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Dry printing fully functional eco-friendly and disposable transient papertronics 干式印刷全功能环保型一次性瞬态纸张电子元件
IF 3.1 4区 工程技术 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-08-29 DOI: 10.1088/2058-8585/ad70c5
Adib Taba, Aarsh Patel, Masoud Mahjouri-Samani
The demand for flexible printed electronics is growing fast, especially with the move toward the Internet of Things. These printed electrons are usually designed for short-term use, after which they are disposed of. The polymeric substrates used in printed electronics comprise the biggest portion of their non-biodegradable E-waste after their disposal. This paper demonstrates the feasibility of printing fully functional transient electronics on flexible, water-soluble, and biodegradable paper substrates using the dry printing approach. The in-situ generation and real-time sintering of silver nanoparticles at room temperature enables the fabrication of complex circuits on such water-soluble papers. A layout similar to an Arduino pro mini board is printed on both sides of a paper substrate with electrical interconnects. Various electrical components are then directly mounted to fabricate a complete, working paper Arduino circuit. Cyclic bending tests demonstrate the mechanical durability and reliability of printed paper circuits under repeated bending stress. The process uniquely achieves robust and complex printed electronics without thermal damage, and the water solubility tests successfully show rapid dissolution of the paper devices in water. Furthermore, the components detached during dissolution are collected and reused, demonstrating the recyclability of the process. Overall, this transformative manufacturing method establishes key technical capabilities to produce next-generation sustainable, green electronics and sensors using renewable materials.
对柔性印刷电子产品的需求正在快速增长,特别是随着物联网的发展。这些印刷电子产品通常是为短期使用而设计的,之后就会被丢弃。印刷电子产品中使用的聚合物基底在废弃后的不可生物降解电子垃圾中占最大比例。本文展示了利用干式印刷方法在柔性、水溶性和可生物降解的纸质基底上印刷全功能瞬态电子器件的可行性。银纳米粒子在室温下的原位生成和实时烧结使得在这种水溶性纸张上制造复杂电路成为可能。类似于 Arduino pro 迷你电路板的布局被印刷在纸基板的两面,并带有电气互连。然后直接安装各种电气元件,制作出一个完整的、可工作的纸质 Arduino 电路。循环弯曲测试证明了印刷纸电路在反复弯曲应力下的机械耐久性和可靠性。该工艺独特地实现了坚固而复杂的印刷电子元件,且不会产生热损伤,水溶性测试成功显示了纸器件在水中的快速溶解。此外,溶解过程中脱落的元件可以收集起来重新使用,这证明了该工艺的可回收性。总之,这种变革性的制造方法建立了利用可再生材料生产下一代可持续绿色电子器件和传感器的关键技术能力。
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引用次数: 0
Flexible intracortical probes for stable neural recording: from the perspective of structure 用于稳定神经记录的灵活皮层内探针:从结构的角度看问题
IF 3.1 4区 工程技术 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-08-29 DOI: 10.1088/2058-8585/ad71dc
Suhao Wang, Qianqian Jiang, Jizhou Song
Electrical neural interfaces provide direct communication pathways between living brain tissue and engineered devices to understand brain function. However, conventional neural probes have remained limited in providing stable, long-lasting recordings because of large mechanical and structural mismatches with respect to brain tissue. The development of flexible probes provides a promising approach to tackle these challenges. In this review, various structural designs of flexible intracortical probes for promoting long-term neural integration, including thin film filament and mesh probe structures that provide similar geometric and mechanical properties to brain tissue and self-deployable probe structure that enables moving the functional sensors away from the insertion trauma, are summarized, highlighting the important role of structural design in improving the long-term recording stability of neural probes.
电气神经接口提供了活体脑组织与工程设备之间的直接通信途径,以了解大脑功能。然而,传统的神经探针在提供稳定、持久的记录方面仍然受到限制,因为它们与脑组织之间存在较大的机械和结构不匹配。柔性探针的开发为应对这些挑战提供了一种前景广阔的方法。在这篇综述中,总结了促进长期神经整合的皮质内柔性探针的各种结构设计,包括与脑组织具有相似几何和机械特性的薄膜丝状和网状探针结构,以及可将功能传感器从插入创面移开的自部署探针结构,强调了结构设计在提高神经探针长期记录稳定性方面的重要作用。
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引用次数: 0
End-of-life options for printed electronics in municipal solid waste streams: a review of the challenges, opportunities, and sustainability implications 城市固体废物流中印刷电子产品的报废选择:对挑战、机遇和可持续性影响的审查
IF 3.1 4区 工程技术 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-08-27 DOI: 10.1088/2058-8585/ad699b
Mohammad Naji Nassajfar, Mariam Abdulkareem, Mika Horttanainen
Although printed electronics (PE) are a more sustainable option than conventional electronics, proper treatment of PE in their end-of-life phase is crucial to decrease their overall environmental impacts and ensure the materials specifically the metal fraction of PE are recovered. Thus, to investigate the state of the art regarding the research and development of material recovery from PE, this study performed a literature review process. It concluded that the majority of the observed articles rather not mention specifically what is recycling option for recycling the PE or introduced a novel recycling method for the metal ink. Only a marginal fraction of the articles covered proper recycling methods for the metal fraction of PE. Then based on the literature review process, this study investigates the suitability of the current waste management system to recover different fractions of PE products.
尽管与传统电子产品相比,印刷电子产品(PE)是一种更具可持续性的选择,但在其报废阶段对其进行适当处理对于减少其对环境的总体影响以及确保回收材料(尤其是 PE 中的金属部分)至关重要。因此,为了调查从聚乙烯中回收材料的研发现状,本研究进行了文献综述。研究得出的结论是,所观察到的大多数文章都没有具体提及什么是回收聚乙烯的回收方案,也没有介绍金属油墨的新型回收方法。只有一小部分文章介绍了聚乙烯金属部分的正确回收方法。因此,本研究在文献综述的基础上,调查了当前废物管理系统是否适合回收不同馏分的聚乙烯产品。
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引用次数: 0
Transparent and flexible fish-tail shaped antenna for ultra-wideband MIMO systems 用于超宽带多输入多输出系统的透明柔性鱼尾形天线
IF 3.1 4区 工程技术 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-08-14 DOI: 10.1088/2058-8585/ad6883
Shilin Lian, Haoyuan Sun, Hua Zhang, Dan Zhang, Tian Liu, Zhejun Jin, Yu Zheng
The article presents an innovative transparent, flexible antenna design tailored specifically for ultra-wideband multiple-input multiple-output (MIMO) systems. Using polyethylene terephthalate substrates as the base material, we enhance the antenna’s radiation performance, transparency, and flexibility. Broadband impedance matching is achieved through a hollow ground plane fed by a fish-tail radiator and coplanar waveguide. Additionally, significant MIMO antenna isolation in ultra-wideband scenarios is achieved through the vertical arrangement of units and neutral lines. The MIMO antennas we manufactured exhibit minimum transparencies of 71.1% and 85.9% with and without reflectors, respectively. Measurement results demonstrate that the antenna operates within the 3–20 GHz frequency range, with over 24 dB of isolation, 2 ± 2 dBi of peak gain, and 45% ± 5% of radiation efficiency, suitable for applications in wearable devices, vehicle intelligence, and other fields.
文章介绍了一种专为超宽带多输入多输出 (MIMO) 系统定制的创新型透明柔性天线设计。我们使用聚对苯二甲酸乙二醇酯基材作为基础材料,提高了天线的辐射性能、透明度和灵活性。通过鱼尾辐射器和共面波导馈入的空心地平面实现了宽带阻抗匹配。此外,通过垂直排列单元和中性线,在超宽带场景中实现了显著的 MIMO 天线隔离。我们制造的 MIMO 天线在有反射器和无反射器时的最小透射率分别为 71.1% 和 85.9%。测量结果表明,该天线可在 3-20 GHz 频率范围内工作,隔离度超过 24 dB,峰值增益为 2 ± 2 dBi,辐射效率为 45% ± 5%,适用于可穿戴设备、车辆智能和其他领域的应用。
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引用次数: 0
Recent advances in encapsulation strategies for flexible transient electronics 柔性瞬态电子封装策略的最新进展
IF 3.1 4区 工程技术 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-08-14 DOI: 10.1088/2058-8585/ad6a6c
Won Bae Han, Suk-Won Hwang, Woon-Hong Yeo
Transient electronics, designed to dissolve, disintegrate, or degrade in a controlled manner after fulfilling their functions without remaining biologically and environmentally harmful byproducts, have emerged as a transformative paradigm with promising applications in temporary biomedical devices, eco-friendly electronics, and security applications. The success of this device development relies significantly on an effective encapsulation to protect their degradable active materials from environmental factors, such as biofluids and water, and secure reliable device functions throughout a desired lifespan. This review article provides an overview of recent advances in various encapsulation strategies for developing flexible, transient electronics. Details include materials selection, key characteristics, water-barrier capabilities, degradation mechanisms, and relevant applications, categorized into inorganic materials, synthetic/natural polymers, and hybrid composites. In addition, our insights into existing challenges and key perspectives for enhancing encapsulation performance are shared.
瞬态电子器件可在完成功能后以受控方式溶解、分解或降解,不会残留对生物和环境有害的副产品,已成为一种变革性范例,在临时生物医学设备、生态友好型电子器件和安全应用方面具有广阔的应用前景。这种装置开发的成功在很大程度上依赖于有效的封装,以保护其可降解活性材料免受生物流体和水等环境因素的影响,并确保装置在所需的使用寿命内发挥可靠的功能。这篇综述文章概述了用于开发柔性瞬态电子器件的各种封装策略的最新进展。详细内容包括材料选择、关键特性、防水能力、降解机制和相关应用,分为无机材料、合成/天然聚合物和混合复合材料。此外,还分享了我们对现有挑战的见解以及提高封装性能的主要观点。
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引用次数: 0
Effects of transparent conducting electrodes and hole transport layers on the performance of MAPbI3 solar cells fabricated on PET substrates 透明导电电极和空穴传输层对 PET 基底上制造的 MAPbI3 太阳能电池性能的影响
IF 3.1 4区 工程技术 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-07-09 DOI: 10.1088/2058-8585/ad5d01
Bishal Bhandari, Justin C Bonner, Robert T Piper, Julia W P Hsu
This study investigates how the performance of perovskite solar cells (PSCs) made on polyethylene terephthalate (PET) substrates depends on transparent conducting electrodes (TCEs) and hole transport layers (HTLs). We fabricated PSCs using commercially available PET/TCEs and compared their performance with PSCs manufactured on Glass/indium tin oxide (ITO) substrates. Poly(3,4-ethylenedioxythiophene):polystyrene sulfonate (PEDOT:PSS) with varying levels of acidity and NiO nanoparticles were used as HTLs. The current density-voltage characteristics of PSCs made on PET/TCEs were found to be significantly lower when highly acidic PEDOT:PSS was used as the HTL. However, this was not observed for PSCs made on Glass/ITO. To investigate the interaction between HTL and TCE, atomic force microscopy was carried out after dipping the TCEs in PEDOT:PSS solutions of different acidity. X-ray photoelectron spectroscopy measurements further revealed differences in the chemical composition between ITO film on PET vs. on glass. Our results indicate that the performance of PSCs depends both on the TCE substrates and HTLs, which can be explained by their chemical interaction.
本研究探讨了在聚对苯二甲酸乙二醇酯(PET)衬底上制造的过氧化物太阳能电池(PSCs)的性能如何取决于透明导电电极(TCEs)和空穴传输层(HTLs)。我们使用市售的 PET/TCE 制作了 PSC,并将其性能与在玻璃/氧化铟锡(ITO)基板上制作的 PSC 进行了比较。不同酸度的聚(3,4-亚乙二氧基噻吩):聚苯乙烯磺酸盐(PEDOT:PSS)和纳米氧化镍颗粒被用作 HTL。当使用高酸性 PEDOT:PSS 作为 HTL 时,在 PET/TCE 上制造的 PSC 的电流密度-电压特性明显降低。然而,在玻璃/ITO 上制成的 PSC 却没有观察到这种情况。为了研究 HTL 与 TCE 之间的相互作用,在将 TCE 浸入不同酸度的 PEDOT:PSS 溶液后进行了原子力显微镜观察。X 射线光电子能谱测量进一步揭示了 PET 上的 ITO 膜与玻璃上的 ITO 膜在化学成分上的差异。我们的研究结果表明,PSC 的性能取决于 TCE 基底和 HTL,这可以用它们之间的化学作用来解释。
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引用次数: 0
Flexible self-powered triboelectric nanogenerator sensor for wind speed measurement driven by moving trains 用于移动列车驱动的风速测量的灵活自供电三电纳米发电机传感器
IF 3.1 4区 工程技术 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-07-09 DOI: 10.1088/2058-8585/ad5c7c
Wentao Dong, Bo Huang, Kaiqi Sheng and Xiao Cheng
Flexible self-powered sensors have been extensively applied to the Internet of Things, structural health monitoring (SHM), and intelligent transportation. It would be more demanding for the power supply to these sensors during the long-term maintenance of the rail transit system. The wind pressure/velocity generated by high-speed trains poses a substantial threat to safety of human, and new sensors without an external power supply should be developed to monitor wind pressure/velocity in the trackside. Flexible self-powered wind triboelectric nanogenerator (W-TENG) sensor with a single-electrode mode based on conductive hydrogel is designed to wind pressure/velocity monitoring without power supply by harvesting wind energy. It is devoted the relationship between the output voltage of the sensors and the wind pressure/velocity driven by high-speed trains. Material selection and structural design methods are adopted to enhance the energy harvesting efficiency and sensing accuracy of self-powered W-TENG sensors. Open-circuit current of 2.8 μA and open-circuit voltage of 12 V are achieved, and the output voltage signal has the linear relationship with trackside wind pressure/velocity. Field tests are implemented to evaluate the performance of self-powered W-TENG sensors in wind pressure/velocity measurement caused by moving trains, providing an idea to SHM application in intelligent transmit systems.
灵活的自供电传感器已广泛应用于物联网、结构健康监测(SHM)和智能交通领域。在轨道交通系统的长期维护过程中,对这些传感器的供电要求更高。高速列车产生的风压/风速对人身安全构成重大威胁,因此应开发无需外部电源的新型传感器来监测轨道旁的风压/风速。基于导电水凝胶的单电极模式柔性自供电风力三电纳米发电机(W-TENG)传感器就是通过收集风能来实现无电源风压/风速监测的。研究了传感器输出电压与高速列车驱动的风压/风速之间的关系。采用材料选择和结构设计方法来提高自供电 W-TENG 传感器的能量收集效率和传感精度。实现了 2.8 μA 的开路电流和 12 V 的开路电压,输出电压信号与轨旁风压/风速呈线性关系。通过现场测试,评估了自供电 W-TENG 传感器在列车运行引起的风压/风速测量中的性能,为 SHM 在智能传输系统中的应用提供了思路。
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引用次数: 0
Flexo-printed polymer waveguides for integration in electro-optical circuit boards 用于集成到光电电路板中的柔性印刷聚合物波导
IF 3.1 4区 工程技术 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-07-03 DOI: 10.1088/2058-8585/ad5c7b
Andreas Evertz, Jonathan Pleuß, Birger Reitz and Ludger Overmeyer
Electro-optical circuit boards (EOCBs) offer great potential for short-ranged data transmission in highly electro-magnetic inflicted environments. Finding a cost-efficient way to manufacture EOCB only using additive printing processes could establish, increase, and secure data transmission in PCB systems. Flexo printing is an efficient manufacturing process that combines high contour resolution and layout flexibility to create optical waveguides. Previous research has shown that printing waveguides on a polymethylmethacrylate substrate can enable optical data transmission for up to 20 cm. However, a thermo-resistant polyimide (PI) substrate is needed to integrate printed waveguides into PCB. Since PI does not meet optical demands, waveguide cores must be separated by printed optical cladding. This research aims to investigate the additive printing process, which stacks various polymers to achieve waveguides that are ready for integration. Further, the integration in PCB is validated according to functional testing of the optical structures. An entire manufacturing process for printed EOCB is presented, which enables the investigation of optical coupling processes in upcoming research.
光电电路板(EOCB)为在高电磁环境中进行短距离数据传输提供了巨大潜力。找到一种仅使用快速成型印刷工艺制造 EOCB 的经济高效的方法,可以在 PCB 系统中建立、增加和保护数据传输。柔版印刷是一种高效的制造工艺,它结合了高轮廓分辨率和布局灵活性来制造光波导。先前的研究表明,在聚甲基丙烯酸甲酯基板上印刷波导可实现长达 20 厘米的光数据传输。然而,要将印刷波导集成到印刷电路板中,需要一种耐热聚酰亚胺(PI)基板。由于聚酰亚胺不符合光学要求,波导芯必须用印刷光学包层隔开。本研究旨在研究增材印刷工艺,该工艺将各种聚合物堆叠在一起,以实现可随时集成的波导。此外,还根据光学结构的功能测试验证了 PCB 中的集成。本研究介绍了印刷 EOCB 的整个制造过程,从而能够在即将开展的研究中对光学耦合过程进行调查。
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引用次数: 0
Inkjet-printed low temperature co-fired ceramics: process development for customized LTCC 喷墨打印低温共烧陶瓷:定制 LTCC 的工艺开发
IF 3.1 4区 工程技术 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-06-26 DOI: 10.1088/2058-8585/ad59b3
Jonas Jäger, Martin Ihle, Kerstin Gläser and André Zimmermann
This paper investigates the utilization of digital printing technologies for the fabrication of low temperature co-fired ceramics (LTCC). LTCC offer great opportunities for applications such as antennas, sensors or actuators due to their outstanding properties like low dielectric loss, low permittivity, low coefficient of thermal expansion and at the same time high reliability in harsh environments (heat, humidity, and radiation). LTCC are multilayer circuits that are typically functionalized by screen-printing. This publication investigates the replacement of screen-printing by digital printing processes, such as inkjet and Aerosol Jet printing, to facilitate a more resource-friendly and customizable manufacturing of LTCC. The use of digital printing technologies not only streamlines small-scale productions and development processes but also offers the advantage of achieving miniaturization down to single-digit microns. In this publication, digital printing processes, filling of vias, lamination processes, co-firing at 850 °C and printing on fired LTCC were investigated. Three layers of nanoparticle silver ink were printed on green LTCC tape and 100% of the embedded printed structures were conductive after co-firing. Filling of vias with inkjet printing was investigated and the most important process parameters were found to be the clustering of vias, the amount of active nozzles and the substrate temperature. Printing on fired LTCC demonstrated high precision, and sintering at 600 °C achieved strong adhesion of printed structures to LTCC. These successful findings culminate in presenting a process chain for fully maskless structured, multilayer LTCC.
本文研究了如何利用数字印刷技术制造低温共烧陶瓷(LTCC)。由于低温共烧陶瓷具有低介电损耗、低介电常数、低热膨胀系数等优异性能,同时在恶劣环境(高温、潮湿和辐射)下具有高可靠性,因此为天线、传感器或执行器等应用提供了巨大的机遇。LTCC 是多层电路,通常通过丝网印刷进行功能化。本出版物研究了用数字印刷工艺(如喷墨和气溶胶喷射印刷)取代丝网印刷的问题,以促进资源友好型和可定制型 LTCC 的制造。数字印刷技术的使用不仅简化了小规模生产和开发流程,而且还具有实现微型化(小至个位数微米)的优势。本出版物研究了数字印刷工艺、通孔填充、层压工艺、850 ℃ 共烧以及在烧结的 LTCC 上进行印刷。在绿色 LTCC 带上印刷了三层纳米银墨水,经过共烧后,100% 的嵌入式印刷结构具有导电性。通过喷墨打印填充通孔的研究发现,最重要的工艺参数是通孔的聚类、活性喷嘴的数量和基底温度。在烧结的 LTCC 上进行喷印显示出很高的精度,而在 600 °C 下烧结则实现了喷印结构与 LTCC 的牢固粘合。这些成功的研究成果最终为完全无掩模结构的多层 LTCC 提供了一条工艺链。
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引用次数: 0
Flexible, self-healing, and degradable polymeric dielectrics cross-linked through metal–ligand for resistive memory device 通过金属配体交联的柔性、自愈合和可降解聚合物电介质用于电阻式存储器件
IF 3.1 4区 工程技术 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-06-25 DOI: 10.1088/2058-8585/ad5028
Yu-Chi Chang, Yi-Yun Liang and Hao-Jung Liu
The ability to self-heal is a crucial feature in nature, where living organisms can repair themselves when subjected to minor injuries. With an increasing emphasis on environmental sustainability, the concept of biomimetic self-healing polymeric materials has emerged as a prominent trend, promising to significantly extend the lifespan and reliability of products. Studies have shown that one-third of proteins in living organisms require metal cofactors to function properly. It is known that protein-metal interactions can enhance the performance of certain biomaterials, and different choices of metals and ligands can create diverse material properties, influencing characteristics such as hardness, toughness, adhesion, and self-healing abilities. Gelatin is a natural polymer derived from the hydrolysis of collagen, and its unique amino acid structure has led to a wide range of applications. In this research, by introducing aluminum ions that form metal coordination complexes with the carboxyl groups in gelatin, an elastic network with self-healing properties was constructed. This gelatin-based material was utilized as an insulating layer in resistive switching devices. Furthermore, by employing a gelatin substrate of the same composition, the device demonstrated strong interfacial adhesion. The device based on the self-healing gelatin film exhibited excellent electrical performance and mechanical properties. Even after self-healing, it maintained a high ON/OFF ratio of up to 105 and a concentrated distribution of switching parameters. Supported by compelling physical and electrical evidence, this study showcases significant development opportunities for biomimetic materials in green electronic devices.
自愈能力是自然界的一个重要特征,生物体在受到轻微伤害时可以自我修复。随着人们对环境可持续性的日益重视,仿生自愈合聚合物材料的概念已成为一个突出的趋势,有望显著延长产品的使用寿命和可靠性。研究表明,生物体内三分之一的蛋白质需要金属辅助因子才能正常发挥作用。众所周知,蛋白质与金属之间的相互作用可提高某些生物材料的性能,而金属和配体的不同选择可产生不同的材料特性,影响材料的硬度、韧性、附着力和自愈能力等特性。明胶是一种天然聚合物,由胶原蛋白水解而来,其独特的氨基酸结构带来了广泛的应用。在这项研究中,通过引入铝离子与明胶中的羧基形成金属配位复合物,构建了一种具有自愈合特性的弹性网络。这种明胶基材料被用作电阻开关器件的绝缘层。此外,通过使用相同成分的明胶基底,该装置还表现出很强的界面粘附性。基于自愈合明胶薄膜的设备具有出色的电气性能和机械性能。即使在自愈合后,它仍能保持高达 105 的高导通/关断比和集中的开关参数分布。在令人信服的物理和电学证据的支持下,这项研究为绿色电子设备中的仿生物材料提供了重要的发展机遇。
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引用次数: 0
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Flexible and Printed Electronics
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