Magnesium alloys are increasingly sought after in aerospace, automotive, biomedical, and electronic applications due to their superior strength-to-weight ratio, but their relatively poor surface integrity and erosion resistance necessitate advanced modification strategies. In this study, the QH21 magnesium alloy was engineered for enhanced surface performance using friction stir processing (FSP) reinforced with hybrid TiO₂–ZnO ceramic coatings. The processing parameters were systematically optimized through Taguchi’s design of experiments (DOE) methodology employing an L16 orthogonal array, with four critical factors: tool rotational speed (800–1400 rpm), traverse speed (15–30 mm/min), axial force (4–10 kN), and reinforcement percentage (3–12%) selected for evaluation. Performance metrics were assessed in terms of erosion factor and microhardness, which directly reflect wear resistance and structural integrity. The results revealed that a parameter set comprising 1000 rpm rotational speed, 15 mm/min traverse speed, 6 kN axial force, and 9% reinforcement minimized the erosion factor to 0.000290, indicating superior surface consolidation and particle–matrix interfacial bonding. Conversely, the maximum microhardness of 109 HV was achieved at 1400 rpm, 25 mm/min, 6 kN, and 12% reinforcement, attributed to intense dynamic recrystallization, grain refinement, and effective dispersion strengthening. Overall, the study demonstrates that optimized hybrid-particle FSP markedly enhances the surface quality and mechanical resilience of QH21 magnesium alloy, rendering it highly suitable for next-generation lightweight structural and functional components.
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