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Manipulation of the magnetic monopole injection for topological transition 操纵磁单极子注入实现拓扑转变
IF 9.7 2区 材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-02-16 DOI: 10.1038/s41427-024-00529-9
Hee-Sung Han, Sergio A. Montoya, Eric E. Fullerton, Weilun Chao, Soong-Geun Je, Ki‐Suk Lee, Mi-Young Im

Manipulating the topological properties of spin textures in magnetic materials is of great interest due to the rich physics and promising technological applications of these materials in advanced electronic devices. A spin texture with desired topological properties can be created by magnetic monopole injection, resulting in topological transitions involving changes in the topological charge. Therefore, controlling magnetic monopole injection has paramount importance for obtaining the desired spin textures but has not yet been reported. Here, we report the use of reliably manipulated magnetic monopole injection in the topological transition from stripe domains to skyrmions in an Fe/Gd multilayer. An easily tunable in-plane magnetic field applied to an Fe/Gd multilayer plays a key role in the magnetic monopole injection by modulating the local exchange energy. Our findings facilitate the efficient management of topological transitions by providing an important method for controlling magnetic monopole injection.

操纵磁性材料中自旋纹理的拓扑特性是人们非常感兴趣的问题,因为这些材料具有丰富的物理特性,而且在先进电子设备中具有广阔的技术应用前景。具有所需拓扑特性的自旋纹理可通过磁单极子注入产生,从而导致拓扑电荷变化的拓扑转变。因此,控制磁单极子注入对获得所需的自旋纹理至关重要,但目前尚未有相关报道。在此,我们报告了在铁/钆多层中从条纹畴到天幕的拓扑转变过程中使用可靠操控的磁单极子注入的情况。应用于 Fe/Gd 多层的易调谐面内磁场通过调节局部交换能,在磁单极子注入中发挥了关键作用。我们的发现为控制磁单极子注入提供了一种重要方法,从而促进了拓扑转变的有效管理。
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引用次数: 0
Wearable respiratory sensors for health monitoring 用于健康监测的可穿戴呼吸传感器
IF 9.7 2区 材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-02-09 DOI: 10.1038/s41427-023-00513-9
Zhifu Yin, Yang Yang, Cong Hu, Jinzhe Li, Boyu Qin, Xue Yang

Real-time monitoring and early warning of human health conditions is an important function of wearable devices. Along with the development of the Internet of Things and the medical drive for early detection and treatment, wearable devices will become increasingly important in the future. Compared with traditional sensors, wearable sensors with mechanical softness and deformability are able to adapt to geometric nonlinearities and deformations caused by motion that occurs in application scenarios, thus ensuring stable and effective signal output under various complex working conditions. Various novel sensing materials have been developed for the detection of various biomarkers of respiration over the past few years. Here, we summarize the latest innovations in wearable respiratory sensors, highlighting the dominant sensing materials, designs, sensing mechanisms, and clinical implications. Finally, the future challenges and directions of wearable respiratory sensors are outlined toward promoting advancement in the field of wearable respiratory monitoring.

对人体健康状况进行实时监测和预警是可穿戴设备的一项重要功能。随着物联网的发展和医学对早期检测和治疗的推动,可穿戴设备在未来将变得越来越重要。与传统传感器相比,具有机械柔软性和可变形性的可穿戴传感器能够适应应用场景中出现的几何非线性和运动引起的变形,从而确保在各种复杂的工作条件下输出稳定有效的信号。在过去的几年里,人们开发了各种新型传感材料,用于检测呼吸的各种生物标记物。在此,我们总结了可穿戴呼吸传感器的最新创新,重点介绍了主要的传感材料、设计、传感机制和临床意义。最后,我们概述了可穿戴呼吸传感器未来的挑战和发展方向,以促进可穿戴呼吸监测领域的进步。
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引用次数: 0
An advanced 3D lymphatic system for assaying human cutaneous lymphangiogenesis in a microfluidic platform 在微流控平台上检测人体皮肤淋巴管生成的先进三维淋巴系统
IF 9.7 2区 材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-02-02 DOI: 10.1038/s41427-023-00527-3
Minseop Kim, Sieun Choi, Dong-Hee Choi, Jinchul Ahn, Dain Lee, Euijeong Song, Hyun Soo Kim, Mijin Kim, Sowoong Choi, Soojung Oh, Minsuh Kim, Seok Chung, Phil June Park

The human cutaneous lymphatic system strictly controls lymphatic functions by coordinating with skin cells. The lymphatic system plays important roles in removing cell waste, residual proteins, various antigens, and immune cells from tissues to maintain homeostasis and activate the immune system through the drainage of interstitial fluid1,2. The skin protects our body from external stimuli such as pathogens through the cutaneous lymphatic system3,4. Herein, to develop an in vitro human cutaneous lymphatic model, we present two 3D microfluidic platforms: a lymphangiogenesis model with a precollecting lymphatic vessel-like structure and an advanced lymphangiogenesis model with a functional cutaneous barrier and a precollecting lymphatic vessel-like structure. In addition, we rapidly analyzed prolymphangiogenic effects using methods that incorporate a high-speed image processing system and a deep learning-based vascular network analysis algorithm by 12 indices. Using these platforms, we evaluated the pro-lymphangiogenic effect of Lymphanax, a natural product derived from fresh ginseng. As a result, we demonstrated that Lymphanax induces robust lymphangiogenesis without any structural abnormalities. In conclusion, we suggest that these innovative platforms are useful for studying the interaction between the skin and lymphatic system as well as evaluating the prolymphangiogenic effects of drugs and cosmetics.

人体皮肤淋巴系统通过与皮肤细胞协调,严格控制淋巴功能。淋巴系统在清除组织中的细胞废物、残留蛋白质、各种抗原和免疫细胞以维持体内平衡和通过间质排出激活免疫系统方面发挥着重要作用1,2。皮肤通过皮肤淋巴系统保护人体免受病原体等外界刺激3,4。在此,为了开发体外人体皮肤淋巴模型,我们展示了两种三维微流控平台:一种是具有前淋巴管样结构的淋巴管生成模型,另一种是具有功能性皮肤屏障和前淋巴管样结构的高级淋巴管生成模型。此外,我们还利用高速图像处理系统和基于深度学习的血管网络分析算法,通过 12 项指标快速分析了前淋巴管生成效应。利用这些平台,我们评估了从新鲜人参中提取的天然产品 Lymphanax 的促淋巴管生成作用。结果表明,Lymphanax 能诱导强有力的淋巴管生成,且无任何结构异常。总之,我们认为这些创新平台有助于研究皮肤与淋巴系统之间的相互作用,以及评估药物和化妆品的促淋巴管生成作用。
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引用次数: 0
Large anomalous transverse transport properties in atomically thin 2D Fe3GaTe2 原子级薄二维 Fe3GaTe2 中的大反常横向输运特性
IF 9.7 2区 材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-01-26 DOI: 10.1038/s41427-023-00525-5
Brahim Marfoua, Jisang Hong

Anomalous transverse conductivities, such as anomalous Hall conductivity (AHC), anomalous Nernst conductivity (ANC), and anomalous thermal Hall conductivity (ATHC), play a crucial role in the emerging field of spintronics. Motivated by the recent fabrication of two-dimensional (2D) ferromagnetic thin film Fe3GaTe2, we investigate the thickness-dependent anomalous transverse conductivities of the 2D Fe3GaTe2 system (from one to four layers). The atomically ultrathin 2D Fe3GaTe2 system shows above-room-temperature ferromagnetism with a large perpendicular magnetic anisotropy energy. Furthermore, we obtain a large AHC of −485 S/cm in the four-layer thickness, and this is further enhanced to −550 S/cm with small electron doping. This AHC is seven times larger than the measured AHC in thicker 2D Fe3GaTe2 (178 nm). The ANC also reaches 0.55 A/K.m in the four-layer structure. Along with these, the four-layer system exhibits a large ATHC (−0.105 ~ −0.135 W/K.m). This ATHC is comparable to the large ATHC found in Weyl semimetal Co3Sn2S2. Based on our results, the atomically ultrathin 2D Fe3GaTe2 system shows outstanding anomalous transverse conductivities and can be utilized as a potential platform for future spintronics and spin caloritronic device applications.

反常横向电导率,如反常霍尔电导率(AHC)、反常奈氏电导率(ANC)和反常热霍尔电导率(ATHC),在新兴的自旋电子学领域发挥着至关重要的作用。受最近制备的二维(2D)铁磁薄膜 Fe3GaTe2 的启发,我们研究了二维 Fe3GaTe2 系统(从一层到四层)随厚度变化的反常横向电导率。原子超薄二维 Fe3GaTe2 系统显示出高于室温的铁磁性,具有很大的垂直磁各向异性能。此外,我们还在四层厚度内获得了-485 S/cm的大AHC,而在掺杂少量电子后,AHC进一步增强到-550 S/cm。这个 AHC 比在更厚的二维 Fe3GaTe2(178 nm)中测得的 AHC 大七倍。在四层结构中,ANC 也达到了 0.55 A/K.m。此外,四层系统还显示出较大的 ATHC(-0.105 ~ -0.135 W/K.m)。这一 ATHC 与在 Weyl 半金属 Co3Sn2S2 中发现的大 ATHC 相当。根据我们的研究结果,原子超薄二维 Fe3GaTe2 系统显示出卓越的反常横向电导率,可作为未来自旋电子学和自旋热电子器件应用的潜在平台。
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引用次数: 0
Mode-dependent magnonic noise 取决于模式的磁噪声
IF 9.7 2区 材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-01-19 DOI: 10.1038/s41427-023-00522-8
Ryo Furukawa, Shoki Nezu, Takuro Eguchi, Koji Sekiguchi

The performance of magnonic devices such as converters, switches, and multiplexers greatly depends on magnonic noise. While a peculiar discrete magnonic noise has been previously reported, the sources of underlying magnon dynamics occurring in high-magnon density conditions have not been clarified. Here, zero-span measurements of the spectrum analyzer were recorded to accurately detect magnonic noise as a fluctuation of the spin-wave amplitude. The results of low-frequency magnonic noise demonstrated a spin-wave mode dependency, indicating the existence of a peculiar magnon surface state. Furthermore, the energy thresholds of four-magnon scattering and autooscillation were determined using magnonic white noise. The noise data obtained in this study can help promote theoretical and experimental research on magnons.

磁子设备(如转换器、开关和多路复用器)的性能在很大程度上取决于磁子噪声。虽然以前曾报道过一种奇特的离散磁子噪声,但在高磁子密度条件下发生的潜在磁子动力学的来源尚未明确。在此,我们记录了频谱分析仪的零跨度测量,以准确检测作为自旋波振幅波动的磁子噪声。低频磁子噪声的结果显示了自旋波模式依赖性,表明存在一种奇特的磁子表面态。此外,还利用磁子白噪声确定了四磁子散射和自振的能量阈值。本研究获得的噪声数据有助于促进有关磁子的理论和实验研究。
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引用次数: 0
Biomaterial-based regenerative therapeutic strategies for spinal cord injury 基于生物材料的脊髓损伤再生治疗策略
IF 9.7 2区 材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-01-19 DOI: 10.1038/s41427-023-00526-4
Keyi Chen, Wei Yu, Genjiang Zheng, Zeng Xu, Chen Yang, Yunhao Wang, Zhihao Yue, Weien Yuan, Bo Hu, Huajiang Chen

As one of the most intractable neurological diseases, spinal cord injury (SCI) often leads to permanent neurological impairment in patients. Unfortunately, due to the complex pathological mechanisms and unique postinjury microenvironment, there is currently no way to completely repair the injured spinal cord. In recent years, with the rapid development of tissue engineering technology, the combination of biomaterials and medicine has provided a new idea for treating SCI. Here, we systematically summarize representative biomaterials, including natural, synthetic, nano, and hybrid materials, and their applications in SCI treatment. In addition, we describe several state-of-the-art fabrication techniques for tissue engineering. Importantly, we provide novel insights for the use of biomaterial-based therapeutic strategies to reduce secondary damage and promote repair. Finally, we discuss several biomaterial clinical studies. This review aims to provide a reference and new insights for the future exploration of spinal cord regeneration strategies.

作为最棘手的神经系统疾病之一,脊髓损伤(SCI)通常会导致患者永久性神经功能损伤。遗憾的是,由于其复杂的病理机制和独特的损伤后微环境,目前还没有完全修复损伤脊髓的方法。近年来,随着组织工程技术的飞速发展,生物材料与医学的结合为治疗 SCI 提供了新的思路。在此,我们系统地总结了具有代表性的生物材料,包括天然材料、合成材料、纳米材料和混合材料,以及它们在 SCI 治疗中的应用。此外,我们还介绍了几种最先进的组织工程制造技术。重要的是,我们为使用基于生物材料的治疗策略减少二次损伤和促进修复提供了新的见解。最后,我们讨论了几项生物材料临床研究。本综述旨在为脊髓再生策略的未来探索提供参考和新见解。
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引用次数: 0
Ultrabroadband absorptive refractory plasmonics for photocatalytic hydrogen evolution reactions 用于光催化氢进化反应的超宽带吸收性难熔等离子体
IF 9.7 2区 材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-01-19 DOI: 10.1038/s41427-023-00523-7
Myeongcheol Go, Inju Hong, Dasol Lee, Sanghoon Kim, Junho Jang, Keon-Woo Kim, Sangmin Shim, Kijung Yong, Junsuk Rho, Jin Kon Kim

As an environmentally friendly and renewable method for hydrogen production powered by solar energy, photocatalytic hydrogen evolution reactions (HERs) using broadband absorbers have received much attention. Here, we report the fabrication and characterization of an ultrabroadband absorber for the photocatalytic HER. The absorber is composed of titanium nitride and titanium dioxide heterostructures deposited onto a porous anodized aluminum oxide template. The absorber shows ultrabroadband absorption in both the visible and near-infrared regions (400–2500 nm), with averages of 99.1% and 80.1%, respectively. Additionally, the presence of the TiO2 layer within the absorber extends the lifetime of the hot carriers by 2.7 times longer than that without the TiO2 layer, enhancing the transfer of hot electrons and improving the efficiency of hydrogen production by 1.9 times. This novel ultrabroadband absorber has potential use in advanced photocatalytic HER applications, providing a sustainable and cost-effective route for hydrogen generation from solar energy.

作为一种利用太阳能制氢的环保型可再生方法,使用宽带吸收器的光催化氢进化反应(HERs)受到了广泛关注。在此,我们报告了一种用于光催化氢进化反应的超宽带吸收器的制造和表征。该吸收器由沉积在多孔阳极氧化铝模板上的氮化钛和二氧化钛异质结构组成。该吸收器在可见光和近红外区域(400-2500 纳米)都显示出超宽带吸收,平均吸收率分别为 99.1% 和 80.1%。此外,吸收器中二氧化钛层的存在使热载流子的寿命比没有二氧化钛层的吸收器延长了 2.7 倍,从而增强了热电子的转移,并将制氢效率提高了 1.9 倍。这种新型超宽带吸收器可用于先进的光催化 HER 应用,为利用太阳能制氢提供了一条可持续且具有成本效益的途径。
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引用次数: 0
The central role of tilted anisotropy for field-free spin–orbit torque switching of perpendicular magnetization 倾斜各向异性在垂直磁化的无场自旋轨道力矩切换中的核心作用
IF 9.7 2区 材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-01-12 DOI: 10.1038/s41427-023-00521-9
Chen-Yu Hu, Wei-De Chen, Yan-Ting Liu, Chao-Chung Huang, Chi-Feng Pai

The discovery of efficient magnetization switching upon device activation by spin Hall effect (SHE)-induced spin–orbit torque (SOT) changed the course of magnetic random-access memory (MRAM) research and development. However, for electronic systems with perpendicular magnetic anisotropy (PMA), the use of SOT is still hampered by the necessity of a longitudinal magnetic field to break magnetic symmetry and achieve deterministic switching. In this work, we demonstrate that robust and tunable field-free current-driven SOT switching of perpendicular magnetization can be controlled by the growth protocol in Pt-based magnetic heterostructures. We further elucidate that such growth-dependent symmetry breaking originates from the laterally tilted magnetic anisotropy of the ferromagnetic layer with PMA, a phenomenon that has been largely neglected in previous studies. We show experimentally and in simulation that in a PMA system with tilted anisotropy, the deterministic field-free switching exhibits a conventional SHE-induced damping-like torque feature, and the resulting current-induced effective field shows a nonlinear dependence on the applied current density. This relationship could be potentially misattributed to an unconventional SOT origin.

自旋霍尔效应(SHE)诱导的自旋轨道力矩(SOT)可在器件激活时实现高效磁化切换,这一发现改变了磁性随机存取存储器(MRAM)的研究和开发进程。然而,对于具有垂直磁各向异性(PMA)的电子系统来说,由于需要纵向磁场来打破磁对称性并实现确定性开关,SOT 的使用仍然受到阻碍。在这项工作中,我们证明了在铂基磁异质结构中,垂直磁化的稳健、可调的无磁场电流驱动 SOT 开关可由生长协议控制。我们进一步阐明,这种依赖于生长的对称性破坏源于具有 PMA 的铁磁层的横向倾斜磁各向异性,而这一现象在以往的研究中基本上被忽视了。我们通过实验和仿真表明,在具有倾斜各向异性的 PMA 系统中,确定性无磁场切换表现出传统的 SHE 诱导阻尼转矩特征,由此产生的电流诱导有效磁场与外加电流密度呈非线性依赖关系。这种关系有可能被误认为是非常规 SOT 的起源。
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引用次数: 0
Strain-induced specific orbital control in a Heusler alloy-based interfacial multiferroics 基于 Heusler 合金的界面多铁氧体中由应变引起的特定轨道控制
IF 9.7 2区 材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-01-10 DOI: 10.1038/s41427-023-00524-6
Jun Okabayashi, T. Usami, Amran Mahfudh Yatmeidhy, Y. Murakami, Y. Shiratsuchi, R. Nakatani, Y. Gohda, K. Hamaya
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引用次数: 0
Role of the structure order in the transport and magnetic properties of high-entropy alloy films 结构顺序在高熵合金薄膜的传输和磁特性中的作用
IF 9.7 2区 材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-01-04 DOI: 10.1038/s41427-023-00518-4
Jia-Wei Chen, Shih-Hsun Chen, Padraic Shafer, Wen-Yen Tzeng, Yi-Cheng Chen, Chih-Wei Luo, Wen-Wei Wu, Jien-Wei Yeh, Ying-Hao Chu

The fabrication and development of high-entropy alloys (HEAs) with exceptional functionalities is a rapidly expanding field with numerous applications. When the role of entropy in HEAs is considered, the extrinsic factors, such as the existence of grains and different phases, need to be separated from the intrinsic configurations of the atomic lattice. Here, we fabricated the CoCrFeNi2Al0.5 HEA/muscovite heterostructures, and some were prepared as epitaxial bilayers and others were prepared as an amorphous system. These two systems are classified into atomic-site disordered (ASD) and structurally disordered (SD) states, respectively, without the extrinsic effects for the determination of the crystal lattice role in high-entropy states. In this study, we determined the role of the structure order in correlation with the structural, electronic, and magnetic properties of HEAs using a combination of energy-dispersive X-ray spectrometry, X-ray diffraction, transmission electron microscopy, magneto-transport, ac magnetometry, and X-ray absorption spectroscopy with magnetic circular dichroism. The ASD state showed fully metallic behavior. In contrast, the SD state showed a metallic behavior with intense magnetic saturation, which was called Kondo-like behavior, under 50 K with a low-temperature coefficient of resistivity of ~64 ppm/°C. The difference between the saturation magnetic moment and the electron relaxation behavior in the ASD and SD states resulted from the existence of the structural order affecting the atomic distance and periodicity to modify the exchange interaction and tune the electron-phonon interaction for scattering. The ferromagnetic behavior contributed by Co, Fe, and Ni atoms was probed by X-ray absorption and magnetic circular dichroism to understand the magnetic interactions in the ASD and SD states.

制造和开发具有特殊功能的高熵合金(HEAs)是一个快速发展的领域,其应用领域众多。在考虑熵在高熵合金中的作用时,需要将晶粒和不同相的存在等外在因素与原子晶格的内在构型区分开来。在这里,我们制备了 CoCrFeNi2Al0.5 HEA/muscovite 异质结构,其中一些制备成了外延双层结构,另一些制备成了非晶态体系。这两种体系被分别划分为原子位点无序(ASD)态和结构无序(SD)态,在确定高熵态中晶格的作用时不需要考虑外在效应。在这项研究中,我们结合使用了能量色散 X 射线光谱法、X 射线衍射法、透射电子显微镜法、磁传输法、交流磁力测定法和带有磁圆二色性的 X 射线吸收光谱法,确定了结构顺序与 HEA 的结构、电子和磁特性之间的相关性。ASD 状态显示出完全的金属特性。与此相反,SD 状态在 50 K 下表现出具有强磁饱和度的金属行为,被称为近藤行为,其低温电阻系数约为 64 ppm/°C。在 ASD 和 SD 状态下,饱和磁矩和电子弛豫行为之间的差异是由于存在影响原子间距和周期性的结构顺序,从而改变了交换相互作用,并调整了电子-声子相互作用以实现散射。通过 X 射线吸收和磁圆二色性探测了 Co、Fe 和 Ni 原子的铁磁行为,以了解 ASD 和 SD 状态下的磁相互作用。
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引用次数: 0
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Npg Asia Materials
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