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Toward understanding the microstructure characteristics, phase selection and magnetic properties of laser additive manufactured Nd-Fe-B permanent magnets 为了了解激光增材制备Nd-Fe-B永磁体的显微结构特征、相选择和磁性能
1区 工程技术 Q1 ENGINEERING, MANUFACTURING Pub Date : 2023-10-18 DOI: 10.1088/2631-7990/ad0472
Bo Yao, Nan KANG, Xiangyu Li, Dou Li, Mohamed El Mansori, Jing Chen, Haiou Yang, Hua Tan, Xin LIN
Abstract Nd-Fe-B permanent magnets are critical components for energy conversion and electronic devices. The key magnetic properties of Nd-Fe-B magnets, especially the coercivity and remanent magnetization, are strongly dependent on the phase characteristics and microstructure. In this work, Nd-Fe-B magnets were prepared using vacuum induction melting (VIM), laser directed energy deposition (LDED) and laser powder bed fusion (LPBF) technologies. The microstructure evolution and phase selection of Nd-Fe-B magnets were clarified in detail. The results indicated that the solidification velocity (V) and cooling rate (R) are key factors in determining the phase selection. In terms of the VIM-casting Nd-Fe-B magnet, a large volume fraction of the soft magnetic α-Fe phase (39.7 vol.%) and Nd2Fe17Bx metastable phase (34.7 vol.%) are formed due to the low R (2.3×10-1 ℃/s), while the hard magnetic Nd2Fe14B phase is only 5.15 vol.%. With increasing V (<10-2 m/s) and R (5.06×103 ℃/s), part of the soft magnetic α-Fe phase (31.7 vol.%) was suppressed, more Nd2Fe17Bx metastable phases (47.5 vol.%) were formed in the LDED-processed Nd-Fe-B magnet, and the hard magnetic Nd2Fe14B phase also had a low value (3.4 vol.%). As a result, the casting- and LDED-processed Nd-Fe-B magnets exhibit poor magnetic properties. In contrast, the high V (>10-2 m/s) and R (1.45×106 ℃/s) led to the formation of the hard magnetic Nd2Fe14B phase (55.8 vol.%) from liquid, and the α-Fe phase and Nd2Fe17Bx phase precipitation were suppressed in the LPBF-processed Nd-Fe-B magnet. Furthermore, the strong crystallographic texture on the {001} crystal plane is another reason for the remanence enhancement in the LPBF-processed Nd-Fe-B magnets. Consequently, a coercivity of 656 kA/m, a remanence of 0.79 T and maximum energy product of 71.5 kJ/m3 was achieved in the LPBF-processed Nd-Fe-B magnet, which indicated excellent magnetic performance, comparable to other additive manufacturing processed Nd-Fe-B magnets from MQP (Nd-lean) Nd-Fe-B powder.
Nd-Fe-B永磁体是能量转换和电子器件的关键部件。Nd-Fe-B磁体的主要磁性能,特别是矫顽力和剩余磁化强度,很大程度上取决于相特性和微观结构。本文采用真空感应熔炼(VIM)、激光定向能沉积(LDED)和激光粉末床熔炼(LPBF)技术制备了Nd-Fe-B磁体。详细阐述了Nd-Fe-B磁体的微观组织演变和相选择。结果表明,凝固速度(V)和冷却速度(R)是决定相选择的关键因素。在vim铸造Nd-Fe-B磁体中,由于R (2.3×10-1℃/s)较低,形成了大量的软磁α-Fe相(39.7 vol.%)和Nd2Fe17Bx亚稳相(34.7 vol.%),而硬磁Nd2Fe14B相仅为5.15 vol.%。随着V (<10-2 m/s)和R (5.06×103℃/s)的增大,led加工的Nd-Fe-B磁体中部分软磁α-Fe相(31.7 vol.%)被抑制,形成了更多的Nd2Fe17Bx亚稳相(47.5% vol.%),硬磁Nd2Fe14B相也出现了低值(3.4 vol.%)。因此,铸造和led加工的Nd-Fe-B磁体表现出较差的磁性能。与此相反,高V (>10-2 m/s)和R (1.45×106℃/s)导致液体形成硬磁性Nd2Fe14B相(55.8% vol.%), lpbf加工的Nd-Fe-B磁体中α-Fe相和Nd2Fe17Bx相的析出受到抑制。此外,{001}晶面上的强晶体织构是lpbf加工的Nd-Fe-B磁体剩余物增强的另一个原因。因此,lpbf加工的Nd-Fe-B磁体的矫顽力为656 kA/m,剩余量为0.79 T,最大能积为71.5 kJ/m3,具有与MQP (Nd-lean) Nd-Fe-B粉末增材制造加工的Nd-Fe-B磁体相当的优异磁性。
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引用次数: 0
Influence of heat treatment on microstructure, mechanical and corrosion behavior of WE43 alloy fabricated by laser-beam powder bed fusion 热处理对激光粉末床熔合WE43合金组织、力学和腐蚀行为的影响
1区 工程技术 Q1 ENGINEERING, MANUFACTURING Pub Date : 2023-10-17 DOI: 10.1088/2631-7990/acfad5
chenrong ling, qiang li, zhe zhang, Youwen Yang, wenhao zhou, wenlong chen, zhi dong, chunrong pan, cijun shuai
Highlights WE43 parts with favorable forming quality are fabricated by laser-beam powder bed fusion and the interaction between laser beam and powder is revealed. After suitable heat treatment, the anisotropic microstructure is eliminated, with nano-scaled Mg 24 Y 5 particles homogeneously precipitated. The yield strength and ultimate tensile strength are improved to (250.2 ± 3.5) MPa and (312 ± 3.7) MPa, respectively, while the elongation still maintains at high level of 15.2%. Homogenized microstructure inhibits the micro galvanic corrosion and promotes the development of passivation film, thus decreasing the degradation rate by an order of magnitude. The porous WE43 scaffolds offer a favorable environment for cell growth.
采用激光粉末床熔接技术制备了具有良好成形质量的WE43零件,并揭示了激光与粉末的相互作用。经过适当热处理后,各向异性组织被消除,纳米级mg24y5颗粒均匀析出。屈服强度和极限抗拉强度分别提高到(250.2±3.5)MPa和(312±3.7)MPa,伸长率仍保持在15.2%的较高水平。均匀化的微观结构抑制了微电偶腐蚀,促进了钝化膜的形成,从而使降解速率降低了一个数量级。多孔WE43支架为细胞生长提供了良好的环境。
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引用次数: 4
Towards a new avenue for rapid synthesis of electrocatalytic electrodes via laser-induced hydrothermal reaction for water splitting 探索激光诱导水热反应快速合成电催化电极的新途径
1区 工程技术 Q1 ENGINEERING, MANUFACTURING Pub Date : 2023-10-16 DOI: 10.1088/2631-7990/ad038f
Yang Sha, menghui zhu, Kun Huang, Yang Zhang, Francis Moissinac, zhizhou zhang, Dongxu Cheng, Paul Mativenga, Zhu Liu
Abstract Electrochemical production of hydrogen from water requires the development of electrocatalysts that are active, stable, and low-cost for water splitting. In comparison with conventional powder-based electrode preparation, synthesis of binder-free electrocatalytic integrated electrodes is highly desirable to improve the catalytic activity and long-term stability for large-scale applications of electrocatalysts. Herein, we demonstrate a laser-induced hydrothermal (LIHR) technique to grow NiMoO4 nanosheets on Nickel foam, which is then calcined under H2/Ar mixed gases to prepare the integrated electrode IE-NiMo-LR. This electrode exhibits superior hydrogen evolution reaction performance, requiring overpotentials of 59, 116 and 143 mV to achieve current densities of 100, 500 and 1000 mA cm-2. During the 350 h chronopotentiometry test at current densities of 100 and 500 mA cm-2, the overpotential remained essentially unchanged. In addition, NiFe-layered double hydroxide grown on Ni foam is fabricated with same LIHR method and coupled with IE-NiMo-IR to achieve water splitting. This combination exhibits excellent durability under industrial current density. The energy consumption and production efficiency of LIHR method are systematically compared with conventional hydrothermal method. The LIHR method significantly improved the production rate by over 19 times, while consuming only 27.78% of the total energy required by conventional hydrothermal method to achieve the same production.
摘要电化学从水中制氢需要开发出活性、稳定、低成本的水分解电催化剂。与传统的粉末电极制备相比,为了提高电催化剂的大规模应用的催化活性和长期稳定性,合成无粘结剂的电催化集成电极是非常理想的。在此,我们展示了激光诱导水热(LIHR)技术在泡沫镍上生长NiMoO4纳米片,然后在H2/Ar混合气体下煅烧制备集成电极ie - nimo4 - lr。该电极具有优异的析氢反应性能,需要59、116和143 mV的过电位才能达到100、500和1000 mA cm-2的电流密度。在100和500 mA cm-2的电流密度下进行350小时时电位测定试验,过电位基本保持不变。此外,采用相同的LIHR方法制备了Ni泡沫上生长的nife层状双氢氧化物,并结合IE-NiMo-IR实现了水裂解。这种组合在工业电流密度下表现出优异的耐久性。对LIHR法的能耗和生产效率与传统水热法进行了系统比较。LIHR法的产量提高了19倍以上,而达到相同产量所需的总能量仅为传统水热法的27.78%。
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引用次数: 0
A brief review on the recent development of phonon engineering and manipulation at nanoscales 简要综述了声子工程和纳米尺度声子操作的最新进展
1区 工程技术 Q1 ENGINEERING, MANUFACTURING Pub Date : 2023-10-13 DOI: 10.1088/2631-7990/acfd68
Siqi Xie, Hongxin Zhu, Xing Zhang, Haidong Wang
Abstract Phonons are the quantum mechanical descriptions of vibrational modes that manifest themselves in many physical properties of condensed matter systems. As the size of electronic devices continues to decrease below mean free paths of acoustic phonons, the engineering of phonon spectra at the nanoscale becomes an important topic. Phonon manipulation allows for active control and management of heat flow, enabling functions such as regulated heat transport. At the same time, phonon transmission, as a novel signal transmission method, holds great potential to revolutionize modern industry like microelectronics technology, and boasts wide-ranging applications. Unlike fermions such as electrons, polarity regulation is difficult to act on phonons as bosons, making the development of effective phonon modulation methods a daunting task. This work reviews the development of phonon engineering and strategies of phonon manipulation at different scales, reports the latest research progress of nanophononic devices such as thermal rectifiers, thermal transistors, thermal memories, and thermoelectric devices, and analyzes the phonon transport mechanisms involved. Lastly, we survey feasible perspectives and research directions of phonon engineering. Thermoelectric analogies, external field regulation, and acousto-optic co-optimization are expected to become future research hotspots.
声子是对振动模式的量子力学描述,它体现在凝聚态系统的许多物理性质中。随着电子器件尺寸不断减小到声子平均自由程以下,纳米尺度声子光谱工程成为一个重要课题。声子操作允许热流的主动控制和管理,使功能,如调节热传输。同时,声子传输作为一种新型的信号传输方式,对微电子技术等现代工业的变革具有巨大的潜力,具有广泛的应用前景。与费米子(如电子)不同,极性调节很难像玻色子一样作用于声子,这使得开发有效的声子调制方法成为一项艰巨的任务。本文综述了声子工程的发展和不同尺度声子操纵策略,报道了热整流器、热晶体管、热存储器和热电器件等纳米声子器件的最新研究进展,并分析了其中涉及的声子输运机制。最后,展望了声子工程的可行前景和研究方向。热电类比、外场调节和声光协同优化有望成为未来的研究热点。
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引用次数: 1
Engineering vascularized organotypic tissues via module assembly 通过模块组装工程血管化的器官型组织
1区 工程技术 Q1 ENGINEERING, MANUFACTURING Pub Date : 2023-10-11 DOI: 10.1088/2631-7990/acfcf2
Zhenzhen Zhou, Changru Liu, Yuting Guo, Yuan Pang, Wei Sun
Abstract Adequate vascularization is a critical determinant for the successful construction and clinical implementation of complex organotypic tissue models. Currently, low cell and vessel density and insufficient vascular maturation make vascularized organotypic tissue construction difficult, greatly limiting its use in tissue engineering and regenerative medicine. To address these limitations, recent studies have adopted pre-vascularized microtissue assembly for the rapid generation of functional tissue analogs with dense vascular networks and high cell density. In this article, we summarize the development of module assembly-based vascularized organotypic tissue construction and its application in tissue repair and regeneration, organ-scale tissue biomanufacturing, as well as advanced tissue modeling.
充分的血管化是复杂器官型组织模型成功构建和临床实施的关键决定因素。目前,由于细胞和血管密度低,血管成熟度不够,使得血管化器官型组织构建困难,极大地限制了其在组织工程和再生医学中的应用。为了解决这些限制,最近的研究采用了预血管化微组织组装来快速生成具有致密血管网络和高细胞密度的功能组织类似物。本文综述了基于模块组装的血管化器官型组织构建及其在组织修复与再生、器官尺度组织生物制造、高级组织建模等方面的应用进展。
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引用次数: 0
Device design principles and bioelectronic applications for flexible organic electrochemical transistors 柔性有机电化学晶体管的器件设计原理及生物电子学应用
1区 工程技术 Q1 ENGINEERING, MANUFACTURING Pub Date : 2023-10-11 DOI: 10.1088/2631-7990/acfd69
Lin Gao, Mengge Wu, Xinge Yu, Junsheng Yu
Organic electrochemical transistors (OECTs) exhibit significant potential for applications in healthcare and human-machine interfaces, due to their tunable synthesis, facile deposition, and excellent biocompatibility. Expanding OECTs to the flexible devices will significantly facilitate stable contact with the skin and enable more possible bioelectronic applications. In this work, we summarize the device physics of flexible OECTs, aiming to offer a foundational understanding and guidelines for material selection and device architecture. Particular attention is paid to the advanced manufacturing approaches, including photolithography and printing techniques, which establish a robust foundation for the commercialization and large-scale fabrication. And abundantly demonstrated examples ranging from biosensors, artificial synapses/neurons, to bioinspired nervous systems are summarized to highlight the considerable prospects of smart healthcare. In the end, the challenges and opportunities are proposed for flexible OECTs. The purpose of this review is not only to elaborate on the basic design principles of flexible OECTs, but also to act as a roadmap for further exploration of wearable OECTs in advanced bio-applications.
摘要有机电化学晶体管(OECTs)由于其可调节的合成、易于沉积和优异的生物相容性,在医疗保健和人机界面方面表现出巨大的应用潜力。将OECTs扩展到柔性器件将大大促进与皮肤的稳定接触,并实现更多可能的生物电子应用。在这项工作中,我们总结了柔性OECTs的器件物理,旨在为材料选择和器件结构提供基本的理解和指导。特别关注先进的制造方法,包括光刻和印刷技术,这为商业化和大规模制造奠定了坚实的基础。并总结了从生物传感器,人工突触/神经元到生物启发神经系统的大量演示示例,以突出智能医疗保健的可观前景。最后,提出了柔性oect面临的挑战和机遇。本文综述的目的不仅是阐述柔性OECTs的基本设计原则,而且为进一步探索可穿戴OECTs在高级生物应用中的发展提供了路线图。
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引用次数: 0
Energy beam-based direct and assisted polishing techniques for diamond: A review 基于能量束的金刚石直接和辅助抛光技术综述
1区 工程技术 Q1 ENGINEERING, MANUFACTURING Pub Date : 2023-10-10 DOI: 10.1088/2631-7990/acfd67
Zhuo Li, Feng Jiang, Zhengyi Jiang, Zige Tian, Tian Qiu, Tao Zhang, Qiuling Wen, Xizhao Lu, Jing Lu, Hui Huang
Abstract Diamond is a highly valuable material with diverse industrial applications, particularly in the fields of semiconductor, optics, and high-power electronics. However, its high hardness and chemical stability make it difficult to realize high-efficiency and ultra-low damage machining of diamond. To address these challenges, several polishing methods have been developed for both single crystal diamond (SCD) and polycrystalline diamond (PCD), including mechanical, chemical, laser, and ion beam processing methods. In this review, the characteristics and application scope of various polishing technologies for SCD and PCD are highlighted. Specifically, various energy beam-based direct and assisted polishing technologies, such as laser polishing, ion beam polishing, plasma-assisted polishing, and laser-assisted polishing, are summarized. The current research progress, material removal mechanism, and influencing factors of each polishing technology are analyzed. Although some of these methods can achieve high material removal rates or reduce surface roughness, no single method can meet all the requirements. Finally, the future development prospects and application directions of different polishing technologies are presented.
金刚石是一种极具价值的材料,具有多种工业用途,特别是在半导体、光学和大功率电子领域。然而,金刚石的高硬度和化学稳定性使其难以实现高效、超低损伤加工。为了解决这些挑战,针对单晶金刚石(SCD)和多晶金刚石(PCD)开发了几种抛光方法,包括机械、化学、激光和离子束加工方法。本文综述了SCD和PCD各种抛光技术的特点和应用范围。详细介绍了激光抛光、离子束抛光、等离子体辅助抛光、激光辅助抛光等基于能量束的直接抛光和辅助抛光技术。分析了各种抛光技术的研究现状、材料去除机理及影响因素。虽然其中一些方法可以实现高材料去除率或降低表面粗糙度,但没有一种方法可以满足所有要求。最后,对不同抛光技术的发展前景和应用方向进行了展望。
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引用次数: 0
Advances in Memristor Based Artificial Neuron Fabrication-Materials, Models, and Applications 基于忆阻器的人工神经元制造研究进展——材料、模型和应用
1区 工程技术 Q1 ENGINEERING, MANUFACTURING Pub Date : 2023-10-09 DOI: 10.1088/2631-7990/acfcf1
Jingyao Bian, Zhiyong Liu, Ye Tao, zhongqiang Wang, Xiaoning Zhao, Ya Lin, Haiyang Xu, Yichun Liu
Abstract Spiking neural network (SNN), widely known as the third-generation neural network, has been frequently investigated due to its excellent spatiotemporal information processing capability, high biological plausibility, and low energy consumption characteristics. Analogous to the working mechanism of human brain, the SNN system transmits information through the spiking action of neurons. Therefore, artificial neurons are critical building blocks for constructing SNN in hardware. Memristors are drawing growing attention due to low consumption, high speed, and nonlinearity characteristics, which are recently introduced to mimic the functions of biological neurons. Researchers have proposed multifarious memristive materials including organic materials, inorganic materials, or even two-dimensional materials. Taking advantage of the unique electrical behavior of these materials, several neuron models are successfully implemented, such as Hodgkin–Huxley model, leaky integrate-and-fire model and integrate-and-fire model. In this review, the recent reports of artificial neurons based on memristive devices are discussed. In addition, we highlight the models and applications through combining artificial neuronal devices with sensors or other electronic devices. Finally, the future challenges and outlooks of memristor-based artificial neurons are discussed, and the development of hardware implementation of brain-like intelligence system based on SNN is also prospected.
摘要:脉冲神经网络(SNN)被称为第三代神经网络,因其具有优异的时空信息处理能力、高生物可信度和低能耗等特点而受到人们的广泛关注。SNN系统与人脑的工作机制类似,通过神经元的尖峰作用传递信息。因此,人工神经元是在硬件上构建SNN的关键组成部分。记忆电阻器以其低功耗、高速度、非线性等特点,近年来被广泛应用于模拟生物神经元的功能,受到越来越多的关注。研究人员提出了多种记忆材料,包括有机材料,无机材料,甚至二维材料。利用这些材料独特的电行为,成功地实现了几种神经元模型,如霍奇金-赫胥黎模型、泄漏集成-发射模型和集成-发射模型。本文综述了近年来基于忆阻装置的人工神经元的研究进展。此外,我们还重点介绍了人工神经元设备与传感器或其他电子设备相结合的模型和应用。最后,讨论了基于忆阻器的人工神经元未来面临的挑战和发展前景,并对基于SNN的类脑智能系统的硬件实现进行了展望。
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引用次数: 0
Two-Photon Polymerization-Based 4D Printing and Its Applications 基于双光子聚合的4D打印及其应用
1区 工程技术 Q1 ENGINEERING, MANUFACTURING Pub Date : 2023-10-06 DOI: 10.1088/2631-7990/acfc03
Bingcong Jian, Honggeng Li, Xiangnan He, Rong Wang, Hui Ying Yang, Qi Ge
Abstract Two-photon polymerization (TPP) is a cutting-edge micro/nanoscale three-dimensional (3D) printing technology based on the principle of two-photon absorption. TPP surpasses the diffraction limit in achieving feature sizes and excels in fabricating intricate 3D micro/nanostructures with exceptional resolution. The concept of 4D entails the fabrication of structures utilizing smart materials capable of undergoing shape, property, or functional changes in response to external stimuli over time. The integration of TPP and 4D printing introduces the possibility of producing responsive structures with micro/nanoscale accuracy, thereby enhancing the capabilities and potential applications of both technologies. This paper comprehensively reviews TPP-based 4D printing technology and its diverse applications. First, the working principles of TPP and its recent advancements are introduced. Second, the optional 4D printing materials suitable for fabrication with TPP are discussed. Finally, this review paper highlights several noteworthy applications of TPP-based 4D printing, including domains such as biomedical microrobots, bioinspired microactuators, autonomous mobile microrobots, transformable devices and robots, as well as anti-counterfeiting microdevices. In conclusion, this paper provides valuable insights into the current status and future prospects of TPP-based 4D printing technology, thereby serving as a guide for researchers and practitioners.
摘要双光子聚合(TPP)是一种基于双光子吸收原理的前沿微/纳米三维(3D)打印技术。TPP在实现特征尺寸方面超越了衍射极限,并且在制造复杂的3D微/纳米结构方面具有卓越的分辨率。4D的概念需要利用智能材料制造结构,这些材料能够随着时间的推移响应外部刺激而发生形状、属性或功能变化。TPP和4D打印的整合引入了生产具有微/纳米级精度的响应结构的可能性,从而增强了这两种技术的能力和潜在应用。本文全面综述了基于tpp的4D打印技术及其多种应用。首先,介绍了TPP的工作原理及其最新进展。其次,讨论了适用于TPP制造的可选4D打印材料。最后,本文重点介绍了基于tpp的4D打印的几个值得注意的应用,包括生物医学微型机器人、仿生微致动器、自主移动微型机器人、可变形设备和机器人以及防伪微型设备等领域。综上所述,本文对基于tpp的4D打印技术的现状和未来前景提供了有价值的见解,对研究人员和从业者具有指导意义。
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引用次数: 0
Electrically-driven ultrafast out-of-equilibrium light emission from hot electrons in suspended graphene/hBN heterostructures 悬浮石墨烯/hBN异质结构中热电子的超快非平衡发光
1区 工程技术 Q1 ENGINEERING, MANUFACTURING Pub Date : 2023-10-03 DOI: 10.1088/2631-7990/acfbc2
Qiang Liu, Wei Xu, Xiaoxi Li, Tongyao Zhang, Chengbing Qin, Fang Luo, Zhihong Zhu, Shiqiao Qin, Mengjian Zhu, Kostya S. Novoselov
Abstract Nanoscale light sources with high speed of electrical modulation and low energy consumption are key components for nanophotonics and optoelectronics. The record-high carrier mobility and ultrafast carrier dynamics of graphene make it promising as an atomically thin light emitter, which can be further integrated into arbitrary platforms by van der Waals forces. However, due to the zero bandgap, graphene is difficult to emit light through the interband recombination of carriers like conventional semiconductors. Here, we demonstrate ultrafast thermal light emitters based on suspended graphene/hexagonal boron nitride (Gr/hBN) heterostructures. Electrons in biased graphene are significantly heated up to 2800 K at modest electric fields, emitting bright photons from the near-infrared to the visible spectral range. By eliminating the heat dissipation channel of the substrate, the radiation efficiency of the suspended Gr/hBN device is about two orders of magnitude greater than that of graphene devices supported on SiO 2 or hBN. We further demonstrate that hot electrons and low-energy acoustic phonons in graphene are weakly coupled to each other and are not in full thermal equilibrium. Direct cooling of high-temperature hot electrons to low-temperature acoustic phonons is enabled by the significant near-field heat transfer at the highly localized Gr/hBN interface, resulting in ultrafast thermal emission with up to 1 GHz bandwidth under electrical excitation. It is found that suspending the Gr/hBN heterostructures on the SiO 2 trenches significantly modifies the light emission due to the formation of the optical cavity and showed a ∼440% enhancement in intensity at the peak wavelength of 940 nm compared to the black-body thermal radiation. The demonstration of electrically driven ultrafast light emission from suspended Gr/hBN heterostructures sheds the light on applications of graphene heterostructures in photonic integrated circuits, such as broadband light sources and ultrafast thermo-optic phase modulators.
具有高速电调制和低能耗的纳米光源是纳米光子学和光电子学的关键器件。石墨烯创纪录的高载流子迁移率和超快的载流子动力学特性使其成为一种极有前途的原子薄光发射器,可以通过范德华力进一步集成到任意平台上。然而,由于零带隙,石墨烯很难像传统半导体那样通过载流子的带间复合发光。在这里,我们展示了基于悬浮石墨烯/六方氮化硼(Gr/hBN)异质结构的超快热光源。偏置石墨烯中的电子在适度的电场下被显著加热到2800 K,从近红外到可见光谱范围内发射明亮的光子。通过消除衬底的散热通道,悬浮式Gr/hBN器件的辐射效率比在sio2或hBN上支撑的石墨烯器件高出约两个数量级。我们进一步证明了石墨烯中的热电子和低能声子彼此弱耦合,并且不是完全热平衡。在高度局域化的Gr/hBN界面上,通过显著的近场传热,高温热电子可以直接冷却到低温声子,从而在电激励下产生带宽高达1 GHz的超快热发射。研究发现,将Gr/hBN异质结构悬浮在sio2沟槽上,由于光学腔的形成,显著改变了光发射,与黑体热辐射相比,在940 nm峰值波长处的强度提高了约440%。悬浮Gr/hBN异质结构的电驱动超快光发射的演示,为石墨烯异质结构在光子集成电路中的应用提供了新的视角,如宽带光源和超快热光相位调制器。
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引用次数: 1
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International Journal of Extreme Manufacturing
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