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Underestimation of particulate dry nitrogen deposition in China 中国颗粒干氮沉降的低估
IF 18.3 1区 地球科学 Q1 GEOSCIENCES, MULTIDISCIPLINARY Pub Date : 2026-01-02 DOI: 10.1038/s41561-025-01873-3
Qianru Zhang, Yuhang Wang, Maodian Liu, Young-Hee Ryu, Mingxu Liu, Huoqing Li, Si-Yi Wei, Junfeng Liu, Shu Tao, Xuejun Wang
Nitrogen is indispensable for global food production and ecosystem carbon sequestration, but excess nitrogen leads to water eutrophication, soil acidification and air pollution. Atmospheric nitrogen deposition is a key yet uncertain component of the biogeochemical cycle. Currently, global networks monitoring particulate nitrogen dry deposition rely mainly on measured concentrations and modelled dry deposition velocities, which remain poorly constrained. Here we develop a spatially explicit dataset by integrating observation-constrained size distribution and dry deposition mechanisms to re-evaluate atmospheric nitrogen deposition across China. We reveal that atmospheric chemistry models underestimate the particle size of fine-mode nitrogen-containing aerosols in China by more than twofold. Additionally, dry particle deposition velocity estimates with different mechanisms diverge by up to two orders of magnitude. Our corrections indicate that atmospheric chemistry models and China’s observation network underestimate particulate nitrogen dry deposition by 2–5 times. Furthermore, most Earth system models underestimate particulate dry deposition of ammonium, a major nitrogen species, by 31%–98%. By integrating these corrections into the Community Land Model, we demonstrate that the effect of nitrogen deposition on China’s terrestrial net ecosystem productivity may have been underestimated by 9%–13%. As China contributes nearly 20% of global nitrogen deposition, its impact on terrestrial carbon sinks and ecosystem health could be greater than previously recognized.
氮对于全球粮食生产和生态系统固碳是不可或缺的,但过量的氮会导致水体富营养化、土壤酸化和空气污染。大气氮沉降是生物地球化学循环的一个关键但不确定的组成部分。目前,监测颗粒氮干沉降的全球网络主要依赖于测量的浓度和模拟的干沉降速度,这些仍然缺乏约束。本文通过整合观测约束尺度分布和干沉降机制,构建空间显式数据集,重新评估中国大气氮沉降。我们发现大气化学模型低估了中国细态含氮气溶胶的粒径两倍以上。此外,不同机制下的干颗粒沉积速度估计相差可达两个数量级。我们的修正表明,大气化学模式和中国观测网络低估了颗粒氮干沉降的2-5倍。此外,大多数地球系统模型低估了铵的颗粒干沉积,这是一种主要的氮物种,低估了31%-98%。通过将这些修正整合到群落土地模型中,我们发现氮沉降对中国陆地生态系统净生产力的影响可能被低估了9%-13%。由于中国贡献了全球近20%的氮沉降,其对陆地碳汇和生态系统健康的影响可能比以前认识到的要大。
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引用次数: 0
Regionally distinct threats from polycyclic aromatic hydrocarbons in global reservoirs 全球储层中多环芳烃的区域性不同威胁
IF 18.3 1区 地球科学 Q1 GEOSCIENCES, MULTIDISCIPLINARY Pub Date : 2026-01-02 DOI: 10.1038/s41561-025-01872-4
Zhao-Feng Guo, Wiebke J. Boeing, Yao-Yang Xu, Edoardo Borgomeo, Othman A. Al-Mashaqbeh, Dong Liu, Xiao-Ru Yang
Polycyclic aromatic hydrocarbons pose inconsistent yet increasing threats to freshwater reservoirs worldwide, with implications for ecosystem health and water security. Although local-scale contamination has been widely documented, a comprehensive global synthesis of polycyclic aromatic hydrocarbon occurrence and drivers in reservoirs remains lacking. Here we developed a framework of data compilation, arrangement and statistics to integrate existing data to determine the geographical distribution and potential sources of polycyclic aromatic hydrocarbon pollution in reservoirs globally. Statistical analyses revealed spatial heterogeneity in dominant components and pollution levels across continents. Almost 38% of water samples exceeded an ecologically relevant threshold (0.20 μg l−1), and 42% of sediment samples surpassed the threshold effect concentration, indicating widespread ecological risks. Cluster analysis and source apportionment of the reservoir-level data identified three distinct polycyclic aromatic hydrocarbon patterns, each shaped by region-specific land-use practices, combustion sources and climatic factors. These findings emphasize and inform the need for region-specific monitoring and management strategies, such as expanding monitoring in subtropical and temperate regions, with a focus on polycyclic aromatic hydrocarbon accumulation in aquatic organisms.
多环芳烃对全球淡水水库的威胁虽不一致,但仍在不断增加,对生态系统健康和水安全产生影响。尽管局部污染已被广泛记录,但油藏中多环芳烃的分布及其驱动因素的综合全球合成仍然缺乏。在此基础上,建立了数据整理和统计框架,整合现有数据,确定全球储集层中多环芳烃污染的地理分布和潜在来源。统计分析揭示了各大洲主要成分和污染水平的空间异质性。近38%的水样超过了生态相关阈值(0.20 μg l−1),42%的沉积物样品超过了阈值效应浓度,表明存在广泛的生态风险。对储层数据进行聚类分析和源分配,确定了三种不同的多环芳烃模式,每种模式都受区域特定的土地利用实践、燃烧源和气候因素的影响。这些发现强调并告知需要采取特定区域的监测和管理策略,例如扩大在亚热带和温带地区的监测,重点关注水生生物中多环芳烃的积累。
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引用次数: 0
Spatially variable response of Antarctica’s ice sheets to orbital forcing during the Pliocene 上新世期间南极冰盖对轨道强迫的空间变化响应
IF 18.3 1区 地球科学 Q1 GEOSCIENCES, MULTIDISCIPLINARY Pub Date : 2026-01-02 DOI: 10.1038/s41561-025-01840-y
Molly O. Patterson, Christiana Rosenberg, Osamu Seki, Masanobu Yamamoto, Oscar E. Romero, Mei Nelissen, Francesca Sangiorgi, Nicholas R. Golledge, Georgia Grant, William D. Arnuk, Benjamin Keisling, Timothy Naish, Richard Levy, Stephen Meyers, Nicholas Sullivan, Jeanine Ash, Denise Kulhanek, Brian W. Romans, Natalia Varela Valenzuela, Harold Jones, Francois Beny, Imogen Browne, Giuseppe Cortese, Isobela M. C. Sousa, Justin P. Dodd, Oliver M. Esper, Jenny Gales, David Harwood, Saki Ishino, Sookwan Kim, Sunghan Kim, Jan S. Laberg, R. Mark Leckie, Juliane Müller, Amelia Shevenell, Shiv Singh, Saiko T. Sugisaki, Tina van de Flierdt, Tim van Peer, Wenshen Xiao, Zhifang Xiong, Laura De Santis, Robert McKay
Variations in Earth’s orbit pace global ice-volume and sea-level changes, but the variability in the response for different sectors of the Antarctic Ice Sheet to orbitally forced climate change remains unclear. Here we present geological records of iceberg-rafted debris and other proxies from locations adjacent to the West Antarctic Ice Sheet (WAIS) with comparisons to an existing East Antarctic Ice Sheet (EAIS) record over the time interval ~3.3–2.3 million years ago. Iceberg calving events from the WAIS recorded in Ross Sea sediment cores show a linear response to orbital forcing at timescales corresponding to obliquity (~40,000 years) and precession (~23,000–19,000 years) modulated by eccentricity (~100,000 years). This contrasts with an existing record adjacent to the EAIS, which does not contain obliquity pacing. Combined with ice-sheet model sensitivity tests, the geological data show that the WAIS is highly dynamic and responsive to oceanic melt driven by changes in Southern Ocean circulation, together with atmospheric forcing through variations in local insolation. Conversely, the EAIS appears less responsive to oceanic forcing, despite being the dominant source of meltwater to the global ocean during the mid-Pliocene. Our results imply a substantial role for atmospheric warming on mid-Pliocene sea-level from both WAIS and EAIS.
地球轨道的变化加快了全球冰量和海平面的变化,但南极冰盖不同部分对轨道强迫气候变化的响应的变化性尚不清楚。本文介绍了南极西部冰盖(WAIS)附近的冰山漂流碎片和其他代用品的地质记录,并将其与南极东部冰盖(EAIS)在330万至230万年前的记录进行了比较。罗斯海沉积物岩心中记录的WAIS冰山崩解事件显示出在时间尺度上对轨道强迫的线性响应,对应于倾角(~ 40000年)和岁差(~ 23000 - 19000年),由偏心率(~ 100000年)调制。这与EAIS附近的现有记录形成对比,该记录不包含倾斜起搏。结合冰盖模式敏感性试验,地质数据表明,WAIS是高度动态的,对由南大洋环流变化驱动的海洋融化以及通过局部日照变化产生的大气强迫具有响应性。相反,尽管EAIS在上新世中期是全球海洋融水的主要来源,但它对海洋强迫的反应似乎较弱。我们的研究结果表明,大气变暖对上新世中期海平面的影响是由WAIS和EAIS引起的。
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引用次数: 0
More intermittent mid-latitude precipitation accompanied extreme early Palaeogene warmth 更间歇性的中纬度降水伴随着古近纪早期的极端温暖
IF 18.3 1区 地球科学 Q1 GEOSCIENCES, MULTIDISCIPLINARY Pub Date : 2025-12-22 DOI: 10.1038/s41561-025-01870-6
Jacob S. Slawson, Piret Plink-Bjorklund, Thomas Reichler, Daniel Baldassare
Warming is pushing Earthʼs system towards unfamiliar climate conditions, complicating predictions. Geological archives of past greenhouse climates provide essential tests for models under extreme forcing. We investigate how precipitation responded to extreme warmth during early Palaeogene global warming events (66–47.8 million years ago)—a period considered a possible analogue for worst-case future scenarios. Here we compile global palaeoclimate data and develop a multi-proxy approach that integrates sedimentary proxies—such as plant fossils, ancient soils and river deposits—providing constraints on global precipitation intermittency (seasonal and interannual variability) and intensity (rainfall rate). The data reveal wet or monsoonal polar regions and aridity punctuated by intense rainfall at mid- and low-latitude continental interiors. This hydroclimate shift occurred 3 million years before and persisted 7 million years after the Palaeocene–Eocene Thermal Maximum—the warmest period of the Cenozoic Era, suggesting that extreme warmth induces nonlinearities in the hydrological cycle’s sensitivity to temperature increase. Polar humidity and mid-latitude aridity further indicate a departure from the expected wet-gets-wetter and dry-gets-drier response. Shifts towards aridity were decoupled from mean annual precipitation and driven by seasonal and interannual precipitation distribution, such as shorter wet-season lengths and longer interannual rainfall recurrence intervals. This highlights the importance of considering precipitation intermittency and intensity, as similar shifts may occur under future warming despite differences in boundary conditions.
气候变暖正将地球系统推向不熟悉的气候条件,使预测变得复杂。过去温室气候的地质档案为极端强迫下的模式提供了必要的检验。我们研究了在早期古近纪全球变暖事件(6660万- 4780万年前),降水是如何对极端温暖做出反应的——这一时期被认为是未来最坏情况的可能类比。在这里,我们汇编了全球古气候数据,并开发了一种多代理方法,该方法整合了沉积代理,如植物化石,古土壤和河流沉积物,提供了对全球降水间歇性(季节和年际变化)和强度(降雨率)的约束。数据显示,在中纬度和低纬度大陆内部,潮湿或季风性极地地区和干旱被强降雨打断。这种水文气候变化发生在古新世-始新世热最大值(新生代最温暖的时期)之前300万年,并持续到700万年之后,这表明极端的温暖导致了水文循环对温度升高的非线性敏感性。极地湿度和中纬度干旱进一步表明,与预期的“越湿越湿”和“越干越干”反应不同。干旱的变化与年平均降水不相关,而受季节和年际降水分布的驱动,如较短的雨季长度和较长的年际降水重现间隔。这突出了考虑降水间歇性和强度的重要性,因为尽管边界条件不同,在未来变暖的情况下也可能发生类似的变化。
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引用次数: 0
Autistic voices are an overlooked minority in geosciences 在地球科学领域,自闭症的声音是被忽视的少数
IF 18.3 1区 地球科学 Q1 GEOSCIENCES, MULTIDISCIPLINARY Pub Date : 2025-12-16 DOI: 10.1038/s41561-025-01882-2
Adam John Jeffery, Steven Leslie Rogers, Kelly Louise Ann Jeffery, Mark Lucherini, Jamie Keith Pringle, Martin Griffin
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引用次数: 0
Poleward migration of tropical cyclones over 1980–2024 is dominated by Pacific variability 1980-2024年热带气旋向极地迁移主要受太平洋变率影响
IF 18.3 1区 地球科学 Q1 GEOSCIENCES, MULTIDISCIPLINARY Pub Date : 2025-12-15 DOI: 10.1038/s41561-025-01866-2
Wenyu Zhou, L. Ruby Leung, Chuan-Chieh Chang, Ming Zhao, Huang-Hsiung Hsu, Hsin-Chien Liang, Chia-Ying Tu, Karthik Balaguru, Jian Lu
Since 1980, tropical cyclones have migrated poleward, but it remains unclear whether this trend reflects long-term climate change or temporary climate variability. Here we investigate the drivers of this poleward migration using multiple observational datasets and global models that permit tropical cyclones. We show that a tripolar pattern of Pacific sea surface temperature variability strongly modulates the interannual variation of cyclone latitudes and largely drove the poleward migration over 1980–2024. The tripolar pattern influences tropical cyclones more effectively than either the El Niño/Southern Oscillation or the Hadley circulation. When its effects are removed, poleward migration is negligible. When it shows negative trends, the model simulates equatorward migration. As the pattern exhibits alternating multi-decadal trends but no long-term trend since 1970, its recent trend—and the associated poleward migration—is unlikely to persist. In ensemble projections under a warming scenario, tropical cyclone activity decreases overall, leading to fewer occurrences at high latitudes despite the poleward expansion of the Hadley cell. These results indicate that climate variability has played a dominant role in the observed poleward migration of tropical cyclones, and that future changes may differ markedly from the recent multi-decadal trends.
自1980年以来,热带气旋向极地移动,但尚不清楚这种趋势是反映长期气候变化还是暂时气候变率。在这里,我们使用多个观测数据集和允许热带气旋的全球模式来研究这种向极地迁移的驱动因素。研究表明,1980-2024年太平洋海表温度变化的三极型强烈调节了气旋纬度的年际变化,并在很大程度上驱动了气旋向极地迁移。三极型对热带气旋的影响比厄尔Niño/南方涛动或哈德利环流更有效。当它的影响被消除时,向极地迁移是可以忽略不计的。当它呈现负趋势时,模型模拟向赤道迁移。由于这种模式显示出交替的多年代际趋势,但自1970年以来没有长期趋势,其最近的趋势——以及相关的极地迁移——不太可能持续下去。在变暖情景下的总体预估中,热带气旋活动总体减少,导致高纬度地区的发生次数减少,尽管哈德利环流向极地扩展。这些结果表明,气候变率在观测到的热带气旋向极地迁移中起主导作用,未来的变化可能与最近的多年代际趋势有显著差异。
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引用次数: 0
Sedimentary conditions drive modern pyrite burial flux to exceed oxidation 沉积条件驱使现代黄铁矿埋藏通量超过氧化
IF 18.3 1区 地球科学 Q1 GEOSCIENCES, MULTIDISCIPLINARY Pub Date : 2025-12-12 DOI: 10.1038/s41561-025-01855-5
Cornelia Mertens, Sarah Paradis, Jordon D. Hemingway
Pyrite (iron sulfide) formation and burial in sediments decreases atmospheric CO2 and increases O2 levels. However, the environmental and sedimentological conditions that regulate pyrite burial remain poorly constrained. Here we investigate such controlling mechanisms using a non-dimensional diagenetic model that extracts the natural variables governing pyrite formation rate and sulfur isotopic composition (δ34S). Both properties are controlled by the local ratios of organic carbon content to sulfate concentration and organic carbon reactivity to sedimentation rate; formation rate is additionally sensitive to reactive iron delivery. Using only globally interpolated boundary conditions, our model accurately predicts signals in 216 sediment cores distributed across the modern ocean. Extrapolating this, we estimate a global pyrite burial flux of 7.0 × 1012 mol S yr−1 (sensitivity test range: 2.5 × 1012 to 19.0 × 1012 mol S yr−1) with a weighted-average δ34S value of −4‰ (range: −8 to +3‰). This flux is substantially larger than terrestrial pyrite oxidation, indicating that the sulfur cycle is currently not in steady state but is instead described by net pyrite burial and thus atmospheric O2 accumulation. Finally, we interpret the geologic pyrite δ34S record within this model framework and identify flooded shelf area as the main control on pyrite burial throughout the Phanerozoic Eon.
沉积物中黄铁矿(硫化铁)的形成和埋藏减少了大气中的二氧化碳,增加了氧气水平。然而,控制黄铁矿埋藏的环境和沉积条件仍然知之甚少。本文采用无量纲成岩模型,提取控制黄铁矿形成速率和硫同位素组成(δ34S)的自然变量,研究这种控制机制。这两种性质均受局部有机碳含量与硫酸盐浓度之比和有机碳反应性与沉降速率之比的控制;形成速率对活性铁的输送也很敏感。仅使用全球插值的边界条件,我们的模型准确地预测了分布在现代海洋中的216个沉积物岩心的信号。据此推断,我们估计全球黄铁矿埋藏通量为7.0 × 1012 mol S yr - 1(灵敏度测试范围:2.5 × 1012 ~ 19.0 × 1012 mol S yr - 1),加权平均δ34S值为−4‰(范围:−8 ~ +3‰)。这一通量大大大于陆地黄铁矿氧化,表明硫循环目前不是处于稳定状态,而是由净黄铁矿埋藏和大气O2积累来描述。最后,在此模式框架内对黄铁矿δ34S的地质记录进行了解释,确定了显生宙黄铁矿埋藏的主要控制因素为水淹陆架。
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引用次数: 0
Southern Ocean net primary production influenced by seismically modulated hydrothermal iron 地震调节热液铁对南大洋净初级产量的影响
IF 18.3 1区 地球科学 Q1 GEOSCIENCES, MULTIDISCIPLINARY Pub Date : 2025-12-09 DOI: 10.1038/s41561-025-01862-6
Casey M. S. Schine, Jens-Erik Lund Snee, Alex Lyford, Gert van Dijken, Kevin R. Arrigo
Iron is the primary limiting nutrient for phytoplankton growth, and consequently CO2 drawdown, in the Southern Ocean. A recurring phytoplankton bloom above the Australian Antarctic Ridge was recently attributed to hydrothermally sourced iron. Here we examine satellite remote-sensing estimates of net primary production, earthquake location catalogues and Lagrangian plume modelling of particle trajectories in surface ocean currents to show that interannual variability in net primary production is related to seismicity and the advective spread of downstream surface waters. By spatially decomposing the relationship between seismicity, advective spread and net primary production, we demonstrate that net primary production at the surface, above the hydrothermal vents, can be predicted by elevated seismicity in the months before the growing season. Farther from the vents, greater advective spread reduces net primary production. We hypothesize that the connection between earthquakes and net primary production is mediated by the link between seismicity and hydrothermal emissions while advective spread controls the dilution of entrained iron; however, the physical mechanism behind the rapid surfacing of hydrothermal iron is still unknown. These findings challenge prevailing views on how geophysical processes influence ocean primary production.
铁是南大洋浮游植物生长的主要限制性营养物质,因此也限制了二氧化碳的减少。最近,澳大利亚南极脊上空浮游植物的反复繁殖被归因于热液来源的铁。本文研究了卫星遥感估算的净初级产量、地震定位目录和表面洋流粒子轨迹的拉格朗日羽流模型,以表明净初级产量的年际变化与地震活动性和下游地表水的平流扩散有关。通过空间分解地震活动性、平流扩散和净初级产量之间的关系,我们证明了热液喷口上方地表的净初级产量可以通过生长季节前几个月的地震活动性升高来预测。离喷口越远,平流扩散越大,净初级产量就越低。我们假设地震和净初级产量之间的联系是由地震活动性和热液排放之间的联系介导的,而平流扩散控制了夹带铁的稀释;然而,热液中铁快速表面的物理机制尚不清楚。这些发现挑战了关于地球物理过程如何影响海洋初级生产的主流观点。
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引用次数: 0
Refining the crust 精炼外壳
IF 16.1 1区 地球科学 Q1 GEOSCIENCES, MULTIDISCIPLINARY Pub Date : 2025-12-08 DOI: 10.1038/s41561-025-01865-3
Simon L. Harley
Heat-producing elements like uranium and thorium are depleted in the lower crust. The geochemistry of crustal rocks suggests ultrahigh melting temperatures are needed to produce this depletion and may also help stabilize the crust.
像铀和钍这样的产热元素在地壳下部被耗尽。地壳岩石的地球化学表明,需要超高的熔化温度来产生这种消耗,这也可能有助于稳定地壳。
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引用次数: 0
Tightening the Sargassum belt 收紧马尾藻带
IF 16.1 1区 地球科学 Q1 GEOSCIENCES, MULTIDISCIPLINARY Pub Date : 2025-12-08 DOI: 10.1038/s41561-025-01886-y
A belt of seaweed has formed across the tropical Atlantic nearly every year since 2011, despite reduction in its extent elsewhere. The causes of this growth are now coming into clearer focus.
自2011年以来,几乎每年都会在热带大西洋上形成一条海藻带,尽管其他地方的海藻带面积有所减少。这种增长的原因现在变得越来越清晰。
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引用次数: 0
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