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Development of nanostructured Ge/C anodes with a multistacking layer fabricated via Ar high-pressure sputtering for high-capacity Li+-ion batteries 开发通过氩高压溅射法制造的具有多堆积层的纳米结构 Ge/C 阳极,用于高容量锂离子电池
IF 2.3 4区 物理与天体物理 Q3 PHYSICS, APPLIED Pub Date : 2024-02-23 DOI: 10.35848/1882-0786/ad2785
Tomoki Omae, Teruya Yamada, Daiki Fujikake, Takahiro Kozawa and Giichiro Uchida
To realize high-capacity Ge anodes for next-generation Li+-ion batteries, a multilayer anode with a C(top)/Ge(middle)/C(bottom) structure was developed, where nanostructured amorphous Ge (a-Ge) and amorphous-like carbon films with a grain size of 10–20 nm were deposited sequentially by high-pressure Ar sputtering at 500 mTorr. Compared with the a-Ge anode, the C(top)/a-Ge(middle)/C(bottom) multistacking layer anode showed improved capacity degradation for repeated lithiation/delithiation reactions and achieved a high capacity of 910 mAh g−1 with no capacity fading after 90 cycles at a C-rate of 0.1.
为了实现下一代锂离子电池的高容量 Ge 阳极,我们开发了一种具有 C(顶部)/Ge(中部)/C(底部)结构的多层阳极,通过在 500 mTorr 条件下进行高压氩气溅射,依次沉积了晶粒尺寸为 10-20 nm 的纳米结构非晶态 Ge(a-Ge)和非晶态类碳薄膜。与 a-Ge 阳极相比,C(上)/a-Ge(中)/C(下)多堆叠层阳极在重复锂化/退锂反应中的容量衰减情况有所改善,在 C 率为 0.1 的条件下,经过 90 个循环后,容量达到 910 mAh g-1,且无容量衰减。
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引用次数: 0
Temperature dependence of liquid-gallium ordering on the surface of epitaxially grown GaN 外延生长氮化镓表面液态镓有序化的温度依赖性
IF 2.3 4区 物理与天体物理 Q3 PHYSICS, APPLIED Pub Date : 2024-02-20 DOI: 10.35848/1882-0786/ad237b
Takuo Sasaki, Takuya Iwata, Kanya Sugitani, Takahiro Kawamura, Toru Akiyama and Masamitu Takahasi
The three-dimensional ordering of the gallium (Ga) adlayers on GaN(0001) and (000 ) surfaces was probed using in situ X-ray scattering under MBE conditions. An ordered bilayer of Ga forms on GaN(0001) but the ordering decreases at substrate temperatures of <450 °C, consistent with the mechanism of non-equilibrium epitaxial growth. Monolayer Ga that forms on GaN(000 ) is laterally disordered and has no temperature dependence, along with droplets of excess Ga. The vertical and lateral B-factors for each Ga layer were confirmed using first-principles molecular dynamics calculations.
在 MBE 条件下,利用原位 X 射线散射探测了 GaN(0001)和(000 )表面镓(Ga)叠层的三维有序性。在氮化镓(0001)上形成了有序的双层镓,但在衬底温度<450 ℃时有序性降低,这与非平衡外延生长的机制一致。在氮化镓(000 )上形成的单层镓是横向无序的,并且与温度无关,同时还有过量的镓滴。第一原理分子动力学计算证实了每个镓层的垂直和横向 B 因子。
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引用次数: 0
Suppression of electromagnetic crosstalk by differential excitation for SAW generation 利用差分激励抑制声表面波产生的电磁串扰
IF 2.3 4区 物理与天体物理 Q3 PHYSICS, APPLIED Pub Date : 2024-02-15 DOI: 10.35848/1882-0786/ad253f
Shunsuke Ota, Yuma Okazaki, Shuji Nakamura, Takehiko Oe, Hermann Sellier, Christopher Bäuerle, Nobu-Hisa Kaneko, Tetsuo Kodera and Shintaro Takada
Surface acoustic waves (SAWs) hold a vast potential in various fields such as spintronics, quantum acoustics, and electron-quantum optics, but an electromagnetic wave emanating from SAW generation circuits has often been a major hurdle. Here, we investigate a differential excitation method of interdigital transducers to generate SAWs while reducing the electromagnetic wave. The results show that electromagnetic waves are suppressed by more than 90 % in all directions. This suppression overcomes the operating limits and improves the scalability of SAW systems. Our results promise to facilitate the development of SAW-based applications in a wide range of research fields.
声表面波(SAW)在自旋电子学、量子声学和电子量子光学等多个领域具有巨大潜力,但声表面波生成电路产生的电磁波往往是一大障碍。在此,我们研究了一种数字间换能器的差分激励方法,以在产生声表面波的同时减少电磁波。结果表明,电磁波在所有方向上都被抑制了 90% 以上。这种抑制克服了声表面波系统的操作限制,提高了其可扩展性。我们的研究成果有望促进基于声表面波的应用在广泛研究领域的发展。
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引用次数: 0
Single-photon level ultrafast time-resolved measurement using two-color dual-comb-based asynchronous linear optical sampling 利用基于双色双梳齿的异步线性光学采样进行单光子级超快时间分辨测量
IF 2.3 4区 物理与天体物理 Q3 PHYSICS, APPLIED Pub Date : 2024-02-14 DOI: 10.35848/1882-0786/ad2112
Prasad Koviri, Hajime Komori, Haochen Tian, Masahiro Ishizeki, Takashi Kato, Akifumi Asahara, Ryosuke Shimizu, Thomas R. Schibli and Kaoru Minoshima
We demonstrated an ultrafast time-resolved measurement method operating at the single-photon level and employing a two-color comb-based asynchronous optical sampling (ASOPS) setup. We harnessed the two-color ASOPS photon counting approach to achieve long-term averaging of the ultralow intensity signal with a synchronized optical trigger signal, which minimizes residual timing jitter between the two combs. A pulse-width limited picosecond cross-correlation signal was successfully obtained with a power level of <1 photon/pulse. This approach enables the thorough study of ultrafast time-resolved detection of entangled photon pairs, quantum mechanical correlations in the time-frequency domain and finds wide use in optical quantum technology.
我们展示了一种在单光子水平上运行的超快时间分辨测量方法,该方法采用了基于双色梳的异步光学采样(ASOPS)装置。我们利用双色 ASOPS 光子计数方法实现了超低强度信号与同步光学触发信号的长期平均,从而最大限度地减少了两个梳状体之间的残余定时抖动。成功获得了脉冲宽度受限的皮秒级交叉相关信号,其功率水平小于 1 光子/脉冲。这种方法可以对纠缠光子对的超快时间分辨探测、时频域量子力学相关性进行深入研究,并在光量子技术中得到广泛应用。
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引用次数: 0
Core–shell yarn-structured triboelectric nanogenerator for harvesting both waterdrop and biomechanics energies 可同时收集水滴能和生物力学能的芯壳纱结构三电纳米发电机
IF 2.3 4区 物理与天体物理 Q3 PHYSICS, APPLIED Pub Date : 2024-01-29 DOI: 10.35848/1882-0786/ad1f06
Haitao Wang, Yasuyoshi Kurokawa, Jia-Han Zhang, Kazuhiro Gotoh, Xin Liu, Satoru Miyamoto and Noritaka Usami
Wearable energy harvesters (WEHs) have garnered significant attention recently due to their promising capabilities in powering wearable devices. In this research, we present a core–shell yarn-structured triboelectric nanogenerator (CY-TENG) that operates in two modes: the single-electrode TENG (SE-TENG) and the droplet-based electricity generator. This design facilitates energy harvesting from both waterdrops and biomechanics. The CY-TENG is fabricated using fluorinated ethylene propylene ultrafine heat-shrink tubes combined with stainless-steel yarns, ensuring its flexibility, durability, and weavability. Such attributes underscore its potential as a dual-function WEH.
由于可穿戴能量收集器(WEHs)在为可穿戴设备供电方面具有广阔的前景,因此近来备受关注。在这项研究中,我们提出了一种芯壳纱线结构的三电纳米发电机(CY-TENG),它有两种工作模式:单电极 TENG(SE-TENG)和基于水滴的发电机。这种设计有利于从水滴和生物力学中收集能量。CY-TENG 采用氟化乙烯丙烯超细热缩管和不锈钢纱线制成,确保了其柔韧性、耐用性和可编织性。这些特性凸显了它作为多功能 WEH 的潜力。
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引用次数: 0
The optical gain variation of Ge nanowires induced by L-valley splitting under the [110] direction stress 在[110]方向应力作用下,L-谷分裂诱导的 Ge 纳米线光增益变化
IF 2.3 4区 物理与天体物理 Q3 PHYSICS, APPLIED Pub Date : 2024-01-24 DOI: 10.35848/1882-0786/ad1db6
Xin Li, Ning Hou and Wen Xiong
The electronic structures of Ge nanowires under the [110] direction stress are calculated via effective-mass k·p theory, and the results manifest eight equivalent L-valleys will be split into fourfold degenerate L1-valleys and L2-valleys. With increasing stress, the electron levels at the L1-valleys and L2-valleys can be pushed close to and away from those at the Γ-valley, respectively, which causes the appearance of a rising inflection point in the Γ-valley filling ratio and gain peak intensity at around 2.5 GPa stress. Moreover, we prove the positive net peak gain with small diameters is apt to be obtained considering the free-carrier absorption loss.
通过有效质量k-p理论计算了[110]方向应力作用下Ge纳米线的电子结构,结果表明八个等效L-valleys将被分成四重退化的L1-valleys和L2-valleys。随着应力的增加,L1-valleys 和 L2-valleys的电子水平会分别向Γ谷靠近和远离Γ谷,从而导致Γ谷填充率和增益峰强度在应力为 2.5 GPa 左右时出现上升拐点。此外,我们还证明,考虑到自由载流子吸收损耗,小直径的正净增益峰值是很容易获得的。
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引用次数: 0
Density functional theory study on the effect of NO annealing for SiC(0001) surface with atomic-scale steps 关于氮氧化物退火对具有原子尺度阶跃的 SiC(0001) 表面影响的密度泛函理论研究
IF 2.3 4区 物理与天体物理 Q3 PHYSICS, APPLIED Pub Date : 2024-01-19 DOI: 10.35848/1882-0786/ad1bc3
Mitsuharu Uemoto, Nahoto Funaki, Kazuma Yokota, Takuji Hosoi and Tomoya Ono
The effect of NO annealing on the electronic structures of the 4H-SiC(0001)/SiO2 interface with atomic-scale steps is investigated. The characteristic behavior of conduction band edge (CBE) states is strongly affected by the atomic configurations in the SiO2 and the step structure, resulting in the discontinuity of the CBE states at the step edges, which prevents electrons from penetrating from the source to drain and decreases the mobile free-electron density. We found that the behavior of the CBE states becomes independent from the atomic configuration of the SiO2 and the density of the discontinuities is reduced after NO annealing.
研究了氮氧化物退火对具有原子尺度阶梯的 4H-SiC(0001)/SiO2 界面电子结构的影响。导带边缘(CBE)态的特征行为受到 SiO2 原子构型和阶梯结构的强烈影响,导致 CBE 态在阶梯边缘不连续,从而阻止电子从源极穿透到漏极,降低了移动自由电子密度。我们发现 CBE 态的行为与二氧化硅的原子构型无关,并且在氮化退火后,不连续态的密度会降低。
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引用次数: 0
Optical and ultrasonic dual-sensitive sensor and its application in photoacoustic microscopy 光学和超声波双敏传感器及其在光声显微镜中的应用
IF 2.3 4区 物理与天体物理 Q3 PHYSICS, APPLIED Pub Date : 2024-01-08 DOI: 10.35848/1882-0786/ad1920
Jiaye Xu, Shiqing Wu, Chao Tao and Xiaojun Liu
Multi-modality imaging is significant for biomedical applications. We propose a dual-sensitive sensor to simultaneously detect optical and ultrasonic signals. Based upon the classical piezoelectric structure, we attach a photosensitive layer made of carbon nanotubes-polydimethylsiloxane (CNTs-PDMS) composite to the surface. The photosensitive layer absorbs light and converts it into ultrasound, while allowing acoustic energy to transmit through concurrently. After optimizing the ratio of PDMS to CNTs, we increase the sensor’s light detection sensitivity and maintain the ultrasound detection sensitivity. Finally, the successful implementation in mouse ear optical attenuation–photoacoustic imaging demonstrates the dual-sensitive sensor’s potential application in multi-modality imaging.
多模态成像对生物医学应用意义重大。我们提出了一种可同时检测光学和超声波信号的双敏传感器。在经典压电结构的基础上,我们在其表面附加了由碳纳米管-聚二甲基硅氧烷(CNTs-PDMS)复合材料制成的光敏层。光敏层吸收光并将其转化为超声波,同时允许声能通过。通过优化 PDMS 与 CNT 的比例,我们提高了传感器的光探测灵敏度,并保持了超声探测灵敏度。最后,在鼠耳光学衰减-光声成像中的成功应用证明了双敏传感器在多模态成像中的潜在应用。
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引用次数: 0
Green-wavelength GaN-based photonic-crystal surface-emitting lasers 基于氮化镓的绿波长光子晶体表面发射激光器
IF 2.3 4区 物理与天体物理 Q3 PHYSICS, APPLIED Pub Date : 2024-01-03 DOI: 10.35848/1882-0786/ad126f
Natsuo Taguchi, Akinori Iwai, Masahiro Noguchi, Hiroaki Takahashi, Atsuo Michiue, Menaka De Zoysa, Takuya Inoue, Kenji Ishizaki and Susumu Noda
Visible-wavelength GaN-based photonic-crystal surface-emitting lasers (PCSELs) have attracted attention for various applications, such as materials processing, high-brightness illuminations, and displays. In this letter, we demonstrate GaN-based PCSELs at green wavelengths. We formed a photonic crystal (PC) in p-GaN and filled holes of the PC with SiO2 to ensure device stability. Through a current injection test under pulsed conditions and spectral analysis, we confirmed that the fabricated device possessed Γ-point single-mode oscillation at wavelengths above 505 nm. Our results have the potential to further expand the applications of PCSELs and semiconductor lasers in visible region.
基于氮化镓的可见光波长光子晶体表面发射激光器(PCSEL)在材料加工、高亮度照明和显示等各种应用领域备受关注。在这封信中,我们展示了绿色波长的氮化镓基 PCSEL。我们在 p-GaN 中形成了光子晶体 (PC),并用二氧化硅填充 PC 中的孔,以确保器件的稳定性。通过脉冲条件下的电流注入测试和光谱分析,我们证实所制造的器件在 505 nm 以上波长具有Γ点单模振荡。我们的研究成果有望进一步拓展 PCSEL 和半导体激光器在可见光区域的应用。
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引用次数: 0
Nitrogen-displacement-related recombination centers generated by electron beam irradiation in n-type and p-type homoepitaxial GaN layers 电子束辐照在 n 型和 p 型同外延氮化镓层中产生的氮置换相关重组中心
IF 2.3 4区 物理与天体物理 Q3 PHYSICS, APPLIED Pub Date : 2024-01-03 DOI: 10.35848/1882-0786/ad16ad
Meguru Endo, Masahiro Horita and Jun Suda
Recombination centers originating from point defects generated by the displacement of N atoms in n-type and p-type GaN were investigated by analyzing Shockley–Read–Hall (SRH) recombination currents in homoepitaxial GaN p–n junctions. These defects were intentionally generated by electron beam (EB) irradiation at 137 keV. The net doping concentrations in p+–n junction diodes were not changed following irradiation although the levels in p–n+ junction diodes decreased as the EB fluence was increased. The SRH recombination current also increased with increases in the fluence. This work additionally evaluated the relationship between recombination lifetimes and trap concentrations obtained by deep level transient spectroscopy.
通过分析同外延氮化镓 p-n 结中的肖克利-雷德-霍尔(SRH)重组电流,研究了 n 型和 p 型氮化镓中由 N 原子位移产生的点缺陷所形成的重组中心。这些缺陷是在 137 keV 的电子束(EB)辐照下有意产生的。辐照后,p+-n 结二极管中的净掺杂浓度没有变化,但随着 EB 通量的增加,p-n+ 结二极管中的掺杂浓度有所下降。SRH 重组电流也随着通量的增加而增加。这项工作还评估了重组寿命与通过深层瞬态光谱获得的陷阱浓度之间的关系。
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引用次数: 0
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Applied Physics Express
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