首页 > 最新文献

Geoscience frontiers最新文献

英文 中文
Do continental lithospheric discontinuities exert control on tectonic plate motion directions? 大陆岩石圈不连续性是否对构造板块运动方向起控制作用?
IF 8.9 1区 地球科学 Q1 GEOSCIENCES, MULTIDISCIPLINARY Pub Date : 2025-09-13 DOI: 10.1016/j.gsf.2025.102154
Yvette D. Kuiper
Plate motion directions, and the orientations of rift zones and oceanic spreading ridges, and of transform faults and fracture zones that are perpendicular to these ridges, are generally controlled by tectonic forces such as slab pull, mantle convection, and mantle plumes. Here, it is hypothesized that within the confines of these general orientations, the exact orientations of these structures, and therefore plate motion directions, are partially controlled by suitably oriented sets of steep continental lithospheric discontinuities (CLDs), which work in concert with these larger tectonic forces.
Previously, the observation has been made that oceanic fracture zones are contiguous with CLDs, such as suture zones and other lithospheric fault zones. Based on high-resolution bathymetry, geological and geophysical data, it is demonstrated here that continents have multiple sets of lineaments parallel to such CLDs, or contiguous with CLDs where they occur farther inland and do not reach the ocean. Published analog experiments suggest that the orientations of transform faults and fracture zones are controlled by these CLDs if the angle between the spreading direction and the CLDs is no more than ∼45°. Spreading ridge segments evolve in an orientation perpendicular to these transform faults and fracture zones, so that the spreading direction becomes parallel to the transform faults and fracture zones. The implication is that the exact plate motion directions are controlled by CLDs, if a set of CLDs is orientated at low angle with the spreading direction. When plate motion directions need to change due to tectonic forces, the new hypothesis predicts that the exact directions may be controlled by a different set of suitably orientated CLDs. During later stages of oceanic spreading, the larger tectonic forces such as slab pull, mantle convection, and mantle plumes become increasingly dominant and plate motion directions may no longer be controlled by the CLDs.
While the hypothesis needs further testing, it has potentially far-reaching implications. For example, Euler pole reconstructions are commonly based on small circle patterns formed by fracture zones and transform faults in the oceanic lithosphere. Oceanic crust older than ∼200 Ma is typically destroyed by subduction, and pre-Mesozoic Euler poles can therefore not be reconstructed based on that method. If the hypothesis presented above is correct, the orientations of CLDs and associated lineament sets may be used as proxies for orientations of past transform faults and fracture zones, at least during early oceanic spreading. The locations of past Euler poles may thus be better estimated based on these CLDs and lineaments, and pre-Mesozoic plate tectonic reconstructions may be much improved in deep geologic time.
板块运动方向、裂谷带和大洋扩张脊以及垂直于这些隆起的转换断层和断裂带的走向,一般受板块拉拔、地幔对流和地幔柱等构造力的控制。在这里,假设在这些一般方向的范围内,这些构造的确切方向,从而板块运动方向,部分地由适当定向的陡峭大陆岩石圈不连续层(CLDs)控制,它们与这些更大的构造力协同工作。在此之前,已经观察到海洋断裂带与cld相邻,如缝合带和其他岩石圈断裂带。基于高分辨率测深、地质和地球物理数据,这里证明了大陆有多组平行于这些叠合带,或与叠合带相邻的叠合带,这些叠合带位于更远的内陆,没有到达海洋。已发表的模拟实验表明,如果扩展方向与断层带之间的夹角不大于45°,则转换断层和断裂带的方向受这些断层带的控制。扩展脊段沿垂直于这些转换断层和断裂带的方向演化,使扩展方向与转换断层和断裂带平行。这意味着,如果一组cld与扩散方向成小角,则确切的板块运动方向由cld控制。当板块运动方向由于构造力而需要改变时,新的假设预测,精确的方向可能由一组不同的合适定向的cld控制。在海洋扩张的后期阶段,较大的构造力如板块拉拔、地幔对流和地幔柱逐渐占主导地位,板块运动方向可能不再受大陆板块的控制。虽然这一假设需要进一步检验,但它具有潜在的深远影响。例如,欧拉极重建通常是基于海洋岩石圈中破裂带和转换断层形成的小圆圈模式。超过~ 200 Ma的海洋地壳通常被俯冲破坏,因此前中生代欧拉极不能基于该方法重建。如果上述假设是正确的,那么至少在早期海洋扩张期间,cld和相关的线集的方向可以作为过去转换断层和断裂带的方向的代表。因此,根据这些叠合带和构造线可以更好地估计过去欧拉极的位置,并且可以在深部地质时期大大改善前中生代板块构造的重建。
{"title":"Do continental lithospheric discontinuities exert control on tectonic plate motion directions?","authors":"Yvette D. Kuiper","doi":"10.1016/j.gsf.2025.102154","DOIUrl":"10.1016/j.gsf.2025.102154","url":null,"abstract":"<div><div>Plate motion directions, and the orientations of rift zones and oceanic spreading ridges, and of transform faults and fracture zones that are perpendicular to these ridges, are generally controlled by tectonic forces such as slab pull, mantle convection, and mantle plumes. Here, it is hypothesized that within the confines of these general orientations, the exact orientations of these structures, and therefore plate motion directions, are partially controlled by suitably oriented sets of steep continental lithospheric discontinuities (CLDs), which work in concert with these larger tectonic forces.</div><div>Previously, the observation has been made that oceanic fracture zones are contiguous with CLDs, such as suture zones and other lithospheric fault zones. Based on high-resolution bathymetry, geological and geophysical data, it is demonstrated here that continents have multiple sets of lineaments parallel to such CLDs, or contiguous with CLDs where they occur farther inland and do not reach the ocean. Published analog experiments suggest that the orientations of transform faults and fracture zones are controlled by these CLDs if the angle between the spreading direction and the CLDs is no more than ∼45°. Spreading ridge segments evolve in an orientation perpendicular to these transform faults and fracture zones, so that the spreading direction becomes parallel to the transform faults and fracture zones. The implication is that the exact plate motion directions are controlled by CLDs, if a set of CLDs is orientated at low angle with the spreading direction. When plate motion directions need to change due to tectonic forces, the new hypothesis predicts that the exact directions may be controlled by a different set of suitably orientated CLDs. During later stages of oceanic spreading, the larger tectonic forces such as slab pull, mantle convection, and mantle plumes become increasingly dominant and plate motion directions may no longer be controlled by the CLDs.</div><div>While the hypothesis needs further testing, it has potentially far-reaching implications. For example, Euler pole reconstructions are commonly based on small circle patterns formed by fracture zones and transform faults in the oceanic lithosphere. Oceanic crust older than ∼200 Ma is typically destroyed by subduction, and pre-Mesozoic Euler poles can therefore not be reconstructed based on that method. If the hypothesis presented above is correct, the orientations of CLDs and associated lineament sets may be used as proxies for orientations of past transform faults and fracture zones, at least during early oceanic spreading. The locations of past Euler poles may thus be better estimated based on these CLDs and lineaments, and pre-Mesozoic plate tectonic reconstructions may be much improved in deep geologic time.</div></div>","PeriodicalId":12711,"journal":{"name":"Geoscience frontiers","volume":"16 6","pages":"Article 102154"},"PeriodicalIF":8.9,"publicationDate":"2025-09-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145105117","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"地球科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
The H2 generation mechanisms of natural gas in the Sulige gas field, Ordos Basin, China 鄂尔多斯盆地苏里格气田天然气生氢机理
IF 8.9 1区 地球科学 Q1 GEOSCIENCES, MULTIDISCIPLINARY Pub Date : 2025-09-12 DOI: 10.1016/j.gsf.2025.102153
Panpan Zhang , Zhijun Jin , Xiaomei Wang , Kun He , Zhenguang Shang , Jinhao Guo , Xuan Tang , Runchao Liu , Runze Cui , Qitu Hu
Due to its renewability, zero-emissions, and low production cost, natural hydrogen (H2) holds considerable potential as a carbon-free energy resource and represents a key focus for enabling energy transition and achieving carbon neutrality. The generation mechanisms and accumulation patterns of H2 need further investigation, particularly with regard to the sources of H2 in sedimentary basin. This knowledge gap hinders the exploration and development of H2 resources. The study reports the concentrations and isotopic compositions of H2 and hydrocarbons of natural gas in the Sulige gas field. The results suggest that the H2 content in natural gas can reach up to 22.98 %, with H2 isotope values (δ2H-H2) ranging from −809‰ to −700‰. Based on comprehensive analysis of carbon and hydrogen isotopes of hydrocarbons, geological conditions, and hydrogen isotope fractionation mechanisms of H2, this study reveals that the H2 in the Upper Paleozoic natural gas is likely derived primarily from organic matter pyrolysis in coal-bearing source rocks, while the H2 in the Lower Paleozoic natural gas is probably generated mainly through water radiolytic in basement granite and metamorphic rocks. The diffusion fractionation model demonstrates that significant isotopic fractionation occurs during the migration of deep-sourced H2 to sedimentary reservoirs, resulting in notably depleted δ2H-H2 values in the Lower Paleozoic natural gas. The H2 generation through organic matter pyrolysis primarily occurs during the late gas generation stage, with peak production concentrated in the Late Triassic to Early Cretaceous periods. Given the genetic correlation between H2 and hydrocarbons, the H2 may accumulate with natural gas in reservoirs. In contrast, H2 generation through water radiolysis in the study area exhibits multi-source characteristics and prolonged duration, demonstrating significant potential for independent accumulation. This study not only elucidates the generation mechanisms of H2 but also provides a significant geological case study for understanding the distribution characteristics and resource potential of H2 in sedimentary basins.
由于其可再生、零排放和低生产成本,天然氢(H2)作为一种无碳能源具有相当大的潜力,是实现能源转型和实现碳中和的关键焦点。H2的生成机制和富集模式有待进一步研究,特别是沉积盆地H2的来源问题。这种知识差距阻碍了H2资源的勘探和开发。研究报告了苏里格气田天然气中H2和碳氢化合物的浓度和同位素组成。结果表明,天然气中H2含量可达22.98%,H2同位素值(δ2H-H2)在−809‰~−700‰之间。综合分析烃类碳、氢同位素、地质条件和氢同位素分馏机理,认为上古生界天然气中的H2可能主要来源于含煤烃源岩中的有机质热解,而下古生界天然气中的H2可能主要来源于基底花岗岩和变质岩中的水辐射裂解。扩散分馏模型表明,深源H2向沉积储层运移过程中发生了明显的同位素分馏,导致下古生界天然气δ2H-H2值明显下降。有机质热解制氢主要发生在晚期生气阶段,高峰期集中在晚三叠世至早白垩世。考虑到H2与烃类的成因相关性,H2可能随天然气在储层中聚集。研究区水溶制氢具有多源、持续时间长的特点,具有较大的独立富集潜力。该研究不仅阐明了H2的生成机制,而且为了解沉积盆地H2的分布特征和资源潜力提供了重要的地质实例研究。
{"title":"The H2 generation mechanisms of natural gas in the Sulige gas field, Ordos Basin, China","authors":"Panpan Zhang ,&nbsp;Zhijun Jin ,&nbsp;Xiaomei Wang ,&nbsp;Kun He ,&nbsp;Zhenguang Shang ,&nbsp;Jinhao Guo ,&nbsp;Xuan Tang ,&nbsp;Runchao Liu ,&nbsp;Runze Cui ,&nbsp;Qitu Hu","doi":"10.1016/j.gsf.2025.102153","DOIUrl":"10.1016/j.gsf.2025.102153","url":null,"abstract":"<div><div>Due to its renewability, zero-emissions, and low production cost, natural hydrogen (H<sub>2</sub>) holds considerable potential as a carbon-free energy resource and represents a key focus for enabling energy transition and achieving carbon neutrality. The generation mechanisms and accumulation patterns of H<sub>2</sub> need further investigation, particularly with regard to the sources of H<sub>2</sub> in sedimentary basin. This knowledge gap hinders the exploration and development of H<sub>2</sub> resources. The study reports the concentrations and isotopic compositions of H<sub>2</sub> and hydrocarbons of natural gas in the Sulige gas field. The results suggest that the H<sub>2</sub> content in natural gas can reach up to 22.98 %, with H<sub>2</sub> isotope values (<em>δ</em><sup>2</sup>H-H<sub>2</sub>) ranging from −809‰ to −700‰. Based on comprehensive analysis of carbon and hydrogen isotopes of hydrocarbons, geological conditions, and hydrogen isotope fractionation mechanisms of H<sub>2</sub>, this study reveals that the H<sub>2</sub> in the Upper Paleozoic natural gas is likely derived primarily from organic matter pyrolysis in coal-bearing source rocks, while the H<sub>2</sub> in the Lower Paleozoic natural gas is probably generated mainly through water radiolytic in basement granite and metamorphic rocks. The diffusion fractionation model demonstrates that significant isotopic fractionation occurs during the migration of deep-sourced H<sub>2</sub> to sedimentary reservoirs, resulting in notably depleted <em>δ</em><sup>2</sup>H-H<sub>2</sub> values in the Lower Paleozoic natural gas. The H<sub>2</sub> generation through organic matter pyrolysis primarily occurs during the late gas generation stage, with peak production concentrated in the Late Triassic to Early Cretaceous periods. Given the genetic correlation between H<sub>2</sub> and hydrocarbons, the H<sub>2</sub> may accumulate with natural gas in reservoirs. In contrast, H<sub>2</sub> generation through water radiolysis in the study area exhibits multi-source characteristics and prolonged duration, demonstrating significant potential for independent accumulation. This study not only elucidates the generation mechanisms of H<sub>2</sub> but also provides a significant geological case study for understanding the distribution characteristics and resource potential of H<sub>2</sub> in sedimentary basins.</div></div>","PeriodicalId":12711,"journal":{"name":"Geoscience frontiers","volume":"16 6","pages":"Article 102153"},"PeriodicalIF":8.9,"publicationDate":"2025-09-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145266545","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"地球科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Causal mechanisms and governance priorities of the SDG-based resource-economy-environment nexus in the human-nature system 人-自然系统中基于可持续发展目标的资源-经济-环境关系的因果机制与治理重点
IF 8.9 1区 地球科学 Q1 GEOSCIENCES, MULTIDISCIPLINARY Pub Date : 2025-09-10 DOI: 10.1016/j.gsf.2025.102152
Yizhong Huan , Pengpeng Mo , Yiming Su , Xiaoyun Li , Yazhu Wang , Yali Tong , Tao Liang , Lingqing Wang , Jian Hu , Guangjin Zhou
The eight Sustainable Development Goals (SDGs) related to resources (2, 6, 7), economy (8, 9), and environment (12, 13, 15), collectively known as REE, form the core of the human-nature system. Understanding their complex interactions is crucial for identifying transformative and effective governance actions. However, the causal mechanisms underlying the REE-related SDGs remain elusive. We used expert elicitation to assess weighted, directed interactions among 69 targets of these SDGs and applied network analysis and machine learning to identify their higher-order impacts, capacity to maintain network robustness, community structures, similarities, and systemic and structural roles. Additionally, we used causal emergence analysis and link prediction to examine potential characteristics of the causal network at macro and micro scales, respectively. The results indicate that prioritizing target 9.4 (sustainable & clean industries) can accelerate overall SDG progress while enhancing synergies and maintaining systemic resilience. In the macro-network, where causal emergence occurs, macronode E dominated by ecological targets plays the strongest facilitating role. In the micro-network, four predicted links with the highest weights indicate that strengthening scientific research and technological innovation is expected to be a potential focal point for positive impact. However, its possible negative effects warrant careful consideration. Additionally, significant trade-offs may arise between energy development and species conservation in the REE nexus that should be avoided. This study offers new insights into the causal mechanisms and priorities of the SDGs in REE, promoting global human-nature system coupling and accelerating the achievement of the 2030 Agenda.
与资源(2、6、7)、经济(8、9)和环境(12、13、15)相关的八个可持续发展目标(sdg),统称为REE,构成了人与自然系统的核心。理解它们之间复杂的相互作用对于确定变革性和有效的治理行动至关重要。然而,与环保相关的可持续发展目标背后的因果机制仍然难以捉摸。我们使用专家启发法来评估这些可持续发展目标的69个目标之间的加权、定向相互作用,并应用网络分析和机器学习来确定它们的高阶影响、维持网络稳健性的能力、社区结构、相似性以及系统和结构角色。此外,我们使用因果出现分析和链接预测分别在宏观和微观尺度上研究因果网络的潜在特征。结果表明,优先考虑目标9.4(可持续清洁产业)可以加速可持续发展目标的整体进展,同时增强协同效应并保持系统弹性。在发生因果发生的宏观网络中,以生态目标为主导的宏观节点E的促进作用最强。在微网络中,权重最高的四个预测环节表明,加强科学研究和技术创新有望成为积极影响的潜在焦点。然而,它可能产生的负面影响值得仔细考虑。此外,在稀土资源关系中,能源开发和物种保护之间可能会产生重大的权衡,这是应该避免的。该研究为可持续发展目标在REE中的因果机制和优先事项提供了新的见解,促进了全球人-自然系统的耦合,加速了2030年议程的实现。
{"title":"Causal mechanisms and governance priorities of the SDG-based resource-economy-environment nexus in the human-nature system","authors":"Yizhong Huan ,&nbsp;Pengpeng Mo ,&nbsp;Yiming Su ,&nbsp;Xiaoyun Li ,&nbsp;Yazhu Wang ,&nbsp;Yali Tong ,&nbsp;Tao Liang ,&nbsp;Lingqing Wang ,&nbsp;Jian Hu ,&nbsp;Guangjin Zhou","doi":"10.1016/j.gsf.2025.102152","DOIUrl":"10.1016/j.gsf.2025.102152","url":null,"abstract":"<div><div>The eight Sustainable Development Goals (SDGs) related to resources (2, 6, 7), economy (8, 9), and environment (12, 13, 15), collectively known as REE, form the core of the human-nature system. Understanding their complex interactions is crucial for identifying transformative and effective governance actions. However, the causal mechanisms underlying the REE-related SDGs remain elusive. We used expert elicitation to assess weighted, directed interactions among 69 targets of these SDGs and applied network analysis and machine learning to identify their higher-order impacts, capacity to maintain network robustness, community structures, similarities, and systemic and structural roles. Additionally, we used causal emergence analysis and link prediction to examine potential characteristics of the causal network at macro and micro scales, respectively. The results indicate that prioritizing target 9.4 (sustainable &amp; clean industries) can accelerate overall SDG progress while enhancing synergies and maintaining systemic resilience. In the macro-network, where causal emergence occurs, macronode E dominated by ecological targets plays the strongest facilitating role. In the micro-network, four predicted links with the highest weights indicate that strengthening scientific research and technological innovation is expected to be a potential focal point for positive impact. However, its possible negative effects warrant careful consideration. Additionally, significant trade-offs may arise between energy development and species conservation in the REE nexus that should be avoided. This study offers new insights into the causal mechanisms and priorities of the SDGs in REE, promoting global human-nature system coupling and accelerating the achievement of the 2030 Agenda.</div></div>","PeriodicalId":12711,"journal":{"name":"Geoscience frontiers","volume":"16 6","pages":"Article 102152"},"PeriodicalIF":8.9,"publicationDate":"2025-09-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145105585","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"地球科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Characteristics and drivers of carbonaceous aerosol pollution in a coastal city of northern China 中国北方沿海城市碳质气溶胶污染特征及其驱动因素
IF 8.9 1区 地球科学 Q1 GEOSCIENCES, MULTIDISCIPLINARY Pub Date : 2025-09-09 DOI: 10.1016/j.gsf.2025.102151
Li Fang , He Meng , Yanjun Yang , Ruiyu Li , Yang Yue , Caiqing Yan
Carbonaceous aerosols significantly impact air quality, human health and climate change, yet their concentration levels and influencing factors exhibit significant regional variability. This study examined the concentration levels and temporal variations of carbonaceous aerosols in Qingdao, a typical coastal city in China, using a year-long, high-time-resolution dataset of organic carbon (OC) and elemental carbon (EC) measurements. The impacts of meteorological conditions, primary emissions, atmospheric oxidants, and sea-land breezes were systematically analyzed by employing an interpretable machine learning model. The results revealed that atmospheric OC and EC concentration levels were relatively low in Qingdao, but secondary organic carbon (SOC) accounted for 43 % of OC, emphasizing the substantial influence of secondary sources. SOC concentrations peaked in the evening, whereas primary organic carbon (POC) and EC concentrations peaked during morning rush hours. The elevated carbonaceous aerosol concentration observed in winter likely resulted from enhanced primary emissions coupled with unfavorable dispersion conditions, whereas intensive photochemical activities during summer facilitated SOC formation. Higher SOC levels were observed during sea-land breeze days than non-sea-land breeze days. The machine learning model indicated that atmospheric oxidants played an important role in SOC formation during sea-land breeze days, while combustion related emissions may be the key factor on non-sea-land breeze days. Furthermore, SOC levels were higher under land breezes compared to sea breezes, likely due to enhanced primary emissions from terrestrial sources coupled with confined pollutant dispersion. These findings revealed complex emission-meteorology-chemistry interactions affecting coastal air quality, informing targeted air pollution mitigation strategies.
碳质气溶胶显著影响空气质量、人类健康和气候变化,但其浓度水平和影响因子表现出显著的区域差异。本研究利用为期一年的高时间分辨率有机碳(OC)和元素碳(EC)测量数据,研究了中国典型沿海城市青岛含碳气溶胶的浓度水平和时间变化。通过采用可解释的机器学习模型,系统地分析了气象条件、一次排放、大气氧化剂和海风的影响。结果表明,青岛市大气OC和EC浓度水平相对较低,但二次有机碳(SOC)占OC的43%,表明二次源对OC的影响较大。有机碳(SOC)浓度在傍晚达到峰值,而原生有机碳(POC)和有机碳(EC)浓度在早高峰时段达到峰值。冬季观测到的碳质气溶胶浓度升高可能是由于一次排放增加加上不利的扩散条件,而夏季强烈的光化学活动促进了有机碳的形成。海陆风日土壤有机碳含量高于非海陆风日。机器学习模型表明,大气氧化剂在海陆风日对有机碳形成起重要作用,而燃烧相关排放可能是非海陆风日的关键因素。此外,与海风相比,陆风下的有机碳水平更高,这可能是由于陆地源的一次排放增加,加上污染物扩散受限。这些发现揭示了影响沿海空气质量的复杂的排放-气象-化学相互作用,为有针对性的空气污染缓解策略提供了信息。
{"title":"Characteristics and drivers of carbonaceous aerosol pollution in a coastal city of northern China","authors":"Li Fang ,&nbsp;He Meng ,&nbsp;Yanjun Yang ,&nbsp;Ruiyu Li ,&nbsp;Yang Yue ,&nbsp;Caiqing Yan","doi":"10.1016/j.gsf.2025.102151","DOIUrl":"10.1016/j.gsf.2025.102151","url":null,"abstract":"<div><div>Carbonaceous aerosols significantly impact air quality, human health and climate change, yet their concentration levels and influencing factors exhibit significant regional variability. This study examined the concentration levels and temporal variations of carbonaceous aerosols in Qingdao, a typical coastal city in China, using a year-long, high-time-resolution dataset of organic carbon (OC) and elemental carbon (EC) measurements. The impacts of meteorological conditions, primary emissions, atmospheric oxidants, and sea-land breezes were systematically analyzed by employing an interpretable machine learning model. The results revealed that atmospheric OC and EC concentration levels were relatively low in Qingdao, but secondary organic carbon (SOC) accounted for 43 % of OC, emphasizing the substantial influence of secondary sources. SOC concentrations peaked in the evening, whereas primary organic carbon (POC) and EC concentrations peaked during morning rush hours. The elevated carbonaceous aerosol concentration observed in winter likely resulted from enhanced primary emissions coupled with unfavorable dispersion conditions, whereas intensive photochemical activities during summer facilitated SOC formation. Higher SOC levels were observed during sea-land breeze days than non-sea-land breeze days. The machine learning model indicated that atmospheric oxidants played an important role in SOC formation during sea-land breeze days, while combustion related emissions may be the key factor on non-sea-land breeze days. Furthermore, SOC levels were higher under land breezes compared to sea breezes, likely due to enhanced primary emissions from terrestrial sources coupled with confined pollutant dispersion. These findings revealed complex emission-meteorology-chemistry interactions affecting coastal air quality, informing targeted air pollution mitigation strategies.</div></div>","PeriodicalId":12711,"journal":{"name":"Geoscience frontiers","volume":"16 6","pages":"Article 102151"},"PeriodicalIF":8.9,"publicationDate":"2025-09-09","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145105640","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"地球科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Lacustrine organic carbon burial dynamics regulate Aptian-Albian greenhouse-cooling climate oscillations 湖相有机碳埋藏动力学调节阿普梯—阿普梯—阿普梯温室降温气候振荡
IF 8.9 1区 地球科学 Q1 GEOSCIENCES, MULTIDISCIPLINARY Pub Date : 2025-09-09 DOI: 10.1016/j.gsf.2025.102150
Dongjun Song , Yifeng Hong , Jingyu Zhang , Xinnan Fang , Shuang Dai
Investigating terrestrial response to typical greenhouse periods is essential to understand past and present climate-carbon-cycle interactions. The Cretaceous climate transition is thought to be related to carbon cycles, yet the role of lacustrine systems in modulating global carbon-climate feedback remains poorly constrained. Here, we present a high-resolution biogeochemical record from an Aptian-Albian paleolake in northwestern China, integrating biomarkers, nitrogen isotopes, and elemental proxies. We reveal that warm-humid climates during the early Aptian amplified lacustrine organic carbon burial via intensified denitrification, methane cycling, and nutrient fluxes, potentially reinforcing oceanic anoxic event 1a (OAE1a) hyperthermal conditions through N2O/CH4 emissions. Subsequent nitrogen limitation triggered cyanobacterial dominance, sustaining carbon sequestration under moderate weathering and contributing to cooling the late Aptian climate. A transient early Albian warming phase shifted the nitrogen pool towards NH4+ and favored the bloom of eukaryotic algae, aligning with global OAE1b carbon burial and serving as one of the contributors to the late early Albian cooling climate. These dynamics demonstrate that paleolakes acted as both carbon sinks and greenhouse gas sources, exerting a critical but previously overlooked feedback on Cretaceous climate oscillations. Our findings highlight the dual role of lacustrine systems in past carbon cycle perturbations, offering insights for refining the relationships between the carbon cycle and climate changes in the Cretaceous.
研究陆地对典型温室期的响应对于理解过去和现在的气候-碳循环相互作用至关重要。白垩纪的气候转变被认为与碳循环有关,但湖泊系统在调节全球碳-气候反馈中的作用仍然很少受到限制。本文采用高分辨率的生物地球化学记录,综合了生物标志物、氮同位素和元素指标。研究发现,阿普梯早期的暖湿气候通过强化反硝化作用、甲烷循环和养分通量放大了湖泊有机碳埋藏,并可能通过N2O/CH4排放强化海洋缺氧事件1a (OAE1a)过热条件。随后的氮限制引发了蓝藻的优势,维持了适度风化下的碳固存,并有助于冷却阿普tian晚期的气候。早期Albian短暂的变暖阶段使氮池向NH4+方向转变,有利于真核藻类的繁殖,与全球OAE1b碳埋藏一致,是早期Albian晚期降温气候的原因之一。这些动态表明,古湖泊既是碳汇又是温室气体源,在白垩纪气候振荡中发挥了重要但以前被忽视的反馈作用。我们的发现强调了湖泊系统在过去碳循环扰动中的双重作用,为完善白垩纪碳循环与气候变化之间的关系提供了见解。
{"title":"Lacustrine organic carbon burial dynamics regulate Aptian-Albian greenhouse-cooling climate oscillations","authors":"Dongjun Song ,&nbsp;Yifeng Hong ,&nbsp;Jingyu Zhang ,&nbsp;Xinnan Fang ,&nbsp;Shuang Dai","doi":"10.1016/j.gsf.2025.102150","DOIUrl":"10.1016/j.gsf.2025.102150","url":null,"abstract":"<div><div>Investigating terrestrial response to typical greenhouse periods is essential to understand past and present climate-carbon-cycle interactions. The Cretaceous climate transition is thought to be related to carbon cycles, yet the role of lacustrine systems in modulating global carbon-climate feedback remains poorly constrained. Here, we present a high-resolution biogeochemical record from an Aptian-Albian paleolake in northwestern China, integrating biomarkers, nitrogen isotopes, and elemental proxies. We reveal that warm-humid climates during the early Aptian amplified lacustrine organic carbon burial via intensified denitrification, methane cycling, and nutrient fluxes, potentially reinforcing oceanic anoxic event 1a (OAE1a) hyperthermal conditions through N<sub>2</sub>O/CH<sub>4</sub> emissions. Subsequent nitrogen limitation triggered cyanobacterial dominance, sustaining carbon sequestration under moderate weathering and contributing to cooling the late Aptian climate. A transient early Albian warming phase shifted the nitrogen pool towards NH<sub>4</sub><sup>+</sup> and favored the bloom of eukaryotic algae, aligning with global OAE1b carbon burial and serving as one of the contributors to the late early Albian cooling climate. These dynamics demonstrate that paleolakes acted as both carbon sinks and greenhouse gas sources, exerting a critical but previously overlooked feedback on Cretaceous climate oscillations. Our findings highlight the dual role of lacustrine systems in past carbon cycle perturbations, offering insights for refining the relationships between the carbon cycle and climate changes in the Cretaceous.</div></div>","PeriodicalId":12711,"journal":{"name":"Geoscience frontiers","volume":"16 6","pages":"Article 102150"},"PeriodicalIF":8.9,"publicationDate":"2025-09-09","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145105642","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"地球科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Shale oil occurrence and mobility mechanisms in brittle mineral-enriched reservoirs: Insights from the Paleogene Kongdian Formation, Bohai Bay Basin 渤海湾盆地古近系孔店组页岩油赋存状态及运移机制
IF 8.9 1区 地球科学 Q1 GEOSCIENCES, MULTIDISCIPLINARY Pub Date : 2025-09-06 DOI: 10.1016/j.gsf.2025.102149
Bixiao Xin , Fang Hao , Jinqiang Tian , Pengfei Guo , Qilu Xu , Wenzhong Han
Understanding shale oil occurrence and mobility is essential for evaluating resource potential and optimizing exploration in lacustrine shale systems. This study investigates the Paleogene Kongdian Formation in the Bohai Bay Basin, integrating organic geochemistry, mineralogical analysis, scanning electron microscopy, solvent extraction, multi-step Rock-Eval pyrolysis, and 2-D NMR to characterize shale oil occurrence states and mobility mechanisms in brittle mineral-enriched reservoirs. Results indicate that shale oil mainly occurs in free and adsorbed states within interparticle pores, dissolution pores, microfractures, and organic pores, with most retained oil hosted in nanopores smaller than 200 nm. Quantitative analyses show that siliceous and calcareous shales possess higher movable oil ratios than clay-rich counterparts, primarily due to their rigid mineral frameworks that resist compaction and preserve interparticle and intragranular pores. These brittle-rich lithofacies exhibit broader pore size distributions, enhanced connectivity, and reduced adsorption affinity, facilitating more efficient oil accumulation and displacement. In contrast, micropore-dominated, clay-rich shales exhibit strong adsorption and limited pore continuity, which hinder hydrocarbon mobility. Appropriate TOC levels (2.0–4.5 wt.%) favor shale oil mobility, while excessive organic content increases adsorption, reducing the proportion of free oil.
Among various geological factors, brittle mineral content and thermal maturity play the dominant roles in controlling shale oil mobility, as they fundamentally shape pore structure and fluid properties. In combination with organic matter abundance and sedimentary features, these factors jointly govern pore network evolution and hydrocarbon occurrence states, thereby determining shale oil enrichment and extractability. These findings enhance the understanding of shale oil enrichment processes and provide a scientific basis for identifying sweet spots and optimizing development strategies in lacustrine shale reservoirs.
了解页岩油的赋存状态和活动性对于评价湖相页岩系统的资源潜力和优化勘探至关重要。以渤海湾盆地古近系孔店组为研究对象,综合运用有机地球化学、矿物学分析、扫描电镜、溶剂萃取、多步岩石热解、二维核磁共振等方法,对脆性富矿储层页岩油赋存状态及运移机制进行了表征。结果表明,页岩油主要以颗粒间孔隙、溶蚀孔隙、微裂缝和有机孔隙中的游离态和吸附态赋存,大部分滞留在小于200 nm的纳米孔中。定量分析表明,硅质和钙质页岩比富含粘土的页岩具有更高的可动油比,这主要是因为它们具有坚硬的矿物框架,可以抵抗压实作用,并保留颗粒间和粒内孔隙。这些富含脆性的岩相具有更宽的孔径分布、更强的连通性和更低的吸附亲和力,有利于更有效的油气聚集和驱油。而以微孔为主、富含粘土的页岩则表现出较强的吸附作用和有限的孔隙连续性,阻碍了油气的运移。适当的TOC含量(2.0-4.5 wt.%)有利于页岩油的流动性,而过高的有机含量会增加吸附,降低游离油的比例。在各种地质因素中,脆性矿物含量和热成熟度对页岩油运移起主导作用,它们从根本上决定了孔隙结构和流体性质。这些因素结合有机质丰度和沉积特征,共同控制孔隙网络演化和油气赋存状态,从而决定页岩油的富集和可采性。这些研究结果增强了对页岩油富集过程的认识,为识别湖相页岩储层甜点和优化开发策略提供了科学依据。
{"title":"Shale oil occurrence and mobility mechanisms in brittle mineral-enriched reservoirs: Insights from the Paleogene Kongdian Formation, Bohai Bay Basin","authors":"Bixiao Xin ,&nbsp;Fang Hao ,&nbsp;Jinqiang Tian ,&nbsp;Pengfei Guo ,&nbsp;Qilu Xu ,&nbsp;Wenzhong Han","doi":"10.1016/j.gsf.2025.102149","DOIUrl":"10.1016/j.gsf.2025.102149","url":null,"abstract":"<div><div>Understanding shale oil occurrence and mobility is essential for evaluating resource potential and optimizing exploration in lacustrine shale systems. This study investigates the Paleogene Kongdian Formation in the Bohai Bay Basin, integrating organic geochemistry, mineralogical analysis, scanning electron microscopy, solvent extraction, multi-step Rock-Eval pyrolysis, and 2-D NMR to characterize shale oil occurrence states and mobility mechanisms in brittle mineral-enriched reservoirs. Results indicate that shale oil mainly occurs in free and adsorbed states within interparticle pores, dissolution pores, microfractures, and organic pores, with most retained oil hosted in nanopores smaller than 200 nm. Quantitative analyses show that siliceous and calcareous shales possess higher movable oil ratios than clay-rich counterparts, primarily due to their rigid mineral frameworks that resist compaction and preserve interparticle and intragranular pores. These brittle-rich lithofacies exhibit broader pore size distributions, enhanced connectivity, and reduced adsorption affinity, facilitating more efficient oil accumulation and displacement. In contrast, micropore-dominated, clay-rich shales exhibit strong adsorption and limited pore continuity, which hinder hydrocarbon mobility. Appropriate TOC levels (2.0–4.5 wt.%) favor shale oil mobility, while excessive organic content increases adsorption, reducing the proportion of free oil.</div><div>Among various geological factors, brittle mineral content and thermal maturity play the dominant roles in controlling shale oil mobility, as they fundamentally shape pore structure and fluid properties. In combination with organic matter abundance and sedimentary features, these factors jointly govern pore network evolution and hydrocarbon occurrence states, thereby determining shale oil enrichment and extractability. These findings enhance the understanding of shale oil enrichment processes and provide a scientific basis for identifying sweet spots and optimizing development strategies in lacustrine shale reservoirs.</div></div>","PeriodicalId":12711,"journal":{"name":"Geoscience frontiers","volume":"16 6","pages":"Article 102149"},"PeriodicalIF":8.9,"publicationDate":"2025-09-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145154544","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"地球科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Present-day temperature and pressure fields in key areas of Northeast China: Implications for unconventional resource evaluation 东北重点地区现今温度和压力场:对非常规资源评价的启示
IF 8.9 1区 地球科学 Q1 GEOSCIENCES, MULTIDISCIPLINARY Pub Date : 2025-09-04 DOI: 10.1016/j.gsf.2025.102148
Yue Huang , Jian Chang , Nansheng Qiu , Nobuo Maeda
The temperature-pressure fields within hydrocarbon-bearing basins are key geological factors controlling hydrocarbon generation, migration, and accumulation. In this study, we focus on the Qingshankou Formation in the northern part of the central depression of the Songliao Basin, China. A multi-parameter weighted evaluation model was created using present temperature-pressure field characteristics, with formation temperature-pressure as core variables, to evaluate shale oil resource potential. In addition, we explored the control mechanisms of temperature-pressure evolution during geological history on shale oil accumulation and further assessed the applicability of the proposed method. Our results show that the geothermal gradient of the Qingshankou Formation decreases from Member 1 to Member 3 (3.84 °C/100 m, 2.93 °C/100 m, and 2.49 °C/100 m, respectively). High-temperature zones are widely distributed in the Gulong sag, with the average temperature of the Gulong shale exceeding 95 °C and reaching an average of approximately 115 °C. Overpressure in the Qingshankou Formation exhibits a west-high to east-low trend. The overpressure zones of the Gulong shale are mainly concentrated in the Qijia-Gulong and Sanzhao sag, with average pressure coefficients of 1.52 and 1.36, respectively. The Opc model identified Class I and II favorable zones, mainly located in the central and southern parts of the Gulong Sag, as well as the central and southwestern Sanzhao Sag, with estimated shale oil resources of 7.1×108 tons and 17.2×108 tons, respectively. Evolutionary profiles from representative wells indicate that elevated temperatures enhance organic matter maturation and light oil generation, improving shale oil mobility, while overpressure suppresses hydrocarbon dissipation and provides a sufficient driving force for oil production. This study demonstrates that present-day temperature-pressure fields effectively reflect the evolution trends of paleo-thermal and pressure regimes. The proposed evaluation method shows strong applicability and scalability, offering a new technical framework and theoretical foundation for the exploration of unconventional hydrocarbon resources.
含油气盆地内的温压场是控制油气生、运、聚的关键地质因素。本文以松辽盆地中央坳陷北部青山口组为研究对象。以地层温度压力为核心变量,利用当前油气场特征,建立多参数加权评价模型,对页岩油资源潜力进行评价。此外,探讨了地代史温压演化对页岩油成藏的控制机制,并进一步评价了该方法的适用性。结果表明:青山口组地温梯度从一段到三段依次减小(3.84°C/100 m, 2.93°C/100 m, 2.49°C/100 m);高温带在古龙凹陷分布广泛,古龙页岩平均温度超过95℃,平均约为115℃。青山口组超压呈西高东低趋势。古龙页岩超压带主要集中在齐家—古龙凹陷和三照凹陷,平均压力系数分别为1.52和1.36。Opc模型确定了ⅰ类和ⅱ类有利带,主要分布在古龙凹陷中部和南部以及三照凹陷中部和西南部,页岩油资源量估计分别为7.1×108 t和17.2×108 t。典型井的演化特征表明,高温促进了有机质成熟和轻质油的生成,提高了页岩油的流动性,而超压则抑制了油气的耗散,为采油提供了充分的动力。研究表明,现今的温度-压力场有效地反映了古热力和压力状态的演化趋势。该评价方法具有较强的适用性和可扩展性,为非常规油气资源勘探提供了新的技术框架和理论基础。
{"title":"Present-day temperature and pressure fields in key areas of Northeast China: Implications for unconventional resource evaluation","authors":"Yue Huang ,&nbsp;Jian Chang ,&nbsp;Nansheng Qiu ,&nbsp;Nobuo Maeda","doi":"10.1016/j.gsf.2025.102148","DOIUrl":"10.1016/j.gsf.2025.102148","url":null,"abstract":"<div><div>The temperature-pressure fields within hydrocarbon-bearing basins are key geological factors controlling hydrocarbon generation, migration, and accumulation. In this study, we focus on the Qingshankou Formation in the northern part of the central depression of the Songliao Basin, China. A multi-parameter weighted evaluation model was created using present temperature-pressure field characteristics, with formation temperature-pressure as core variables, to evaluate shale oil resource potential. In addition, we explored the control mechanisms of temperature-pressure evolution during geological history on shale oil accumulation and further assessed the applicability of the proposed method. Our results show that the geothermal gradient of the Qingshankou Formation decreases from Member 1 to Member 3 (3.84 °C/100 m, 2.93 °C/100 m, and 2.49 °C/100 m, respectively). High-temperature zones are widely distributed in the Gulong sag, with the average temperature of the Gulong shale exceeding 95 °C and reaching an average of approximately 115 °C. Overpressure in the Qingshankou Formation exhibits a west-high to east-low trend. The overpressure zones of the Gulong shale are mainly concentrated in the Qijia-Gulong and Sanzhao sag, with average pressure coefficients of 1.52 and 1.36, respectively. The Opc model identified Class I and II favorable zones, mainly located in the central and southern parts of the Gulong Sag, as well as the central and southwestern Sanzhao Sag, with estimated shale oil resources of <span><math><mrow><mn>7.1</mn><mo>×</mo><msup><mrow><mn>10</mn></mrow><mrow><mn>8</mn></mrow></msup></mrow></math></span> tons and <span><math><mrow><mn>17.2</mn><mo>×</mo><msup><mrow><mn>10</mn></mrow><mrow><mn>8</mn></mrow></msup></mrow></math></span> tons, respectively. Evolutionary profiles from representative wells indicate that elevated temperatures enhance organic matter maturation and light oil generation, improving shale oil mobility, while overpressure suppresses hydrocarbon dissipation and provides a sufficient driving force for oil production. This study demonstrates that present-day temperature-pressure fields effectively reflect the evolution trends of paleo-thermal and pressure regimes. The proposed evaluation method shows strong applicability and scalability, offering a new technical framework and theoretical foundation for the exploration of unconventional hydrocarbon resources.</div></div>","PeriodicalId":12711,"journal":{"name":"Geoscience frontiers","volume":"16 6","pages":"Article 102148"},"PeriodicalIF":8.9,"publicationDate":"2025-09-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145105641","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"地球科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Extreme drought affects lake water quality, quantity, morphometry: Evidence from China’s largest fresh water lake under the 2022 global drought 极端干旱影响湖泊水质、水量和形态:2022年全球干旱下中国最大淡水湖的证据
IF 8.9 1区 地球科学 Q1 GEOSCIENCES, MULTIDISCIPLINARY Pub Date : 2025-09-04 DOI: 10.1016/j.gsf.2025.102146
Xihua Wang , Zejun Liu , Y. Jun Xu , Boyang Mao , Shunqing Jia
Extreme drought poses a significant threat to humanity. In the summer of 2022, the world experienced the worst drought in recent years, with a precipitation deficit and an abnormal high temperature, profoundly affecting human life and the aquatic environment. However, the drought influence on large freshwater lakes remains unclear. In this study, we selected China’s largest freshwater lake (Poyang Lake) as the research object and investigated the lake water area, quantity, lake morphology and water quality in 2018 (normal season) and 2022 (extreme drought period). Results showed that standardized precipitation index (SPI), standardized runoff index (SRI) and standardized precipitation-evapotranspiration index (SPEI) reached moderate to severe drought in the summer of 2022. From 2018 to 2022, lake water area decreased (1789.62 km2), water quantity reduced (15.40 × 109 m3) and lake shoreline decreased (2923.70 km). The shoreline development index, size ratio and energy factor decreased by 4.87, 198.53 m and 963.60, specifically. The dynamic ratio, relative depth and Schindler’s ratio increased by 1457.10, 0.04 and 13.48 m−1, respectively. The water chemical indicators varied significantly in two years and the water hydrochemical types changed from SO4·Cl − Ca·Mg type and HCO3 − Ca·Mg type to SO4·Cl − Ca·Mg type from 2018 to 2022. Water-rock interaction, alternating cation adsorption and anthropogenic influence on water quality represented different patterns in two periods. Our findings demonstrate significant differences in water resources and quality between common and extreme drought conditions in China’s largest fresh water lake, which can inform research on climate change effects on international large freshwater lakes.
极端干旱对人类构成重大威胁。2022年夏季,全球经历了近年来最严重的干旱,降水不足,气温异常高,深刻影响了人类生活和水生环境。然而,干旱对大型淡水湖的影响尚不清楚。本研究以中国最大的淡水湖鄱阳湖为研究对象,对2018年(正常季节)和2022年(极端干旱期)的湖泊水域面积、数量、湖泊形态和水质进行了调查。结果表明:2022年夏季,标准化降水指数(SPI)、标准化径流指数(SRI)和标准化降水-蒸散指数(SPEI)达到中至重度干旱;2018 - 2022年,湖泊水域面积减少1789.62 km2,水量减少15.40 × 109 m3,湖泊岸线减少2923.70 km。岸线发育指数、尺度比和能量因子分别下降4.87、198.53 m和963.60 m。动态比、相对深度和Schindler’s比分别增加了1457.10、0.04和13.48 m−1。水化学指标在两年内变化显著,2018 - 2022年水化学类型由SO4·Cl - Ca·Mg型和HCO3 - Ca·Mg型转变为SO4·Cl - Ca·Mg型。水岩相互作用、交替阳离子吸附和人为对水质的影响在两个时期表现出不同的模式。研究结果表明,中国最大的淡水湖在普通干旱和极端干旱条件下的水资源和水质存在显著差异,为气候变化对国际大型淡水湖的影响研究提供了参考。
{"title":"Extreme drought affects lake water quality, quantity, morphometry: Evidence from China’s largest fresh water lake under the 2022 global drought","authors":"Xihua Wang ,&nbsp;Zejun Liu ,&nbsp;Y. Jun Xu ,&nbsp;Boyang Mao ,&nbsp;Shunqing Jia","doi":"10.1016/j.gsf.2025.102146","DOIUrl":"10.1016/j.gsf.2025.102146","url":null,"abstract":"<div><div>Extreme drought poses a significant threat to humanity. In the summer of 2022, the world experienced the worst drought in recent years, with a precipitation deficit and an abnormal high temperature, profoundly affecting human life and the aquatic environment. However, the drought influence on large freshwater lakes remains unclear. In this study, we selected China’s largest freshwater lake (Poyang Lake) as the research object and investigated the lake water area, quantity, lake morphology and water quality in 2018 (normal season) and 2022 (extreme drought period). Results showed that standardized precipitation index (SPI), standardized runoff index (SRI) and standardized precipitation-evapotranspiration index (SPEI) reached moderate to severe drought in the summer of 2022. From 2018 to 2022, lake water area decreased (1789.62 km<sup>2</sup>), water quantity reduced (15.40 × 10<sup>9</sup> m<sup>3</sup>) and lake shoreline decreased (2923.70 km). The shoreline development index, size ratio and energy factor decreased by 4.87, 198.53 m and 963.60, specifically. The dynamic ratio, relative depth and Schindler’s ratio increased by 1457.10, 0.04 and 13.48 m<sup>−1</sup>, respectively. The water chemical indicators varied significantly in two years and the water hydrochemical types changed from SO<sub>4</sub>·Cl − Ca·Mg type and HCO<sub>3</sub> − Ca·Mg type to SO<sub>4</sub>·Cl − Ca·Mg type from 2018 to 2022. Water-rock interaction, alternating cation adsorption and anthropogenic influence on water quality represented different patterns in two periods. Our findings demonstrate significant differences in water resources and quality between common and extreme drought conditions in China’s largest fresh water lake, which can inform research on climate change effects on international large freshwater lakes.</div></div>","PeriodicalId":12711,"journal":{"name":"Geoscience frontiers","volume":"16 6","pages":"Article 102146"},"PeriodicalIF":8.9,"publicationDate":"2025-09-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145060209","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"地球科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Thermokarst disturbance responses to climate change across the circumpolar permafrost regions from 1990 to 2023 1990 - 2023年环极多年冻土区热岩溶扰动对气候变化的响应
IF 8.9 1区 地球科学 Q1 GEOSCIENCES, MULTIDISCIPLINARY Pub Date : 2025-09-02 DOI: 10.1016/j.gsf.2025.102147
Ya Liu , Haijun Qiu , Ninglian Wang , Dongdong Yang , Kailiang Zhao , Guoqing Yang , Wenchao Huangfu , Wanqi Luo
Warming climate drives permafrost degradation and forms serious thermokarst disturbances, with significant impacts on geomorphology, hydrology, and ecological processes. However, the long-term monitoring of thermokarst disturbances and their next development remains a challenge across the circumpolar permafrost regions. Here, we calculate six spectral indices from Landsat images to represent greenness, wetness, and brightness, quantifying the spatiotemporal characteristics of thermokarst landscape dynamics and further revealing their development with a warming climate. Additionally, DNMI, NDWI, and NDVI are selected to verify the occurrence and severity of retrogressive thaw slumps, thermokarst lake expansion, and drainage by the LandTrendr algorithm on the Google Earth Engine platform. Three major types of thermokarst events show a consistent disturbance year, correlating with the summer temperature increase point around 2000. Their correlation analysis also reveals that the subsequent landscape development of thermokarst disturbances is related to the warming context, showing vegetation greening and soil wetting trends. These findings highlight the dynamic characteristics of thermokarst disturbances from 1990 to 2023, providing a comprehensive understanding of thermokarst development under a changing climate.
气候变暖导致多年冻土退化,形成严重的热岩溶扰动,对地貌、水文和生态过程产生重大影响。然而,对热岩溶扰动及其下一步发展的长期监测仍然是整个极地多年冻土区的一个挑战。在此基础上,我们利用Landsat图像计算了代表绿度、湿度和亮度的6个光谱指数,量化了热岩溶景观动态的时空特征,并进一步揭示了它们随气候变暖的发展。利用谷歌Earth Engine平台上的LandTrendr算法,选择DNMI、NDWI和NDVI来验证退行性融塌、热岩溶湖扩张和排水的发生和严重程度。三种主要热岩溶事件表现出一致的扰动年,与2000年左右的夏季增温点相关。二者的相关分析还表明,热岩溶扰动的后续景观发展与气候变暖背景有关,表现为植被绿化和土壤湿润趋势。这些发现突出了1990 - 2023年热岩溶扰动的动态特征,为全面了解气候变化下的热岩溶发育提供了依据。
{"title":"Thermokarst disturbance responses to climate change across the circumpolar permafrost regions from 1990 to 2023","authors":"Ya Liu ,&nbsp;Haijun Qiu ,&nbsp;Ninglian Wang ,&nbsp;Dongdong Yang ,&nbsp;Kailiang Zhao ,&nbsp;Guoqing Yang ,&nbsp;Wenchao Huangfu ,&nbsp;Wanqi Luo","doi":"10.1016/j.gsf.2025.102147","DOIUrl":"10.1016/j.gsf.2025.102147","url":null,"abstract":"<div><div>Warming climate drives permafrost degradation and forms serious thermokarst disturbances, with significant impacts on geomorphology, hydrology, and ecological processes. However, the long-term monitoring of thermokarst disturbances and their next development remains a challenge across the circumpolar permafrost regions. Here, we calculate six spectral indices from Landsat images to represent greenness, wetness, and brightness, quantifying the spatiotemporal characteristics of thermokarst landscape dynamics and further revealing their development with a warming climate. Additionally, DNMI, NDWI, and NDVI are selected to verify the occurrence and severity of retrogressive thaw slumps, thermokarst lake expansion, and drainage by the LandTrendr algorithm on the Google Earth Engine platform. Three major types of thermokarst events show a consistent disturbance year, correlating with the summer temperature increase point around 2000. Their correlation analysis also reveals that the subsequent landscape development of thermokarst disturbances is related to the warming context, showing vegetation greening and soil wetting trends. These findings highlight the dynamic characteristics of thermokarst disturbances from 1990 to 2023, providing a comprehensive understanding of thermokarst development under a changing climate.</div></div>","PeriodicalId":12711,"journal":{"name":"Geoscience frontiers","volume":"16 6","pages":"Article 102147"},"PeriodicalIF":8.9,"publicationDate":"2025-09-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145105584","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"地球科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
How energy intensity and global energy dynamics shape renewable energy transition in APEC economies 能源强度和全球能源动态如何影响亚太经合组织经济体的可再生能源转型
IF 8.9 1区 地球科学 Q1 GEOSCIENCES, MULTIDISCIPLINARY Pub Date : 2025-08-23 DOI: 10.1016/j.gsf.2025.102134
Guixian Tian , Xiang Hua , Danyu Li , Junyi Tian
This study examines the critical factors influencing the adoption of modern renewable energy in selected APEC countries from 1997 to 2023, with a focus on their implications for sustainable development and environmental sustainability. Using dynamic panel data estimation techniques (Arellano–Bond and system dynamic panel-data estimation), we analyze the interplay between energy intensity, world energy balances, economic globalization, and the shadow economy in shaping the share of modern renewables in total final energy consumption. Our results indicate that higher energy intensity reduces renewable energy adoption, reflecting systemic challenges in integrating clean energy into high-demand systems. Conversely, world energy balances and economic globalization enhance renewable energy penetration, driven by decarbonization policies, technological advancements, and cross-border collaboration. Surprisingly, the shadow economy also plays a positive role, suggesting that informal sector activities may facilitate small-scale renewable energy investments. From a sustainability perspective, these findings underscore the need for APEC economies to prioritize energy efficiency, strengthen international cooperation, and implement inclusive policies that support renewable energy transitions. By addressing structural barriers and leveraging globalization, APEC nations can accelerate progress toward Sustainable Development Goals (SDGs), particularly SDG 7 (Affordable and Clean Energy) and SDG 13 (Climate Action). Policymakers are encouraged to design targeted interventions, including green financing mechanisms, technology transfer programs, and regulatory incentives, to align economic growth with long-term environmental sustainability.
本研究考察了1997年至2023年间影响APEC国家采用现代可再生能源的关键因素,重点研究了这些因素对可持续发展和环境可持续性的影响。利用动态面板数据估计技术(Arellano-Bond和系统动态面板数据估计),我们分析了能源强度、世界能源平衡、经济全球化和影子经济在塑造现代可再生能源在最终能源消费总量中的份额方面的相互作用。我们的研究结果表明,较高的能源强度降低了可再生能源的采用,反映了将清洁能源整合到高需求系统中的系统性挑战。相反,在脱碳政策、技术进步和跨境合作的推动下,世界能源平衡和经济全球化促进了可再生能源的渗透。令人惊讶的是,影子经济也发挥了积极作用,表明非正规部门的活动可能促进小规模的可再生能源投资。从可持续发展的角度来看,这些发现强调了亚太经合组织经济体需要优先考虑能源效率,加强国际合作,实施支持可再生能源转型的包容性政策。通过解决结构性障碍和利用全球化,亚太经合组织国家可以加速实现可持续发展目标,特别是可持续发展目标7(负担得起的清洁能源)和可持续发展目标13(气候行动)。鼓励政策制定者设计有针对性的干预措施,包括绿色融资机制、技术转让项目和监管激励措施,使经济增长与长期环境可持续性保持一致。
{"title":"How energy intensity and global energy dynamics shape renewable energy transition in APEC economies","authors":"Guixian Tian ,&nbsp;Xiang Hua ,&nbsp;Danyu Li ,&nbsp;Junyi Tian","doi":"10.1016/j.gsf.2025.102134","DOIUrl":"10.1016/j.gsf.2025.102134","url":null,"abstract":"<div><div>This study examines the critical factors influencing the adoption of modern renewable energy in selected APEC countries from 1997 to 2023, with a focus on their implications for sustainable development and environmental sustainability. Using dynamic panel data estimation techniques (Arellano–Bond and system dynamic panel-data estimation), we analyze the interplay between energy intensity, world energy balances, economic globalization, and the shadow economy in shaping the share of modern renewables in total final energy consumption. Our results indicate that higher energy intensity reduces renewable energy adoption, reflecting systemic challenges in integrating clean energy into high-demand systems. Conversely, world energy balances and economic globalization enhance renewable energy penetration, driven by decarbonization policies, technological advancements, and cross-border collaboration. Surprisingly, the shadow economy also plays a positive role, suggesting that informal sector activities may facilitate small-scale renewable energy investments. From a sustainability perspective, these findings underscore the need for APEC economies to prioritize energy efficiency, strengthen international cooperation, and implement inclusive policies that support renewable energy transitions. By addressing structural barriers and leveraging globalization, APEC nations can accelerate progress toward Sustainable Development Goals (SDGs), particularly SDG 7 (Affordable and Clean Energy) and SDG 13 (Climate Action). Policymakers are encouraged to design targeted interventions, including green financing mechanisms, technology transfer programs, and regulatory incentives, to align economic growth with long-term environmental sustainability.</div></div>","PeriodicalId":12711,"journal":{"name":"Geoscience frontiers","volume":"16 6","pages":"Article 102134"},"PeriodicalIF":8.9,"publicationDate":"2025-08-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144996840","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"地球科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
期刊
Geoscience frontiers
全部 Acc. Chem. Res. ACS Applied Bio Materials ACS Appl. Electron. Mater. ACS Appl. Energy Mater. ACS Appl. Mater. Interfaces ACS Appl. Nano Mater. ACS Appl. Polym. Mater. ACS BIOMATER-SCI ENG ACS Catal. ACS Cent. Sci. ACS Chem. Biol. ACS Chemical Health & Safety ACS Chem. Neurosci. ACS Comb. Sci. ACS Earth Space Chem. ACS Energy Lett. ACS Infect. Dis. ACS Macro Lett. ACS Mater. Lett. ACS Med. Chem. Lett. ACS Nano ACS Omega ACS Photonics ACS Sens. ACS Sustainable Chem. Eng. ACS Synth. Biol. Anal. Chem. BIOCHEMISTRY-US Bioconjugate Chem. BIOMACROMOLECULES Chem. Res. Toxicol. Chem. Rev. Chem. Mater. CRYST GROWTH DES ENERG FUEL Environ. Sci. Technol. Environ. Sci. Technol. Lett. Eur. J. Inorg. Chem. IND ENG CHEM RES Inorg. Chem. J. Agric. Food. Chem. J. Chem. Eng. Data J. Chem. Educ. J. Chem. Inf. Model. J. Chem. Theory Comput. J. Med. Chem. J. Nat. Prod. J PROTEOME RES J. Am. Chem. Soc. LANGMUIR MACROMOLECULES Mol. Pharmaceutics Nano Lett. Org. Lett. ORG PROCESS RES DEV ORGANOMETALLICS J. Org. Chem. J. Phys. Chem. J. Phys. Chem. A J. Phys. Chem. B J. Phys. Chem. C J. Phys. Chem. Lett. Analyst Anal. Methods Biomater. Sci. Catal. Sci. Technol. Chem. Commun. Chem. Soc. Rev. CHEM EDUC RES PRACT CRYSTENGCOMM Dalton Trans. Energy Environ. Sci. ENVIRON SCI-NANO ENVIRON SCI-PROC IMP ENVIRON SCI-WAT RES Faraday Discuss. Food Funct. Green Chem. Inorg. Chem. Front. Integr. Biol. J. Anal. At. Spectrom. J. Mater. Chem. A J. Mater. Chem. B J. Mater. Chem. C Lab Chip Mater. Chem. Front. Mater. Horiz. MEDCHEMCOMM Metallomics Mol. Biosyst. Mol. Syst. Des. Eng. Nanoscale Nanoscale Horiz. Nat. Prod. Rep. New J. Chem. Org. Biomol. Chem. Org. Chem. Front. PHOTOCH PHOTOBIO SCI PCCP Polym. Chem.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
0
微信
客服QQ
Book学术公众号 扫码关注我们
反馈
×
意见反馈
请填写您的意见或建议
请填写您的手机或邮箱
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
现在去查看 取消
×
提示
确定
Book学术官方微信
Book学术文献互助
Book学术文献互助群
群 号:604180095
Book学术
文献互助 智能选刊 最新文献 互助须知 联系我们:info@booksci.cn
Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。
Copyright © 2023 Book学术 All rights reserved.
ghs 京公网安备 11010802042870号 京ICP备2023020795号-1