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Polarization-encoded color images for information encryption enabled by HfN refractory plasmonic metasurfaces 极化编码彩色图像,用于HfN难熔等离子体超表面的信息加密
IF 7.5 2区 物理与天体物理 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-11-09 DOI: 10.1515/nanoph-2025-0502
Yu-Cheng Chu, Tzu-Yu Peng, Chen-Yu Wang, Shyr-Shyan Yeh, Jia-Wern Chen, Yu-Jung Lu
Polarization control plasmonic nanostructures provide a unique route to manipulate light–matter interactions at the nanoscale and are particularly powerful for information security applications, where polarization-encoded color images can be used for optical encryption and anticounterfeiting. Conventional plasmonic materials such as Au and Ag, however, suffer from poor thermal stability, limiting their integration into robust, CMOS-compatible devices. Here, we present a polarization-encoded color image platform based on refractory HfN plasmonic metasurfaces, which combine gold-like optical properties with exceptional hardness, compositional tunability, and superior high-temperature resilience. Periodically patterned HfN nanoantennas with widths of 200 nm exhibit well-defined localized surface plasmon resonances in the visible spectrum (628 and 564 nm) and can be selectively excited by orthogonal linear polarizations. We designed and realized a polarization-encoded color image in which distinct color channels are revealed under x- and y-polarized illumination, enabling decryption of hidden information. Under unpolarized illumination, the superposition of color channels effectively conceals the message, achieving robust optical encryption. Our results establish HfN plasmonic nanostructures as a key material platform for next-generation nanophotonics, uniquely combining gold-like optical properties with exceptional thermal robustness. Even after high-temperature annealing, HfN retains its plasmonic response, enabling reliable polarization-resolved color image encoding and decryption. This breakthrough paves the way for thermally resilient metasurfaces for secure data encryption, anticounterfeiting, and robust operation in extreme environments.
偏振控制等离子体纳米结构提供了一种在纳米尺度上操纵光-物质相互作用的独特途径,对于信息安全应用尤其强大,其中偏振编码的彩色图像可用于光学加密和防伪。然而,传统的等离子体材料,如Au和Ag,热稳定性差,限制了它们集成到强大的cmos兼容器件中。在这里,我们提出了一种基于难熔HfN等离子体超表面的偏振编码彩色图像平台,它结合了像金一样的光学性质,特殊的硬度,成分可调性和优越的高温弹性。宽度为200 nm的周期性图像化HfN纳米天线在可见光谱(628和564 nm)中表现出明确的局部表面等离子体共振,并且可以通过正交线性极化选择性激发。我们设计并实现了一种偏振编码的彩色图像,该图像在x和y偏振照明下显示出不同的颜色通道,从而实现了隐藏信息的解密。在非偏振照明下,彩色通道的叠加有效地隐藏了信息,实现了鲁棒的光加密。我们的研究结果建立了HfN等离子体纳米结构作为下一代纳米光子学的关键材料平台,独特地结合了类似金的光学特性和出色的热鲁棒性。即使在高温退火后,HfN仍保持其等离子体响应,从而实现可靠的偏振分辨彩色图像编码和解密。这一突破为热弹性超表面的安全数据加密、防伪和极端环境下的稳健运行铺平了道路。
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引用次数: 0
Optimizing the localization precision in coherent scattering microscopy using structured light 利用结构光优化相干散射显微镜定位精度
IF 7.5 2区 物理与天体物理 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-11-07 DOI: 10.1515/nanoph-2025-0435
Ulrich Hohenester, Felix Hitzelhammer, Georg Krainer, Peter Banzer, Thomas Juffmann
We employ the concept of quantum Fisher information to optimize the focused excitation fields in coherent scattering microscopy. Our optimization goal is to achieve the best possible localization precision for small scatterers located above a glass coverslip, while keeping the intensity of the total incoming excitation fields fixed. For small numerical aperture (NA) values, the optimal fields have linear or circular polarization, and the excitation beam can be well approximated by a Gaussian one. For larger NA values, the optimal beam acquires radial polarization. We show that the high localization precision can be attributed to high field strengths at the scatterer position, and correspondingly a large number of scattered and detected photons. Finally, we evaluate the performance of the optimized beams in interferometric scattering microscopy (i scat ), and further optimize these fields for i scat localization using the concept of Fisher information.
我们采用量子费雪信息的概念来优化相干散射显微镜的聚焦激发场。我们的优化目标是在保持总入射激励场强度不变的情况下,对位于玻璃盖盖上方的小散射体实现尽可能高的定位精度。对于较小的数值孔径(NA),最优场为线偏振或圆偏振,激发光束可以很好地近似为高斯光束。当NA值较大时,最优光束获得径向偏振。研究表明,高定位精度可归因于散射体位置的高场强,以及相应的大量散射和检测光子。最后,我们评估了优化光束在干涉散射显微镜(i scat)中的性能,并利用Fisher信息的概念进一步优化这些场以进行i scat定位。
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引用次数: 0
Spin angular momentum modulation via spin–orbit interaction in fractional orbital angular momentum beams 分数轨道角动量光束中自旋-轨道相互作用的自旋角动量调制
IF 7.5 2区 物理与天体物理 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-11-07 DOI: 10.1515/nanoph-2025-0430
Xusheng Chen, Fanfei Meng, Kang Du, Min Lin, Luping Du
Light exhibits both spin and orbital angular momentum (SAM and OAM). These two forms of angular momentum remain independent in paraxial fields, but become coupled in confined fields through spin–orbit interactions (SOI). The SOI mechanism allows for the manipulation of SAM to generate structured light fields featuring nontrivial topological characteristics, such as optical skyrmions. Conventional OAM beams, nonetheless, carry discrete integer topological charges (TCs), leading to discrete SAM states. This discrete property poses a persistent challenge for achieving continuous control of SAM. To tackle this fundamental issue, we explored fractional orbital angular momentum (FOAM) beams, whose TCs are extended from integers to fractions, to realize continuous and precise control of SAM. A direct mathematical relationship between the fractional effective TCs of FOAM beams and the orientation distributions of the SAM vector has been derived. This theoretical prediction has been experimentally verified using our home-built near-field mapping system, by which the distinct SAM distributions of surface cosine waves regulated by FOAM beams were mapped out. As a potential application, we also devised an inverse detection method to accurately measure the fractional effective TCs of FOAM, which achieved theoretical and experimental accuracies of 10 −5 and 10 −2 , respectively. These advancements may enhance our fundamental understanding of the SOI mechanism, and hence could create novel opportunities for light field manipulation, optical communication, and other related areas.
光同时显示自旋和轨道角动量(SAM和OAM)。这两种形式的角动量在近轴场中保持独立,但在受限场中通过自旋轨道相互作用(SOI)耦合。SOI机制允许对SAM进行操作,以产生具有非平凡拓扑特征的结构光场,例如光学天空。然而,传统的OAM波束携带离散整数拓扑电荷(TCs),导致离散的SAM状态。这种离散性对实现SAM的连续控制提出了持续的挑战。为了解决这一基本问题,我们探索了分数轨道角动量(FOAM)光束,将其tc从整数扩展到分数,以实现SAM的连续精确控制。推导了泡沫塑料梁的分数阶有效热载荷与SAM矢量方向分布之间的直接数学关系。用自制的近场成图系统对这一理论预测进行了实验验证,绘制出泡沫梁调节的表面余弦波的不同SAM分布。作为一种潜在的应用,我们还设计了一种逆检测方法来精确测量FOAM的有效tc分数,该方法的理论和实验精度分别为10−5和10−2。这些进展可能增强我们对SOI机制的基本理解,因此可能为光场操纵、光通信和其他相关领域创造新的机会。
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引用次数: 0
On-chip polarization management for stable nonlinear signal generation in thin-film lithium niobate 铌酸锂薄膜中稳定非线性信号产生的片上极化管理
IF 7.5 2区 物理与天体物理 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-11-07 DOI: 10.1515/nanoph-2025-0339
Junhyung Lee, Sunghyun Moon, Yongchan Park, Uijoon Park, Hansol Kim, Changhyun Kim, Minho Choi, Jin-Il Lee, Hyeon Hwang, Min-Kyo Seo, Dae-Hwan Ahn, Hojoong Jung, Hyounghan Kwon
Nonlinear signal generation requires precise control of the input polarization to satisfy phase-matching conditions. Conventional polarization management using external fiber polarization controllers or bulk wave plates increases coupling complexity and can degrade polarization fidelity and conversion efficiency in nonlinear photonic systems. Here, we demonstrate on-chip polarization control in thin-film lithium niobate nonlinear photonic circuits. Integrated polarization modulators enable real-time tuning of arbitrary input polarization states and thus provide on-demand control of nonlinear conversion in a periodically poled lithium niobate waveguide. A closed-loop feedback system, which integrates auto-compensation and automatic fiber-chip alignment routines, automatically optimizes the second-harmonic generation intensity and maintains performance over extended periods despite polarization scrambling and environmental perturbations. This integrated approach reduces coupling complexity and offers a scalable route toward fully reconfigurable nonlinear photonic systems.
非线性信号的产生需要精确控制输入极化以满足相位匹配条件。在非线性光子系统中,使用外部光纤偏振控制器或体波片的传统偏振管理增加了耦合复杂性,降低了偏振保真度和转换效率。在这里,我们展示了薄膜铌酸锂非线性光子电路的片上极化控制。集成偏振调制器能够实时调谐任意输入偏振状态,从而在周期性极化铌酸锂波导中提供非线性转换的按需控制。闭环反馈系统集成了自动补偿和自动光纤芯片对准程序,自动优化二次谐波产生强度,并在极化置乱和环境扰动的情况下长时间保持性能。这种集成的方法降低了耦合的复杂性,并为完全可重构的非线性光子系统提供了可扩展的途径。
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引用次数: 0
Near-unity fueling light into a single plasmonic nanocavity 近乎统一地将光注入一个等离子体纳米腔
IF 7.5 2区 物理与天体物理 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-11-06 DOI: 10.1515/nanoph-2025-0331
Haiming Ye, Junhao Ge, Zhengyi Lu, Dudu Song, Jiamin Ji, Zhaoyang Peng, Shunping Zhang, Hongxing Xu
Plasmonic nanocavities have emerged as a powerful platform for extreme light confinement, enabling transformative applications in single-molecule Raman spectroscopy, ultra-sensitive sensing, strong light–matter interactions, etc. By harnessing localized surface plasmons, these nanostructures support unprecedented field enhancement, exceeding 1,000-fold in the sub-nanometer gap. However, a fundamental trade-off exists between deep sub-wavelength field localization and its efficient coupling to free-space light, limiting their practical performance. Here, we show that by balancing the electric and magnetic resonance, more than 55 % of a focused Gaussian beam can be fueled into a nanocube-on-mirror nanocavity. With few concentric gratings, the coupling efficiency can even go up to >95 % at optimal conditions. This design can work at both visible and telecommunication wavelengths and show robust tolerance to fabrication imperfections. Our work indicates that the long-standing conflict between deep field localization and efficient external coupling in plasmonic systems can be resolved by multiscale structure design, promising the use of a single metal nanoparticle for advanced nanophotonic or optoelectronic devices.
等离子体纳米腔已经成为一个强大的极端光约束平台,在单分子拉曼光谱、超灵敏传感、强光-物质相互作用等方面实现了变革性的应用。通过利用局部表面等离子体,这些纳米结构支持前所未有的场增强,在亚纳米间隙中超过1000倍。然而,在深亚波长场定位及其与自由空间光的有效耦合之间存在一个基本的权衡,限制了它们的实际性能。在这里,我们展示了通过平衡电和磁共振,超过55%的聚焦高斯光束可以被燃料注入到纳米立方体-镜面纳米腔中。在较低的同心光栅条件下,耦合效率最高可达95%。这种设计可以在可见光和电信波长下工作,并且对制造缺陷表现出强大的容忍度。我们的工作表明,等离子体系统中深场定位和有效外部耦合之间的长期冲突可以通过多尺度结构设计来解决,这有望将单个金属纳米颗粒用于先进的纳米光子或光电器件。
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引用次数: 0
Second-harmonic generation in NbOI 2 -integrated silicon nitride microdisk resonators nboi2集成氮化硅微盘谐振器中二次谐波的产生
IF 7.5 2区 物理与天体物理 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-11-06 DOI: 10.1515/nanoph-2025-0428
Ning Liu, Qiang Liu, Yutian Lin, Zhihong Zhu, Ken Liu
In recent years, two-dimensional (2D) niobium oxide dihalides (e.g., NbOI 2 ) have garnered significant research interest in nonlinear photonics due to their prominent second-order nonlinear optical properties. Integrating these materials with high-quality-factor optical microcavities represents a crucial approach for developing high-performance on-chip nonlinear optical devices. This work demonstrates NbOI 2 -integrated silicon nitride (Si 3 N 4 ) microdisk resonators that achieve second-harmonic generation under low-power (sub-milliwatt) continuous-wave laser pumping, leveraging the superior second-order nonlinearity of NbOI 2 and the strong optical field confinement capability of Si 3 N 4 microdisks. The conversion efficiency of the device is calculated to be about 0.024 %/W. The intrinsic lack of inversion symmetry in NbOI 2 crystals avoids the laborious layer-number-dependent symmetry screening typically required for other 2D materials, while the developed van der Waals transfer technique provides a universal strategy for integrating niobium oxide dihalides with photonic microcavities. This study not only establishes a material-photon co-design strategy for on-chip nonlinear light sources but also lays a critical foundation for advancing quantum photonic chips and on-chip metrology systems.
近年来,二维(2D)氧化铌二卤化物(例如nboi2)由于其突出的二阶非线性光学性质而在非线性光子学中获得了重要的研究兴趣。将这些材料与高质量因数的光学微腔集成是开发高性能片上非线性光学器件的重要途径。本研究展示了nboi2集成的氮化硅(si3n4)微盘谐振器,利用nboi2优越的二阶非线性和si3n4微盘强大的光场约束能力,在低功率(亚毫瓦)连续波激光泵浦下实现了二次谐波产生。经计算,该器件的转换效率约为0.024% /W。nboi2晶体固有的反演对称性缺乏避免了其他二维材料通常需要的繁琐的层数依赖的对称筛选,而开发的范德华转移技术为氧化铌二卤化物与光子微腔的集成提供了一种通用策略。本研究不仅建立了片上非线性光源的材料-光子协同设计策略,而且为推进量子光子芯片和片上计量系统的发展奠定了重要基础。
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引用次数: 0
Single-shot Stokes polarimetry of plasmon-coupled single-molecule fluorescence 等离子体耦合单分子荧光的单次Stokes偏振法
IF 7.5 2区 物理与天体物理 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-11-06 DOI: 10.1515/nanoph-2025-0352
Sarojini Mahajan, Yuyang Wang, Teun A.P.M. Huijben, Rodolphe Marie, Peter Zijlstra
The photophysical properties of single-molecule emitters are altered by nanophotonic structures such as single plasmonic nanoparticles. The intensity and spectral properties of plasmon-coupled emitters have been studied extensively, but little is known about the effect of plasmon coupling on emission polarization. Here, we examine how particle-emitter coupling modifies the polarization of single fluorophores in both experiment and simulation. We quantify degree of linear polarization using Stokes polarimetry with a polarization-sensitive camera and quantify the Stokes parameters with a single-shot acquisition without requiring additional optics in the detection path. We then perform polarization-resolved measurements of plasmon-coupled fluorescence from single-molecule emitters using an approach based on DNA-PAINT. We quantify the effect of the setup and associated noise sources on the measured Stokes parameters. We then quantify the angle of linear polarization (AoLP) and the degree of linear polarization (DoLP) for thousands of single molecules. We compare our results to a numerical model that propagates the plasmon-coupled single-molecule emission through the optical setup to yield the polarized point spread function in the camera plane. Simulations and experiments are in good agreement and shed new light on the polarization of antenna-coupled fluorophores, while it establishes single-shot polarimetry as a promising and straightforward method to quantify polarization properties at the single-molecule level.
单等离子体纳米粒子等纳米光子结构改变了单分子发射体的光物理性质。等离子体耦合发射体的强度和光谱特性已经得到了广泛的研究,但对等离子体耦合对发射极化的影响知之甚少。在这里,我们研究了粒子-发射器耦合如何在实验和模拟中改变单个荧光团的偏振。我们使用Stokes偏振法和偏振敏感相机来量化线偏振度,并通过单次采集来量化Stokes参数,而不需要在检测路径中添加额外的光学器件。然后,我们使用基于DNA-PAINT的方法对来自单分子发射器的等离子体耦合荧光进行偏振分辨测量。我们量化了设置和相关噪声源对测量的斯托克斯参数的影响。然后,我们量化了数千个单分子的线偏振角(AoLP)和线偏振度(DoLP)。我们将我们的结果与通过光学装置传播等离子体耦合单分子发射的数值模型进行比较,以产生相机平面上的偏振点扩展函数。模拟和实验结果吻合良好,对天线耦合荧光团的极化现象有了新的认识,同时建立了单次极化法作为一种在单分子水平上量化极化特性的有前途和直接的方法。
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引用次数: 0
Continuously tunable broadband adiabatic coupler for programmable photonic processors 用于可编程光子处理器的连续可调谐宽带绝热耦合器
IF 7.5 2区 物理与天体物理 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-11-06 DOI: 10.1515/nanoph-2025-0402
Xiang Liu, Peipeng Xu, Yingxuan Zhao, Zhen Sheng, Fuwan Gan
Programmable integrated photonic circuits are poised to drive a new revolution in information systems by synergizing with high-speed digital signals. Central to this vision is the ability to reconfigure optical signal processing for multi-functional photonic integration. Here, we design and experimentally demonstrate a thermo-optically reconfigurable adiabatic coupler monolithically integrated on a silicon photonics platform. The device combines adiabatic directional couplers with titanium nitride (TiN) micro-heaters embedded in the adiabatic transition region, enabling dynamic coupling ratio tuning via the localized thermo-optic modulation. Experimental results confirm continuous coupling ratio adjustment from 50:50 to 70:30 across 80-nm bandwidth (1,520–1,600 nm), with insertion loss kept below 0.25 dB. Leveraging its tunability, the device enables programmable spectral routing with free spectral ranges (FSR) of 20 nm and 40 nm. The proposed approach offers enhanced flexibility and scalability for high-density photonic systems, providing a promising pathway toward next-generation programmable photonic circuits and optical computing architectures.
可编程集成光子电路与高速数字信号的协同作用将推动信息系统的新革命。这一愿景的核心是重新配置光信号处理以实现多功能光子集成的能力。在这里,我们设计并实验证明了一个热光学可重构绝热耦合器单片集成在硅光子学平台。该器件将绝热定向耦合器与嵌入绝热过渡区的氮化钛(TiN)微加热器相结合,通过局部热光调制实现动态耦合比调谐。实验结果证实,在80nm带宽(1520 ~ 1600nm)范围内,耦合比可在50:50 ~ 70:30范围内连续调节,插入损耗保持在0.25 dB以下。利用其可调性,该器件可实现20 nm和40 nm自由光谱范围(FSR)的可编程光谱路由。所提出的方法为高密度光子系统提供了增强的灵活性和可扩展性,为下一代可编程光子电路和光计算架构提供了一条有前途的途径。
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引用次数: 0
In honor of Federico Capasso, a visionary in nanophotonics, on the occasion of his 75th birthday 为了纪念费德里科·卡帕索,一位纳米光子学的梦想家,在他75岁生日之际
IF 7.5 2区 物理与天体物理 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-11-06 DOI: 10.1515/nanoph-2025-0449
Alexandra Boltasseva, Nader Engheta, Giuseppe Strangi, Dennis Couwenberg
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引用次数: 0
Atomic state interferometry for complex vector light 复矢量光的原子态干涉测量
IF 7.5 2区 物理与天体物理 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-11-06 DOI: 10.1515/nanoph-2025-0491
Kuntal Samanta, Sphinx J. Svensson, Sonja Franke-Arnold, Niclas Westerberg
Features of complex vector light become important in any interference effects, including scattering, diffraction, and nonlinear processes. Here, we are investigating the role of polarization-structured light in atomic state interferometers. Unlike optical or atomic path interferometers, these facilitate local interference between atomic transition amplitudes and hence the orthogonal optical polarization components driving these transitions. We develop a fully analytical description for the interaction of generalized structured light with an atomic four state system, that is, multiply connected via optical as well as magnetic transitions. Our model allows us to identify spatially dependent dark states, associated with spatially structured absorption coefficients, which are defined by the geometry of the polarization state and the magnetic field direction. We illustrate this for a range of optical beams including polarization vortices, optical skyrmions, and polarization lattices. This results in a new interpretation and an enhanced understanding of atomic state interferometry, and a versatile mechanism to modify and control optical absorption as a function of polarization and magnetic field alignment.
复杂矢量光的特性在任何干涉效应中都很重要,包括散射、衍射和非线性过程。在这里,我们正在研究偏振结构光在原子态干涉仪中的作用。与光学或原子路径干涉仪不同,这些干涉仪促进了原子跃迁幅度之间的局部干涉,因此驱动这些跃迁的正交光学偏振分量。我们对广义结构光与原子四态系统的相互作用进行了充分的分析描述,即通过光学和磁跃迁多重连接。我们的模型允许我们识别空间依赖的暗态,与空间结构吸收系数相关,吸收系数由极化态的几何形状和磁场方向定义。我们举例说明了这一范围的光束,包括偏振涡旋,光学天空,和偏振晶格。这对原子态干涉测量学有了新的解释和更好的理解,并提供了一种修改和控制光吸收作为偏振和磁场对准函数的通用机制。
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引用次数: 0
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Nanophotonics
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