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The impact of solar elevation angle on the net radiative effect of tropical cyclone clouds
IF 9 1区 地球科学 Q1 METEOROLOGY & ATMOSPHERIC SCIENCES Pub Date : 2025-02-22 DOI: 10.1038/s41612-025-00964-7
Liang Hu, Dae-Hui Kim, J. Scott Tyo, Elizabeth A. Ritchie

In this study solar elevation angle is shown to have a dominant impact on the net radiation due to tropical cyclone (TC) clouds. As solar elevation angle increases, net cooling effects from TC clouds dominate over net warming effects. From 2001 to 2020, the radiative effect of TC clouds remained stable. However, because of the strong dependency on solar elevation angle, future changes in seasonal occurrence could affect this contribution.

这项研究表明,太阳仰角对热带气旋(TC)云层造成的净辐射有主要影响。随着太阳仰角的增加,热带气旋云的净冷却效应超过了净变暖效应。从 2001 年到 2020 年,热带气旋云的辐射效应保持稳定。然而,由于对太阳仰角的依赖性很强,未来季节性发生的变化可能会影响这一贡献。
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引用次数: 0
Typhoon induced mesoscale cyclonic eddy a long neglected linkage between atmosphere ocean and climate
IF 9 1区 地球科学 Q1 METEOROLOGY & ATMOSPHERIC SCIENCES Pub Date : 2025-02-21 DOI: 10.1038/s41612-025-00946-9
Jia-Yi Lin, Hua Ho, Ganesh Gopalakrishnan, Zhe-Wen Zheng, Ruo-Shan Tseng, Jiayi Pan, Chung-Ru Ho, Quanan Zheng

This study investigates typhoon-induced mesoscale cyclonic eddies (TIME) in the western North Pacific. A total of 69 potential TIME candidates (1995–2018) were identified using global mesoscale eddy trajectory atlas and JTWC typhoon data. Subsequently, systematic analysis procedures were applied to those candidates. Analysis revealed that three cyclonic ocean eddies (COEs) were likely triggered by typhoons Rosie (1997), Nida (2009), and Ma-on (2011). Numerical modeling with a regional ocean modeling system (ROMS) reconstructed the ocean environment during these events. Semi-idealized experiments confirmed that typical TIME events arise from the energy transfer between kinetic and potential energy, with vertical diffusion and horizontal advection contributing significantly to COE spin-up. Divergence and vertical advection terms suppress excessive COE growth. Given the increasing intensity and slower movement of typhoons due to global warming, more TIMEs are expected in the future. Stronger, longer-lasting TIMEs may have significant climate impacts and should be a focus of future research.

{"title":"Typhoon induced mesoscale cyclonic eddy a long neglected linkage between atmosphere ocean and climate","authors":"Jia-Yi Lin, Hua Ho, Ganesh Gopalakrishnan, Zhe-Wen Zheng, Ruo-Shan Tseng, Jiayi Pan, Chung-Ru Ho, Quanan Zheng","doi":"10.1038/s41612-025-00946-9","DOIUrl":"https://doi.org/10.1038/s41612-025-00946-9","url":null,"abstract":"<p>This study investigates typhoon-induced mesoscale cyclonic eddies (TIME) in the western North Pacific. A total of 69 potential TIME candidates (1995–2018) were identified using global mesoscale eddy trajectory atlas and JTWC typhoon data. Subsequently, systematic analysis procedures were applied to those candidates. Analysis revealed that three cyclonic ocean eddies (COEs) were likely triggered by typhoons Rosie (1997), Nida (2009), and Ma-on (2011). Numerical modeling with a regional ocean modeling system (ROMS) reconstructed the ocean environment during these events. Semi-idealized experiments confirmed that typical TIME events arise from the energy transfer between kinetic and potential energy, with vertical diffusion and horizontal advection contributing significantly to COE spin-up. Divergence and vertical advection terms suppress excessive COE growth. Given the increasing intensity and slower movement of typhoons due to global warming, more TIMEs are expected in the future. Stronger, longer-lasting TIMEs may have significant climate impacts and should be a focus of future research.</p>","PeriodicalId":19438,"journal":{"name":"npj Climate and Atmospheric Science","volume":"82 2 1","pages":""},"PeriodicalIF":9.0,"publicationDate":"2025-02-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143470610","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"地球科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Impact of the centennial changes in ENSO on the rise of the Chinese Qing empire
IF 9 1区 地球科学 Q1 METEOROLOGY & ATMOSPHERIC SCIENCES Pub Date : 2025-02-21 DOI: 10.1038/s41612-025-00950-z
Weiyi Sun, Bin Wang, Jian Liu, David A. Bello, Ulf Büntgen, Elena Xoplaki, Deliang Chen, Hui Shi, Nicola Di Cosmo

The demise of the Ming Dynasty (1368–1644) and the rise of the Qing Dynasty (1644–1912) marked an epochal moment in Chinese and world history. Attention has been given to the North China droughts during 1627–1643 that destabilized the Ming Dynasty. However, there is little attention paid to how climate influenced the rise of a minority Manchu state in Northeast China and its conquest of the Ming. Here, we find that contrasting climate conditions between North and Northeast China persisted over a six-decade period (1581–1644), which diversely affected economic, societal, and political changes at the regional level. Five successive megadroughts ravaged North China, while relatively wet and mild climate conditions prevailed in the Manchu homeland of Northeast China. Furthermore, in the early decades of Manchu rule in North China (1645–1680), increased precipitation facilitated the Qing Dynasty’s consolidation. Reconstructions and climate model simulations revealed that these unusual climatic patterns were influenced by the centennial variation of clustering El Niño-Southern Oscillation (ENSO) events and were amplified by the Little Ice Age cooling. These findings shed light on how long-term contrasting future climate changes could lead to divergent socioeconomic responses, potentially increasing the risk of conflict between neighboring states.

{"title":"Impact of the centennial changes in ENSO on the rise of the Chinese Qing empire","authors":"Weiyi Sun, Bin Wang, Jian Liu, David A. Bello, Ulf Büntgen, Elena Xoplaki, Deliang Chen, Hui Shi, Nicola Di Cosmo","doi":"10.1038/s41612-025-00950-z","DOIUrl":"https://doi.org/10.1038/s41612-025-00950-z","url":null,"abstract":"<p>The demise of the Ming Dynasty (1368–1644) and the rise of the Qing Dynasty (1644–1912) marked an epochal moment in Chinese and world history. Attention has been given to the North China droughts during 1627–1643 that destabilized the Ming Dynasty. However, there is little attention paid to how climate influenced the rise of a minority Manchu state in Northeast China and its conquest of the Ming. Here, we find that contrasting climate conditions between North and Northeast China persisted over a six-decade period (1581–1644), which diversely affected economic, societal, and political changes at the regional level. Five successive megadroughts ravaged North China, while relatively wet and mild climate conditions prevailed in the Manchu homeland of Northeast China. Furthermore, in the early decades of Manchu rule in North China (1645–1680), increased precipitation facilitated the Qing Dynasty’s consolidation. Reconstructions and climate model simulations revealed that these unusual climatic patterns were influenced by the centennial variation of clustering El Niño-Southern Oscillation (ENSO) events and were amplified by the Little Ice Age cooling. These findings shed light on how long-term contrasting future climate changes could lead to divergent socioeconomic responses, potentially increasing the risk of conflict between neighboring states.</p>","PeriodicalId":19438,"journal":{"name":"npj Climate and Atmospheric Science","volume":"15 1","pages":""},"PeriodicalIF":9.0,"publicationDate":"2025-02-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143462913","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"地球科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
A new last two millennium reanalysis based on hybrid gain analog offline EnKF and an expanded proxy database
IF 9 1区 地球科学 Q1 METEOROLOGY & ATMOSPHERIC SCIENCES Pub Date : 2025-02-21 DOI: 10.1038/s41612-025-00961-w
Fen Wu, Liang Ning, Zhengyu Liu, Jian Liu, Wenqing Hu, Mi Yan, Fangmiao Xing, Lili Lei, Haohao Sun, Kefan Chen, Yanmin Qin, Benyue Li, Chuanxi Xu

This paper systemically assesses the performances of two assimilation methods, i.e., the Offline Ensemble Kalman Filter (OEnKF) and the Hybrid Gain Analog Offline EnKF (HGAOEnKF) with three proxy databases, on reconstructing the temperature and precipitation during the last two millennia. The results show that, among three databases, increasing the number of proxy records significantly improves the reconstruction skill for both assimilation methods, with a larger improvement in HGAOEnKF. In the instrumental era, six reconstructions have comparable skill (similar correlation coefficients, CEs, and RMSEs) when validated against out-of-sample proxy records and instrumental reanalyses. During the pre-industrial era, HGAOEnKF shows better assimilation performance by improving the background field of assimilation when the number of proxy records is limited. Compared with the temperature reconstruction, the skill of precipitation reconstruction is relatively lower. The proxy records from the ocean contribute more to the temperature reconstruction skill with both assimilation methods. Finally, a new reanalysis product (NNU-2ka Reanalysis) is generated through the HGAOEnKF with the expanded proxy database.

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引用次数: 0
Anomalous temperature in North Tropical Atlantic linked to Brazilian Cerrado fires
IF 9 1区 地球科学 Q1 METEOROLOGY & ATMOSPHERIC SCIENCES Pub Date : 2025-02-21 DOI: 10.1038/s41612-025-00945-w
Hyo-Jeong Kim, Jin-Soo Kim, Yoo-Geun Ham, Jae-Heung Park, David Milodowski, Luiz E. O. C. Aragão, Mathew Williams

Brazilian Cerrado has the largest annual burned area (BA) in South America, with strong interannual variability. However, there is limited understanding of which climatic drivers lead to the interannual variability of Cerrado fires. This study found sea surface temperature anomalies (SSTAs) in the North Tropical Atlantic (NTA) are positively correlated with the Cerrado BA. Positive SSTAs over the NTA modulate the intertropical convergence zone (ITCZ) position, which suppresses atmospheric convection over the Cerrado region. While NTA SSTA peaks March, the precipitation reduction in Cerrado is pronounced during June–August, since the ITCZ shifts northward and the local monsoon weakens. This leads to moisture deficits for the following months, significantly enhancing fire activity in August–October. This result implies NTA can exert an independent influence on Cerrado in addition to the traditionally considered factor, the El Niño–Southern Oscillation. This improves the predictability of fire activity because NTA precedes the fire season by 7 months.

巴西的塞拉多地区是南美洲年烧毁面积最大的地区(BA),而且年际变化很大。然而,人们对导致塞拉多火灾年际变化的气候驱动因素了解有限。这项研究发现,北热带大西洋(NTA)的海面温度异常与 Cerrado BA 呈正相关。北热带大西洋的正海面温度异常会调节热带辐合带(ITCZ)的位置,从而抑制 Cerrado 地区的大气对流。虽然 NTA SSTA 在 3 月份达到峰值,但由于 ITCZ 向北移动,当地季风减弱,Cerrado 的降水量在 6-8 月份明显减少。这导致随后几个月的水汽不足,大大增加了 8-10 月的火灾活动。这一结果表明,除了传统意义上的厄尔尼诺-南方涛动因素外,NTA 还能对 Cerrado 产生独立的影响。这提高了火灾活动的可预测性,因为 NTA 比火灾季节早 7 个月。
{"title":"Anomalous temperature in North Tropical Atlantic linked to Brazilian Cerrado fires","authors":"Hyo-Jeong Kim, Jin-Soo Kim, Yoo-Geun Ham, Jae-Heung Park, David Milodowski, Luiz E. O. C. Aragão, Mathew Williams","doi":"10.1038/s41612-025-00945-w","DOIUrl":"https://doi.org/10.1038/s41612-025-00945-w","url":null,"abstract":"<p>Brazilian Cerrado has the largest annual burned area (BA) in South America, with strong interannual variability. However, there is limited understanding of which climatic drivers lead to the interannual variability of Cerrado fires. This study found sea surface temperature anomalies (SSTAs) in the North Tropical Atlantic (NTA) are positively correlated with the Cerrado BA. Positive SSTAs over the NTA modulate the intertropical convergence zone (ITCZ) position, which suppresses atmospheric convection over the Cerrado region. While NTA SSTA peaks March, the precipitation reduction in Cerrado is pronounced during June–August, since the ITCZ shifts northward and the local monsoon weakens. This leads to moisture deficits for the following months, significantly enhancing fire activity in August–October. This result implies NTA can exert an independent influence on Cerrado in addition to the traditionally considered factor, the El Niño–Southern Oscillation. This improves the predictability of fire activity because NTA precedes the fire season by 7 months.</p>","PeriodicalId":19438,"journal":{"name":"npj Climate and Atmospheric Science","volume":"37 1","pages":""},"PeriodicalIF":9.0,"publicationDate":"2025-02-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143470611","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"地球科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Beaufort sea ice loss contributes to enhanced health exposure to fire weather over Southeast Asia
IF 9 1区 地球科学 Q1 METEOROLOGY & ATMOSPHERIC SCIENCES Pub Date : 2025-02-20 DOI: 10.1038/s41612-025-00954-9
Guanyu Liu, Jing Li, Tong Ying, Yueming Dong, Zhenyu Zhang, Chongzhao Zhang, Qiurui Li

Fires are a major source of air pollutants in Southeast Asia. Over the past few decades, there has been an increase in fire activities in this region, and the causes are not entirely clear. By analyzing multiple observational and reanalysis datasets, as well as conducting climate model simulations, we uncover a distinct positive impact of Arctic sea ice loss on Southeast Asian fire weather. There is a possibility that the fall in the autumn Sea Ice Concentration (SIC) over the Beaufort Sea the year prior contributes to the increase in boreal spring fire activity in Southeast Asia. This sea ice reduction generates a local low warm anomaly, triggering an upper atmosphere Rossby wave train that propagates from the tropical Pacific to Southeast Asia and arrives in Southeast Asia as a high-pressure anomaly with descending air. Moreover, two meridional cells originating from equatorial and polar regions intensify the sinking airflow. This Arctic-driven teleconnection causes high pressure with warmer and dryer surfaces in Southeast Asia, creating favorable conditions for fire ignition and expansion. Based on the fire weather classification criteria, a negative change in SIC of one standard deviation below the climatological mean will expose over 500 million people to very high levels of fire pollution across Southeast Asia, and the number of people exposed to extreme fires will be 1000 times greater than in the present scenario. The above-mentioned mechanism has great implications for projecting decadal air quality and developing relevant health policies to cope with climate change in Southeast Asia.

{"title":"Beaufort sea ice loss contributes to enhanced health exposure to fire weather over Southeast Asia","authors":"Guanyu Liu, Jing Li, Tong Ying, Yueming Dong, Zhenyu Zhang, Chongzhao Zhang, Qiurui Li","doi":"10.1038/s41612-025-00954-9","DOIUrl":"https://doi.org/10.1038/s41612-025-00954-9","url":null,"abstract":"<p>Fires are a major source of air pollutants in Southeast Asia. Over the past few decades, there has been an increase in fire activities in this region, and the causes are not entirely clear. By analyzing multiple observational and reanalysis datasets, as well as conducting climate model simulations, we uncover a distinct positive impact of Arctic sea ice loss on Southeast Asian fire weather. There is a possibility that the fall in the autumn Sea Ice Concentration (SIC) over the Beaufort Sea the year prior contributes to the increase in boreal spring fire activity in Southeast Asia. This sea ice reduction generates a local low warm anomaly, triggering an upper atmosphere Rossby wave train that propagates from the tropical Pacific to Southeast Asia and arrives in Southeast Asia as a high-pressure anomaly with descending air. Moreover, two meridional cells originating from equatorial and polar regions intensify the sinking airflow. This Arctic-driven teleconnection causes high pressure with warmer and dryer surfaces in Southeast Asia, creating favorable conditions for fire ignition and expansion. Based on the fire weather classification criteria, a negative change in SIC of one standard deviation below the climatological mean will expose over 500 million people to very high levels of fire pollution across Southeast Asia, and the number of people exposed to extreme fires will be 1000 times greater than in the present scenario. The above-mentioned mechanism has great implications for projecting decadal air quality and developing relevant health policies to cope with climate change in Southeast Asia.</p>","PeriodicalId":19438,"journal":{"name":"npj Climate and Atmospheric Science","volume":"146 1","pages":""},"PeriodicalIF":9.0,"publicationDate":"2025-02-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143462912","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"地球科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Rapid decline and mortality of a Pleistocene-aged forest now submerged in the northern Gulf of Mexico, USA
IF 9 1区 地球科学 Q1 METEOROLOGY & ATMOSPHERIC SCIENCES Pub Date : 2025-02-20 DOI: 10.1038/s41612-025-00951-y
Grant L. Harley, Kristine L. DeLong, Marcus Lofverstrom, Carl Andy Reese, Ellen V. Bergan, Samuel J. Bentley, Kehui Xu, Kelli Moran, Karen E. King, Alicia Caporaso

The Gulf and Atlantic Coastal Plains of the southern United States are characterized by a wide continental shelf that was subaerially exposed for ca. 80,000 years during glacial-interval marine regressions and transgressions. Given their present submergence, little is known about the vegetation dynamics, particularly at annual time scales, of these formerly terrestrial sites due to erosional processes associated with marine transgressions. Here, we present an annually resolved and well-replicated 489-year tree-ring chronology from macrobotanical specimens—anatomically identified as Taxodium distichum (L.) Rich.—collected in situ from a recently exposed submerged forest in 18 m water depth in the northern Gulf of Mexico. This chronology not only reveals historical vegetation dynamics at annual resolutions during Marine Isotope Stages 3–5a, but it also captures a catastrophic mortality event likely connected to intense storm activity, perhaps driven by freshwater fluxes from Heinrich events. Our findings are supported by coupled climate model simulations from the last glaciation, providing new insights into the environmental history of the southeastern US coastal regions.

{"title":"Rapid decline and mortality of a Pleistocene-aged forest now submerged in the northern Gulf of Mexico, USA","authors":"Grant L. Harley, Kristine L. DeLong, Marcus Lofverstrom, Carl Andy Reese, Ellen V. Bergan, Samuel J. Bentley, Kehui Xu, Kelli Moran, Karen E. King, Alicia Caporaso","doi":"10.1038/s41612-025-00951-y","DOIUrl":"https://doi.org/10.1038/s41612-025-00951-y","url":null,"abstract":"<p>The Gulf and Atlantic Coastal Plains of the southern United States are characterized by a wide continental shelf that was subaerially exposed for ca. 80,000 years during glacial-interval marine regressions and transgressions. Given their present submergence, little is known about the vegetation dynamics, particularly at annual time scales, of these formerly terrestrial sites due to erosional processes associated with marine transgressions. Here, we present an annually resolved and well-replicated 489-year tree-ring chronology from macrobotanical specimens—anatomically identified as <i>Taxodium distichum</i> (L.) Rich.—collected in situ from a recently exposed submerged forest in 18 m water depth in the northern Gulf of Mexico. This chronology not only reveals historical vegetation dynamics at annual resolutions during Marine Isotope Stages 3–5a, but it also captures a catastrophic mortality event likely connected to intense storm activity, perhaps driven by freshwater fluxes from Heinrich events. Our findings are supported by coupled climate model simulations from the last glaciation, providing new insights into the environmental history of the southeastern US coastal regions.</p>","PeriodicalId":19438,"journal":{"name":"npj Climate and Atmospheric Science","volume":"1 1","pages":""},"PeriodicalIF":9.0,"publicationDate":"2025-02-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143462911","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"地球科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Age inequality in temperature-related fall mortality among old people in China in a warming climate
IF 9 1区 地球科学 Q1 METEOROLOGY & ATMOSPHERIC SCIENCES Pub Date : 2025-02-19 DOI: 10.1038/s41612-025-00939-8
Yi Lin, Jinlei Qi, Jianxiong Hu, Jiangmei Liu, Guanhao He, Peng Yin, Tao Liu, Ziqiang Lin, Fengrui Jing, Jinling You, Wenjun Ma, Maigeng Zhou

This study aimed to quantify the age-specific risk and burden of fall-related mortality attributable to ambient temperature among older adults in China. Using data in 2759 counties/districts during 2005–2022, we found that both high and low temperatures significantly increased the risk of fall-related mortality, with a notably higher risk associated with high temperatures, particularly among the oldest old and people in Southern China. Projections indicate that the fall-related mortality burden associated with temperature will increase in the future, primarily affecting the oldest old, and the increase is mainly driven by climate change. These findings highlight the need for effective adaptation strategies to reduce the impact of temperature on fall-related mortality among older adults, particularly facing double challenges of climate change and population aging.

{"title":"Age inequality in temperature-related fall mortality among old people in China in a warming climate","authors":"Yi Lin, Jinlei Qi, Jianxiong Hu, Jiangmei Liu, Guanhao He, Peng Yin, Tao Liu, Ziqiang Lin, Fengrui Jing, Jinling You, Wenjun Ma, Maigeng Zhou","doi":"10.1038/s41612-025-00939-8","DOIUrl":"https://doi.org/10.1038/s41612-025-00939-8","url":null,"abstract":"<p>This study aimed to quantify the age-specific risk and burden of fall-related mortality attributable to ambient temperature among older adults in China. Using data in 2759 counties/districts during 2005–2022, we found that both high and low temperatures significantly increased the risk of fall-related mortality, with a notably higher risk associated with high temperatures, particularly among the oldest old and people in Southern China. Projections indicate that the fall-related mortality burden associated with temperature will increase in the future, primarily affecting the oldest old, and the increase is mainly driven by climate change. These findings highlight the need for effective adaptation strategies to reduce the impact of temperature on fall-related mortality among older adults, particularly facing double challenges of climate change and population aging.</p>","PeriodicalId":19438,"journal":{"name":"npj Climate and Atmospheric Science","volume":"16 1","pages":""},"PeriodicalIF":9.0,"publicationDate":"2025-02-19","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143451906","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"地球科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Two contrasting tropical convection modes from the eastern Pacific to northern Africa that drive Eurasian teleconnections in boreal summer
IF 9 1区 地球科学 Q1 METEOROLOGY & ATMOSPHERIC SCIENCES Pub Date : 2025-02-18 DOI: 10.1038/s41612-025-00944-x
Zhiwei Zhu, Liaoyuan Shao, Rui Lu, Wenjian Hua

Eurasian teleconnections in boreal summer significantly influence regional climates and extremes, yet their dynamic origins remain largely unclear. Here, we revealed two critical modes of tropical convection that drive these Eurasian teleconnections in boreal summer. The first mode is characterized by suppressed convection in the equatorial eastern Pacific, coupled with enhanced convection extending from the equatorial Atlantic to northern Africa. In contrast, the second mode displays similar suppressed convection in the equatorial eastern Pacific, but features enhanced convection in the Gulf of Mexico and the equatorial Atlantic. These two modes result in markedly different atmospheric teleconnections, leading to distinct surface air temperature anomalies across the Eurasian continent. Both modes arise from the combined effects of sea surface temperature anomalies in the eastern Pacific and the North Atlantic/Indian Ocean. This study offers new insights into dynamics and seasonal predictions of boreal summer Eurasian climates.

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引用次数: 0
Sulfate formation through copper-catalyzed SO2 oxidation by NO2 at aerosol surfaces
IF 9 1区 地球科学 Q1 METEOROLOGY & ATMOSPHERIC SCIENCES Pub Date : 2025-02-18 DOI: 10.1038/s41612-025-00934-z
Pai Liu, Yu-Xin Liu, Qishen Huang, Xinyue Chao, Mingrui Zhong, Jiayi Yin, Xiaowu Zhang, Lin-Fang Li, Xi-Yuan Kang, Zhe Chen, Shufeng Pang, Weigang Wang, Yun-Hong Zhang, Maofa Ge

Severe urban air pollution in China is driven by a synergistic conversion of SO2, NOx, and NH3 into fine particulate matter (PM2.5). Field studies indicated NO2 as an important oxidizer to SO2 in polluted atmospheres with low photochemical reactivity, but this rapid reaction cannot be explained by the aqueous reactive nitrogen chemistry in acidic urban aerosols. Here, using an aerosol optical tweezer and Raman spectroscopy, we show that the multiphase SO2 oxidation by NO2 is accelerated for two-order-of-magnitude by a copper catalyst. This reaction occurs on aerosol surfaces, is independent of pH between 3 and 5, and produces sulfate by a rate of up to 10 µg m-3air hr-1 when reactive copper reaches a millimolar concentration in aerosol water – typical of severe haze events in North China Plain. Since copper and NO2 are companion emitters in air pollution, they can act synergistically in converting SO2 into sulfate in China’s haze.

{"title":"Sulfate formation through copper-catalyzed SO2 oxidation by NO2 at aerosol surfaces","authors":"Pai Liu, Yu-Xin Liu, Qishen Huang, Xinyue Chao, Mingrui Zhong, Jiayi Yin, Xiaowu Zhang, Lin-Fang Li, Xi-Yuan Kang, Zhe Chen, Shufeng Pang, Weigang Wang, Yun-Hong Zhang, Maofa Ge","doi":"10.1038/s41612-025-00934-z","DOIUrl":"https://doi.org/10.1038/s41612-025-00934-z","url":null,"abstract":"<p>Severe urban air pollution in China is driven by a synergistic conversion of SO<sub>2</sub>, NOx, and NH<sub>3</sub> into fine particulate matter (PM<sub>2.5</sub>). Field studies indicated NO<sub>2</sub> as an important oxidizer to SO<sub>2</sub> in polluted atmospheres with low photochemical reactivity, but this rapid reaction cannot be explained by the aqueous reactive nitrogen chemistry in acidic urban aerosols. Here, using an aerosol optical tweezer and Raman spectroscopy, we show that the multiphase SO<sub>2</sub> oxidation by NO<sub>2</sub> is accelerated for two-order-of-magnitude by a copper catalyst. This reaction occurs on aerosol surfaces, is independent of pH between 3 and 5, and produces sulfate by a rate of up to 10 µg m<sup>-3</sup><sub>air</sub> hr<sup>-1</sup> when reactive copper reaches a millimolar concentration in aerosol water – typical of severe haze events in North China Plain. Since copper and NO<sub>2</sub> are companion emitters in air pollution, they can act synergistically in converting SO<sub>2</sub> into sulfate in China’s haze.</p>","PeriodicalId":19438,"journal":{"name":"npj Climate and Atmospheric Science","volume":"24 1","pages":""},"PeriodicalIF":9.0,"publicationDate":"2025-02-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143443721","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"地球科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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npj Climate and Atmospheric Science
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