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Development of CuCl-HCl electrolysis for hydrogen production via Cu-Cl thermochemical cycle Cu-Cl热化学循环CuCl-HCl电解制氢的研究进展
Pub Date : 2010-01-01 DOI: 10.1787/9789264087156-30-EN
Y. Gong, E. Chalkova, N. Akinfiev, V. Balashov, M. Fedkin, S. Lvov
The Cu-Cl thermochemical cycle is among the most attractive technologies proposed for hydrogen production due to moderate temperature requirements and high efficiency. In the present study, one of the main steps of the cycle – H2 gas production via CuCl-HCl electrolysis – was investigated using a newly designed electrolyser system. The electrolysis reaction was performed with the applied voltage from 0.35 to 0.9 V. The current efficiency of the electrolysis system was evaluated based on the observed rate of hydrogen production. The effects of temperature and reagent flow rate on the electrolysis performance were studied. Several types of anion-exchange and cation-exchange membranes were tested in the electrolyser, and their performance was compared with respect to process efficiency and tolerance to copper crossover.
Cu-Cl热化学循环因其温度适中和效率高而成为最有吸引力的制氢技术之一。本研究采用新设计的电解槽系统,对循环的主要步骤之一——CuCl-HCl电解制氢进行了研究。在0.35 ~ 0.9 V的电压范围内进行电解反应。根据观察到的产氢率来评价电解系统的电流效率。研究了温度和试剂流速对电解性能的影响。在电解槽中测试了几种阴离子交换膜和阳离子交换膜,并比较了它们的工艺效率和对铜交叉的耐受性。
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引用次数: 4
Sustainable electricity supply in the world by 2050 for economic growth and automotive fuel 到2050年全球可持续电力供应为经济增长和汽车提供燃料
Pub Date : 2010-01-01 DOI: 10.1787/9789264087156-37-EN
P. Kruger
Over the next 40 years, the combustion of fossil fuels for generation of electricity and vehicle transportation will be significantly reduced. In addition to the business-as-usual growth in electric energy demand for the growing world population, new electricity-intensive industries, such as battery electric vehicles and hydrogen fuel-cell vehicles will result in further growth in world consumption of electric energy. Planning for a sustainable supply of electric energy in the diverse economies of the world should be carried out with appropriate technology for selecting the appropriate large-scale energy resources based on their specific energy. Analysis of appropriate technology for the available large-scale energy resources with diminished use of fossil-fuel combustion shows that sustainable electricity supply can be achieved with equal contributions of renewable energy resources for large numbers of small-scale distributed applications and nuclear energy resources for the smaller number of large-scale centralised applications.
在未来的40年里,用于发电和车辆运输的化石燃料的燃烧将大大减少。随着世界人口的不断增长,电力需求将一如既往地增长,除此之外,新的电力密集型产业,如电池电动汽车和氢燃料电池汽车,将导致世界电力能源消费的进一步增长。在世界不同经济体中规划可持续的电力供应应采用适当的技术,以便根据其具体能源选择适当的大规模能源。在减少使用化石燃料燃烧的情况下,对现有大规模能源的适当技术进行的分析表明,对大量小规模分布式应用的可再生能源和对少数大规模集中式应用的核能的同等贡献,可以实现可持续电力供应。
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引用次数: 0
Canadian nuclear hydrogen R&D programme 加拿大核氢研发计划
Pub Date : 2010-01-01 DOI: 10.1787/9789264087156-9-EN
S. Suppiah, L. Stolberg, H. Boniface, G. Tan, S. McMahon, S. York, W. Zhang
Canada is developing the heavy-water-moderated supercritical water reactor as its Generation IV nuclear system. The medium temperature copper-chlorine (Cu-Cl) cycle has been selected as a suitable process for integration with this reactor system for large-scale production of hydrogen. A collaborative programme uniting the University of Ontario Institute of Technology (UOIT), Argonne National Laboratory (ANL) and Atomic Energy of Canada Limited (AECL) is underway for the development of the complete cycle for pilot plant demonstration. Canada’s Generation IV National Programme also supports the international efforts on VHTR through R&D on areas that are synergistic with the Canadian efforts on SCWR. Some of the latest results in the development of the Cu-Cl cycle and Canada’s contributions to the sulphur-iodine cycle are described in this paper.
加拿大正在开发重水慢化超临界水反应堆作为其第四代核系统。选择中温铜-氯(Cu-Cl)循环作为与该反应器系统集成用于大规模制氢的合适工艺。由安大略理工大学(UOIT)、阿贡国家实验室(ANL)和加拿大原子能有限公司(AECL)联合开展的一项合作计划正在进行中,目的是开发中试工厂示范的完整周期。加拿大的第四代国家方案还通过与加拿大在SCWR方面的努力具有协同作用的领域的研发,支持在VHTR方面的国际努力。本文介绍了Cu-Cl循环发展的一些最新成果和加拿大对硫-碘循环的贡献。
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引用次数: 4
Materials development for SOEC SOEC材料开发
Pub Date : 2010-01-01 DOI: 10.1787/9789264087156-13-EN
S. Elangovan, J. Hartvigsen, F. Zhao, I. Bay, D. Larsen
Emphasis on energy security issues has brought much-needed attention to economic production of hydrogen as the secondary energy carrier for non-electrical markets as well as to meet increasing demand for crude upgrading and desulphurisation. While steam reforming of methane is the current method of production of hydrogen, the fossil fuel feed consumes non-renewable fuel while emitting greenhouse gases. Thus, in the long run, efficient, environmentally-friendly and economic means of hydrogen production using nuclear and renewable energy needs to be developed. Steam electrolysis, particularly using high temperature ceramic membrane processes, provides an attractive option for efficient generation of high purity hydrogen.
对能源安全问题的强调引起了人们对氢作为非电力市场的二次能源载体的经济生产以及满足日益增长的原油升级和脱硫需求的迫切关注。虽然甲烷的蒸汽重整是目前生产氢气的方法,但化石燃料饲料消耗不可再生燃料,同时排放温室气体。因此,从长远来看,需要开发利用核能和可再生能源的高效、环保和经济的制氢手段。蒸汽电解,特别是使用高温陶瓷膜工艺,为高效产生高纯度氢提供了一个有吸引力的选择。
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引用次数: 0
High-temperature steam electrolysis for hydrogen production 高温蒸汽电解制氢
Pub Date : 2010-01-01 DOI: 10.1787/9789264087156-12-EN
J. Mougin, G. Gousseau, B. Morel, F. Lefebvre-Joud, F. Naour, F. Chauveau, J. Grenier
High-temperature steam electrolysis (HTSE) coupled with nuclear energy is one of the most promising options for hydrogen mass production. CEA (the French Atomic Energy Commission) is carrying out research in this field, from materials, cells and components developments to stack design including components and stack testing.
高温蒸汽电解(HTSE)与核能相结合是最有希望大规模生产氢的选择之一。CEA(法国原子能委员会)正在开展这一领域的研究,从材料、电池和组件开发到包括组件和堆栈测试在内的堆栈设计。
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引用次数: 0
CEA assessment of the sulphur-iodine cycle for hydrogen production 硫碘循环制氢的CEA评价
Pub Date : 2010-01-01 DOI: 10.1787/9789264087156-18-EN
P. Carles, X. Vitart, P. Yvon
The sulphur-iodine cycle is a promising process for hydrogen production using nuclear heat: • it is a purely thermochemical cycle, implying that hydrogen production will scale with volume rather than surface; • it only involves fluids, thus avoiding the often difficult handling of solids; • its heat requirements are well matched to the temperatures available from a Generation IV very/high temperature reactor.
硫碘循环是一个很有前途的利用核热制氢的过程:•它是一个纯粹的热化学循环,这意味着氢的生产将与体积而不是表面成比例;•它只涉及流体,从而避免了通常难以处理的固体;•其热需求与第四代极/高温反应堆的可用温度相匹配。
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引用次数: 0
Exergy analysis of the Cu-Cl cycle Cu-Cl循环的能量分析
Pub Date : 2010-01-01 DOI: 10.1787/9789264087156-31-EN
J. Borgard, D. Doizi, P. Carles
The CuCl cycle is a hybrid thermochemical cycle to produce hydrogen using both electricity and heat to split water into hydrogen and oxygen. Already described in the early 70s, it has recently been revisited because of its low maximal temperature and its high potential efficiency. Furthermore, raw materials are cheap, which allows a drastic diminution of constraints for industrial deployment.
CuCl循环是一种混合热化学循环,利用电和热将水分解成氢和氧来产生氢。早在上世纪70年代初,人们就已经对它进行了描述,但由于它的最高温度低、潜在效率高,最近又重新对它进行了研究。此外,原材料价格低廉,这大大减少了工业部署的限制。
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引用次数: 0
French research strategy to use nuclear reactors for hydrogen production 法国研究利用核反应堆生产氢气的战略
Pub Date : 2010-01-01 DOI: 10.1787/9789264087156-5-EN
P. Yvon, P. Carles, F. Naour
The demand for hydrogen, driven by classical applications such as fertilisers or oil refining as well as new applications (synthetic fuels, fuel cells,…) is growing significantly. Presently, most of the hydrogen produced in the world uses methane or another fossil feedstock, which is not a sustainable option, given the limited fossil resources and need to reduce CO2 emissions. This stimulates the need to develop alternative processes of production which do not suffer from these drawbacks.
在化肥、炼油等传统应用以及新应用(合成燃料、燃料电池等)的推动下,对氢的需求正在显著增长。目前,世界上生产的大部分氢气都使用甲烷或其他化石原料,考虑到有限的化石资源和减少二氧化碳排放的需要,这不是一个可持续的选择。这就刺激了开发不受这些缺点影响的替代生产工艺的需要。
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引用次数: 2
Nuclear hydrogen production programme in the United States 美国的核制氢计划
Pub Date : 2010-01-01 DOI: 10.1787/9789264087156-4-EN
C. Sink
The Nuclear Hydrogen Initiative (NHI) is focused on demonstrating the economic, commercial-scale production of hydrogen using process heat derived from nuclear energy. NHI-supported research has concentrated to date on three technologies compatible with the Next Generation Nuclear Plant (NGNP): high temperature steam electrolysis (HTE); sulphur-iodine (S-I) thermochemical; and hybrid sulphur (HyS) thermochemical. In 2009 NHI will down select to a single technology on which to focus its future development efforts, for which the next step will be a pilot-scale experiment.
核能氢倡议(NHI)的重点是展示利用核能产生的过程热经济、商业规模的氢生产。迄今为止,nhi支持的研究主要集中在与下一代核电站(NGNP)兼容的三种技术上:高温蒸汽电解(HTE);硫碘(S-I)热化学;和混合硫(HyS)热化学。2009年,日本国民健康保险公司将选择一种技术作为其未来发展的重点,下一步将是试点规模的实验。
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引用次数: 1
Proposed chemical plant initiated accident scenarios in a sulphur-iodine cycle plant coupled to a pebble bed modular reactor 拟建的化工厂引发了一个硫碘循环厂与一个卵石床模块化反应堆耦合的事故情景
Pub Date : 2010-01-01 DOI: 10.1787/9789264087156-43-EN
N. Brown, S. Revankar, V. Şeker, T. Downar
In the sulphur-iodine (S-I) cycle nuclear hydrogen generation scheme the chemical plant acts as the heat sink for the very high temperature nuclear reactor (VHTR). Thus, any accident which occurs in the chemical plant must feedback to the nuclear reactor. There are many different types of accidents which can occur in a chemical plant. These accidents include intra-reactor piping failure, inter-reactor piping failure, reaction chamber failure and heat exchanger failure.
在硫碘(S-I)循环核制氢方案中,化工厂充当了高温核反应堆(VHTR)的散热器。因此,化工厂发生的任何事故都必须反馈给核反应堆。化工厂可能发生许多不同类型的事故。这些事故包括反应堆内管道故障、反应堆间管道故障、反应室故障和热交换器故障。
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引用次数: 0
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Nuclear science abstracts
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