. This methodology allows one to overcome scattering and achieve robust super-resolution fluorescence imaging, circumventing the need for heavy computational steps.
{"title":"Replica-Assisted Super-Resolution Fluorescence Imaging in Scattering Media","authors":"Tengfei Wu, YoonSeok Baek, Fei Xia, Sylvain Gigan, Hilton B de Aguiar","doi":"10.1021/acsphotonics.4c02468","DOIUrl":"https://doi.org/10.1021/acsphotonics.4c02468","url":null,"abstract":"Far-field super-resolution fluorescence microscopy has been rapidly developed for applications ranging from cell biology to nanomaterials. However, it remains a significant challenge to achieve super-resolution imaging at depth in opaque materials. In this study, we present a super-resolution microscopy technique for imaging hidden fluorescent objects through scattering media, started by exploiting the inherent object replica generation arising from the memory effect, i.e., the seemingly informationless emission speckle can be regarded as a random superposition of multiple object copies. Inspired by the concept of super-resolution optical fluctuation imaging, we use temporally fluctuating speckles to excite fluorescence signals and perform high-order cumulant analysis on the fluctuation, which can not only improve the image resolution but also increase the speckle contrast to isolate only the bright object replicas. A super-resolved image can be finally retrieved by simply unmixing the sparsely distributed replicas with their location map. This methodology allows one to overcome scattering and achieve robust super-resolution fluorescence imaging, circumventing the need for heavy computational steps.","PeriodicalId":23,"journal":{"name":"ACS Photonics","volume":"10 1","pages":""},"PeriodicalIF":7.0,"publicationDate":"2025-03-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143532713","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Energy-Efficient Ultrashort-Pulse Characterization Using Nanophotonic Parametric Amplification
IF 7 1区 物理与天体物理 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-03-03 DOI: 10.1021/acsphotonics.4c02620
Thomas Zacharias, Robert Gray, Ryoto Sekine, James Williams, Selina Zhou, Alireza Marandi
The growth of ultrafast nanophotonic circuits necessitates the development of energy-efficient on-chip pulse characterization techniques. Nanophotonic realizations of Frequency Resolved Optical Gating (FROG), a common pulse characterization technique in bulk optics, have been challenging due to their noncollinear nature and the lack of efficient nonlinear optical processes in the integrated platform. Here, we experimentally demonstrate a novel FROG-based technique compatible with the nanophotonic platform that leverages the high gain-bandwidth of a dispersion-engineered degenerate optical parametric amplifier (DOPA) for energy-efficient ultrashort pulse characterization. We demonstrate on-chip pulse characterization of sub-80 fs, ∼1 fJ pulses using just ∼60 fJ of gate pulse energy, which is several orders of magnitude lower than the gate pulse energy required for characterizing similar pulses in the bulk counterpart. In the future, we anticipate our work will enable the characterization of ultraweak-ultrashort pulses with energies at the single photon level.
{"title":"Energy-Efficient Ultrashort-Pulse Characterization Using Nanophotonic Parametric Amplification","authors":"Thomas Zacharias, Robert Gray, Ryoto Sekine, James Williams, Selina Zhou, Alireza Marandi","doi":"10.1021/acsphotonics.4c02620","DOIUrl":"https://doi.org/10.1021/acsphotonics.4c02620","url":null,"abstract":"The growth of ultrafast nanophotonic circuits necessitates the development of energy-efficient on-chip pulse characterization techniques. Nanophotonic realizations of Frequency Resolved Optical Gating (FROG), a common pulse characterization technique in bulk optics, have been challenging due to their noncollinear nature and the lack of efficient nonlinear optical processes in the integrated platform. Here, we experimentally demonstrate a novel FROG-based technique compatible with the nanophotonic platform that leverages the high gain-bandwidth of a dispersion-engineered degenerate optical parametric amplifier (DOPA) for energy-efficient ultrashort pulse characterization. We demonstrate on-chip pulse characterization of sub-80 fs, ∼1 fJ pulses using just ∼60 fJ of gate pulse energy, which is several orders of magnitude lower than the gate pulse energy required for characterizing similar pulses in the bulk counterpart. In the future, we anticipate our work will enable the characterization of ultraweak-ultrashort pulses with energies at the single photon level.","PeriodicalId":23,"journal":{"name":"ACS Photonics","volume":"35 1","pages":""},"PeriodicalIF":7.0,"publicationDate":"2025-03-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143539153","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Energy-Efficient Ultrashort-Pulse Characterization Using Nanophotonic Parametric Amplification
IF 6.5 1区 物理与天体物理 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-03-03 DOI: 10.1021/acsphotonics.4c0262010.1021/acsphotonics.4c02620
Thomas Zacharias, Robert Gray, Ryoto Sekine, James Williams, Selina Zhou and Alireza Marandi*, 

The growth of ultrafast nanophotonic circuits necessitates the development of energy-efficient on-chip pulse characterization techniques. Nanophotonic realizations of Frequency Resolved Optical Gating (FROG), a common pulse characterization technique in bulk optics, have been challenging due to their noncollinear nature and the lack of efficient nonlinear optical processes in the integrated platform. Here, we experimentally demonstrate a novel FROG-based technique compatible with the nanophotonic platform that leverages the high gain-bandwidth of a dispersion-engineered degenerate optical parametric amplifier (DOPA) for energy-efficient ultrashort pulse characterization. We demonstrate on-chip pulse characterization of sub-80 fs, ∼1 fJ pulses using just ∼60 fJ of gate pulse energy, which is several orders of magnitude lower than the gate pulse energy required for characterizing similar pulses in the bulk counterpart. In the future, we anticipate our work will enable the characterization of ultraweak-ultrashort pulses with energies at the single photon level.

{"title":"Energy-Efficient Ultrashort-Pulse Characterization Using Nanophotonic Parametric Amplification","authors":"Thomas Zacharias,&nbsp;Robert Gray,&nbsp;Ryoto Sekine,&nbsp;James Williams,&nbsp;Selina Zhou and Alireza Marandi*,&nbsp;","doi":"10.1021/acsphotonics.4c0262010.1021/acsphotonics.4c02620","DOIUrl":"https://doi.org/10.1021/acsphotonics.4c02620https://doi.org/10.1021/acsphotonics.4c02620","url":null,"abstract":"<p >The growth of ultrafast nanophotonic circuits necessitates the development of energy-efficient on-chip pulse characterization techniques. Nanophotonic realizations of Frequency Resolved Optical Gating (FROG), a common pulse characterization technique in bulk optics, have been challenging due to their noncollinear nature and the lack of efficient nonlinear optical processes in the integrated platform. Here, we experimentally demonstrate a novel FROG-based technique compatible with the nanophotonic platform that leverages the high gain-bandwidth of a dispersion-engineered degenerate optical parametric amplifier (DOPA) for energy-efficient ultrashort pulse characterization. We demonstrate on-chip pulse characterization of sub-80 fs, ∼1 fJ pulses using just ∼60 fJ of gate pulse energy, which is several orders of magnitude lower than the gate pulse energy required for characterizing similar pulses in the bulk counterpart. In the future, we anticipate our work will enable the characterization of ultraweak-ultrashort pulses with energies at the single photon level.</p>","PeriodicalId":23,"journal":{"name":"ACS Photonics","volume":"12 3","pages":"1316–1320 1316–1320"},"PeriodicalIF":6.5,"publicationDate":"2025-03-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143641205","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Reconfigurable Ion-Migration Driven Memristor for Multistate Neuromorphic Associative Learning
IF 7 1区 物理与天体物理 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-03-02 DOI: 10.1021/acsphotonics.5c00023
Jiaji Yang, Xin Li, Junzhe Gu, Feilong Yu, Jin Chen, Juntong Liu, Yuxin Song, Xianjie Lin, Xiaoshuang Chen, Wei Lu, Guanhai Li
The development of adaptive, multistate neuromorphic and photonic-memristive devices is essential for advancing intelligent systems capable of complex learning and decision-making. However, conventional devices face limitations in achieving simultaneous, tunable electrical and optical responses required for such biomimetic functions, often necessitating complex circuitry or material-specific modifications that hinder scalability and integration. Here, we present a reconfigurable, ion-migration driven WSe2-based memristor that addresses these challenges by enabling multistate, reversible switching between photoconductive and photovoltaic states. First-principles calculations were employed to investigate the Pd migration mechanism, revealing how controlled Pd ion movement dynamically modulates the device’s band structure and contributes to its multistate functionality. Ultimately, the device achieves notable rectification ratios─up to 3 orders of magnitude─and a photovoltage modulation range of approximately ±0.5 V. These capabilities allow the device to emulate associative learning and multicondition decision-making in response to both external stimuli and internal states, directly supporting neuromorphic applications. These advancements, combined with an integration-friendly fabrication process, underscore the device’s potential for secure communication, adaptive signal processing, and scalable neuromorphic systems.
{"title":"Reconfigurable Ion-Migration Driven Memristor for Multistate Neuromorphic Associative Learning","authors":"Jiaji Yang, Xin Li, Junzhe Gu, Feilong Yu, Jin Chen, Juntong Liu, Yuxin Song, Xianjie Lin, Xiaoshuang Chen, Wei Lu, Guanhai Li","doi":"10.1021/acsphotonics.5c00023","DOIUrl":"https://doi.org/10.1021/acsphotonics.5c00023","url":null,"abstract":"The development of adaptive, multistate neuromorphic and photonic-memristive devices is essential for advancing intelligent systems capable of complex learning and decision-making. However, conventional devices face limitations in achieving simultaneous, tunable electrical and optical responses required for such biomimetic functions, often necessitating complex circuitry or material-specific modifications that hinder scalability and integration. Here, we present a reconfigurable, ion-migration driven WSe<sub>2</sub>-based memristor that addresses these challenges by enabling multistate, reversible switching between photoconductive and photovoltaic states. First-principles calculations were employed to investigate the Pd migration mechanism, revealing how controlled Pd ion movement dynamically modulates the device’s band structure and contributes to its multistate functionality. Ultimately, the device achieves notable rectification ratios─up to 3 orders of magnitude─and a photovoltage modulation range of approximately ±0.5 V. These capabilities allow the device to emulate associative learning and multicondition decision-making in response to both external stimuli and internal states, directly supporting neuromorphic applications. These advancements, combined with an integration-friendly fabrication process, underscore the device’s potential for secure communication, adaptive signal processing, and scalable neuromorphic systems.","PeriodicalId":23,"journal":{"name":"ACS Photonics","volume":"15 1","pages":""},"PeriodicalIF":7.0,"publicationDate":"2025-03-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143532712","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Computed Tomography Using Meta-Optics
IF 6.5 1区 物理与天体物理 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-03-01 DOI: 10.1021/acsphotonics.4c0236210.1021/acsphotonics.4c02362
Maksym V. Zhelyeznyakov, Johannes E. Fröch, Shane Colburn, Steven L. Brunton and Arka Majumdar*, 

Computer vision tasks require processing large amounts of data to perform image classification, segmentation, and feature extraction. Optical preprocessors can potentially reduce the number of floating-point operations required by computer vision tasks, enabling low-power and low-latency operation. However, existing optical preprocessors are mostly learned and hence strongly depend on the training data and thus lack universal applicability. In this paper, we present a meta-optic imager, which implements the Radon transform, obviating the need for training the optics. High-quality image reconstruction with a large compression ratio of 9.2% is presented through the use of the simultaneous algebraic reconstruction technique. We also demonstrate image classification with 90% accuracy on a further compressed (0.6% of total measured pixels) Radon data set through a neural network trained on digitally transformed images. Our work shows the efficacy of data-independent encoding in an optical encoder. While our platform is based on meta-optics, we note that such encoding can be performed with other optics as well.

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ACS Photonics
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