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Cosmology Due to Thermodynamics of Apparent Horizon 视界热力学下的宇宙学
IF 2.5 4区 物理与天体物理 Q2 PHYSICS, MULTIDISCIPLINARY Pub Date : 2025-08-25 DOI: 10.1002/andp.202500204
S. I. Kruglov
<p>This study proposes new entropy of the apparent horizon <span></span><math> <semantics> <mrow> <msub> <mi>S</mi> <mi>h</mi> </msub> <mo>=</mo> <mrow> <mo>(</mo> <mn>1</mn> <mo>/</mo> <mi>β</mi> <mo>)</mo> </mrow> <mo>arctan</mo> <mrow> <mo>(</mo> <mi>β</mi> <msub> <mi>S</mi> <mrow> <mi>B</mi> <mi>H</mi> </mrow> </msub> <mo>)</mo> </mrow> </mrow> <annotation>$S_h=(1/beta)arctan (beta S_{BH})$</annotation> </semantics></math>, where <span></span><math> <semantics> <msub> <mi>S</mi> <mrow> <mi>B</mi> <mi>H</mi> </mrow> </msub> <annotation>$S_{BH}$</annotation> </semantics></math> is the Bekenstein–Hawking entropy. As parameter <span></span><math> <semantics> <mrow> <mi>β</mi> <mo>→</mo> <mn>0</mn> </mrow> <annotation>$beta rightarrow 0$</annotation> </semantics></math> one comes to the Bekenstein–Hawking entropy. This allows to consider the generalized Friedmann–Lemaître–Robertson–Walker (FLRW) equations for the barotropic matter fluid with <span></span><math> <semantics> <mrow> <mi>p</mi> <mo>=</mo> <mi>w</mi> <mi>ρ</mi> </mrow> <annotation>$p=wrho$</annotation> </semantics></math> for arbitrary equation of state parameter <span></span><math> <semantics> <mi>w</mi> <annotation>$w$</annotation> </semantics></math>. The modified Friedmann's equations are found. The addition term in the second modified Friedmann's equation plays the role of a dynamical cosmological constant. The dark energy density, pressure, and the deceleration parameter are found. It is shown that at some parameters <span></span><math> <semantics> <mi>w</mi> <annotation>$w$</annotation> </semantics></math> and <span></span><math> <semantics> <mi>β</
本文提出了视界S h = (1 / β) arctan (β)的新熵S B H) $S_h=(1/beta)arctan (beta S_{BH})$,S B H $S_{BH}$是贝肯斯坦-霍金熵。当参数β→0 $beta rightarrow 0$得到贝肯斯坦-霍金熵。这允许考虑具有p = w ρ $p=wrho$的正压流体对于任意状态参数w $w$方程的广义friedman - lemare - trer - robertson - walker (FLRW)方程。得到了修正后的弗里德曼方程。第二个修正的弗里德曼方程中的附加项起着动力学宇宙学常数的作用。得到了暗能量密度、压力和减速参数。结果表明,在某些参数w $w$和β $beta$下,可以得到两个阶段,加速和减速或永恒膨胀。利用全息原理所考虑的模型可以描述宇宙膨胀和宇宙加速的后期。因此,考虑了视界广义熵的全息暗能量模型。结果表明,基于该熵的熵宇宙学等价于基于F (T) $F(T)$函数的远平行引力宇宙学。基于广义熵的新宇宙学对于描述暴胀和宇宙演化的后期可能很有意义。
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引用次数: 0
Ionization Phase-Shifts Between Two Laser-Dressed States of Potassium Atoms 钾原子的两个激光修饰态之间的电离相移
IF 2.5 4区 物理与天体物理 Q2 PHYSICS, MULTIDISCIPLINARY Pub Date : 2025-08-23 DOI: 10.1002/andp.202500091
Wankai Li, Yixuan Wang, Xing Li, Tao Yang, Dongdong Zhang, Dajun Ding

Resonance-enhanced multiphoton ionization (REMPI) in potassium atom is investigated within the strong coupling regime using photoelectron momentum imaging techniques. The kinetic energy distribution of the ionized electrons reveals the eigenenergies of the dressed states, which exhibit Autler–Townes (AT) splitting. This splitting is proportional to the laser field strength. Partial wave analysis of the photoelectrons angular distributions (PAD) uncovers relative phase shifts between the dressed states, shedding light on attosecond ionization time delays. The observed phase shift between the two electron wave packets by the AT splitting arises from the combined effects of the Coulomb phase and the quantum defect phase.

利用光电子动量成像技术研究了强耦合条件下钾原子的共振增强多光子电离(REMPI)。电离电子的动能分布揭示了打扮态的本征能,表现为奥特勒-汤斯(Autler-Townes, AT)分裂。这种分裂与激光场强成正比。光电子角分布(PAD)的部分波分析揭示了修饰态之间的相对相移,揭示了阿秒电离时间延迟。通过AT分裂观察到的两个电子波包之间的相移是由库仑相和量子缺陷相的共同作用引起的。
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引用次数: 0
Refining Tc Prediction in Hydrides via Symbolic-Regression-Enhanced Electron-Localization-Function-Based Descriptors 基于符号回归增强的电子定位函数描述符改进氢化物中Tc的预测
IF 2.5 4区 物理与天体物理 Q2 PHYSICS, MULTIDISCIPLINARY Pub Date : 2025-08-22 DOI: 10.1002/andp.202500280
Francesco Belli, Sean Torres, Julia Contreras-García, Eva Zurek

Hydrogen-based materials are able to possess extremely high superconducting critical temperatures, Tcs$T_mathrm{c}{rm s}$, due to hydrogen's low atomic mass and strong electron–phonon interaction. Recently, a descriptor based on the Electron Localization Function (ELF) has enabled the rapid estimation of the Tc$T_mathrm{c}$ of hydrogen-containing compounds from electronic networking properties, but its applicability has been limited by the small size and homogeneity of the training dataset used. Herein, the model is re-examined, compiling a publicly available combined dataset of 244 binary and ternary hydride superconductors. The analysis shows that though ELF-based networking remains a valuable descriptor, its predictive power declines with increasing compositional complexity. However, by introducing the molecularity index, defined as the highest value of the ELF at which two hydrogen atoms connect, and applying symbolic regression, the accuracy of the predictions can be substantially enhanced. These results establish a more robust framework for assessing superconductivity in hydride materials, facilitating accelerated screening of novel candidates through integration with crystal structure prediction methods or high-throughput searches.

氢基材料由于氢的低原子质量和强电子-声子相互作用,能够具有极高的超导临界温度(tcs {c}{rm s}$)。最近,一种基于电子定位函数(ELF)的描述符已经能够从电子网络性质中快速估计含氢化合物的tc $T_ maththrm {c}$,但其适用性受到所用训练数据集的小尺寸和同质性的限制。在此,该模型被重新检验,编译了244个二元和三元氢化物超导体的公开组合数据集。分析表明,尽管基于elf的网络仍然是一个有价值的描述符,但其预测能力随着组合复杂性的增加而下降。然而,通过引入分子指数(定义为两个氢原子连接时的极低频最高值)并应用符号回归,可以大大提高预测的准确性。这些结果为评估氢化物材料的超导性建立了一个更强大的框架,通过与晶体结构预测方法或高通量搜索的结合,促进了新的候选材料的加速筛选。
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引用次数: 0
Two-Band Superconductivity and Transition Temperature Limited by Thermal Fluctuations in Ruddlesden–Popper Nickelates at Ambient and High Pressures Ruddlesden-Popper镍酸盐在环境和高压下的双带超导性和热波动限制的转变温度
IF 2.5 4区 物理与天体物理 Q2 PHYSICS, MULTIDISCIPLINARY Pub Date : 2025-08-20 DOI: 10.1002/andp.202500293
Evgeny F. Talantsev
<p>Recently, two research groups reported the observation of ambient-pressure superconductivity in few-nanometers-thick La<sub>3-x</sub>Pr<sub>x</sub>Ni<sub>2</sub>O<sub>7-δ</sub> (x = 0.0, 0.15, and 1.0) films with the onset transition temperature <span></span><math> <semantics> <mrow> <msub> <mi>T</mi> <mrow> <mi>c</mi> <mo>,</mo> <mi>o</mi> <mi>n</mi> <mi>s</mi> <mi>e</mi> <mi>t</mi> </mrow> </msub> <mo>≅</mo> <mn>40</mn> <mspace></mspace> <mi>K</mi> </mrow> <annotation>${{T}_{c,onset}} cong 40 {rm{K}}$</annotation> </semantics></math> and zero resistance temperature <span></span><math> <semantics> <mrow> <msub> <mi>T</mi> <mrow> <mi>c</mi> <mo>,</mo> <mi>z</mi> <mi>e</mi> <mi>r</mi> <mi>o</mi> </mrow> </msub> <mo>≤</mo> <mn>14</mn> <mspace></mspace> <mi>K</mi> </mrow> <annotation>${{T}_{c,zero}} le 14 {rm{K}}$</annotation> </semantics></math>. In this study, the reported self-field critical current density <span></span><math> <semantics> <mrow> <msub> <mi>J</mi> <mi>c</mi> </msub> <mrow> <mo>(</mo> <mrow> <mi>s</mi> <mi>f</mi> <mo>,</mo> <mi>T</mi> </mrow> <mo>)</mo> </mrow> </mrow> <annotation>${{J}_c}( {sf,T} )$</annotation> </semantics></math> and upper critical field <span></span><math> <semantics> <mrow> <msub> <mi>B</mi> <mrow> <mi>c</mi> <mn>2</mn> </mrow> </msub> <mrow> <mo>(</mo> <mi>T</mi> <mo>)</mo> </mrow> </mrow> <annotation>${{B}_{c2}}( T )$</annotation> </semantics></math> for these films are analyzed. The La<sub>3-x</sub>Pr<sub>x</sub>Ni<sub>2</sub>O<sub>7-δ</sub> films are find to exh
最近,两个研究小组报道了在几纳米厚的La3-xPrxNi2O7-δ (x = 0.0, 0.15和1.0)薄膜中观察到的大气压超导性,其起始转变温度为tc。温度t = 40 K ${{T}_{c,onset}} cong 40 {rm{K}}$和零电阻温度t c;z e r o≤14k ${{T}_{c,zero}} le 14 {rm{K}}$。本研究中报道的自场临界电流密度J c (s f),T) ${{J}_c}( {sf,T} )$和上临界场b2 (T) ${{B}_{c2}}( T )$对这些影片进行了分析。La3-xPrxNi2O7-δ薄膜具有较大的平面内伦敦穿透深度,λ ab (0) = 2.0 ~ 6.6 μ m ${lambda}_{textit{ab}}(0)=2.0-6.6 umu rm{m}$;Ginzburg-Landau参数κ c(0) = 500−1200 ${{kappa }_c}( 0 ) = 500 - 1200$。推导出的λ a b (0) ${{lambda }_{ab}}( 0 )$值在独立报告的λ的不确定范围内a b (T = 1.8 K) = 3.7±1.9 1.4 μ m ${{lambda }_{ab}}( {T ,{=} 1.8 {rm{K}}} ) ,{=}, 3.7 pm _{1.9}^{1.4} umu {rm{m}}$。 如此大的λ ab (0) ${{lambda }_{ab}}( 0 )$ 解释La3-xPrxNi2O7-δ薄膜的宽电阻转变,因为λ a b (0) ${{lambda }_{ab}}( 0 )$ 意味着低超流密度(ρ s≡1 λ ab 2) ${{rho }_s} equiv frac{1}{{lambda _{ab}^2}}$ ),因此有很大的热波动。结果表明,计算得到的相波动温度为T ~ f ~ c ${{T}_{fluc}}$ 满足不等式T c, z e r o, T f l u c ${{T}_{c,zero}} &lt; {{T}_{fluc}}$ . 我们还发现,J c (s f, T)的数据 ${{J}_c}( {sf,T} )$ b2c (T) ${{B}_{c2}}( T )$ 与双间隙模型非常吻合,其中,超导能隙Δ(0)与临界温度2 Δ L(0)之比为k B T c, L = 3.6 ~ 4.0 $frac{{2{{{{Delta}}}_L}( 0 )}}{{{{k}_B}{{T}_{c,L}}}} = 3.6 - 4.0$ 和2 Δ S (0) k BT c, S = 1.0−3。 (大波段和小波段分别为0 $frac{{2{{{{Delta}}}_S}( 0 )}}{{{{k}_B}{{T}_{c,S}}}} = 1.0 - 3.0$)。此外,高压缩Ruddlesden-Popper镍酸盐Lan+1NinO2n+ 1 (n = 2,3)和常压Lan+1NinO2n+2 (n = 5)薄膜表现出双带超导性。
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引用次数: 0
Investigating the Impact of Electromagnetic Fields on Local Quantum Fisher Information and Coherence in Graphene 研究电磁场对石墨烯中局部量子费雪信息和相干性的影响
IF 2.5 4区 物理与天体物理 Q2 PHYSICS, MULTIDISCIPLINARY Pub Date : 2025-08-19 DOI: 10.1002/andp.202500188
Abdelghani El Houri, Ayyoub El Mouatasim, Aziz Khribach, Younes Moqine, Brahim Adnane, Rachid Houça

This study explores the temporal evolution of local quantum Fisher information and coherence in a graphene monolayer subjected to a polarized electromagnetic field, revealing significant effects driven by system parameters. In the absence of the field, the analysis highlights the crucial role of the initial state's purity in the dynamics of both local quantum Fisher information and coherence, influencing their amplitude and decay over time. Introducing an electromagnetic field unveils a strong dependence of these quantities on the polarization and amplitude parameters. For linear polarization, local quantum Fisher information and coherence reach their maximum values at specific field phases, while for circular polarization, the system's response becomes more complex, exhibiting pronounced variations and a gradual decrease in coherence at higher field intensities. These findings emphasize the importance of controlling electromagnetic parameters to manipulate quantum information in graphene and open up new prospects for applications in quantum electronics and information processing.

本研究探讨了极化电磁场作用下石墨烯单层中局部量子Fisher信息和相干性的时间演化,揭示了系统参数驱动的显著影响。在没有场的情况下,分析强调了初始态的纯度在局部量子费雪信息和相干动力学中的关键作用,影响它们的振幅和随时间的衰减。引入电磁场揭示了这些量对极化和振幅参数的强烈依赖。对于线偏振,局部量子费雪信息和相干性在特定场相达到最大值,而对于圆偏振,系统的响应变得更加复杂,在高场强下表现出明显的变化和相干性逐渐降低。这些发现强调了控制电磁参数在石墨烯中操纵量子信息的重要性,并为量子电子学和信息处理领域的应用开辟了新的前景。
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引用次数: 0
Mechanisms of Noise Generation in Superconducting Quantum Interference Device Based Gradiometers Under Vibrations 基于超导量子干涉器件的梯度计振动下噪声产生机制研究
IF 2.5 4区 物理与天体物理 Q2 PHYSICS, MULTIDISCIPLINARY Pub Date : 2025-08-18 DOI: 10.1002/andp.202500101
Fan Song, Zhaohui Zhang, Tianyao Zhang, Xiaoyan Zhao, Jianmei Guo, Lu Yin, Chunlei Li, Liang Liang, Lei Han

Superconducting quantum interference device (SQUID) gradiometers are sensitive instruments for detecting magnetic fields and are widely used in magnetocardiography (MCG). However, their performance is compromised by vibrations from foundations or refrigeration equipment. Vibration-induced effects on SQUID gradiometers occur through two main mechanisms. First, an initial angular deviation between the pickup coils prevents cancellation of the reversed magnetic flux from external fields. Vibration converts this inherent interference into a time-varying flux disturbance at the vibration frequency. Second, bubbles from boiling liquid helium passing through the gradiometer loops increase the gradiometer's noise floor in the frequency domain. Vibration alters the dynamic behavior of these bubbles. Finite element simulations are conducted to examine the influence of these mechanisms across various vibration frequencies, and the SQUID gradiometer's noise power spectral density is measured at six vibration frequencies. The noise contains both narrowband and broadband components: The narrowband noise primarily occurs at the vibration frequencies and their second harmonics when the pickup coil's angular displacement aligns with or is perpendicular to the vibration direction. Meanwhile, the introduction of vibrations elevates the broadband noise level relative to the non-vibration state. Moreover, the broadband noise exhibits distinct peaks at the gradiometer's intrinsic resonance frequency of 15 Hz.

超导量子干涉装置(SQUID)梯度仪是一种灵敏的磁场检测仪器,在心脏磁图(MCG)中有着广泛的应用。然而,它们的性能受到地基或制冷设备振动的影响。振动对SQUID梯度仪的影响主要有两种机制。首先,拾取线圈之间的初始角度偏差阻止了来自外部磁场的反向磁通的抵消。振动将这种固有干扰转化为振动频率处的时变通量扰动。其次,沸腾液氦产生的气泡通过梯度计回路,增加了梯度计在频域的本底噪声。振动改变了这些气泡的动态行为。通过有限元模拟研究了这些机制在不同振动频率下的影响,并测量了SQUID梯度仪在6个振动频率下的噪声功率谱密度。噪声包含窄带和宽带两个分量:窄带噪声主要发生在拾取线圈的角位移与振动方向对齐或垂直时的振动频率及其二次谐波处。同时,相对于非振动状态,振动的引入提高了宽带噪声水平。此外,宽带噪声在梯度仪15 Hz的固有共振频率处呈现出明显的峰值。
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引用次数: 0
Oscillator Chain: A Simple Model for Universal Description of Excitation of Waveguiding Modes in Thin Films 振子链:薄膜中波导模式激发的一个简单模型
IF 2.5 4区 物理与天体物理 Q2 PHYSICS, MULTIDISCIPLINARY Pub Date : 2025-08-17 DOI: 10.1002/andp.202500219
Kestutis Staliunas

There is no simple and universal analytical description of various micro-optical systems related with Fano resonances. This especially concerns modulated thin films, which, when coupled to external fields, show Fano resonances. Usually, such micro-optic schemes are simulated numerically, frequently by the use of commercial software. The study fills this gap of the lack of universal analytical description by introducing and exploring a simple mechanical equivalent, the oscillator chain, which mimics such schemes involving Fano resonances. The model does not necessarily provide the rigorous description of complicated micro-optical schemes, however does capture the main properties of such Fano-related micro-optical systems. The model captures different modifications of the thin film arrangement as well: thin film with amplification, non-Hermitical thin films, and others. It also covers the case of multiple Fano resonances in a thin film. The model is validated by comparing with the rigorously calculated wave propagation in the thin films.

对于各种与法诺共振相关的微光学系统,目前还没有一个简单而通用的分析描述。这尤其涉及到调制薄膜,当耦合到外场时,会显示出范诺共振。通常,这种微光学方案是通过使用商业软件进行数值模拟的。该研究通过引入和探索一种简单的机械等效,即振荡器链,来模拟涉及法诺共振的方案,从而填补了缺乏通用分析描述的空白。该模型不一定提供复杂的微光学方案的严格描述,但确实捕获了此类法诺相关微光学系统的主要特性。该模型还捕获了薄膜排列的不同修改:带放大的薄膜、非厄米薄膜等。它还涵盖了薄膜中多个范诺共振的情况。通过与严格计算的波在薄膜中的传播进行比较,验证了模型的正确性。
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引用次数: 0
Entanglement and Magic Correlations Generated by Discrete Beam-Splitters 离散分束器产生的纠缠和魔法相关
IF 2.5 4区 物理与天体物理 Q2 PHYSICS, MULTIDISCIPLINARY Pub Date : 2025-08-15 DOI: 10.1002/andp.202500288
Lingxuan Feng, Shunlong Luo

Beam-splitters are basic and instrumental tools not only in the study of foundational issues in quantum mechanics, but also in various applications of quantum information processing. In the continuous-variable scenario involving quantum optical states and Gaussian quantum information, interference phenomena are widely investigated and characterized via beam-splitters. In this work, within the framework of stabilizer quantum computation in finite quantum systems, entanglement and magic correlations generated by discrete beam-splitters are explored. Two types of magic correlations are distinguished: mutual magic (analogous to quantum mutual information) and non-local magic. Explicit formulas for these correlations are derived in the qubit scenario where the beam-splitter is implemented by the controlled-NOT gate, with the H$H$-type magic states playing a particularly prominent role as input states. Extending to prime-dimensional qudit systems, it is shown that fiducial states of mutually unbiased bases also play a remarkable role. Basic properties of these magic correlations are revealed and illustrated through some typical examples.

分束器不仅是研究量子力学基础问题的基本工具,而且在量子信息处理的各种应用中都有应用。在涉及量子光态和高斯量子信息的连续变量场景中,干涉现象被广泛研究并通过分束器进行表征。本文在有限量子系统中稳定量子计算的框架内,探讨了离散分束器产生的纠缠和幻相关。两种类型的魔法关联被区分:互魔法(类似于量子互信息)和非局部魔法。这些相关性的显式公式在量子位场景中推导出来,其中分束器由受控非门实现,H$ H$类型的魔法状态作为输入状态起着特别突出的作用。推广到素维量子系统,证明了互无偏基的基态也起着显著的作用。通过一些典型的例子,揭示并说明了这些神奇关联的基本性质。
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引用次数: 0
Non-Markovian Protection and Thermal Fragility of Quantum Resources in a Spin-1/2 Ising–Heisenberg Diamond Chain 自旋1/2伊辛-海森堡钻石链中量子资源的非马尔可夫保护和热脆弱性
IF 2.5 4区 物理与天体物理 Q2 PHYSICS, MULTIDISCIPLINARY Pub Date : 2025-08-15 DOI: 10.1002/andp.202500258
Fadwa Benabdallah, M. Y. Abd-Rabbou, Mohammed Daoud

This research investigates the dynamics of entanglement and uncertainty-induced nonlocality (UIN) in a spin-1/2 Ising-Heisenberg diamond chain subjected to local non-Markovian decoherence channels. By examining amplitude damping (AD) and random telegraph noise (RTN) in both zero and finite temperature regimes, the study reveals nuanced distinctions in the degradation and revival of quantum correlations. The interplay between intrinsic spin couplings, thermal effects, and memory-induced coherence backflow highlights the complex behavior of quantum resources under realistic noise conditions. Concurrence emerges as a sensitive marker of entanglement recovery in dephasing environments, while uncertainty-induced nonlocality proves more resilient in high-temperature or dissipative regimes. The analysis further demonstrates that moderate thermal activation and external magnetic fields can nontrivially enhance or suppress quantum features depending on system parameters. These findings offer a detailed perspective on the robustness and complementarity of different quantum correlation measures, providing guiding principles for the design of thermally stable and noise-resilient quantum information protocols.

本文研究了在局部非马尔可夫退相干通道作用下,自旋1/2的伊辛-海森堡钻石链中的纠缠动力学和不确定性诱导的非定域性(UIN)。通过检查零温度和有限温度下的振幅阻尼(AD)和随机电报噪声(RTN),该研究揭示了量子相关性退化和恢复的细微差别。本征自旋耦合、热效应和记忆诱导相干回流之间的相互作用突出了量子资源在现实噪声条件下的复杂行为。并发性是失相环境中纠缠恢复的敏感标志,而不确定性引起的非定域性在高温或耗散状态下更具弹性。分析进一步表明,适度的热激活和外磁场可以根据系统参数显著增强或抑制量子特征。这些发现为不同量子相关度量的鲁棒性和互补性提供了详细的视角,为热稳定和噪声弹性量子信息协议的设计提供了指导原则。
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引用次数: 0
Clusters Stagnating During Condensation: Metastable Material or a Separate State of Matter? 凝聚过程中停滞的团簇:亚稳态物质还是物质的独立状态?
IF 2.5 4区 物理与天体物理 Q2 PHYSICS, MULTIDISCIPLINARY Pub Date : 2025-08-14 DOI: 10.1002/andp.202500237
Nicholas R. Jaramillo, Cole A. Ritchie, Michelle L. Pantoya, Igor E. Agranovski, Igor Altman

Condensation stagnation, that is, the existence of a delay between nucleation and growth during gas-phase particle formation, is a crucial phenomenon that affects associated processes and manifests itself as the presence of supercritical clusters in resulting particulates. In previous work, this unique phenomenon was experimentally demonstrated in a magnesium (Mg) particle flame, and an empirical explanation for the mechanisms responsible for the phenomenon was provided. The occurrence of stagnant clusters was revealed using specially designed sampling. The analysis of collected products, however, could not provide details about their evolution, so no information on the cluster's lifespan (i.e., stagnation time) was available. In the current manuscript, the results of spectroscopic studies of the Mg particle flame in air are reported. The recently developed advanced processing analysis of pyrometry data makes it possible to identify the light emission signature of stagnant clusters and, accordingly, estimate their lifespan, that is, the time during which clusters have physical properties (e.g., emissivity) different from those of mature nano-oxides. The obtained time on the order of 10 ms seems to be sufficiently long, which allows one to consider stagnant clusters as a separate state of matter, and not as a metastable metal oxide material.

冷凝停滞,即在气相颗粒形成过程中,在成核和生长之间存在延迟,是影响相关过程的关键现象,并表现为在产生的颗粒中存在超临界团簇。在之前的工作中,这种独特的现象在镁(Mg)颗粒火焰中得到了实验证明,并为该现象的机制提供了经验解释。通过特别设计的采样,揭示了停滞集群的发生。但是,对收集到的产品的分析不能提供有关其演变的详细信息,因此没有关于集群生命周期(即停滞时间)的信息。本文报道了空气中Mg粒子火焰的光谱研究结果。最近开发的高温数据的高级处理分析使识别停滞团簇的发光特征成为可能,并据此估计它们的寿命,即团簇具有与成熟纳米氧化物不同的物理性质(例如,发射率)的时间。获得的10毫秒量级的时间似乎足够长,这使得人们可以将停滞的团簇视为物质的一种独立状态,而不是亚稳的金属氧化物材料。
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引用次数: 0
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Annalen der Physik
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