首页 > 最新文献

Radiation Measurements最新文献

英文 中文
A survey of dosimetry capabilities and trends in Latin America and the Caribbean region: Implications for occupational dosimetry 拉丁美洲和加勒比区域剂量学能力和趋势调查:对职业剂量学的影响
IF 2.2 3区 物理与天体物理 Q2 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2026-02-06 DOI: 10.1016/j.radmeas.2026.107636
Juan C. Mora , Mariella Terán , Helen Khoury , Daniel Molina , Patricia Mora , Nancy Puerta , Leslie Anne Vironneau Janicek , Sebastian Gossio , Denison de Souza-Santos , Omar Garcia , Julieta Rearte , Marina Di Giorgio , V. Correcher
<div><div>This study presents a comprehensive regional assessment of dosimetry capabilities in Latin America and the Caribbean countries (LAC). The study was conducted using surveys coordinated, elaborated and analyzed by the steering committee of the Latin American Network for the Optimization of Occupational Radiation Protection (REPROLAM). All the work was supported by the Technical Cooperation of International Atomic Energy Agency (TC IAEA) through the RLA9088 and RLA9091 regional projects. The investigation covers five different dosimetry fields: external, internal, computational, biological, and retrospective dosimetry. Answers from participants of 16 countries were received: A total of 32 individual monitoring services for external dosimetry, 24 centers for internal dosimetry, 38 researchers for computational dosimetry, 12 biological dosimetry laboratories members of the Latin American Biological Dosimetry Network (LBDNet), and 16 retrospective dosimetry facilities. In the case of external dosimetry, an analysis of the results from 13 countries reveals that thermoluminescent dosimetry (TLD) remains the main technology for external monitoring (79% of services), with a growing adoption of optically stimulated luminescence dosimetry (OSLD) systems. Using both TLD and OSLD, over 160,000 occupationally exposed workers are monitored regionally, predominantly in medical applications (75%). Internal dosimetry services (16 direct, 15 indirect services) focus primarily on thyroid monitoring due to extensive <span><math><mrow><msup><mrow></mrow><mrow><mn>131</mn></mrow></msup><mi>I</mi></mrow></math></span> use in nuclear medicine in the region, but the results showed a lack of homogeneity in calibration and reporting levels. Monte Carlo-based computational dosimetry employs MCNP as the preferred code (25% of users). Biological dosimetry is well-established in the region through the LBDNet, with 21 laboratories capable of performing dicentric chromosome assays for emergency triage. LBDNet demonstrated to be a robust emergency response network. Retrospective dosimetry in the region relies predominantly on luminescence techniques. While dosimetry laboratories and techniques are well established in the region, several gaps have been identified which should be addressed in further approaches. These gaps include insufficient implementation of lens of the eye dosimetry (<span><math><mrow><msub><mrow><mi>H</mi></mrow><mrow><mi>p</mi></mrow></msub><mrow><mo>(</mo><mn>3</mn><mo>)</mo></mrow></mrow></math></span>), limited neutron dosimetry capacity, poor implementation of quality management system (60% of the IMS) and insufficient ISO/IEC 17025 accreditation (70% of those implementing a QMS, i.e. 42% of the total), a lack of standardized internal dosimetry protocols in the different laboratories, and the need for organizing periodic regional intercomparison exercises, which started with the 2023 intercomparison. The results of these surveys provide a baseline
本研究对拉丁美洲和加勒比国家(LAC)的剂量学能力进行了全面的区域评估。这项研究是利用拉丁美洲最佳职业辐射防护网络指导委员会协调、拟订和分析的调查进行的。所有工作均由国际原子能机构技术合作(TC IAEA)通过RLA9088和RLA9091区域项目提供支持。调查涵盖五个不同的剂量学领域:外部、内部、计算、生物和回顾性剂量学。收到了来自16个国家参与者的答复:共有32个外部剂量学单独监测服务机构、24个内部剂量学中心、38个计算剂量学研究人员、12个拉丁美洲生物剂量学网络成员生物剂量学实验室和16个回顾性剂量学设施。在外部剂量测定方面,对来自13个国家的结果的分析表明,热释光剂量测定(TLD)仍然是外部监测的主要技术(79%的服务),越来越多地采用光激发发光剂量测定(OSLD)系统。使用TLD和OSLD,区域监测了16万多名职业暴露工人,主要是在医疗应用中(75%)。内部剂量测定服务(16个直接服务,15个间接服务)主要侧重于甲状腺监测,因为该地区在核医学中广泛使用了131 - i,但结果显示校准和报告水平缺乏同质性。基于蒙特卡罗的计算剂量学采用MCNP作为首选代码(25%的用户)。生物剂量学通过LBDNet在该区域建立了完善的体系,有21个实验室能够为紧急分诊进行双中心染色体测定。LBDNet已被证明是一个强大的应急响应网络。该地区的回顾性剂量测定主要依靠发光技术。虽然该区域已建立剂量测定实验室和技术,但已经确定了一些差距,应在进一步的方法中加以解决。这些差距包括眼球透镜剂量测定(Hp(3))实施不足,中子剂量测定能力有限,质量管理体系实施不力(IMS的60%)和ISO/IEC 17025认证不足(实施质量管理体系的70%,即总数的42%),不同实验室缺乏标准化的内部剂量测定方案,以及需要组织定期的区域相互比较演习,从2023年开始相互比较。这些调查的结果为本区域剂量学基础设施的发展提供了一个基线,包括支持相互比较演习和培训倡议,以加强各国的职业辐射防护。原子能机构和其他组织继续支持这些国家的发展,对于优化工人的辐射防护是必不可少的。
{"title":"A survey of dosimetry capabilities and trends in Latin America and the Caribbean region: Implications for occupational dosimetry","authors":"Juan C. Mora ,&nbsp;Mariella Terán ,&nbsp;Helen Khoury ,&nbsp;Daniel Molina ,&nbsp;Patricia Mora ,&nbsp;Nancy Puerta ,&nbsp;Leslie Anne Vironneau Janicek ,&nbsp;Sebastian Gossio ,&nbsp;Denison de Souza-Santos ,&nbsp;Omar Garcia ,&nbsp;Julieta Rearte ,&nbsp;Marina Di Giorgio ,&nbsp;V. Correcher","doi":"10.1016/j.radmeas.2026.107636","DOIUrl":"10.1016/j.radmeas.2026.107636","url":null,"abstract":"&lt;div&gt;&lt;div&gt;This study presents a comprehensive regional assessment of dosimetry capabilities in Latin America and the Caribbean countries (LAC). The study was conducted using surveys coordinated, elaborated and analyzed by the steering committee of the Latin American Network for the Optimization of Occupational Radiation Protection (REPROLAM). All the work was supported by the Technical Cooperation of International Atomic Energy Agency (TC IAEA) through the RLA9088 and RLA9091 regional projects. The investigation covers five different dosimetry fields: external, internal, computational, biological, and retrospective dosimetry. Answers from participants of 16 countries were received: A total of 32 individual monitoring services for external dosimetry, 24 centers for internal dosimetry, 38 researchers for computational dosimetry, 12 biological dosimetry laboratories members of the Latin American Biological Dosimetry Network (LBDNet), and 16 retrospective dosimetry facilities. In the case of external dosimetry, an analysis of the results from 13 countries reveals that thermoluminescent dosimetry (TLD) remains the main technology for external monitoring (79% of services), with a growing adoption of optically stimulated luminescence dosimetry (OSLD) systems. Using both TLD and OSLD, over 160,000 occupationally exposed workers are monitored regionally, predominantly in medical applications (75%). Internal dosimetry services (16 direct, 15 indirect services) focus primarily on thyroid monitoring due to extensive &lt;span&gt;&lt;math&gt;&lt;mrow&gt;&lt;msup&gt;&lt;mrow&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mn&gt;131&lt;/mn&gt;&lt;/mrow&gt;&lt;/msup&gt;&lt;mi&gt;I&lt;/mi&gt;&lt;/mrow&gt;&lt;/math&gt;&lt;/span&gt; use in nuclear medicine in the region, but the results showed a lack of homogeneity in calibration and reporting levels. Monte Carlo-based computational dosimetry employs MCNP as the preferred code (25% of users). Biological dosimetry is well-established in the region through the LBDNet, with 21 laboratories capable of performing dicentric chromosome assays for emergency triage. LBDNet demonstrated to be a robust emergency response network. Retrospective dosimetry in the region relies predominantly on luminescence techniques. While dosimetry laboratories and techniques are well established in the region, several gaps have been identified which should be addressed in further approaches. These gaps include insufficient implementation of lens of the eye dosimetry (&lt;span&gt;&lt;math&gt;&lt;mrow&gt;&lt;msub&gt;&lt;mrow&gt;&lt;mi&gt;H&lt;/mi&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mi&gt;p&lt;/mi&gt;&lt;/mrow&gt;&lt;/msub&gt;&lt;mrow&gt;&lt;mo&gt;(&lt;/mo&gt;&lt;mn&gt;3&lt;/mn&gt;&lt;mo&gt;)&lt;/mo&gt;&lt;/mrow&gt;&lt;/mrow&gt;&lt;/math&gt;&lt;/span&gt;), limited neutron dosimetry capacity, poor implementation of quality management system (60% of the IMS) and insufficient ISO/IEC 17025 accreditation (70% of those implementing a QMS, i.e. 42% of the total), a lack of standardized internal dosimetry protocols in the different laboratories, and the need for organizing periodic regional intercomparison exercises, which started with the 2023 intercomparison. The results of these surveys provide a baseline","PeriodicalId":21055,"journal":{"name":"Radiation Measurements","volume":"193 ","pages":"Article 107636"},"PeriodicalIF":2.2,"publicationDate":"2026-02-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146122549","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Summing-induced signal distortion mechanisms and suppression methods in SiPM array gamma spectroscopy detectors SiPM阵列伽玛能谱探测器中和致信号失真机理及抑制方法
IF 2.2 3区 物理与天体物理 Q2 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2026-02-05 DOI: 10.1016/j.radmeas.2026.107633
Bao Wang , Xiongjie Zhang , Dongyang Wang , Wenming Dong , Dong Li , Shiliang Liu , Haoran Zhang , Jiangni Liu , Haixian Zhou , Qi Liu , Haitao Wang , Ning Chen , Renbo Wang
Pulse height analysis (PHA) is commonly used in scintillation γ-ray spectroscopy because it is simple and fast. However, in systems utilizing summed outputs from multi-channel silicon photomultiplier (SiPM) arrays, PHA becomes increasingly susceptible to waveform distortions inherent to the summing architecture. Such distortions alter the signal shape and significantly degrade the energy resolution. In this study, we systematically investigate the characteristics and origins of such abnormal signals using a 16-channel SiPM array coupled to a NaI(Tl) scintillator. By analyzing the pulse area-to-height ratio distributions, we show that summing-induced distortions tend to exhibit broadened pulse shapes and deviate significantly from the single-event signal profile. To mitigate this issue, a threshold-based waveform discrimination method is introduced. This method identifies and rejects abnormal pulses based on receiver operating characteristic (ROC) curve optimization, offering practical improvement in spectral performance when PHA must be retained for speed or simplicity. However, waveform correction alone cannot restore distorted signals. To address this limitation, we further explore pulse area analysis (PAA) as an alternative approach that is inherently less sensitive to distortion effects. Our experiments show that PAA improves energy resolution by 24.25% over conventional PHA, reaching 9.40% at 662 keV. These findings highlight the limitations of amplitude-based methods under summed readout architectures and suggest that PAA, when applicable, offers a more robust solution for compact gamma spectroscopy using SiPM arrays. This work provides both theoretical insights and practical strategies for mitigating signal anomalies in modern scintillation detectors.
脉冲高度分析(PHA)是闪烁γ射线光谱分析中常用的一种方法,具有简单、快速等优点。然而,在利用多通道硅光电倍增管(SiPM)阵列的求和输出的系统中,PHA越来越容易受到求和结构固有的波形畸变的影响。这样的失真改变了信号的形状并显著降低了能量分辨率。在这项研究中,我们系统地研究了这种异常信号的特征和来源,使用16通道SiPM阵列耦合到NaI(Tl)闪烁体。通过分析脉冲的面积与高度比分布,我们发现叠加引起的畸变倾向于表现出宽的脉冲形状,并明显偏离单事件信号轮廓。为了解决这一问题,提出了一种基于阈值的波形判别方法。该方法基于接收机工作特性(ROC)曲线优化来识别和抑制异常脉冲,在为速度或简单而必须保留PHA的情况下,可切实提高光谱性能。然而,仅靠波形校正无法恢复失真信号。为了解决这一限制,我们进一步探索脉冲面积分析(PAA)作为一种固有的对失真效应不太敏感的替代方法。实验表明,PAA的能量分辨率比传统PHA提高了24.25%,在662 keV时达到9.40%。这些发现突出了基于振幅的方法在总结读出架构下的局限性,并表明PAA在适用的情况下,为使用SiPM阵列的紧凑伽马能谱提供了更强大的解决方案。这项工作为减轻现代闪烁探测器中的信号异常提供了理论见解和实践策略。
{"title":"Summing-induced signal distortion mechanisms and suppression methods in SiPM array gamma spectroscopy detectors","authors":"Bao Wang ,&nbsp;Xiongjie Zhang ,&nbsp;Dongyang Wang ,&nbsp;Wenming Dong ,&nbsp;Dong Li ,&nbsp;Shiliang Liu ,&nbsp;Haoran Zhang ,&nbsp;Jiangni Liu ,&nbsp;Haixian Zhou ,&nbsp;Qi Liu ,&nbsp;Haitao Wang ,&nbsp;Ning Chen ,&nbsp;Renbo Wang","doi":"10.1016/j.radmeas.2026.107633","DOIUrl":"10.1016/j.radmeas.2026.107633","url":null,"abstract":"<div><div>Pulse height analysis (PHA) is commonly used in scintillation γ-ray spectroscopy because it is simple and fast. However, in systems utilizing summed outputs from multi-channel silicon photomultiplier (SiPM) arrays, PHA becomes increasingly susceptible to waveform distortions inherent to the summing architecture. Such distortions alter the signal shape and significantly degrade the energy resolution. In this study, we systematically investigate the characteristics and origins of such abnormal signals using a 16-channel SiPM array coupled to a NaI(Tl) scintillator. By analyzing the pulse area-to-height ratio distributions, we show that summing-induced distortions tend to exhibit broadened pulse shapes and deviate significantly from the single-event signal profile. To mitigate this issue, a threshold-based waveform discrimination method is introduced. This method identifies and rejects abnormal pulses based on receiver operating characteristic (ROC) curve optimization, offering practical improvement in spectral performance when PHA must be retained for speed or simplicity. However, waveform correction alone cannot restore distorted signals. To address this limitation, we further explore pulse area analysis (PAA) as an alternative approach that is inherently less sensitive to distortion effects. Our experiments show that PAA improves energy resolution by 24.25% over conventional PHA, reaching 9.40% at 662 keV. These findings highlight the limitations of amplitude-based methods under summed readout architectures and suggest that PAA, when applicable, offers a more robust solution for compact gamma spectroscopy using SiPM arrays. This work provides both theoretical insights and practical strategies for mitigating signal anomalies in modern scintillation detectors.</div></div>","PeriodicalId":21055,"journal":{"name":"Radiation Measurements","volume":"193 ","pages":"Article 107633"},"PeriodicalIF":2.2,"publicationDate":"2026-02-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146122749","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Design of a collimator-free SPECT system based on multi-layer grid scintillator array 基于多层网格闪烁体阵列的无准直器SPECT系统设计
IF 2.2 3区 物理与天体物理 Q2 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2026-02-03 DOI: 10.1016/j.radmeas.2026.107631
Xue Yang , Changran Geng , Lu Han , Feng Tian , Ningxin Dong , Xiaobin Tang
Traditional single-photon emission computed tomography (SPECT) systems exhibit a tradeoff between spatial resolution and sensitivity because of the use of mechanical collimators. To address this issue, this paper proposes a collimator-free SPECT detector design based on a staggered multilayer grid scintillator array, to enable image reconstruction without requiring conventional mechanical collimation. Based on the experimental and simulation results, the system parameters were evaluated and a practical configuration incorporating 25 mm-long elongated scintillators, 6 mm-thick grid layers, and 40 mm layer spacing was established. To preliminarily assess the clinical-scale system performance, a clinical-scale system featuring a 15-detector annular array with a 300 mm rotation radius was simulated to emulate realistic cardiac SPECT imaging conditions. The results demonstrated that the system had a 0.76% detection efficiency on a clinical scale (compared to 0.1% for conventional SPECT), successfully resolving point sources spaced 2 mm apart. The cylinder model imaging results demonstrated that the mean activity recovery coefficient (ARC) of the reconstructed images for each cylinder was between 0.5 and 0.6. This preliminary result validates the feasibility of a collimator-free SPECT system and lays the foundation for further improvements in reconstruction accuracy. The proposed approach offers a potentially viable solution for concurrently enhancing spatial resolution and detection sensitivity in SPECT systems, with promising applications in myocardial perfusion imaging.
传统的单光子发射计算机断层扫描(SPECT)系统表现出空间分辨率和灵敏度之间的权衡,因为使用机械准直器。为了解决这一问题,本文提出了一种基于交错多层网格闪烁体阵列的无准直器SPECT检测器设计,使图像重建无需传统的机械准直。基于实验和仿真结果,对系统参数进行了评估,建立了长度为25 mm的细长闪烁体、厚度为6 mm的栅格层、层间距为40 mm的实际配置。为了初步评估临床规模系统的性能,模拟了一个临床规模系统,该系统具有15个检测器环形阵列,旋转半径为300 mm,以模拟真实的心脏SPECT成像条件。结果表明,该系统在临床规模上的检测效率为0.76%(相比之下,传统SPECT的检测效率为0.1%),成功地分辨出间隔2mm的点源。柱模型成像结果表明,每个柱的平均活度恢复系数(ARC)在0.5 ~ 0.6之间。该初步结果验证了无准直器SPECT系统的可行性,为进一步提高重建精度奠定了基础。该方法为同时提高SPECT系统的空间分辨率和检测灵敏度提供了一种潜在可行的解决方案,在心肌灌注成像中具有广阔的应用前景。
{"title":"Design of a collimator-free SPECT system based on multi-layer grid scintillator array","authors":"Xue Yang ,&nbsp;Changran Geng ,&nbsp;Lu Han ,&nbsp;Feng Tian ,&nbsp;Ningxin Dong ,&nbsp;Xiaobin Tang","doi":"10.1016/j.radmeas.2026.107631","DOIUrl":"10.1016/j.radmeas.2026.107631","url":null,"abstract":"<div><div>Traditional single-photon emission computed tomography (SPECT) systems exhibit a tradeoff between spatial resolution and sensitivity because of the use of mechanical collimators. To address this issue, this paper proposes a collimator-free SPECT detector design based on a staggered multilayer grid scintillator array, to enable image reconstruction without requiring conventional mechanical collimation. Based on the experimental and simulation results, the system parameters were evaluated and a practical configuration incorporating 25 mm-long elongated scintillators, 6 mm-thick grid layers, and 40 mm layer spacing was established. To preliminarily assess the clinical-scale system performance, a clinical-scale system featuring a 15-detector annular array with a 300 mm rotation radius was simulated to emulate realistic cardiac SPECT imaging conditions. The results demonstrated that the system had a 0.76% detection efficiency on a clinical scale (compared to 0.1% for conventional SPECT), successfully resolving point sources spaced 2 mm apart. The cylinder model imaging results demonstrated that the mean activity recovery coefficient (ARC) of the reconstructed images for each cylinder was between 0.5 and 0.6. This preliminary result validates the feasibility of a collimator-free SPECT system and lays the foundation for further improvements in reconstruction accuracy. The proposed approach offers a potentially viable solution for concurrently enhancing spatial resolution and detection sensitivity in SPECT systems, with promising applications in myocardial perfusion imaging.</div></div>","PeriodicalId":21055,"journal":{"name":"Radiation Measurements","volume":"193 ","pages":"Article 107631"},"PeriodicalIF":2.2,"publicationDate":"2026-02-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146122748","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Characterization of lithium fluoride fluorescent nuclear track detectors for linear energy transfer measurements in light-ion beams using confocal microscopy 用共聚焦显微镜表征用于光离子束线性能量传递测量的氟化锂荧光核径迹探测器
IF 2.2 3区 物理与天体物理 Q2 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2026-01-24 DOI: 10.1016/j.radmeas.2026.107623
I.D. Muñoz , M. Sankowska , A. Kilian , O. Jäkel , P. Bilski
Fluorescent nuclear track detectors (FNTDs) enable measurement of the linear energy transfer (LET) of heavy charged particles. Lithium fluoride (LiF) is widely used in solid-state dosimetry and has been shown to function as an FNTD, with all previous studies employing wide-field microscopy (WM). Compared with WM, confocal microscopy (CM) – while more complex and time-consuming – provides superior image quality, potentially allowing improved ion track visualization and detection. This study aims to establish the feasibility of imaging LiF crystals with CM to visualize ion tracks and measure LET. Single LiF crystals were irradiated with high-energy quasi-monoenergetic 4He-, 12C-, and 16O-ions. Following irradiation, samples underwent thermal treatment to enhance fluorescence intensity and were subsequently imaged with a confocal microscope. Single-ion tracks were reconstructed from the resulting images, and fluorescence intensity was correlated with the LET in water (LETw). The results demonstrate that it is feasible to image single ion tracks in LiF using CM. Detection efficiency reached nearly 100 % for 16O-ions at LETw = 50.4 keV μm−1 and for 12C-ions at (31.8 and 10.6) keV μm−1. Reduced efficiencies (∼50 %) were observed for 16O-ions at 18.9 keV μm−1 and for 12C-ions at 17.9 keV μm−1. For 4He-ions, the efficiency was approximately 30 %. The mean fluorescence track intensity increased with LETw, consistent with previous findings. CM shows potential for LET measurements using LiF-based FNTDs. However, at this stage, no significant improvement was observed for CM compared with WM.
荧光核径迹探测器(FNTDs)能够测量重带电粒子的线性能量传递(LET)。氟化锂(LiF)广泛应用于固态剂量学,并已被证明具有FNTD的功能,所有先前的研究都采用宽视场显微镜(WM)。与WM相比,共聚焦显微镜(CM)虽然更复杂和耗时,但提供了更好的图像质量,有可能改善离子轨迹的可视化和检测。本研究旨在建立用CM成像LiF晶体以显示离子轨迹和测量LET的可行性。用高能准单能4He-、12C-和16o -离子辐照单晶。辐照后,对样品进行热处理以增强荧光强度,随后用共聚焦显微镜成像。根据所得图像重建了单离子轨迹,荧光强度与水中LET (LETw)相关。结果表明,用CM成像LiF中单离子轨迹是可行的。在lew = 50.4 keV μm - 1和(31.8和10.6)keV μm - 1下,16o -离子和12c -离子的检测效率接近100%。在18.9 keV μm - 1和17.9 keV μm - 1下,16o离子和12c离子的效率分别降低了50%。对于4he离子,效率约为30%。平均荧光径迹强度随LETw增加而增加,与先前的发现一致。CM显示了使用基于liff的FNTDs进行LET测量的潜力。然而,在这个阶段,与WM相比,CM没有明显的改善。
{"title":"Characterization of lithium fluoride fluorescent nuclear track detectors for linear energy transfer measurements in light-ion beams using confocal microscopy","authors":"I.D. Muñoz ,&nbsp;M. Sankowska ,&nbsp;A. Kilian ,&nbsp;O. Jäkel ,&nbsp;P. Bilski","doi":"10.1016/j.radmeas.2026.107623","DOIUrl":"10.1016/j.radmeas.2026.107623","url":null,"abstract":"<div><div>Fluorescent nuclear track detectors (FNTDs) enable measurement of the linear energy transfer (LET) of heavy charged particles. Lithium fluoride (LiF) is widely used in solid-state dosimetry and has been shown to function as an FNTD, with all previous studies employing wide-field microscopy (WM). Compared with WM, confocal microscopy (CM) – while more complex and time-consuming – provides superior image quality, potentially allowing improved ion track visualization and detection. This study aims to establish the feasibility of imaging LiF crystals with CM to visualize ion tracks and measure LET. Single LiF crystals were irradiated with high-energy quasi-monoenergetic <sup>4</sup>He-, <sup>12</sup>C-, and <sup>16</sup>O-ions. Following irradiation, samples underwent thermal treatment to enhance fluorescence intensity and were subsequently imaged with a confocal microscope. Single-ion tracks were reconstructed from the resulting images, and fluorescence intensity was correlated with the LET in water (LET<sub>w</sub>). The results demonstrate that it is feasible to image single ion tracks in LiF using CM. Detection efficiency reached nearly 100 % for <sup>16</sup>O-ions at LET<sub>w</sub> = 50.4 keV μm<sup>−1</sup> and for <sup>12</sup>C-ions at (31.8 and 10.6) keV μm<sup>−1</sup>. Reduced efficiencies (∼50 %) were observed for <sup>16</sup>O-ions at 18.9 keV μm<sup>−1</sup> and for <sup>12</sup>C-ions at 17.9 keV μm<sup>−1</sup>. For <sup>4</sup>He-ions, the efficiency was approximately 30 %. The mean fluorescence track intensity increased with LET<sub>w</sub>, consistent with previous findings. CM shows potential for LET measurements using LiF-based FNTDs. However, at this stage, no significant improvement was observed for CM compared with WM.</div></div>","PeriodicalId":21055,"journal":{"name":"Radiation Measurements","volume":"192 ","pages":"Article 107623"},"PeriodicalIF":2.2,"publicationDate":"2026-01-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146078831","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Optimizing the feasibility of N-Vinyl caprolactam polymer gel dosimeter using saccharide sensitizer for medical dosimetry 糖敏化剂优化n -乙烯基己内酰胺聚合物凝胶剂量计用于医学剂量测定的可行性
IF 2.2 3区 物理与天体物理 Q2 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2026-01-16 DOI: 10.1016/j.radmeas.2026.107622
Molham M. Eyadeh , Khalid A. Rabaeh , Dua'a I. Bani Hamdan , Ali M. Almomani
In this work, the influence of glucose on the dose sensitivity of N-vinyl caprolactam based gel dosimeters (NVCL) is studied. Moreover, the radiation properties of the NVCL-glucose gel dosimeters such as temperature dependence, dose rate and energy dependence and temporal stability were investigated. The improved NVCL-glucose polymers were exposed to megavoltage photon beams from a medical linear accelerator at doses up to 20 Gy. The exposures were carried out at photon energies of 6–15 MV, dose rates between 50 and 500 cGy/min, and temperatures ranging from 10 °C to 30 °C. The transverse relaxation rate (R2) of the gel samples was measured using a time-domain NMR relaxometer with a magnetic field strength of 0.5 T. The R2-dose response was found to be linear up to a radiation dose of 10 Gy, where the dose sensitivity of the improved polymers exhibited a significant enhancement, achieving 0.37 s−1 Gy−1, which is twice the R2-dose sensitivity of previous NVCL systems. Additionally, it was observed that the NVCL-glucose polymers were independent of dose rate and radiation energy. A decrease in R2 dose sensitivity was observed with increasing scanning temperature. The optimized NVCL–glucose formulation remained stable for at least 7 days after irradiation, with no significant change in the R2 dose response over this period. These findings highlight the potential of NVCL-glucose dosimeters for practical application in MRI/NMR based 3-D dose verification.
本文研究了葡萄糖对n -乙烯基己内酰胺凝胶剂量计(NVCL)剂量敏感性的影响。此外,研究了nvcl -葡萄糖凝胶剂量仪的温度依赖性、剂量率依赖性和能量依赖性以及时间稳定性。将改进的nvcl -葡萄糖聚合物暴露于来自医用直线加速器的高达20 Gy的兆伏光子光束中。照射的光子能量为6 ~ 15 MV,剂量率为50 ~ 500 cGy/min,温度为10℃~ 30℃。利用0.5 t磁场强度的时域核磁共振弛豫仪测量了凝胶样品的横向弛豫率(R2),发现R2剂量响应在辐射剂量为10 Gy时呈线性,其中改进聚合物的剂量灵敏度显着增强,达到0.37 s−1 Gy−1,是以前NVCL系统R2剂量灵敏度的两倍。此外,还观察到nvcl -葡萄糖聚合物与剂量率和辐射能量无关。R2剂量敏感性随扫描温度升高而降低。优化后的nvcl -葡萄糖制剂在辐照后至少7天保持稳定,在此期间R2剂量反应没有显著变化。这些发现突出了nvcl -葡萄糖剂量计在基于MRI/NMR的三维剂量验证中的实际应用潜力。
{"title":"Optimizing the feasibility of N-Vinyl caprolactam polymer gel dosimeter using saccharide sensitizer for medical dosimetry","authors":"Molham M. Eyadeh ,&nbsp;Khalid A. Rabaeh ,&nbsp;Dua'a I. Bani Hamdan ,&nbsp;Ali M. Almomani","doi":"10.1016/j.radmeas.2026.107622","DOIUrl":"10.1016/j.radmeas.2026.107622","url":null,"abstract":"<div><div>In this work, the influence of glucose on the dose sensitivity of N-vinyl caprolactam based gel dosimeters (NVCL) is studied. Moreover, the radiation properties of the NVCL-glucose gel dosimeters such as temperature dependence, dose rate and energy dependence and temporal stability were investigated. The improved NVCL-glucose polymers were exposed to megavoltage photon beams from a medical linear accelerator at doses up to 20 Gy. The exposures were carried out at photon energies of 6–15 MV, dose rates between 50 and 500 cGy/min, and temperatures ranging from 10 °C to 30 °C. The transverse relaxation rate (R<sub>2</sub>) of the gel samples was measured using a time-domain NMR relaxometer with a magnetic field strength of 0.5 T. The R<sub>2</sub>-dose response was found to be linear up to a radiation dose of 10 Gy, where the dose sensitivity of the improved polymers exhibited a significant enhancement, achieving 0.37 s<sup>−1</sup> Gy<sup>−1</sup>, which is twice the R<sub>2</sub>-dose sensitivity of previous NVCL systems. Additionally, it was observed that the NVCL-glucose polymers were independent of dose rate and radiation energy. A decrease in R<sub>2</sub> dose sensitivity was observed with increasing scanning temperature. The optimized NVCL–glucose formulation remained stable for at least 7 days after irradiation, with no significant change in the R<sub>2</sub> dose response over this period. These findings highlight the potential of NVCL-glucose dosimeters for practical application in MRI/NMR based 3-D dose verification.</div></div>","PeriodicalId":21055,"journal":{"name":"Radiation Measurements","volume":"192 ","pages":"Article 107622"},"PeriodicalIF":2.2,"publicationDate":"2026-01-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146039055","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Radiation exposure assessment in interventional radiology: Staff personal dosimetry and radiation protection in percutaneous transhepatic cholangiography 介入放射学中的辐射暴露评估:工作人员个人剂量测定和经皮经肝胆管造影中的辐射防护
IF 2.2 3区 物理与天体物理 Q2 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2026-01-16 DOI: 10.1016/j.radmeas.2026.107621
Isaías Petronis , Denise Y. Nersissian , Francisco S. Cancio , Nancy K. Umisedo , Elisabeth M. Yoshimura
Interventional radiology (IR) procedures are the key source of radiation exposure for healthcare workers. Personal dosimetry is essential to ensure that dose limits are respected and radiation protection is maintained. This study aimed to estimate the average radiation dose received by the healthcare team during the most common IR procedure at a university hospital in São Paulo, Brasil. Cumulative personal dose equivalent, Hp(10), was measured outside the lead apron using thermoluminescent dosimetry (TL) in 57 percutaneous transhepatic biliary cholangiography procedures, divided into biliary drain insertions and biliary drain replacement. Three interventional radiologists participate in each procedure, with distinct roles and positions around the patient. The effective dose per procedure for the three roles of the interventional radiologists were estimated. For the primary interventional radiologist, the values were (54 ± 2) μSv and (32 ± 1) μSv in primary drain insertion and drain replacement, respectively. Additionally, as patient dose indicator, the kerma-area product medians were estimated as 34.3 Gy cm2 and 13.4 Gy cm2 in primary drain insertions and drain replacements, respectively. Under controlled equipment settings, which simulates clinical procedures with acrylic slabs, TL readings showed strong linear correlations with measurements from an ionization chamber (R2 = 0.979) and with the equipment dose indicator. The expected relationship between patient and staff doses was confirmed, in both clinical procedures and controlled settings. Finally, based on the results, recommendations were made regarding radiation protection at this facility, aiming to reduce both patient and staff exposure during this procedure.
介入放射(IR)程序是卫生保健工作者辐照的主要来源。个人剂量测定对于确保遵守剂量限值和维持辐射防护至关重要。本研究旨在估计巴西圣保罗一所大学医院的医疗团队在最常见的IR过程中接受的平均辐射剂量。在57例经皮经肝胆道造影手术中,采用热释光剂量法(TL)测量铅圈外累积个人剂量当量Hp(10),分为胆道插入和胆道置换。每个手术都有三位介入放射科医生参与,他们在患者周围扮演着不同的角色和位置。估计了介入放射科医生三个角色的每次手术的有效剂量。对于初级介入放射科医师,初级插入引流管和更换引流管的数值分别为(54±2)μSv和(32±1)μSv。此外,作为患者剂量指标,初次插入引流管和更换引流管时的角膜面积产物中值分别估计为34.3 Gy cm2和13.4 Gy cm2。在受控的设备设置下,用丙烯酸板模拟临床程序,TL读数与电离室的测量值(R2 = 0.979)和设备剂量指示器显示出很强的线性相关性。在临床程序和对照环境中,证实了患者和工作人员剂量之间的预期关系。最后,根据结果,对该设施的辐射防护提出了建议,旨在减少患者和工作人员在此过程中的暴露。
{"title":"Radiation exposure assessment in interventional radiology: Staff personal dosimetry and radiation protection in percutaneous transhepatic cholangiography","authors":"Isaías Petronis ,&nbsp;Denise Y. Nersissian ,&nbsp;Francisco S. Cancio ,&nbsp;Nancy K. Umisedo ,&nbsp;Elisabeth M. Yoshimura","doi":"10.1016/j.radmeas.2026.107621","DOIUrl":"10.1016/j.radmeas.2026.107621","url":null,"abstract":"<div><div>Interventional radiology (IR) procedures are the key source of radiation exposure for healthcare workers. Personal dosimetry is essential to ensure that dose limits are respected and radiation protection is maintained. This study aimed to estimate the average radiation dose received by the healthcare team during the most common IR procedure at a university hospital in <em>São Paulo,</em> <em>Bra</em><em>s</em><em>il</em>. Cumulative personal dose equivalent, <em>H</em><sub>p</sub>(10), was measured outside the lead apron using thermoluminescent dosimetry (TL) in 57 percutaneous transhepatic biliary cholangiography procedures, divided into biliary drain insertions and biliary drain replacement. Three interventional radiologists participate in each procedure, with distinct roles and positions around the patient. The effective dose per procedure for the three roles of the interventional radiologists were estimated. For the primary interventional radiologist, the values were (54 ± 2) μSv and (32 ± 1) μSv in primary drain insertion and drain replacement, respectively. Additionally, as patient dose indicator, the kerma-area product medians were estimated as 34.3 Gy cm<sup>2</sup> and 13.4 Gy cm<sup>2</sup> in primary drain insertions and drain replacements, respectively. Under controlled equipment settings, which simulates clinical procedures with acrylic slabs, TL readings showed strong linear correlations with measurements from an ionization chamber (R<sup>2</sup> = 0.979) and with the equipment dose indicator. The expected relationship between patient and staff doses was confirmed, in both clinical procedures and controlled settings. Finally, based on the results, recommendations were made regarding radiation protection at this facility, aiming to reduce both patient and staff exposure during this procedure.</div></div>","PeriodicalId":21055,"journal":{"name":"Radiation Measurements","volume":"192 ","pages":"Article 107621"},"PeriodicalIF":2.2,"publicationDate":"2026-01-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146038977","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Study on a rapid measurement method for the deposition velocity of 220Rn progeny based on an imaging plate 基于成像板的220Rn子代沉积速度快速测量方法研究
IF 2.2 3区 物理与天体物理 Q2 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2026-01-15 DOI: 10.1016/j.radmeas.2026.107620
Yufan Liu, Kexin Wang, Wenjie Xu, Jialu Feng, Tao Ao, Lidan Lv, Qingzhi Zhou, Zhengzhong He
The study of the deposition behavior of 220Rn progeny is crucial for the assessment of public and occupational radiation doses and for controlling progeny concentration in a thoron chamber. To address the difficulty of maintaining stable environmental conditions over long durations when studying deposition velocity variations, a rapid and accurate method for the deposition velocity measurement of 220Rn progeny is proposed in this study, based on a BAS-TR imaging plate (IP), which has advantages of high sensitivity, large detection area and portability. In this research, measurement procedures were optimized based on the analysis of uncertainty, whereby the total time for a single measurement can be limited within 8 h. A dedicated Python program was developed for the automatic processing of IP count data, and key parameters such as IP detection efficiency, IP scanner sensitivity, and IP fading correction were determined through experiments. Comparative experiment was conducted between IP and a calibrated alpha spectroscopy, with results showing good agreement between two method. This method was preliminarily applied on 220Rn progeny deposition velocity measurement using collection plates of different sizes. Compared to traditional techniques, multi-sample, large-area measurements of deposition velocity can be completed within 8 hours using the proposed method, thereby providing an new efficient approach for the study of the deposition of 220Rn progeny and other radionuclides.
研究220Rn子体的沉积行为对于评估公众和职业辐射剂量以及控制钍室子体浓度至关重要。针对研究沉积速度变化时难以长时间保持稳定环境条件的问题,本研究提出了一种基于BAS-TR成像板(IP)的220Rn子代沉积速度快速准确测量方法,该方法具有灵敏度高、检测面积大、便携性好等优点。本研究在不确定度分析的基础上对测量程序进行了优化,将单次测量的总时间控制在8 h以内。开发了专用Python程序对IP计数数据进行自动处理,并通过实验确定了IP检测效率、IP扫描器灵敏度、IP衰落校正等关键参数。将IP法与标定后的α光谱法进行了对比实验,结果表明两者吻合较好。该方法初步应用于不同尺寸采集板的220Rn子代沉积速度测量。与传统方法相比,该方法可在8小时内完成多样品、大面积的沉积速度测量,为研究220Rn子代及其他放射性核素的沉积提供了一种新的高效方法。
{"title":"Study on a rapid measurement method for the deposition velocity of 220Rn progeny based on an imaging plate","authors":"Yufan Liu,&nbsp;Kexin Wang,&nbsp;Wenjie Xu,&nbsp;Jialu Feng,&nbsp;Tao Ao,&nbsp;Lidan Lv,&nbsp;Qingzhi Zhou,&nbsp;Zhengzhong He","doi":"10.1016/j.radmeas.2026.107620","DOIUrl":"10.1016/j.radmeas.2026.107620","url":null,"abstract":"<div><div>The study of the deposition behavior of <span><math><mrow><msup><mrow></mrow><mrow><mn>220</mn></mrow></msup><mi>Rn</mi></mrow></math></span> progeny is crucial for the assessment of public and occupational radiation doses and for controlling progeny concentration in a thoron chamber. To address the difficulty of maintaining stable environmental conditions over long durations when studying deposition velocity variations, a rapid and accurate method for the deposition velocity measurement of <span><math><mrow><msup><mrow></mrow><mrow><mn>220</mn></mrow></msup><mi>Rn</mi></mrow></math></span> progeny is proposed in this study, based on a BAS-TR imaging plate (IP), which has advantages of high sensitivity, large detection area and portability. In this research, measurement procedures were optimized based on the analysis of uncertainty, whereby the total time for a single measurement can be limited within 8 h. A dedicated Python program was developed for the automatic processing of IP count data, and key parameters such as IP detection efficiency, IP scanner sensitivity, and IP fading correction were determined through experiments. Comparative experiment was conducted between IP and a calibrated alpha spectroscopy, with results showing good agreement between two method. This method was preliminarily applied on <span><math><mrow><msup><mrow></mrow><mrow><mn>220</mn></mrow></msup><mi>Rn</mi></mrow></math></span> progeny deposition velocity measurement using collection plates of different sizes. Compared to traditional techniques, multi-sample, large-area measurements of deposition velocity can be completed within 8 hours using the proposed method, thereby providing an new efficient approach for the study of the deposition of <span><math><mrow><msup><mrow></mrow><mrow><mn>220</mn></mrow></msup><mi>Rn</mi></mrow></math></span> progeny and other radionuclides.</div></div>","PeriodicalId":21055,"journal":{"name":"Radiation Measurements","volume":"192 ","pages":"Article 107620"},"PeriodicalIF":2.2,"publicationDate":"2026-01-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145981056","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Commissioning of radiophotoluminescent dosimetry system for radiotherapy dosimetry audits - feasibility and pilot study results in Bulgaria 用于放射治疗剂量测定审计的放射光致发光剂量测定系统的调试——保加利亚的可行性和试点研究结果
IF 2.2 3区 物理与天体物理 Q2 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2026-01-14 DOI: 10.1016/j.radmeas.2026.107619
Gueorgui Gueorguiev , Tsvetelina Todorova , Bozhidar Vladimirov , Filip Simeonov , Katia Sergieva
This study depicts how a nationwide remote dosimetry audit (RDA) system in radiotherapy, utilizing radiophotoluminescent dosemeters, was commissioned and validated in Bulgaria. The work outlines the commissioning process of the dosimetry system, presents the organization of the RDA feasibility study, and describes how a preliminary clinical audit was carried out in Bulgaria, with determination of absorbed dose correction factors as an integral part of the commissioning process. After successful commissioning of the RDA system, the dosimetric accuracy of the absorbed dose to water at the reference point under reference conditions was evaluated during both the feasibility study and the clinical audit. Across all investigated photon beam energies (6 MV, 10 MV, 15 MV, 6 MV FFF, and 10 MV FFF), the differences between the stated doses and the RPLD-measured doses ranged from −1.5 % to +4.0 % during the feasibility phase and from −1.5 % to +2.0 % during the first clinical audits, with all deviations remaining well within the ±5 % acceptance tolerance. The findings of the feasibility study and the preliminary clinical results indicate that the proposed RDA methodology is viable for implementation in Bulgarian radiotherapy centers.
本研究描述了如何在保加利亚使用放射光致发光剂量计进行全国范围的放射治疗远程剂量审计(RDA)系统的委托和验证。该工作概述了剂量测定系统的调试过程,介绍了RDA可行性研究的组织,并描述了如何在保加利亚进行初步临床审计,并将确定吸收剂量校正系数作为调试过程的一个组成部分。在RDA系统成功调试后,在可行性研究和临床审核期间,评估了参考条件下参考点对水的吸收剂量的剂量学准确性。在所有研究的光子束能量(6 MV、10 MV、15 MV、6 MV FFF和10 MV FFF)中,所述剂量与rpld测量剂量之间的差异在可行性阶段为- 1.5%至+ 4.0%,在第一次临床审计期间为- 1.5%至+ 2.0%,所有偏差都保持在±5%的可接受公差范围内。可行性研究的结果和初步临床结果表明,拟议的RDA方法在保加利亚放射治疗中心实施是可行的。
{"title":"Commissioning of radiophotoluminescent dosimetry system for radiotherapy dosimetry audits - feasibility and pilot study results in Bulgaria","authors":"Gueorgui Gueorguiev ,&nbsp;Tsvetelina Todorova ,&nbsp;Bozhidar Vladimirov ,&nbsp;Filip Simeonov ,&nbsp;Katia Sergieva","doi":"10.1016/j.radmeas.2026.107619","DOIUrl":"10.1016/j.radmeas.2026.107619","url":null,"abstract":"<div><div>This study depicts how a nationwide remote dosimetry audit (RDA) system in radiotherapy, utilizing radiophotoluminescent dosemeters, was commissioned and validated in Bulgaria. The work outlines the commissioning process of the dosimetry system, presents the organization of the RDA feasibility study, and describes how a preliminary clinical audit was carried out in Bulgaria, with determination of absorbed dose correction factors as an integral part of the commissioning process. After successful commissioning of the RDA system, the dosimetric accuracy of the absorbed dose to water at the reference point under reference conditions was evaluated during both the feasibility study and the clinical audit. Across all investigated photon beam energies (6 MV, 10 MV, 15 MV, 6 MV FFF, and 10 MV FFF), the differences between the stated doses and the RPLD-measured doses ranged from −1.5 % to +4.0 % during the feasibility phase and from −1.5 % to +2.0 % during the first clinical audits, with all deviations remaining well within the ±5 % acceptance tolerance. The findings of the feasibility study and the preliminary clinical results indicate that the proposed RDA methodology is viable for implementation in Bulgarian radiotherapy centers.</div></div>","PeriodicalId":21055,"journal":{"name":"Radiation Measurements","volume":"192 ","pages":"Article 107619"},"PeriodicalIF":2.2,"publicationDate":"2026-01-14","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145980461","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Uniformity of heating across sample holders during luminescence measurements 发光测量时样品夹加热均匀性
IF 2.2 3区 物理与天体物理 Q2 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2026-01-13 DOI: 10.1016/j.radmeas.2026.107617
J.A. Winzar, G.A.T. Duller, H.M. Roberts
For luminescence research, samples are often heated prior to and/or during measurement to measure the thermoluminescence (TL) signal or to remove charge from shallow traps. The reproducibility and repeatability of luminescence measurements will be influenced by how consistently and uniformly the samples are heated, both within a single aliquot and between different readers or sample positions. While the effects of temperature lag during heating have been intensively studied, the spatial uniformity of temperature across samples has received less attention.
This study presents spatially-resolved measurements of the temperature of the heating strip, a steel cup and an aluminium single grain disc in a Risø TL/OSL DA20 reader. Temperature is calculated using black body emissions from the three materials, detected with an Electron Multiplying Charge Coupled Device (EMCCD). The results show that temperature is not spatially uniform across any of the three materials, although the degree of variation differs between them. The largest temperature variation is observed across the steel cup (∼18 % at a temperature of 500 °C), followed by the heating strip (∼8 % at a temperature of 500 °C), and then the single grain disc (∼2 % at a temperature of 250 °C). The steel cup also has greater anisotropy in temperature compared to the single grain disc. This study suggests that spatial variation in temperature can be minimised by using sample holders made of materials with high thermal conductivity (e.g. aluminium or silver), and that the impact of thermal variation can be reduced by restricting samples to the central portion of a sample holder (e.g. the central 2 mm of a sample holder (i.e. ‘small aliquots’)).
对于发光研究,通常在测量之前和/或测量期间对样品进行加热,以测量热释光(TL)信号或从浅阱中去除电荷。发光测量的再现性和可重复性将受到样品加热的一致性和均匀性的影响,无论是在单个等温线内还是在不同的读取器或样品位置之间。虽然加热过程中温度滞后的影响已经得到了深入的研究,但样品间温度的空间均匀性却受到较少的关注。本研究提出了在Risø TL/OSL DA20读取器中加热带,钢杯和铝单晶粒盘的空间分辨率测量。用电子倍增电荷耦合器件(EMCCD)检测三种材料的黑体辐射来计算温度。结果表明,三种材料的温度在空间上并不均匀,尽管它们之间的变化程度不同。温度变化最大的是钢杯(在500℃温度下为~ 18%),其次是加热带(在500℃温度下为~ 8%),然后是单晶圆盘(在250℃温度下为~ 2%)。与单晶粒圆盘相比,钢杯在温度上也具有更大的各向异性。该研究表明,可以通过使用高导热材料(例如铝或银)制成的样品架来最小化温度的空间变化,并且可以通过将样品限制在样品架的中心部分(例如样品架的中心2毫米(即“小等分”))来减少热变化的影响。
{"title":"Uniformity of heating across sample holders during luminescence measurements","authors":"J.A. Winzar,&nbsp;G.A.T. Duller,&nbsp;H.M. Roberts","doi":"10.1016/j.radmeas.2026.107617","DOIUrl":"10.1016/j.radmeas.2026.107617","url":null,"abstract":"<div><div>For luminescence research, samples are often heated prior to and/or during measurement to measure the thermoluminescence (TL) signal or to remove charge from shallow traps. The reproducibility and repeatability of luminescence measurements will be influenced by how consistently and uniformly the samples are heated, both within a single aliquot and between different readers or sample positions. While the effects of temperature lag during heating have been intensively studied, the spatial uniformity of temperature across samples has received less attention.</div><div>This study presents spatially-resolved measurements of the temperature of the heating strip, a steel cup and an aluminium single grain disc in a Risø TL/OSL DA20 reader. Temperature is calculated using black body emissions from the three materials, detected with an Electron Multiplying Charge Coupled Device (EMCCD). The results show that temperature is not spatially uniform across any of the three materials, although the degree of variation differs between them. The largest temperature variation is observed across the steel cup (∼18 % at a temperature of 500 °C), followed by the heating strip (∼8 % at a temperature of 500 °C), and then the single grain disc (∼2 % at a temperature of 250 °C). The steel cup also has greater anisotropy in temperature compared to the single grain disc. This study suggests that spatial variation in temperature can be minimised by using sample holders made of materials with high thermal conductivity (e.g. aluminium or silver), and that the impact of thermal variation can be reduced by restricting samples to the central portion of a sample holder (e.g. the central 2 mm of a sample holder (i.e. ‘small aliquots’)).</div></div>","PeriodicalId":21055,"journal":{"name":"Radiation Measurements","volume":"192 ","pages":"Article 107617"},"PeriodicalIF":2.2,"publicationDate":"2026-01-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145981057","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
A new method for the determination of 210Po in environmental samples using plastic scintillation resins 建立了用塑料闪烁树脂测定环境样品中210Po的新方法
IF 2.2 3区 物理与天体物理 Q2 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2026-01-12 DOI: 10.1016/j.radmeas.2026.107618
Jordi Rotger , Joana Tent , Hector Bagán , Anna Rigol , Àlex Tarancón
We have developed a new method using a selective plastic scintillation resin (PSresin) based on Aliquat-336 for analysing 210Po in water samples. The PSresin effectively isolates 210Po while removing main interferences such as 210Pb and 210Bi by loading the sample in a HCl 1 mol L−1 medium and rinsing with HCl 1 mol L−1 and 6.25 mol L−1, consecutively. We optimized the rinse volumes and conducted a search for suitable chemical analogues of polonium to be used as tracers throughout the procedure. Zinc and cadmium were identified as the most suitable elements for preconcentration and separation of 210Po on the PSresin. We compared our PSresin method with reference methods (UNE-EN ISO 13161 and IAEA/AQ/12) based on alpha spectrometry by analysing drinking water samples. The results showed that the PSresin method is faster and provides accurate results, although the alpha spectrometry methods achieve lower detection limits.
我们开发了一种基于Aliquat-336的选择性塑料闪烁树脂(PSresin)分析水样中210Po的新方法。通过将样品装于HCl 1 mol L−1介质中,连续用HCl 1 mol L−1和6.25 mol L−1洗涤,PSresin可以有效地分离210Po,同时去除210Pb和210Bi等主要干扰。我们优化了漂洗体积,并在整个过程中寻找合适的化学类似物作为示踪剂。锌和镉是最适合在PSresin上富集分离210Po的元素。通过对饮用水样品的α光谱分析,将PSresin方法与参考方法(UNE-EN ISO 13161和IAEA/AQ/12)进行了比较。结果表明,虽然α光谱法的检出限较低,但PSresin法速度更快,结果准确。
{"title":"A new method for the determination of 210Po in environmental samples using plastic scintillation resins","authors":"Jordi Rotger ,&nbsp;Joana Tent ,&nbsp;Hector Bagán ,&nbsp;Anna Rigol ,&nbsp;Àlex Tarancón","doi":"10.1016/j.radmeas.2026.107618","DOIUrl":"10.1016/j.radmeas.2026.107618","url":null,"abstract":"<div><div>We have developed a new method using a selective plastic scintillation resin (PSresin) based on Aliquat-336 for analysing <sup>210</sup>Po in water samples. The PSresin effectively isolates <sup>210</sup>Po while removing main interferences such as <sup>210</sup>Pb and <sup>210</sup>Bi by loading the sample in a HCl 1 mol L<sup>−1</sup> medium and rinsing with HCl 1 mol L<sup>−1</sup> and 6.25 mol L<sup>−1</sup>, consecutively. We optimized the rinse volumes and conducted a search for suitable chemical analogues of polonium to be used as tracers throughout the procedure. Zinc and cadmium were identified as the most suitable elements for preconcentration and separation of <sup>210</sup>Po on the PSresin. We compared our PSresin method with reference methods (UNE-EN ISO 13161 and IAEA/AQ/12) based on alpha spectrometry by analysing drinking water samples. The results showed that the PSresin method is faster and provides accurate results, although the alpha spectrometry methods achieve lower detection limits.</div></div>","PeriodicalId":21055,"journal":{"name":"Radiation Measurements","volume":"192 ","pages":"Article 107618"},"PeriodicalIF":2.2,"publicationDate":"2026-01-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145981058","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
期刊
Radiation Measurements
全部 Acc. Chem. Res. ACS Applied Bio Materials ACS Appl. Electron. Mater. ACS Appl. Energy Mater. ACS Appl. Mater. Interfaces ACS Appl. Nano Mater. ACS Appl. Polym. Mater. ACS BIOMATER-SCI ENG ACS Catal. ACS Cent. Sci. ACS Chem. Biol. ACS Chemical Health & Safety ACS Chem. Neurosci. ACS Comb. Sci. ACS Earth Space Chem. ACS Energy Lett. ACS Infect. Dis. ACS Macro Lett. ACS Mater. Lett. ACS Med. Chem. Lett. ACS Nano ACS Omega ACS Photonics ACS Sens. ACS Sustainable Chem. Eng. ACS Synth. Biol. Anal. Chem. BIOCHEMISTRY-US Bioconjugate Chem. BIOMACROMOLECULES Chem. Res. Toxicol. Chem. Rev. Chem. Mater. CRYST GROWTH DES ENERG FUEL Environ. Sci. Technol. Environ. Sci. Technol. Lett. Eur. J. Inorg. Chem. IND ENG CHEM RES Inorg. Chem. J. Agric. Food. Chem. J. Chem. Eng. Data J. Chem. Educ. J. Chem. Inf. Model. J. Chem. Theory Comput. J. Med. Chem. J. Nat. Prod. J PROTEOME RES J. Am. Chem. Soc. LANGMUIR MACROMOLECULES Mol. Pharmaceutics Nano Lett. Org. Lett. ORG PROCESS RES DEV ORGANOMETALLICS J. Org. Chem. J. Phys. Chem. J. Phys. Chem. A J. Phys. Chem. B J. Phys. Chem. C J. Phys. Chem. Lett. Analyst Anal. Methods Biomater. Sci. Catal. Sci. Technol. Chem. Commun. Chem. Soc. Rev. CHEM EDUC RES PRACT CRYSTENGCOMM Dalton Trans. Energy Environ. Sci. ENVIRON SCI-NANO ENVIRON SCI-PROC IMP ENVIRON SCI-WAT RES Faraday Discuss. Food Funct. Green Chem. Inorg. Chem. Front. Integr. Biol. J. Anal. At. Spectrom. J. Mater. Chem. A J. Mater. Chem. B J. Mater. Chem. C Lab Chip Mater. Chem. Front. Mater. Horiz. MEDCHEMCOMM Metallomics Mol. Biosyst. Mol. Syst. Des. Eng. Nanoscale Nanoscale Horiz. Nat. Prod. Rep. New J. Chem. Org. Biomol. Chem. Org. Chem. Front. PHOTOCH PHOTOBIO SCI PCCP Polym. Chem.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
0
微信
客服QQ
Book学术公众号 扫码关注我们
反馈
×
意见反馈
请填写您的意见或建议
请填写您的手机或邮箱
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
现在去查看 取消
×
提示
确定
Book学术官方微信
Book学术文献互助
Book学术文献互助群
群 号:604180095
Book学术
文献互助 智能选刊 最新文献 互助须知 联系我们:info@booksci.cn
Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。
Copyright © 2023 Book学术 All rights reserved.
ghs 京公网安备 11010802042870号 京ICP备2023020795号-1