Pub Date : 2024-06-26DOI: 10.1016/j.eehl.2024.05.008
Adewale Adewuyi , Qilin Li
The detection of per- and polyfluoroalkyl substances (PFAS) in water presents a significant challenge for developing countries, requiring urgent attention. This review focuses on understanding the emergence of PFAS in drinking water, health concerns, and removal strategies for PFAS in water systems in developing countries. This review indicates the need for more studies to be conducted in many developing nations due to limited information on the environmental status and fate of PFAS. The health consequences of PFAS in water are enormous and cannot be overemphasized. Efforts are ongoing to legislate a national standard for PFAS in drinking water. Currently, there are few known mitigation efforts from African countries, in contrast to several developing nations in Asia. Therefore, there is an urgent need to develop economically viable techniques that could be integrated into large-scale operations to remove PFAS from water systems in the region. However, despite the success achieved with removing long-chain PFAS from water, more studies are required on strategies for eliminating short-chain moieties in water.
{"title":"Emergency of per- and polyfluoroalkyl substances in drinking water: Status, regulation, and mitigation strategies in developing countries","authors":"Adewale Adewuyi , Qilin Li","doi":"10.1016/j.eehl.2024.05.008","DOIUrl":"10.1016/j.eehl.2024.05.008","url":null,"abstract":"<div><p>The detection of per- and polyfluoroalkyl substances (PFAS) in water presents a significant challenge for developing countries, requiring urgent attention. This review focuses on understanding the emergence of PFAS in drinking water, health concerns, and removal strategies for PFAS in water systems in developing countries. This review indicates the need for more studies to be conducted in many developing nations due to limited information on the environmental status and fate of PFAS. The health consequences of PFAS in water are enormous and cannot be overemphasized. Efforts are ongoing to legislate a national standard for PFAS in drinking water. Currently, there are few known mitigation efforts from African countries, in contrast to several developing nations in Asia. Therefore, there is an urgent need to develop economically viable techniques that could be integrated into large-scale operations to remove PFAS from water systems in the region. However, despite the success achieved with removing long-chain PFAS from water, more studies are required on strategies for eliminating short-chain moieties in water.</p></div>","PeriodicalId":29813,"journal":{"name":"Eco-Environment & Health","volume":"3 3","pages":"Pages 355-368"},"PeriodicalIF":0.0,"publicationDate":"2024-06-26","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2772985024000498/pdfft?md5=c072a0dbaa7f59500f4c8b4edbd05a29&pid=1-s2.0-S2772985024000498-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142089714","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-06-26DOI: 10.1016/j.eehl.2024.05.007
Ye Li , Xiaoyu Sha , Yuan Wang , Yanfang Zhao , Junjie Zhang , Ping Wang , Xiangfeng Chen , Baoshan Xing , Lei Wang
Plastic pollution is widely present in terrestrial and aquatic ecosystems, and microplastics (MPs) can be detected in organisms. In situ detection methods for MPs in organisms have attracted widespread attention. Traditional imaging characterization methods of MPs, including stereo microscopes and fluorescence microscopy, are typically used to image artificially added microsphere standards under laboratory conditions. However, they cannot specifically identify MPs in biological samples. Thus, there is a need for a detection technique that can provide spatial distribution information of MPs in biological samples as well as measure their quality and quantity. In this perspective, to obtain high-resolution images with chemical composition analysis, we compared ion sources for ionizing plastic macromolecules and mass analyzers for analyzing macromolecules. Matrix-assisted laser desorption/ionization (MALDI) is suitable for imaging characterization, while time-of-flight (TOF) and Orbitrap mass spectrometry are suitable for polymer mass spectrometry analysis. Furthermore, we propose a technique that combines MALDI with TOF or Orbitrap, which holds promise for the in situ imaging of MPs in biological samples.
{"title":"In situ imaging of microplastics in living organisms based on mass spectrometry technology","authors":"Ye Li , Xiaoyu Sha , Yuan Wang , Yanfang Zhao , Junjie Zhang , Ping Wang , Xiangfeng Chen , Baoshan Xing , Lei Wang","doi":"10.1016/j.eehl.2024.05.007","DOIUrl":"10.1016/j.eehl.2024.05.007","url":null,"abstract":"<div><div>Plastic pollution is widely present in terrestrial and aquatic ecosystems, and microplastics (MPs) can be detected in organisms. <em>In situ</em> detection methods for MPs in organisms have attracted widespread attention. Traditional imaging characterization methods of MPs, including stereo microscopes and fluorescence microscopy, are typically used to image artificially added microsphere standards under laboratory conditions. However, they cannot specifically identify MPs in biological samples. Thus, there is a need for a detection technique that can provide spatial distribution information of MPs in biological samples as well as measure their quality and quantity. In this perspective, to obtain high-resolution images with chemical composition analysis, we compared ion sources for ionizing plastic macromolecules and mass analyzers for analyzing macromolecules. Matrix-assisted laser desorption/ionization (MALDI) is suitable for imaging characterization, while time-of-flight (TOF) and Orbitrap mass spectrometry are suitable for polymer mass spectrometry analysis. Furthermore, we propose a technique that combines MALDI with TOF or Orbitrap, which holds promise for the <em>in situ</em> imaging of MPs in biological samples.</div></div>","PeriodicalId":29813,"journal":{"name":"Eco-Environment & Health","volume":"3 4","pages":"Pages 412-417"},"PeriodicalIF":0.0,"publicationDate":"2024-06-26","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142535305","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-06-11DOI: 10.1016/j.eehl.2024.05.005
Chao Guo , Shiwen Hu , Pengfei Cheng, Kuan Cheng, Yang Yang, Guojun Chen, Qi Wang, Ying Wang, Tongxu Liu
Perfluoroalkyl acids (PFAAs) are emerging organic pollutants that have attracted significant attention in the fields of environmental chemistry and toxicology. Although PFAAs are pervasive in soils and sediments, there is a paucity of research regarding their environmental forms and driving mechanisms. This review provides an overview of the classification and biotoxicity of per- and polyfluoroalkyl substances (PFAS), organic pollutant forms, PFAS extraction and analytical methods, the prediction of PFAS distribution in soils, and current PFAS remediation strategies. Four predominant PFAA forms have been proposed in soils: (i) aqueous-extracted PFAAs, (ii) organic-solvent extracted PFAAs, (iii) embedded or sequestered PFAAs, and (iv) covalently bound PFAAs. Furthermore, it suggests suitable extraction methods and predictive models for different PFAA forms, which are instrumental in the research on PFAA speciation and prediction in soils. Simultaneously, it was proposed that elemental cycling and microbial activity may affect the speciation of PFAS. Additionally, the categorization of PFAA forms facilitated the analysis of pollution remediation. Understanding the interplay between PFAA speciation, element cycling, and bacterial activity during soil remediation is essential for understanding remediation mechanisms and assessing the long-term stability of remediation methods. Future studies should expand the investigation of varying PFAA forms in different media, consider the potential binding forms of PFAAs to minerals, organic matter, and microbes, and evaluate the possible mechanisms of PFAA speciation variation.
{"title":"Speciation and biogeochemical behavior of perfluoroalkyl acids in soils and their environmental implications: A review","authors":"Chao Guo , Shiwen Hu , Pengfei Cheng, Kuan Cheng, Yang Yang, Guojun Chen, Qi Wang, Ying Wang, Tongxu Liu","doi":"10.1016/j.eehl.2024.05.005","DOIUrl":"10.1016/j.eehl.2024.05.005","url":null,"abstract":"<div><div>Perfluoroalkyl acids (PFAAs) are emerging organic pollutants that have attracted significant attention in the fields of environmental chemistry and toxicology. Although PFAAs are pervasive in soils and sediments, there is a paucity of research regarding their environmental forms and driving mechanisms. This review provides an overview of the classification and biotoxicity of per- and polyfluoroalkyl substances (PFAS), organic pollutant forms, PFAS extraction and analytical methods, the prediction of PFAS distribution in soils, and current PFAS remediation strategies. Four predominant PFAA forms have been proposed in soils: (i) aqueous-extracted PFAAs, (ii) organic-solvent extracted PFAAs, (iii) embedded or sequestered PFAAs, and (iv) covalently bound PFAAs. Furthermore, it suggests suitable extraction methods and predictive models for different PFAA forms, which are instrumental in the research on PFAA speciation and prediction in soils. Simultaneously, it was proposed that elemental cycling and microbial activity may affect the speciation of PFAS. Additionally, the categorization of PFAA forms facilitated the analysis of pollution remediation. Understanding the interplay between PFAA speciation, element cycling, and bacterial activity during soil remediation is essential for understanding remediation mechanisms and assessing the long-term stability of remediation methods. Future studies should expand the investigation of varying PFAA forms in different media, consider the potential binding forms of PFAAs to minerals, organic matter, and microbes, and evaluate the possible mechanisms of PFAA speciation variation.</div></div>","PeriodicalId":29813,"journal":{"name":"Eco-Environment & Health","volume":"3 4","pages":"Pages 505-515"},"PeriodicalIF":0.0,"publicationDate":"2024-06-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141409451","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-06-11DOI: 10.1016/j.eehl.2024.05.006
To investigate the association of long-term exposure to air pollution with incident arrhythmia from various causes, this prospective cohort study included 442,386 participants from the UK Biobank cohort. Residential annual average exposures at baseline were evaluated, including fine particles (PM2.5), coarse particles (PM2.5–10), nitrogen dioxide (NO2), and nitrogen oxides (NOx). We further constructed a composite air pollution score (APS) to evaluate the concomitant exposure to these four pollutants. The associations of air pollutants with various arrhythmia subtypes were assessed utilizing the Cox proportional hazards model, and the hazard ratios (HRs) for incident arrhythmias were estimated. A total of 41,021 patients with incident arrhythmia were recorded. The HRs of overall arrhythmia associated with a 10 μg/m3 increment in PM2.5, PM2.5–10, NO2, and NOx were 1.26, 0.95, 1.03, and 1.02, respectively. The HR was 1.08 in the highest quintile of the APS compared to the lowest one. For cause-specific arrhythmias, the HRs per unit increment in APS were 1.45, 1.67, 1.51, 1.80, 2.63, and 4.66 for atrial fibrillation, atrioventricular block, ventricular fibrillation/tachycardia, intraventricular block, supraventricular tachycardia, and ventricular premature beats, respectively. Females, older individuals, overweight or obese individuals, and those with low education attainment, low income, or cardiometabolic morbidities had higher HRs associated with pollutants. Long-term exposure to air pollution is linked to increased incidence risks of atrial and ventricular arrhythmias. More focus should be shifted to the impact of air pollution on other arrhythmias besides atrial fibrillation.
{"title":"Long-term exposure to air pollution and incidence risk of various arrhythmias: A prospective cohort study","authors":"","doi":"10.1016/j.eehl.2024.05.006","DOIUrl":"10.1016/j.eehl.2024.05.006","url":null,"abstract":"<div><div>To investigate the association of long-term exposure to air pollution with incident arrhythmia from various causes, this prospective cohort study included 442,386 participants from the UK Biobank cohort. Residential annual average exposures at baseline were evaluated, including fine particles (PM<sub>2.5</sub>), coarse particles (PM<sub>2.5–10</sub>), nitrogen dioxide (NO<sub>2</sub>), and nitrogen oxides (NO<sub>x</sub>). We further constructed a composite air pollution score (APS) to evaluate the concomitant exposure to these four pollutants. The associations of air pollutants with various arrhythmia subtypes were assessed utilizing the Cox proportional hazards model, and the hazard ratios (HRs) for incident arrhythmias were estimated. A total of 41,021 patients with incident arrhythmia were recorded. The HRs of overall arrhythmia associated with a 10 μg/m<sup>3</sup> increment in PM<sub>2.5</sub>, PM<sub>2.5–10</sub>, NO<sub>2</sub>, and NO<sub>x</sub> were 1.26, 0.95, 1.03, and 1.02, respectively. The HR was 1.08 in the highest quintile of the APS compared to the lowest one. For cause-specific arrhythmias, the HRs per unit increment in APS were 1.45, 1.67, 1.51, 1.80, 2.63, and 4.66 for atrial fibrillation, atrioventricular block, ventricular fibrillation/tachycardia, intraventricular block, supraventricular tachycardia, and ventricular premature beats, respectively. Females, older individuals, overweight or obese individuals, and those with low education attainment, low income, or cardiometabolic morbidities had higher HRs associated with pollutants. Long-term exposure to air pollution is linked to increased incidence risks of atrial and ventricular arrhythmias. More focus should be shifted to the impact of air pollution on other arrhythmias besides atrial fibrillation.</div></div>","PeriodicalId":29813,"journal":{"name":"Eco-Environment & Health","volume":"3 4","pages":"Pages 445-451"},"PeriodicalIF":0.0,"publicationDate":"2024-06-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141415537","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-05-29DOI: 10.1016/j.eehl.2024.05.004
Sarah E. Morgan , Lisa A. DeLouise
This project reports on the use of a novel nanomembrane filtering technology to isolate and analyze the bioactivity of microplastic (MP)-containing debris from Lake Ontario water samples. Environmental MPs are a complex mixture of polymers and sorbed chemicals that are persistent and can exhibit a wide range of toxic effects. Since human exposure to MPs is unavoidable, it is necessary to characterize their bioactivity to assess potential health risks. This work seeks to quantify MP presence in the nearshore waters of Lake Ontario and begin to characterize the bioactivity of the filtrate containing MPs. We utilized silicon nitride (SiN) nanomembrane technology to isolate debris sized between 8 and 20 μm from lake water samples collected at various times and locations. MPs were identified with Nile red staining. Cell-based assays were conducted directly on the filtered debris to test for cell viability, aryl hydrocarbon receptor (AhR) activity, and interleukin 6 (IL-6) levels as a measure of proinflammatory response. All samples contained MPs. None of the isolated debris impacted cell viability. However, AhR activity and IL-6 levels varied over time. Additionally, no associations were observed between the amount of plastic and bioactivity. Observed differences in activity are likely due to variations in the physiochemical properties of debris between samples. Our results highlight the need for increased sampling to fully characterize the bioactivity of MPs in human cells and to elucidate the role that sample physiochemical and spatiotemporal properties play in this activity.
{"title":"Assessing bioactivity of environmental water samples filtered using nanomembrane technology and mammalian cell lines","authors":"Sarah E. Morgan , Lisa A. DeLouise","doi":"10.1016/j.eehl.2024.05.004","DOIUrl":"10.1016/j.eehl.2024.05.004","url":null,"abstract":"<div><p>This project reports on the use of a novel nanomembrane filtering technology to isolate and analyze the bioactivity of microplastic (MP)-containing debris from Lake Ontario water samples. Environmental MPs are a complex mixture of polymers and sorbed chemicals that are persistent and can exhibit a wide range of toxic effects. Since human exposure to MPs is unavoidable, it is necessary to characterize their bioactivity to assess potential health risks. This work seeks to quantify MP presence in the nearshore waters of Lake Ontario and begin to characterize the bioactivity of the filtrate containing MPs. We utilized silicon nitride (SiN) nanomembrane technology to isolate debris sized between 8 and 20 μm from lake water samples collected at various times and locations. MPs were identified with Nile red staining. Cell-based assays were conducted directly on the filtered debris to test for cell viability, aryl hydrocarbon receptor (AhR) activity, and interleukin 6 (IL-6) levels as a measure of proinflammatory response. All samples contained MPs. None of the isolated debris impacted cell viability. However, AhR activity and IL-6 levels varied over time. Additionally, no associations were observed between the amount of plastic and bioactivity. Observed differences in activity are likely due to variations in the physiochemical properties of debris between samples. Our results highlight the need for increased sampling to fully characterize the bioactivity of MPs in human cells and to elucidate the role that sample physiochemical and spatiotemporal properties play in this activity.</p></div>","PeriodicalId":29813,"journal":{"name":"Eco-Environment & Health","volume":"3 3","pages":"Pages 347-354"},"PeriodicalIF":0.0,"publicationDate":"2024-05-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2772985024000450/pdfft?md5=29bd23b5241cc8c21143e08879295925&pid=1-s2.0-S2772985024000450-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142083329","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-05-22DOI: 10.1016/j.eehl.2024.05.003
Jia Jia , Qian Liu , E. Zhao , Xin Li , Xiong Xiong , Chenxi Wu
Microplastics (MPs) in aquatic environments easily support biofilm development, which can interact with other environmental pollutants and act as harbors for microorganisms. Recently, numerous studies have investigated the fate and behavior of MP biofilms in aquatic environments, highlighting their roles in the spread of pathogens and antibiotic resistance genes (ARGs) to aquatic organisms and new habitats. The prevalence and effects of MP biofilms in aquatic environments have been extensively investigated in recent decades, and their behaviors in aquatic environments need to be synthesized systematically with updated information. This review aims to reveal the development of MP biofilm and its interactions with antibiotics, ARGs, and pathogens in aquatic environments. Recent research has shown that the adsorption capabilities of MPs to antibiotics are enhanced after the biofilm formation, and the adsorption of biofilms to antibiotics is biased towards chemisorption. ARGs and microorganisms, especially pathogens, are selectively enriched in biofilms and significantly different from those in surrounding waters. MP biofilm promotes the propagation of ARGs through horizontal gene transfer (HGT) and vertical gene transfer (VGT) and induces the emergence of antibiotic-resistant pathogens, resulting in increased threats to aquatic ecosystems and human health. Some future research needs and strategies in this review are also proposed to better understand the antibiotic resistance induced by MP biofilms in aquatic environments.
{"title":"Biofilm formation on microplastics and interactions with antibiotics, antibiotic resistance genes and pathogens in aquatic environment","authors":"Jia Jia , Qian Liu , E. Zhao , Xin Li , Xiong Xiong , Chenxi Wu","doi":"10.1016/j.eehl.2024.05.003","DOIUrl":"10.1016/j.eehl.2024.05.003","url":null,"abstract":"<div><div>Microplastics (MPs) in aquatic environments easily support biofilm development, which can interact with other environmental pollutants and act as harbors for microorganisms. Recently, numerous studies have investigated the fate and behavior of MP biofilms in aquatic environments, highlighting their roles in the spread of pathogens and antibiotic resistance genes (ARGs) to aquatic organisms and new habitats. The prevalence and effects of MP biofilms in aquatic environments have been extensively investigated in recent decades, and their behaviors in aquatic environments need to be synthesized systematically with updated information. This review aims to reveal the development of MP biofilm and its interactions with antibiotics, ARGs, and pathogens in aquatic environments. Recent research has shown that the adsorption capabilities of MPs to antibiotics are enhanced after the biofilm formation, and the adsorption of biofilms to antibiotics is biased towards chemisorption. ARGs and microorganisms, especially pathogens, are selectively enriched in biofilms and significantly different from those in surrounding waters. MP biofilm promotes the propagation of ARGs through horizontal gene transfer (HGT) and vertical gene transfer (VGT) and induces the emergence of antibiotic-resistant pathogens, resulting in increased threats to aquatic ecosystems and human health. Some future research needs and strategies in this review are also proposed to better understand the antibiotic resistance induced by MP biofilms in aquatic environments.</div></div>","PeriodicalId":29813,"journal":{"name":"Eco-Environment & Health","volume":"3 4","pages":"Pages 516-528"},"PeriodicalIF":0.0,"publicationDate":"2024-05-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141138273","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-05-22DOI: 10.1016/j.eehl.2024.05.002
Jie Yang , Lianzhen Li , Chen Tu , Ruijie Li , Yongming Luo
Mineral particles, ubiquitous in soils, influence crop plant growth by carrying nutrients and pollutants. While the uptake of dissolved mineral nutrients is well-established, the direct incorporation of irregular mineral particles into plants remains unclear. This study investigated the uptake and transport of kaolin particles, representative of minerals, by wheat and lettuce seedlings using hydroponic and soil cultures. Covalent labeling and advanced microscopy revealed that kaolin enters root steles at lateral root emergence sites, followed by transport to shoots. Fluorescent dyes and lanthanum (La)-labeled kaolin particles demonstrated that wheat surpassed lettuce in kaolin uptake in hydroponics, but both plants showed similar levels of particles in the shoots. Translocation factors (TFs) for kaolin were significantly higher in soil (0.089 for wheat, 0.039 for lettuce) compared to hydroponics (0.001 for wheat, 0.003 for lettuce). These findings provide compelling evidence for the direct uptake and transport of kaolin particles in crop plants. This opens new avenues for research on the interactions between plant and mineral particles, including other colloidal particles, in terrestrial ecosystems.
{"title":"Crop plants transport irregularly shaped mineral particles from root to shoot: Tracking and quantifying","authors":"Jie Yang , Lianzhen Li , Chen Tu , Ruijie Li , Yongming Luo","doi":"10.1016/j.eehl.2024.05.002","DOIUrl":"10.1016/j.eehl.2024.05.002","url":null,"abstract":"<div><div>Mineral particles, ubiquitous in soils, influence crop plant growth by carrying nutrients and pollutants. While the uptake of dissolved mineral nutrients is well-established, the direct incorporation of irregular mineral particles into plants remains unclear. This study investigated the uptake and transport of kaolin particles, representative of minerals, by wheat and lettuce seedlings using hydroponic and soil cultures. Covalent labeling and advanced microscopy revealed that kaolin enters root steles at lateral root emergence sites, followed by transport to shoots. Fluorescent dyes and lanthanum (La)-labeled kaolin particles demonstrated that wheat surpassed lettuce in kaolin uptake in hydroponics, but both plants showed similar levels of particles in the shoots. Translocation factors (TFs) for kaolin were significantly higher in soil (0.089 for wheat, 0.039 for lettuce) compared to hydroponics (0.001 for wheat, 0.003 for lettuce). These findings provide compelling evidence for the direct uptake and transport of kaolin particles in crop plants. This opens new avenues for research on the interactions between plant and mineral particles, including other colloidal particles, in terrestrial ecosystems.</div></div>","PeriodicalId":29813,"journal":{"name":"Eco-Environment & Health","volume":"3 4","pages":"Pages 458-465"},"PeriodicalIF":0.0,"publicationDate":"2024-05-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141141160","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-05-09DOI: 10.1016/j.eehl.2024.05.001
{"title":"Exhalation metabolomics: A new force in revealing the impact of ozone pollution on respiratory health","authors":"","doi":"10.1016/j.eehl.2024.05.001","DOIUrl":"10.1016/j.eehl.2024.05.001","url":null,"abstract":"","PeriodicalId":29813,"journal":{"name":"Eco-Environment & Health","volume":"3 4","pages":"Pages 407-411"},"PeriodicalIF":0.0,"publicationDate":"2024-05-09","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141038350","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-05-09DOI: 10.1016/j.eehl.2024.04.009
Yanwei Liu , Hongwei Liu , Yingying Guo , Dawei Lu , Xingwang Hou , Jianbo Shi , Yongguang Yin , Yong Cai , Guibin Jiang
Atmospheric Hg(0) dry deposition is a vital process that significantly affects the global distribution and cycling of Hg. However, significant knowledge gaps and challenges remain in understanding atmospheric Hg(0) deposition and its subsequent post-deposition processes. Hg isotope fractionation has emerged as the most powerful tool for evaluating the impact of atmospheric Hg(0) deposition and unraveling key processes associated with it. By focusing on Hg isotope fractionation processes, Hg isotopic compositions, and influencing factors, this review presents current knowledge, recent advances, and new insights into atmospheric Hg(0) deposition and post-deposition processes over vegetation, soil, snow, and water surfaces. This review also points out the knowledge gaps pertaining to atmospheric Hg(0) deposition and highlights the need for further investigation into the associated processes, mechanisms, isotope fractionation, and modeling. Further research into Hg isotope fractionation in atmospheric Hg(0) deposition and post-deposition processes will advance source and process tracing, paleoclimate reconstruction, and the modeling of Hg isotope distribution on regional and global scales.
{"title":"Atmospheric Hg(0) dry deposition over environmental surfaces: Insights from mercury isotope fractionation","authors":"Yanwei Liu , Hongwei Liu , Yingying Guo , Dawei Lu , Xingwang Hou , Jianbo Shi , Yongguang Yin , Yong Cai , Guibin Jiang","doi":"10.1016/j.eehl.2024.04.009","DOIUrl":"10.1016/j.eehl.2024.04.009","url":null,"abstract":"<div><div>Atmospheric Hg(0) dry deposition is a vital process that significantly affects the global distribution and cycling of Hg. However, significant knowledge gaps and challenges remain in understanding atmospheric Hg(0) deposition and its subsequent post-deposition processes. Hg isotope fractionation has emerged as the most powerful tool for evaluating the impact of atmospheric Hg(0) deposition and unraveling key processes associated with it. By focusing on Hg isotope fractionation processes, Hg isotopic compositions, and influencing factors, this review presents current knowledge, recent advances, and new insights into atmospheric Hg(0) deposition and post-deposition processes over vegetation, soil, snow, and water surfaces. This review also points out the knowledge gaps pertaining to atmospheric Hg(0) deposition and highlights the need for further investigation into the associated processes, mechanisms, isotope fractionation, and modeling. Further research into Hg isotope fractionation in atmospheric Hg(0) deposition and post-deposition processes will advance source and process tracing, paleoclimate reconstruction, and the modeling of Hg isotope distribution on regional and global scales.</div></div>","PeriodicalId":29813,"journal":{"name":"Eco-Environment & Health","volume":"3 4","pages":"Pages 543-555"},"PeriodicalIF":0.0,"publicationDate":"2024-05-09","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141029850","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-05-08DOI: 10.1016/j.eehl.2024.04.007
Per- and polyfluoroalkyl substances (PFAS) can pass through the placenta and adversely affect fetal development. However, there is a lack of comparison of legacy and emerging PFAS levels among different biosamples in pregnant women and their offspring. This study, based on the Shanghai Maternal–Child Pairs Cohort, analyzed the concentrations of 16 PFAS in the maternal serum, cord serum, and breast milk samples from 1,076 mother-child pairs. The placental and breastfeeding transfer efficiencies of PFAS were determined in maternal-cord and maternal-milk pairs, respectively. The binding affinities of PFAS to five transporters were simulated using molecular docking. The results suggested that PFAS were frequently detected in different biosamples. The median concentration of perfluorooctane sulfonate (PFOS) was the highest at 8.85 ng/mL, followed by perfluorooctanoic acid (PFOA) at 7.13 ng/mL and 6:2 chlorinated polyfluorinated ether sulfonate at 5.59 ng/mL in maternal serum. The median concentrations of PFOA were highest in cord serum (4.23 ng/mL) and breast milk (1.08 ng/mL). PFAS demonstrated higher placental than breastfeeding transfer efficiencies. The transfer efficiencies and the binding affinities of most PFAS to proteins exhibited alkyl chain length-dependent patterns. Furthermore, we comprehensively assessed the estimated daily intakes (EDIs) of PFAS in breastfeeding infants of different age groups and used the hazard quotient (HQ) to characterize the potential health risk. EDIs decreased with infant age, and PFOS had higher HQs than PFOA. These findings highlight the significance of considering PFAS exposure, transfer mechanism, and health risks resulting from breast milk intake in early life.
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