The Cover Feature shows chlorine-modified soluble melem-based graphitic carbon nitrite (CNCl), which showed better photocatalytic performance than g-C3N4 in the decomposition of methyl orange. CNCl showed much improved dispersibility and solubility in water, DMSO and other solvents. Time-resolved two-dimensional infrared vibrational spectroscopy and other analytical methods were used to understand the photocatalytic performance of CNCl on a microscopic level. More information can be found in the Research Article by J. Wang and co-workers (DOI: 10.1002/cphc.202400356).