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Extraction of interfacial thermal resistance across an organic/semiconductor interface using optical-interference contactless thermometry 利用光干涉非接触测温法提取有机物/半导体界面的界面热阻
IF 2.3 4区 物理与天体物理 Q1 Engineering Pub Date : 2024-03-06 DOI: 10.35848/1882-0786/ad2b01
Jiawen Yu, Hiroaki Hanafusa and Seiichiro Higashi
We have developed an experimental method to extract interfacial thermal resistance (ITR) at an organic/semiconductor interface based on optical-interference contactless thermometry. The proposed technique was applied to a SU-8/SiC bilayer sample, and clear oscillations in reflectivity induced by optical interference during pulse heating and cooling were observed. After fitting the observed reflectivity waveform with simulation results by a two-dimensional (2D) double-layer heat conduction model and multi-reflection calculations, ITR was extracted as 190 mm2 K W−1, which resulted in a temperature drop of 11 K at the interface. Moreover, the 2D transient temperature distribution of the sample throughout pulse heating and cooling was obtained.
我们开发了一种基于光干涉非接触测温法提取有机物/半导体界面热阻(ITR)的实验方法。我们将所提出的技术应用于 SU-8/SiC 双层样品,观察到在脉冲加热和冷却过程中光干涉引起的反射率的明显振荡。将观察到的反射率波形与二维(2D)双层热传导模型和多反射计算的模拟结果拟合后,提取出的 ITR 为 190 mm2 K W-1,这导致界面处的温度下降了 11 K。此外,还获得了样品在整个脉冲加热和冷却过程中的二维瞬态温度分布。
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引用次数: 0
Nanosecond recombination lifetimes and spin relaxation times in (110) InGaAs/AlGaAs quantum wells at room temperature 室温下 (110) InGaAs/AlGaAs 量子阱中的纳秒级重组寿命和自旋弛豫时间
IF 2.3 4区 物理与天体物理 Q1 Engineering Pub Date : 2024-03-06 DOI: 10.35848/1882-0786/ad2907
Satoshi Iba and Yuzo Ohno
Quantum wells in InGaAs/AlGaAs with (110) orientation are attractive as active layers in spin-controlled lasers with circularly polarized emission, while the spin relaxation time is expected to be larger than for (100)-oriented layers. However, the hitherto reported recombination lifetimes (40 ps) and spin relaxation times (440 ps) of (110) InGaAs/AlGaAs structures are insufficient. Here it is shown that higher growth temperatures and higher V/III beam equivalent pressure ratios than previously used in crystal growth by molecular beam epitaxy lead to recombination and spin relaxation times in the nanosecond range at RT, meeting the requirements for application in spin lasers.
具有(110)取向的 InGaAs/AlGaAs 量子阱作为具有圆偏振发射的自旋控制激光器的有源层具有吸引力,而自旋弛豫时间预计比(100)取向层更长。然而,迄今为止所报道的 (110) InGaAs/AlGaAs 结构的重组寿命(40 ps)和自旋弛豫时间(440 ps)是不够的。这里的研究表明,与以前通过分子束外延方法生长晶体时使用的温度和 V/III 束等效压力比相比,更高的生长温度和 V/III 束等效压力比可以使晶体在 RT 时的重组和自旋弛豫时间达到纳秒级,从而满足自旋激光器的应用要求。
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引用次数: 0
A two-stage insulation method for suppressing thermal crosstalk in microarray sensitive units 抑制微阵列敏感单元热串扰的两级绝缘方法
IF 2.3 4区 物理与天体物理 Q1 Engineering Pub Date : 2024-03-06 DOI: 10.35848/1882-0786/ad2b00
Shining Zhu, Xin Li, Zhengjie Luo, Xuguang Jia, Yue Qin, Hao Guo, Jun Tang, Zhonghao Li, Huanfei Wen, Zongmin Ma and Jun Liu
Thermal crosstalk between array structures is a key factor in limiting the sensitivity of micro-nano array sensors. We propose a two-stage thermally isolated structure with thermal holes and heat dissipation layer and pulsed voltage heating to reduce thermal crosstalk. Through finite element thermal simulation analysis as well as thermal interference test, the results show that the thermal crosstalk of the two-stage structure is reduced by 12.89% and 39.67%, respectively, in the steady state compared to the structure with no thermal isolation, and pulsed voltage heating leads to the thermal crosstalk of the two-stage structure to be <10%.
阵列结构之间的热串扰是限制微纳阵列传感器灵敏度的关键因素。我们提出了一种带有导热孔和散热层的两级热隔离结构,并通过脉冲电压加热来减少热串扰。通过有限元热仿真分析和热干扰测试,结果表明与没有热隔离的结构相比,两级结构的热串扰在稳态下分别减少了 12.89% 和 39.67%,脉冲电压加热使两级结构的热串扰小于 10%。
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引用次数: 0
Facile and controllable chemical doping of conducting polymers with an ionic liquid dopant 用离子液体掺杂剂对导电聚合物进行简便、可控的化学掺杂
IF 2.3 4区 物理与天体物理 Q1 Engineering Pub Date : 2024-03-02 DOI: 10.35848/1882-0786/ad2f66
Hisaaki Tanaka, Shun-ichiro Ito, Toru Matsui, T. Takenobu
A facile method for chemical doping of conducting polymers is demonstrated with an ionic liquid containing FeCl4 - anions as the oxidizing agents. A drop of the ionic liquid on the film of a typical semicrystalline polymer immediately changed the room temperature conductivity to 500 S/cm. The highly conductive state originated from both the high doping level and the high crystallinity of the doped film, as confirmed by optical absorption and X-ray diffraction measurements, respectively. Furthermore, the doping level was continuously controlled by the gate voltage of the ionic-liquid-gated transistor structure through an electrochemical dedoping process.
使用含有 FeCl4 阴离子的离子液体作为氧化剂,展示了一种对导电聚合物进行化学掺杂的简便方法。在典型的半结晶聚合物薄膜上滴上一滴离子液体,室温下的导电率立即变为 500 S/cm。光学吸收和 X 射线衍射测量分别证实,这种高导电状态源于掺杂薄膜的高掺杂水平和高结晶度。此外,通过电化学掺杂过程,离子液体门控晶体管结构的栅极电压可持续控制掺杂水平。
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引用次数: 0
Realizing reliable linearity and Forming-free in conductive bridging random access memory synapse by alloy electrode engineering 通过合金电极工程实现导电桥接随机存取存储器突触的可靠线性度和无成形性
IF 2.3 4区 物理与天体物理 Q1 Engineering Pub Date : 2024-03-02 DOI: 10.35848/1882-0786/ad2f65
Ao Chen, Puyi Zhang, Yiwei Zheng, Xiaoxu Yuan, Guokun Ma, Yiheng Rao, Houzhao Wan, Nengfan Liu, Qin Chen, Daohong Yang, Hao Wang
In this work, by Alloy electrode engineering, the Ti-Ag device performed the Forming-free property because Ag ions were promoted to migrate into the GeTeOx layer to form a thicker conductive filament. This facilitated a uniform change in conductance with the pulse number, and the alloy synapse achieved a significant improvement in linearity (350%), which demonstrated its enhancement in recognition accuracy. To further validate its potential as a comprehensive artificial synapse, the multi-essential synaptic behaviors, including spike-timing-dependent plasticity, spike-rate-dependent plasticity, paired-pulse facilitation, post-tetanic potentiation, and excitatory postsynaptic current, were achieved successfully.
在这项工作中,通过合金电极工程,钛-银器件实现了无成型特性,因为银离子被促进迁移到 GeTeOx 层中,形成更粗的导电丝。这有利于电导率随脉冲数的变化而均匀变化,合金突触的线性度也得到了显著提高(350%),从而证明了其识别准确性的增强。为了进一步验证其作为综合性人工突触的潜力,我们成功实现了多种重要的突触行为,包括尖峰计时相关可塑性、尖峰速率相关可塑性、配对脉冲促进、四肽后电位和兴奋性突触后电流。
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引用次数: 0
Development of nanostructured Ge/C anodes with a multistacking layer fabricated via Ar high-pressure sputtering for high-capacity Li+-ion batteries 开发通过氩高压溅射法制造的具有多堆积层的纳米结构 Ge/C 阳极,用于高容量锂离子电池
IF 2.3 4区 物理与天体物理 Q1 Engineering Pub Date : 2024-02-23 DOI: 10.35848/1882-0786/ad2785
Tomoki Omae, Teruya Yamada, Daiki Fujikake, Takahiro Kozawa and Giichiro Uchida
To realize high-capacity Ge anodes for next-generation Li+-ion batteries, a multilayer anode with a C(top)/Ge(middle)/C(bottom) structure was developed, where nanostructured amorphous Ge (a-Ge) and amorphous-like carbon films with a grain size of 10–20 nm were deposited sequentially by high-pressure Ar sputtering at 500 mTorr. Compared with the a-Ge anode, the C(top)/a-Ge(middle)/C(bottom) multistacking layer anode showed improved capacity degradation for repeated lithiation/delithiation reactions and achieved a high capacity of 910 mAh g−1 with no capacity fading after 90 cycles at a C-rate of 0.1.
为了实现下一代锂离子电池的高容量 Ge 阳极,我们开发了一种具有 C(顶部)/Ge(中部)/C(底部)结构的多层阳极,通过在 500 mTorr 条件下进行高压氩气溅射,依次沉积了晶粒尺寸为 10-20 nm 的纳米结构非晶态 Ge(a-Ge)和非晶态类碳薄膜。与 a-Ge 阳极相比,C(上)/a-Ge(中)/C(下)多堆叠层阳极在重复锂化/退锂反应中的容量衰减情况有所改善,在 C 率为 0.1 的条件下,经过 90 个循环后,容量达到 910 mAh g-1,且无容量衰减。
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引用次数: 0
Temperature dependence of liquid-gallium ordering on the surface of epitaxially grown GaN 外延生长氮化镓表面液态镓有序化的温度依赖性
IF 2.3 4区 物理与天体物理 Q1 Engineering Pub Date : 2024-02-20 DOI: 10.35848/1882-0786/ad237b
Takuo Sasaki, Takuya Iwata, Kanya Sugitani, Takahiro Kawamura, Toru Akiyama and Masamitu Takahasi
The three-dimensional ordering of the gallium (Ga) adlayers on GaN(0001) and (000 ) surfaces was probed using in situ X-ray scattering under MBE conditions. An ordered bilayer of Ga forms on GaN(0001) but the ordering decreases at substrate temperatures of <450 °C, consistent with the mechanism of non-equilibrium epitaxial growth. Monolayer Ga that forms on GaN(000 ) is laterally disordered and has no temperature dependence, along with droplets of excess Ga. The vertical and lateral B-factors for each Ga layer were confirmed using first-principles molecular dynamics calculations.
在 MBE 条件下,利用原位 X 射线散射探测了 GaN(0001)和(000 )表面镓(Ga)叠层的三维有序性。在氮化镓(0001)上形成了有序的双层镓,但在衬底温度<450 ℃时有序性降低,这与非平衡外延生长的机制一致。在氮化镓(000 )上形成的单层镓是横向无序的,并且与温度无关,同时还有过量的镓滴。第一原理分子动力学计算证实了每个镓层的垂直和横向 B 因子。
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引用次数: 0
Multi-focus manipulation system based on SNES aberration self-calibration 基于 SNES 像差自我校准的多焦操控系统
IF 2.3 4区 物理与天体物理 Q1 Engineering Pub Date : 2024-02-20 DOI: 10.35848/1882-0786/ad2afe
Linxian Liu, Jiahao Liu, Chunxu Ding, Jiamiao Yang, Jia Gao, Yuan Qu, Qiaozhi He, Rongjun Shao
Wavefront shaping using digital micromirror devices (DMDs) allows inertia-free focus manipulation with numerous modulation modes and high refresh rates. However, the aberration caused by the curvature of DMD affects the focusing performance. Here, we propose an aberration self-calibration method based on separable natural evolution strategies (SNES). This method searches optimal Zernike coefficients of aberration globally and completes compensation using super-pixel encoding. Compared to the genetic algorithm method, we improve the speed by 62% and achieve better-focused spots. It enables simultaneous scanning of 25 independent focal spots. This advancement supports wavefront shaping applications in optical imaging, industrial inspection, and laser processing.
使用数字微镜设备(DMD)进行波前整形可实现无惯性聚焦操作,具有多种调制模式和高刷新率。然而,DMD 的曲率造成的像差会影响聚焦性能。在此,我们提出了一种基于可分离自然演化策略(SNES)的像差自校准方法。该方法在全局范围内搜索最佳畸变 Zernike 系数,并利用超级像素编码完成补偿。与遗传算法相比,我们将速度提高了 62%,并获得了更好的聚焦光斑。它能同时扫描 25 个独立的焦点。这一进步为光学成像、工业检测和激光加工中的波前整形应用提供了支持。
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引用次数: 0
Improvement of film quality and solar cell properties of perovskite by the addition of N-benzylhydroxylamine 通过添加 N-苄基羟胺改善过氧化物的薄膜质量和太阳能电池性能
IF 2.3 4区 物理与天体物理 Q1 Engineering Pub Date : 2024-02-16 DOI: 10.35848/1882-0786/ad2a05
Keisuke Nagasawa, Takeshi Sano, Viet Chau Nguyen, Yutaka Okuyama, Yuya Sayama, Ryosuke Oikawa, Keigo Hoshi, Takayuki Chiba, Junji Kido
In this study on perovskite solar cells (PVSCs), we incorporated N-benzylhydroxylamine (N-BzHoA) as an additive into the precursor solution. The addition of N-BzHoA suppressed the formation of unwanted PbI2 and δ-phase perovskite without affecting the band gap, confirming uniform and large grains in the perovskite film. The fabricated inverted PVSCs exhibited remarkably improved properties compared to the control device, with a power conversion efficiency (PCE) of 17.49%, reduced hysteresis, and more than 89% retention of the initial capacity after 100 h of light exposure. Thus, this study highlights the effectiveness of N-BzHoA as an effective additive for inverted PVSCs.
在这项关于透辉石太阳能电池(PVSC)的研究中,我们在前驱体溶液中加入了 N-苄基羟胺(N-BzHoA)作为添加剂。N-BzHoA 的加入抑制了不需要的 PbI2 和 δ 相包晶石的形成,且不影响带隙,证实了包晶石薄膜中晶粒的均匀性和大型化。与对照器件相比,所制备的倒置 PVSCs 性能显著提高,功率转换效率 (PCE) 达到 17.49%,滞后现象减少,光照射 100 小时后的初始容量保持率超过 89%。因此,本研究强调了 N-BzHoA 作为倒置式光伏电池有效添加剂的有效性。
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引用次数: 0
Lightweight and high-precision materials property prediction using pre-trained Graph Neural Networks and its application to small dataset 使用预训练的图神经网络进行轻量级和高精度材料属性预测及其在小型数据集中的应用
IF 2.3 4区 物理与天体物理 Q1 Engineering Pub Date : 2024-02-16 DOI: 10.35848/1882-0786/ad2a06
Kento Nishio, Kiyou Shibata, Teruyasu Mizoguchi
Large data sets are essential for building deep learning models. However, generating large datasets with higher theoretical levels and larger computational models remains difficult due to the high cost of first-principles calculation. Here, we propose a lightweight and highly accurate machine learning approach using pre-trained Graph Neural Networks (GNNs) for industrially important but difficult to scale models. The proposed method was applied to a small dataset of graphene surface systems containing surface defects, and achieved comparable accuracy with six orders of magnitude faster learning than when the GNN was trained from scratch.
大型数据集对于构建深度学习模型至关重要。然而,由于第一原理计算成本高昂,生成具有更高理论水平和更大计算模型的大型数据集仍然困难重重。在这里,我们提出了一种轻量级、高精度的机器学习方法,使用预先训练好的图神经网络(GNN)来建立工业上重要但难以扩展的模型。我们将所提出的方法应用于含有表面缺陷的石墨烯表面系统的小型数据集,与从头开始训练 GNN 相比,该方法以快六个数量级的学习速度达到了相当的准确性。
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引用次数: 0
期刊
Applied Physics Express
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