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Low-smoke fuels for residential heating linked to an increase in ultrafine particle emissions 住宅供暖用低烟燃料与超细颗粒物排放增加有关
IF 18.3 1区 地球科学 Q1 GEOSCIENCES, MULTIDISCIPLINARY Pub Date : 2026-03-02 DOI: 10.1038/s41561-026-01942-1
Chunshui Lin, Darius Ceburnis, Anna Trubetskaya, Lu Lei, Shan Wang, Yi Liu, Wei Yuan, Haitao Cui, William Smith, Robert Johnson, Kirsten N. Fossum, Vasily Lebedev, Vincent Carré, Rory F. D. Monaghan, Douglas Worsnop, Lidia Morawska, Tao Wang, Ru-Jin Huang, Colin O’Dowd, Jurgita Ovadnevaite
Despite national variations, current air quality standards worldwide focus on reducing mass concentrations of atmospheric particulate matter to lower public health risks. However, these standards fall short in addressing the adverse health effects associated with ultrafine particles, which can penetrate deeper into the human lungs and even pass the blood–brain barrier. Here we present experimental, model and field data in addition to a lung deposition analysis to show there is a rise in ultrafine particle resulting from the transition to ‘low-smoke’ fuels in the residential sector. These low-smoke fuels, designed to lower particulate mass emissions, have unexpectedly led to a two-to-threefold increase in the emissions of ultrafine particle numbers, resulting in a higher contribution to lung deposition particles than all their smoky counterparts combined. Current air quality models underestimate ultrafine particles by a factor of ten, suggesting an underestimation of the health impacts when only particle mass was considered. These ultrafine particle events contrast sharply with the haze events that typically involve larger accumulation mode particles. Our findings highlight the urgent need to revise air quality standards to include ultrafine particles, ensuring air quality management strategies reduce mass concentration without the cost of increasing ultrafine particle number.
尽管各国存在差异,但目前世界各地的空气质量标准侧重于降低大气颗粒物的质量浓度,以降低公共健康风险。然而,这些标准不足以解决与超细颗粒有关的不良健康影响,超细颗粒可以深入人体肺部,甚至通过血脑屏障。在这里,我们提供了实验、模型和现场数据以及肺沉积分析,以表明住宅部门过渡到“低烟”燃料导致超细颗粒增加。这些旨在降低颗粒质量排放的低烟燃料,出人意料地导致超细颗粒排放量增加了两到三倍,导致肺部沉积颗粒的贡献高于所有烟雾颗粒的总和。目前的空气质量模型将超细颗粒低估了十倍,这表明,如果只考虑颗粒质量,就低估了对健康的影响。这些超细颗粒事件与通常涉及较大积聚模式颗粒的雾霾事件形成鲜明对比。我们的研究结果强调,迫切需要修订空气质量标准,将超细颗粒包括在内,确保空气质量管理策略在不增加超细颗粒数量的情况下降低质量浓度。
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引用次数: 0
Overlooked bedload transport in Himalayan rivers threatens regional security 喜马拉雅河流中被忽视的河床搬运威胁着地区安全
IF 16.1 1区 地球科学 Q1 GEOSCIENCES, MULTIDISCIPLINARY Pub Date : 2026-03-02 DOI: 10.1038/s41561-026-01927-0
Zheng Chen, Dieter Rickenmann, Alexandre Badoux, Siming He, Xixi Lu
Bedload transport in high Himalayan rivers has been overlooked, hindering the development of morphodynamic models that explicitly couple river hydraulics, sediment transport, and channel morphology to predict responses to extreme floods under global warming. This knowledge gap increases risks to regional hydropower, ecosystems, and food security.
高海拔喜马拉雅河流的河床输运一直被忽视,这阻碍了形态动力学模型的发展,这些模型明确地将河流水力学、泥沙输运和河道形态结合起来,以预测全球变暖下极端洪水的响应。这种知识差距增加了对区域水电、生态系统和粮食安全的风险。
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引用次数: 0
Publisher Correction: Early Pleistocene ecosystem turnover in South Siberia linked to abrupt regional cooling 出版者更正:西伯利亚南部早更新世生态系统更替与区域突然变冷有关
IF 16.1 1区 地球科学 Q1 GEOSCIENCES, MULTIDISCIPLINARY Pub Date : 2026-02-27 DOI: 10.1038/s41561-026-01946-x
Joseph B. Novak, Alexander A. Prokopenko, Pavel E. Tarasov, James M. Russell, Emma R. Lindemuth, Koji Shichi, Kenji Kashiwaya, John Peck, Richard S. Vachula, George E. A. Swann, Pratigya J. Polissar
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引用次数: 0
Daily variations of carbon, nitrogen and oxygen ions in a thin lunar atmosphere 月球稀薄大气中碳、氮、氧离子的日常变化
IF 18.3 1区 地球科学 Q1 GEOSCIENCES, MULTIDISCIPLINARY Pub Date : 2026-02-27 DOI: 10.1038/s41561-026-01933-2
Kentaro Terada, Ryusei Nishihira, Shoichiro Yokota, Yoshifumi Saito, Kazushi Asamura, Masaki N. Nishino, Shota Notsu
The giant impact hypothesis, generally considered as the origin of the Moon, predicts a dry Moon lacking volatile elements, but in situ observations provide evidence that volatile elements such as carbon, nitrogen and oxygen are stored on the lunar surface and are being supplied to its exosphere. Such volatile sources and dynamics remain poorly understood. Here we investigate the chemical composition and time variations in the lunar exosphere using an ion mass analyser onboard the Kaguya satellite. We reported sporadic changes in the C+/O+ ratio occurring immediately after meteoroid showers. We also observed daily variations in the C+/O+ and N+/O+ ion ratios, suggesting two possible sources: a nitrogen-rich reservoir with a higher N/C ratio than the solar value or N-free CO/CO2 gases. Our findings indicate that the mechanism for the production of C+, N+ and O+ ions during the daytime is solar wind sputtering—ejection through collision with solar wind particles—of the nitrogen-rich reservoir, whereas micrometeoroid impacts and photoionization are not dominant processes. We propose that the nitrogen-rich regolith reported in Apollo samples and indigenous volcanic gases constitute the source of volatile ions in a thin lunar atmosphere.
大碰撞假说,通常被认为是月球的起源,预测一个干燥的月球缺乏挥发性元素,但现场观测提供的证据表明,挥发性元素,如碳、氮和氧,储存在月球表面,并被供应给它的外逸层。这种不稳定的来源和动态仍然知之甚少。在这里,我们研究了化学成分和时间变化在月球外逸层使用离子质量分析仪的月亮卫星上。我们报告了流星雨后C+/O+比值的零星变化。我们还观察到C+/O+和N+/O+离子比的日变化,提出了两种可能的来源:N/C比高于太阳值的富氮水库或无N的CO/CO2气体。我们的研究结果表明,白天产生C+, N+和O+离子的机制是太阳风溅射-通过与太阳风粒子的碰撞喷射-富氮库,而微流星体撞击和光电离不是主导过程。我们提出,阿波罗号样品中报告的富氮风化层和本地火山气体构成了稀薄月球大气中挥发性离子的来源。
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引用次数: 0
Pervasive underreporting of harmful field interactions hampers intervention efforts 普遍漏报有害的现场相互作用妨碍了干预工作
IF 16.1 1区 地球科学 Q1 GEOSCIENCES, MULTIDISCIPLINARY Pub Date : 2026-02-24 DOI: 10.1038/s41561-026-01930-5
Maya Almaraz, Melisa A. Diaz, Anne U. Gold
Harmful interactions are prevalent in geoscience fieldwork but often go unreported, hindering efforts to build welcoming and collaborative field cultures.
有害的相互作用在地球科学实地工作中很普遍,但往往没有被报道,阻碍了建立欢迎和合作的实地文化的努力。
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引用次数: 0
Nitrogen management to achieve China’s Sustainable Development Goals 氮管理助力中国实现可持续发展目标
IF 16.1 1区 地球科学 Q1 GEOSCIENCES, MULTIDISCIPLINARY Pub Date : 2026-02-23 DOI: 10.1038/s41561-026-01919-0
Binhui Chen, Xiuming Zhang, Baojing Gu
Nitrogen, serving as both a vital nutrient and a potent pollutant, has an important role in the pursuit of global Sustainable Development Goals (SDGs). However, the comprehensive impact of nitrogen on SDG achievement remains relatively unclear. Here we utilize the Coupled Human and Natural Systems (CHANS) model to build a framework for assessing the influence of nitrogen on SDGs in China during 2020. Our analysis reveals that nitrogen use and loss in China affect 11 out of the 17 SDGs, with notable regional disparities. In general, regions with higher economic development perform better in the nitrogen-related SDG (SDG-N) scores within the economy dimension, but score lower in the society and environment dimensions. Our simulations indicate that comprehensive nitrogen management is crucial to foster synergy among SDGs, which could enhance SDG-N index scores in China by 8–26%, resulting in substantial national benefits, including US$162 billion (US$98–208 billion) in savings on fertilizer and food imports, increased agricultural yields, improved public health, enhanced ecosystem resilience and climate mitigation. Importantly, these benefits can be achieved with a modest net implementation cost of only US$34 billion (US$27–41 billion), making it a cost-effective and sustainable solution for advancing China’s SDG agenda. A framework assessing the impact of nitrogen on China’s SDGs reveals effects on 11 out of the 17 SDG goals in 2020, with regional disparities. This highlights the need for revised economic strategies to improve nitrogen management.
氮既是一种重要的营养物质,也是一种强有力的污染物,在实现全球可持续发展目标(sdg)方面发挥着重要作用。然而,氮对实现可持续发展目标的综合影响仍相对不清楚。本文利用人类与自然系统耦合(CHANS)模型构建了2020年氮肥对中国可持续发展目标影响的评估框架。我们的分析表明,中国的氮利用和损失影响了17个可持续发展目标中的11个,且存在显著的区域差异。总体而言,经济发展水平较高的地区在经济维度氮相关可持续发展目标(SDG- n)得分较高,但在社会和环境维度得分较低。我们的模拟表明,综合氮管理对于促进可持续发展目标之间的协同作用至关重要,它可以将中国的可持续发展目标n指数得分提高8-26%,从而带来可观的国家效益,包括节省1620亿美元(980 - 2080亿美元)的化肥和粮食进口、提高农业产量、改善公共健康、增强生态系统恢复力和减缓气候变化。重要的是,实现这些效益的净实施成本仅为340亿美元(270 - 410亿美元),这使其成为推进中国可持续发展议程的具有成本效益和可持续的解决方案。一个评估氮对中国可持续发展目标影响的框架显示,到2020年,氮对17个可持续发展目标中的11个目标的影响存在地区差异。这突出表明需要修订经济战略以改善氮的管理。
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引用次数: 0
Millennial-aged peat carbon outgassed by large humic lakes in the Congo Basin 刚果盆地的大型腐殖质湖泊排出了千年泥炭碳
IF 18.3 1区 地球科学 Q1 GEOSCIENCES, MULTIDISCIPLINARY Pub Date : 2026-02-23 DOI: 10.1038/s41561-026-01924-3
Travis W. Drake, Jordon D. Hemingway, Matti Barthel, Antoine de Clippele, Negar Haghipour, Jose N. Wabakanghanzi, Kristof Van Oost, Johan Six
Congo Basin lakes Mai Ndombe and Tumba are major CO 2 sources. Here we show that their dissolved inorganic carbon is some 2,170–3,515 14 C years old and partially (39–40%) originates from the surrounding peatlands. This implies a loss pathway for peat carbon, in which microbes respire old carbon within the peat and the resulting CO 2 is transported to the lakes and outgassed, linking these immense ancient stores to the modern carbon cycle.
刚果盆地的迈恩东贝湖和通巴湖是二氧化碳的主要来源。在这里,我们发现它们溶解的无机碳大约有2170 - 3515 - 14 C的历史,部分(39-40%)来自周围的泥炭地。这意味着泥炭碳的损失途径,其中微生物呼吸泥炭中的旧碳,产生的二氧化碳被输送到湖泊并排出气体,将这些巨大的古代储存与现代碳循环联系起来。
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引用次数: 0
Climate feedback of forest fires amplified by atmospheric chemistry 森林火灾的气候反馈被大气化学放大
IF 18.3 1区 地球科学 Q1 GEOSCIENCES, MULTIDISCIPLINARY Pub Date : 2026-02-19 DOI: 10.1038/s41561-026-01926-1
Wei Chen, Yuzhong Zhang, Yufei Zou, Zhen Zhang
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引用次数: 0
Urban black-carbon radiative heating intensified by biogenic–anthropogenic interactions 生物-人为相互作用加剧了城市黑碳辐射加热
IF 18.3 1区 地球科学 Q1 GEOSCIENCES, MULTIDISCIPLINARY Pub Date : 2026-02-13 DOI: 10.1038/s41561-026-01922-5
Yunjiang Zhang, Shijie Cui, Jingyi Li, Ming Wang, Xiaofeng Xu, Jiandong Wang, Jie Fang, Hanrui Lang, Bo Zheng, Sheng Zhong, Peng Sun, Haiwei Li, Yun Wu, Jianlin Hu, Junfeng Wang, Mindong Chen, Olivier Favez, Didier Hauglustaine, Philippe Ciais, Kaspar R. Daellenbach, André S. H. Prévôt, Xinlei Ge
Black carbon is a global climate forcer due to its strong radiative absorption, which is highly sensitive to coating formation regulated by anthropogenic and biogenic emissions. However, how cross-regional biogenic sources modulate urban black carbon coating and radiative effects remains poorly understood. Here we integrate observations and model simulations to investigate such biogenic–anthropogenic interactions in eastern China. The results show that biogenic volatile organic compounds from vegetation-rich regions undergo atmospheric oxidation to produce oxygenated organic compounds, which are subsequently advected into downwind urban areas. These products enhance regional atmospheric oxidation capacity and supply additional precursors, thereby promoting secondary organic aerosol production. This biogenic-induced strengthening of regional photochemistry drives the formation of highly oxidized secondary organic aerosol coatings on black carbon and increases its fraction within the total particle population. Consequently, black carbon absorption efficiency increases more steeply with the coating carbon oxidation state under biogenic-rich conditions, yielding an average ~20% enhancement in radiative absorption from the lensing effect relative to biogenic-poor periods. Our findings reveal that cross-regional biogenic–anthropogenic interactions enhance both the formation and particle population fraction of secondary organic aerosol coatings on urban black carbon, potentially further amplifying its radiative effects as biogenic emissions increase under future warming scenarios.
黑碳具有很强的辐射吸收性,对人为和生物源排放调节的涂层形成高度敏感,是全球气候的驱动因素。然而,跨区域生物源如何调节城市黑碳涂层和辐射效应仍然知之甚少。在此,我们结合观测和模式模拟来研究中国东部这种生物-人为相互作用。结果表明,来自植被丰富地区的生物源性挥发性有机化合物经过大气氧化生成含氧有机化合物,随后平流到下风城区。这些产品增强了区域大气氧化能力,并提供了额外的前体,从而促进了二次有机气溶胶的生产。这种生物诱导的区域光化学强化驱动了黑碳上高度氧化的二次有机气溶胶涂层的形成,并增加了其在总粒子群中的比例。因此,在生物源丰富的条件下,黑碳吸收效率随着涂层碳氧化状态的增加而急剧增加,相对于生物源贫乏的时期,透镜效应导致的辐射吸收平均提高了约20%。我们的研究结果表明,跨区域的生物-人为相互作用增强了城市黑碳上的二次有机气溶胶涂层的形成和粒子种群比例,在未来变暖情景下,随着生物源排放的增加,可能进一步放大其辐射效应。
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引用次数: 0
Multi-year La Niña–El Niño transition influenced Earth’s extreme energy uptake in 2022–2023 多年的La Niña-El Niño转变影响了地球在2022-2023年的极端能量吸收
IF 18.3 1区 地球科学 Q1 GEOSCIENCES, MULTIDISCIPLINARY Pub Date : 2026-02-12 DOI: 10.1038/s41561-026-01921-6
Ko Tsuchida, Yu Kosaka, Shoshiro Minobe
Earth’s energy uptake—defined as the global mean net incoming radiation at the top of the atmosphere—surged in 2022–2023, contributing to record global surface temperatures and widespread climate extremes in 2023–2024. Yet, the causes of this extreme energy uptake remain unclear, reflecting limited knowledge of how internal climate variability shapes Earth’s energy imbalance. Here we investigate the drivers of the observed extreme energy uptake by using multi-model climate simulations and satellite-based observations. We show that the transition from the multi-year La Niña to El Niño was key to Earth’s extreme energy uptake in 2022–2023, upon the externally forced positive imbalance. Our sampling analyses from the multi-model simulation dataset highlight the dominant influence of the La Niña-to-El Niño sequence on enhanced energy uptake, with crucial importance of multi-year persistence in preceding La Niña. When combined with estimates of the externally forced component derived under Shared Socio-economic Pathway scenarios, the contribution associated with the La Niña-to-El Niño transition explains about 75% of the observed extreme energy uptake. Our finding underscores the role of internal climate variability in shaping Earth’s energy budget and its potential amplification under a warming climate.
地球的能量吸收(定义为大气顶部的全球平均净入射辐射)在2022-2023年激增,导致2023-2024年创纪录的全球地表温度和广泛的极端气候。然而,这种极端能量吸收的原因仍然不清楚,反映了对内部气候变化如何影响地球能量不平衡的有限了解。本文通过多模式气候模拟和卫星观测,探讨了观测到的极端能量吸收的驱动因素。我们发现,在外部强迫的正不平衡下,从多年La Niña到El Niño的转变是地球在2022-2023年极端能量吸收的关键。我们对多模式模拟数据集的抽样分析强调了La Niña-to-El Niño序列对增强能量吸收的主要影响,其中La Niña之前的多年持续性至关重要。当与共享社会经济路径情景下的外部强迫分量估算相结合时,与La Niña-to-El Niño转变相关的贡献解释了观测到的极端能量摄取的75%左右。我们的发现强调了内部气候变化在塑造地球能量收支方面的作用,以及在气候变暖的情况下其潜在的放大作用。
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引用次数: 0
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Nature Geoscience
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