首页 > 最新文献

The European Physical Journal E最新文献

英文 中文
Simple method for the direct measurement of cohesive forces between microscopic particles 直接测量微观粒子间内聚力的简单方法
IF 1.8 4区 物理与天体物理 Q4 CHEMISTRY, PHYSICAL Pub Date : 2025-01-09 DOI: 10.1140/epje/s10189-024-00459-y
Johnathan Hoggarth, Kari Dalnoki-Veress

We present a simple and inexpensive method for measuring weak cohesive interactions. This technique is applied to the specific case of oil droplets with a depletion interaction, dispersed in an aqueous solution. The experimental setup involves creating a short string of droplets while immobilizing a single droplet. The droplets are held together via depletion interactions, and a single cohesive bond holds together nearest neighbours. Initially, the buoyant droplets are held in a flat horizontal chamber. The droplets float to the top of the chamber and are in contact with a flat glass interface. In the horizontal configuration, there is no component of the effective buoyant force acting in the plane of the chamber. The angle of the chamber is gradually increased, and the effective buoyant force acting on the string of droplets slowly increases. At a critical point, when the combination of gravity and buoyancy is equal to the cohesive force, the droplet string will detach from the immobile droplet. Our method allows for a simple direct measurement of cohesive forces on the tens of pico-Newton scale. To illustrate the validity of this technique, the droplet radii and concentration of depletant are varied, and their impact on the cohesive force is measured. This method offers a simple, accessible, and reproducible means of exploring cohesive interactions beyond the specific case of oil droplets and a depletion interaction.

(Top) Side and top-down view schematic of the experimental chamber. (Bottom) Stable and unstable dangling chain of droplets. The chain detaches from the stationary droplet once the effective buoyant force is greater than the cohesive force

我们提出了一种测量弱内聚相互作用的简单而廉价的方法。该技术适用于分散在水溶液中具有耗竭相互作用的油滴的具体情况。实验装置包括在固定单个液滴的同时制造一串短液滴。液滴通过耗竭相互作用聚集在一起,一个单一的粘性键将最近的邻居聚集在一起。最初,有浮力的液滴被保持在一个平坦的水平腔室中。液滴漂浮到腔室的顶部,并与平面玻璃界面接触。在水平结构中,没有有效浮力的分量作用在腔室的平面上。腔体角度逐渐增大,作用在水滴串上的有效浮力逐渐增大。在一个临界点上,当重力和浮力的组合等于黏结力时,液滴串将与不动的液滴分离。我们的方法允许在几十皮牛顿尺度上简单地直接测量内聚力。为了说明该方法的有效性,研究了液滴半径和消耗剂浓度的变化,以及它们对黏结力的影响。该方法提供了一种简单、可接近、可重复的方法,用于探索油滴和耗竭相互作用之外的内聚相互作用。(上)实验室的侧面和自上而下的示意图。(下)稳定和不稳定的悬浮液滴链。当有效浮力大于内聚力时,链就会从静止液滴上脱离
{"title":"Simple method for the direct measurement of cohesive forces between microscopic particles","authors":"Johnathan Hoggarth,&nbsp;Kari Dalnoki-Veress","doi":"10.1140/epje/s10189-024-00459-y","DOIUrl":"10.1140/epje/s10189-024-00459-y","url":null,"abstract":"<p>We present a simple and inexpensive method for measuring weak cohesive interactions. This technique is applied to the specific case of oil droplets with a depletion interaction, dispersed in an aqueous solution. The experimental setup involves creating a short string of droplets while immobilizing a single droplet. The droplets are held together via depletion interactions, and a single cohesive bond holds together nearest neighbours. Initially, the buoyant droplets are held in a flat horizontal chamber. The droplets float to the top of the chamber and are in contact with a flat glass interface. In the horizontal configuration, there is no component of the effective buoyant force acting in the plane of the chamber. The angle of the chamber is gradually increased, and the effective buoyant force acting on the string of droplets slowly increases. At a critical point, when the combination of gravity and buoyancy is equal to the cohesive force, the droplet string will detach from the immobile droplet. Our method allows for a simple direct measurement of cohesive forces on the tens of pico-Newton scale. To illustrate the validity of this technique, the droplet radii and concentration of depletant are varied, and their impact on the cohesive force is measured. This method offers a simple, accessible, and reproducible means of exploring cohesive interactions beyond the specific case of oil droplets and a depletion interaction.</p><p>(Top) Side and top-down view schematic of the experimental chamber. (Bottom) Stable and unstable dangling chain of droplets. The chain detaches from the stationary droplet once the effective buoyant force is greater than the cohesive force</p>","PeriodicalId":790,"journal":{"name":"The European Physical Journal E","volume":"48 1","pages":""},"PeriodicalIF":1.8,"publicationDate":"2025-01-09","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142939052","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Weak non-linearities of amorphous polymer under creep in the vicinity of the glass transition 非晶聚合物在玻璃化转变附近蠕变的弱非线性
IF 1.8 4区 物理与天体物理 Q4 CHEMISTRY, PHYSICAL Pub Date : 2025-01-09 DOI: 10.1140/epje/s10189-024-00468-x
Martin Roman-Faure, Hélène Montes, François Lequeux, Antoine Chateauminois

The creep behavior of an amorphous poly(etherimide) polymer is investigated in the vicinity of its glass transition in a weakly non linear regime where the acceleration of the creep response is driven by local configurational rearrangements. From the time shifts of the creep compliance curves under stresses from 1 to 15 MPa and in the temperature range between (T_g -10K) and (T_g), where (T_g) is the glass transition temperature, we determine a macroscopic acceleration factor. The macroscopic acceleration is shown to vary as (e^{-(Sigma /Y)}) temperature with (n=2 pm 0.2), where (Sigma ) is the macroscopic stress and Y is a decreasing function of compliance. Because at the beginning of creep, the stress is homogeneous, the macroscopic acceleration is thus similar to the local one, in agreement with the recent theory of Long et al. (Phys Rev Mat 2:105601, 2018) which predicts (n=2). For larger compliances, the decrease of Y is interpreted as a signature of the development of stress disorder during creep.

Left: The acceleration of creep kinetics in a weakly non-linear regime in the vicinity of the glass transition is described through an acceleration function F which depends on both the applied stress and the compliance J(t) as a result of the stress induced shift of the relaxation time of nanometric domains (from top to bottom: increasing applied creep stresses). Right : Description of an amorphous polymer glass as a disordered medium made up of nanometric domains with widely distributed relaxation times.

本文研究了一种非晶聚醚酰亚胺聚合物在其玻璃化转变附近的蠕变行为,在弱非线性状态下,蠕变响应的加速是由局部构型重排驱动的。根据应力范围为1 ~ 15 MPa,温度范围为(T_g -10K) ~ (T_g) ((T_g)为玻璃化转变温度)的蠕变柔顺曲线的时移,确定了宏观加速度因子。宏观加速度随(e^{-(Sigma /Y)})温度随(n=2 pm 0.2)变化,其中(Sigma )为宏观应力,Y为柔度的递减函数。因为在蠕变开始时,应力是均匀的,因此宏观加速度与局部加速度相似,这与Long等人最近的理论(Phys Rev Mat 2:105601, 2018)预测(n=2)一致。对于较大的柔度,Y的减小被解释为蠕变过程中应力紊乱发展的标志。左:蠕变动力学在玻璃化转变附近的弱非线性状态下的加速是通过加速度函数F来描述的,加速度函数F取决于施加的应力和柔度J(t),这是应力引起的纳米域弛豫时间位移的结果(从上到下:增加施加的蠕变应力)。右图:描述了一种非晶聚合物玻璃,它是由具有广泛分布的弛豫时间的纳米结构域组成的无序介质。
{"title":"Weak non-linearities of amorphous polymer under creep in the vicinity of the glass transition","authors":"Martin Roman-Faure,&nbsp;Hélène Montes,&nbsp;François Lequeux,&nbsp;Antoine Chateauminois","doi":"10.1140/epje/s10189-024-00468-x","DOIUrl":"10.1140/epje/s10189-024-00468-x","url":null,"abstract":"<p>The creep behavior of an amorphous poly(etherimide) polymer is investigated in the vicinity of its glass transition in a weakly non linear regime where the acceleration of the creep response is driven by local configurational rearrangements. From the time shifts of the creep compliance curves under stresses from 1 to 15 MPa and in the temperature range between <span>(T_g -10K)</span> and <span>(T_g)</span>, where <span>(T_g)</span> is the glass transition temperature, we determine a macroscopic acceleration factor. The macroscopic acceleration is shown to vary as <span>(e^{-(Sigma /Y)})</span> temperature with <span>(n=2 pm 0.2)</span>, where <span>(Sigma )</span> is the macroscopic stress and <i>Y</i> is a decreasing function of compliance. Because at the beginning of creep, the stress is homogeneous, the macroscopic acceleration is thus similar to the local one, in agreement with the recent theory of Long et al. (Phys Rev Mat 2:105601, 2018) which predicts <span>(n=2)</span>. For larger compliances, the decrease of <i>Y</i> is interpreted as a signature of the development of stress disorder during creep.</p><p>Left: The acceleration of creep kinetics in a weakly non-linear regime in the vicinity of the glass transition is described through an acceleration function F which depends on both the applied stress and the compliance J(t) as a result of the stress induced shift of the relaxation time of nanometric domains (from top to bottom: increasing applied creep stresses). Right : Description of an amorphous polymer glass as a disordered medium made up of nanometric domains with widely distributed relaxation times.</p>","PeriodicalId":790,"journal":{"name":"The European Physical Journal E","volume":"48 1","pages":""},"PeriodicalIF":1.8,"publicationDate":"2025-01-09","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142939051","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Extrinsic and intrinsic effects setting viscosity in complex fluids and life processes: the role of fundamental physical constants 复杂流体和生命过程中粘度的外在和内在影响:基本物理常数的作用
IF 1.8 4区 物理与天体物理 Q4 CHEMISTRY, PHYSICAL Pub Date : 2025-01-03 DOI: 10.1140/epje/s10189-024-00467-y
K. Trachenko, P. G. Tello, S. A. Kauffman, S. Succi

Understanding the values and origin of fundamental physical constants, one of the grandest challenges in modern science, has been discussed in particle physics, astronomy and cosmology. More recently, it was realized that fundamental constants have a biofriendly window set by life processes involving motion and flow. This window is related to intrinsic fluid properties such as energy and length scales in condensed matter set by fundamental constants. Here, we discuss important extrinsic factors governing the viscosity of complex fluids operating in life processes due to collective effects. We show that both extrinsic and intrinsic factors affecting viscosity need to be taken into account when estimating the biofriendly range of fundamental constants from life processes, and our discussion provides a straightforward recipe for doing this. Remarkably, the viscosity of a complex fluid such as blood with significant extrinsic effects is not far from the intrinsic viscosity calculated using the fundamental constants only, and we discuss the reason for this in terms of dynamics of contact points between cells.

理解基本物理常数的值和起源是现代科学中最大的挑战之一,在粒子物理学、天文学和宇宙学中都有讨论。最近,人们意识到,基本常数有一个生物友好的窗口,由涉及运动和流动的生命过程设置。这个窗口与固有的流体性质有关,如由基本常数设定的凝聚态物质的能量和长度尺度。在这里,我们讨论了在生命过程中由于集体效应而控制复杂流体粘度的重要外在因素。我们表明,在估计生命过程中基本常数的生物友好范围时,需要考虑影响粘度的外在因素和内在因素,我们的讨论为这样做提供了一个简单的方法。值得注意的是,具有显著外在效应的复杂流体(如血液)的粘度与仅使用基本常数计算的本征粘度相差不远,我们从细胞间接触点的动力学角度讨论了这一现象的原因。
{"title":"Extrinsic and intrinsic effects setting viscosity in complex fluids and life processes: the role of fundamental physical constants","authors":"K. Trachenko,&nbsp;P. G. Tello,&nbsp;S. A. Kauffman,&nbsp;S. Succi","doi":"10.1140/epje/s10189-024-00467-y","DOIUrl":"10.1140/epje/s10189-024-00467-y","url":null,"abstract":"<p>Understanding the values and origin of fundamental physical constants, one of the grandest challenges in modern science, has been discussed in particle physics, astronomy and cosmology. More recently, it was realized that fundamental constants have a biofriendly window set by life processes involving motion and flow. This window is related to intrinsic fluid properties such as energy and length scales in condensed matter set by fundamental constants. Here, we discuss important extrinsic factors governing the viscosity of complex fluids operating in life processes due to collective effects. We show that both extrinsic and intrinsic factors affecting viscosity need to be taken into account when estimating the biofriendly range of fundamental constants from life processes, and our discussion provides a straightforward recipe for doing this. Remarkably, the viscosity of a complex fluid such as blood with significant extrinsic effects is not far from the intrinsic viscosity calculated using the fundamental constants only, and we discuss the reason for this in terms of dynamics of contact points between cells.</p>","PeriodicalId":790,"journal":{"name":"The European Physical Journal E","volume":"48 1","pages":""},"PeriodicalIF":1.8,"publicationDate":"2025-01-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1140/epje/s10189-024-00467-y.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142912969","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
A hitchhiker’s guide to active motion 主动运动的搭便车指南
IF 1.8 4区 物理与天体物理 Q4 CHEMISTRY, PHYSICAL Pub Date : 2025-01-03 DOI: 10.1140/epje/s10189-024-00465-0
Tobias Plasczyk, Paul A. Monderkamp, Hartmut Löwen, René Wittmann

Intelligent decisions in response to external informative input can allow organisms to achieve their biological goals while spending very little of their own resources. In this paper, we develop and study a minimal model for a navigational task, performed by an otherwise completely motorless particle that possesses the ability of hitchhiking in a bath of active Brownian particles (ABPs). Hitchhiking refers to identifying and attaching to suitable surrounding bath particles. Using a reinforcement learning algorithm, such an agent, which we refer to as intelligent hitchhiking particle (IHP), is enabled to persistently navigate in the desired direction. This relatively simple IHP can also anticipate and react to characteristic motion patterns of their hosts, which we exemplify for a bath of chiral ABPs (cABPs). To demonstrate that the persistent motion of the IHP will outperform that of the bath particles in view of long-time ballistic motion, we calculate the mean-squared displacement and discuss its dependence on the density and persistence time of the bath ABPs by means of an analytic model.

Illustration of an intelligent hitchhiking particle (IHP) in a bath of active Brownian particles (ABPs). The IHP fulfills a navigational task by holding on to an ABP only if its orientation points upwards, enabling persistent motion.

响应外部信息输入的智能决策可以使生物体在花费很少的自身资源的情况下实现其生物目标。在本文中,我们开发和研究了一个导航任务的最小模型,该模型由一个完全无运动的粒子执行,该粒子具有搭便车活动布朗粒子(ABPs)浴的能力。搭便车是指识别并附着在周围合适的浴液颗粒上。使用强化学习算法,这样的代理,我们称之为智能搭便车粒子(IHP),能够持续地在期望的方向上导航。这种相对简单的IHP还可以预测并对宿主的特征运动模式做出反应,我们以手性ABPs (cABPs)为例。考虑到长时间的弹道运动,为了证明射流粒子的持续运动优于熔池粒子的持续运动,我们计算了均方位移,并通过解析模型讨论了其与熔池射流粒子密度和持续时间的关系。智能搭便车粒子(IHP)在活跃布朗粒子(ABPs)浴中的图示。只有当ABP的方向指向上方时,IHP才会抓住它来完成导航任务,从而实现持续运动。
{"title":"A hitchhiker’s guide to active motion","authors":"Tobias Plasczyk,&nbsp;Paul A. Monderkamp,&nbsp;Hartmut Löwen,&nbsp;René Wittmann","doi":"10.1140/epje/s10189-024-00465-0","DOIUrl":"10.1140/epje/s10189-024-00465-0","url":null,"abstract":"<p>Intelligent decisions in response to external informative input can allow organisms to achieve their biological goals while spending very little of their own resources. In this paper, we develop and study a minimal model for a navigational task, performed by an otherwise completely motorless particle that possesses the ability of <i>hitchhiking</i> in a bath of active Brownian particles (ABPs). Hitchhiking refers to identifying and attaching to suitable surrounding bath particles. Using a reinforcement learning algorithm, such an agent, which we refer to as intelligent hitchhiking particle (IHP), is enabled to persistently navigate in the desired direction. This relatively simple IHP can also anticipate and react to characteristic motion patterns of their hosts, which we exemplify for a bath of chiral ABPs (cABPs). To demonstrate that the persistent motion of the IHP will outperform that of the bath particles in view of long-time ballistic motion, we calculate the mean-squared displacement and discuss its dependence on the density and persistence time of the bath ABPs by means of an analytic model.</p><p>Illustration of an intelligent hitchhiking particle (IHP) in a bath of active Brownian particles (ABPs). The IHP fulfills a navigational task by holding on to an ABP only if its orientation points upwards, enabling persistent motion.</p>","PeriodicalId":790,"journal":{"name":"The European Physical Journal E","volume":"48 1","pages":""},"PeriodicalIF":1.8,"publicationDate":"2025-01-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1140/epje/s10189-024-00465-0.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142912970","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Bifurcation analysis and control of the full velocity difference model with delayed velocity difference 时滞速度差全速度差模型的分岔分析与控制
IF 1.8 4区 物理与天体物理 Q4 CHEMISTRY, PHYSICAL Pub Date : 2024-12-08 DOI: 10.1140/epje/s10189-024-00462-3
Wenhuan Ai, Guoao Li, Jianhua Zhang, Xiaoshuang Zhu, Dawei Liu

With the increase in the number of urban vehicles, various traffic problems have gradually emerged. Studying the causes of traffic congestion and proposing effective mitigation strategies have important practical significance. This paper proposes a macroscopic traffic flow model that considers the delayed speed difference. This paper applies nonlinear bifurcation to describe and predict nonlinear traffic phenomena on highways from the perspective of global stability of the traffic system. By using the traveling wave transformation, the proposed car-following model is converted into a macroscopic traffic flow model. Next, this paper employs the linear stability analysis to find the bifurcation points of the stability transition in the traffic system, exploring the qualitative characteristics of the inhomogeneous continuous traffic flow model. Theoretical derivations demonstrate the existence of bifurcation points within the model. Additionally, this paper plots the density-time space diagrams and phase plane diagrams of the system to visually present the sudden changes in traffic flow as variable parameters pass through these bifurcation points. Finally, this paper designs a feedback controller to regulate the Hopf bifurcation, aiming to delay or eliminate the occurrence of Hopf bifurcations in the stochastic system.

Graphical abstract

随着城市车辆数量的增加,各种交通问题逐渐显现。研究交通拥堵的成因并提出有效的缓解策略具有重要的现实意义。本文提出了一个考虑延迟速度差的宏观交通流模型。本文从交通系统全局稳定性的角度出发,运用非线性分岔理论来描述和预测公路上的非线性交通现象。通过行波变换,将所提出的车辆跟随模型转化为宏观交通流模型。其次,本文采用线性稳定性分析方法寻找交通系统稳定性过渡的分岔点,探讨非齐次连续交通流模型的定性特征。理论推导证明了模型中存在分岔点。并绘制了系统的密度-时间-空间图和相平面图,直观地呈现了变参数经过这些分岔点时交通流的突变。最后,本文设计了一个反馈控制器来调节Hopf分岔,目的是延迟或消除随机系统中Hopf分岔的发生。图形抽象
{"title":"Bifurcation analysis and control of the full velocity difference model with delayed velocity difference","authors":"Wenhuan Ai,&nbsp;Guoao Li,&nbsp;Jianhua Zhang,&nbsp;Xiaoshuang Zhu,&nbsp;Dawei Liu","doi":"10.1140/epje/s10189-024-00462-3","DOIUrl":"10.1140/epje/s10189-024-00462-3","url":null,"abstract":"<div><p>With the increase in the number of urban vehicles, various traffic problems have gradually emerged. Studying the causes of traffic congestion and proposing effective mitigation strategies have important practical significance. This paper proposes a macroscopic traffic flow model that considers the delayed speed difference. This paper applies nonlinear bifurcation to describe and predict nonlinear traffic phenomena on highways from the perspective of global stability of the traffic system. By using the traveling wave transformation, the proposed car-following model is converted into a macroscopic traffic flow model. Next, this paper employs the linear stability analysis to find the bifurcation points of the stability transition in the traffic system, exploring the qualitative characteristics of the inhomogeneous continuous traffic flow model. Theoretical derivations demonstrate the existence of bifurcation points within the model. Additionally, this paper plots the density-time space diagrams and phase plane diagrams of the system to visually present the sudden changes in traffic flow as variable parameters pass through these bifurcation points. Finally, this paper designs a feedback controller to regulate the Hopf bifurcation, aiming to delay or eliminate the occurrence of Hopf bifurcations in the stochastic system.</p><h3>Graphical abstract</h3><div><figure><div><div><picture><source><img></source></picture></div></div></figure></div></div>","PeriodicalId":790,"journal":{"name":"The European Physical Journal E","volume":"47 11","pages":""},"PeriodicalIF":1.8,"publicationDate":"2024-12-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142789215","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Characterization of dynamic interplay among different channels during immiscible displacement in porous media under different flow rates 不同流量下多孔介质非混相驱替过程中不同通道间动态相互作用的表征
IF 1.8 4区 物理与天体物理 Q4 CHEMISTRY, PHYSICAL Pub Date : 2024-12-07 DOI: 10.1140/epje/s10189-024-00463-2
Yusong Xu, Yingxue Hu, Kaixin Chen, Yuanqing Liu, Jiangang Liu, Weiwei Hao, Tianjiang Wu, Chuanqing Huang, Junwei Su

Although immiscible displacement in porous media has been extensively studied, a more comprehensive analysis of the underlying dynamic behaviors is still necessary. In this work, we conducted experimental and theoretical analyses on the dynamic interplay among channels during immiscible displacement under varying flow rates. In a rock-structured microfluidic chip, we observed typical displacement patterns, including viscous fingering and capillary fingering, and analyzed their frontiers and efficiencies. Interestingly, we discovered a novel 'V'-shaped recovery rate pattern, which differs from the monotonic curve considered in previous research. The recovery rate reaches its lowest point at an injection rate of 1 μL/min (42%), increasing to 55 and 65% at rates of 16 and 0.1 μL/min, respectively. This increase may attribute to all-directional displacement at lower rates and multi-fingering displacement at higher rates, contrasting with primary fingering displacement observed at intermediate rates. Furthermore, we developed a dual-tube model to investigate the dynamic mechanisms between adjacent channels during the displacement process. At high injection rates, an increase in low-viscosity fluid rapidly reduces overall average viscosity of the channels, accelerating displacement while hindering the displacement process in neighboring channels. Conversely, at low injection rates, increased capillary forces at pore-throat junctions delay breakthrough in one channel, promoting simultaneous displacement in parallel channels and ensuring stability. These findings significantly enhance our understanding of the interplay between viscous and capillary forces in porous media during displacement processes.

Graphical abstract

尽管多孔介质中的非混相驱替已经得到了广泛的研究,但对其潜在的动力学行为进行更全面的分析仍然是必要的。在这项工作中,我们对不同流量下非混相驱替过程中通道间的动态相互作用进行了实验和理论分析。在岩石结构微流控芯片中,我们观察了典型的位移模式,包括粘性指移和毛细指移,并分析了它们的边界和效率。有趣的是,我们发现了一个新的“V”型回收率模式,不同于以往研究中考虑的单调曲线。在注射速度为1 μL/min时,回收率最低(42%),在注射速度为16 μL/min和0.1 μL/min时,回收率分别提高到55%和65%。这种增加可能归因于低速率下的全方位位移和高速率下的多指位移,与中速率下观察到的主要指位移形成对比。此外,我们开发了一个双管模型来研究相邻通道在位移过程中的动力机制。在高注入速率下,低粘度流体的增加迅速降低了通道的总体平均粘度,加速了驱替,同时阻碍了邻近通道的驱替过程。相反,在低注入速率下,孔喉连接处毛细力的增加会延迟一个通道的突破,从而促进平行通道的同时位移并确保稳定性。这些发现大大增强了我们对多孔介质中粘性力和毛细力在驱替过程中的相互作用的理解。图形抽象
{"title":"Characterization of dynamic interplay among different channels during immiscible displacement in porous media under different flow rates","authors":"Yusong Xu,&nbsp;Yingxue Hu,&nbsp;Kaixin Chen,&nbsp;Yuanqing Liu,&nbsp;Jiangang Liu,&nbsp;Weiwei Hao,&nbsp;Tianjiang Wu,&nbsp;Chuanqing Huang,&nbsp;Junwei Su","doi":"10.1140/epje/s10189-024-00463-2","DOIUrl":"10.1140/epje/s10189-024-00463-2","url":null,"abstract":"<div><p>Although immiscible displacement in porous media has been extensively studied, a more comprehensive analysis of the underlying dynamic behaviors is still necessary. In this work, we conducted experimental and theoretical analyses on the dynamic interplay among channels during immiscible displacement under varying flow rates. In a rock-structured microfluidic chip, we observed typical displacement patterns, including viscous fingering and capillary fingering, and analyzed their frontiers and efficiencies. Interestingly, we discovered a novel 'V'-shaped recovery rate pattern, which differs from the monotonic curve considered in previous research. The recovery rate reaches its lowest point at an injection rate of 1 μL/min (42%), increasing to 55 and 65% at rates of 16 and 0.1 μL/min, respectively. This increase may attribute to all-directional displacement at lower rates and multi-fingering displacement at higher rates, contrasting with primary fingering displacement observed at intermediate rates. Furthermore, we developed a dual-tube model to investigate the dynamic mechanisms between adjacent channels during the displacement process. At high injection rates, an increase in low-viscosity fluid rapidly reduces overall average viscosity of the channels, accelerating displacement while hindering the displacement process in neighboring channels. Conversely, at low injection rates, increased capillary forces at pore-throat junctions delay breakthrough in one channel, promoting simultaneous displacement in parallel channels and ensuring stability. These findings significantly enhance our understanding of the interplay between viscous and capillary forces in porous media during displacement processes.</p><h3>Graphical abstract</h3>\u0000<div><figure><div><div><picture><source><img></source></picture></div></div></figure></div></div>","PeriodicalId":790,"journal":{"name":"The European Physical Journal E","volume":"47 11","pages":""},"PeriodicalIF":1.8,"publicationDate":"2024-12-07","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142789377","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
The dynamics of a reacting polymer attached to a surface 附着在表面上的聚合物的反应动力学
IF 1.8 4区 物理与天体物理 Q4 CHEMISTRY, PHYSICAL Pub Date : 2024-12-02 DOI: 10.1140/epje/s10189-024-00464-1
Barry Friedman, Chuck Yeung

Scaling arguments are presented for end-to-wall reaction and end-to-end reactions of grafted chains for non-self-avoiding and self-avoiding chains with and without hydrodynamic interaction. The most realistic minimal model for the experiments of Kim and Lee (J Phys Chem Lett 12:4576, 2021. https://doi.org/10.1021/acs.jpclett.1c00962) is a chain tethered to a plane, the chain having excluded volume and hydrodynamic interaction with end-to-end reactions. From our scaling argument, such a chain obeys a law of mass action where the macroscopic reaction rate is proportional to the microscopic reaction rate multiplied by the probability that the chain ends are close together. More precisely, this means for long chains there is no diffusion controlled limit. In addition, a polymer attached to a plane where the end reacts with the entire plane, end-to-wall reactions, was also investigated. For sufficiently long polymers, this system is always diffusion controlled, even with excluded volume and hydrodynamic interaction. We test the scaling arguments for the simplest case of a non-self-avoiding chains obeying Rouse dynamics. The numerical results agree with the scaling analysis for both end-to-wall and end-to-end reactions of the grafted chain. In particular, our numerical simulations support the end-to-end reaction of a tethered non-self-avoiding is the marginal case in the scaling sense.

提出了接枝链端壁反应和端到端反应的标度参数,适用于有和没有流体动力相互作用的非自避链和自避链。Kim和Lee的实验中最现实的最小模型[J] .物理化学学报,12(5):776,2021。https://doi.org/10.1021/acs.jpclett.1c00962)是拴在平面上的链,链排除了端到端反应的体积和流体动力学相互作用。从我们的标度论证来看,这样的链遵循质量作用定律,即宏观反应速率与微观反应速率乘以链端靠近的概率成正比。更准确地说,这意味着对于长链来说,没有扩散控制的极限。此外,还研究了附着在一个平面上的聚合物,其端部与整个平面发生反应,即端壁反应。对于足够长的聚合物,即使排除了体积和水动力相互作用,该系统也始终是扩散控制的。我们对服从劳斯动力学的非自回避链的最简单情况进行了尺度论证。数值结果与接枝链端到端和端到端反应的标度分析一致。特别是,我们的数值模拟支持端到端反应系绳非自我回避是边际情况下的尺度意义。
{"title":"The dynamics of a reacting polymer attached to a surface","authors":"Barry Friedman,&nbsp;Chuck Yeung","doi":"10.1140/epje/s10189-024-00464-1","DOIUrl":"10.1140/epje/s10189-024-00464-1","url":null,"abstract":"<p>Scaling arguments are presented for end-to-wall reaction and end-to-end reactions of grafted chains for non-self-avoiding and self-avoiding chains with and without hydrodynamic interaction. The most realistic minimal model for the experiments of Kim and Lee (J Phys Chem Lett 12:4576, 2021. https://doi.org/10.1021/acs.jpclett.1c00962) is a chain tethered to a plane, the chain having excluded volume and hydrodynamic interaction with end-to-end reactions. From our scaling argument, such a chain obeys a law of mass action where the macroscopic reaction rate is proportional to the microscopic reaction rate multiplied by the probability that the chain ends are close together. More precisely, this means for long chains there is no diffusion controlled limit. In addition, a polymer attached to a plane where the end reacts with the entire plane, end-to-wall reactions, was also investigated. For sufficiently long polymers, this system is always diffusion controlled, even with excluded volume and hydrodynamic interaction. We test the scaling arguments for the simplest case of a non-self-avoiding chains obeying Rouse dynamics. The numerical results agree with the scaling analysis for both end-to-wall and end-to-end reactions of the grafted chain. In particular, our numerical simulations support the end-to-end reaction of a tethered non-self-avoiding is the marginal case in the scaling sense.</p>","PeriodicalId":790,"journal":{"name":"The European Physical Journal E","volume":"47 11","pages":""},"PeriodicalIF":1.8,"publicationDate":"2024-12-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142757969","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
A study of novel linear Diophantine fuzzy topological numbers and their application to communicable diseases 新型线性丢番图模糊拓扑数及其在传染病中的应用研究
IF 1.8 4区 物理与天体物理 Q4 CHEMISTRY, PHYSICAL Pub Date : 2024-12-01 DOI: 10.1140/epje/s10189-024-00460-5
Siti Norziahidayu Amzee Zamri, Muhammad Azeem, Muhammad Imran, Muhammad Kamran Jamil, Bandar Almohsen

The idea of linear Diophantine fuzzy sets (LDFs) is a novel tool for analysis, soft computing, and optimization. Recently, the concept of a linear Diophantine fuzzy graph has been proposed in 2022. The aim of this research is to extend topological numbers to LDFSs. A real value assigned to a particular graph is known as a topological graph theoretic parameter. We extend the bound of the crisp graph toward the linear Diophantine fuzzy graph (LDFG), including the edge and vertex deletion operations via LDFG theoretic parameters. We also investigate the interesting bound of the LDFGs via LDFG theoretic parameters. Finally, for decision-making problems, we developed an algorithm by exploiting the relationship between LDFG theoretic parameters and LDFSs. Based on the established approach, we discussed a numerical example of an application of a medical diagnosis using the linear Diophantine fuzzy Sombor graph parameter and the first, fifth, and sixth versions of the linear Diophantine fuzzy Sombor graph parameters.

A way to the extension of fuzzy topological numbers.

线性丢番图模糊集的思想是一种新的分析、软计算和优化工具。最近,线性丢番图模糊图的概念在2022年被提出。本研究的目的是将拓扑数扩展到LDFSs。给定给特定图的实值称为拓扑图理论参数。我们将清晰图的界扩展到线性丢芬图(LDFG),包括通过LDFG理论参数的边和顶点删除操作。我们还通过LDFG理论参数研究了LDFG的有趣界。最后,针对决策问题,利用LDFG理论参数与ldfs之间的关系,开发了一种算法。基于所建立的方法,我们讨论了一个使用线性丢芬图模糊Sombor图参数和线性丢芬图模糊Sombor图参数的第一、第五和第六版本的医学诊断应用的数值例子。模糊拓扑数的一种扩展方法。
{"title":"A study of novel linear Diophantine fuzzy topological numbers and their application to communicable diseases","authors":"Siti Norziahidayu Amzee Zamri,&nbsp;Muhammad Azeem,&nbsp;Muhammad Imran,&nbsp;Muhammad Kamran Jamil,&nbsp;Bandar Almohsen","doi":"10.1140/epje/s10189-024-00460-5","DOIUrl":"10.1140/epje/s10189-024-00460-5","url":null,"abstract":"<p>The idea of linear Diophantine fuzzy sets (LDFs) is a novel tool for analysis, soft computing, and optimization. Recently, the concept of a linear Diophantine fuzzy graph has been proposed in 2022. The aim of this research is to extend topological numbers to LDFSs. A real value assigned to a particular graph is known as a topological graph theoretic parameter. We extend the bound of the crisp graph toward the linear Diophantine fuzzy graph (LDFG), including the edge and vertex deletion operations via LDFG theoretic parameters. We also investigate the interesting bound of the LDFGs via LDFG theoretic parameters. Finally, for decision-making problems, we developed an algorithm by exploiting the relationship between LDFG theoretic parameters and LDFSs. Based on the established approach, we discussed a numerical example of an application of a medical diagnosis using the linear Diophantine fuzzy Sombor graph parameter and the first, fifth, and sixth versions of the linear Diophantine fuzzy Sombor graph parameters.</p><p>A way to the extension of fuzzy topological numbers.</p>","PeriodicalId":790,"journal":{"name":"The European Physical Journal E","volume":"47 11","pages":""},"PeriodicalIF":1.8,"publicationDate":"2024-12-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142757940","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Universality class of interacting directed single- and double-strand homopolymers 相互作用的定向单链和双链均聚物的普遍性类别
IF 1.8 4区 物理与天体物理 Q4 CHEMISTRY, PHYSICAL Pub Date : 2024-11-27 DOI: 10.1140/epje/s10189-024-00461-4
Richard Dengler

This work examines a field theory for directed homopolymers in a good solvent. The field theory is based on a lattice model for single- and double-strand polymers with length variables, direction-dependent pairing energy and interactions. As for the less explicit O(n)-symmetric model, there is a close relation to the conventional one-component branched polymer and the associated Lee-Yang problem. We derive results in the limiting cases of nearly complete denaturation and nearly complete renaturation. The single-strand critical exponent (nu _{varphi }) is calculated in two-loop order. A plausible physical realization is RNA molecules with a periodic base sequence like AUAU.

这项研究探讨了良好溶剂中定向均聚物的场理论。该场理论基于具有长度变量、方向配对能和相互作用的单链和双链聚合物晶格模型。至于不那么明确的 O(n)- 对称模型,则与传统的单组分支化聚合物和相关的李-杨问题有密切关系。我们得出了近乎完全变性和近乎完全再变性的极限情况下的结果。单链临界指数 (nu _{varphi }) 是以双环阶计算的。具有类似 AUAU 周期性碱基序列的 RNA 分子是一种可信的物理实现。
{"title":"Universality class of interacting directed single- and double-strand homopolymers","authors":"Richard Dengler","doi":"10.1140/epje/s10189-024-00461-4","DOIUrl":"10.1140/epje/s10189-024-00461-4","url":null,"abstract":"<div><p>This work examines a field theory for directed homopolymers in a good solvent. The field theory is based on a lattice model for single- and double-strand polymers with length variables, direction-dependent pairing energy and interactions. As for the less explicit O(n)-symmetric model, there is a close relation to the conventional one-component branched polymer and the associated Lee-Yang problem. We derive results in the limiting cases of nearly complete denaturation and nearly complete renaturation. The single-strand critical exponent <span>(nu _{varphi })</span> is calculated in two-loop order. A plausible physical realization is RNA molecules with a periodic base sequence like AUAU.</p></div>","PeriodicalId":790,"journal":{"name":"The European Physical Journal E","volume":"47 11","pages":""},"PeriodicalIF":1.8,"publicationDate":"2024-11-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142714656","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Modeling straight and circle swimmers: from single swimmer to collective motion 直泳和环泳运动员建模:从单泳到集体运动
IF 1.8 4区 物理与天体物理 Q4 CHEMISTRY, PHYSICAL Pub Date : 2024-11-18 DOI: 10.1140/epje/s10189-024-00458-z
Francesco Michele Ventrella, Guido Boffetta, Massimo Cencini, Filippo De Lillo

We propose a simple numerical model for the motion of microswimmers based on the immersed boundary method. The swimmer, either pusher or puller, is represented by a distribution of point forces corresponding to the body and the flagellum. We study in particular the minimal model consisting of only three beads (two for the body and one for the flagellum) connected by rigid, inextensible links. When the beads are collinear, standard straight swimming is realized and, in the absence of propulsion, we demonstrate that the model recovers Jeffery’s equation for a thin rod. Conversely, by imposing an angle between body and flagellum the swimmer moves on circular orbits. We discuss how two swimmers, in collinear or non-collinear geometry, scatter upon encounter. Finally, we explore the dynamics of a large number of swimmers reacting to one another only via hydrodynamic interactions, and exemplify their complex collective dynamics in both straight and circular swimmers.

我们提出了一种基于沉浸边界法的微型游泳者运动的简单数值模型。游泳者,无论是推动者还是牵引者,都由与身体和鞭毛相对应的点力分布来表示。我们特别研究了仅由三颗珠子(两颗代表身体,一颗代表鞭毛)组成的最小模型,这三颗珠子由刚性、不可拉伸的链接连接。当珠子相互平行时,可实现标准的直线游动,在没有推进力的情况下,我们证明该模型恢复了杰弗里方程中的细杆。相反,如果在身体和鞭毛之间施加一个角度,游泳者就会在圆形轨道上运动。我们讨论了两个处于共线或非共线几何形状中的游泳者如何在相遇时分散。最后,我们探讨了大量游动体仅通过流体动力学相互作用相互反应的动力学,并举例说明了直线游动体和环形游动体的复杂集体动力学。
{"title":"Modeling straight and circle swimmers: from single swimmer to collective motion","authors":"Francesco Michele Ventrella,&nbsp;Guido Boffetta,&nbsp;Massimo Cencini,&nbsp;Filippo De Lillo","doi":"10.1140/epje/s10189-024-00458-z","DOIUrl":"10.1140/epje/s10189-024-00458-z","url":null,"abstract":"<p>We propose a simple numerical model for the motion of microswimmers based on the immersed boundary method. The swimmer, either pusher or puller, is represented by a distribution of point forces corresponding to the body and the flagellum. We study in particular the minimal model consisting of only three beads (two for the body and one for the flagellum) connected by rigid, inextensible links. When the beads are collinear, standard straight swimming is realized and, in the absence of propulsion, we demonstrate that the model recovers Jeffery’s equation for a thin rod. Conversely, by imposing an angle between body and flagellum the swimmer moves on circular orbits. We discuss how two swimmers, in collinear or non-collinear geometry, scatter upon encounter. Finally, we explore the dynamics of a large number of swimmers reacting to one another only via hydrodynamic interactions, and exemplify their complex collective dynamics in both straight and circular swimmers.</p>","PeriodicalId":790,"journal":{"name":"The European Physical Journal E","volume":"47 11","pages":""},"PeriodicalIF":1.8,"publicationDate":"2024-11-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142646615","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
期刊
The European Physical Journal E
全部 Acc. Chem. Res. ACS Applied Bio Materials ACS Appl. Electron. Mater. ACS Appl. Energy Mater. ACS Appl. Mater. Interfaces ACS Appl. Nano Mater. ACS Appl. Polym. Mater. ACS BIOMATER-SCI ENG ACS Catal. ACS Cent. Sci. ACS Chem. Biol. ACS Chemical Health & Safety ACS Chem. Neurosci. ACS Comb. Sci. ACS Earth Space Chem. ACS Energy Lett. ACS Infect. Dis. ACS Macro Lett. ACS Mater. Lett. ACS Med. Chem. Lett. ACS Nano ACS Omega ACS Photonics ACS Sens. ACS Sustainable Chem. Eng. ACS Synth. Biol. Anal. Chem. BIOCHEMISTRY-US Bioconjugate Chem. BIOMACROMOLECULES Chem. Res. Toxicol. Chem. Rev. Chem. Mater. CRYST GROWTH DES ENERG FUEL Environ. Sci. Technol. Environ. Sci. Technol. Lett. Eur. J. Inorg. Chem. IND ENG CHEM RES Inorg. Chem. J. Agric. Food. Chem. J. Chem. Eng. Data J. Chem. Educ. J. Chem. Inf. Model. J. Chem. Theory Comput. J. Med. Chem. J. Nat. Prod. J PROTEOME RES J. Am. Chem. Soc. LANGMUIR MACROMOLECULES Mol. Pharmaceutics Nano Lett. Org. Lett. ORG PROCESS RES DEV ORGANOMETALLICS J. Org. Chem. J. Phys. Chem. J. Phys. Chem. A J. Phys. Chem. B J. Phys. Chem. C J. Phys. Chem. Lett. Analyst Anal. Methods Biomater. Sci. Catal. Sci. Technol. Chem. Commun. Chem. Soc. Rev. CHEM EDUC RES PRACT CRYSTENGCOMM Dalton Trans. Energy Environ. Sci. ENVIRON SCI-NANO ENVIRON SCI-PROC IMP ENVIRON SCI-WAT RES Faraday Discuss. Food Funct. Green Chem. Inorg. Chem. Front. Integr. Biol. J. Anal. At. Spectrom. J. Mater. Chem. A J. Mater. Chem. B J. Mater. Chem. C Lab Chip Mater. Chem. Front. Mater. Horiz. MEDCHEMCOMM Metallomics Mol. Biosyst. Mol. Syst. Des. Eng. Nanoscale Nanoscale Horiz. Nat. Prod. Rep. New J. Chem. Org. Biomol. Chem. Org. Chem. Front. PHOTOCH PHOTOBIO SCI PCCP Polym. Chem.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
0
微信
客服QQ
Book学术公众号 扫码关注我们
反馈
×
意见反馈
请填写您的意见或建议
请填写您的手机或邮箱
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
现在去查看 取消
×
提示
确定
Book学术官方微信
Book学术文献互助
Book学术文献互助群
群 号:604180095
Book学术
文献互助 智能选刊 最新文献 互助须知 联系我们:info@booksci.cn
Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。
Copyright © 2023 Book学术 All rights reserved.
ghs 京公网安备 11010802042870号 京ICP备2023020795号-1