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Solvent-Engineered Strategy Synthesis of Multicolor Fluorescent Carbon Dots for Advanced Solid-State Lighting Applications 溶剂工程策略合成用于先进固态照明应用的多色荧光碳点
IF 7 1区 物理与天体物理 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-11-05 DOI: 10.1021/acsphotonics.4c01188
Qingxin Zeng, Haiyan Qi, Tao Jing, Jun Li, Siqi Shen, Hongxu Zhao, Yang Gao
At present, achieving tunable fluorescent carbon dots (CDs) with narrow full width at half-maximum (FWHM) and high fluorescence quantum yields (QYs) remains a significant challenge. In our study, l-tryptophan and o-phenylenediamine were utilized as precursors, systematically controlling their band gaps and surface states by varying the solvent type. The blue (B-CDs), yellow-green (YG-CDs), and red (R-CDs) fluorescent CDs were successfully prepared, with optimal excitation wavelengths (λex) of 444, 537, and 597 nm, respectively. Especially, these multicolor CDs (M-CDs) exhibited impressive QYs of 53.69, 54.88, and 58.79%, and narrow FWHM of 71, 64, and 34 nm, respectively. Their distinct optical properties were achieved by manipulating the carbonization and dehydration processes through a solvent selection. The variations in optical properties were primarily attributed to increased amino nitrogen content, quantum size, and coordinated effects of surface oxidation states. Furthermore, M-CDs were successfully incorporated into polyvinyl alcohol (PVA) to produce transparent and flexible fluorescent films, demonstrating their excellent and stable optical quality. Finally, the potential of M-CDs in optoelectronic applications was showcased by fabricating bright light-emitting diodes (LEDs).
目前,实现具有窄半最大全宽(FWHM)和高荧光量子产率(QYs)的可调谐荧光碳点(CD)仍然是一项重大挑战。在我们的研究中,利用 l-色氨酸和邻苯二胺作为前驱体,通过改变溶剂类型来系统控制它们的带隙和表面状态。成功制备出了蓝色(B-CDs)、黄绿色(YG-CDs)和红色(R-CDs)荧光光盘,其最佳激发波长(λex)分别为 444、537 和 597 nm。特别是,这些多色光盘(M-CDs)分别表现出令人印象深刻的 53.69%、54.88% 和 58.79% 的 QYs,以及 71、64 和 34 nm 的窄 FWHM。它们独特的光学特性是通过选择溶剂操纵碳化和脱水过程实现的。光学性质的变化主要归因于氨基氮含量的增加、量子尺寸以及表面氧化态的协调效应。此外,还成功地将 M-CD 与聚乙烯醇(PVA)结合,制备出透明柔韧的荧光薄膜,证明了其卓越稳定的光学品质。最后,通过制造明亮的发光二极管(LED),展示了 M-CD 在光电应用方面的潜力。
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引用次数: 0
Reconfigurable Electro-Optic FET Based on Ferroelectric Electrostatic Doping toward Optical Field Programmable Gate Arrays 基于铁电静电掺杂的可重构光电场效应晶体管,面向光场可编程门阵列
IF 7 1区 物理与天体物理 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-11-05 DOI: 10.1021/acsphotonics.4c01260
Yong Zhang, Feng Guo, Zheng-Dong Luo, Ruijuan Tian, Danyang Yao, Xiaoqing Chen, Cizhe Fang, Xuetao Gan, Yan Liu, Yue Hao, Genquan Han
Silicon photonic integrated circuits have been extremely well developed and have gradually moved toward large-scale production. However, the limitations of current scaling have forced researchers to explore new avenues to achieve more compact integration and to develop more cost-effective silicon photonics components. Silicon photonic FPGAs are more area-efficient and flexible compared to traditional on-chip optical circuits due to their reconfigurable nature, which allows for the optimization of silicon photonic devices after fabrication. This feature enables a wide range of applications and performance requirements to be met with a single chip design, thereby reducing costs and enabling the rapid prototyping of new photonic circuits. Here, leveraging ferroelectric-doped graphene into a silicon field programmable gate array, we propose a compact reconfigurable electro-optical device with superior nonvolatility and reconfigurability, broadening the range of applications for programmable silicon photonics. Nonvolatile multilevel memory with electrical write and optical readout is implemented. This innovative memory system supports 10 distinct levels of electro-optical storage, providing enhanced capacity and flexibility. Carrier-enhanced and -depleted modes can be reconfigured by electrical programming on the same optical logic gate. Reconfigurable logic computing in the electronic and optical domain that takes advantage of this feature is demonstrated. Our work provides a compact new approach for programmable electro-optic field programmable gate arrays with low power consumption.
硅光子集成电路已经发展得非常成熟,并逐步走向大规模生产。然而,由于目前规模的限制,研究人员不得不探索新的途径,以实现更紧凑的集成,并开发出更具成本效益的硅光子元件。硅光子 FPGA 与传统的片上光路相比,具有更高的面积效率和灵活性,这得益于其可重新配置的特性,即硅光子器件可以在制造后进行优化。这一特性使得单芯片设计能够满足广泛的应用和性能要求,从而降低成本,实现新光子电路的快速原型开发。在这里,我们利用掺铁石墨烯到硅现场可编程门阵列中,提出了一种紧凑型可重新配置的电子光学器件,它具有卓越的非挥发性和可重新配置性,拓宽了可编程硅光子学的应用范围。我们实现了具有电写入和光读出功能的非易失性多级存储器。这种创新的存储器系统支持 10 个不同级别的电光存储,提供了更大的容量和灵活性。载流子增强模式和载流子耗尽模式可通过同一光学逻辑门上的电子编程进行重新配置。我们展示了利用这一特点在电子和光学领域进行的可重构逻辑计算。我们的工作为低功耗可编程电光场可编程门阵列提供了一种紧凑的新方法。
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引用次数: 0
High-Quality Atom-Manipulation by Pancharatnam–Berry Metasurface for High-Sensitivity Miniaturized Optically Pumped Magnetometers 利用潘查拉特南-浆果金属表面的高质量原子操纵技术实现高灵敏度微型光泵浦磁力计
IF 7 1区 物理与天体物理 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-11-05 DOI: 10.1021/acsphotonics.4c01694
Jin Li, Shuo Sun, Xiaoxun Li, Yaoyao Feng, Yi Zhang, Xiangyu Huang, Pengcheng Du, Jiahao Zhang, Liang Chen, Ángel S. Sanz, Luis L. Sánchez-Soto
Precise atom-manipulation by light plays a pivotal role in optically pumped magnetometers (OPMs), involving the fundamental interaction between light and atoms, as it significantly enhances the sensitivity and stability of magnetic field measurements. However, the available laser beams matched with a vapor of alkali metal atoms (such as rubidium or cesium) cannot simultaneously provide a perfect circularly polarized state and the desired profile (Gaussian beam), which are essential conditions for polarizing alkali metal atoms used in OPMs. Currently, the conventional approaches adopt a complex optical system involving beam shapers (i.e., spatial light modulators), waveplates, and additional functional lenses, which bring limitations of bulkiness, complex adjustments, and high cost in OPMs. Here, we report a new high-quality atom-manipulation approach using an angular-tilted Pancharatnam–Berry (PB) metasurface for high-sensitivity miniaturized OPMs. By precisely engineering the nanostructures of each amorphous silicon meta-atom, the metasurface is capable of efficiently converting incident light at a specific wavelength (770 nm) into a desired circularly polarized state with a predetermined deflection angle. Simultaneously, it has the ability to shape the wavefront to generate an ideal Gaussian profile, accurately achieving atom spin polarization for high-sensitivity miniaturized X-ray-guided OPMs. The deflection angle can efficiently eliminate zero-level noise and achieve full conversion. We experimentally found that the angular-tilted PB metasurface-based OPM with a potassium small vapor cell can implement a sensitivity lower than 400 fT/Hz1/2, which is higher performance than conventional optical methods. This approach provides a new perspective for miniaturized OPMs to precisely measure the magnetic field in various applications.
光对原子的精确操纵在光泵磁强计(OPM)中起着举足轻重的作用,它涉及光与原子之间的基本相互作用,因为它能显著提高磁场测量的灵敏度和稳定性。然而,与碱金属原子(如铷或铯)蒸汽相匹配的现有激光束无法同时提供完美的圆偏振态和所需的轮廓(高斯光束),而这正是使 OPM 中使用的碱金属原子偏振的必要条件。目前,传统方法采用了复杂的光学系统,包括光束整形器(即空间光调制器)、波板和附加功能透镜,这给 OPM 带来了体积庞大、调整复杂和成本高昂等限制。在此,我们报告了一种新的高质量原子操纵方法,该方法采用了角度倾斜的 Pancharatnam-Berry (PB) 元表面,适用于高灵敏度微型化 OPM。通过精确设计每个非晶硅元原子的纳米结构,该元表面能够有效地将特定波长(770 nm)的入射光转换成具有预定偏转角的所需圆偏振态。同时,它还能塑造波阵面,生成理想的高斯轮廓,准确实现原子自旋极化,从而实现高灵敏度的微型 X 射线制导 OPM。偏转角可以有效消除零级噪声,实现完全转换。我们在实验中发现,基于角度倾斜 PB 元表面的 OPM 与钾小蒸气电池可实现低于 400 fT/Hz1/2 的灵敏度,比传统光学方法性能更高。这种方法为微型 OPM 在各种应用中精确测量磁场提供了新的视角。
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引用次数: 0
Reconfigurable Electro-Optic FET Based on Ferroelectric Electrostatic Doping toward Optical Field Programmable Gate Arrays 基于铁电静电掺杂的可重构光电场效应晶体管,面向光场可编程门阵列
IF 6.5 1区 物理与天体物理 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-11-05 DOI: 10.1021/acsphotonics.4c0126010.1021/acsphotonics.4c01260
Yong Zhang, Feng Guo, Zheng-Dong Luo, Ruijuan Tian, Danyang Yao, Xiaoqing Chen, Cizhe Fang, Xuetao Gan*, Yan Liu*, Yue Hao and Genquan Han, 

Silicon photonic integrated circuits have been extremely well developed and have gradually moved toward large-scale production. However, the limitations of current scaling have forced researchers to explore new avenues to achieve more compact integration and to develop more cost-effective silicon photonics components. Silicon photonic FPGAs are more area-efficient and flexible compared to traditional on-chip optical circuits due to their reconfigurable nature, which allows for the optimization of silicon photonic devices after fabrication. This feature enables a wide range of applications and performance requirements to be met with a single chip design, thereby reducing costs and enabling the rapid prototyping of new photonic circuits. Here, leveraging ferroelectric-doped graphene into a silicon field programmable gate array, we propose a compact reconfigurable electro-optical device with superior nonvolatility and reconfigurability, broadening the range of applications for programmable silicon photonics. Nonvolatile multilevel memory with electrical write and optical readout is implemented. This innovative memory system supports 10 distinct levels of electro-optical storage, providing enhanced capacity and flexibility. Carrier-enhanced and -depleted modes can be reconfigured by electrical programming on the same optical logic gate. Reconfigurable logic computing in the electronic and optical domain that takes advantage of this feature is demonstrated. Our work provides a compact new approach for programmable electro-optic field programmable gate arrays with low power consumption.

硅光子集成电路已经发展得非常成熟,并逐步走向大规模生产。然而,由于目前规模的限制,研究人员不得不探索新的途径,以实现更紧凑的集成,并开发出更具成本效益的硅光子元件。硅光子 FPGA 与传统的片上光路相比,具有更高的面积效率和灵活性,这得益于其可重新配置的特性,即硅光子器件可以在制造后进行优化。这一特性使得单芯片设计能够满足广泛的应用和性能要求,从而降低成本,实现新光子电路的快速原型开发。在这里,我们利用掺铁石墨烯到硅现场可编程门阵列中,提出了一种紧凑型可重新配置的电子光学器件,它具有卓越的非挥发性和可重新配置性,拓宽了可编程硅光子学的应用范围。我们实现了具有电写入和光读出功能的非易失性多级存储器。这种创新的存储器系统支持 10 个不同级别的电光存储,提供了更大的容量和灵活性。载流子增强模式和载流子耗尽模式可通过同一光学逻辑门上的电子编程进行重新配置。我们展示了利用这一特点在电子和光学领域进行的可重构逻辑计算。我们的工作为低功耗可编程电光场可编程门阵列提供了一种紧凑的新方法。
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引用次数: 0
Tunable Photoinduced Liquid Crystal Retarders for All-Optical Diffractive Deep Neural Networks 用于全光学衍射深度神经网络的可调光诱导液晶缓速器
IF 7 1区 物理与天体物理 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-11-05 DOI: 10.1021/acsphotonics.4c01284
Quanzhou Long, Lisheng Yao, Junjie Shao, Fion Sze Yan Yeung, Lingxiao Zhou, Wanlong Zhang, Xiaocong Yuan
An all-optical diffractive deep neural network (D2NN) consists of deep-learning-based design of passive diffractive layers and uses light to perform massive computations at the speed of light with zero extra power consumption, exhibiting advantages of large bandwidth, high interconnection, and parallel processing capability. In this paper, we introduce a novel approach utilizing a 5-layer all-optical D2NN constructed with photoinduced liquid crystal (LC) alignment technology to create LC-based tunable phase retarders as artificial neural layers. The D2NN architecture leverages microscale multidomain LC retarders as optical neurons to manipulate the geometric phase of incident light. We systematically simulate pixel-level displacements to enhance alignment tolerance during experiments, achieving robust resilience against misalignment interference with a 2-pixel tolerance in the x and y directions. By actively tuning the LC retarders with external voltage, we optimize the alignment strategy for all network layers, incorporating specially designed concave or convex lenses at each LC retarder for precise alignment in the x, y, and z directions. Through training with a handwritten dataset from MNIST, the D2NN demonstrates a simulated accuracy of 94.17% with a 2 pixel misalignment tolerance. Experimental validation achieves a classification accuracy of 89% with 500 random digits from the test dataset. This research showcases the potential for network miniaturization, integration, and compatibility with visible light, underscoring the practical applicability of an all-optical D2NN for diverse real-world applications.
全光衍射深度神经网络(D2NN)由基于深度学习设计的无源衍射层组成,利用光以光速执行海量计算,零额外功耗,具有大带宽、高互联和并行处理能力等优势。在本文中,我们介绍了一种利用光诱导液晶(LC)配向技术构建 5 层全光 D2NN 的新方法,以创建基于 LC 的可调相位延迟器作为人工神经层。D2NN 架构利用微尺度多域 LC 缓速器作为光学神经元来操纵入射光的几何相位。在实验过程中,我们系统地模拟像素级位移,以提高对准容差,从而在 x 和 y 方向上以 2 个像素的容差实现对错位干扰的稳健恢复。通过利用外部电压主动调整 LC 缓速器,我们优化了所有网络层的对准策略,在每个 LC 缓速器上都加入了专门设计的凹透镜或凸透镜,以实现 x、y 和 z 方向的精确对准。通过使用来自 MNIST 的手写数据集进行训练,D2NN 的模拟准确率达到 94.17%,误差容限为 2 像素。通过从测试数据集中随机抽取 500 个数字进行实验验证,分类准确率达到 89%。这项研究展示了网络微型化、集成化和与可见光兼容的潜力,强调了全光学 D2NN 在现实世界各种应用中的实际适用性。
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引用次数: 0
Tunable Photoinduced Liquid Crystal Retarders for All-Optical Diffractive Deep Neural Networks 用于全光学衍射深度神经网络的可调光诱导液晶缓速器
IF 6.5 1区 物理与天体物理 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-11-05 DOI: 10.1021/acsphotonics.4c0128410.1021/acsphotonics.4c01284
Quanzhou Long, Lisheng Yao, Junjie Shao, Fion Sze Yan Yeung, Lingxiao Zhou, Wanlong Zhang* and Xiaocong Yuan*, 

An all-optical diffractive deep neural network (D2NN) consists of deep-learning-based design of passive diffractive layers and uses light to perform massive computations at the speed of light with zero extra power consumption, exhibiting advantages of large bandwidth, high interconnection, and parallel processing capability. In this paper, we introduce a novel approach utilizing a 5-layer all-optical D2NN constructed with photoinduced liquid crystal (LC) alignment technology to create LC-based tunable phase retarders as artificial neural layers. The D2NN architecture leverages microscale multidomain LC retarders as optical neurons to manipulate the geometric phase of incident light. We systematically simulate pixel-level displacements to enhance alignment tolerance during experiments, achieving robust resilience against misalignment interference with a 2-pixel tolerance in the x and y directions. By actively tuning the LC retarders with external voltage, we optimize the alignment strategy for all network layers, incorporating specially designed concave or convex lenses at each LC retarder for precise alignment in the x, y, and z directions. Through training with a handwritten dataset from MNIST, the D2NN demonstrates a simulated accuracy of 94.17% with a 2 pixel misalignment tolerance. Experimental validation achieves a classification accuracy of 89% with 500 random digits from the test dataset. This research showcases the potential for network miniaturization, integration, and compatibility with visible light, underscoring the practical applicability of an all-optical D2NN for diverse real-world applications.

全光衍射深度神经网络(D2NN)由基于深度学习设计的无源衍射层组成,利用光以光速执行海量计算,零额外功耗,具有大带宽、高互联和并行处理能力等优势。在本文中,我们介绍了一种利用光诱导液晶(LC)配向技术构建 5 层全光 D2NN 的新方法,以创建基于 LC 的可调相位延迟器作为人工神经层。D2NN 架构利用微尺度多域 LC 缓速器作为光学神经元来操纵入射光的几何相位。我们系统地模拟像素级位移,以提高实验过程中的对准容差,从而在 x 和 y 方向上以 2 个像素的容差实现对错位干扰的稳健恢复。通过利用外部电压主动调整 LC 缓速器,我们优化了所有网络层的对准策略,在每个 LC 缓速器上都加入了专门设计的凹透镜或凸透镜,以实现 x、y 和 z 方向的精确对准。通过使用来自 MNIST 的手写数据集进行训练,D2NN 的模拟准确率达到 94.17%,误差容限为 2 像素。通过从测试数据集中随机抽取 500 个数字进行实验验证,分类准确率达到 89%。这项研究展示了网络微型化、集成化和与可见光兼容的潜力,强调了全光学 D2NN 在现实世界各种应用中的实际适用性。
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引用次数: 0
Dual-Wavelength Exciton-Polariton Condensation via Relaxation of Multiple Vibrational Quanta in Organic Microcavities 通过有机微腔中多个振动量子的弛豫实现双波长激子-极化子凝聚
IF 7 1区 物理与天体物理 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-11-04 DOI: 10.1021/acsphotonics.4c01195
Liuqing Yang, Xuekai Ma, Teng Long, Han Huang, Jiahuan Ren, Chunling Gu, Cunbin An, Bo Liao, Hongbing Fu, Qing Liao
The relaxation of organic polaritons is a key aspect for understanding nonequilibrium bosonic condensation in organic microcavities. In this work, dual-branch vibrational quanta-assisted polariton condensation is experimentally observed in organic single-crystal-filled microcavities. By precisely modulating the thickness of the planar optical resonator, we can tune the ground states of two lower polariton branches to perfectly match the energies of two vibrational modes and consequently trigger polariton condensation in both branches. These condensates have nearly identical thresholds. Dynamical analysis indicates that efficient energy relaxation of the photogenerated excitons to the two vibrational modes through the nonradiation of two separately vibrational quanta enables polaritons to populate the ground states of these two lower polariton branches. Our work is evidence of the importance of the vibrational quanta relaxation mechanism for polariton condensation and provides a pathway for multicolor polariton condensation and future laser displays.
有机极化子的弛豫是理解有机微腔中非平衡态玻色子凝聚的一个关键方面。在这项工作中,我们在有机单晶填充微腔中实验观察到了双支振动量子辅助极化子凝聚。通过精确调节平面光学谐振器的厚度,我们可以调整两个较低极化子分支的基态,使其与两个振动模式的能量完全匹配,从而引发两个分支的极化子凝聚。这些凝聚物的阈值几乎完全相同。动力学分析表明,通过两个独立振动量子的非辐射,光生激子有效地能量弛豫到两个振动模式,使极化子能够填充这两个低极化子分支的基态。我们的工作证明了振动量子弛豫机制对极化子凝聚的重要性,并为多色极化子凝聚和未来的激光显示提供了一条途径。
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引用次数: 0
Dual-Wavelength Exciton-Polariton Condensation via Relaxation of Multiple Vibrational Quanta in Organic Microcavities 通过有机微腔中多个振动量子的弛豫实现双波长激子-极化子凝聚
IF 6.5 1区 物理与天体物理 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-11-04 DOI: 10.1021/acsphotonics.4c0119510.1021/acsphotonics.4c01195
Liuqing Yang, Xuekai Ma, Teng Long, Han Huang, Jiahuan Ren, Chunling Gu, Cunbin An, Bo Liao, Hongbing Fu* and Qing Liao*, 

The relaxation of organic polaritons is a key aspect for understanding nonequilibrium bosonic condensation in organic microcavities. In this work, dual-branch vibrational quanta-assisted polariton condensation is experimentally observed in organic single-crystal-filled microcavities. By precisely modulating the thickness of the planar optical resonator, we can tune the ground states of two lower polariton branches to perfectly match the energies of two vibrational modes and consequently trigger polariton condensation in both branches. These condensates have nearly identical thresholds. Dynamical analysis indicates that efficient energy relaxation of the photogenerated excitons to the two vibrational modes through the nonradiation of two separately vibrational quanta enables polaritons to populate the ground states of these two lower polariton branches. Our work is evidence of the importance of the vibrational quanta relaxation mechanism for polariton condensation and provides a pathway for multicolor polariton condensation and future laser displays.

有机极化子的弛豫是理解有机微腔中非平衡态玻色子凝聚的一个关键方面。在这项工作中,我们在有机单晶填充微腔中实验观察到了双支振动量子辅助极化子凝聚。通过精确调节平面光学谐振器的厚度,我们可以调整两个较低极化子分支的基态,使其与两个振动模式的能量完全匹配,从而引发两个分支的极化子凝聚。这些凝聚物的阈值几乎完全相同。动力学分析表明,通过两个独立振动量子的非辐射,光生激子有效地能量弛豫到两个振动模式,使极化子能够填充这两个低极化子分支的基态。我们的工作证明了振动量子弛豫机制对极化子凝聚的重要性,并为多色极化子凝聚和未来的激光显示提供了一条途径。
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引用次数: 0
Probing Spectral-Hole-Burning in Non-Hermitian Scatterings: Differentiating Far-Field Interference and Near-Field Coupling 探测非ermitian散射中的谱孔燃烧:区分远场干扰和近场耦合
IF 7 1区 物理与天体物理 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-11-03 DOI: 10.1021/acsphotonics.4c01085
Wen-jie Zhou, Jingfeng Liu, Renming Liu, Juan-feng Zhu, Dmitrii Gromyko, Cheng-wei Qiu, Lin Wu
Scattering spectra from radiative non-Hermitian systems often exhibit intricate line shapes, where peaks typically garner the most attention for mode identification. However, in multimode systems, the valleys between these peaks may contain valuable information. This “coupling” feature arises from the nonorthogonality of modes in both far and near fields, giving rise to diverse and complex spectra-hole-burning (SHB) patterns. Traditionally, the interpretation of these SHBs has focused on Rabi splitting or Fano resonances, often concentrating solely on either far-field interference or near-field coupling. However, it is essential to recognize that both phenomena coexist in non-Hermitian scatterings. In this study, we develop a quantitative quantum model to probe scattering SHB by simultaneously extracting near-field coupling rates between system quasinormal modes, nonradiative decay rates into a heat reservoir, and radiative decay rates into a vacuum reservoir for far-field interference. We apply our model to illustrate the concept of geometric engineering in tuning the ratio of far-field interference and near-field coupling, exemplified by a silver dimer transitioning from cube-dimer to sphere-dimer or cube-dimer to nanocube-on-mirror configurations. Through this, we establish a universal design guideline for non-Hermitian scattering by creating a two-mode SHB library based on arbitrarily tunable far-field interference and near-field coupling. The developed model serves as a generalized diagnostic tool for probing the SHB mechanisms in all types of non-Hermitian scattering problems, promising to advance our understanding of intricate phenomena and facilitate the design of tailored optical devices with enhanced performance and functionality.
辐射非ermitian 系统的散射光谱通常呈现出错综复杂的线形,其中峰值通常是模式识别中最受关注的部分。然而,在多模系统中,这些峰值之间的谷值可能包含有价值的信息。这种 "耦合 "特征源于远场和近场模式的非正交性,从而产生了多样而复杂的谱孔燃烧(SHB)模式。传统上,对这些 SHB 的解释主要集中在拉比分裂或法诺共振上,通常只关注远场干扰或近场耦合。然而,必须认识到这两种现象在非赫米散射中同时存在。在本研究中,我们建立了一个定量量子模型,通过同时提取系统准正常模式之间的近场耦合率、进入热库的非辐射衰减率以及进入远场干涉真空库的辐射衰减率,来探测散射 SHB。我们应用我们的模型来说明几何工程学在调整远场干涉和近场耦合比率方面的概念,以银二聚体从立方二聚体过渡到球形二聚体或立方二聚体过渡到镜面纳米立方体配置为例。通过这种方法,我们建立了一个基于任意可调远场干涉和近场耦合的双模 SHB 库,从而为非赫米散射建立了通用的设计准则。所开发的模型可作为通用诊断工具,用于探测所有类型非赫米散射问题中的 SHB 机制,有望推动我们对复杂现象的理解,并促进具有更高性能和功能的定制光学器件的设计。
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引用次数: 0
Probing Spectral-Hole-Burning in Non-Hermitian Scatterings: Differentiating Far-Field Interference and Near-Field Coupling 探测非ermitian散射中的谱孔燃烧:区分远场干扰和近场耦合
IF 6.5 1区 物理与天体物理 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-11-03 DOI: 10.1021/acsphotonics.4c0108510.1021/acsphotonics.4c01085
Wen-jie Zhou, Jingfeng Liu, Renming Liu, Juan-feng Zhu, Dmitrii Gromyko, Cheng-wei Qiu* and Lin Wu*, 

Scattering spectra from radiative non-Hermitian systems often exhibit intricate line shapes, where peaks typically garner the most attention for mode identification. However, in multimode systems, the valleys between these peaks may contain valuable information. This “coupling” feature arises from the nonorthogonality of modes in both far and near fields, giving rise to diverse and complex spectra-hole-burning (SHB) patterns. Traditionally, the interpretation of these SHBs has focused on Rabi splitting or Fano resonances, often concentrating solely on either far-field interference or near-field coupling. However, it is essential to recognize that both phenomena coexist in non-Hermitian scatterings. In this study, we develop a quantitative quantum model to probe scattering SHB by simultaneously extracting near-field coupling rates between system quasinormal modes, nonradiative decay rates into a heat reservoir, and radiative decay rates into a vacuum reservoir for far-field interference. We apply our model to illustrate the concept of geometric engineering in tuning the ratio of far-field interference and near-field coupling, exemplified by a silver dimer transitioning from cube-dimer to sphere-dimer or cube-dimer to nanocube-on-mirror configurations. Through this, we establish a universal design guideline for non-Hermitian scattering by creating a two-mode SHB library based on arbitrarily tunable far-field interference and near-field coupling. The developed model serves as a generalized diagnostic tool for probing the SHB mechanisms in all types of non-Hermitian scattering problems, promising to advance our understanding of intricate phenomena and facilitate the design of tailored optical devices with enhanced performance and functionality.

辐射非ermitian 系统的散射光谱通常呈现出错综复杂的线形,其中峰值通常是模式识别中最受关注的部分。然而,在多模系统中,这些峰值之间的谷值可能包含有价值的信息。这种 "耦合 "特征源于远场和近场模式的非正交性,从而产生了多样而复杂的谱孔燃烧(SHB)模式。传统上,对这些 SHB 的解释主要集中在拉比分裂或法诺共振上,通常只关注远场干扰或近场耦合。然而,必须认识到这两种现象在非赫米散射中同时存在。在本研究中,我们建立了一个定量量子模型,通过同时提取系统准正常模式之间的近场耦合率、进入热库的非辐射衰减率以及进入远场干涉真空库的辐射衰减率,来探测散射 SHB。我们应用我们的模型来说明几何工程学在调整远场干涉和近场耦合比率方面的概念,以银二聚体从立方二聚体过渡到球形二聚体或立方二聚体过渡到镜面纳米立方体配置为例。通过这种方法,我们建立了一个基于任意可调远场干涉和近场耦合的双模 SHB 库,从而为非赫米提散射建立了通用的设计准则。所开发的模型可作为通用诊断工具,用于探测所有类型非赫米散射问题中的 SHB 机制,有望推动我们对复杂现象的理解,并促进具有更高性能和功能的定制光学器件的设计。
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ACS Photonics
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