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Enhanced visible-light manipulation of the ferromagnetism in 3D cobalt nanosphere by sphere size engineering 利用球形尺寸工程增强三维钴纳米球铁磁性的可见光操纵
IF 4 2区 物理与天体物理 Q2 PHYSICS, APPLIED Pub Date : 2026-03-02 DOI: 10.1063/5.0306460
Shishun Zhao, Jian Wang, Yifan Zhao, Rui Wang, Ye Quan, Yating Shi, Ge Wang, Meng Zhao, Ming Liu
Rapid and energy-efficient magnetization control is essential for advancing next-generation magnetic sensors and memory technologies. Photovoltaic gating of magnetism via light irradiation leverages advances in solar-cell engineering and electric-field-controlled magnetism, offering enhanced tunability at reduced power consumption. In this study, we report the fabrication of a cobalt nanosphere-photovoltaic material thin-film device. By systematically tuning the nanosphere diameter, concentration, and film thickness, we achieved an 11.5% reduction in magnetization under visible-light illumination (200 mW/cm2, 6.93 × 1017 photons cm−2 s−1). Notably, the relative magnetization reduction scales linearly with 1/r2, where r is the effective nanosphere radius. This behavior is attributed to a surface-electrical potential conservation mechanism, suggesting that increasing the surface-area-to-volume ratio enhances magneto-optical tunability. These insights provide a rational design strategy for light-modulated magnetic nanodevices with potential applications in reconfigurable sensors and memory elements.
快速和节能的磁化控制对于推进下一代磁传感器和存储技术至关重要。通过光照射的光伏门控磁性利用了太阳能电池工程和电场控制磁性的进步,在降低功耗的情况下提供了增强的可调性。在这项研究中,我们报道了钴纳米球光伏材料薄膜器件的制造。通过系统地调整纳米球直径、浓度和薄膜厚度,我们在可见光照射下(200 mW/cm2, 6.93 × 1017光子cm−2 s−1)的磁化强度降低了11.5%。值得注意的是,相对磁化强度降低与1/r2呈线性关系,其中r为有效纳米球半径。这种行为归因于表面电势守恒机制,表明增加表面积与体积比可以增强磁光可调性。这些见解为光调制磁性纳米器件在可重构传感器和存储元件中的潜在应用提供了一种合理的设计策略。
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引用次数: 0
Enhanced Raman scattering by fast GaN phonon-polaritons 快速GaN声子极化子增强拉曼散射
IF 4 2区 物理与天体物理 Q2 PHYSICS, APPLIED Pub Date : 2026-03-02 DOI: 10.1063/5.0307163
Mayssoune Mina, Toni Alhaddad, Olivier Pagès
Phonon-polaritons propagating in crystal volume offer the possibility of transferring information throughout matter (via phonons) at high (photon-like) velocity and tunable frequency/wavelength in the far-infrared. However, from the phonon-polariton Raman cross section, the phonon and photon advantages seem mutually exclusive. Either the phonon-polaritons are fast (photon-like) but hardly supported by the lattice (not phonon-like), or they are well supported by the lattice (testified by a high Raman efficiency) but slow (not photon-like). An optimal phonon–photon coupling is currently being searched for in hexagonal GaN by near-forward Raman scattering across parallel crystal faces with an in-plane singular c→-axis. Two accessible phonons, i.e., the ordinary A1 and E1 ones, plus two refractive indices, i.e., the ordinary and extraordinary ones, generate various phonon-polariton candidates. Notably, in perfect forward Raman scattering and in crossed polarizations of the incident (∥c→) and scattered lights, which, altogether, maximizes the transferred wavevector to the crystal at minimum scattering angle, a fast phonon-polariton, stemming from the bottleneck of the E1 dispersion on entry to the deep photon-like regime, is activated. It is well supported by the lattice since its Raman signal is strong and sharp, enhanced by multi-reflection of the laser beam between crystal faces at near-normal incidence. This fast Raman-enhanced phonon-polariton is interesting for infrared photonics in that it cumulates the advantages of a photon (speed) and of a phonon (Raman intensity). Besides, it commutates from a phonon-polariton to a phonon by deviating from normal incidence or by permuting the incident and scattered polarizations, with potential applications as a vibrational switch.
声子-极化子在晶体体积中传播,提供了在远红外中以高(光子样)速度和可调频率/波长在整个物质中(通过声子)传递信息的可能性。然而,从声子-极化子拉曼截面来看,声子和光子的优势似乎是相互排斥的。声子极化子要么是快速的(类光子),但几乎没有晶格支持(不是类声子),要么是晶格支持得很好(由高拉曼效率证明),但速度很慢(不是类光子)。在六角形氮化镓中,通过近正向拉曼散射在平面奇异c→-轴平行晶面上寻找最佳声子-光子耦合。两个可达声子,即普通A1和E1声子,加上两个折射率,即普通折射率和特殊折射率,产生各种声子极化子候选者。值得注意的是,在完美的前拉曼散射和入射光(∥c→)和散射光的交叉极化中,在最小散射角下最大限度地向晶体转移波向量,一个快速声子极化子被激活,这是由于E1色散进入深光子区时的瓶颈造成的。由于它的拉曼信号强而锐利,在近正入射的情况下,激光在晶体表面之间的多次反射增强了它的拉曼信号,因此得到了晶格的良好支持。这种快速拉曼增强声子极化子对于红外光子学来说是有趣的,因为它积累了光子(速度)和声子(拉曼强度)的优点。此外,它通过偏离正常入射或通过排列入射和散射极化,从声子-极化子转换为声子,具有作为振动开关的潜在应用。
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引用次数: 0
Surface acoustic wave enabled all-optical determination of the interlayer elastic constants of a van der Waals interface 利用表面声波实现了范德华界面层间弹性常数的全光学测定
IF 4 2区 物理与天体物理 Q2 PHYSICS, APPLIED Pub Date : 2026-03-02 DOI: 10.1063/5.0311186
N. Yu. Frolov, A. Yu. Klokov, A. I. Sharkov, M. V. Pugachev, A. Yu. Kuntsevich
Understanding the properties of two-dimensional material interfaces with the substrate is necessary for device applications. Surface acoustic wave propagation through a layered material flake on a substrate could provide unique information on the transverse rigidity of the flake-to-substrate interaction. Ultrasonic waves were generated by a focused femtosecond laser pulse at the surface of a model system—fused silica with hBN flake transferred above. Using an all-optical spatially resolved pump–probe interferometric technique, the spatial dependencies of the surface vertical velocity profiles were measured. The measurements reveal the appearance of surface acoustic wave dispersion in the hBN flake region compared to the fused silica surface. Multilayer modeling allows us to access the longitudinal and shear elastic coupling constants c33* and c44* between hexagonal BN and the substrate.
了解与基板的二维材料界面的性质对于器件应用是必要的。表面声波通过层状材料薄片在衬底上的传播可以提供关于薄片与衬底相互作用的横向刚度的独特信息。利用聚焦飞秒激光脉冲在模型系统熔融二氧化硅表面产生超声波,并在其上转移hBN薄片。利用全光学空间分辨泵浦-探针干涉技术,测量了表面垂直速度分布的空间依赖性。测量结果显示,与熔融二氧化硅表面相比,hBN薄片区域表面声波色散的外观。多层建模使我们能够获得六边形BN与衬底之间的纵向和剪切弹性耦合常数c33*和c44*。
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引用次数: 0
Enhanced pseudocapacitance rectification by doping metalloid phosphorus in high entropy oxide (CrMnFeCoNi)3O4 在高熵氧化物(crmnnfeconi)3O4中掺杂类金属磷增强假电容整流
IF 4 2区 物理与天体物理 Q2 PHYSICS, APPLIED Pub Date : 2026-03-02 DOI: 10.1063/5.0290764
Jia-Xin Li, Bi Chen, Wei-Bin Zhang, Ashkar Batol, Huan Gou, Jun Pang, Nan-Sen Zhou, Xue-Jing Ma
Metalloid phosphorus-doped spinel-type high-entropy oxide (CrMnFeCoNi)3O4 is synthesized to solve the challenges of limited pseudocapacitance rectification for supercapacitor diodes. It demonstrates both pseudocapacitive energy storage and ionic rectification in a 1 M KOH electrolyte. This material achieves a high specific capacitance of 394.05 F g−1 at 0.5 A g−1 along with a reverse rectification ratio of 0.85 at 3 mV s−1. These properties are driven by phosphorus electronegativity, which enhances electron transfer, creates oxygen vacancies, and accelerates ion transport. The assembled supercapacitor diodes delivered a high energy density of 241.35 W h kg−1 at a power density of 5250 W kg−1 while maintaining a rectification ratio RRI of 6.95–8.8 at scan rates of 3–30 mV s−1 and a sustained RRII of 0.86. After 1000 cycles, the diode retained 84% rectification efficiency with minimal capacitance decay. This work advances iontronic circuits through dual-functional electrodes.
合成了类金属磷掺杂尖晶石型高熵氧化物(crmnnfeconi)3O4,解决了超级电容二极管有限赝电容整流的难题。在1 M KOH的电解液中证明了赝电容储能和离子整流。该材料在0.5 a g−1时具有394.05 F g−1的高比电容,在3 mV s−1时具有0.85的反向整流比。这些特性是由磷的电负性驱动的,磷的电负性增强了电子转移,产生了氧空位,加速了离子传递。在5250 W kg−1的功率密度下,组装的超级电容二极管提供了241.35 W h kg−1的高能量密度,同时在3-30 mV s−1的扫描速率下保持了6.95-8.8的整流比RRI和0.86的持续RRII。经过1000次循环后,二极管保持了84%的整流效率,电容衰减最小。这项工作通过双功能电极推进了离子电子电路。
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引用次数: 0
Temperature imaging of chips with high spatiotemporal resolution using diamond nitrogen-vacancy centers 基于金刚石氮空位中心的高时空分辨率芯片温度成像
IF 4 2区 物理与天体物理 Q2 PHYSICS, APPLIED Pub Date : 2026-03-02 DOI: 10.1063/5.0305268
Wanshan Shen, Xin Li, Xiaojiang Wang, Zhitong Yin, Lixia Zhen, Huanfei Wen, Zongmin Ma, Jun Tang, Jun Liu
The operating temperature of a chip is a critical factor determining its operational efficiency and service life. In industrial control environments, temperature imaging of a chip plays a vital role in detecting localized heat accumulation and heat dissipation system failures. Although many advanced techniques have been proposed, achieving high spatiotemporal resolution temperature imaging on the chip still presents significant challenges. In this study, we proposed a temperature imaging method based on ensemble diamond nitrogen-vacancy (NV) centers and applied it to the temperature imaging of interdigital electrodes. This method achieved temperature imaging of the chip surface with a spatial resolution of 863 nm and a temporal resolution of up to 2.05 s, capturing the changes in thermal distribution with different applied voltages. The results indicate that NV centers can overcome the limitations of traditional temperature measurement methods in terms of spatiotemporal resolution, offering a promising measurement solution for chip temperature detection.
芯片的工作温度是决定其工作效率和使用寿命的关键因素。在工业控制环境中,芯片的温度成像在检测局部热积累和散热系统故障方面起着至关重要的作用。尽管已经提出了许多先进的技术,但在芯片上实现高时空分辨率的温度成像仍然面临着重大挑战。本文提出了一种基于金刚石氮空位中心的温度成像方法,并将其应用于指间电极的温度成像。该方法实现了空间分辨率为863 nm、时间分辨率高达2.05 s的芯片表面温度成像,捕获了不同外加电压下热分布的变化。结果表明,NV中心可以克服传统温度测量方法在时空分辨率方面的局限性,为芯片温度检测提供了一种有前景的测量解决方案。
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引用次数: 0
Ferroelectric control of the layer-polarized anomalous Hall effect in a 2D TiClAsH bilayer via superposition engineering 利用叠加技术控制二维TiClAsH双分子层的层极化反常霍尔效应
IF 4 2区 物理与天体物理 Q2 PHYSICS, APPLIED Pub Date : 2026-03-02 DOI: 10.1063/5.0309665
Cong Li, Jia Li, Hongli Zhang, Xiaolong Wang, Tong Wei, Limin Liu, Linyang Li, Guodong Liu
Ferrovalley (FV) materials have attracted much attention due to their unique spin-valley coupled properties. In this work, we predict FV single-layer TiClAsH, which has 77 meV of intrinsic valley polarization. The electronic correlation effect can drive the topological phase transition from the FV state to the quantum anomalous Hall state, and its critical half-valley metallic phase can achieve complete spin polarization. By breaking the mirror symmetry of bilayer TiClAsH, the layer-locked Berry curvature distribution is achieved, and furthermore, the layer-polarized anomalous Hall effect (LPAHE) is induced. Meanwhile, reversible LPAHE switching can be achieved through sliding control of ferroelectricity. Our findings offer a good material platform to manipulate the spin splitting, valley polarization, ferroelectricity, and topological states for multi-functional device applications.
铁谷材料因其独特的自旋谷耦合特性而备受关注。在这项工作中,我们预测了具有77 meV本征谷极化的FV单层TiClAsH。电子相关效应可以驱动拓扑相变从FV态向量子反常霍尔态转变,其临界半谷金属相可以实现完全自旋极化。通过破坏双层TiClAsH的镜像对称性,实现了层锁态的Berry曲率分布,并诱导了层极化的反常霍尔效应(LPAHE)。同时,通过铁电性的滑动控制可以实现可逆的LPAHE开关。我们的发现提供了一个很好的材料平台来操纵自旋分裂、谷极化、铁电性和拓扑状态,用于多功能器件的应用。
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引用次数: 0
Revealing trace water effect on the structural and optical evolutions of blue CsPbBr3 perovskite quantum dots 揭示微量水对蓝色CsPbBr3钙钛矿量子点结构和光学演化的影响
IF 4 2区 物理与天体物理 Q2 PHYSICS, APPLIED Pub Date : 2026-03-02 DOI: 10.1063/5.0324585
Yongfeng Liu, Mingyu Guo, Qingyu Xie, Zhangcheng Pan, Bowen Zhang, Liang Zhao, Shengnan Tian, Dongdong Yan, Haimei Zhu
Quantum confined blue CsPbBr3 perovskite quantum dots (PeQDs) demonstrate superior spectral stability and easy tunability by particle size relative to their mixed halide counterparts. However, their practical application is hampered by their susceptibility to moisture-induced degradation. Herein, the structural and optical evolutions of blue CsPbBr3 PeQDs induced by trace water are systematically studied and their mechanism is elucidated. Experimental results show that trace water (H2O) induces red shift of spectra from blue to green, accompanying significant increase in photoluminescent quantum yield and one order lower non-radiative recombination rate. Furthermore, the H2O-treated PeQDs' size presents obvious increase from 6.3 to 8.0 nm without obvious change in crystalline pattern. By combining experimental characterizations, first-principles calculations, and verification experiments, we demonstrate that appropriate H2O exposure is responsible for substituting oleic acid ligand on PeQDs, resulting in particle growth and spectral red shift. Our work establishes that water attacks PeQDs via acid–base chemistry at surface ligand sites—a mechanistic insight critical for enhancing moisture stability in blue CsPbBr3 PeQDs.
相对于混合卤化物,量子受限蓝CsPbBr3钙钛矿量子点(PeQDs)在粒径上表现出优越的光谱稳定性和易于调性。然而,它们的实际应用受到水分诱导降解的影响。本文系统地研究了微量水诱导蓝色CsPbBr3 PeQDs的结构和光学演变,并阐明了其机理。实验结果表明,微量水(H2O)引起光谱由蓝向绿的红移,光致发光量子产率显著提高,非辐射复合率降低一个数量级。此外,经过h2o处理的PeQDs的尺寸从6.3 nm明显增大到8.0 nm,但晶型没有明显变化。通过结合实验表征、第一性原理计算和验证实验,我们证明了适当的水暴露是导致peqd上油酸配体取代的原因,导致颗粒生长和光谱红移。我们的研究表明,水通过表面配体位点的酸碱化学作用攻击peqd,这是增强蓝色CsPbBr3 peqd水分稳定性的关键机制。
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引用次数: 0
Giant room-temperature nonvolatile magnon on–off modulation ratio in a multiferroic Pt/Bi1.05La0.05FeO3/Pt sandwiched structure 多铁Pt/Bi1.05La0.05FeO3/Pt夹层结构中巨室温非易失性磁导子开关调制比
IF 4 2区 物理与天体物理 Q2 PHYSICS, APPLIED Pub Date : 2026-03-02 DOI: 10.1063/5.0314548
Jun Miao, Xin Cui, Wei Ye Deng, Yi Wang, Qi Liang Li
We experimentally demonstrated magnon transmission in a vertical geometry consisting of multiferroic Bi1.05La0.05FeO3 (BLFO) and heavy-metal Pt layers. Notably, a giant nonvolatile on–off modulation ratio of ∼120% under zero-field operation, together with high magnon drag efficiency (∼3.51 × 10−3 V A−1), was observed in a vertical Pt/BLFO/Pt device at room temperature. The magnon-mediated drag effect in the nonlocal Pt/BLFO/Pt symmetrical layers was investigated via the magnetic field, angle, and current density dependence. The intrinsic giant on–off modulation of the magnon signal, along withnonvolatile transport under zero-field operation and polarization-controlled Néel vectors of multiferroics, moves a possible step toward the practical utilization of multiferroic vertical magnon devices. This work may contribute to magnonic transport with high-speed, miniaturization and ultralow energy consumption.
我们通过实验证明了由多铁Bi1.05La0.05FeO3 (BLFO)和重金属Pt层组成的垂直几何结构中的磁导子传输。值得注意的是,在室温下,在垂直Pt/BLFO/Pt器件中观察到零场工作下高达120%的巨大非易失性开关调制比,以及高磁振子阻力效率(~ 3.51 × 10−3 V a−1)。通过磁场、角度和电流密度的依赖关系研究了非局部Pt/BLFO/Pt对称层中磁非介导的阻力效应。磁振子信号固有的巨大开关调制,以及零场操作下的非易失性输运和多铁质的偏振控制n矢量,使多铁质垂直磁振子器件的实际应用迈出了可能的一步。这项工作将有助于实现高速、小型化和超低能耗的磁输运。
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引用次数: 0
Thermal interface material of carbon fiber enhanced micro-nano Cu sintering for power module thermal management 碳纤维热界面材料增强微纳Cu烧结用于功率模块热管理
IF 4 2区 物理与天体物理 Q2 PHYSICS, APPLIED Pub Date : 2026-03-02 DOI: 10.1063/5.0320544
Canyu Liu, Tianqi Liu, Changqing Liu
The pursuit of higher power and density in wide bandgap power modules makes thermal management a critical challenge. Thermal interface materials (TIMs) play a critical role by filling microscopic air gaps and thereby enhancing heat transfer for power electronics. Combining the recent development of nano metal sintering technology and exceptional intrinsic thermal conductivity of certain carbon allotropes, micro-nano Cu sintering with carbon fiber (CF) reinforcement was promoted as potential high performance and cost-effective TIM for power modules. In this work, a Cu/CF composite paste was synthesized and sintered by the thermal-compressing process, followed by the detailed investigation and simulation on its sintered interfacial microstructure and mechanical and thermal properties. This work demonstrated a significant improvement of thermal and mechanical properties through the optimization of CF doping ratio. The addition of 5 wt. % CF increased the average shear strength of Cu sintering joints by 65.3% to 44.8 MPa, which is attributed to enhanced interface adhesion from the nano Ni particle coating on the CF surface. Thermal conductivity rose from 77.1 to 87.4 W/(m K) and 107 W/(m K) with 5 and 10 wt. % CF doped, respectively. Furthermore, adding 10 wt. % CF increased thermal diffusivity by 27.4%, which helps alleviate transient thermal loads. This work highlights the strong potential of Cu/CF composites as future TIM for high-density power modules.
在宽带隙功率模块中追求更高的功率和密度使得热管理成为一个关键的挑战。热界面材料(TIMs)通过填充微小的空气间隙,从而增强电力电子设备的传热,发挥着关键作用。结合纳米金属烧结技术的最新发展和某些碳同素异素体优异的固有导热性,碳纤维(CF)增强微纳米Cu烧结被推广为具有潜力的高性能和低成本的功率模块TIM。本文采用热压烧结工艺合成了Cu/CF复合浆料,并对其烧结界面微观结构、力学性能和热性能进行了详细的研究和模拟。本工作表明,通过优化CF掺杂比,可以显著改善材料的热性能和力学性能。添加5 wt. %的CF使Cu烧结接头的平均抗剪强度提高了65.3%,达到44.8 MPa,这是由于CF表面的纳米Ni颗粒涂层增强了界面附着力。当掺5%和10%的CF时,导热系数分别从77.1上升到87.4 W/(m K)和107 W/(m K)。此外,添加10 wt. %的CF增加了27.4%的热扩散率,有助于减轻瞬态热负荷。这项工作突出了Cu/CF复合材料作为高密度功率模块的未来TIM的强大潜力。
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引用次数: 0
Narrowband signal generation by spintronic THz emitters 自旋电子太赫兹发射器产生窄带信号
IF 4 2区 物理与天体物理 Q2 PHYSICS, APPLIED Pub Date : 2026-03-02 DOI: 10.1063/5.0313284
Bikash Das Mohapatra, Evangelos Th. Papaioannou, Georg Schmidt
We report a technique for generating narrowband, high-frequency electrical signals using spintronic terahertz emitters (STEs) integrated onto coplanar waveguides (CPWs). Conventional STE operation typically yields ultrashort, broadband pulses spanning tens of terahertz. Our method employs multiple STEs positioned at precisely defined intervals along the CPW to produce a burst like signal, where the inter-emitter spacing determines the time delay between pulses, thus the fundamental burst frequency, which theoretically can be tuned across the STE bandwidth. Meander-shaped CPW geometries are used to enable compact integration and uniform optical excitation. First test devices demonstrate electrical signals up to 30 GHz with a bandwidth of 4.7 GHz corresponding to a quality factor of 6.38.
我们报告了一种利用集成在共面波导(cpw)上的自旋电子太赫兹发射器(STEs)产生窄带高频电信号的技术。传统的STE操作通常会产生跨越数十太赫兹的超短宽带脉冲。我们的方法采用沿CPW精确定义间隔的多个STE来产生类似突发的信号,其中发射器间的间距决定了脉冲之间的时间延迟,从而确定了基本突发频率,理论上可以在STE带宽上进行调谐。弯曲形状的CPW几何形状用于实现紧凑的集成和均匀的光激发。第一个测试设备演示了高达30 GHz的电信号,带宽为4.7 GHz,对应的质量因子为6.38。
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引用次数: 0
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Applied Physics Letters
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