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An upconversion device based on high-performance dual-layer white organic electroluminescent devices 基于高性能双层白色有机电致发光器件的上转换装置
IF 1.6 4区 物理与天体物理 Q4 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-09-06 DOI: 10.1063/5.0222205
Weigao Wang, Yiyang Li, Yili Wan, Yu Duan, Hua An, Zhengchun Peng
Large-area imaging techniques in the short-wave infrared spectral region remain a pressing need. Organic light-emitting diodes and infrared photodetectors can be combined to form a near-infrared (NIR) to visible upconversion device, which has great potential to replace traditional infrared imaging systems. The integration of a white organic light-emitting diode (WOLED) with infrared photodetectors has become essential to realize full-color displays for its simple preparation process and high compatibility. This work has designed and optimized a WOLED to achieve stable emission with high brightness (19 470 cd m−2) and high external quantum efficiency (EQE = 18.08%) at a wide voltage range, thereby reducing chromaticity drift caused by voltage fluctuations. Moreover, photon-generated holes in the NIR-sensitive photodetector are able to inject into the WOLED for visible light emission. Consequently, we have obtained a high-performance upconversion device with a luminance on-off ratio exceeding 5 × 103 at 850 nm NIR and a high color stability over a wide range of operating voltage. Our efforts have accomplished a high-performance upconversion device from NIR to white visible light, laying the groundwork for a preliminary exploration of full-color displays.
短波红外光谱区的大面积成像技术仍是一项迫切需要。有机发光二极管和红外光电探测器可以组合成近红外到可见光的上转换器件,这在取代传统红外成像系统方面具有巨大潜力。白光有机发光二极管(WOLED)与红外光电探测器的集成因其制备工艺简单、兼容性强而成为实现全彩显示的关键。这项研究对 WOLED 进行了设计和优化,使其在宽电压范围内实现高亮度(19 470 cd m-2)和高外部量子效率(EQE = 18.08%)的稳定发射,从而减少了电压波动引起的色度漂移。此外,近红外敏感光电探测器中光子产生的空穴能够注入 WOLED,从而发射可见光。因此,我们获得了一种高性能的上转换器件,其在 850 纳米近红外波段的亮度开关比超过 5 × 103,并且在宽工作电压范围内具有很高的色彩稳定性。我们的努力实现了从近红外到白色可见光的高性能上转换器件,为全彩显示的初步探索奠定了基础。
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引用次数: 0
Improved sensitivity for subsurface imaging by contact resonance atomic force microscopy using Fano peaks 利用法诺峰提高接触共振原子力显微镜表面下成像的灵敏度
IF 1.6 4区 物理与天体物理 Q4 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-09-06 DOI: 10.1063/5.0219230
Yuyang Wang, Mingyu Duan, Yuan-Liu Chen
Subsurface detection using contact resonance atomic force microscopy (CR-AFM) has been well-documented and proven capable of nondestructively detecting subsurface defects at depths of hundreds of nanometers. In CR-AFM, the frequency of the contact resonance mode is often used as the actuating frequency of the probe. However, as many frequencies are available in the probe’s vibrational spectrum, each with a significant impact on the final measurement result, a focused study on frequency selection is necessary. This paper investigates contact resonance peaks through theoretical modeling and experimental verification. The peaks were categorized into two types based on their symmetry. Comparative studies were conducted on the traditionally used symmetric resonance peaks and the less-studied asymmetric resonance peaks. The results reveal the detection capability for subsurface measurements due to different peak selections, identifying the peak types most suitable for these measurements. This study demonstrates that using Fano peaks in CR-AFM can enhance subsurface imaging resolution and reduce surface damage, making it a valuable technique for detailed nanoscale analysis.
使用接触共振原子力显微镜(CR-AFM)进行次表层检测已得到充分证实,并证明能够无损检测数百纳米深度的次表层缺陷。在 CR-AFM 中,接触共振模式的频率通常用作探头的驱动频率。然而,由于探头的振动频谱中有许多频率,每个频率都会对最终测量结果产生重大影响,因此有必要对频率选择进行重点研究。本文通过理论建模和实验验证研究了接触共振峰。根据峰的对称性将其分为两种类型。对传统上使用的对称共振峰和研究较少的非对称共振峰进行了比较研究。结果揭示了不同峰值选择对地下测量的探测能力,确定了最适合这些测量的峰值类型。这项研究表明,在 CR-AFM 中使用法诺峰可提高次表层成像分辨率并减少表面损伤,使其成为进行详细纳米尺度分析的重要技术。
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引用次数: 0
An experimental study of the impact of various infill parameters on the compressive strength of 3D printed PETG/CF 各种填充参数对 3D 打印 PETG/CF 抗压强度影响的实验研究
IF 1.6 4区 物理与天体物理 Q4 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-09-06 DOI: 10.1063/5.0212544
Shashwath Patil, T. Sathish, Jayant Giri, Bassem F. Felemban
This study examines the effect of different infill patterns and percentages on the compressive strength attributes of carbon fiber-reinforced PETG samples printed using fused deposition modeling, employing response surface methodology. Carbon fiber-enhanced PETG (polyethylene terephthalate glycol) composites represent a cutting-edge advancement in additive manufacturing, drawing significant interest due to their impressive mechanical attributes. The experimentation involves modifying printing parameters such as the infill pattern (tri-hexagon, cubic, or line) and infill density (40%, 60%, and 80%). These parameter values were obtained through a central composite experimental design utilizing response surface methodology. The compressive strength of the 3D-printed carbon fiber-reinforced PETG specimens is assessed following ASTM D695 standards. Research indicates that increasing the density of the infill results in enhanced compressive strength. Specifically, specimens featuring an 80% infill density with a tri-hexagon pattern demonstrate a notable compressive strength of 39.16 MPa. By employing regression analysis and optimization techniques, the study predicts experimental outcomes accurately. These findings offer valuable insights into refining the manufacturing process of carbon fiber-reinforced PETG components. This advancement holds potential benefits across various engineering fields, particularly in automotive and aerospace industries, where strength and durability are essential.
本研究采用响应面方法,研究了不同填充模式和百分比对使用熔融沉积模型打印的碳纤维增强 PETG 样品抗压强度属性的影响。碳纤维增强 PETG(聚对苯二甲酸乙二酯)复合材料代表了增材制造领域的前沿进展,因其令人印象深刻的机械属性而备受关注。实验涉及修改打印参数,如填充图案(三六边形、立方体或直线)和填充密度(40%、60% 和 80%)。这些参数值是利用响应面方法,通过中心复合实验设计获得的。3D 打印碳纤维增强 PETG 试样的抗压强度按照 ASTM D695 标准进行评估。研究表明,增加填充密度可提高抗压强度。具体来说,填充密度为 80% 的三六边形试样的抗压强度高达 39.16 兆帕。通过采用回归分析和优化技术,该研究准确地预测了实验结果。这些发现为完善碳纤维增强 PETG 组件的制造工艺提供了宝贵的见解。这一进步有望惠及各个工程领域,尤其是对强度和耐用性要求极高的汽车和航空航天领域。
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引用次数: 0
Opportunities and challenges of bamboo fiber composites in additive manufacturing: A comprehensive review 竹纤维复合材料在增材制造中的机遇与挑战:综述
IF 1.6 4区 物理与天体物理 Q4 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-09-06 DOI: 10.1063/5.0227267
Muthuselvan Balasubramanian, R. Saravanan, T. Sathish, Jayant Giri, Rustem Zairov, S. M. Mozammil Hasnain, Rakhymzhan Turmanov
This study explores the transformative impact of three-dimensional printing, or additive manufacturing, in the development of bamboo-based 3D printing parts. Recently, there has been growing interest in incorporating natural fibers, such as bamboo, into polymers to enhance the structural integrity and strength of 3D-printed polymeric materials. This paper thoroughly examines the opportunities and obstacles associated with using additive manufacturing techniques to print bamboo fiber composites. This study includes an analysis of the mechanical properties, thermal properties, biodegradability, and environmental benefits of bamboo fiber composites. It also covers the processing methods and the printing parameters of bamboo fiber composites. This paper review focuses on the future prospects of bamboo fiber composites as a sustainable material in additive manufacturing based on the analysis of the existing literature and the recent research developments.
本研究探讨了三维打印或增材制造在开发以竹子为基础的三维打印部件方面的变革性影响。最近,人们越来越关注将竹子等天然纤维融入聚合物中,以增强三维打印聚合物材料的结构完整性和强度。本文深入研究了使用增材制造技术打印竹纤维复合材料的相关机遇和障碍。本研究包括对竹纤维复合材料的机械性能、热性能、生物降解性和环境效益的分析。研究还包括竹纤维复合材料的加工方法和打印参数。本文在分析现有文献和最新研究进展的基础上,重点探讨了竹纤维复合材料作为可持续材料在增材制造中的应用前景。
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引用次数: 0
Comprehensive device modeling and performance analysis of (Cs, FA)Pb(I, Br)3 based perovskite–silicon tandem solar cells 基于(Cs, FA)Pb(I, Br)3的过氧化物硅串联太阳能电池的综合器件建模和性能分析
IF 1.6 4区 物理与天体物理 Q4 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-09-06 DOI: 10.1063/5.0225140
Zhenhui Wu, Zhaoyao Pan, Jinpeng Yang
The utilization of perovskite films as the top subcell to form a perovskite–silicon tandem solar cell has emerged as an attractive approach to achieve higher power conversion efficiency (PCE) that could surpass the Shockley–Queisser limit for single silicon junction. Despite these efforts, precisely understanding and predicting the underlying mechanism necessary for obtaining higher PCE remains a challenging task. In particular, the absorption due to back electrode reflection during calculations has often been neglected, resulting in an underestimation when comparing theoretical calculations to experimental conditions. In this study, we conduct a comprehensive investigation of perovskite–silicon tandem solar cells with considering the back electrode reflection to study the detailed influence on film quality of perovskite films, where a detailed analysis of multiple factors such as bulk and interface defects, doping levels, and carrier mobility from (Cs, FA)Pb(I, Br)3 has been conducted to unveil their effects on device performance. Our results revealed that lower bulk/interface defect concentrations and higher carrier mobility are critical factors contributing to the best device performance, where the highest PCE would reach up to 37.40%. Further comparison with experimental results also confirms the importance of employing effective methods to reduce surface/interface trap densities in order to enhance overall performance. These findings offer valuable theoretical insights for the guidance of experimental designs of perovskite–silicon tandem solar cells.
利用包晶体薄膜作为顶部子电池来形成包晶体-硅串联太阳能电池,已成为实现更高功率转换效率(PCE)的一种极具吸引力的方法,其功率转换效率可超过单晶硅结的肖克利-奎塞尔极限。尽管做出了这些努力,但准确理解和预测获得更高的 PCE 所必需的基本机制仍然是一项具有挑战性的任务。特别是在计算过程中,背电极反射引起的吸收往往被忽视,导致理论计算与实验条件比较时出现低估。在本研究中,我们对透辉石-硅串联太阳能电池进行了全面研究,考虑到背电极反射对透辉石薄膜质量的详细影响,详细分析了(Cs, FA)Pb(I, Br)3的体缺陷和界面缺陷、掺杂水平和载流子迁移率等多种因素,以揭示它们对器件性能的影响。我们的研究结果表明,较低的块体/界面缺陷浓度和较高的载流子迁移率是获得最佳器件性能的关键因素,最高 PCE 可达到 37.40%。与实验结果的进一步比较也证实了采用有效方法降低表面/界面陷阱密度以提高整体性能的重要性。这些发现为指导过氧化物硅串联太阳能电池的实验设计提供了宝贵的理论依据。
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引用次数: 0
Efficient method for twist-averaged coupled cluster calculation of gap energy: Bulk study of stannic oxide 捻平均耦合簇计算间隙能的高效方法:氧化锡的块体研究
IF 1.6 4区 物理与天体物理 Q4 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-09-05 DOI: 10.1063/5.0212542
Maliheh Shaban Tameh, Wayne L. Gladfelter, Jason D. Goodpaster
We study the gap energy of the semiconducting oxide SnO2 through ab initio calculations including both density functional theory (DFT) and coupled cluster methods. The effectiveness of twist averaging in reducing finite-size errors is evaluated across different functionals. We report an overestimation of gap energy when applying finite-size scaling to reach the thermodynamic limit in equation-of-motion (EOM) CCSD calculations. To mitigate one-body and many-body errors, we integrate twist averaging with a post-processing correction mechanism that compares finite-size and infinite-size DFT calculations using hybrid functionals. While inspired by the Kwee, Zhang, and Krakauer approach, our method is specifically tailored to hybrid functionals for a more accurate treatment of exchange-correlation effects. Our approach ensures that the many-body interactions are accurately captured in the estimated gap for an infinite system. We introduce unique single twist angles that provide cost-effective and accurate energies compared to to full twist averaging in EOM-CCSD calculations. Applying this approach to SnO2, we calculate a fundamental gap of 3.46 eV, which closely matches the 3.59 eV gap obtained from two-photon spectroscopy experiments, demonstrating the accuracy of this method.
我们通过包括密度泛函理论(DFT)和耦合簇方法在内的原子序数计算研究了半导体氧化物 SnO2 的间隙能。在不同的函数中,我们评估了扭转平均法在减少有限尺寸误差方面的有效性。我们报告了在运动方程 (EOM) CCSD 计算中应用有限尺寸缩放以达到热力学极限时对间隙能的高估。为了减轻单体和多体误差,我们将扭转平均与后处理校正机制结合起来,利用混合函数比较有限尺寸和无限尺寸 DFT 计算。虽然受到 Kwee、Zhang 和 Krakauer 方法的启发,但我们的方法是专门为混合函数定制的,以便更准确地处理交换相关效应。我们的方法确保在无限系统的估计间隙中准确捕捉多体相互作用。我们引入了独特的单扭曲角,与 EOM-CCSD 计算中的全扭曲平均相比,它能提供经济高效的精确能量。将这种方法应用于二氧化锡,我们计算出的基本间隙为 3.46 eV,这与双光子光谱实验获得的 3.59 eV 间隙非常接近,证明了这种方法的准确性。
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引用次数: 0
Optimizing process parameters to minimize wear-induced material loss in bronze-based hybrid metal matrix composites using the Taguchi method 利用田口方法优化工艺参数,最大限度地降低铜基混合金属基复合材料的磨损引起的材料损耗
IF 1.6 4区 物理与天体物理 Q4 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-09-05 DOI: 10.1063/5.0203081
Sreenivasa R., Ramesh B. T., Jayant Giri, Mohammad Khalid Al-Sadoon, Arun Kumar Bongale, T. Sathish, Ashok R. Banagar
Metal matrix composites have captured considerable interest in tribological applications, largely owing to their remarkable characteristics, which include a high strength-to-weight ratio and a low wear rate. This investigation delves into the exploration of hybrid metal matrix composites, where cobalt and chromium play the role of reinforcing agents within a bronze foundation. These composites were manufactured through a powder metallurgy process, utilizing cobalt and chromium metal powders with a particle size of 40 μm. Various weight percentage ratios (2.5%, 5.0%, and 7.5%) were utilized to create these composite specimens. To assess their tribological performance, the composite samples were subjected to a sliding wear test using a pin on disk machine, following the ASTM G99 standards. The wear characteristics of these composites were analyzed using the Taguchi method, considering parameters such as the applied load, speed, reinforcement percentage, and sliding distance. In addition, we conducted an analysis of variance on the collected data. To analyze the wear behavior of these hybrid metal matrix composites based on bronze, we utilized both multiple linear regression analysis and a signal-to-noise ratio assessment. The results indicate that the inclusion of cobalt and chromium metal powders as reinforcement materials enhances the tribological properties of the bronze matrix material.
金属基复合材料在摩擦学应用中备受关注,这主要归功于其卓越的特性,包括高强度重量比和低磨损率。本研究深入探讨了混合金属基复合材料,其中钴和铬在青铜基底中扮演了增强剂的角色。这些复合材料是通过粉末冶金工艺制造的,使用的是粒径为 40 μm 的钴和铬金属粉末。这些复合材料试样采用了不同的重量百分比率(2.5%、5.0% 和 7.5%)。为了评估其摩擦学性能,复合材料试样按照 ASTM G99 标准,使用圆盘销钉机进行了滑动磨损测试。我们采用田口方法分析了这些复合材料的磨损特性,并考虑了施加载荷、速度、增强百分比和滑动距离等参数。此外,我们还对收集到的数据进行了方差分析。为了分析这些基于青铜的混合金属基复合材料的磨损行为,我们采用了多元线性回归分析和信噪比评估。结果表明,加入钴和铬金属粉末作为增强材料可提高青铜基体材料的摩擦学性能。
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引用次数: 0
Active damping for acoustic levitation in air 空气中声学悬浮的主动阻尼
IF 1.6 4区 物理与天体物理 Q4 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-09-05 DOI: 10.1063/5.0210800
Vincent Bos, Jasper Wesselingh, Gerard J. Verbiest, Peter G. Steeneken
Acoustic levitation is an attractive and versatile technique that offers several advantages in terms of particle size, range, reconfigurability, and ease of use with respect to alternative levitating techniques. In this paper, we study the use of active damping to improve the response time and positioning precision of an acoustic levitator operating in air. We use a laser Doppler vibrometer to measure the velocity of a levitated particle. Using this information, a control algorithm is designed and implemented to provide active damping. By system identification and modeling, we demonstrate that the active damper mechanism is well-predictable by models and can be electronically reconfigured and controlled.
与其他悬浮技术相比,声学悬浮是一种极具吸引力的多功能技术,在粒度、范围、可重构性和易用性方面具有多项优势。在本文中,我们研究了如何利用主动阻尼来改善空气中声学悬浮器的响应时间和定位精度。我们使用激光多普勒测振仪测量悬浮粒子的速度。利用这一信息,我们设计并实施了一种控制算法,以提供主动阻尼。通过系统识别和建模,我们证明主动阻尼器机制可以通过模型很好地预测,并且可以通过电子方式重新配置和控制。
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引用次数: 0
A high-efficiency tunable relativistic magnetron with diffraction output 具有衍射输出的高效可调相对论磁控管
IF 1.6 4区 物理与天体物理 Q4 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-09-05 DOI: 10.1063/5.0230930
Kunpeng Chen, Haodong Xu, Zeyang Liu, Yuwei Fan
In this paper, a high-efficiency tunable relativistic magnetron with diffraction output (HTRMDO) is presented and studied numerically. To increase the tuning bandwidth and power efficiency, the outer radius of the resonant cavity and the magnetic field are simultaneously varied. The simulation results show that the HTRMDO has a tuning range between 1.280 and 2.430 GHz, corresponding to a tuning bandwidth of 62.0% with a center frequency of 1.855 GHz. In the tuning range, the maximum power efficiency is 71.9% and the minimum power efficiency is 36.0%, which complies with the 3 dB principle. Moreover, its output mode remains constant as TE31. This is a record tuning bandwidth and power efficiency for the continuously tunable relativistic magnetron.
本文介绍了一种具有衍射输出的高效可调相对论磁控管(HTRMDO),并对其进行了数值研究。为了提高调谐带宽和功率效率,谐振腔的外半径和磁场同时变化。仿真结果表明,HTRMDO 的调谐范围在 1.280 至 2.430 GHz 之间,调谐带宽为 62.0%,中心频率为 1.855 GHz。在调谐范围内,最大功率效率为 71.9%,最小功率效率为 36.0%,符合 3 dB 原则。此外,其输出模式恒定为 TE31。这是连续可调相对论磁控管在调谐带宽和功率效率方面的最高纪录。
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引用次数: 0
Preparation of polymer composites with electrostatic spinning promotes wound regeneration: A review 用静电纺丝法制备聚合物复合材料可促进伤口再生:综述
IF 1.6 4区 物理与天体物理 Q4 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-09-05 DOI: 10.1063/5.0215772
Wanying Yang, Cong Yang, Guanghui Jing, Sen Wang, Jing Li, Xiaonan Zhang, Peng Liu, Ning Yu
Wound dressings play a critical role in promoting healing by protecting wounds from external contaminants and providing an optimal environment for tissue regeneration. Traditional dressings, such as gauze and cotton, offer basic physical barriers but lack the ability to maintain a moist wound environment, which is essential for healing. Modern dressings, particularly those incorporating electrospun nanofibers, have emerged as advanced solutions that can sustain moisture, absorb exudate, and support cell growth and migration. This Review covers recent advances in electrospinning technologies and the design of composite materials that integrate natural and synthetic polymers, bioactive agents, and nanomaterials to enhance wound healing. In addition, it highlights key studies demonstrating the efficacy of these composites in various wound models. The primary objective of this Review is to inspire and guide future research endeavors, address existing limitations, and shed light on the promising research prospects in the field of wound healing and tissue regeneration.
伤口敷料在促进伤口愈合方面起着至关重要的作用,它可以保护伤口免受外部污染物的侵袭,并为组织再生提供最佳环境。传统的敷料,如纱布和棉布,可提供基本的物理屏障,但缺乏维持伤口湿润环境的能力,而这对伤口愈合至关重要。现代敷料,尤其是含有电纺纳米纤维的敷料,已经成为一种先进的解决方案,可以保持湿度、吸收渗出物、支持细胞生长和迁移。本综述介绍了电纺技术和复合材料设计的最新进展,这些材料融合了天然和合成聚合物、生物活性剂和纳米材料,可促进伤口愈合。此外,它还重点介绍了在各种伤口模型中证明这些复合材料功效的主要研究。本综述的主要目的是启发和指导未来的研究工作,解决现有的局限性,并阐明伤口愈合和组织再生领域大有可为的研究前景。
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引用次数: 0
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