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Extreme ultraviolet transient gratings 极紫外瞬态光栅
IF 6 2区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2023-06-26 DOI: 10.1080/23746149.2023.2220363
F. Bencivenga, F. Capotondi, L. Foglia, R. Mincigrucci, C. Masciovecchio
ABSTRACT The recent construction of free electron lasers allows extending laboratory-based laser experiments to shorter wavelengths, accessing wavevectors typical of nanoscale dynamics and adding element and chemical state specificity by exploiting electronic transitions from core levels. The high pulse energies available ensure that this new wavelength range can be advantageously used for nonlinear optics, as in the pioneering case of transient grating spectroscopy: a time-resolved four-wave mixing technique in which two pump pulses are crossed at the sample to generate a spatially periodic excitation whose dynamics is monitored via diffraction of a probe pulse. We will show how extreme ultraviolet photon pulses have been successfully deployed in the last seven years to carry out transient grating experiments, mainly performed at the FERMI free electron laser, addressing a variety of scientific questions, ranging from the study of thermal transport in semiconductors approaching the ballistic regime to the modelling of ultrafast demagnetization at the nanoscale. We will also discuss possible future developments of the transient grating method specifying the impact this could have in various fields of scientific research ranging from molecular chirality to spintronics.
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引用次数: 4
Atomic force microscopy and other scanning probe microscopy methods to study nanoscale domains in model lipid membranes 原子力显微镜和其他扫描探针显微镜方法研究模型脂质膜的纳米级结构域
IF 6 2区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2023-05-02 DOI: 10.1080/23746149.2023.2197623
Morgan Robinson, Carina T Filice, D. McRae, Z. Leonenko
ABSTRACT The cell membrane is a fundamental biological structure, which is only 6–10 nm thick. It is composed of hundreds of lipid types, which form small and dynamic lipid domains or rafts. These rafts are thought to be a major aspect of cell organization, to provide support for various transmembrane proteins and are central to the communication of cells with their environs. Understanding the functions of lipid rafts presents an exciting opportunity to understand the molecular mechanisms of biologically important processes, as well as to uncover fundamental molecular mechanisms of membrane-associated diseases. Due to the high complexity of cell membranes, model membranes composed of synthetic lipids have been developed and are widely used to mimic biomembranes in an effort to study the structure and dynamics of lipid domains and their role in cell function. Atomic force microscopy (AFM), Kelvin probe force microscopy (KPFM) and atomic force spectroscopy (AFS) significantly advanced the study of nanodomains in model lipid membranes and monolayers. We review applications of these methods to the study of model membranes, which are widely used to mimic eukaryotic and bacterial cells, as well as neuronal cellular membranes in Alzheimer’s disease (AD). Graphical Abstract
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引用次数: 1
On spatial beam self-cleaning from the perspective of optical wave thermalization in multimode graded-index fibers 从多模渐变折射率光纤中的光波热化角度看空间光束自清洁
IF 6 2区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2023-04-24 DOI: 10.1080/23746149.2023.2228018
M. Ferraro, F. Mangini, M. Zitelli, S. Wabnitz
The input power-induced transformation of the transverse intensity profile at the output of graded-index multimode optical fibers from speckles into a bell-shaped beam sitting on a low intensity background is known as spatial beam self-cleaning. Its remarkable properties are the output beam brightness improvement and robustness to fiber bending and squeezing. These properties permit to overcome the limitations of multimode fibers in terms of low output beam quality, which is very promising for a host of technological applications. In this review, we outline recent progress in the understanding of spatial beam self-cleaning, which can be seen as a state of thermal equilibrium in the complex process of modal four-wave mixing. In other words, the associated nonlinear redistribution of the mode powers which ultimately favors the fundamental mode of the fiber can be described in the framework of statistical mechanics applied to the gas of photons populating the fiber modes. On the one hand, this description has been corroborated by a series of experiments by different groups. On the other hand, some open issues still remain, and we offer a perspective for future studies in this emerging and controversial field of research.
梯度折射率多模光纤输出端的横向强度分布在低强度背景下从散斑到钟形光束的输入功率诱导转换称为空间光束自清洁。其显著的性能是提高了输出光束的亮度和抗光纤弯曲和挤压。这些特性允许克服多模光纤在低输出光束质量方面的限制,这对于许多技术应用是非常有前途的。在这篇综述中,我们概述了空间光束自清洁的最新进展,它可以被看作是模态四波混频复杂过程中的一种热平衡状态。换句话说,相关的模式功率的非线性再分布最终有利于光纤的基本模式,可以在应用于填充光纤模式的光子气体的统计力学框架中描述。一方面,这一描述已被不同小组的一系列实验所证实。另一方面,一些尚未解决的问题仍然存在,我们为这一新兴和有争议的研究领域的未来研究提供了一个视角。
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引用次数: 2
Opportunities in the design of metal@oxide core-shell nanoparticles metal@oxide核壳纳米颗粒设计的机遇
IF 6 2区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2023-02-28 DOI: 10.1080/23746149.2023.2175623
Paulo C. D. Mendes, Yizhen Song, Wenrui Ma, Terry Z. H. Gani, K. Lim, S. Kawi, S. Kozlov
ABSTRACT Nanoparticles composed of metallic cores encapsulated in oxide shells emerged in the last decade as an attractive class of nanocomposite materials due to their high stability and unique properties provided by the high contact area between the metal and oxide components. Diverse metal-oxide interactions in metal@oxide core@shell nanoparticles enable tuning their electronic structure, spectroscopic properties, and surface reactivity for applications in sensing, electrochemistry, batteries as well as thermal and photocatalysis. Herein, we review the recent literature on the synthesis, characterization, simulations, and applications of metal@oxide nanocomposites. In particular, we discuss how the properties of metal@oxide nanoparticles can be tuned for a given application by changing the size of the metal core, the thickness and porosity of the oxide shell, as well as their composition, e.g. by alloying the core or doping the shell. Understanding of structure-property relations in metal@oxide systems provides vast opportunities for the rational design of advanced metal@oxide nanocomposites, making this class of materials promising for a wide range of applications. Graphical abstract
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引用次数: 0
Quantum sensing and imaging with spin defects in hexagonal boron nitride 六方氮化硼中自旋缺陷的量子传感与成像
IF 6 2区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2023-02-22 DOI: 10.1080/23746149.2023.2206049
Sumukh Vaidya, Xingyu Gao, S. Dikshit, I. Aharonovich, Tongcang Li
Color centers in hexagonal boron nitride (hBN) have recently emerged as promising candidates for a new wave of quantum applications. Thanks to hBN's high stability and 2-dimensional (2D) layered structure, color centers in hBN can serve as robust quantum emitters that can be readily integrated into nanophotonic and plasmonic structures on a chip. More importantly, the recently discovered optically addressable spin defects in hBN provide a quantum interface between photons and electron spins for quantum sensing applications. The most well-studied hBN spin defects, the negatively charged boron vacancy ($V_B^-$) spin defects, have been used for quantum sensing of static magnetic fields, magnetic noise, temperature, strain, nuclear spins, paramagnetic spins in liquids, RF signals, and beyond. In particular, hBN nanosheets with spin defects can form van der Waals (vdW) heterostructures with 2D magnetic or other materials for in situ quantum sensing and imaging. This review summarizes the rapidly evolving field of nanoscale and microscale quantum sensing with spin defects in hBN. We introduce basic properties of hBN spin defects, quantum sensing protocols, and recent experimental demonstrations of quantum sensing and imaging with hBN spin defects. We also discuss methods to enhance their sensitivity. Finally, we envision some potential developments and applications of hBN spin defects.
六方氮化硼(hBN)中的色心最近成为新一轮量子应用的有希望的候选者。由于hBN的高稳定性和二维(2D)层状结构,hBN中的色心可以作为强大的量子发射器,可以很容易地集成到芯片上的纳米光子和等离子体结构中。更重要的是,最近在hBN中发现的光学可寻址自旋缺陷为量子传感应用提供了光子和电子自旋之间的量子界面。研究最深入的hBN自旋缺陷,带负电荷的硼空位($V_B^-$)自旋缺陷,已被用于静态磁场、磁噪声、温度、应变、核自旋、液体中的顺磁自旋、RF信号等的量子传感。特别是,具有自旋缺陷的hBN纳米片可以与2D磁性或其他材料形成范德华(vdW)异质结构,用于原位量子传感和成像。本文综述了hBN中自旋缺陷在纳米尺度和微尺度量子传感领域的快速发展。我们介绍了hBN自旋缺陷的基本性质、量子传感协议,以及最近利用hBN旋转缺陷进行量子传感和成像的实验演示。我们还讨论了提高其敏感性的方法。最后,我们展望了hBN自旋缺陷的一些潜在发展和应用。
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引用次数: 17
Background signals in stimulated Raman scattering microscopy and current solutions to avoid them 受激拉曼散射显微镜中的背景信号和避免它们的当前解决方案
IF 6 2区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2023-02-13 DOI: 10.1080/23746149.2023.2176258
L. Genchi, S. Laptenok, C. Liberale
ABSTRACT Stimulated Raman scattering (SRS) microscopy has gained popularity in recent years due to its linearity to molecule concentration and laser intensity, and to the lack of the nonresonant background that affects its analogous technique, coherent anti-Stokes Raman scattering. However, SRS is not a background-free technique. In fact, there are other optical processes – nonlinear transient scattering and nonlinear transient absorption – that can be detrimental to the contrast and sensitivity of SRS microscopy. In this review, we provide a description of these competing optical processes and present an up-to-date description of current solutions to minimize their effect on SRS measurements. Graphical Abstract
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引用次数: 2
Ultra-stable and versatile high-energy resolution setup for attosecond photoelectron spectroscopy 阿秒光电子能谱的超稳定和通用高能分辨率装置
IF 6 2区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2023-01-21 DOI: 10.1080/23746149.2023.2250105
Sizuo Luo, Robin Weissenbilder, H. Laurell, Mattias Ammitzböll, V'enus Poulain, D. Busto, Lana Neoričić, Chen Guo, S. Zhong, D. Kroon, R. Squibb, R. Feifel, M. Gisselbrecht, A. L’Huillier, C. Arnold
Attosecond photoelectron spectroscopy is often performed with interferometric experimental setups that require outstanding stability. We demonstrate and characterize in detail an actively stabilized, versatile, high spectral resolution attosecond beamline. The active-stabilization system can remain ultra-stable for several hours with an RMS stability of 13 as and a total pump-probe delay scanning range of sim 400 fs. A tunable femtosecond laser source to drive high-order harmonic generation allows for precisely addressing atomic and molecular resonances. Furthermore, the interferometer includes a spectral shaper in 4f-geometry in the probe arm as well as a tunable bandpass filter in the pump arm, which offer additional high flexibility in terms of tunability as well as narrowband or polychromatic probe pulses. We show that spectral phase measurements of photoelectron wavepackets with the rainbow RABBIT technique (reconstruction of attosecond beating by two photon transitions) with narrowband probe pulses can significantly improve the photoelectron energy resolution. In this setup, the temporal-spectral resolution of photoelectron spectroscopy can reach a new level of accuracy and precision.
阿秒光电子能谱通常使用需要卓越稳定性的干涉实验装置进行。我们详细展示并表征了一种主动稳定、通用、高光谱分辨率的阿秒光束线。主动稳定系统可以在几个小时内保持超稳定,RMS稳定性为13 as,总泵探头延迟扫描范围为sim 400 fs。驱动高次谐波产生的可调谐飞秒激光源可以精确寻址原子和分子共振。此外,干涉仪包括探针臂中4f几何形状的光谱整形器以及泵臂中的可调谐带通滤波器,其在可调谐性以及窄带或多色探针脉冲方面提供额外的高灵活性。我们表明,用彩虹RABIT技术(通过两光子跃迁重建阿秒拍频)和窄带探测脉冲对光电子波包的光谱相位测量可以显著提高光电子能量分辨率。在这种装置中,光电子能谱的时间光谱分辨率可以达到一个新的精度和精度水平。
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引用次数: 0
Atom electronics in single-molecule transistors: single-atom access and manipulation 单分子晶体管中的原子电子学:单原子存取和操纵
IF 6 2区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2023-01-15 DOI: 10.1080/23746149.2023.2165148
Y. Ouyang, Feng Wang, Minhao Zhang, Yuyuan Qin, Yuanzhi Tan, W. Ji, F. Song
ABSTRACT The aim of atom electronics, i.e. the final scale of electronics, is to make use of specific individual atoms as active electronic components. Here, we review recent researches on atom electronics in single-molecule transistors (SMTs) through single-atom access and manipulation. We begin by describing the basic concepts and characteristics of atom electronics in SMTs, before discussing some of the most recent examples, including atomic transistors and atomic storage. In our concluding remarks, we discuss some perspectives on fabrication, integration, and other potential atomic devices in which high precision access to, and manipulation of single atoms could be of great significance. This will affect integrated circuits, quantum computing, and other devices that will drive the electronics of the future. Graphical abstract
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引用次数: 0
Spin injection, relaxation, and manipulation in GaN-based semiconductors 氮化镓基半导体中的自旋注入、弛豫和操纵
IF 6 2区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2023-01-12 DOI: 10.1080/23746149.2022.2158757
Zhenhao Sun, N. Tang, Shixiong Zhang, Shuai Chen, Xingchen Liu, B. Shen
ABSTRACT GaN-based semiconductors are deemed to be a potential candidate for developing spintronic devices owing to the artificially controllable spin-orbit coupling and the high Curie temperature of GaN-based diluted magnetic semiconductors. Spin injection, spin relaxation dynamics, and spin manipulation are the key issues in the development of GaN-based spintronic devices, which have been reviewed in this article. In the end, a brief section presents the research progress of GaN-based spintronic devices. Graphical Abstract
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引用次数: 0
Quantum machine learning: from physics to software engineering 量子机器学习:从物理学到软件工程
IF 6 2区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2023-01-04 DOI: 10.1080/23746149.2023.2165452
A. Melnikov, Mohammad Kordzanganeh, A. Alodjants, R. Lee
Quantum machine learning is a rapidly growing field at the intersection of quantum technology and artificial intelligence. This review provides a two-fold overview of several key approaches that can offer advancements in both the development of quantum technologies and the power of artificial intelligence. Among these approaches are quantum-enhanced algorithms, which apply quantum software engineering to classical information processing to improve keystone machine learning solutions. In this context, we explore the capability of hybrid quantum-classical neural networks to improve model generalization and increase accuracy while reducing computational resources. We also illustrate how machine learning can be used both to mitigate the effects of errors on presently available noisy intermediate-scale quantum devices, and to understand quantum advantage via an automatic study of quantum walk processes on graphs. In addition, we review how quantum hardware can be enhanced by applying machine learning to fundamental and applied physics problems as well as quantum tomography and photonics. We aim to demonstrate how concepts in physics can be translated into practical engineering of machine learning solutions using quantum software.
量子机器学习是量子技术和人工智能交叉的一个快速发展的领域。这篇综述对几种关键方法进行了双重概述,这些方法可以在量子技术的发展和人工智能的力量方面取得进展。这些方法包括量子增强算法,它将量子软件工程应用于经典信息处理,以改进关键的机器学习解决方案。在这种背景下,我们探索了混合量子经典神经网络在减少计算资源的同时提高模型泛化能力和准确性的能力。我们还说明了如何使用机器学习来减轻误差对目前可用的有噪声的中等规模量子设备的影响,并通过图上量子行走过程的自动研究来理解量子优势。此外,我们还回顾了如何通过将机器学习应用于基础和应用物理问题以及量子断层扫描和光子学来增强量子硬件。我们旨在展示如何使用量子软件将物理学中的概念转化为机器学习解决方案的实际工程。
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引用次数: 22
期刊
Advances in Physics: X
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