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Orbital angular momentum mode femtosecond fiber laser with over 100 MHz repetition rate 重复频率超过100mhz的轨道角动量模飞秒光纤激光器
Pub Date : 2023-01-01 DOI: 10.7498/aps.72.20231085
None Hang Wu, None Liao Chen, None Shuai Li, None Yvfan Du, None Chi Zhang, None Xinliang Zhang
Orbital Angular Momentum (OAM) lasers have potential demand in many applications such as large capacity communication systems, laser processing, particle manipulation and quantum optics. OAM mode femtosecond fiber laser has become the research focus with the advantages of simple structure, low cost and high peak power. The current OAM mode femtosecond fiber lasers have made breakthroughs in the repetition frequency, pulse width, spectrum width and other key parameters, but it is difficult to achieve good overall performance. Besides, the repetition rate is currently in tens of MHz. In this paper, a large-bandwidth mode coupler is made based on the mode phase matching principle. Among them, the first order mode coupler with 3dB polarization dependent loss is made by the technology of strong fused biconical taper, and the second order mode coupler with 0.3dB polarization dependent loss is made by the technology of weak fused biconical taper. Combined with the nonlinear polarization rotation mode-locking mechanism, OAM mode femtosecond fiber lasers with over 100 MHZ repetition rate are built. The achievement of the key parameters is attributed to the selection of dispersion shifted fibers that can accurately adjust intracavity dispersion. Compared to traditional dispersion compensation fibers (DCF), the group velocity dispersion is reduced by an order of magnitude, so it can better adjust intracavity dispersion to achieve the indicators of large spectral bandwidth and narrow pulse width. In addition, the diameter of the fiber is 8μm, which is the same as that of a single mode fiber. Compared to DCF, the fusion loss can be ignored, so only a shorter gain Erbium-doped fiber is required that ensure a shorter overall cavity length and achieve high repetition frequency. The experimental results show that the first order OAM mode fiber laser has 113.6 MHz repetition rate, 98 fs half-height full pulse width, and 101nm 10-dB bandwidth. Second-order OAM mode fiber laser has 114.9 MHz repetition rate, 60 fs half-height full pulse width, and 100nm 10-dB bandwidth. Compared with the reported schemes, our scheme has better performance in key parameters such as repetition rate, pulse width and spectral width. We believe that the OAM mode fiber laser with good over performance is expected to be more widely used in OAM communication, particle manipulation and other research fields.
轨道角动量激光器在大容量通信系统、激光加工、粒子操纵和量子光学等领域具有潜在的应用需求。OAM模式飞秒光纤激光器以其结构简单、成本低、峰值功率高等优点成为研究热点。目前的OAM模式飞秒光纤激光器在重复频率、脉宽、谱宽等关键参数上取得了突破,但难以实现良好的综合性能。此外,重复频率目前在几十兆赫。本文基于模式相位匹配原理,制作了一种大带宽模式耦合器。其中,具有3dB极化依赖损耗的一阶模式耦合器采用强熔接双锥技术制造,具有0.3dB极化依赖损耗的二阶模式耦合器采用弱熔接双锥技术制造。结合非线性偏振旋转锁模机构,构建了重复频率超过100 MHZ的OAM模式飞秒光纤激光器。关键参数的实现归功于色散位移光纤的选择,该光纤可以准确地调节腔内色散。与传统色散补偿光纤(DCF)相比,群速度色散降低了一个数量级,因此可以更好地调节腔内色散,实现大频谱带宽和窄脉宽的指标。光纤直径为8μm,与单模光纤直径相同。与DCF相比,融合损耗可以忽略不计,因此只需要更短的增益掺铒光纤,就可以保证更短的总腔长和更高的重复频率。实验结果表明,一阶OAM模式光纤激光器具有113.6 MHz的重复频率、98 fs的半高全脉冲宽度和101nm的10db带宽。二阶OAM模式光纤激光器具有114.9 MHz重复频率,60 fs半高全脉宽,100nm 10db带宽。与已有的方案相比,我们的方案在重复率、脉冲宽度和谱宽等关键参数上具有更好的性能。我们相信,具有良好超性能的OAM模式光纤激光器有望在OAM通信、粒子操纵等研究领域得到更广泛的应用。
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引用次数: 0
Magnetic and spin transport properties of a two-dimensional magnetic semiconductor kagome lattice Nb<sub>3</sub>Cl<sub>8</sub> monolayer 二维磁性半导体kagome晶格Nb&lt;sub&gt;3&lt;/sub&gt;Cl&lt;sub&gt;8&lt;/sub&gt单层
Pub Date : 2023-01-01 DOI: 10.7498/aps.73.20231163
None Fan Xiao-Zheng, None Li Yi-Lian, None Wu Yi, None Chen Jun-Cai, None Xu Guo-Liang, None An Yi-Peng
Two-dimensional semiconductor materials with intrinsic magnetism have great application prospects in realizing spintronic devices with low power consumption, small size and high efficiency. Some two-dimensional materials with special lattice structures, such as kagome lattice crystals, are favored by researchers because of their novel properties in magnetism and electronic properties. Recently, a new two-dimensional magnetic semiconductor material Nb3Cl8 monolayer with kagome lattice structure was successfully prepared, which provides a new platform for exploring two-dimensional magnetic semiconductor devices with kagome structure. In this work, we study the electronic structure and magnetic anisotropy of Nb3Cl8 monolayer. We also further construct its p-n junction diode and study its spin transport properties by using density functional theory combined with non-equilibrium Green's function method. The results show that the phonon spectrum of the Nb3Cl8 monolayer has no negative frequency, confirming its dynamic stability. The band gap of the spin-down state (1.157 eV) is significantly larger than that of the spin-up state (0.639 eV). The magnetic moment of the Nb3Cl8 monolayer is 0.997 μB, and its easy magnetization axis is in the plane and along the x axis direction based on its energy of magnetic anisotropy. Nb atoms make the main contribution to the magnetic anisotropy. When the strain is applied, the band gap of the spin-down states will decrease, while the band gap of the spin-up state is monotonously decreased from the negative (compress) to positive (tensile) strain. As the strain variable goes from -6% to 6%, the contribution of Nb atoms to the total magnetic moment gradually increases. Moreover, strain causes the easy magnetization axis of the Nb3Cl8 monolayer to flip vertically from in-plane to out-plane. The designed p-n junction diode nanodevice based on Nb3Cl8 monolayer exhibits an obvious rectification effect. In addition, the current in the spin-up state is larger than that in the spin-down state, exhibiting a spin-polarized transport behavior. Moreover, a negative differential resistance (NDR) phenomenon is also observed, which could be used in the NDR devices. These results demonstrate that the Nb3Cl8 monolayer material has great potential application in the next generation of high-performance spintronic devices, and further experimental verification and exploration of this material and related two-dimensional materials are needed.
具有本征磁性的二维半导体材料在实现低功耗、小尺寸、高效率的自旋电子器件方面具有广阔的应用前景。一些具有特殊晶格结构的二维材料,如kagome晶格晶体,因其新颖的磁性和电子性质而受到研究人员的青睐。最近,一种新的二维磁性半导体材料Nb<sub>3& gt; /sub>Cl<sub>8</sub>成功制备了具有kagome晶格结构的单层材料,为探索具有kagome结构的二维磁性半导体器件提供了新的平台。在这项工作中,我们研究了Nb<sub>3</sub>Cl<sub>8</sub>单层。我们还进一步构造了它的<em>p-n</em>利用密度泛函理论结合非平衡格林函数方法研究了结二极管的自旋输运性质。结果表明:Nb<sub>3</sub>Cl<sub>8</sub>单层无负频率,证实了其动态稳定性。自旋向下态的带隙(1.157 eV)明显大于自旋向上态的带隙(0.639 eV)。Nb<sub>3</sub>Cl<sub>8</sub>单层为0.997 μ<sub>B</sub>,其易磁化轴在平面内,沿<em>x</em>轴向基于其能量的磁各向异性。Nb原子对磁各向异性起主要作用。当施加应变时,自旋向下状态的带隙减小,而自旋向上状态的带隙从负(压缩)应变单调减小到正(拉伸)应变。随着应变变量从-6%增大到6%,Nb原子对总磁矩的贡献逐渐增大。应变导致Nb<sub>3</sub>Cl<sub>8</sub>单层从平面内垂直翻转到平面外。设计的<em>p & n</em>基于Nb<sub>3</sub>Cl<sub>8</sub>单层具有明显的整流效果。此外,自旋向上态的电流大于自旋向下态的电流,表现出自旋极化输运行为。此外,还观察到负差分电阻(NDR)现象,该现象可用于NDR器件。这些结果表明:Nb<sub>3</sub>Cl<sub>8<单层材料在下一代高性能自旋电子器件中具有巨大的应用潜力,需要对该材料及相关二维材料进行进一步的实验验证和探索。
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引用次数: 0
In-plane optical anisotropy of quasi-one-dimensional layered semiconductor Nb<sub>4</sub>P<sub>2</sub>S<sub>21</sub> single crystal 准一维层状半导体Nb&lt;sub&gt;4&lt;/sub&gt;P&lt;sub&gt;2&lt;/sub&gt;S&lt;sub&gt;21&lt;/sub&gt;单晶
Pub Date : 2023-01-01 DOI: 10.7498/aps.72.20231539
None Cheng Qiu-Zhen, None Huang Yin, None Li Yu-Hui, None Zhang Kai, None Xian Guo-Yu, None Liu He-Yuan, None Che Bing-Yu, None Pan Lu-Lu, None Han Ye-Chao, None Zhu Ke, None Qi Qi, None Xie Yao-Feng, None Pan Jin-Bo, None Chen Hai-Long, None Li Yong-Feng, None Guo Hui, None Yang Hai-Tao, None Gao Hong-Jun
Transition-metal phosphorous chalcogenide MPS (M = transition metal), an emerging type of two-dimensional (2D) van der Waals material with the unique optical and opto-electronic properties, has received much attention. The quasi-one-dimensional chain structure of Nb4P2S21 will possess the strong anisotropic optical and photoelectric properties. Therefore, the single crystal and low-dimensional materials of Nb4P2S21 have potential applications in new polarization controllers, polarization-sensitive photoelectronic detectors, etc. However, there is still a lack of research on the anisotropic optical properties of the high-quality Nb4P2S21 single crystals. Herein, the millimeter-sized Nb4P2S21 single crystals are successfully prepared by the chemical vapor transport method. The chemical composition, the crystal structure and the anisotropic optical properties of the Nb4P2S21 single crystals are carefully analyzed. The energy dispersive X-ray spectroscopy results show that the element distribution is uniform and the element ratio is close to the stoichiometric ratio. The X-ray diffraction and the transmission electron microscopy results show a good crystallinity. The absorption spectra shows that the optical band gap of the Nb4P2S21 single crystal is 1.8 eV. Interestingly, the Nb4P2S21 single crystal can be mechanically exfoliated to obtain few-layer material. The thickness-dependent Raman spectra show that the Raman vibration peaks of bulk and few-layer Nb4P2S21 each have only a weak shift, indicating a weak interlayer interaction in the Nb4P2S21 single crystal. In order to make an in-depth study of the optical properties of Nb4P2S21 single crystals, the polarized-dependent Raman spectra and the femtosecond transient absorption (TA) spectra by using pump pulses and probe pulses with a wavelength of 400 nm and a wavelength range of 500–700 nm are recorded. Importantly, the polarized-dependent Raman scattering spectra with the angle-dependent measurements reveal that the intensity of Raman peak at 202 cm–1 and at 489 cm–1 show a 2-fold symmetry and a 4-fold symmetry in the parallel and vertical polarization configurations, respectively. Moreover, the results of ultrafast carrier dynamics with the in-plane rotation angles of Nb4P2S21 single crystals in the parallel polarization configurations, clearly indicate that both the hot carrier number and the relaxation rate after photoexcitation have the in-plane anisotropic properties. These results are useful in understanding the in-plane anisotropic optical properties of Nb4P2S21 sin
过渡金属硫化物磷<i>M</i>PS (<i>M</i>过渡金属(transition metal)是一种新兴的二维(2D)范德华材料,具有独特的光学和光电性质,受到了广泛的关注。Nb<sub>4& gt; /sub>P<sub>2</sub>S<sub>21</sub>将具有较强的各向异性光学和光电性能。因此,Nb<sub>4& gt; /sub>P<sub>2</sub>S<sub>21</sub>在新型偏振控制器、偏振敏感光电探测器等方面具有潜在的应用前景。然而,对于高质量的Nb<sub>4& gt; /sub>P<sub>2</sub>S<sub>21</sub>单一的晶体。在此,毫米尺寸的Nb<sub>4</sub>P<sub>2</sub> 21</sub>采用化学气相输运法制备了单晶。Nb<sub>4& gt; /sub>P<sub>2</sub>S<sub>21</sub>仔细分析单晶。能量色散x射线谱分析结果表明,元素分布均匀,元素比接近化学计量比。x射线衍射和透射电镜结果表明,该材料具有良好的结晶度。吸收光谱表明:Nb<sub>4</sub>P<sub>2</sub>S<sub>21</sub>单晶为1.8 eV。有趣的是,Nb<sub>4& gt; /sub>P<sub>2& gt; /sub>单晶可以机械剥离,得到少层材料。随厚度变化的拉曼光谱表明,体层和少层Nb<sub>4</sub>P<sub>2</sub>S<sub>21</sub>每一个都只有一个弱位移,表明在Nb<sub>4& gt; /sub>P<sub>2</sub>S<sub>21</sub>单晶。为了深入研究Nb<sub>4</sub>P<sub>2</sub>S<sub>21</sub>记录了波长为400 nm和500 ~ 700 nm的泵浦脉冲和探测脉冲作用下的单晶、偏振相关拉曼光谱和飞秒瞬态吸收光谱。重要的是,偏振相关的拉曼散射光谱与角度相关的测量结果表明,拉曼强度在202 cm<sup> -1</sup>在489厘米<sup> -1</sup>在平行极化构型和垂直极化构型中分别表现出2倍对称性和4倍对称性。此外,在Nb<sub>4</sub>P<sub>2</sub>S<sub>21</sub>平行极化构型的单晶清楚地表明,光激发后的热载流子数和弛豫速率都具有面内各向异性。这些结果有助于理解Nb<sub>4</sub>P<sub>2</sub>S<sub>21</sub>这可以进一步促进其在低维角相关光电子学中的应用。
{"title":"In-plane optical anisotropy of quasi-one-dimensional layered semiconductor Nb&lt;sub&gt;4&lt;/sub&gt;P&lt;sub&gt;2&lt;/sub&gt;S&lt;sub&gt;21&lt;/sub&gt; single crystal","authors":"None Cheng Qiu-Zhen, None Huang Yin, None Li Yu-Hui, None Zhang Kai, None Xian Guo-Yu, None Liu He-Yuan, None Che Bing-Yu, None Pan Lu-Lu, None Han Ye-Chao, None Zhu Ke, None Qi Qi, None Xie Yao-Feng, None Pan Jin-Bo, None Chen Hai-Long, None Li Yong-Feng, None Guo Hui, None Yang Hai-Tao, None Gao Hong-Jun","doi":"10.7498/aps.72.20231539","DOIUrl":"https://doi.org/10.7498/aps.72.20231539","url":null,"abstract":"Transition-metal phosphorous chalcogenide <i>M</i>PS (<i>M</i> = transition metal), an emerging type of two-dimensional (2D) van der Waals material with the unique optical and opto-electronic properties, has received much attention. The quasi-one-dimensional chain structure of Nb<sub>4</sub>P<sub>2</sub>S<sub>21</sub> will possess the strong anisotropic optical and photoelectric properties. Therefore, the single crystal and low-dimensional materials of Nb<sub>4</sub>P<sub>2</sub>S<sub>21</sub> have potential applications in new polarization controllers, polarization-sensitive photoelectronic detectors, etc. However, there is still a lack of research on the anisotropic optical properties of the high-quality Nb<sub>4</sub>P<sub>2</sub>S<sub>21</sub> single crystals. Herein, the millimeter-sized Nb<sub>4</sub>P<sub>2</sub>S<sub>21</sub> single crystals are successfully prepared by the chemical vapor transport method. The chemical composition, the crystal structure and the anisotropic optical properties of the Nb<sub>4</sub>P<sub>2</sub>S<sub>21</sub> single crystals are carefully analyzed. The energy dispersive X-ray spectroscopy results show that the element distribution is uniform and the element ratio is close to the stoichiometric ratio. The X-ray diffraction and the transmission electron microscopy results show a good crystallinity. The absorption spectra shows that the optical band gap of the Nb<sub>4</sub>P<sub>2</sub>S<sub>21</sub> single crystal is 1.8 eV. Interestingly, the Nb<sub>4</sub>P<sub>2</sub>S<sub>21</sub> single crystal can be mechanically exfoliated to obtain few-layer material. The thickness-dependent Raman spectra show that the Raman vibration peaks of bulk and few-layer Nb<sub>4</sub>P<sub>2</sub>S<sub>21</sub> each have only a weak shift, indicating a weak interlayer interaction in the Nb<sub>4</sub>P<sub>2</sub>S<sub>21</sub> single crystal. In order to make an in-depth study of the optical properties of Nb<sub>4</sub>P<sub>2</sub>S<sub>21</sub> single crystals, the polarized-dependent Raman spectra and the femtosecond transient absorption (TA) spectra by using pump pulses and probe pulses with a wavelength of 400 nm and a wavelength range of 500–700 nm are recorded. Importantly, the polarized-dependent Raman scattering spectra with the angle-dependent measurements reveal that the intensity of Raman peak at 202 cm<sup>–1</sup> and at 489 cm<sup>–1</sup> show a 2-fold symmetry and a 4-fold symmetry in the parallel and vertical polarization configurations, respectively. Moreover, the results of ultrafast carrier dynamics with the in-plane rotation angles of Nb<sub>4</sub>P<sub>2</sub>S<sub>21</sub> single crystals in the parallel polarization configurations, clearly indicate that both the hot carrier number and the relaxation rate after photoexcitation have the in-plane anisotropic properties. These results are useful in understanding the in-plane anisotropic optical properties of Nb<sub>4</sub>P<sub>2</sub>S<sub>21</sub> sin","PeriodicalId":10252,"journal":{"name":"Chinese Physics","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"2023-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"135319624","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
The optimizing numerical simulation of beam ions loss due to toroidal field ripple on EXL-50U spherical torus EXL-50U球面环面环面场纹波对束流离子损耗的优化数值模拟
Pub Date : 2023-01-01 DOI: 10.7498/aps.72.20230749
None Hao Bao-Long, None Li Ying-Ying, None Chen Wei, None Hao Guang-Zhou, None Gu Xiang, None Sun Tian-Tian, None Wang Yu-Min, None Dong Jia-Qi, None Yuan Bao-Shan, None Peng Yuan-Kai, None Shi Yue-jiang, None Xie Hua-sheng, None Liu Min-Sheng, None ENN TEAM
Realization of high performance plasma of EXL-50U is very sensitive to NBI (neutral beam injection) heating, and it is expected that the fast ions of NBI are confined well and their energy is transferred to the background plasma by collision moderating. In this paper, the loss of fast ion ripple is simulated based on the equilibrium configuration, fast ion distribution and device waviness data given by the integrated simulation. It is found that the loss fraction of fast ion ripple is about 37%, and the local hot spot is about 0.6 MW/m2, which is unacceptable for the experimental operation of the device. The optimization method includes moving the plasma position and adding FI (ferritic steel plug-in) to reduce the ripple degree, increasing the Ip (plasma current) and optimizing the NBI injection angle. The results show that the ripple distribution must be controlled and the Ip must be increased to more than 600 kA, so that the fast ion loss can be reduced to 3%–4% and the local heat spot can be reduced by an order of magnitude. In this paper, the evaluation methods of fast ion ripple loss in device design are summarized, including the fast ion distribution in phase space, the overlap degree of ripple loss area, and the particle tracking on the time scale of total factor slowing down. The engineering and physical ways to reduce ripple loss are also summarized to provide simulation support for integrated simulation iterative optimization and plant operation.
EXL-50U高性能等离子体的实现对NBI(中性束注入)加热非常敏感,预计NBI中的快离子将被很好地约束并通过碰撞减速将其能量转移到背景等离子体中。本文基于综合仿真给出的平衡态、快离子分布和器件波度数据,对快离子纹波的损耗进行了模拟。研究发现,快速离子纹波的损耗率约为37%,局部热点约为0.6 MW/m<sup>2</sup>,这对于器件的实验运行是不可接受的。优化方法包括移动等离子体位置,加入FI(铁素体钢插件)降低纹波度,增加<i> /i><sub>p</sub>(等离子体电流)和优化NBI注入角。结果表明,必须控制纹波分布,并且<i> i> /i><sub>p</sub>必须提高到600 kA以上,才能使快离子损失降低到3% ~ 4%,使局部热点降低一个数量级。本文综述了器件设计中快速离子纹波损失的评价方法,包括快速离子在相空间中的分布、纹波损失面积的重叠程度以及全因子慢化时间尺度上的粒子跟踪。总结了减少纹波损耗的工程和物理方法,为集成仿真迭代优化和工厂运行提供仿真支持。
{"title":"The optimizing numerical simulation of beam ions loss due to toroidal field ripple on EXL-50U spherical torus","authors":"None Hao Bao-Long, None Li Ying-Ying, None Chen Wei, None Hao Guang-Zhou, None Gu Xiang, None Sun Tian-Tian, None Wang Yu-Min, None Dong Jia-Qi, None Yuan Bao-Shan, None Peng Yuan-Kai, None Shi Yue-jiang, None Xie Hua-sheng, None Liu Min-Sheng, None ENN TEAM","doi":"10.7498/aps.72.20230749","DOIUrl":"https://doi.org/10.7498/aps.72.20230749","url":null,"abstract":"Realization of high performance plasma of EXL-50U is very sensitive to NBI (neutral beam injection) heating, and it is expected that the fast ions of NBI are confined well and their energy is transferred to the background plasma by collision moderating. In this paper, the loss of fast ion ripple is simulated based on the equilibrium configuration, fast ion distribution and device waviness data given by the integrated simulation. It is found that the loss fraction of fast ion ripple is about 37%, and the local hot spot is about 0.6 MW/m<sup>2</sup>, which is unacceptable for the experimental operation of the device. The optimization method includes moving the plasma position and adding FI (ferritic steel plug-in) to reduce the ripple degree, increasing the <i>I</i><sub>p</sub> (plasma current) and optimizing the NBI injection angle. The results show that the ripple distribution must be controlled and the <i>I</i><sub>p</sub> must be increased to more than 600 kA, so that the fast ion loss can be reduced to 3%–4% and the local heat spot can be reduced by an order of magnitude. In this paper, the evaluation methods of fast ion ripple loss in device design are summarized, including the fast ion distribution in phase space, the overlap degree of ripple loss area, and the particle tracking on the time scale of total factor slowing down. The engineering and physical ways to reduce ripple loss are also summarized to provide simulation support for integrated simulation iterative optimization and plant operation.","PeriodicalId":10252,"journal":{"name":"Chinese Physics","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"2023-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"135356168","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Directed Transport of Deformable Self-propulsion Particles in an Asymmetric Periodic Channel 非对称周期通道中可变形自推进粒子的定向输运
Pub Date : 2023-01-01 DOI: 10.7498/aps.72.20230825
None Guo Rui-Xue, None Ai Bao-Quan
Molecular motor can effectively convert chemical energy into mechanical energy in living organisms, and its research is currently at the forefront of study in biology and physics . The dynamic process of its guided movement, along with the crucial role they play in intra-cellular material transport, has significantly aroused the interest of many researchers. Theoretical and experimental researches have allowed detailed examinations of the motion attributes of these molecular motors. The Brownian ratchet model important. It provides an illustration of a non-equilibrium system that transforms thermal fluctuation into guided transport by utilizing temporal or spatial asymmetry. The mechanism has been extensively explored and studied across fields including physics, biology and nanotechnology. Investigations into a variety of ratchets and identification of optimum conditions contribute to a deeper understanding of guided Brownian particle transport.Preceding studies on ratchet systems largely concentrated on the rectification motions of diverse types of particles – active, polar and chiral – in asymmetric structures. However, the transport of deformable particles in asymmetric channel has not been examined relatively unexamined. Particles in soft material systems such as cell monolayer, tissue, foam, and emulsion are frequently deformable. The shape deformation of these soft particles significantly affects the system's dynamic behavior. Thus, understanding the guided transport of these deformable particles within a confined structure is crucial.In order to explain this problem more clearlyt, we numerically simulate the guided transportation of active, deformable particles within a two-dimensional, periodic, asymmetric channel. We identify the factors that influence the transport of these particles within a confined structure. The main feature of the deformable particle model is that the particle’s shape is characterized by multiple degree of freedom. For active deformable particles, self-propulsion speed disrupts thermodynamic equilibrium, leading to guided transport in spatially asymmetric condition. Our findings demonstrate that a particle's direction of movement is entirely determined by the channel's asymmetric parameter, and it tends to be attracted towards increased stability. Augmenting particle self-propulsion speed and particle softness can facilitate ratchet transport. When v0[请说明这是什么物理量] is large, the particle’s tensile effect becomes more apparent, and particle softening significantly enhances directed transport. In contrast, an increase in density and rotational diffusion can slow particle rectification. Increased density can obstruct particles, making channel passage more difficult. Elevated rotational diffusion reduces persistence length, challenging particle transition through channels. With constant density, a greater number of particles will also encourage rectification. These research fi
分子马达是生物体内能有效地将化学能转化为机械能的装置,目前对分子马达的研究处于生物学和物理学的前沿。其引导运动的动态过程,以及在细胞内物质运输中所起的关键作用,引起了许多研究者的极大兴趣。理论和实验研究使得对这些分子马达的运动特性进行了详细的研究。布朗棘轮模型很重要。它提供了一个非平衡系统的例子,通过利用时间或空间不对称将热波动转化为引导输运。这一机制在物理学、生物学和纳米技术等领域得到了广泛的探索和研究。对各种棘轮的研究和最佳条件的确定有助于更深入地理解引导布朗粒子输运。以前对棘轮系统的研究主要集中在不对称结构中不同类型粒子(活性、极性和手性)的整流运动。然而,可变形粒子在不对称通道中的输运尚未得到研究。软材料系统中的颗粒,如细胞单层、组织、泡沫和乳液,经常是可变形的。这些软颗粒的形状变形对系统的动力学行为有显著影响。因此,理解这些可变形粒子在受限结构中的导向输运是至关重要的。为了更清楚地解释这个问题,我们数值模拟了二维、周期性、不对称通道中活动的、可变形粒子的导向输运。我们确定了影响这些粒子在受限结构内传输的因素。可变形粒子模型的主要特征是粒子的形状具有多自由度。对于主动可变形粒子,自推进速度破坏热力学平衡,导致空间不对称条件下的引导输运。我们的发现表明,粒子的运动方向完全由通道的不对称参数决定,它倾向于被吸引到增加的稳定性。提高粒子自推进速度和粒子柔软度有利于棘轮运输。当<i>v</i><sub>0</sub>[j]大时,颗粒的拉伸效应更加明显,颗粒的软化明显增强了定向输运。相反,密度和旋转扩散的增加会减缓颗粒整流。增加的密度会阻碍颗粒,使通道通过更加困难。升高的旋转扩散减少了持续时间,挑战了粒子通过通道的转变。在密度不变的情况下,更多的颗粒也会促进整流。这些研究结果为研究受限结构中可变形颗粒的输运行为提供了有价值的见解。它们还为软物质领域的应用实验提供了重要的理论支持。
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引用次数: 0
Phase transition regulation, magnetocaloric effect, and abnormal thermal expansion 相变调节、磁热效应和异常热膨胀
Pub Date : 2023-01-01 DOI: 10.7498/aps.72.20231118
None Yuan Lin, None Fengxia Hu, None Baogen Shen
As a common phenomenon in nature, phase transition has caught people’s attention for a long time. Thus, it has been applied to various fields, such as refrigeration, information and energy storage, and negative thermal expansion. With the virtues of environmental friendliness, high efficiency, noiselessness and easy miniaturization, solid refrigeration technique based on magnetocaloric, electrocaloric, and mechanocaloric effects, is a promising candidate to replace vapor compression technique. Among them, magnetocaloric effect has the longest research history. However, the shortcomings of magnetocaloric effect driven by a single magnetic field limit its solid-state refrigeration application, such as insufficient amplitude of caloric effect, large hysteresis loss, and narrow refrigeration temperature span. To solve these problems, multifield tuning and multicaloric effect came into people's sight. This review introduces our recent research on improving the caloric effect by applying multifield, such as boosting the entropy change, enlarging the transition temperature span, tuning the transition temperature, and lowering the hysteresis losses. Meanwhile, the thermodynamics of multifield and coupled-caloric effect is presented. On the other hand, abnormal thermal expansion (zero thermal expansion, negative thermal expansion) materials have important applications in precision manufacturing. The phase transition and lattice effect dominated by magnetic atoms in the giant magnetocaloric materials with strong magnetic-crystal coupling provide an ideal platform for exploring abnormal thermal expansion. This review also introduces our recent research on abnormal thermal expansion in magnetocaloric materials and prospects relevant research in future.
相变作为自然界的一种普遍现象,长期以来一直受到人们的关注。因此,它已被应用于制冷、信息和储能、负热膨胀等各个领域。基于磁热效应、电热效应和机械能效应的固体制冷技术具有环保、高效、无噪音和易于小型化等优点,是取代蒸汽压缩技术的一个很有前途的选择。其中,磁热效应的研究历史最为悠久。然而,单磁场驱动的磁热效应存在热效应幅度不足、磁滞损耗大、制冷温度跨度窄等缺点,限制了其在固态制冷中的应用。为了解决这些问题,多场调谐和多色效应进入了人们的视野。本文综述了近年来国内外在提高热效应方面的研究进展,包括提高热效应的熵变、增大相变温度跨度、调节相变温度、降低磁滞损耗等。同时,对多场效应和耦合热效应进行了热力学分析。另一方面,异常热膨胀(零热膨胀、负热膨胀)材料在精密制造中有着重要的应用。强磁晶耦合巨磁热材料中磁性原子主导的相变和晶格效应为研究异常热膨胀提供了理想的平台。介绍了近年来在磁热材料异常热膨胀方面的研究进展,并对今后的研究进行了展望。
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引用次数: 0
Regulation of thermal conductivity of bilayer graphene nanoribbon through interlayer covalent bond and tensile strain 通过层间共价键和拉伸应变调节双层石墨烯纳米带的导热性
Pub Date : 2023-01-01 DOI: 10.7498/aps.72.20231230
None Li Yao-Long, None Li Zhe, None Li Song-Yuan, None Zhang Ren-Liang
The interlayer bonding of graphene is a modification method of graphene, which can change the mechanical and conductivity of graphene, but also affect its thermal properties. In this paper, the non-equilibrium molecular dynamics method is used to study the thermal conductivity of bilayer graphene nanoribbon which is local carbon sp3 hybridization (covalent bond formed between layers) under different concentration and angle of interlayer Covalent bond chain and different tensile strain. The mechanism of the change of the thermal conductivity of bilayer graphene nanoribbon is analyzed through the density of phonon states. The results are as follows. The thermal conductivity of bilayer graphene nanoribbon decreases with the increase of the interlayer covalent bond concentration due to the intensification of phonon scattering and the reduction of phonon group velocities and effective phonon mean free path. Moreover, the decrease rate of thermal conductivity depends on the distribution angle of covalent bond chain. With the increase of interlayer covalent bond concentration, when the interlayer covalent bond chain is parallel to the direction of heat flow, the thermal conductivity decreases the slowest because the heat transfer channel along the heat flow direction is gradually affected; when the interlayer covalent bond chain is at an angle to the direction of heat flow, the thermal conductivity decreases more rapidly, and the larger the angle, the faster the thermal conductivity decreases. The rapid decline of thermal conductivity is due to the formation of interfacial thermal resistance at the interlayer covalent bond chain, where strong phonon-interface scattering occurs. In addition, it is found that the thermal conductivity of bilayer graphene nanoribbon with interlayer bonding will be further reduced by tensile strain due to the intensification of phonon scattering and the reduction of phonon group velocities. The results show that the thermal conductivity of bilayer graphene nanoribbon can be controlled by interlayer bonding and tensile strain. These conclusions are of great significance for the design and thermal control of graphene based nanodevices.
石墨烯的层间键合是石墨烯的一种改性方法,可以改变石墨烯的力学和电导率,但也会影响其热性能。本文采用非平衡分子动力学方法研究了局部碳sp<sup>3</sup>层间共价键链在不同浓度、不同角度和不同拉伸应变下的杂化(层间形成的共价键)。通过声子态密度分析了双层石墨烯纳米带导热系数变化的机理。结果如下:随着层间共价键浓度的增加,声子散射加剧,声子群速度和有效声子平均自由程降低,导致双层石墨烯纳米带的导热系数降低。导热系数的下降速率与共价键链的分布角度有关。随着层间共价键浓度的增加,当层间共价键链与热流方向平行时,由于沿热流方向的换热通道逐渐受到影响,导热系数降低的最慢;当层间共价键链与热流方向成一定角度时,导热系数下降得更快,角度越大,导热系数下降得越快。热导率的快速下降是由于在层间共价键链上形成了界面热阻,在那里发生了强烈的声子界面散射。此外,发现层间键合的双层石墨烯纳米带由于声子散射的加剧和声子群速度的降低,在拉伸应变的作用下,其导热系数会进一步降低。结果表明,双层石墨烯纳米带的热导率可以通过层间键合和拉伸应变来控制。这些结论对石墨烯基纳米器件的设计和热控制具有重要意义。
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引用次数: 0
Theoretical and experimental progress of mesoscopic statistical thermodynamics 介观统计热力学的理论与实验进展
Pub Date : 2023-01-01 DOI: 10.7498/aps.72.20231608
Hai-Tao Quan, Hui Dong, Chang-Pu Sun
Does thermodynamics still hold true for mecroscopic small systems with only limited degrees of freedom? Do concepts such as temperature, entropy, work done, heat transfer, isothermal processes, and the Carnot cycle remain valid? Does the thermodynamic theory for small systems need modifying or supplementing compared with traditional thermodynamics applicable to macroscopic systems? Taking a single-particle system for example, we investigate the applicability of thermodynamic concepts and laws in small systems. We have found that thermodynamic laws still hold true in small systems at an ensemble-averaged level. After considering the information erasure of the Maxwell's demon, the second law of thermodynamics is not violated. Additionally, 'small systems' bring some new features. Fluctuations in thermodynamic quantities become prominent. In any process far from equilibrium, the distribution functions of thermodynamic quantities satisfy certain rigorously established identities. These identities are known as fluctuation theorems. The second law of thermodynamics can be derived from them. Therefore, fluctuation theorems can be considered an upgradation to the second law of thermodynamics. They enable physicists to obtain equilibrium properties (e.g. free energy difference) by measuring physical quantities associated with non-equilibrium processes (e.g. work distributions). Furthermore, despite some distinct quantum features, the performance of quantum heat engine does not outperform that of classical heat engine. The introduction of motion equations into small system makes the relationship between thermodynamics and mechanics closer than before. Physicists can study energy dissipation in non-equilibrium process and optimize the power and efficiency of heat engine from the first principle. These findings enrich the content of thermodynamic theory and provide new ideas for establishing a general framework for non-equilibrium thermodynamics.
热力学对于只有有限自由度的微观小系统仍然成立吗?温度、熵、做功、传热、等温过程和卡诺循环等概念还有效吗?与传统的宏观热力学相比,小系统热力学理论是否需要修改或补充?以单粒子系统为例,研究了热力学概念和定律在小系统中的适用性。我们已经发现热力学定律在小系统的总体平均水平上仍然成立。在考虑麦克斯韦妖的信息擦除后,热力学第二定律没有被违反。此外,“小型系统”带来了一些新功能。热力学量的波动变得突出。在任何远离平衡态的过程中,热力学量的分布函数都满足某些严格建立的恒等式。这些恒等式被称为涨落定理。热力学第二定律可以从它们推导出来。因此,涨落定理可以看作是热力学第二定律的升级。它们使物理学家能够通过测量与非平衡过程(如功分布)相关的物理量来获得平衡特性(如自由能差)。此外,尽管量子热机具有一些明显的量子特征,但其性能并不优于经典热机。在小系统中引入运动方程,使热力学和力学的关系更加紧密。物理学家可以从热力学第一原理出发,研究非平衡过程中的能量耗散,优化热机的功率和效率。这些发现丰富了热力学理论的内容,为建立非平衡态热力学的一般框架提供了新的思路。
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引用次数: 0
Invesigation of the electronic structure and Optoelectronic properties of Si-doped <i>β</i>-Ga<sub>2</sub>O<sub>3</sub> using GGA+U method based on first-principle si掺杂&lt;i&gt;β&lt;/i&gt;-Ga&lt;sub&gt;2&lt;/sub&gt;O&lt;sub&gt;3&lt;/sub&gt;采用基于第一性原理的GGA+U方法
Pub Date : 2023-01-01 DOI: 10.7498/aps.72.20231147
None Zhang Ying-Nan, None Zhang Min, None Zhang Pai, None Hu Wen-Bo
In this work, the formation energy, band structure, state density, differential charge density and optoelectronic properties of undoped and Si doped β-Ga2O3 are calculated using GGA+U method based on density functional theory. The results show that the Si-substituted tetrahedron Ga(1) is more easily synthesized in experiments, and the obtained β-Ga2O3 band gap and Ga 3d state peak are in good agreement with the experimental results, and the effective doping is more likely to be obtained under oxygen-poor conditions. After Si doping, the total energy band moves to the low-energy end, and Fermi level enters the conduction band, showing n-type conductive characterastic. Si 3s orbital electrons occupy the bottom of the conduction band, the degree of electronic coocupy is strengthened, and the conductivity is improved. The dielectric function ε2(ω) results show that with the increase of Si doping concentration, the ability to stimulate conductive electrons first increases and then decreases, which is in good agreement with the quantitative analysis results of conductivity. The optical band gap increases and the absorption band edge rises slowly with the increase of Si doping concentration. The results of absorption spectra show that Si-doped β-Ga2O3 has strong deep ultraviolet photoelectric detection ability. The calculated results provide a theoretical reference for the further experimental investigation and the optimization innovation of Si-doped β-Ga2O3 and relative device design.
本文研究了未掺杂和Si掺杂的<i>β</i>-Ga<sub>2</sub>O<sub>3</sub>采用基于密度泛函理论的GGA+U方法计算。结果表明,硅取代四面体Ga(1)在实验中更容易合成,得到的<i>β</i>- ga>sub>2</sub>O<sub>3</sub>带隙和Ga三维态峰与实验结果吻合较好,贫氧条件下更容易得到有效掺杂。Si掺杂后,总能带向低能端移动,费米能级进入导带,呈现n型导电特性。Si 3s轨道电子占据导带底部,电子占据程度增强,电导率提高。介电函数ε2(ω)结果表明,随着Si掺杂浓度的增加,激发导电电子的能力先增大后减小,这与电导率的定量分析结果吻合较好。随着Si掺杂浓度的增加,光学带隙增大,吸收带边缓慢上升。吸收光谱结果表明,si掺杂的<i>β</i>-Ga<sub>2</sub>O<sub>3</sub>具有较强的深紫外光电检测能力。计算结果为si掺杂<i>β</i>- ga>sub>2</sub>O<sub>3</sub>以及相关装置的设计。
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引用次数: 0
Research on polarization characteristics of background light based on modified polarization difference imaging method 基于改进偏振差成像方法的背景光偏振特性研究
Pub Date : 2023-01-01 DOI: 10.7498/aps.72.20230639
None Xu Jing-Han, None Wu Guo-Jun, None Dong Jing, None Yu Yang, None Feng Fei, None Liu Bo
The random scattering event of light by water medium is the primary reason for the degradation in underwater imaging. Underwater polarization imaging technology can enhance the signal-to-noise ratio of imaging effectively by utilizing the polarization information difference between background scattered light and target light. However, as scattering events increase in the water body, it is difficult to maintain the polarization characteristics of light, which reduces the effect of removing scattering based on polarization characteristics. In addition, the polarization rules of background scattered light in water is unclear, and there is a lack of quantitative description of the polarization characteristics of scattered light. Therefore, researching the polarization transmission characteristics of underwater scattered light is of great significance for the de-scattering work of underwater polarization imaging.In order to clarify the polarization characteristics of underwater background scattered light, especially the polarization angle information, this paper proposes a method for ascertaining polarization angle of background light based on modified polarization difference imaging method. In this method, the coupling relationship between optimal weight coefficient and enhancement measure evaluation (EME) value of the Stokes vector difference result is analyzed, and the background light polarization angle is calculated based on the optimal weight coefficient. Combined with the experiments, the EME distribution trend of the optimal weight coefficient and the modified polarization difference imaging method results in different turbidity water bodies were determined, the scattering suppression limit was explored, and the trend of background scattered light polarization direction with turbidity of water was analyzed. The results show that the proposed method can obtain the exact polarization angle of background scattered light in different water environments, revealing a trend where the polarization direction of background scattered light becomes orthogonal to the incident light direction as the turbidity of the water increases. This research provides a methodological basis for determining the polarization direction of the background scattered light in underwater imaging.
水介质对光的随机散射是导致水下成像质量下降的主要原因。水下偏振成像技术利用背景散射光与目标光的偏振信息差,可以有效提高成像的信噪比。然而,随着水体中散射事件的增加,光的偏振特性难以保持,这降低了基于偏振特性去除散射的效果。此外,背景散射光在水中的偏振规律尚不清楚,缺乏对散射光偏振特性的定量描述。因此,研究水下散射光的偏振透射特性对水下偏振成像的去散射工作具有重要意义。为了明确水下背景散射光的偏振特性,特别是偏振角信息,本文提出了一种基于改进偏振差成像法的背景光偏振角确定方法。该方法分析Stokes矢量差分结果的最优权系数与增强措施评价(EME)值之间的耦合关系,并基于最优权系数计算背景光偏振角。结合实验,确定了最优权重系数和改进偏振差成像方法结果在不同浑浊度水体中的EME分布趋势,探索了散射抑制极限,分析了背景散射光偏振方向随水体浑浊度的变化趋势。结果表明,该方法能够准确地获得不同水体环境下背景散射光的偏振角,并呈现出随着水体浑浊度的增加,背景散射光的偏振方向与入射光方向正交的趋势。该研究为水下成像中背景散射光偏振方向的确定提供了方法学依据。
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引用次数: 0
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Chinese Physics
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