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Quantum-to-classical modeling of monolayer Ge2Se2 and its application in photovoltaic devices. 单层 Ge2Se2 的量子到经典模型及其在光伏设备中的应用。
IF 2.6 4区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-09-11 eCollection Date: 2024-01-01 DOI: 10.3762/bjnano.15.94
Anup Shrivastava, Shivani Saini, Dolly Kumari, Sanjai Singh, Jost Adam

Since the discovery of graphene in 2004, the unique properties of two-dimensional materials have sparked intense research interest regarding their use as alternative materials in various photonic applications. Transition metal dichalcogenide monolayers have been proposed as transport layers in photovoltaic cells, but the promising characteristics of group IV-VI dichalcogenides are yet to be thoroughly investigated. This manuscript reports on monolayer Ge2Se2 (a group IV-VI dichalcogenide), its optoelectronic behavior, and its potential application in photovoltaics. When employed as a hole transport layer, the material fosters an astonishing device performance. We use ab initio modeling for the material prediction, while classical drift-diffusion drives the device simulations. Hybrid functionals calculate electronic and optical properties to maintain high accuracy. The structural stability has been verified using phonon spectra. The E-k dispersion reveals the investigated material's key electronic properties. The calculations reveal a direct bandgap of 1.12 eV for monolayer Ge2Se2. We further extract critical optical parameters using the Kubo-Greenwood formalism and Kramers-Kronig relations. A significantly large absorption coefficient and a high dielectric constant inspired the design of a monolayer Ge2Se2-based solar cell, exhibiting a high open circuit voltage of V oc = 1.11 V, a fill factor of 87.66%, and more than 28% power conversion efficiency at room temperature. Our findings advocate monolayer Ge2Se2 for various optoelectronic devices, including next-generation solar cells. The hybrid quantum-to-macroscopic methodology presented here applies to broader classes of 2D and 3D materials and structures, showing a path to the computational design of future photovoltaic materials.

自 2004 年发现石墨烯以来,二维材料的独特特性引发了人们对其在各种光子应用中用作替代材料的浓厚研究兴趣。过渡金属二掺杂化合物单层已被提议用作光伏电池的传输层,但 IV-VI 族二掺杂化合物的良好特性仍有待深入研究。本手稿报告了单层 Ge2Se2(一种 IV-VI 族二卤化物)、其光电行为及其在光伏领域的潜在应用。当作为空穴传输层使用时,这种材料能产生惊人的器件性能。我们使用 ab initio 建模进行材料预测,同时使用经典漂移扩散驱动器件模拟。混合函数计算电子和光学特性,以保持高精度。声子光谱验证了结构的稳定性。E-k 色散揭示了所研究材料的关键电子特性。计算显示单层 Ge2Se2 的直接带隙为 1.12 eV。我们利用 Kubo-Greenwood 公式和 Kramers-Kronig 关系进一步提取了临界光学参数。明显较大的吸收系数和较高的介电常数激发了单层 Ge2Se2 太阳能电池的设计灵感,该电池在室温下具有 V oc = 1.11 V 的高开路电压、87.66% 的填充因子和超过 28% 的功率转换效率。我们的研究结果主张将单层 Ge2Se2 用于各种光电设备,包括下一代太阳能电池。本文介绍的量子到微观混合方法适用于更广泛的二维和三维材料与结构,为未来光伏材料的计算设计指明了道路。
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引用次数: 0
Introducing third-generation periodic table descriptors for nano-qRASTR modeling of zebrafish toxicity of metal oxide nanoparticles. 引入第三代元素周期表描述符,对金属氧化物纳米颗粒的斑马鱼毒性进行纳米-qRASTR建模。
IF 2.6 4区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-09-10 eCollection Date: 2024-01-01 DOI: 10.3762/bjnano.15.93
Supratik Kar, Siyun Yang

Metal oxide nanoparticles (MONPs) are widely used in medicine and environmental remediation because of their unique properties. However, their size, surface area, and reactivity can cause toxicity, potentially leading to oxidative stress, inflammation, and cellular or DNA damage. In this study, a nano-quantitative structure-toxicity relationship (nano-QSTR) model was initially developed to assess zebrafish toxicity for 24 MONPs. Previously established 23 first- and second-generation periodic table descriptors, along with five newly proposed third-generation descriptors derived from the periodic table, were employed. Subsequently, to enhance the quality and predictive capability of the nano-QSTR model, a nano-quantitative read across structure-toxicity relationship (nano-qRASTR) model was created. This model integrated read-across descriptors with modeled descriptors from the nano-QSTR approach. The nano-qRASTR model, featuring three attributes, outperformed the previously reported simple QSTR model, despite having one less MONP. This study highlights the effective utilization of the nano-qRASTR algorithm in situations with limited data for modeling, demonstrating superior goodness-of-fit, robustness, and predictability (R 2 = 0.81, Q 2 LOO = 0.70, Q 2 F1/R 2 PRED = 0.76) compared to simple QSTR models. Finally, the developed nano-qRASTR model was applied to predict toxicity data for an external dataset comprising 35 MONPs, addressing gaps in zebrafish toxicity assessment.

金属氧化物纳米粒子(MONPs)因其独特的性能而被广泛应用于医学和环境修复领域。然而,它们的尺寸、表面积和反应性会导致毒性,可能导致氧化应激、炎症、细胞或 DNA 损伤。在本研究中,初步建立了一个纳米定量结构-毒性关系(nano-QSTR)模型,以评估 24 种 MONPs 的斑马鱼毒性。采用了之前建立的 23 个第一代和第二代元素周期表描述符,以及从元素周期表中新提出的 5 个第三代描述符。随后,为了提高纳米 QSTR 模型的质量和预测能力,又创建了一个纳米定量跨结构毒性关系(nano-qRASTR)模型。该模型整合了纳米 QSTR 方法中的跨读描述符和建模描述符。纳米 QRASTR 模型具有三个属性,尽管少了一个 MONP,但其性能优于之前报道的简单 QSTR 模型。这项研究强调了在建模数据有限的情况下对纳米 QRASTR 算法的有效利用,与简单 QSTR 模型相比,纳米 QRASTR 算法具有更高的拟合度、稳健性和可预测性(R 2 = 0.81,Q 2 LOO = 0.70,Q 2 F1/R 2 PRED = 0.76)。最后,所开发的纳米 QRASTR 模型被用于预测由 35 种 MONPs 组成的外部数据集的毒性数据,以填补斑马鱼毒性评估方面的空白。
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引用次数: 0
Photocatalytic methane oxidation over a TiO2/SiNWs p-n junction catalyst at room temperature. 室温下 TiO2/SiNWs p-n 结催化剂的光催化甲烷氧化作用。
IF 2.6 4区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-09-02 eCollection Date: 2024-01-01 DOI: 10.3762/bjnano.15.92
Qui Thanh Hoai Ta, Luan Minh Nguyen, Ngoc Hoi Nguyen, Phan Khanh Thinh Nguyen, Dai Hai Nguyen

Rapid recombination of charge carriers in semiconductors is a main drawback for photocatalytic oxidative coupling of methane (OCM) reactions. Herein, we propose a novel catalyst by developing a p-n junction titania-silicon nanowires (TiO2/SiNWs) heterostructure. The structure is fabricated by atomic layer deposition of TiO2 on p-type SiNWs. The TiO2/SiNWs heterostructure exhibited an outstanding OCM performance under simulated solar light irradiation compared to the single components. This enhanced efficiency was attributed to the intrinsic electrical field formed between n-type TiO2 and p-type SiNWs, which forces generated charge carriers to move in opposite directions and suppresses charge recombination. Besides, surface morphology and optical properties of the the p-n TiO2/SiNWs catalyst are also beneficial for the photocatalytic activity. It is expected that the results of this study will provide massive guidance in synthesizing an efficient photocatalyst for CH4 conversion under mild conditions.

半导体中电荷载流子的快速重组是光催化甲烷氧化偶联(OCM)反应的主要缺点。在此,我们通过开发一种 p-n 结二氧化钛-硅纳米线(TiO2/SiNWs)异质结构,提出了一种新型催化剂。该结构是通过在 p 型硅纳米线上原子层沉积 TiO2 制成的。与单一成分相比,TiO2/SiNWs 异质结构在模拟太阳光照射下表现出卓越的 OCM 性能。效率的提高归功于 n 型 TiO2 和 p 型 SiNWs 之间形成的固有电场,该电场迫使产生的电荷载流子向相反的方向移动,从而抑制了电荷重组。此外,p-n TiO2/SiNWs 催化剂的表面形貌和光学特性也有利于提高光催化活性。预计本研究的结果将为在温和条件下合成一种用于转化 CH4 的高效光催化剂提供大量指导。
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引用次数: 0
Local work function on graphene nanoribbons. 石墨烯纳米带的局部功函数
IF 2.6 4区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-08-29 eCollection Date: 2024-01-01 DOI: 10.3762/bjnano.15.91
Daniel Rothhardt, Amina Kimouche, Tillmann Klamroth, Regina Hoffmann-Vogel

Graphene nanoribbons show exciting electronic properties related to the exotic nature of the charge carriers and to local confinement as well as atomic-scale structural details. The local work function provides evidence for such structural, electronic, and chemical variations at surfaces. Kelvin prove force microscopy can be used to measure the local contact potential difference (LCPD) between a probe tip and a surface, related to the work function. Here we use this technique to map the LCPD of graphene nanoribbons grown on a Au(111) substrate. The LCPD data shows charge transfer between the graphene nanoribbons and the gold substrate. Our results are corroborated with density functional theory calculations, which verify that the maps reflect the doping of the nanoribbons. Our results help to understand the relation between atomic structure and electronic properties both in high-resolution images and in the distance dependence of the LCPD.

石墨烯纳米带显示出令人兴奋的电子特性,这与电荷载流子的奇异性质、局部约束以及原子尺度的结构细节有关。局部功函数为表面的这种结构、电子和化学变化提供了证据。开尔文证明力显微镜可用于测量探针尖端与表面之间与功函数相关的局部接触电位差(LCPD)。在此,我们使用该技术绘制了生长在金(111)基底上的石墨烯纳米带的 LCPD 图。LCPD 数据显示了石墨烯纳米带与金基底之间的电荷转移。密度泛函理论计算证实了我们的结果,该计算验证了图谱反映了纳米带的掺杂情况。我们的研究结果有助于理解高分辨率图像和 LCPD 的距离依赖性中原子结构与电子特性之间的关系。
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引用次数: 0
Direct electron beam writing of silver using a β-diketonate precursor: first insights. 使用β-二酮酸酯前驱体的直接电子束写银:初探。
IF 2.6 4区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-08-26 eCollection Date: 2024-01-01 DOI: 10.3762/bjnano.15.90
Katja Höflich, Krzysztof Maćkosz, Chinmai S Jureddy, Aleksei Tsarapkin, Ivo Utke

Direct electron beam writing is a powerful tool for fabricating complex nanostructures in a single step. The electron beam locally cleaves the molecules of an adsorbed gaseous precursor to form a deposit, similar to 3D printing but without the need for a resist or development step. Here, we employ for the first time a silver β-diketonate precursor for focused electron beam-induced deposition (FEBID). The used compound (hfac)AgPMe3 operates at an evaporation temperature of 70-80 °C and is compatible with commercially available gas injection systems used in any standard scanning electron microscope. Growth of smooth 3D geometries could be demonstrated for tightly focused electron beams, albeit with low silver content in the deposit volume. The electron beam-induced deposition proved sensitive to the irradiation conditions, leading to varying compositions of the deposit and internal inhomogeneities such as the formation of a layered structure consisting of a pure silver layer at the interface to the substrate covered by a deposit layer with low silver content. Imaging after the deposition process revealed morphological changes such as the growth of silver particles on the surface. While these effects complicate the application for 3D printing, the unique deposit structure with a thin, compact silver film beneath the deposit body is interesting from a fundamental point of view and may offer additional opportunities for applications.

直接电子束写入是一种功能强大的工具,只需一步即可制造出复杂的纳米结构。电子束在局部裂解吸附的气态前驱体分子,形成沉积物,类似于三维打印,但无需光刻胶或显影步骤。在这里,我们首次采用了β-二酮酸银前驱体进行聚焦电子束诱导沉积(FEBID)。所使用的 (hfac)AgPMe3 化合物的蒸发温度为 70-80 °C,与任何标准扫描电子显微镜中使用的市售气体注入系统兼容。尽管沉积体积中的银含量较低,但在电子束紧密聚焦的情况下,也能生长出光滑的三维几何形状。事实证明,电子束诱导沉积对辐照条件非常敏感,会导致沉积物成分的变化和内部的不均匀性,例如形成分层结构,在与基底的界面上形成纯银层,银含量较低的沉积层覆盖在纯银层上。沉积过程后的成像显示了形态变化,如表面银颗粒的生长。虽然这些影响使三维打印的应用变得复杂,但从根本上看,沉积体下方有一层薄而紧密的银膜的独特沉积结构非常有趣,并可能为应用提供更多机会。
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引用次数: 0
Recent updates in applications of nanomedicine for the treatment of hepatic fibrosis. 应用纳米药物治疗肝纤维化的最新进展。
IF 2.6 4区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-08-23 eCollection Date: 2024-01-01 DOI: 10.3762/bjnano.15.89
Damai Ria Setyawati, Fransiska Christydira Sekaringtyas, Riyona Desvy Pratiwi, A'liyatur Rosyidah, Rohimmahtunnissa Azhar, Nunik Gustini, Gita Syahputra, Idah Rosidah, Etik Mardliyati, Tarwadi, Sjaikhurrizal El Muttaqien

Over recent decades, nanomedicine has played an important role in the enhancement of therapeutic outcomes compared to those of conventional therapy. At the same time, nanoparticle drug delivery systems offer a significant reduction in side effects of treatments by lowering the off-target biodistribution of the active pharmaceutical ingredients. Cancer nanomedicine represents the most extensively studied nanotechnology application in the field of pharmaceutics and pharmacology since the first nanodrug for cancer treatment, liposomal doxorubicin (Doxil®), has been approved by the FDA. The advancement of cancer nanomedicine and its enormous technological success also included various other target diseases, including hepatic fibrosis. This confirms the versatility of nanomedicine for improving therapeutic activity. In this review, we summarize recent updates of nanomedicine platforms for improving therapeutic efficacy regarding liver fibrosis. We first emphasize the challenges of conventional drugs for penetrating the biological barriers of the liver. After that, we highlight design principles of nanocarriers for achieving improved drug delivery of antifibrosis drugs through passive and active targeting strategies.

近几十年来,与传统疗法相比,纳米医学在提高治疗效果方面发挥了重要作用。同时,纳米颗粒给药系统通过降低活性药物成分的脱靶生物分布,大大减少了治疗的副作用。自第一种用于癌症治疗的纳米药物脂质体多柔比星(Doxil®)获得美国食品及药物管理局批准以来,癌症纳米药物是制药学和药理学领域研究最为广泛的纳米技术应用。癌症纳米药物的发展及其巨大的技术成功还包括其他各种目标疾病,包括肝纤维化。这证实了纳米药物在提高治疗活性方面的多功能性。在本综述中,我们总结了纳米药物平台在改善肝纤维化疗效方面的最新进展。我们首先强调了传统药物在穿透肝脏生物屏障方面所面临的挑战。然后,我们强调了纳米载体的设计原则,以通过被动和主动靶向策略实现抗肝纤维化药物的更好给药。
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引用次数: 0
Unveiling the potential of alginate-based nanomaterials in sensing technology and smart delivery applications. 揭示海藻酸盐纳米材料在传感技术和智能传输应用中的潜力。
IF 2.6 4区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-08-22 eCollection Date: 2024-01-01 DOI: 10.3762/bjnano.15.88
Shakhzodjon Uzokboev, Khojimukhammad Akhmadbekov, Ra'no Nuritdinova, Salah M Tawfik, Yong-Ill Lee

Sensors are applied to many fields nowadays because of their high sensitivity, low cost, time-saving, user-friendly, and excellent selectivity. Current biomedical and pharmaceutical science has one focus on developing nanoparticle-based sensors, especially biopolymeric nanoparticles. Alginate is a widely used biopolymer in a variety of applications. The hydrogel-forming characteristic, the chemical structure with hydroxy and carboxylate moieties, biocompatibility, biodegradability, and water solubility of alginate have expanded opportunities in material and biomedical sciences. Recently, research on alginate-based nanoparticles and their applications has begun. These materials are gaining popularity because of their wide usage potential in the biomedical and pharmaceutical fields. Many review papers describe applications of alginate in the drug delivery field. The current study covers the structural and physicochemical properties of alginate-based nanoparticles. The prospective applications of alginate-based nanomaterials in various domains are discussed, including drug delivery and environmental sensing applications for humidity, heavy metals, and hydrogen peroxide. Moreover, biomedical sensing applications of alginate-based nanoparticles regarding various analytes such as glucose, cancer cells, pharmaceutical drugs, and human motion will also be reviewed in this paper. Future research scopes highlight existing challenges and solutions.

传感器具有灵敏度高、成本低、省时省力、使用方便、选择性强等优点,如今已被广泛应用于许多领域。当前生物医学和制药科学的一个重点是开发基于纳米粒子的传感器,尤其是生物聚合物纳米粒子。藻酸盐是一种应用广泛的生物聚合物。海藻酸盐的水凝胶形成特性、羟基和羧基的化学结构、生物相容性、生物可降解性和水溶性为材料和生物医学科学提供了更多机会。最近,有关海藻酸盐纳米粒子及其应用的研究已经开始。这些材料因其在生物医学和制药领域的广泛应用潜力而越来越受欢迎。许多综述论文介绍了海藻酸盐在药物输送领域的应用。目前的研究涵盖了海藻酸盐纳米颗粒的结构和理化特性。文章讨论了海藻酸盐纳米材料在各个领域的应用前景,包括药物输送以及湿度、重金属和过氧化氢的环境传感应用。此外,本文还将综述藻酸盐基纳米粒子在生物医学传感方面的应用,涉及葡萄糖、癌细胞、药物和人体运动等各种分析物。未来的研究范围强调了现有的挑战和解决方案。
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引用次数: 0
Signal generation in dynamic interferometric displacement detection. 动态干涉位移检测中的信号生成。
IF 2.6 4区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-08-20 eCollection Date: 2024-01-01 DOI: 10.3762/bjnano.15.87
Knarik Khachatryan, Simon Anter, Michael Reichling, Alexander von Schmidsfeld

Laser interferometry is a well-established and widely used technique for precise displacement measurements. In a non-contact atomic force microscope (NC-AFM), it facilitates the force measurement by recording the periodic displacement of an oscillating microcantilever. To understand signal generation in a NC-AFM-based Michelson-type interferometer, we evaluate the non-linear response of the interferometer to the harmonic displacement of the cantilever in the time domain. As the interferometer signal is limited in amplitude because of the spatial periodicity of the interferometer light field, an increasing cantilever oscillation amplitude creates an output signal with an increasingly complex temporal structure. By the fit of a model to the measured time-domain signal, all parameters governing the interferometric displacement signal can precisely be determined. It is demonstrated, that such an analysis specifically allows for the calibration of the cantilever oscillation amplitude with 2% accuracy.

激光干涉仪是一种成熟且广泛应用的精确位移测量技术。在非接触式原子力显微镜(NC-AFM)中,它通过记录摆动微悬臂的周期性位移来促进力测量。为了了解基于 NC-AFM 的迈克尔逊型干涉仪的信号生成情况,我们在时域中评估了干涉仪对悬臂谐波位移的非线性响应。由于干涉仪光场的空间周期性,干涉仪信号的振幅是有限的,悬臂振荡振幅的增加会产生一个时间结构越来越复杂的输出信号。通过对测量到的时域信号进行模型拟合,可以精确地确定干涉位移信号的所有参数。结果表明,通过这种分析,悬臂振幅的校准精度可达 2%。
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引用次数: 0
Effect of wavelength and liquid on formation of Ag, Au, Ag/Au nanoparticles via picosecond laser ablation and SERS-based detection of DMMP. 波长和液体对通过皮秒激光烧蚀形成银、金、银/金纳米粒子的影响以及基于 SERS 的 DMMP 检测。
IF 2.6 4区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-08-19 eCollection Date: 2024-01-01 DOI: 10.3762/bjnano.15.86
Sree Satya Bharati Moram, Chandu Byram, Venugopal Rao Soma

The present study investigates the effects of input wavelength (1064, 532, and 355 nm) and surrounding liquid environment (distilled water and aqueous NaCl solution) on the picosecond laser ablation on silver (Ag), gold (Au), and Ag/Au alloy targets. The efficacy of the laser ablation technique was meticulously evaluated by analyzing the ablation rates, surface plasmon resonance peak positions, and particle size distributions of the obtained colloids. The nanoparticles (NPs) were characterized using the techniques of UV-visible absorption, transmission electron microscopy, and energy-dispersive X-ray spectroscopy. Furthermore, NPs of various sizes ranging from 6 to 35 nm were loaded onto a filter paper by a simple and effective drop-casting approach to achieve flexible surface-enhanced Raman spectroscopy (SERS) substrates/sensors. These substrates were tested using a simple, portable Raman device to identify various hazardous chemicals (malachite green, methyl salicylate, and thiram). The stability of the substrates was also systematically investigated by determining the decay percentages in the SERS signals over 60 days. The optimized SERS substrate was subsequently employed to detect chemical warfare agent (CWA) simulants such as methyl salicylate (a CWA simulant for sulfur mustard) and dimethyl methyl phosphonate (has some structural similarities to the G-series nerve agents) at different laser excitations (325, 532, and 633 nm). A notably higher SERS efficiency for CWA simulants was observed at a 325 nm Raman excitation. Our findings reveal that a higher ablation yield was observed at IR irradiation than those obtained at the other wavelengths. A size decrease of the NPs was noticed by changing the liquid environment to an electrolyte. These findings have significant implications for developing more efficient and stable SERS substrates for chemical detection applications.

本研究探讨了输入波长(1064、532 和 355 纳米)和周围液体环境(蒸馏水和氯化钠水溶液)对银(Ag)、金(Au)和银/金合金靶上皮秒激光烧蚀的影响。通过分析所获得胶体的烧蚀率、表面等离子体共振峰位置和粒度分布,对激光烧蚀技术的功效进行了细致的评估。利用紫外可见吸收、透射电子显微镜和能量色散 X 射线光谱技术对纳米粒子(NPs)进行了表征。此外,通过简单有效的滴注方法,将 6 至 35 纳米不同大小的 NPs 装载到滤纸上,实现了灵活的表面增强拉曼光谱(SERS)基底/传感器。使用简单的便携式拉曼设备对这些基底进行了测试,以识别各种危险化学品(孔雀石绿、水杨酸甲酯和福双美)。此外,还通过测定 60 天内 SERS 信号的衰减率,对基底的稳定性进行了系统研究。优化后的 SERS 基底随后被用于在不同的激光激发波长(325、532 和 633 纳米)下检测化学战剂(CWA)模拟物,如水杨酸甲酯(硫芥子气的 CWA 模拟物)和甲基膦酸二甲酯(与 G 系列神经毒剂有一些结构相似之处)。在 325 纳米拉曼激发下,CWA 模拟物的 SERS 效率明显更高。我们的研究结果表明,与其他波长相比,红外照射下的烧蚀率更高。将液体环境改为电解质后,NPs 的尺寸有所减小。这些发现对于开发更高效、更稳定的 SERS 基底用于化学检测应用具有重要意义。
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引用次数: 0
Interface properties of nanostructured carbon-coated biological implants: an overview. 纳米结构碳涂层生物植入物的界面特性:综述。
IF 2.6 4区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-08-16 eCollection Date: 2024-01-01 DOI: 10.3762/bjnano.15.85
Mattia Bartoli, Francesca Cardano, Erik Piatti, Stefania Lettieri, Andrea Fin, Alberto Tagliaferro

The interfaces between medical implants and living tissues are of great complexity because of the simultaneous occurrence of a wide variety of phenomena. The engineering of implant surfaces represents a crucial challenge in material science, but the further improvement of implant properties remains a critical task. It can be achieved through several processes. Among them, the production of specialized coatings based on carbon-based materials stands very promising. The use of carbon coatings allows one to simultaneously fine-tune tribological, mechanical, and chemical properties. Here, we review applications of nanostructured carbon coatings (nanodiamonds, carbon nanotubes, and graphene-related materials) for the improvement of the overall properties of medical implants. We are focusing on biological interactions, improved corrosion resistance, and overall mechanical properties, trying to provide a complete overview within the field.

医疗植入物与活体组织之间的界面非常复杂,因为会同时出现各种各样的现象。植入体表面工程是材料科学领域的一项重要挑战,但进一步提高植入体的性能仍是一项关键任务。这可以通过几种工艺来实现。其中,以碳基材料为基础的专用涂层的生产非常有前景。使用碳涂层可以同时微调摩擦学、机械和化学特性。在此,我们回顾了纳米结构碳涂层(纳米金刚石、碳纳米管和石墨烯相关材料)在改善医疗植入物整体性能方面的应用。我们将重点关注生物相互作用、耐腐蚀性能的改善以及整体机械性能,力图为该领域提供一个完整的概述。
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引用次数: 0
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Beilstein Journal of Nanotechnology
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