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Recent developments in the modeling of (n,γ) reactions with FIFRELIN 用FIFRELIN模拟(n,γ)反应的最新进展
Pub Date : 2022-10-17 DOI: 10.12681/hnps.3606
A. Chalil, T. Materna, O. Litaize, A. Chebboubi
Nowadays, the accuracy of experimental results relies more and more on detailed simulations. In the STEREO experiment, the interaction of neutrinos in the liquid scintillator is signed by a n-capture on a Gd atom. The FIFRELIN predictions of the Gd γ-cascades were shown to significantly improve the Data/MC agreement. In the CRAB method, lately proposed to calibrate cryogenic particle detectors at low energy (100 eV), the FIFRELIN cascades of the W and Ge isotopes played a central role in the feasibility study of the method. The FIFRELIN code employs a Monte Carlo Hauser-Feshbach framework based on Bečvár’s algorithm. A sample of nuclear level schemes is generated for a specific isotope of interest, taking into account the uncertainties from nuclear structure. In this work, new improvements on the FIRELIN de-excitation process are reported. Angular correlations of γ-rays in the de-excitation process have been implemented in order to provide a more accurate description of the γ-ray cascades. The anisotropy of the γ-rays with respect to the axis of a previously emitted γ-ray is modeled using the angular correlation formalism, which requires input of the spins and multipolarities of the states involved in the FIFRELIN cascade. Furthermore, the simulation of primary γ-rays emitted from (n,γ) reactions has been updated using the EGAF database.
目前,实验结果的准确性越来越依赖于详细的模拟。在STEREO实验中,液体闪烁体中中微子的相互作用以Gd原子上的n捕获为标志。Gd γ-级联的FIFRELIN预测结果显著提高了数据/MC一致性。在最近提出的用于校准低能量(100 eV)低温粒子探测器的CRAB方法中,W和Ge同位素的FIFRELIN级联在该方法的可行性研究中发挥了核心作用。FIFRELIN代码采用了基于Bečvár算法的蒙特卡罗Hauser-Feshbach框架。考虑到核结构的不确定性,为感兴趣的特定同位素生成了核能级方案样本。在这项工作中,报告了对FIRELIN去激励过程的新改进。为了更准确地描述γ射线级联,在退激发过程中实现了γ射线的角相关性。γ射线相对于先前发射的γ射线轴的各向异性使用角相关形式化建模,这需要输入FIFRELIN级联中涉及的自旋和多极态。此外,使用EGAF数据库更新了(n,γ)反应发射的初级γ射线的模拟。
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引用次数: 0
A Technique for Metallic Waste Characterization and Segregation in Management Routes 金属废弃物表征与管理路线分离技术研究
Pub Date : 2022-10-17 DOI: 10.12681/hnps.3564
D. Mavrikis, A. Markopoulos, Elena Dalla, A. Ioannidou, A. Savidou
Adequate radiological characterization is important for optimization of metallic waste management. For decommissioning planning, the objective is to obtain a radiological understanding of the involved installation. The characterization at this stage could be carried out by means of: 1) neutron activation calculations based on reactor design and neutron flux; 2) dose rate measurements; 3) in-situ gamma spectrometry; 4) sampling for determination of the scaling factors in activated and contaminated components. During dismantling, in-situ characterization is carried out to classify and package the generated waste. Then, the packages are monitored for assessment of activity and determination of the management route.  The selection of cutting and decontamination techniques should be based on accurate determination of the radionuclides inside the material and/ or on the surface contamination. . It is important to decide in which cases the decontamination will be efficient as well as to select the appropriate decontamination techniques based on whether the waste is slightly activated or contaminated or both. Α Semi-empirical technique for optimization of determination of contamination and activation of components and metallic waste is under development based on combination of gamma spectrometry measurements and MCNPX Monte Carlo simulations. Firstly, the technique aims at reduction of the uncertainties related to the density and activity distribution. The specific activities inside and on the surface of the materials could be determined by using the measurement results of the proposed non-destructive technique in combination with the use of the scaling factors for activation and/ or contamination.
充分的放射学表征对金属废物管理的优化是重要的。对于退役计划,目标是获得有关装置的放射学知识。这一阶段的表征可以通过以下方法进行:1)基于反应堆设计和中子通量的中子活化计算;2)剂量率测量;3)原位伽马能谱法;4)取样测定活化组分和污染组分的标度因子。在拆卸过程中,进行现场表征,对产生的废物进行分类和包装。然后,对这些包进行监控,以评估活动并确定管理路线。切割和去污技术的选择应以准确测定材料内部和/或表面污染的放射性核素为基础。重要的是要决定在哪些情况下去污是有效的,并根据废物是轻微活化还是受到污染,或两者兼而有之,选择适当的去污技术。Α基于伽马能谱测量和MCNPX蒙特卡罗模拟的结合,正在开发用于优化测定成分和金属废物的污染和活化的半经验技术。首先,该技术旨在减少与密度和活度分布相关的不确定性。材料内部和表面的特定活性可以通过使用所提出的非破坏性技术的测量结果,结合使用活化和/或污染的比例因子来确定。
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引用次数: 0
Simulation of a MicroMegas detector for low-energy α-particle tracking using Garfield++ garfield++对MicroMegas低能α粒子跟踪的仿真研究
Pub Date : 2022-10-17 DOI: 10.12681/hnps.3715
M. Davis, M. Diakaki, M. Kokkoris, V. Michalopoulou-Petropoulou, R. Vlastou
In the present work, the simulated detector was a MicroMegas gaseous one, regularly being used for neutron-induced fission studies at NCSR ‘Demokritos’. The initial code tests involved the linear response of the detector with respect to the energy deposition of 5 MeV α-particles. This study was carried out in two distinct steps: First, by collecting simulated data for the deposited charge in the anode electrode for different particle trajectories, as well as, for the same trajectory, but for different gas pressures, ranging between 0.8 and 1.2 atm and then by comparing them with the corresponding results obtained using SRIM2008 regarding the α-particle energy losses inside the detector, with the same set of parameters. Finally, a simulated spectrum of 5 MeV α-particles, having trajectories randomly distributed within the whole detector volume, was obtained using Garfield++ and was compared to an experimental one. The similarities and discrepancies observed are discussed and analyzed.
在目前的工作中,模拟的探测器是MicroMegas气体探测器,经常用于NCSR ' Demokritos '的中子诱导裂变研究。最初的代码测试涉及探测器对5 MeV α-粒子能量沉积的线性响应。本研究分为两个不同的步骤:首先,收集不同粒子轨迹下阳极电极沉积电荷的模拟数据,以及相同轨迹下不同气压(0.8 ~ 1.2 atm)下沉积电荷的模拟数据,然后将其与SRIM2008在相同参数下得到的探测器内部α-粒子能量损失的模拟结果进行比较。最后,利用Garfield++模拟得到了5 MeV α-粒子在整个探测器体积内轨迹随机分布的谱图,并与实验谱图进行了比较。对所观察到的异同进行了讨论和分析。
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引用次数: 0
Dose rate assessment of 137Cs to mussels and pelagic fish from the combined use of field measurements, satellite data and the ERICA Assessment Tool 综合利用实地测量、卫星数据和ERICA评估工具评估137Cs对贻贝和远洋鱼类的剂量率
Pub Date : 2022-10-17 DOI: 10.12681/hnps.3575
G. Mavrokefalou, M. Sotiropoulou
Cesium-137 (137Cs) is the most important indicator of radioactive pollution in the marine environment due to its half-life (Tph: 30.2 years), its high fission yield, its solubility (70% in ionic form) and its bioavailability (similar to potassium). Soluble radionuclides, like 137Cs, in the seawater are associated with physicogeochemical and biological parameters of the marine environment (e.g. temperature, water density, biota exchange processes, water mass translocation etc.). Considering this characteristic, we investigate the potential relation between 137Cs activity concentration and sea surface temperature (SST). The parameter of SST is selected, as the element of cesium in the seawater is conservative and its horizontal and vertical dispersion depends on the water mass translocation and water currents. Water mass translocation and water currents are processes that are both governed by the SST. SST also influences the uptake of 137Cs in some marine organisms as it makes it more bioavailable and affects the biological retention time and the elimination rate. The study area is the Gulf of Corinth (Greece). Cs-137 in the Gulf of Corinth originates from water runnoff from the land (Chernobyl fallout from 1986) and a small influence exists from the Ionian and Aegean Sea water currents. A total of 17 measurements spanning 2004-2005, of 137Cs activity concentrations were retrieved from the Environmental Radioactivity Laboratory (ERL) database of NCSR “D”. Furthermore, SST measurements issued from NASA’s Moderate Resolution Imaging Spectroradiometer (MODIS). Databases of 137Cs activity concentrations and SST are used for regression analysis and definition of a linear model. The estimated 137Cs activity concentrations obtained by the model are then compared with the newest measured values obtained by seawater samples from September and November 2018 (a total of 8 seawater samples). Estimated concentrations present a relative difference of about 9% to the measured values. In order to conduct the risk assessment analysis in the studied area, the dose rates are calculated for marine organisms. The selected marine organisms are mussels and pelagic fish that are abundant in the area and have significant commercial value, with mussels also being an important bioindicator of marine pollution. The total dose rates in these organisms (resulting by both the internal and external exposure) vary from 3.30 × 101 to 5.40 × 101 μGy/year for the mussels and from 2.97 × 10-1 to 4.86 × 10-1 μGy/year for pelagic fish, which are much lower that the intervention levels, indicating low impact due to the 137Cs exposure.
铯-137 (137Cs)是海洋环境中最重要的放射性污染指标,因为它的半衰期(Tph: 30.2年)、高裂变产率、溶解度(70%以离子形式存在)和生物利用度(类似于钾)。海水中的可溶性放射性核素,如137Cs,与海洋环境的物理地球化学和生物参数(如温度、水密度、生物群交换过程、水质量转运等)有关。考虑到这一特点,我们研究了137Cs活度浓度与海温(SST)的潜在关系。选取海表温度参数,是因为海水中的铯元素较为保守,其水平和垂直弥散取决于水体转位和水流。水团移位和水流都是受海温控制的过程。海温还影响一些海洋生物对137Cs的吸收,因为它使其更具生物可利用性,并影响其生物滞留时间和消除率。研究区域为科林斯湾(希腊)。科林斯湾的铯-137来自陆地的径流(1986年切尔诺贝利的放射性尘埃),爱奥尼亚和爱琴海的水流也有很小的影响。从NCSR“D”环境放射性实验室(ERL)数据库中检索了2004-2005年期间共17次测量的137Cs活性浓度。此外,海温的测量数据来自NASA的中分辨率成像光谱仪(MODIS)。利用137Cs活性浓度和海表温度数据库进行回归分析和线性模型的定义。然后将该模型获得的137Cs活度浓度估计值与2018年9月和11月(共8个海水样本)海水样品获得的最新测量值进行比较。估计浓度与实测值的相对差异约为9%。为了在研究区域进行风险评估分析,计算了海洋生物的剂量率。选择的海洋生物是贻贝和远洋鱼类,这些生物在该地区数量丰富,具有重要的商业价值,贻贝也是海洋污染的重要生物指标。这些生物的总剂量率(由内照射和外照射引起的)在3.30 × 101 ~ 5.40 × 101 μGy/年之间变化,贻贝和中上层鱼类的总剂量率在2.97 × 10-1 ~ 4.86 × 10-1 μGy/年之间,远低于干预水平,表明137Cs暴露的影响较小。
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引用次数: 0
Empirical Description of Isotope Production in 0.01-2.5GeV p+natFe Reactions 0.01 ~ 2.5 gev p+natFe反应同位素生成的经验描述
Pub Date : 2022-10-17 DOI: 10.12681/hnps.3620
Kostantinos Korakas, Athanasia Miliadou, Theodora-Ilektra Katsigianni, Diamantis Tasioudis, N. Nicolis
Experimental excitation functions of isotopes produced in  reactions are compared with the results of empirical cross section formulas. We consider excitation functions of 16 isotopes (36Cl, 38Ar, 42,43K, 44Ti, 46,47,48Sc, 48,51Cr, 52Fe, 52,54Mn and 55,56,57Co) produced in  reactions at bombarding energies from threshold up to 2.6 GeV. They are compared with the predictions of the empirical formulas of Rudstam, Silberberg-Tsao and SPACS. In the middle-energy range, the formulas provide (in the stated order) a progressively improved description of the experimental excitation functions of the dominant isotopes. At the highest energies, the limiting values of the dominant excitation functions are well described by the EPAX formula (Version 2.1). The predictive power of these formulas could be questioned at low energies close to the threshold, reaction products with a mass much smaller than the target and possibly low cross section channels.
对反应产生的同位素的实验激发函数与经验截面公式的结果进行了比较。我们考虑了16种同位素(36Cl, 38Ar, 42,43k, 44Ti, 46,47,48sc, 48,51cr, 52Fe, 52,54mn和55,56,57co)在轰击能阈值高达2.6 GeV的反应中产生的激发函数。并与Rudstam、Silberberg-Tsao和SPACS经验公式的预测结果进行了比较。在中能量范围内,这些公式(按规定的顺序)提供了对主要同位素的实验激发函数的逐步改进的描述。在最高能量处,主导激发函数的极限值由EPAX公式(版本2.1)很好地描述。这些公式的预测能力在接近阈值的低能量、质量远小于目标的反应产物和可能的低截面通道时受到质疑。
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引用次数: 0
Comparison of Real and Generated by MCNP Simulation Spectrums for Validation of Neutron Activation Calculations 验证中子活化计算的MCNP仿真谱与真实谱的比较
Pub Date : 2022-10-17 DOI: 10.12681/hnps.3565
A. Markopoulos, D. Mavrikis, E. Ntalla, A. Ioannidou, A. Savidou
The objective for decommissioning planning, is to obtain a radiological understanding of the involved installation. The characterization at this stage could be carried out by means of: (a) neutron activation calculations based on reactor design and neutron flux; (b) dose rate measurements; (c) in-situ gamma spectrometry; (d) sampling for determination of the scaling factors in activated and contaminated components.Neutron activation calculations contains several uncertainties. These uncertainties are based on the input data - such as material data (composition and impurities), neutron flux and energy, nuclear data libraries - and on the methodology of the process and the simulation codes.Taking into consideration all these modeling uncertainties, this work is focused on the development of a technique for validation of the calculations. A non-destructive gamma spectrometry technique by using MCNP6 simulations is under development for interpretation of the resulting gamma-ray spectra of the radionuclides in activated components. In particular, a spectrum will be produced, based on the activities of the main radionuclides in the activated component and the results of MCNP6 simulations. This spectrum will be compared with the experimental spectrum.Furthermore, the radiological characterization of activated components, which appeared with surface contamination, is essential for the decision making process during decommissioning. The cutting techniques to be followed in order to reduce the production of secondary waste and limit the doses to personnel and the selection of decontamination techniques should be based on accurate determination of the radionuclides inside the material and/ or in the surface contamination. The proposed method could also be helpful in this case. The activities inside and on the surface of the components could be determined by comparing the experimental spectrum with that produced by MCNP6 simulations, using the arisen activities from the scaling factors and the dose rate measurements.
退役计划的目标是获得有关装置的放射学知识。这一阶段的表征可以通过以下方法进行:(a)基于反应堆设计和中子通量的中子活化计算;(b)剂量率测量;(c)原位伽马能谱法;(d)取样以确定活化和污染组分中的比例因子。中子活化计算包含几个不确定因素。这些不确定性基于输入数据——例如材料数据(成分和杂质)、中子通量和能量、核数据库——以及过程的方法和模拟代码。考虑到所有这些建模的不确定性,本工作的重点是开发一种验证计算的技术。目前正在开发一种利用MCNP6模拟的非破坏性伽马能谱技术,用于解释活性组分中放射性核素的伽马能谱。特别是,将根据活化组分中主要放射性核素的活性和MCNP6模拟的结果产生一个光谱。该光谱将与实验光谱进行比较。此外,在退役决策过程中,活性组分的放射学表征对表面污染至关重要。为减少二次废物的产生和限制对人员的剂量而采用的切割技术和选择除污技术应以准确确定材料内部和/或表面污染中的放射性核素为基础。所提出的方法在这种情况下也可能有所帮助。利用比例因子和剂量率测量产生的活性,将实验谱与MCNP6模拟产生的活性进行比较,可以确定组分内部和表面的活性。
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引用次数: 0
Cross Section Measurements of (n,x) Reactions at 17.9 MeV Using Highly Enriched Ge Isotopes 用高富集Ge同位素测量17.9 MeV下(n,x)反应的截面
Pub Date : 2022-10-17 DOI: 10.12681/hnps.3621
S. Chasapoglou, M. Axiotis, G. Gkatis, S. Harissopulos, M. Kokkoris, A. Lagoyannis, C. Lederer-Woods, V. Michalopoulou, M. Savva, I. Stamatelatos, A. Stamatopoulos, T. Vasilopoulou, R. Vlastou
Τhe 70Ge(n,2n)69Ge, 72Ge(n,a)69mZn, 72Ge(n,p)72Ga and 73Ge(n,p)73Ga reactions have been measured by means of the activation technique at neutron energy 17.9 MeV. The quasimonoenergetic neutron beam was produced via the 2H(d,n)3He reaction at the 5.5 MV Tandem Van de Graaff accelerator of NCSR “Demokritos.” Isotopically highly enriched targets of 70Ge, 72Ge and 73Ge, provided by the nTOF collaboration at CERN, have been used, thus allowing accurate cross section measurements since no corrections are needed to compensate for the parasitic reactions from neighboring isotopes that exist in the case of using natural Ge target. The cross section has been deduced with respect to the 27Al(n,α)24Na reference reaction.
Τhe 70Ge(n,2n)69Ge、72Ge(n,a)69mZn、72Ge(n,p)72Ga和73Ge(n,p)73Ga反应在中子能17.9 MeV下进行了活化测量。在NCSR“Demokritos”的5.5 MV串联Van de Graaff加速器上,通过2H(d,n)3He反应产生准单能中子束。使用了由欧洲核子研究中心nTOF合作提供的同位素高度富集的70Ge、72Ge和73Ge靶,因此可以实现精确的横截面测量,因为在使用天然Ge靶时不需要校正邻近同位素的寄生反应。推导了27Al(n,α)24Na参考反应的截面。
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引用次数: 1
Characterisation of the new HPGe detectors at INPP/NCSR “Demokritos”... and future (n,2n) reactions to be studied 新型高能锗探测器在INPP/NCSR“Demokritos”上的表征以及未来的(n,2n)反应
Pub Date : 2022-10-17 DOI: 10.12681/hnps.3580
M. Peoviti, M. Axiotis, E. Georgali, S. Harissopulos, A. Lagoyannis, N. Patronis
Within the present work the HPGe detectors of the Institute of Nuclear and Particle Physics at NCSR “Demokritos” were fully characterized in terms of their efficiency. The three n-type 80% relative efficiency HPGe were recently acquired in the framework of the CALIBRA project. All detectors are equipped with carbon epoxy windows that allow detection of low energy γ-rays. Beside the efficiency characterization, the three detectors were fully modeled by means of GEANT4. In all cases the simulated detector geometries were fine-tuned so as to fully reproduce the experimental efficiency data at different source-to-detector distances. Finally, as a demonstration of the new offered abilities, the efficiency characterization and the GEANT4 modeling of the three HPGe detectors was used for a feasibility study of possible/future (n,2n) activation measurements on medium-weight nuclei.
在本工作中,NCSR“Demokritos”核与粒子物理研究所的HPGe探测器在其效率方面得到了充分的表征。最近在CALIBRA项目的框架内获得了三个n型80%相对效率的HPGe。所有探测器都配备了碳环氧树脂窗口,允许检测低能γ射线。除了效率表征外,还利用GEANT4对三种探测器进行了全面建模。在所有情况下,模拟的探测器几何形状都经过了微调,以便完全再现不同源到探测器距离下的实验效率数据。最后,为了证明新提供的能力,三种HPGe探测器的效率表征和GEANT4建模用于中重核可能/未来(n,2n)活化测量的可行性研究。
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引用次数: 0
On the Dominance of Deformation in Nuclear Physics, its Link to Symplectic Symmetry, and its Roots in an Effective Field Theory 论形变在核物理中的主导地位及其与辛对称的联系及其在有效场论中的根源
Pub Date : 2022-10-17 DOI: 10.12681/hnps.3613
J. Draayer, D. Kekejian, G. Sargsyan, T. Dydtrych, R. Baker, K. Launey
A brief historical review of the important role symmetries have played in our gaining a deeper understanding nuclear structure is presented.We then focus our attention on the special role that symplectic symmetry plays in exposing a “Dominance of Deformation” that is found through enhanced B(E2) rates across the Chart of the Nuclides, and in addition, we will show how the No-Core Symplectic Shell Model (NC-SpSM) seems to emerge from a Symplectic Effective Field Theory(Sp-EFT), where the latter prepares away forward for gaining a truly ab initio understanding of the structure of atomic nuclei. As space permits, various spectra, B(E2) transition rates, and nuclear radii of selected light to medium-mass nuclei are shown.
简要回顾了对称性在我们加深对核结构的认识中所起的重要作用。然后,我们将注意力集中在辛对称在揭示“变形优势”方面所起的特殊作用上,这种优势是通过核素图中增强的B(E2)速率发现的,此外,我们将展示无核辛壳模型(NC-SpSM)似乎是从辛有效场论(Sp-EFT)中产生的,后者为获得对原子核结构的真正从头开始理解做好了准备。在篇幅允许的情况下,给出了选定的轻质量到中等质量原子核的各种光谱、B(E2)跃迁速率和核半径。
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引用次数: 0
Neutron Scattering from Porous Materials and Confined Fluids: Applications to CO2 Sequestration and Oil Recovery 多孔材料和受限流体中的中子散射:在CO2封存和采油中的应用
Pub Date : 2022-10-17 DOI: 10.12681/hnps.3579
K. Stefanopoulos
In the current study we briefly review the advantages of utilising elastic neutron scattering techniques to reveal the structure of porous materials and pore-confined fluids. Furthermore, we highlight the benefits of utilising in situ CO2 injection and neutron scattering in model porous systems as well as in sedimentary rocks to explore the pore morphology, the pore accessibility and the structural properties of pore-confined CO2. This information is important for the design of optimal CO2 sequestration as well as gas and oil recovery projects.
在本研究中,我们简要回顾了利用弹性中子散射技术揭示多孔材料和孔隙约束流体结构的优点。此外,我们强调了在模型孔隙系统以及沉积岩中利用原位CO2注入和中子散射来探索孔隙形态、孔隙可达性和孔隙限制CO2的结构特性的好处。这些信息对于设计最佳的二氧化碳封存以及油气开采项目非常重要。
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引用次数: 0
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HNPS Advances in Nuclear Physics
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