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Too little or too much? Exploring the effectiveness of different policies in air pollution control from technical and non-technical pathways 太少还是太多?从技术和非技术角度探讨不同空气污染控制政策的有效性
IF 8 2区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2024-09-04 DOI: 10.1016/j.jenvman.2024.122375

Most environmental policy studies focus on the technical pathway effect but ignore the non-technical pathway. This paper analyzes the synergistic governance effects of three types of environmental policies on the technical and non-technical pathways. The super-efficient slacks-based measure-data envelopment analysis (SBM-DEA) assesses the green total factor productivity, while the Malmquist index decomposes into pure technical efficiency. The findings indicate that: (1) command-and-control policy has the ‘too-little-of-a-good-thing’ effect, but the policy intensity in most Chinese provinces is strong enough to reduce air pollution, while market-based incentive policy may be ‘too-much-of-a-good-thing’, but Chinese provinces have not reached the inflection point; (2) there are considerable differences in the environmental effects of different policies through technical and non-technical pathways; (3) different policies have various focuses. Command-and-control policy focuses on the non-technical pathway, whereas market-based incentive policy can induce technological progress.

大多数环境政策研究关注技术途径效应,却忽视了非技术途径。本文分析了三种环境政策对技术和非技术途径的协同治理效应。基于松弛的超效率计量-数据包络分析(SBM-DEA)评估了绿色全要素生产率,而马尔奎斯特指数则分解为纯技术效率。研究结果表明(1)指令性控制政策具有 "过少的好东西 "效应,但中国大多数省份的政策力度足以减少空气污染,而基于市场的激励政策可能是 "过多的好东西",但中国各省尚未达到拐点;(2)不同政策通过技术和非技术途径产生的环境效应存在相当大的差异;(3)不同政策具有不同的侧重点。命令与控制政策侧重于非技术途径,而基于市场的激励政策则可促进技术进步。
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引用次数: 0
Carbon and social impacts in the EU's consumption of fossil and mineral raw materials 欧盟化石和矿物原材料消费中的碳和社会影响
IF 8 2区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2024-09-04 DOI: 10.1016/j.jenvman.2024.122291

Fossil and mineral raw materials cause unintended and detrimental environmental and social impacts via extraction, production and combustion processes. In this study, we analyse how consumer demand in the European Union (EU) drives environmental and social impacts in mining sectors worldwide. We employ multi-regional input-output analysis to quantify positive (i.e., income, female and male employment) and negative (greenhouse gas emissions, accidents at work, and modern slavery) impacts of raw materials. We trace these environmental and social impacts across the EU's trading partners to identify sectoral and regional hotspots of international spillovers embodied in the EU's consumer demand. We estimate that the EU's consumption is associated with significant spillover impacts primarily in Central Asia, Asia Pacific, and Africa. We contextualise these results within a three-pillar framework to highlight the importance of a comprehensive and partnership-based approach to curbing environmental and social spillovers embodied in the EU's consumption of raw materials. Specifically, we highlight three potential practical policy strategies: leveraging EU domestic instruments and regulations, strengthening the Green Deal and SDG diplomacy and financing, and promoting responsible consumption, recycling and innovation. Our results underline the need for further reforms in mining industries and trade policies to reduce adverse social and environmental impacts.

化石和矿物原料在开采、生产和燃烧过程中会对环境和社会造成意想不到的有害影响。在本研究中,我们分析了欧盟(EU)的消费需求如何推动全球采矿业对环境和社会的影响。我们采用多地区投入产出分析法来量化原材料的正面(即收入、男女就业)和负面(温室气体排放、工伤事故和现代奴隶制)影响。我们在欧盟贸易伙伴中追踪这些环境和社会影响,以确定欧盟消费需求中体现的国际溢出效应的部门和地区热点。我们估计,欧盟的消费主要对中亚、亚太地区和非洲产生了显著的溢出效应。我们将这些结果置于一个三支柱框架内,以强调采用一种全面的、基于伙伴关系的方法来遏制欧盟原材料消费所体现的环境和社会溢出效应的重要性。具体而言,我们强调了三种潜在的实用政策战略:利用欧盟国内工具和法规,加强绿色交易和可持续发展目标外交和融资,以及促进负责任的消费、回收和创新。我们的研究结果表明,有必要进一步改革采矿业和贸易政策,以减少对社会和环境的不利影响。
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引用次数: 0
Nitrogen removal performance of bioretention cells under freeze-thaw cycles: Effects of filler structure and microbial community 冻融循环下生物滞留池的脱氮性能:填料结构和微生物群落的影响。
IF 8 2区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2024-09-04 DOI: 10.1016/j.jenvman.2024.122380

Cold climates have an adverse effect on the nitrogen-removal capacity of bioretention cells, especially during freeze-thaw cycles (FTCs). To explore the effects of FTCs on the nitrogen removal performance of bioretention cells, this research compared the effects of FTCs on the pore structure and microbial community composition of the filler, and analyzed the nitrogen removal performance of the bioretention cell before (RT), during (FTC) and after (RRT) FTCs. The results demonstrated that RRT filler had a much greater number of pores with equivalent diameter <500 μm than RT filler, and that RRT had a higher pore volume and pore density than RT. Microbial community analysis revealed that the diversity and richness of the microbial community in FTC were lower than in RT, and the relative abundance of Lacunisphaera, Pseudomonas, and Dokdonella decreased significantly. There was no significant difference in microbial community richness between RRT and RT, however RRT diversity was lower. RRT has a higher relative abundance of nitrifying bacteria (Subgroup_10, Bryobacter, etc.) than RT, but a lower relative abundance of denitrifying bacteria (Pseudomonas, Dokdonella, Arenimonas, etc.). The nitrogen removal efficiency of FTC was inhibited, resulting in a decrease of 13.0 ± 4.86%, 19.7 ± 9.17%, and 26.6 ± 1.74% in the removal rates of ammonia nitrogen(NH4+-N), nitrate nitrogen(NO3-N), and total nitrogen(TN) when compared to RT, respectively. RRT improved nitrification and increased NH4+-N removal rate by 10.3 ± 2.69% compared to RT. However, because of denitrification inhibition, the nitrogen removal performance of RRT was not able to reach RT levels, and its NO3-N and TN removal rates decreased by 100 ± 4.70% and 58.3 ± 3.71%, respectively. This study has demonstrated that FTCs can permanently harm the bioretention cell's filler structure and microbial community, resulting in a significant decrease in the nitrogen removal performance of the bioretention cell designed according to warm climate conditions after experiencing FTCs.

寒冷气候对生物滞留池的脱氮能力有不利影响,尤其是在冻融循环(FTC)期间。为了探索冻融循环对生物滞留池脱氮性能的影响,本研究比较了冻融循环对填料孔隙结构和微生物群落组成的影响,并分析了生物滞留池在冻融循环前(RT)、冻融循环中(FTC)和冻融循环后(RRT)的脱氮性能。结果表明,与RT相比,RRT填料具有更多直径相当的孔隙(4+-N)、硝酸盐氮(NO3--N)和总氮(TN)。与 RT 相比,RRT 改善了硝化作用,NH4+-N 去除率提高了 10.3 ± 2.69%。然而,由于反硝化作用受到抑制,RRT 的脱氮性能无法达到 RT 的水平,其 NO3-N 和 TN 的去除率分别下降了 100 ± 4.70% 和 58.3 ± 3.71%。本研究表明,FTC 会对生物滞留池的填料结构和微生物群落造成永久性伤害,导致根据温暖气候条件设计的生物滞留池在经历 FTC 后脱氮性能显著下降。
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引用次数: 0
Balancing growth and sustainability: COP 28 policy implications of green energy, industrialization, foreign direct investment, and globalization in South Asia 平衡增长与可持续性:第二十八届缔约方会议对南亚绿色能源、工业化、外国直接投资和全球化的政策影响
IF 8 2区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2024-09-04 DOI: 10.1016/j.jenvman.2024.122290

This research investigates the intricate relationships between economic variables and how they affect South Asian nation's ability to develop sustainably. Given the growing concerns about climate change and global warming brought on by emissions of greenhouse gases, this study looks into the connection between emissions of CO2, green energy, industrialization, foreign direct investment, economic globalization, and financial development from 1995 to 2022. Second-generation panel techniques were employed in this study to look at the relationship between variables because of the potential of residual cross-sectional dependency and heterogeneity. The empirical outcomes display that green energy, economic globalization, and financial development reduce CO2 emissions by 1.839%, 1.223%, and 3.902% respectively. Industrialization and foreign direct investment degrade the environment by 4.302% and 1.893% respectively. A bidirectional causality link between green energy, industrialization, economic globalization, and CO2 emissions was found by Dumitrescu and Hurlin (D-H). Based on our findings, we recommend legislative support for renewable energy, cleaner technologies, and strict environmental regulations, aligning with the Sustainable Development Goals (SDGs). Encouraging FDI, sustainable practices, and financial development can drive economic growth while preserving the environment. As we approach COP28, this holistic approach to sustainable development becomes increasingly vital for South Asian countries to achieve their SDG targets and combat climate change.

本研究探讨了经济变量之间错综复杂的关系,以及这些变量如何影响南亚国家的可持续发展能力。鉴于人们日益关注温室气体排放带来的气候变化和全球变暖问题,本研究探讨了 1995 年至 2022 年期间二氧化碳排放、绿色能源、工业化、外国直接投资、经济全球化和金融发展之间的联系。由于可能存在残余横截面依赖性和异质性,本研究采用了第二代面板技术来研究变量之间的关系。实证结果显示,绿色能源、经济全球化和金融发展分别减少了 1.839%、1.223% 和 3.902%的二氧化碳排放量。工业化和外国直接投资分别使环境恶化了 4.302% 和 1.893%。Dumitrescu 和 Hurlin(D-H)发现,绿色能源、工业化、经济全球化和二氧化碳排放之间存在双向因果关系。根据我们的研究结果,我们建议立法支持可再生能源、清洁技术和严格的环境法规,并与可持续发展目标(SDGs)保持一致。鼓励外国直接投资、可持续实践和金融发展可以在保护环境的同时推动经济增长。随着 COP28 的临近,这种可持续发展的整体方法对南亚国家实现可持续发展目标和应对气候变化越来越重要。
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引用次数: 0
Intermittent aeration mitigating carbon emission from landfills with gas-water joint regulation 间歇曝气通过气水联合调节减少垃圾填埋场的碳排放
IF 8 2区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2024-09-04 DOI: 10.1016/j.jenvman.2024.122347

Landfill is a significant source of atmospheric CH4 and CO2 emissions. In this study, four landfill reactor systems were constructed to investigate the effects of different ventilation methods, including continuous aeration (20 h d−1) and intermittent aeration (continuous aeration for 4 h d−1 and 2 h of aeration every 12 h, twice a day), on properties of landfilled waste and emissions of CH4 and CO2, in comparison to a traditional landfill. Compared with continuous aeration, intermittent aeration could reduce the potential global warming effect of the CH4 and CO2 emissions, especially multiple intermittent aeration. The CH4 and CO2 emissions could be predicted by the multiple linear regression model based on the contents of carbon, sulfur and/or pH during landfill stabilization. Both intermittent and continuous aeration could enhance the methane oxidation activity of landfilled waste. The aerobic methane oxidation activity of landfilled waste reached the maximums of 50.77–73.78 μg g−1 h−1 after aeration for 5 or 15 d, which was higher than the anaerobic methane oxidation activity (0.45–1.27 μg g−1 h−1). CO2 was the predominant form of organic carbon loss in the bioreactor landfills. Candidatus Methylomirabilis, Methylobacter, Methylomonas and Crenothrix were the main methane-oxidating microorganisms (MOM) in the landfills. Total, NO2-N, pH and Fe3+ were the main environmental variables influencing the MOM community, among which NO2-N and pH had the significant impact on the MOM community. Partial least squares path modelling indicated that aeration modes mainly influenced the emissions of CH4 and CO2 by affecting the degradation of landfilled waste, environmental variables and microbial activities. The results would be helpful for designing aeration systems to reduce the emissions of CH4 and CO2, and the cost during landfill stabilization.

垃圾填埋是大气中甲烷和二氧化碳的重要排放源。本研究构建了四个垃圾填埋反应器系统,以研究与传统垃圾填埋场相比,不同通风方法(包括连续曝气(20 h d-1)和间歇曝气(连续曝气 4 h d-1,每 12 h 曝气 2 h,每天 2 次))对填埋废物的性质以及 CH4 和 CO2 排放的影响。与连续曝气相比,间歇曝气可减少 CH4 和 CO2 排放对全球变暖的潜在影响,尤其是多次间歇曝气。根据垃圾填埋场稳定化过程中碳、硫和/或 pH 的含量,可以通过多元线性回归模型预测 CH4 和 CO2 的排放量。间歇曝气和连续曝气都能提高垃圾填埋场的甲烷氧化活性。曝气 5 或 15 d 后,填埋垃圾的好氧甲烷氧化活性达到 50.77-73.78 μg g-1 h-1 的最大值,高于厌氧甲烷氧化活性(0.45-1.27 μg g-1 h-1)。二氧化碳是生物反应器填埋场中有机碳损失的主要形式。甲烷氧化微生物(MOM)主要有甲基米拉氏菌、甲基细菌、甲基单胞菌和 Crenothrix。影响甲烷氧化微生物群落的主要环境变量是总氮、NO2--N、pH值和Fe3+,其中NO2--N和pH值对甲烷氧化微生物群落的影响最大。偏最小二乘法路径模型表明,曝气模式主要通过影响填埋垃圾的降解、环境变量和微生物活动来影响 CH4 和 CO2 的排放。这些结果将有助于设计曝气系统,以减少 CH4 和 CO2 的排放,并降低垃圾填埋场稳定化过程中的成本。
{"title":"Intermittent aeration mitigating carbon emission from landfills with gas-water joint regulation","authors":"","doi":"10.1016/j.jenvman.2024.122347","DOIUrl":"10.1016/j.jenvman.2024.122347","url":null,"abstract":"<div><p>Landfill is a significant source of atmospheric CH<sub>4</sub> and CO<sub>2</sub> emissions. In this study, four landfill reactor systems were constructed to investigate the effects of different ventilation methods, including continuous aeration (20 h d<sup>−1</sup>) and intermittent aeration (continuous aeration for 4 h d<sup>−1</sup> and 2 h of aeration every 12 h, twice a day), on properties of landfilled waste and emissions of CH<sub>4</sub> and CO<sub>2</sub>, in comparison to a traditional landfill. Compared with continuous aeration, intermittent aeration could reduce the potential global warming effect of the CH<sub>4</sub> and CO<sub>2</sub> emissions, especially multiple intermittent aeration. The CH<sub>4</sub> and CO<sub>2</sub> emissions could be predicted by the multiple linear regression model based on the contents of carbon, sulfur and/or pH during landfill stabilization. Both intermittent and continuous aeration could enhance the methane oxidation activity of landfilled waste. The aerobic methane oxidation activity of landfilled waste reached the maximums of 50.77–73.78 μg g<sup>−1</sup> h<sup>−1</sup> after aeration for 5 or 15 d, which was higher than the anaerobic methane oxidation activity (0.45–1.27 μg g<sup>−1</sup> h<sup>−1</sup>). CO<sub>2</sub> was the predominant form of organic carbon loss in the bioreactor landfills. <em>Candidatus</em> Methylomirabilis, <em>Methylobacter</em>, <em>Methylomonas</em> and <em>Crenothrix</em> were the main methane-oxidating microorganisms (MOM) in the landfills. Total, NO<sub>2</sub><sup>−</sup>-N, pH and Fe<sup>3+</sup> were the main environmental variables influencing the MOM community, among which NO<sub>2</sub><sup>−</sup>-N and pH had the significant impact on the MOM community. Partial least squares path modelling indicated that aeration modes mainly influenced the emissions of CH<sub>4</sub> and CO<sub>2</sub> by affecting the degradation of landfilled waste, environmental variables and microbial activities. The results would be helpful for designing aeration systems to reduce the emissions of CH<sub>4</sub> and CO<sub>2</sub>, and the cost during landfill stabilization.</p></div>","PeriodicalId":356,"journal":{"name":"Journal of Environmental Management","volume":null,"pages":null},"PeriodicalIF":8.0,"publicationDate":"2024-09-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142136995","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Preparation of 97% pure nickel-cobalt alloy from waste Ni-MH batteries by using waste glass as a fluxing agent 利用废玻璃作为助熔剂从废镍氢电池中制备纯度为 97% 的镍钴合金
IF 8 2区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2024-09-04 DOI: 10.1016/j.jenvman.2024.122371

With the e-waste growing rapidly all over the globe due to growing demand of electronics, smartphones, etc., coming up with an efficient and sustainable recycling process is the need of the hour. The present work reports a novel and sustainable process of manufacturing Ni alloy by bringing together three major waste streams such as waste Ni-MH batteries, e-waste plastics, and waste glass. The chosen temperature (1550 °C) favours the reduction of nickel-oxide by e-waste plastic as the reductant and sends rare earth elements present in the waste Ni-MH battery as oxide mixture to the slag phase. Waste glass powder used in this process functions as the fluxing agent, hence not requiring any additional flux. The reduction mechanism is gas-based, controlled mainly by hydrogen and carbon monoxide gases released as a result of decomposition of e-waste plastic as reaction commenced from cold zone (∼300 °C) to hot zone (1550 °C) in the horizontal tubular furnace. Formation of nickel alloy and enrichment of slag with mixture of rare earth oxides were confirmed by XRD, SEM-EDS, and Rietveld refining analysis performed on the XRD spectra of slag phase. ICP-OES (Inductively coupled plasma optical emission spectroscopy) and LIBS (laser induced breakdown spectrometer KT-100S) confirmed the high metal content in the alloy, thereby emphasizing the purity (∼98%) which is close to the composition of nickel super alloy. A maximum of 61% by weight REO enrichment was achieved in the slag phase, having La2O3:44.6%, Pr2O3:14.8%, and Nd2O3: 1.6% under optimised experimental conditions (1550 °C, 15 min, and 20% waste glass powder). This scientific investigation evinces a promising route for efficient utilisation of waste streams emanating from e-waste, thereby devising a sustainable recycling technique and protecting the environment, too.

由于对电子产品、智能手机等的需求日益增长,电子垃圾在全球范围内迅速增长,因此当务之急是开发一种高效、可持续的回收工艺。本研究报告介绍了一种新型、可持续的镍合金制造工艺,它将废镍氢电池、电子废塑料和废玻璃等三大废物流结合在一起。所选温度(1550 °C)有利于电子废塑料作为还原剂还原氧化镍,并将废镍氢电池中的稀土元素作为氧化物混合物送入熔渣相。该工艺中使用的废玻璃粉可作为助熔剂,因此不需要额外的助熔剂。还原机制以气体为基础,主要由电子废塑料分解时释放的氢气和一氧化碳气体控制,反应从水平管式炉的冷区(300 °C)开始到热区(1550 °C)进行。通过 XRD、SEM-EDS 和对渣相 XRD 光谱进行的 Rietveld 精炼分析,确认了镍合金的形成和渣中稀土氧化物混合物的富集。ICP-OES(电感耦合等离子体光发射光谱)和 LIBS(激光诱导击穿光谱仪 KT-100S)证实了合金中的高金属含量,从而强调了合金的纯度(∼98%)接近镍超级合金的成分。在优化的实验条件(1550 °C、15 分钟和 20% 的废玻璃粉)下,渣相中的 REO 富集度最高达到 61%(按重量计),其中 La2O3:44.6%,Pr2O3:14.8%,Nd2O3:1.6%。这项科学研究为有效利用电子废弃物产生的废物流提供了一条可行的途径,从而设计出一种可持续的回收技术,同时也保护了环境。
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引用次数: 0
Machine learning-driven prediction of phosphorus adsorption capacity of biochar: Insights for adsorbent design and process optimization 机器学习驱动的生物炭磷吸附能力预测:对吸附剂设计和工艺优化的启示
IF 8 2区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2024-09-04 DOI: 10.1016/j.jenvman.2024.122405

Phosphorus (P) pollution in aquatic environments poses significant environmental challenges, necessitating the development of effective remediation strategies, and biochar has emerged as a promising adsorbent for P removal at the cost of extensive research resources worldwide. In this study, a machine learning approach was proposed to simulate and predict the performance of biochar in removing P from water. A dataset consisting of 190 types of biochar was compiled from literature, encompassing various variables including biochar characteristics, water quality parameters, and operating conditions. Subsequently, the random forest and CatBoost algorithms were fine-tuned to establish a predictive model for P adsorption capacity. The results demonstrated that the optimized CatBoost model exhibited high prediction accuracy with an R2 value of 0.9573, and biochar dosage, initial P concentration in water, and C content in biochar were identified as the predominant factors. Furthermore, partial dependence analysis was employed to examine the impact of individual variables and interactions between two features, providing valuable insights for adsorbent design and operating condition optimization. This work presented a comprehensive framework for applying a machine learning approach to address environmental issues and provided a valuable tool for advancing the design and implementation of biochar-based water treatment systems.

水生环境中的磷(P)污染对环境构成了重大挑战,因此有必要制定有效的补救策略,而生物炭作为一种很有前景的去除磷的吸附剂,在全球范围内耗费了大量的研究资源。本研究提出了一种机器学习方法来模拟和预测生物炭去除水中 P 的性能。研究人员从文献中收集了 190 种生物炭数据集,其中包括生物炭特性、水质参数和运行条件等各种变量。随后,对随机森林算法和 CatBoost 算法进行了微调,以建立一个 P 吸附能力预测模型。结果表明,优化后的 CatBoost 模型具有较高的预测精度,R2 值为 0.9573,生物炭用量、水中初始 P 浓度和生物炭中 C 含量被确定为主要因素。此外,还采用了部分依存分析来研究单个变量和两个特征之间相互作用的影响,为吸附剂设计和操作条件优化提供了有价值的见解。这项研究提出了一个应用机器学习方法解决环境问题的综合框架,并为推进基于生物炭的水处理系统的设计和实施提供了宝贵的工具。
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引用次数: 0
Perfluorooctanoic acid effect and microbial mechanism to methane production in anaerobic digestion 全氟辛酸对厌氧消化产甲烷的影响和微生物机理
IF 8 2区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2024-09-04 DOI: 10.1016/j.jenvman.2024.122412

Perfluorooctanoic acid (PFOA) as emerging pollutants was largely produced and stable in nature environment. Its fate and effect to the wasted sludge digestion process and corresponding microbial mechanism was rarely reported. This study investigated the different dose of PFOA to the wasted sludge digestion process, where the methane yield and microbial mechanism was illustrated. The PFOA added before digestion were 0–10000 μg/L, no significant variation in daily and accumulated methane production between each group. The 9th day methane yield was significantly higher than other days (p < 0.05). The soluble protein was significantly decreased after 76 days digestion (p < 0.001). The total PFOA in sludge (R2 = 0.8817) and liquid (R2 = 0.9083) phase after digestion was exponentially correlated with PFOA dosed. The PFOA in liquid phase was occupied 54.10 ± 18.38% of the total PFOA in all reactors. The dewatering rate was keep decreasing with the increase of PFOA added (R2 = 0.7748, p < 0.001). The mcrA abundance was significantly correlated with the pH value and organic matter concentration in the reactors. Chloroflexi was the predominant phyla, Aminicenantales, Bellilinea and Candidatus_Cloacimonas were predominant genera in all reactors. Candidatus_Methanofastidiosum and Methanolinea were predominant archaea in all reactors. The function prediction by FAPROTAX and Tax4fun implied that various PFOA dosage resulted in significant function variation. The fermentation and anaerobic chemoheterotrophy function were improved with the PFOA dose. Co-occurrence network implied the potent cooperation among the organic matter degradation and methanogenic microbe in the digestion system. PFOA has little impact to the methane generation while affect the microbe function significantly, its remaining in the digested sludge should be concerned to reduce its potential environmental risks.

全氟辛酸(PFOA)作为一种新出现的污染物,在自然环境中产生量大,且性质稳定。其对废弃污泥消化过程的归宿和影响以及相应的微生物机理却鲜有报道。本研究考察了不同剂量的 PFOA 对废弃污泥消化过程的影响,其中甲烷产量和微生物机理得到了说明。消化前添加的 PFOA 剂量为 0-10000 μg/L,各组间的日产甲烷量和累积产甲烷量无显著差异。第 9 天的甲烷产量明显高于其他天数(p < 0.05)。消化 76 天后,可溶性蛋白质明显减少(p < 0.001)。消化后污泥(R2 = 0.8817)和液相(R2 = 0.9083)中的全氟辛烷磺酸总量与全氟辛烷磺酸剂量呈指数相关。在所有反应器中,液相中的 PFOA 占 PFOA 总量的 54.10 ± 18.38%。随着 PFOA 添加量的增加,脱水率不断下降(R2 = 0.7748,p < 0.001)。mcrA 丰度与反应器中的 pH 值和有机物浓度显著相关。在所有反应器中,Chloroflexi 是主要的门,Aminicenantales、Bellilinea 和 Candidatus_Cloacimonas 是主要的属。所有反应器中最主要的古细菌是甲烷酵母菌(Candidatus_Methanofastidiosum)和甲醇酵母菌(Methanolinea)。FAPROTAX 和 Tax4fun 的功能预测表明,不同的全氟辛烷磺酸用量会导致功能的显著变化。发酵和厌氧化学营养功能随着全氟辛酸剂量的增加而提高。共生网络表明,消化系统中的有机物降解和产甲烷微生物之间存在着强有力的合作。PFOA对甲烷生成的影响较小,而对微生物功能的影响较大,应关注其在消化污泥中的残留,以降低其潜在的环境风险。
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引用次数: 0
The impact of green roofs’ composition on its overall life cycle 绿色屋顶的构成对其整体生命周期的影响。
IF 8 2区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2024-09-03 DOI: 10.1016/j.jenvman.2024.122363

Green roof systems have been developed to improve the environmental, economic, and social aspects of sustainability. Selecting the appropriate version of the green roof composition plays an important role in the life cycle assessment of a green roof. In this study, 10 compositions of an intensive green roof for moderate zone and 4 green roof compositions for different climatic conditions were designed and comprehensively assessed in terms of their environmental and economic impacts within the “Cradle-to-Cradle” system boundary. The assessment was carried out over a 50-year period for a moderate climate zone. The results showed that asphalt strips and concrete slab produced the highest total emissions. It was found that most greenhouse gases emissions were released in the operational energy consumption phase and in the production phase. The energy consumption phase (48.78%) for automatic irrigation and maintenance caused the highest Global Warming Potential (GWP) value (758.39 kg CO2e) in the worst variant, which also caused the highest life cycle cost (878.47€). On the contrary, in the best variant, planting more vegetation and lower maintenance and irrigation requirements led to a reduction in GWP (445.0 kg CO2e), but in terms of cost (506.6€) this composition didn't represent the best variant. The Global Warming Potential Biogenic (GWP-bio) compared to the Global Warming Potential Total (GWP-total) represents a proportion ranging from 0.8% to 78% depending on the proposed vegetation. Overall higher biogenic carbon values (up to 1525 kg CO2e) were observed for the proposed tall vegetation of Magnolia, Red Mulberry, Hawthorne, Cherry, and Crab-apple Tree. Based on the results of the multicriteria analysis, which included core environmental & economic parameters, biogenic carbon emission levels, the outcome of this paper proposed optimal green roof composition. Optimal intensive green roof composition was subjected to a sensitivity analysis to determine the impact of changing climatic conditions on CO2 emissions and life cycle costs. The results of the sensitivity analysis show that the optimal variant of the green roof can be implemented in the cold and subtropical zone with regard to CO2 emissions, but not with regard to life cycle costs.

开发绿色屋顶系统是为了改善环境、经济和社会方面的可持续性。在屋顶绿化的生命周期评估中,选择合适的屋顶绿化组合方式起着重要作用。在这项研究中,我们设计了 10 种适中地带的密集型绿色屋顶组合和 4 种不同气候条件下的绿色屋顶组合,并在 "从摇篮到摇篮 "系统边界内对其环境和经济影响进行了全面评估。评估在中等气候区进行,为期 50 年。结果表明,沥青带和混凝土板的总排放量最高。结果发现,大部分温室气体排放是在运行能耗阶段和生产阶段释放的。在最差的方案中,用于自动灌溉和维护的能耗阶段(48.78%)造成了最高的全球变暖潜势值(758.39 千克二氧化碳当量),也造成了最高的生命周期成本(878.47 欧元)。相反,在最佳方案中,种植更多植被,降低维护和灌溉要求,导致全球升温潜能值降低(445.0 千克 CO2e),但就成本而言(506.6 欧元),这一构成并不代表最佳方案。全球升温潜能值生物值(GWP-bio)与全球升温潜能值总值(GWP-total)相比,所占比例从 0.8%到 78%不等,取决于所建议的植被。从总体上看,木兰、红桑、山楂、樱桃和柰树等拟建高大植被的生物碳值较高(高达 1525 千克 CO2e)。基于多标准分析(包括核心环境和经济参数、生物碳排放水平)的结果,本文提出了最佳屋顶绿化组合。对最佳密集型绿色屋顶构成进行了敏感性分析,以确定气候条件变化对二氧化碳排放量和生命周期成本的影响。敏感性分析的结果表明,在寒冷和亚热带地区,可以实施二氧化碳排放方面的最佳绿色屋顶变体,但生命周期成本方面则不行。
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引用次数: 0
Comparative assessment of microbiome and resistome of influent and effluent of sewage treatment plant and common effluent treatment plant located in Delhi, India using shotgun approach 使用霰弹枪方法比较评估印度德里污水处理厂和普通污水处理厂进水和出水的微生物组和抗微生物组。
IF 8 2区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2024-09-03 DOI: 10.1016/j.jenvman.2024.122342

Antimicrobial resistance (AMR) is a significant threat that demands surveillance to identify and analyze trends of the emerging antibiotic resistance genes (ARGs) and potential microbial carriers. The influent of the wastewater treatment plants (WWTPs) reflects the microbes derived from the population and effluent being the source of dissemination of potential pathogenic microbes and AMR. The present study aimed to monitor microbial communities and antibiotic resistance genes in WWTPs employing a whole metagenome shotgun sequencing approach. The samples were collected from a sewage treatment plant (STP) and a common effluent treatment plant (CETP) in Delhi, India. The results showed the influent of STP to be rich in Bifidobacterium, Bacteroides, Escherichia, Arcobacter, and Pseudomonas residents of gut microbiota and known to cause diseases in humans and animals; whereas the CETP sample was abundant in Aeromonas, Escherichia, and Shewanella known to be involved in the degradation of different compounds. Interestingly, the effluent samples from both STPs and CETP were rich in microbial diversity, comprising organic and xenobiotic compound degrading and disease-causing bacteria, indicating the effluent being the source of dissemination of concerning bacteria to the environment. The functional profile at both sites displayed similarity with an abundance of housekeeping function genes as analyzed by Clusters of Orthologous Genes (COG), KEGG Orthology (KO), and subsystem databases. Resistome profiling by MEGARes showed the dominance of ARGs corresponding to beta-lactams having relative abundance ranging from 16% to 34% in all the metagenome datasets, followed by tetracycline (8%–16%), aminoglycosides (7%–9%), multi-drug (5%–9%), and rifampin (3%–9%). Also, AMR genes oxa, ant3-DPRIME, and rpoB, which are of clinical importance were predominantly and most prevalently present in all the samples. The presence of AMR in effluents from both types of treatment plants indicates that wastewater from both sources contributes to the spread of pathogenic bacteria and resistance genes, increasing the environmental AMR burden and therefore requires tertiary treatment before discharge. This work will facilitate further research towards the identification of suitable biomarkers for monitoring antibiotic resistance.

抗生素耐药性(AMR)是一个重大威胁,需要对其进行监控,以识别和分析新出现的抗生素耐药基因(ARGs)和潜在微生物载体的趋势。污水处理厂(WWTP)的进水反映了来自人口的微生物,而出水则是潜在病原微生物和 AMR 的传播源。本研究采用全元基因组枪式测序方法,旨在监测污水处理厂中的微生物群落和抗生素耐药性基因。样本采集自印度德里的一家污水处理厂(STP)和一家普通污水处理厂(CETP)。结果表明,污水处理厂的进水富含肠道微生物群中的双歧杆菌、乳杆菌、埃希氏菌、弓形杆菌和假单胞菌,已知它们会导致人类和动物疾病;而 CETP 样品中则富含气单胞菌、埃希氏菌和雪旺菌,已知它们会参与不同化合物的降解。有趣的是,污水处理厂和 CETP 的污水样本中微生物种类丰富,包括有机和异生物化合物降解菌和致病菌,表明污水是相关细菌向环境传播的源头。通过同源基因簇 (COG)、KEGG 正选 (KO) 和子系统数据库分析,这两个地点的功能特征与大量的管家功能基因相似。通过 MEGARes 进行的耐药性基因组分析表明,在所有元基因组数据集中,与β-内酰胺类药物相对应的 ARGs 占主导地位,其相对丰度从 16% 到 34% 不等,其次是四环素(8%-16%)、氨基糖苷类(7%-9%)、多种药物(5%-9%)和利福平(3%-9%)。此外,在所有样本中,具有重要临床意义的 AMR 基因 oxa、ant3-DPRIME 和 rpoB 也是主要和最常见的。两类污水处理厂的废水中都存在 AMR,这表明这两种来源的废水都助长了病原菌和耐药基因的传播,增加了环境中的 AMR 负担,因此需要在排放前进行三级处理。这项工作将促进进一步研究,以确定监测抗生素耐药性的合适生物标志物。
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引用次数: 0
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Journal of Environmental Management
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