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Dominance of open burning signatures in PM2.5 near coal plant should redefine pollutant priorities of India 煤厂附近的 PM2.5 以露天焚烧为主,应重新定义印度的污染物优先事项
IF 8.5 1区 地球科学 Q1 METEOROLOGY & ATMOSPHERIC SCIENCES Pub Date : 2024-11-20 DOI: 10.1038/s41612-024-00836-6
Iravati Ray, Shoumick Mitra, Jariya Kayee, Shufang Yuan, S. M. Shiva Nagendra, Xianfeng Wang, Reshmi Das
India, heavily reliant on coal for power generation, has been a significant emitter of particulate matter (PM) bound lead (Pb) and other heavy metals. It is crucial to understand whether implementation of stricter norms in recent years have effectively reduced emissions from coal combustion. This study aims to investigate and quantify the primary sources of PM2.5 in an area housing a major lignite-fired power plant in South India using Pb isotopic compositions and elemental concentrations. Characteristic ratios such as V/Pb and Cu/Pb demonstrate negligible influence from coal combustion, and indicate that summer aerosols are influenced by open burning. In Pb triple-isotope space the PM2.5 aerosols plot away from coal, overlapping with open burning signatures. These indicate that the atmosphere is predominantly influenced by open burning of solid waste and biomass rather than coal combustion, suggesting a promising decrease in coal emissions. Bayesian mixing model demonstrates that solid waste & biomass burning is the largest anthropogenic contributor towards atmospheric Pb (up to 26%), even in a region of coal combustion and presence of medium and small-scale industries. The dominance of open burning as a pollution source in the vicinity of a lignite fired power plant highlights the necessity for better waste management strategies.
印度严重依赖煤炭发电,一直是含铅(Pb)和其他重金属的颗粒物(PM)的主要排放国。了解近年来实施的更严格规范是否有效减少了燃煤排放至关重要。本研究旨在利用铅同位素组成和元素浓度,调查和量化印度南部一个主要褐煤燃烧发电厂所在地区 PM2.5 的主要来源。V/Pb 和 Cu/Pb 等特征比率表明燃煤的影响微乎其微,并表明夏季气溶胶受到露天燃烧的影响。在铅三重同位素空间中,PM2.5 气溶胶的分布远离煤炭,与露天燃烧特征重叠。这表明大气主要受到固体废弃物和生物质露天焚烧的影响,而不是煤炭燃烧的影响,表明煤炭排放有望减少。贝叶斯混合模型表明,即使在燃煤和存在中小型工业的地区,固体废物和生物质燃烧也是大气中铅的最大人为来源(高达 26%)。露天焚烧是褐煤发电厂附近的主要污染源,这凸显了改善废物管理策略的必要性。
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引用次数: 0
Climate model trend errors are evident in seasonal forecasts at short leads 气候模式趋势误差在短时季节预测中很明显
IF 8.5 1区 地球科学 Q1 METEOROLOGY & ATMOSPHERIC SCIENCES Pub Date : 2024-11-20 DOI: 10.1038/s41612-024-00832-w
Jonathan D. Beverley, Matthew Newman, Andrew Hoell
Climate models exhibit errors in their simulation of historical trends of variables including sea surface temperature, winds, and precipitation, with important implications for regional and global climate projections. Here, we show that the same trend errors are also present in a suite of initialised seasonal re-forecasts for the years 1993–2016. These re-forecasts are produced by operational models that are similar to Coupled Model Intercomparison Project (CMIP)-class models and share their historical external forcings (e.g. CO2/aerosols). The trend errors, which are often well-developed at very short lead times, represent a roughly linear change in the model mean biases over the 1993–2016 re-forecast record. The similarity of trend errors in both the re-forecasts and historical simulations suggests that climate model trend errors likewise result from evolving mean biases, responding to changing external radiative forcings, instead of being an erroneous long-term response to external forcing. Therefore, these trend errors may be investigated by examining their short-lead development in initialised seasonal forecasts/re-forecasts, which we suggest should also be made by all CMIP models.
气候模式在模拟海面温度、风和降水等变量的历史趋势时会出现误差,这对区域和全球气候预测有重要影响。在此,我们展示了 1993-2016 年的一套初始化季节再预测也存在同样的趋势误差。这些再预测由与耦合模式相互比较项目(CMIP)类模式相似的业务模式生成,并共享其历史外部作用力(如二氧化碳/气溶胶)。在 1993-2016 年的再预报记录中,趋势误差通常在很短的前导时间内就会形成,代表了模式平均偏差的大致线性变化。重新预测和历史模拟中趋势误差的相似性表明,气候模式趋势误差同样是由不断变化的平均偏差引起的,是对不断变化的外部辐射强迫的响应,而不是对外部强迫的长期错误响应。因此,这些趋势误差可以通过研究其在初始化季节预报/再预报中的短时发展来研究,我们建议所有的 CMIP 模式也应该这样做。
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引用次数: 0
Attributing the recent weakening of the South Asian subtropical westerlies 南亚副热带西风近期减弱的原因是
IF 8.5 1区 地球科学 Q1 METEOROLOGY & ATMOSPHERIC SCIENCES Pub Date : 2024-11-19 DOI: 10.1038/s41612-024-00777-0
Pankaj Upadhyaya, Saroj K. Mishra, John T. Fasullo, In-Sik Kang
Over the last four decades (1980–2020), the summer westerlies that prevail in South Asia along the monsoon trough region have weakened by about 25% based on multiple reanalysis datasets. Trends in a range of climate model simulations suggest that the weakening is driven by multiple anthropogenic forcings. Over the period, sea-level pressure has increased by 0.6–1.0 hPa over South Asia’s northwestern regions, induced by cooling due to aerosol emission and changes in land use and land cover, and has decreased over the Arabian Peninsula mainly due to warming by greenhouse gases. These changes in temperature and pressure act to weaken the regional pressure gradient, deflecting the subtropical westerlies from South Asia toward the Arabian Peninsula and weakening the winds in the monsoon trough and its adjacent region. The slowing down of winds appears to result in an anomalous moisture loading and increase in rainfall over the semi-arid northwestern South Asia. This weakening and its associated changes in regional climate are highly relevant to policymaking across South Asia.
根据多个再分析数据集,在过去四十年(1980-2020 年)里,南亚季风槽区域盛行的夏季西风减弱了约 25%。一系列气候模型模拟的趋势表明,这种减弱是由多种人为影响因素造成的。在此期间,南亚西北部地区的海平面气压上升了 0.6-1.0 hPa,这是由于气溶胶排放以及土地利用和土地覆盖的变化造成的降温,而阿拉伯半岛的海平面气压下降则主要是由于温室气体造成的升温。温度和气压的这些变化削弱了区域气压梯度,使副热带西风从南亚转向阿拉伯半岛,并削弱了季风槽及其邻近地区的风力。风速减慢似乎导致南亚西北部半干旱地区水汽负荷异常,降雨量增加。这种减弱及其相关的区域气候变化与整个南亚的政策制定高度相关。
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引用次数: 0
Hybrid physics-AI outperforms numerical weather prediction for extreme precipitation nowcasting 物理-人工智能混合技术在极端降水预报方面优于数值天气预报
IF 8.5 1区 地球科学 Q1 METEOROLOGY & ATMOSPHERIC SCIENCES Pub Date : 2024-11-18 DOI: 10.1038/s41612-024-00834-8
Puja Das, August Posch, Nathan Barber, Michael Hicks, Kate Duffy, Thomas Vandal, Debjani Singh, Katie van Werkhoven, Auroop R. Ganguly
Precipitation nowcasting, which is critical for flood emergency and river management, has remained challenging for decades, although recent developments in deep generative modeling (DGM) suggest the possibility of improvements. River management centers, such as the Tennessee Valley Authority, have been using Numerical Weather Prediction (NWP) models for nowcasting, but they have been struggling with missed detections even from best-in-class NWP models. While decades of prior research achieved limited improvements beyond advection and localized evolution, recent attempts have shown progress from so-called physics-free machine learning (ML) methods, and even greater improvements from physics-embedded ML approaches. Developers of DGM for nowcasting have compared their approaches with optical flow (a variant of advection) and meteorologists’ judgment, but not with NWP models. Further, they have not conducted independent co-evaluations with water resources and river managers. Here we show that the state-of-the-art physics-embedded deep generative model, specifically NowcastNet, outperforms the High Resolution Rapid Refresh (HRRR) model, which is the latest generation of NWP, along with advection and persistence, especially for heavy precipitation events. Thus, for grid-cell extremes over 16 mm/h, NowcastNet demonstrated a median critical success index (CSI) of 0.30, compared with median CSI of 0.04 for HRRR. However, despite hydrologically-relevant improvements in point-by-point forecasts from NowcastNet, caveats include overestimation of spatially aggregate precipitation over longer lead times. Our co-evaluation with ML developers, hydrologists and river managers suggest the possibility of improved flood emergency response and hydropower management.
降水预报对洪水应急和河流管理至关重要,但几十年来,降水预报一直面临挑战,尽管最近在深度生成建模(DGM)方面取得的进展表明,降水预报有可能得到改善。田纳西流域管理局等河流管理中心一直在使用数值天气预报(NWP)模型进行降水预报,但即使是同类最佳的 NWP 模型也会出现漏报现象。虽然之前几十年的研究在平流和局部演变之外取得的改进有限,但最近的尝试表明,所谓的无物理学机器学习(ML)方法取得了进展,而嵌入物理学的 ML 方法则取得了更大的改进。用于预报的 DGM 的开发者将他们的方法与光流(平流的一种变体)和气象学家的判断进行了比较,但没有与 NWP 模型进行比较。此外,他们还没有与水资源和河流管理人员进行独立的共同评估。在这里,我们展示了最先进的物理嵌入式深度生成模型,特别是 NowcastNet,在平流和持续性方面优于高分辨率快速刷新(HRRR)模型,后者是最新一代的 NWP,尤其是在强降水事件中。因此,对于超过 16 毫米/小时的网格单元极端降水,NowcastNet 的关键成功指数 (CSI) 中值为 0.30,而 HRRR 的关键成功指数中值为 0.04。不过,尽管 NowcastNet 的逐点预报在水文相关方面有所改进,但也存在一些问题,包括在较长的准备时间内高估了空间上的降水总量。我们与 ML 开发人员、水文学家和河流管理人员共同进行的评估表明,洪水应急响应和水电管理有可能得到改善。
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引用次数: 0
Distinct tropospheric anomalies during sudden stratospheric warming events accompanied by strong and weak Ural Ridge 平流层突然变暖事件期间伴随着强乌拉尔山脉和弱乌拉尔山脉的不同对流层异常现象
IF 8.5 1区 地球科学 Q1 METEOROLOGY & ATMOSPHERIC SCIENCES Pub Date : 2024-11-17 DOI: 10.1038/s41612-024-00826-8
Chongyang Zhang, Jiankai Zhang, Amanda C. Maycock, Wenshou Tian
Different tropospheric precursor anomalies leading to sudden stratospheric warmings (SSWs) may result in different circulation evolution. This study finds that there are distinct differences in tropospheric circulation evolutions during SSWs following anomalously strong- (SUR-SSWs) and weak- (WUR-SSWs) Ural ridge. SUR-SSWs exhibit enhanced East Asian trough in the following week, while enhanced Greenland ridge and negative tropospheric annular mode anomalies can persist for 1 month. In contrast, WUR-SSWs exhibit surface cooling over northern Eurasia without notable tropospheric annular mode anomalies. During SUR-SSWs, waves induced by the enhanced Ural wave source tend to propagate below the tropopause, amplifying the East Asian trough. Additionally, due to decreased wave phase speed, the preexisting Ural ridge anomalies migrate westward and amplify the Greenland ridge. Before WUR-SSWs, preexisting cooling over Northeast Asia migrates westward and amplifies northern Eurasia cooling. Thus, the Ural ridge anomalies prior to SSWs significantly influence post-SSW tropospheric circulation.
导致平流层骤暖(SSWs)的对流层前兆异常可能会导致不同的环流演变。本研究发现,在乌拉尔脊异常强(SUR-SSWs)和弱(WUR-SSWs)之后的SSWs期间,对流层环流演变存在明显差异。SUR-SSWs在接下来的一周里会出现增强的东亚低谷,而增强的格陵兰脊和对流层环模负异常会持续一个月。相反,WUR-SSW 在欧亚大陆北部表现出地表冷却,但对流层环模异常并不显著。在SUR-SSW期间,增强的乌拉尔波源诱发的波往往在对流层顶以下传播,从而放大了东亚低谷。此外,由于波相速度降低,先前存在的乌拉尔海脊异常向西移动,放大了格陵兰海脊。在 WUR-SSWs 出现之前,东北亚上空原有的降温向西移动,放大了欧亚大陆北部的降温。因此,西南气旋之前的乌拉尔海脊异常会对西南气旋之后的对流层环流产生重大影响。
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引用次数: 0
Dry soil moisture on the Tibetan plateau drives synchronous extreme heatwaves in Europe and East Asia 青藏高原干燥的土壤水分导致欧洲和东亚出现同步极端热浪
IF 8.5 1区 地球科学 Q1 METEOROLOGY & ATMOSPHERIC SCIENCES Pub Date : 2024-11-17 DOI: 10.1038/s41612-024-00831-x
Jilan Jiang, Yimin Liu, Jun Meng, Guoxiong Wu, Bian He, Tingting Ma, Wen Bao, Jingfang Fan
Recently, extreme heatwaves have frequently concurrently swept across Europe and East Asia, causing severe cascading socioeconomic consequences. However, the nonlinear synchronization relationship between these heatwaves and their underlying physical mechanisms remains poorly understood. Utilizing the event synchronization climate network method, atmospheric dynamic diagnostics, and numerical experiments, we revealed robust synchronization between heatwaves over Europe and East Asia, strongly associated with dry soil moisture conditions over the Tibetan Plateau from the preceding winter to summer. Dry soil moisture triggers an equivalent barotropic anticyclone north of the Tibetan Plateau, coinciding with the subtropical westerly jet waveguide and initiating circumglobal atmospheric Rossby waves propagating westward and eastward. Consequently, an equivalent barotropic anticyclone develops over Europe. These anticyclones induce simultaneous heatwaves across Europe and East Asia by increasing downward solar radiation and adiabatic sinking, amplified by positive land-atmosphere feedback. Our findings significantly enhance the understanding and predictive capabilities of these synchronous heatwaves across Eurasia.
最近,极端热浪频频同时席卷欧洲和东亚,造成了严重的连锁社会经济后果。然而,人们对这些热浪之间的非线性同步关系及其背后的物理机制仍然知之甚少。利用事件同步气候网络方法、大气动态诊断和数值实验,我们揭示了欧洲和东亚热浪之间的强同步性,这与青藏高原从冬季到夏季的干燥土壤水分条件密切相关。干燥的土壤水分触发了青藏高原以北的等效气压反气旋,与副热带西风喷流波导相吻合,并引发了向西和向东传播的环全球大气罗斯比波。因此,欧洲上空出现了等效的气压反气旋。这些反气旋通过增加向下的太阳辐射和绝热下沉,在陆地-大气正反馈的作用下,在欧洲和东亚同时引发热浪。我们的发现极大地增强了对欧亚大陆同步热浪的理解和预测能力。
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引用次数: 0
Few shot learning for Korean winter temperature forecasts 学习韩国冬季气温预报的几个镜头
IF 8.5 1区 地球科学 Q1 METEOROLOGY & ATMOSPHERIC SCIENCES Pub Date : 2024-11-12 DOI: 10.1038/s41612-024-00813-z
Seol-Hee Oh, Yoo-Geun Ham
To address the challenge of limited training samples, this study employs the model-agnostic meta-learning (MAML) algorithm along with domain-knowledge-based data augmentation to predict winter temperatures on the Korean Peninsula. While data augmentation has been achieved by using global climate model simulations, the proposed augmentation is purely based on the observed data by defining the labels using large-scale climate variabilities associated with the Korean winter temperatures. The MAML-applied convolutional neural network (CNN) (referred to as the MAML model) demonstrates superior correlation skills for Korean temperature anomalies compared to a reference model (i.e., the CNN without MAML) and state-of-the-art dynamical forecast models across all target lead months during the boreal winter seasons. Sensitivity experiments show that the domain-knowledge-based data augmentation enhances the forecast skill of the MAML model. Moreover, occlusion sensitivity results reveal that the MAML model better captures the physical precursors that influence Korean winter temperatures, resulting in more accurate predictions.
为了应对训练样本有限的挑战,本研究采用了模型无关元学习(MAML)算法和基于领域知识的数据扩增来预测朝鲜半岛的冬季气温。虽然数据扩增是通过全球气候模型模拟实现的,但建议的扩增则纯粹基于观测数据,利用与韩国冬季气温相关的大尺度气候变异来定义标签。与参考模型(即不含 MAML 的 CNN)和最先进的动态预报模型相比,应用了 MAML 的卷积神经网络(CNN)(简称 MAML 模型)在北方冬季所有目标前导月的韩国气温异常方面表现出卓越的相关性技能。灵敏度实验表明,基于领域知识的数据增强增强了 MAML 模型的预报技能。此外,闭塞敏感性结果表明,MAML 模型能更好地捕捉影响韩国冬季气温的物理前兆,从而获得更准确的预测结果。
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引用次数: 0
Uneven global retreat of persistent mountain snow cover alongside mountain warming from ERA5-land 从ERA5-陆地看全球持续性高山积雪的不均匀退缩与高山变暖的同时发生
IF 8.5 1区 地球科学 Q1 METEOROLOGY & ATMOSPHERIC SCIENCES Pub Date : 2024-11-10 DOI: 10.1038/s41612-024-00829-5
Manuel Tobias Blau, Pratik Kad, Jenny V. Turton, Kyung-Ja Ha
The warming of mountains has become evident in recent years, with a mean global warming rate of 1.19 °C from 1979 to 2022. However, unveiling the global divergent decline of persistent mountain snow cover in the face of climate shifts remains unexplored. However, the global decline of persistent mountain snow cover due to climate change is not well understood. This study uses reanalysis and satellite data to examine changes in snow cover lasting over six months across our global mountain regions. We reveal a significant global mean decline of 7.79% in persistent snow cover over the past 44 years. The regional snow cover trends exhibit a heterogeneous and non-linear response to its regional warming rate. Our findings highlight the interplay between global warming and snow cover, emphasizing the need for sustainable development strategies to address the potential impacts of diminishing mountain snow.
近年来,山地变暖的趋势十分明显,从1979年到2022年,全球平均变暖速度为1.19 °C。然而,揭示全球持续性高山积雪覆盖在气候变迁中不同程度下降的问题仍有待探索。然而,人们对气候变化导致的全球持续性高山积雪面积下降还不甚了解。本研究利用再分析和卫星数据研究了全球山区持续六个月以上的积雪覆盖变化。我们发现,在过去 44 年中,全球平均持续积雪覆盖率大幅下降了 7.79%。区域积雪覆盖率的变化趋势与其区域变暖速率呈现出异质性和非线性反应。我们的研究结果凸显了全球变暖与积雪覆盖之间的相互作用,强调了制定可持续发展战略以应对山区积雪减少的潜在影响的必要性。
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引用次数: 0
Nested cross-validation Gaussian process to model dimethylsulfide mesoscale variations in warm oligotrophic Mediterranean seawater 用嵌套交叉验证高斯过程模拟地中海暖寡营养海水中的二甲基硫醚中尺度变化
IF 8.5 1区 地球科学 Q1 METEOROLOGY & ATMOSPHERIC SCIENCES Pub Date : 2024-11-09 DOI: 10.1038/s41612-024-00830-y
Karam Mansour, Stefano Decesari, Marco Paglione, Silvia Becagli, Matteo Rinaldi
The study proposes an approach to elucidate spatiotemporal mesoscale variations of seawater Dimethylsulfide (DMS) concentrations, the largest natural source of atmospheric sulfur aerosol, based on the Gaussian Process Regression (GPR) machine learning model. Presently, the GPR was trained and evaluated by nested cross-validation across the warm-oligotrophic Mediterranean Sea, a climate hot spot region, leveraging the high-resolution satellite measurements and Mediterranean physical reanalysis together with in-situ DMS observations. The end product is daily gridded fields with a spatial resolution of 0.083° × 0.083° (~9 km) that spans 23 years (1998–2020). Extensive observations of atmospheric methanesulfonic acid (MSA), a typical biogenic secondary aerosol component from DMS oxidation, are consistent with the parameterized high-resolution estimates of sea-to-air DMS flux (FDMS). This represents substantial progress over existing coarse-resolution DMS global maps which do not accurately depict the seasonal patterns of MSA in the Mediterranean atmospheric boundary layer.
该研究提出了一种基于高斯过程回归(GPR)机器学习模型的方法,用于阐明海水二甲基硫化物(DMS)浓度的时空中尺度变化,DMS是大气硫气溶胶的最大天然来源。目前,利用高分辨率卫星测量和地中海物理再分析以及现场二甲基硫化物观测数据,通过嵌套交叉验证,对气候热点地区地中海的暖-异养地中海进行了 GPR 训练和评估。最终结果是空间分辨率为 0.083°×0.083°(约 9 千米)的日网格场,时间跨度为 23 年(1998-2020 年)。大气中的甲磺酸(MSA)是二甲基亚砜氧化作用产生的典型生物次生气溶胶成分,其广泛观测结果与海气二甲基亚砜通量(FDMS)的参数化高分辨率估算结果一致。与现有的粗分辨率二甲基亚砜全球地图相比,这是一项重大进步,因为现有的粗分辨率二甲基亚砜全球地图无法准确描绘地中海大气边界层中二甲基亚砜的季节性模式。
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引用次数: 0
Antarctic extreme seasons under 20th and 21st century climate change 20 世纪和 21 世纪气候变化下的南极极端季节
IF 8.5 1区 地球科学 Q1 METEOROLOGY & ATMOSPHERIC SCIENCES Pub Date : 2024-11-07 DOI: 10.1038/s41612-024-00822-y
Thomas J. Bracegirdle, Thomas Caton Harrison, Caroline R. Holmes, Hua Lu, Patrick Martineau, Tony Phillips
In this study, available large ensemble datasets in the Coupled Model Intercomparison Phase 6 (CMIP6) archive were used to provide the first multi-variate overview of the evolution of extreme seasons over Antarctica and the Southern Ocean during the 20th and 21st centuries following medium-to-high radiative forcing scenarios. The results show significant differences between simulated changes in background mean climate and changes in low (10th percentile) and high (90th percentile) extreme seasons. Regional winter warming is most pronounced for cold extremes. In summer, there are more pronounced increases in high extremes in precipitation and westerly wind during the ozone hole formation period (late 20th century), affecting coastal regions and, in particular, the Antarctic Peninsula. At midlatitudes, there is a reduction in the range of summer season wind extremes. Suggested mechanisms for these differences are provided relating to sea ice retreat and westerly jet position.
在这项研究中,利用耦合模式相互比较阶段 6(CMIP6)档案中的现有大型集合数据集,首次对中高辐射强迫情景下 20 世纪和 21 世纪南极洲和南大洋极端季节的演变进行了多变量概述。结果显示,背景平均气候的模拟变化与低(第10百分位数)和高(第90百分位数)极端季节的变化之间存在显著差异。在极端寒冷季节,区域冬季变暖最为明显。在夏季,臭氧洞形成期(20 世纪末)的高极端降水和西风的增加更为明显,影响到沿海地区,特别是南极半岛。在中纬度地区,夏季极端风的范围有所缩小。提出了造成这些差异的与海冰消退和西风喷流位置有关的机制。
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引用次数: 0
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npj Climate and Atmospheric Science
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