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Weather-sensitive renewable energy sources do not subject power systems to blackouts 对天气敏感的可再生能源不会导致电力系统停电
IF 56.7 1区 材料科学 Q1 ENERGY & FUELS Pub Date : 2024-10-21 DOI: 10.1038/s41560-024-01657-w
Power grids with high penetration of weather-dependent renewable energy sources (WD-RESs) tend to have reduced blackout intensities and weather vulnerability. WD-RESs such as wind and solar are not responsible for the occurrence of blackouts in bad weather conditions.
依赖天气的可再生能源(WD-RES)渗透率高的电网往往会降低停电强度和天气脆弱性。风能和太阳能等依赖天气的可再生能源不会造成恶劣天气条件下的停电。
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引用次数: 0
Producing methane through organocatalysis 通过有机催化生产甲烷
IF 56.7 1区 材料科学 Q1 ENERGY & FUELS Pub Date : 2024-10-21 DOI: 10.1038/s41560-024-01656-x
Fei Li, Mei Wang
Electrochemical reduction of carbon dioxide to fuels and chemicals is usually mediated by metal-based catalysts. Now, a carbon electrode modified with an organic molecular catalyst demonstrates promising activity and selectivity for carbon dioxide electroreduction to methane via an unusual pathway.
通过电化学方法将二氧化碳还原成燃料和化学品,通常需要使用金属催化剂。现在,一种经有机分子催化剂修饰的碳电极显示出良好的活性和选择性,可通过一种不寻常的途径将二氧化碳电还原成甲烷。
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引用次数: 0
Impacts of renewable energy resources on the weather vulnerability of power systems 可再生能源对电力系统天气脆弱性的影响
IF 56.7 1区 材料科学 Q1 ENERGY & FUELS Pub Date : 2024-10-21 DOI: 10.1038/s41560-024-01652-1
Jin Zhao, Fangxing Li, Qiwei Zhang

The high penetration of weather-dependent renewable energy sources (WD-RESs) such as wind and solar has raised concerns about the security of electric power systems during abnormal weather conditions. The role of RESs has been discussed in worldwide blackout events, yet remains controversial. In this study, we find that although WD-RESs are non-dispatchable and weather sensitive, blackout intensities and extreme weather vulnerability are mitigated in high-penetration WD-RES grids. The causal effects of WD-RESs on blackouts generally decrease in high-penetration WD-RES power systems, and WD-RESs are not mainly responsible for the occurrence of blackouts in extreme weather conditions. The results of our research contribute to the debate on RES integration and power system security, offer a guide for the study of power system resilience and provide a reference for the ambitious high-penetration RES goals of the future.

风能和太阳能等依赖天气的可再生能源(WD-RES)的高渗透率引发了人们对异常天气条件下电力系统安全性的担忧。可再生能源在全球停电事件中的作用已被讨论过,但仍存在争议。在本研究中,我们发现尽管可再生能源不可调度且对天气敏感,但在高渗透率的可再生能源电网中,停电强度和极端天气脆弱性得到了缓解。在高渗透率 WD-RES 电力系统中,WD-RES 对停电的因果效应普遍降低,WD-RES 并不是极端天气条件下发生停电的主要原因。我们的研究成果有助于关于可再生能源整合和电力系统安全的讨论,为电力系统弹性研究提供了指导,并为未来雄心勃勃的高渗透率可再生能源目标提供了参考。
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引用次数: 0
A bending test protocol for characterizing the mechanical performance of flexible photovoltaics 用于鉴定柔性光伏机械性能的弯曲测试协议
IF 56.7 1区 材料科学 Q1 ENERGY & FUELS Pub Date : 2024-10-18 DOI: 10.1038/s41560-024-01651-2
Kenjiro Fukuda, Lulu Sun, Baocai Du, Masahito Takakuwa, Jiachen Wang, Takao Someya, Lluis F. Marsal, Yinhua Zhou, Yiwang Chen, Hongzheng Chen, S. Ravi P. Silva, Derya Baran, Luigi A. Castriotta, Thomas M. Brown, Changduk Yang, Weiwei Li, Anita W. Y. Ho-Baillie, Thomas Österberg, Nitin P. Padture, Karen Forberich, Christoph J. Brabec, Osbel Almora

Flexible photovoltaic (PV) devices are a promising research field with potential for wearable, portable, indoor and internet-of-things applications. Substantial progress has been made in recent years, with flexible emerging PVs reporting power conversion efficiencies (PCEs) of over 24%. Yet, there is a need for a unifying protocol to assess PV performance, compare research results, and evaluate state-of-the-art achievements in flexible PVs. Here we present a protocol for measuring PCE over 1,000 bending cycles under 1% strain. Moreover, several good practice guidelines are proposed, including those related to bending procedures, flexibility testing with and without encapsulation, and ambient conditions during testing (for example, temperature, humidity and illumination). Notably, the importance of the uniform application of the bending radius and the testing of parallel and perpendicular orientations of the bending axis with respect to the direction of the electric current are emphasized. These recommendations aim to promote consistency in device comparison and allow for better reproducibility.

柔性光伏(PV)设备是一个前景广阔的研究领域,在可穿戴、便携、室内和物联网应用方面具有潜力。近年来,柔性新兴光伏技术取得了长足进步,其功率转换效率(PCE)超过了 24%。然而,我们需要一个统一的协议来评估光伏性能、比较研究成果并评估柔性光伏的最新成就。在此,我们提出了一个在 1%应变下进行 1000 次弯曲循环的 PCE 测量协议。此外,我们还提出了若干良好实践指南,包括与弯曲程序、有无封装的柔性测试以及测试期间的环境条件(如温度、湿度和光照)相关的指南。值得注意的是,该指南强调了统一使用弯曲半径以及测试弯曲轴相对于电流方向的平行和垂直方向的重要性。这些建议旨在促进设备比较的一致性,并实现更好的可重复性。
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引用次数: 0
Exploring the cost and emissions impacts, feasibility and scalability of battery electric ships 探索电池电动船舶的成本和排放影响、可行性和可扩展性
IF 56.7 1区 材料科学 Q1 ENERGY & FUELS Pub Date : 2024-10-14 DOI: 10.1038/s41560-024-01655-y
Hee Seung Moon, Won Young Park, Thomas Hendrickson, Amol Phadke, Natalie Popovich

The United States’ greenhouse gas (GHG) emissions reduction goals, along with targets set by the International Maritime Organization, create an opportunity for battery electric shipping. In this study, we model life-cycle costs and GHG emissions from shipping electrification, leveraging ship activity datasets from across the United States in 2021. We estimate that retrofitting 6,323 domestic ships under 1,000 gross tonnage to battery electric vessels would reduce US domestic shipping GHG emissions by up to 73% by 2035 from 2022 levels. By 2035, electrifying up to 85% of these ships could become cost effective versus internal combustion engine ships if they cover 99% of annual trips and charge from a deeply decarbonized grid. We find that charging demands from electrifying these ships could be concentrated at just 20 of 150 major ports nationwide. This study demonstrates that retrofitting to battery electric vessels has economic potential and could significantly accelerate GHG emission reductions.

美国的温室气体(GHG)减排目标以及国际海事组织设定的目标为电池电动航运创造了机遇。在本研究中,我们利用 2021 年全美船舶活动数据集,对航运电气化的生命周期成本和温室气体排放进行了建模。我们估计,将 6,323 艘总吨位在 1,000 吨以下的国内船舶改装为电池电动船,到 2035 年,美国国内航运业的温室气体排放量将比 2022 年的水平最多减少 73%。到 2035 年,与内燃机船舶相比,如果这些船舶的电气化覆盖 99% 的年航程,并通过深度去碳化的电网充电,那么这些船舶中高达 85% 的电气化船舶将具有成本效益。我们发现,在全国 150 个主要港口中,这些船舶电气化后的充电需求可能只集中在 20 个港口。这项研究表明,改装为电池电动船具有经济潜力,并能显著加快温室气体减排速度。
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引用次数: 0
Raising the bar for breakdown 提高故障处理标准
IF 49.7 1区 材料科学 Q1 ENERGY & FUELS Pub Date : 2024-10-14 DOI: 10.1038/s41560-024-01650-3
Erkan Aydin
Perovskite solar cells can be damaged when partially shaded, owing to currents flowing in reverse. Two research groups have now increased the breakdown voltage of the perovskite devices (the tolerance against this reverse bias degradation), one by using multilayer charge-selective contact stacks on the cathode side, and the other by using relatively thick, dense electrodes on the anode side.
由于电流反向流动,过氧化物太阳能电池在部分遮光的情况下会受到损坏。目前,两个研究小组已经提高了过氧化物设备的击穿电压(对这种反向偏压衰减的耐受能力),一个小组在阴极侧使用了多层电荷选择性接触堆,另一个小组在阳极侧使用了相对较厚的致密电极。
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引用次数: 0
Geospatial variation in carbon accounting of hydrogen production and implications for the US Inflation Reduction Act 制氢碳核算的地理空间差异及对《美国通货膨胀削减法》的影响
IF 56.7 1区 材料科学 Q1 ENERGY & FUELS Pub Date : 2024-10-14 DOI: 10.1038/s41560-024-01653-0
Valeria Vallejo, Quoc Nguyen, Arvind P. Ravikumar

Low-carbon hydrogen is considered a key component of global energy system decarbonization strategy. The US Inflation Reduction Act incentivizes low-carbon hydrogen production through tax credits that vary based on life-cycle greenhouse gas emissions intensity of hydrogen. Blue hydrogen or hydrogen produced from natural gas coupled with carbon capture and sequestration is one such pathway. Here we develop a geospatial, measurement-informed model to estimate supply-chain specific life-cycle greenhouse gas emissions intensity of blue hydrogen produced with natural gas sourced from the Marcellus and Permian shale basins. We find that blue hydrogen production using Permian gas has a life-cycle emissions intensity of 7.4‚Äâkg‚Äâcarbon dioxide equivalent per kg hydrogen (kgCO2e‚Äâkg‚àí1‚ÄâH2), more than twice that of hydrogen produced using Marcellus gas of 3.3‚ÄâkgCO2e‚Äâkg‚àí1‚ÄâH2. Eligibility for tax credits should therefore be based on life-cycle assessments that are supply-chain specific and measurement informed to ensure blue hydrogen projects are truly low carbon.

低碳氢被认为是全球能源系统去碳化战略的关键组成部分。美国《减少通货膨胀法》通过税收减免激励低碳氢气生产,税收减免根据氢气的生命周期温室气体排放强度而有所不同。蓝色氢气或利用天然气生产的氢气与碳捕集与封存技术相结合,就是这样一种途径。在此,我们开发了一个地理空间测量模型,以估算利用马塞勒斯和二叠纪页岩盆地的天然气生产蓝氢的供应链特定生命周期温室气体排放强度。我们发现,使用二叠纪天然气生产的蓝色氢气的生命周期排放强度为每千克氢气 7.4 千克二氧化碳当量(kgCO2e'Äâkg'àí1'ÄâH2),是使用马塞勒斯天然气生产的氢气 3.3 千克二氧化碳当量(kgCO2e'Äâkg'àí1'ÄâH2)的两倍多。因此,税收抵免的资格应建立在生命周期评估的基础上,生命周期评估应针对供应链并进行测量,以确保蓝色氢能项目是真正的低碳项目。
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引用次数: 0
Electrochemical regeneration of high-purity CO2 from (bi)carbonates in a porous solid electrolyte reactor for efficient carbon capture 在多孔固体电解质反应器中从(生物)碳酸盐中电化学再生高纯度二氧化碳以实现高效碳捕获
IF 56.7 1区 材料科学 Q1 ENERGY & FUELS Pub Date : 2024-10-11 DOI: 10.1038/s41560-024-01654-z
Xiao Zhang, Zhiwei Fang, Peng Zhu, Yang Xia, Haotian Wang

Carbon dioxide (CO2) and absorbent regeneration are the most energy-intensive processes in carbon capture loops. Conventional carbon capture technologies typically consume substantial amounts of heat and involve multiple steps for regeneration. Here we demonstrated one-step electrochemical regeneration of CO2 and alkaline absorbent from carbon-containing solutions in a modular porous solid electrolyte (PSE) reactor. By performing hydrogen evolution and oxidation redox reactions, our PSE reactor selectively split NaHCO3/Na2CO3 solutions, which typically come from air contactors after CO2 absorption, into NaOH absorbent in the catholyte and high-purity CO2 gas in the PSE layer. No chemicals were consumed and no by-products were generated. High Na+-ion transport number (~90%), high capture capacity retention (~90%), low energy consumptions (50 kJ molCO2−1 and 118 kJ molCO2−1 at 1 mA cm−2 and 100 mA cm−2 for bicarbonate, respectively) and long-term stability (>100 hours) were demonstrated. We achieved industrially relevant carbon regeneration rates of up to 1 A cm−2 (~18 mmol cm−2 h−1), highlighting the promising application potential.

二氧化碳(CO2)和吸收剂再生是碳捕集循环中最耗能的过程。传统的碳捕集技术通常需要消耗大量热量,并涉及多个再生步骤。在这里,我们在模块化多孔固体电解质(PSE)反应器中演示了一步式电化学再生含碳溶液中的二氧化碳和碱性吸收剂。通过氢进化和氧化还原反应,我们的 PSE 反应器可选择性地将 NaHCO3/Na2CO3 溶液(通常来自吸收二氧化碳后的空气接触器)分离成阴溶液中的 NaOH 吸收剂和 PSE 层中的高纯度二氧化碳气体。既不消耗化学品,也不产生副产品。结果表明,该方法具有高 Na+ 离子传输数(约 90%)、高捕集能力保持率(约 90%)、低能耗(在 1 mA cm-2 和 100 mA cm-2 条件下,碳酸氢盐的能耗分别为 50 kJ molCO2-1 和 118 kJ molCO2-1)和长期稳定性(100 小时)。我们实现了高达 1 A cm-2 (约 18 mmol cm-2 h-1)的工业相关碳再生率,凸显了其巨大的应用潜力。
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引用次数: 0
Fair energy finance increases global equity in the green energy transition 公平的能源融资提高了绿色能源转型中的全球公平性
IF 49.7 1区 材料科学 Q1 ENERGY & FUELS Pub Date : 2024-10-07 DOI: 10.1038/s41560-024-01607-6
Five climate–energy–economy models are used to explore the effect of reducing the cost gap in energy financing between developed and developing countries through fair-finance. Such convergence is projected to increase energy availability, affordability, and sustainability in developing countries, thereby improving energy justice.
本报告使用了五个气候-能源-经济模型来探讨通过公平融资缩小发达国家与发展中国家之间能源融资成本差距的效果。预计这种趋同将提高发展中国家的能源可用性、可负担性和可持续性,从而改善能源公正。
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引用次数: 0
Assessing cathode–electrolyte interphases in batteries 评估电池中的阴极-电解质间相
IF 56.7 1区 材料科学 Q1 ENERGY & FUELS Pub Date : 2024-10-07 DOI: 10.1038/s41560-024-01639-y
Jie Xiao, Nicole Adelstein, Yujing Bi, Wenjuan Bian, Jordi Cabana, Corie L. Cobb, Yi Cui, Shen J. Dillon, Marca M. Doeff, Saiful M. Islam, Kevin Leung, Mengya Li, Feng Lin, Jun Liu, Hongmei Luo, Amy C. Marschilok, Ying Shirley Meng, Yue Qi, Ritu Sahore, Kayla G. Sprenger, Robert C. Tenent, Michael F. Toney, Wei Tong, Liwen F. Wan, Chongmin Wang, Stephen E. Weitzner, Bingbin Wu, Yaobin Xu

The cathode–electrolyte interphase plays a pivotal role in determining the usable capacity and cycling stability of electrochemical cells, yet it is overshadowed by its counterpart, the solid–electrolyte interphase. This is primarily due to the prevalence of side reactions, particularly at low potentials on the negative electrode, especially in state-of-the-art Li-ion batteries where the charge cutoff voltage is limited. However, as the quest for high-energy battery technologies intensifies, there is a pressing need to advance the study of cathode–electrolyte interphase properties. Here, we present a comprehensive approach to analyse the cathode–electrolyte interphase in battery systems. We underscore the importance of employing model cathode materials and coin cell protocols to establish baseline performance. Additionally, we delve into the factors behind the inconsistent and occasionally controversial findings related to the cathode–electrolyte interphase. We also address the challenges and opportunities in characterizing and simulating the cathode–electrolyte interphase, offering potential solutions to enhance its relevance to real-world applications.

阴极-电解质相间层在决定电化学电池的可用容量和循环稳定性方面发挥着关键作用,但与之相对应的固态-电解质相间层相比,阴极-电解质相间层的作用却黯然失色。这主要是由于副反应的普遍存在,特别是在负极电位较低时,尤其是在充电截止电压有限的最先进锂离子电池中。然而,随着人们对高能电池技术的不断追求,迫切需要推进对正极-电解质相间特性的研究。在此,我们提出了一种分析电池系统中阴极-电解质相间的综合方法。我们强调了采用模型阴极材料和纽扣电池协议建立基线性能的重要性。此外,我们还深入探讨了与阴极-电解质相生相克相关的研究结果不一致且偶尔存在争议的背后因素。我们还探讨了表征和模拟阴极-电解质相间过程所面临的挑战和机遇,并提供了潜在的解决方案,以提高其与实际应用的相关性。
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引用次数: 0
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Nature Energy
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