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Nuclear safety and regulatory considerations for nuclear hydrogen production 核安全和核制氢的监管考虑
Pub Date : 2010-01-01 DOI: 10.1787/9789264087156-41-EN
William Reckley
The use of a nuclear power plant to produce hydrogen or for other process heat applications will present challenges to the licensing process. Potential safety and regulatory issues have been evaluated to identify possible research needs, policy concerns and licensing approaches. A brief description of nuclear power plant licensing in the United States and a discussion of specific issues for using nuclear power plants for process heat applications are presented.
使用核电站生产氢气或用于其他过程热应用将对许可程序提出挑战。对潜在的安全和监管问题进行了评估,以确定可能的研究需求、政策关注点和许可方法。简要介绍了美国核电厂的许可情况,并讨论了使用核电厂进行过程热应用的具体问题。
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引用次数: 3
Conceptual design of the HTTR-IS nuclear hydrogen production system HTTR-IS核制氢系统概念设计
Pub Date : 2010-01-01 DOI: 10.1787/9789264087156-44-EN
Hidenori Sato, N. Sakaba, Naoki Sano, H. Ohashi, Yuu Tachibana, K. Kunitomi
One of the key safety issues for nuclear hydrogen production is the heat transfer tube rupture in intermediated heat exchangers (IHX) which provide heat to process heat applications. This study focused on the detection method and system behaviour assessments during the IHX tube rupture scenario (IHXTR) in the HTTR coupled with IS process hydrogen production system (HTTR-IS system). The results indicate that monitoring the integral of secondary helium gas supply would be the most effective detection method. Furthermore, simultaneous actuation of two isolation valves could reduce the helium gas transportation from primary to secondary cooling systems. The results of system behaviour show that evaluation items do not exceed the acceptance criteria during the scenario. Maximum fuel temperature also does not exceed initial value and therefore the reactor core was not seriously damaged and cooled sufficiently.
核制氢的关键安全问题之一是为过程热应用提供热量的中间热交换器(IHX)的传热管破裂。本研究的重点是在HTTR和IS制氢系统(htr -IS系统)中IHX管破裂场景(IHXTR)的检测方法和系统行为评估。结果表明,监测二次氦气供应积分是最有效的检测方法。此外,同时驱动两个隔离阀可以减少氦气从一次冷却系统到二次冷却系统的输送。系统行为的结果表明,评估项目在场景中没有超过可接受标准。最高燃料温度也没有超过初始值,因此反应堆堆芯没有严重损坏,也没有得到充分冷却。
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引用次数: 1
Development status of the hybrid sulphur thermochemical hydrogen production process 杂化硫热化学制氢工艺的发展现状
Pub Date : 2010-01-01 DOI: 10.1787/9789264087156-26-EN
W. Summers
The DOE Nuclear Hydrogen Initiative has selected two sulphur cycles, the sulphur iodine (SI) cycle and the HyS process, as the first priority thermochemical processes for development and potential demonstration with the next generation nuclear plant. Both cycles share a common high temperature reaction step – the catalytic thermal decomposition of sulphuric acid. However, they are fundamentally different in the methods used for the hydrogen production step.
美国能源部核氢计划选择了两个硫循环,硫碘(SI)循环和HyS过程,作为下一代核电站开发和潜在示范的首要热化学过程。这两个循环都有一个共同的高温反应步骤——硫酸的催化热分解。然而,它们在制氢步骤中使用的方法是根本不同的。
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引用次数: 0
Alternate VHTR/HTE interface for mitigating tritium transport and structure creep 减少氚输运和结构蠕变的VHTR/HTE交替界面
Pub Date : 2010-01-01 DOI: 10.1787/9789264087156-48-EN
R. Vilim
High temperature creep in structures at the interface between the nuclear plant and the hydrogen plant and the migration of tritium from the core through structures in the interface are two key challenges for the very high temperature reactor (VHTR) coupled to the high temperature electrolysis (HTE) process. The severity of these challenges, however, can be reduced by lowering the temperature at which the interface operates. Preferably this should be accomplished in a way that does not reduce combined plant efficiency and other performance measures. A means for doing so is described. A heat pump is used to raise the temperature of near-waste heat from the PCU to the temperature at which nine-tenths of the HTE process heat is needed. In addition to mitigating tritium transport and creep of structures, structural material commodity costs are reduced and plant efficiency is increased by 1%.
核电厂和氢气厂界面结构的高温蠕变以及氚从堆芯通过界面结构的迁移是与高温电解(HTE)过程耦合的极高温反应堆(VHTR)面临的两个关键挑战。然而,这些挑战的严重性可以通过降低界面工作温度来降低。最好以不降低工厂综合效率和其他性能指标的方式完成这一工作。描述了这样做的一种方法。热泵用于将来自PCU的废热的温度提高到需要HTE过程热量的十分之九的温度。除了减轻结构的氚传输和蠕变外,还降低了结构材料的商品成本,工厂效率提高了1%。
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引用次数: 3
Heat pump cycle by hydrogen-absorbing alloys to assist high-temperature gas-cooled reactor in producing hydrogen 热泵循环由吸氢合金辅助高温气冷反应堆产氢
Pub Date : 2010-01-01 DOI: 10.1787/9789264087156-46-EN
S. Fukada, Nobutaka Hayashi
A chemical heat pump system using two hydrogen-absorbing alloys is proposed to utilise heat exhausted from a high-temperature source such as a high-temperature gas-cooled reactor (HTGR), more efficiently. The heat pump system is designed to produce H2 based on the S-I cycle more efficiently. The overall system proposed here consists of HTGR, He gas turbines, chemical heat pumps and reaction vessels corresponding to the three-step decomposition reactions comprised in the S-I process. A fundamental research is experimentally performed on heat generation in a single bed packed with a hydrogen-absorbing alloy that may work at the H2 production temperature. The hydrogen-absorbing alloy of Zr(V1-XFeX)2 is selected as a material that has a proper plateau pressure for the heat pump system operated between the input and output temperatures of HTGR and reaction vessels of the S-I cycle. Temperature jump due to heat generated when the alloy absorbs H2 proves that the alloy–H2 system can heat up the exhaust gas even at 600°C without any external mechanical force.
提出了一种使用两种吸氢合金的化学热泵系统,以更有效地利用高温气冷反应堆(HTGR)等高温源排出的热量。热泵系统的设计是为了更有效地基于S-I循环产生氢气。本文提出的整个系统由高温气冷堆、He燃气轮机、化学热泵和S-I工艺中三步分解反应对应的反应容器组成。在单床上进行了一项基础实验研究,该实验用吸氢合金填充,可以在氢气产生温度下工作。选择Zr(V1-XFeX)2吸氢合金作为在HTGR输入和输出温度与S-I循环反应容器之间运行的热泵系统具有适当平台压力的材料。合金吸收H2时产生的热导致的温度跳升证明合金- H2体系在不受任何机械外力作用的情况下,即使在600℃也能对废气进行加热。
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引用次数: 3
The concept of nuclear hydrogen production based on MHR-T reactor 基于MHR-T反应堆的核制氢概念
Pub Date : 2010-01-01 DOI: 10.1787/9789264087156-8-EN
N. Ponomarev-Stepnoy, A. Stolyarevskiy, N. Kodochigov
The concept focused on nuclear power for steam reforming of methane and, later, on hydrogen production from water by high temperature solid oxide electrolysis. The programme arises from the premise that the use of hydrogen could grow world wide by a factor of about sixteen over the next century. Anticipating that the main source of hydrogen will continue to be steam reforming of natural gas during much of that period, by 2025, about a quarter of the world’s production of natural gas would be devoted to hydrogen generation, considering both its use as both the energy source and the source of the raw material. The use of nuclear reactors instead of natural gas as the heat source for steam reforming of methane could reduce the total use of natural gas by almost half.
这个概念集中在甲烷蒸汽重整的核能上,后来又集中在高温固体氧化物电解从水中制氢上。该计划的前提是,到下个世纪,全球对氢的使用可能会增长约16倍。预计在此期间,氢气的主要来源将继续是天然气的蒸汽重整,到2025年,考虑到氢气作为能源和原材料的双重用途,世界上大约四分之一的天然气产量将用于制氢。使用核反应堆代替天然气作为甲烷蒸汽重整的热源,可以使天然气的总使用量减少近一半。
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引用次数: 0
Degradation mechanisms in solid oxide electrolysis anodes 固体氧化物电解阳极的降解机理
Pub Date : 2010-01-01 DOI: 10.1787/9789264087156-15-EN
Vivekanand Sharma, B. Yildiz
High temperature steam electrolysis is one of the most efficient processes for hydrogen generation from water with no CO2 emissions using electricity and heat from nuclear or concentrated solar plants. Solid Oxide Electrolytic Cells (SOEC) are the proposed technology being researched and developed for this purpose. Over a long period of operation of the cells, various sources for degradation in the cells’ electrochemical performance prevail, and hence the cell resistance increases and the process becomes inefficient. Our research is aimed at identifying the mechanisms for the loss in the electrochemical performance of the cell, particularly of the oxygen electrode, namely the anode.
高温蒸汽电解是利用核能或集中式太阳能发电厂的电力和热量,在不排放二氧化碳的情况下从水中制氢的最有效方法之一。固体氧化物电解电池(SOEC)是为此目的而研究和开发的拟议技术。在电池的长时间运行中,电池电化学性能的各种退化来源普遍存在,因此电池电阻增加,过程变得低效。我们的研究旨在确定电池电化学性能损失的机制,特别是氧电极,即阳极。
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引用次数: 0
Status of the INL high-temperature electrolysis research program –experimental and modeling INL高温电解研究项目现状-实验与建模
Pub Date : 2009-04-01 DOI: 10.1787/9789264087156-11-EN
J. O'Brien, C. Stoots, M. McKellar, E. Harvego, K. Condie, G. Housley, J. Herring, J. Hartvigsen
This paper provides a status update on the high-temperature electrolysis (HTE) research and development program at the Idaho National Laboratory (INL), with an overview of recent large-scale system modeling results and the status of the experimental program. System analysis results have been obtained using the commercial code UniSim, augmented with a custom high-temperature electrolyzer module. The process flow diagrams for the system simulations include an advanced nuclear reactor as a source of high-temperature process heat, a power cycle and a coupled steam electrolysis loop. Several reactor types and power cycles have been considered, over a range of reactor coolant outlet temperatures. In terms of experimental research, the INL has recently completed an Integrated Laboratory Scale (ILS) HTE test at the 15 kW level. The initial hydrogen production rate for the ILS test was in excess of 5000 liters per hour. Details of the ILS design and operation will be presented. Current small-scale experimental research is focused on improving the degradation characteristics of the electrolysis cells and stacks. Small-scale testing ranges from single cells to multiple-cell stacks. The INL is currently in the process of testing several state-of-the-art anode-supported cells and is working to broaden its relationship with industry in order to improve the long-term performance of the cells.
本文介绍了爱达荷国家实验室(INL)高温电解(HTE)研究与开发项目的最新情况,概述了最近大规模系统建模的结果和实验项目的现状。使用商业代码UniSim,并添加定制的高温电解槽模块,获得了系统分析结果。系统模拟的工艺流程图包括一个先进的核反应堆作为高温工艺热源,一个动力循环和一个耦合蒸汽电解回路。在反应堆冷却剂出口温度范围内,已经考虑了几种反应堆类型和动力循环。在实验研究方面,实验室最近完成了一项15千瓦级的综合实验室规模(ILS) HTE测试。ILS试验的初始产氢速率超过每小时5000升。将介绍盲降系统的设计和操作细节。目前的小规模实验研究主要集中在改善电解电池和电解堆的降解特性上。小规模测试范围从单单元到多单元堆叠。INL目前正在测试几种最先进的阳极支持电池,并正在努力扩大与工业界的关系,以提高电池的长期性能。
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引用次数: 6
Heat exchanger temperature response for duty-cycle transients in the NGNP/HTE. NGNP/HTE中热交换器占空比瞬态温度响应。
Pub Date : 2009-03-12 DOI: 10.1787/9789264087156-47-EN
Richard B. Vilim
Control system studies were performed for the Next Generation Nuclear Plant (NGNP) interfaced to the High Temperature Electrolysis (HTE) plant. Temperature change and associated thermal stresses are important factors in determining plant lifetime. In the NGNP the design objective of a 40 year lifetime for the Intermediate Heat Exchanger (IHX) in particular is seen as a challenge. A control system was designed to minimize temperature changes in the IHX and more generally at all high-temperature locations in the plant for duty-cycle transients. In the NGNP this includes structures at the reactor outlet and at the inlet to the turbine. This problem was approached by identifying those high-level factors that determine temperature rates of change. First are the set of duty cycle transients over which the control engineer has little control but which none-the-less must be addressed. Second is the partitioning of the temperature response into a quasi-static component and a transient component. These two components are largely independent of each other and when addressed as such greater understanding of temperature change mechanisms and how to deal with them is achieved. Third is the manner in which energy and mass flow rates are managed. Generally one aims for a temperature distribution that minimizes spatial non-uniformity of thermal expansion in a component with time. This is can be achieved by maintaining a fixed spatial temperature distribution in a component during transients. A general rule of thumb for heat exchangers is to maintain flow rate proportional to thermal power. Additionally the product of instantaneous flow rate and heat capacity should be maintained the same on both sides of the heat exchanger. Fourth inherent mechanisms for stable behavior should not be compromised by active controllers that can introduce new feedback paths and potentially create under-damped response. Applications of these principles to the development of a plant control strategy for the reference NGNP/HTE plant can be found in the body of this report. The outcome is an integrated plant/control system design. The following conclusions are drawn from the analysis: (1) The plant load schedule can be managed to maintain near-constant hot side temperatures over the load range in both the nuclear and chemical plant. (2) The reactor open-loop response is inherently stable resulting mainly from a large Doppler temperature coefficient compared to the other reactivity temperature feedbacks. (3) The typical controller used to manage reactor power production to maintain reactor outlet temperature at a setpoint introduces a feedback path that tends to destabilize reactor power production in the NGNP. (4) A primary loop flow controller that forces primary flow to track PCU flow rate is effective in minimizing spatial temperature differentials within the IHX. (5) Inventory control in both the primary and PCU system during ramp load change transients is an effective means of main
对与高温电解(HTE)厂对接的下一代核电厂(NGNP)进行了控制系统研究。温度变化和相关的热胁迫是决定植物寿命的重要因素。在NGNP中,中间热交换器(IHX) 40年使用寿命的设计目标尤其被视为一项挑战。设计了一个控制系统,以尽量减少IHX的温度变化,更广泛地说,在工厂的所有高温位置,用于占空比瞬变。在NGNP中,这包括反应堆出口和涡轮机进口的结构。这个问题是通过确定那些决定温度变化率的高级因素来解决的。首先是一组占空比暂态,控制工程师对其几乎没有控制能力,但仍然必须加以解决。其次是将温度响应划分为准静态分量和瞬态分量。这两个组成部分在很大程度上是相互独立的,当这样解决时,对温度变化机制和如何处理它们的更好理解就实现了。第三是管理能量和质量流率的方式。一般来说,人们的目标是使一个部件的热膨胀随时间的空间不均匀性最小化的温度分布。这可以通过在瞬态期间保持组件的固定空间温度分布来实现。热交换器的一般经验法则是保持流量与热功率成正比。另外,换热器两侧的瞬时流量与热容量的乘积应保持相同。第四,稳定行为的固有机制不应被主动控制器破坏,因为主动控制器可能引入新的反馈路径,并可能产生欠阻尼响应。在本报告的正文中可以找到这些原则在为参考NGNP/HTE工厂制定工厂控制战略方面的应用。其结果是一个集成的工厂/控制系统设计。分析得出以下结论:(1)核电站和化工厂的负荷计划都可以在负荷范围内保持热侧温度接近恒定。(2)与其他反应性温度反馈相比,反应器开环响应具有固有的稳定性,这主要是由于反应器的多普勒温度系数较大。(3)典型的用于管理反应堆功率生产以保持反应堆出口温度在一个设定值的控制器引入了一个反馈路径,该路径倾向于使NGNP中的反应堆功率生产不稳定。(4)主回路流量控制器强制主流量跟踪PCU流量,有效地减少了IHX内的空间温差。(5)在坡道负荷变化瞬态期间,主系统和PCU系统的库存控制是在减少电力负荷时保持高NGNP热效率的有效手段。(6)当设备容量限制使库存控制无法有效实施时,汽轮机旁通控制是应对发电机负荷阶跃变化的有效手段。(7)涡轮旁通控制能有效地限制PCU轴在发电机负荷失转情况下的超速。(8)该控制策略能有效地限制瞬态期间IHX空间温度分布的时间变化。从本质上讲,IHX的行为方式可以使IHX的每个点在瞬态过程中经历大约相同的温度变化率。(9)发现闭环布雷顿循环的稳定性对汽机性能图上的操作位置很敏感。这里存在着相互竞争的利益:更稳定的运行意味着在降低整体循环效率的曲线上运行。今后的工作应更详细地处理在这项工作过程中暴露出来的因素。具体而言:(1)在使用反应器出口温度控制器时,应进行稳定性分析,以识别控制反应器出口温度稳定性的现象。目标是确定一个性能更好的控制器。(2)未来的模拟应采用多轴节点。本工作中使用的堆芯单轴节点模型会产生初始堆芯反应堆出口温度扰动,这是一个数值伪影。(3)上述关于Brayton循环稳定性和效率对性能曲线特征和使用的依赖的权衡需要更好地理解。(4)氙气的作用在本工作中被忽视,需要在今后的工作中纳入。
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引用次数: 2
SESSION V - ADS Experiments and Test Facilities 第五部分- ADS实验和测试设施
Pub Date : 2008-01-01 DOI: 10.1787/9789264044791-8-EN
H. Abderrahim, M. Tanigaki
The GUINEVERE project is a European project in the framework of FP6 IP-EUROTRANS. The IP-EUROTRANS project aims at addressing the main issues for ADS development in the framework of partitioning and transmutation for nuclear waste volume and radiotoxicity reduction. The GUINEVERE project is carried out in the context of Domain 2 of IP-EUROTRANS, ECATS, devoted to specific experiments for the coupling of an accelerator, a target and a subcritical core. These experiments should provide an answer to the questions of on-line reactivity monitoring, subcriticality determination and operational procedures (loading, start-up, shutdown, etc.) in an ADS by 2009-2010. The GUINEVERE project will make use of the VENUS reactor, serving as a lead fast critical facility, coupled to a continuous beam accelerator. In order to achieve this goal, the VENUS facility has to be adapted and a modified GENEPI-C accelerator has to be designed and constructed. During the years 2007 and 2008, the VENUS facility will be modified in order to allow the experimental programme to start in 2009. The paper describes the main achievements with regard to the modifications for the VENUS facility.
GUINEVERE项目是FP6 IP-EUROTRANS框架下的欧洲项目。IP-EUROTRANS项目的目的是在核废料体积和减少放射性毒性的分割和嬗变框架内处理ADS发展的主要问题。GUINEVERE项目是在IP-EUROTRANS, ECATS领域2的背景下进行的,致力于加速器,目标和亚临界堆芯耦合的特定实验。这些实验将在2009-2010年之前为ADS的在线反应性监测、亚临界确定和操作程序(加载、启动、关闭等)提供答案。GUINEVERE项目将利用VENUS反应堆作为领先的快速临界设备,与连续束流加速器相结合。为了实现这一目标,必须对VENUS设施进行改造,并且必须设计和建造一个改进的GENEPI-C加速器。在2007年和2008年期间,VENUS设施将进行改造,以便于2009年启动实验项目。本文介绍了VENUS设施改造的主要成果。
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引用次数: 0
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Nuclear science abstracts
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