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Inter-basin groundwater flow in the Ordos Basin: Evidence of environmental isotope and hydrological investigations 鄂尔多斯盆地跨流域地下水流动:环境同位素和水文调查证据
IF 8.5 1区 地球科学 Q1 GEOSCIENCES, MULTIDISCIPLINARY Pub Date : 2024-11-17 DOI: 10.1016/j.gsf.2024.101967
Yitong Zhang , Jiaqi Chen , Jiansheng Chen , Wang Wang
The Ordos Basin, located in arid and semi-arid region of China, is famous for its abundant groundwater resources and artesian features. The source of groundwater recharge, whether from local precipitation or external sources, has been debated. This study aims to elucidate the groundwater circulation mechanism in the Ordos Basin through scientific expedition, environmental isotope method, and hydrological drilling exploration, providing valuable insights for other artesian basins. Comprehensive analysis indicates that groundwater in the Ordos Basin is recharged by modern precipitation, primarily from high-elevation areas outside the basin. Deep groundwater from these external sources ascends to the aquifer through basement fault zones. Evidence from hydrogen and oxygen isotopes, hydraulic gradients, and water quantities suggests that the Tibetan Plateau is the most potential recharge source. Based on the distribution of Cenozoic basalt and data from seismic observation wells, we propose that leakage water from the Tibetan Plateau rift valley is transported to the Ordos Basin through fast channels, possibly lava tubes, and then upwelling through basement fault zones. This work provides a new perspective on the mechanism of inter-basin groundwater circulation.
鄂尔多斯盆地位于中国干旱半干旱区,以其丰富的地下水资源和自流地貌而闻名。地下水补给的来源是来自当地降水还是外部来源一直存在争议。本研究旨在通过科学考察、环境同位素方法和水文钻探勘探等手段阐明鄂尔多斯盆地地下水循环机制,为其他自流盆地提供有价值的参考。综合分析表明,鄂尔多斯盆地地下水补给主要来自盆地外高海拔地区的现代降水。来自这些外部水源的深层地下水通过基底断裂带上升到含水层。氢、氧同位素、水力梯度和水量的证据表明,青藏高原是最潜在的补给源。根据新生代玄武岩的分布和地震观测井的资料,我们认为青藏高原裂谷的泄漏水通过快速通道(可能是熔岩管)输送到鄂尔多斯盆地,然后通过基底断裂带上涌。本研究为研究流域间地下水循环机制提供了新的视角。
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引用次数: 0
Consistent crystal orientation of core and rim pyrites indicates an epitaxial growth of rim in Carlin-type gold deposits 卡林型金矿岩心与边缘黄铁矿晶体取向一致,表明边缘呈外延生长
IF 8.5 1区 地球科学 Q1 GEOSCIENCES, MULTIDISCIPLINARY Pub Date : 2024-11-17 DOI: 10.1016/j.gsf.2024.101966
Jingdan Xiao , Zhuojun Xie , Yong Xia , Phillip Gopon , Qinping Tan
The gold-bearing arsenian pyrite in Carlin-type gold deposits typically grows around the gold/arsenic-poor pyrite core, forming core–rim textured pyrite. However, the causes of rim pyrite precipitation around the early-formed core pyrite and the growth mechanisms of the rim pyrite remain unclear. Here, we combined scanning electron microscopy, electron probe micro-analysis, and nanoscale secondary ion mass spectrometry to investigate the textural and chemical characteristics of core–rim textured pyrite from the giant Shuiyindong and Lannigou gold deposits. Furthermore, we used electron backscattered diffraction and transmission electron microscopy to characterize their crystallographic structure. The results indicated that core–rim textured pyrite is the dominant pyrite type in the ore. This type of pyrite is characterized by the sharp core–rim interfaces, euhedral-subhedral morphology, and oscillating zoning. The gold/arsenic-rich rim and gold/arsenic-poor core formed during the main-ore and pre-ore stages, respectively. Crystallographically, the rim showed that a crystallographic orientation is similar to that of the core along the (0 1 0) crystal facet, indicating that the core pyrite serves as a template for the epitaxial growth of rim pyrite. Textural and chemical features indicate that the epitaxy occurs in the process of direct precipitation of main-ore pyrite over the pre-ore pyrite. As Carlin ore fluids dissolve the iron-bearing carbonates, iron concentrations in the fluids increase, thereby creating a supersaturation environment suitable for the nucleation of main-ore pyrite. Because the minimal lattice misfit would minimize the surface free energy and the (0 1 0) facet of pyrite has a lower surface energy than other facets, the nucleated pyrite would readily grow along the (0 1 0) facet of preexisting pyrite via epitaxy. Our findings highlight that the widespread preexisting pyrite facilitates late-stage pyrite precipitation. For Carlin-type gold deposits, the pre-ore pyrite is essential owing to its promoting the precipitation of gold-bearing pyrite.
卡林型金矿床含金砷黄铁矿主要生长在贫金贫砷黄铁矿岩心周围,形成芯缘织构黄铁矿。然而,在早期形成的岩心黄铁矿周围形成边缘黄铁矿的原因和边缘黄铁矿的生长机制尚不清楚。结合扫描电镜、电子探针显微分析和纳米级二次离子质谱等方法,研究了水银洞和兰尼沟大型金矿床核缘结构黄铁矿的结构和化学特征。此外,我们利用电子背散射衍射和透射电镜对其晶体结构进行了表征。结果表明,核-环构形黄铁矿为矿石中主要的黄铁矿类型,该类型黄铁矿具有核-环界面尖锐、正面体-亚面体形态和振荡分带的特征。富金/砷边缘和贫金/砷核分别形成于主矿期和成矿前期。在晶体学上,沿(0 ~ 10)晶面,边缘显示出与岩心相似的晶体取向,表明岩心黄铁矿为边缘黄铁矿的外延生长提供了模板。结构和化学特征表明,外延发生在主矿黄铁矿直接沉淀到预矿黄铁矿上的过程中。随着卡林矿流体溶解含铁碳酸盐,流体中的铁浓度增加,形成了适合主矿黄铁矿成核的过饱和环境。由于最小的晶格错配会使表面自由能最小化,而黄铁矿的(0 0 0)面比其他面具有更低的表面能,因此成核的黄铁矿很容易通过外延沿着预先存在的黄铁矿的(0 0 0)面生长。我们的研究结果强调,广泛存在的黄铁矿促进了晚期黄铁矿的沉淀。对于卡林型金矿床,矿前黄铁矿对含金黄铁矿的沉淀起着重要的促进作用。
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引用次数: 0
Magmatic initial and saturated water thresholds determine copper endowments: Insights from apatite F-Cl-OH compositions 岩浆初始水和饱和水阈值决定了铜禀赋:磷灰石F-Cl-OH成分的启示
IF 8.5 1区 地球科学 Q1 GEOSCIENCES, MULTIDISCIPLINARY Pub Date : 2024-11-09 DOI: 10.1016/j.gsf.2024.101962
Yingcai Sun , Qiushi Zhou , Rui Wang , Madeleine C.S. Humphreys
Magmatic volatiles (H2O, F, Cl), especially water, are critical in the formation of porphyry copper deposit, for its significance as a carrier for metals. However, accurately quantifying the water contents of deep ore-forming magma remain a challenge. Here, we used apatite and forward modelling methods to reconstruct magmatic water evolution histories, with special concern on the control of initial magmatic H2O contents and water saturation threshold to porphyry mineralization. Samples investigated include granitoid rocks and apatite from highly copper-mineralized and barren localities. Generally, our research suggested that both ore-related and ore-barren magma systems are hydrous, the modeled magmatic water contents vary significantly among systems whether mineralized or not, and the major difference lies in the threshold of water saturation (6.0 wt.% for barren, and up to 10.0 wt.% for highly mineralized). Combined with whole rock geochemistry data (high K2O and Sr/Y contents) and modeling result (high modeled water thresholds), we think the ore-related magmas are stored at deeper depth with higher water solubility. In conclusion, we propose that the level of magmatic water saturation plays a crucial role in the formation of porphyry copper systems. Fertile magma has higher water solubility to which deeper storage depth is a critical contributing factor, and can get significantly water enriched upon saturation.
岩浆挥发物(H2O、F、Cl),尤其是水,对斑岩铜矿床的形成至关重要,因为它是金属的重要载体。然而,准确量化深部成矿岩浆的含水量仍然是一项挑战。在此,我们采用磷灰石和前向建模方法重建岩浆水演化历史,特别关注岩浆初始 H2O 含量和水饱和阈值对斑岩成矿作用的控制。调查的样本包括花岗岩和来自铜矿化程度高和贫瘠地区的磷灰石。总体而言,我们的研究表明,与矿石有关的岩浆系统和贫矿岩浆系统都是含水岩浆系统,无论是否成矿,不同岩浆系统的模型岩浆含水量都有很大差异,主要区别在于水饱和阈值(贫矿为 6.0 wt.%,高度成矿可达 10.0 wt.%)。结合全岩地球化学数据(K2O 和 Sr/Y 含量高)和建模结果(建模水阈值高),我们认为与矿石有关的岩浆储藏在更深的地方,水溶性更高。总之,我们认为岩浆水饱和度在斑岩铜系统的形成过程中起着至关重要的作用。肥沃岩浆具有较高的水溶性,而较深的储藏深度是一个关键因素,饱和后可显著富水。
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引用次数: 0
Laboratory experiments of carbon mineralization potential of the main terrestrial basalt reservoirs in China 中国主要陆相玄武岩储层碳矿化潜力的实验室实验
IF 8.5 1区 地球科学 Q1 GEOSCIENCES, MULTIDISCIPLINARY Pub Date : 2024-11-07 DOI: 10.1016/j.gsf.2024.101961
Yanning Pan , Yunhua Liu , Zengqian Hou , Qiang Sun , Nianzhi Jiao , Guochen Dong , Jihua Liu , Gaoxue Yang , Huiting Zhang , Hailiang Jia , Hao Huang
Against the background of realizing the goal of “carbon peaking and carbon neutrality”, using basaltic rocks for carbon mineralization is one of the most promising approaches to reduce the rise in atmospheric CO2 concentrations. This study conducted a series of experiments to assess carbon mineralization in nine basalt samples from the main terrestrial basalt reservoirs in China within CO2-H2O/brine-rock systems at low temperatures (≤35 °C). The results indicate that the secondary carbonates formed in the CO2-H2O/brine-basalt system are predominantly calcite rather than Mg-carbonate minerals at low temperatures (≤35 °C). Hence, at low temperatures (≤35 °C), basalt rich in Ca-bearing minerals promotes the formation of stable carbonate minerals more effectively than basalt containing Mg-bearing minerals. Furthermore, under conditions of low temperatures (≤35 °C) and pressures of approximately 3 MPa, the results suggest that alkaline olivine basalt, with a higher content of Ca-minerals and typical alkaline minerals (nepheline and Na-sanidine), exhibits the highest pH value and the highest amount of calcite. Hence, the alkaline minerals, nepheline and Na-sanidine, serve as pH buffers to increase the pH and promote the precipitation of calcite within CO2-H2O– basalt systems at low temperatures (≤35 °C). Among the nine evaluated basalts, basalt from the Shandong Linqu-Changle volcanic basin exhibits the highest rate of carbon mineralization at low temperatures (≤35 °C). Hence, Cenozoic alkaline olivine basalt from Shandong Linqu-Changle volcanic basin is one of the most promising basalt reservoirs in China for future in- situ carbonation. As for ex- situ carbonation, compared with olivine, diopside or Ca-plagioclase may be more appropriate for increasing ocean negative emissions.
在实现 "碳封顶、碳中和 "目标的背景下,利用玄武岩进行碳矿化是降低大气二氧化碳浓度上升的最有前景的方法之一。本研究在低温(≤35 °C)CO2-H2O/卤素岩体系中,对来自中国主要陆相玄武岩储层的九个玄武岩样品进行了一系列碳矿化评估实验。结果表明,在低温(≤35 ℃)条件下,CO2-H2O/卤水-玄武岩体系中形成的次生碳酸盐主要是方解石,而不是碳酸镁矿物。因此,在低温(≤35 °C)条件下,富含含钙矿物的玄武岩比含有含镁矿物的玄武岩更有效地促进稳定碳酸盐矿物的形成。此外,在低温(≤35 °C)和约 3 兆帕的压力条件下,结果表明,碱性橄榄石玄武岩含有较多的钙矿物和典型的碱性矿物(霞石和钠矽烷),显示出最高的 pH 值和最高的方解石含量。因此,碱性矿物(霞石和 Na-sanidine )可作为 pH 缓冲剂,在低温(≤35 °C)条件下提高 CO2-H2O 玄武岩体系的 pH 值,促进方解石的沉淀。在评估的九种玄武岩中,山东临朐昌乐火山盆地的玄武岩在低温(≤35 °C)下的碳矿化率最高。因此,山东临朐-昌乐火山盆地的新生代碱性橄榄岩玄武岩是中国最有希望进行原位碳化的玄武岩储层之一。至于原地碳化,与橄榄石相比,透辉石或钙斜长石可能更适合增加海洋负排放。
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引用次数: 0
Detection of Earth’s free oscillation and analysis of the non-synchronous oscillation phenomenon of normal modes 地球自由振荡的探测和正常模式非同步振荡现象的分析
IF 8.5 1区 地球科学 Q1 GEOSCIENCES, MULTIDISCIPLINARY Pub Date : 2024-11-04 DOI: 10.1016/j.gsf.2024.101957
Yingqi Zhang , Gong Xu , Chenchen Wang , Yaxin Zhao , Zheng Mu , Yunhao Fan , Changwei Jing
Earth’s free oscillation can provide essential constraints for refining Earth models, inverting seismic source mechanisms, and studying the deep internal structure of the Earth. Large earthquakes can simultaneously excite numerous normal modes. Due to the Earth’s ellipticity, rotation, and internal heterogeneities, these normal modes undergo splitting, with the frequencies of singlets of normal modes becoming very close (only a few µHz apart). This imposes greater demands on the detection of normal modes. This paper introduces a novel method for normal mode detection based on the normal time–frequency transform (NTFT). Compared to classical FT spectrum methods and recent optimal sequence estimation (OSE), the proposed method not only detects more weak normal modes but also reveals the spatial distribution of the phase of each normal mode. Taking the detection of 0S2 as an example, the phase measurements of each singlet are spatially inconsistent. This phenomenon can provide prior information for other methods, such as product spectrum analysis (PSA), spherical harmonic stacking (SHS), multistation experiments (MSE), and OSE. Additionally, understanding the phase distribution patterns contributes to further study of geological structures, offering crucial foundational data and observational support.
地球的自由振荡可以为完善地球模型、反演震源机制和研究地球深层内部结构提供重要的约束条件。大地震可以同时激发许多法向模态。由于地球的椭圆性、自转和内部异质性,这些法向模态会发生分裂,法向模态单体的频率会变得非常接近(仅相差几微赫)。这就对法向模的探测提出了更高的要求。本文介绍了一种基于正常时频变换(NTFT)的正常模式检测新方法。与经典的时频变换频谱方法和最新的最优序列估计(OSE)方法相比,本文提出的方法不仅能检测到更多微弱的正常模式,还能揭示每个正常模式相位的空间分布。以 0S2 的检测为例,每个单子的相位测量值在空间上是不一致的。这种现象可以为其他方法提供先验信息,如积谱分析(PSA)、球谐波堆叠(SHS)、多站实验(MSE)和 OSE。此外,了解相位分布模式有助于进一步研究地质结构,提供重要的基础数据和观测支持。
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引用次数: 0
A novel flood conditioning factor based on topography for flood susceptibility modeling 基于地形的洪水调节因子在洪水敏感性模拟中的应用
IF 8.5 1区 地球科学 Q1 GEOSCIENCES, MULTIDISCIPLINARY Pub Date : 2024-11-01 DOI: 10.1016/j.gsf.2024.101960
Jun Liu, Xueqiang Zhao, Yangbo Chen, Huaizhang Sun, Yu Gu, Shichao Xu
Flood is one of the most devastating natural hazards. Employing machine learning models to construct flood susceptibility maps has become a pivotal step for decision-makers in disaster prevention and management. Existing flood conditioning factors inadequately account for regional characteristics of flood in the depiction of topography, potentially leading to an overestimation of flood susceptibility in flat areas. Addressing this gap, this study proposes a novel flood conditioning factor, local convexity factor (LCF), to enhance the accuracy of flood susceptibility modeling. Initially, LCF is computed based on a standard normal Gaussian surface to highlight elevation variations in local terrain. Subsequently, LCF is applied to flood susceptibility modeling using seven machine learning models across four distinct basins. Comparative analysis is conducted between flood susceptibility maps with and without the application of LCF to evaluate its impact on flood susceptibility modeling. The results demonstrate that the proposed LCF can enhance the accuracy of flood susceptibility modeling to varying degrees, across the four basins investigated. The Fujiang basin exhibited the most substantial improvement, with its AUC improved from 0.861 to 0.886, Producer’s Agreement improved from 0.869 to 0.899, and Overall Agreement improved from 0.778 to 0.811. Comparation with hydrodynamic inundation maps shows that particularly in relatively flat terrain areas, flood susceptibility maps incorporating LCF offer more precise delineation between flood-prone and non-flood-prone zones. This research holds potential for widespread application in the prediction of flood susceptibility using machine learning models, providing a novel perspective for enhancing their accuracy.
洪水是最具破坏性的自然灾害之一。利用机器学习模型构建洪水易感度图已成为灾害预防和管理决策者的关键一步。现有的洪水调节因子在描述地形时没有充分考虑洪水的区域特征,可能导致对平坦地区洪水易感性的高估。针对这一不足,本研究提出了一种新的洪水调节因子——局部凸度因子(LCF),以提高洪水敏感性模型的准确性。最初,LCF是基于标准正态高斯曲面计算的,以突出局部地形的高程变化。随后,LCF应用于4个不同流域的7个机器学习模型的洪水敏感性建模。对比分析了应用LCF和未应用LCF的洪水易感性图,评价了其对洪水易感性建模的影响。结果表明,LCF在不同程度上提高了4个流域洪水敏感性模型的精度。富江盆地改善最为明显,AUC由0.861提高到0.886,生产者协议由0.869提高到0.899,总体协议由0.778提高到0.811。与水动力淹没图的比较表明,特别是在相对平坦的地形地区,纳入LCF的洪水易发性图可以更精确地描绘洪水易发区和非洪水易发区。该研究在利用机器学习模型预测洪水易感性方面具有广泛的应用潜力,为提高机器学习模型的准确性提供了一个新的视角。
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引用次数: 0
Fifteen years of Geoscience Frontiers and moving forward 地球科学前沿》十五年及展望
IF 8.5 1区 地球科学 Q1 GEOSCIENCES, MULTIDISCIPLINARY Pub Date : 2024-11-01 DOI: 10.1016/j.gsf.2024.101955
Xuanxue Mo
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引用次数: 0
Analyzing failure mechanisms and predicting step-like displacement: Rainfall and RWL dynamics in lock-unlock landslides 分析破坏机制并预测阶梯状位移:锁定-解锁滑坡中的降雨和 RWL 动力学
IF 8.5 1区 地球科学 Q1 GEOSCIENCES, MULTIDISCIPLINARY Pub Date : 2024-10-30 DOI: 10.1016/j.gsf.2024.101959
Xuekun Xiang , Haijia Wen , Jiafeng Xiao , Xiongfeng Wang , Hongyue Yin , Junhao Huang
Lock-unlock landslides have thick sliding zones that store a lot of energy. This makes them start quickly, happen suddenly, and have serious consequences. Therefore, it becomes urgent to study the deformation and failure mechanisms of such landslides and develop rational predictive models. Taking the Jiuxianping landslide as an example, this study investigates the regularity of landslide displacement changes using multi-source data, focusing on the abrupt displacement patterns in the unlock phase. Furthermore, employing Transient Release and Inhalation Method tests combined with Geo-Studio’s SEEP/W and SIGMA/W modules for fluid–solid coupled simulation calculations, the evolution process of landslide failure mechanisms and deformation characteristics is analyzed and discussed. Lastly, utilizing data mining analysis of multi-source data, a hybrid optimized machine learning predictive model is established for model prediction comparison. The study reveals that: (1) The rise in infiltration line elevates pore water pressure, affecting the stability of the sliding zone, leading to “unlock effects” and step-like displacement deformation; (2) Simulation shows that YY208 is closer to the actual situation, located at the far bank position, while YY210 is greatly influenced by the “buoyancy effect”, resulting in a slowdown in deformation velocity; (3) After data preprocessing, overall actual displacement prediction performs better than simulation displacement prediction in terms of Mean Absolute Error, Mean Squared Error and Correlation Coefficient, but noise reduction processing can improve the periodic prediction effect of simulation displacement.
锁定-解锁型山体滑坡有很厚的滑动带,可以储存大量能量。这使得它们启动迅速,发生突然,后果严重。因此,研究这类滑坡的变形和破坏机理,并建立合理的预测模型已迫在眉睫。本研究以酒仙坪滑坡为例,利用多源数据研究了滑坡位移变化的规律性,重点研究了解锁阶段的突变位移模式。此外,结合 Geo-Studio 的 SEEP/W 和 SIGMA/W 模块进行流固耦合模拟计算,采用瞬态释放和吸入法试验,分析和讨论了滑坡崩塌机理和变形特征的演化过程。最后,利用多源数据的数据挖掘分析,建立了一个混合优化的机器学习预测模型,用于模型预测比较。研究结果表明(1) 渗透线的上升使孔隙水压力升高,影响滑动带的稳定性,导致 "解锁效应 "和阶梯状位移变形;(2) 模拟结果表明,YY208 位于远岸位置,更接近实际情况,而 YY210 受 "浮力效应 "影响较大,导致变形速度减慢;(3) 经过数据预处理后,实际位移预测在平均绝对误差、平均平方误差和相关系数方面均优于模拟位移预测,但降噪处理可改善模拟位移的周期预测效果。
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引用次数: 0
Achieving environmental quality through stringent environmental policies: Comparative evidence from G7 countries by multiple environmental indicators 通过严格的环境政策实现环境质量:七国集团国家多种环境指标的比较证据
IF 8.5 1区 地球科学 Q1 GEOSCIENCES, MULTIDISCIPLINARY Pub Date : 2024-10-29 DOI: 10.1016/j.gsf.2024.101956
Mustafa Tevfik Kartal , Shahriyar Mukhtarov , Dervis Kirikkaleli
Compatible with the increasing public interest on climate change, countries have taken measures to combat climate change and support environmental sustainability. Considering this fact, this study investigates whether environmental measures, proxied by the environmental policy stringency (EPS) index, are efficient in achieving sustainability of environment in G7 countries as the leading economies; uses multiple environmental sustainability indicators, and applies quantile methods from 1991/Q1 to through 2020/Q4. The results show that (i) EPS curbs carbon dioxide emissions in France and the United States across all quantiles. Also, it has a declining effect in Germany and Italy at lower quantiles and in Canada at lower and higher quantiles; (ii) EPS declines ecological footprint in United States across all quantiles, while it curbs in Canada and Germany at lower quantiles as well as in Italy and United Kingdom at higher quantiles; (iii) EPS stimulates load capacity factor in France, United Kingdom, and United States across all quantiles and in Canada at higher quantiles; (iv) causal effect of EPS on the environment varies throughout quantiles; (v) the robustness of the results by quantile regression method is verified. Overall, the results reveal that the effect of EPS on environmental sustainability differentiates across environmental indicators, countries, and quantiles. In ensuring environmental quality, EPS is completely helpful in the United States, fully inefficient in Japan, and has a mixed effect in remaining G7 countries.
随着公众对气候变化的日益关注,各国纷纷采取措施应对气候变化,支持环境的可持续发展。考虑到这一事实,本研究调查了以环境政策严格性指数(EPS)为代表的环境措施是否能有效地实现作为主要经济体的 G7 国家的环境可持续性;研究使用了多个环境可持续性指标,并采用了 1991/Q1 至 2020/Q4 的量化方法。结果表明:(i) EPS 在法国和美国的所有量级都能抑制二氧化碳排放。此外,在德国和意大利,在较低的量值以及加拿大在较低和较高的量值下,EPS 的效果都在下降;(ii) 在美国,EPS 在所有量值下都会减少生态足迹,而在加拿大和德国,在较低的量值以及意大利和英国在较高的量值下,EPS 都会减少生态足迹;(iii) 在法国、英国和美国,EPS 在所有量纲下都会刺激负载能力系数,而在加拿大,EPS 在较高量纲下会刺激负载能力系数;(iv) EPS 对环境的因果效应在不同量纲下各不相同;(v) 量纲回归法验证了结果的稳健性。总体而言,研究结果表明,EPS 对环境可持续性的影响在不同环境指标、不同国家和不同数量级之间存在差异。在确保环境质量方面,美国的 EPS 完全有效,日本的 EPS 完全无效,其余七国集团国家的 EPS 效果参差不齐。
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引用次数: 0
Aerosol spatiotemporal dynamics, source analysis and influence mechanisms over typical drylands 典型旱地上空的气溶胶时空动态、来源分析和影响机制
IF 8.5 1区 地球科学 Q1 GEOSCIENCES, MULTIDISCIPLINARY Pub Date : 2024-10-28 DOI: 10.1016/j.gsf.2024.101958
Yunfei Zhang , Xiangyue Chen , Fengtao Zhao , Qianrou Xia , Hanchen Xing , Mengdi Du
As globally important dust source areas, drylands not only have extremely fragile ecosystems that are exceptionally sensitive to global climate change but also have important implications for global warming and carbon cycling. However, the detailed dryland aerosol characteristics are not clear, especially the influence mechanisms of dryland aerosols, which are poorly understood. In this paper, Utilizing the Xinjiang Uygur Autonomous Region (XJ) as a target area, based on high spatial resolution aerosol optical depth (AOD) data, combined with the trend analysis, backward trajectory, source analysis, and machine learning methods, we systematically analyzed the multiscale dynamic characteristics of aerosols in XJ over a long period. Simultaneously, we also quantitatively explored the source distributions of high aerosols at typical sites at different time scales. Furthermore, we discussed the specific effects of natural and anthropogenic factors on aerosols in XJ and its subregions. The results show that 72.45% of the AOD in XJ presents an increasing trend from 2000 to 2019, 27.56% of which passed the significance test, mainly concentrated in northern Xinjiang (NXJ). The AOD in southern Xinjiang (SXJ) is the largest (0.240 ± 0.154), followed by eastern Xinjiang (EXJ) (0.157 ± 0.038), and the AOD in NXJ is the smallest (0.134 ± 0.028); however, the AOD in NXJ has the most obvious increasing trend, peaking in 2011, and the AOD in XJ remains low and stable at 5000 m elevation and above. The backward trajectory shows that nearly half of the potential paths of high AOD in SXJ are from the Taklamakan Desert, most of the potential paths in NXJ are from transboundary transmission, mostly through exposed lake beds, and most of the potential paths in EXJ are from the northwest, with characteristics similar to those of NXJ. The exposed lake beds provide salt dust, which further exacerbates the complexity and hazards of aerosols in NXJ and EXJ. The potential source areas for AOD in SXJ are concentrated in the northeast of the target site, those in NXJ are concentrated in the west of the target site, and those in EXJ are in the northwest and east. The AOD in SXJ (63.92%) and EXJ (74.83%) or XJ (57.77%) is dominated by natural factors, whereas the magnitude of AOD in NXJ (84.01%) is largely explained by anthropogenic factors.
作为全球重要的尘源地区,旱地不仅生态系统极其脆弱,对全球气候变化异常敏感,而且对全球变暖和碳循环也有重要影响。然而,详细的旱地气溶胶特征并不清楚,尤其是对旱地气溶胶的影响机制知之甚少。本文以新疆维吾尔自治区(XJ)为研究对象,基于高空间分辨率气溶胶光学深度(AOD)数据,结合趋势分析、回溯轨迹、源解析和机器学习等方法,系统分析了XJ地区气溶胶的长期多尺度动态特征。同时,我们还定量探索了不同时间尺度下典型站点的高气溶胶源分布。此外,我们还讨论了自然和人为因素对 XJ 及其子区域气溶胶的具体影响。结果表明,从 2000 年到 2019 年,新疆 72.45%的 AOD 呈上升趋势,其中 27.56%通过了显著性检验,主要集中在北疆(NXJ)。南疆(SXJ)的AOD最大(0.240±0.154),其次是东疆(EXJ)(0.157±0.038),北疆(NXJ)的AOD最小(0.134±0.028);但北疆(NXJ)的AOD上升趋势最明显,在2011年达到峰值,而XJ的AOD在海拔5000米及以上保持低位稳定。后向轨迹显示,SXJ地区近一半的高AOD潜在路径来自塔克拉玛干沙漠,NXJ地区的大部分潜在路径来自跨界传输,主要通过裸露的湖床,EXJ地区的大部分潜在路径来自西北部,其特征与NXJ相似。裸露的湖床提供了盐尘,进一步加剧了 NXJ 和 EXJ 地区气溶胶的复杂性和危害性。SXJ 的 AOD 潜在源区集中在目标地点的东北部,NXJ 的 AOD 潜在源区集中在目标地点的西部,EXJ 的 AOD 潜在源区集中在西北部和东部。SXJ(63.92%)和 EXJ(74.83%)或 XJ(57.77%)的 AOD 主要由自然因素造成,而 NXJ 的 AOD(84.01%)则主要由人为因素造成。
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Geoscience frontiers
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